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873
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3.37k
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581
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1
433
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634 values
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large_stringlengths
1
683
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large_stringlengths
1
245
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large_stringclasses
11 values
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346 values
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64
64
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64
64
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5
288
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large_stringlengths
24
2.64k
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float64
-0.8
90,205,160,000B
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large_stringlengths
2
864
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float64
-230
30.1k
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3 values
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float64
0
4k
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4 values
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1
23.6k
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96 values
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large_stringlengths
3
716
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large_stringlengths
3
539
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large_stringlengths
5
293
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large_stringlengths
5
271
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large_stringlengths
5
271
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large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
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float64
-230
30.1k
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float64
0
2.16k
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large_stringlengths
4
882
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a20466eb704b4286a24630c1e60bd7a4
NCCCC[C@@H](C(=O)O)N(C(=O)OCC1c2ccccc2-c2ccccc21)C(=O)OCC1c2ccccc2-c2ccccc21>>NCCCC[C@@H](C(=O)F)N(C(=O)OCC1c2ccccc2-c2ccccc21)C(=O)OCC1c2ccccc2-c2ccccc21
N1=CC=CC=C1.N1=C(F)N=C(F)N=C1F.C(=O)(OCC1C2=CC=CC=C2C2=CC=CC=C12)N([C@@H](CCCCN)C(=O)O)C(=O)OCC1C2=CC=CC=C2C2=CC=CC=C12>>C(=O)(OCC1C2=CC=CC=C2C2=CC=CC=C12)N([C@@H](CCCCN)C(=O)F)C(=O)OCC1C2=CC=CC=C2C2=CC=CC=C12
O[C:7]([C@H:6]([CH2:5][CH2:4][CH2:3][CH2:2][NH2:1])[N:10]([C:11](=[O:12])[O:13][CH2:14][CH:15]1[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2-[c:22]2[cH:23][cH:24][cH:25][cH:26][c:27]21)[C:28](=[O:29])[O:30][CH2:31][CH:32]1[c:33]2[cH:34][cH:35][cH:36][cH:37][c:38]2-[c:39]2[cH:40][cH:41][cH:42][cH:43][c:44]21)=[O:8]>>[NH2:1...
NCCCC[C@@H](C(=O)O)N(C(=O)OCC1c2ccccc2-c2ccccc21)C(=O)OCC1c2ccccc2-c2ccccc21
NCCCC[C@@H](C(=O)F)N(C(=O)OCC1c2ccccc2-c2ccccc21)C(=O)OCC1c2ccccc2-c2ccccc21
null
null
ClCCl
Functional Group Interconversion
OtherReaction
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
O=C(NC(=O)OCC1c2ccccc2-c2ccccc21)OCC1c2ccccc2-c2ccccc21
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5](-[C:6]=[O;D1;H0:7])-[C:8]=[O;D1;H0:9]>>[C:4]-[C:3](-[#7:5](-[C:6]=[O;D1;H0:7])-[C:8]=[O;D1;H0:9])-[C;H0;D3;+0:1](-[F;D1;H0:10])=[O;D1;H0:2]
null
[]
null
null
8
HOUR
Bis-FMOC-L-Lysine (5 g, 8.46 mmol) (Bachem) was dissolved in dichloromethane (50 mL). Pyridine (0.69 mL, 8.46 mmol) (Aldrich) and cyanuric fluoride (1.14 g, 8.46 mmol) (Aldrich) were successively added at room temperature and the mixture was stirred overnight. Ice cold water (100 mL) was added and the resulting slurry ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1ccc2c(c1)Cc1ccccc12.c1ccc2c(c1)Cc1ccccc12
null
ClCCl
null
8
NCCCC[C@@H](C(=O)O)N(C(=O)OCC1c2ccccc2-c2ccccc21)C(=O)OCC1c2ccccc2-c2ccccc21>ClCCl>NCCCC[C@@H](C(=O)F)N(C(=O)OCC1c2ccccc2-c2ccccc21)C(=O)OCC1c2ccccc2-c2ccccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0c4289f38f9b4359b0462549c3b30f31
O=C(N[C@@H](Cc1c[nH]c2ccccc12)C(=O)O)OCC1c2ccccc2-c2ccccc21>>O=C(N[C@@H](Cc1c[nH]c2ccccc12)C(=O)F)OCC1c2ccccc2-c2ccccc21
N1=CC=CC=C1.N1=C(F)N=C(F)N=C1F.C(=O)(OCC1C2=CC=CC=C2C2=CC=CC=C12)N[C@@H](CC1=CNC2=CC=CC=C12)C(=O)O>>C(=O)(OCC1C2=CC=CC=C2C2=CC=CC=C12)N[C@@H](CC1=CNC2=CC=CC=C12)C(=O)F
O[C:15]([C@@H:4]([NH:3][C:2](=[O:1])[O:18][CH2:19][CH:20]1[c:21]2[cH:22][cH:23][cH:24][cH:25][c:26]2-[c:27]2[cH:28][cH:29][cH:30][cH:31][c:32]21)[CH2:5][c:6]1[cH:7][nH:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]12)=[O:16]>>[O:1]=[C:2]([NH:3][C@@H:4]([CH2:5][c:6]1[cH:7][nH:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]12)[C:...
O=C(N[C@@H](Cc1c[nH]c2ccccc12)C(=O)O)OCC1c2ccccc2-c2ccccc21
O=C(N[C@@H](Cc1c[nH]c2ccccc12)C(=O)F)OCC1c2ccccc2-c2ccccc21
null
null
ClCCl
Functional Group Interconversion
OtherReaction
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
O=C(NCCc1c[nH]c2ccccc12)OCC1c2ccccc2-c2ccccc21
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7]>>[C:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](-[F;D1;H0:8])=[O;D1;H0:2]
null
[]
null
null
6.5
HOUR
FMOC-L-Tryptophan (5 g, 11.72 mmol) (Bachem) was dissolved in dichloromethane (60 mL). Pyridine (0.95 mL, 11.72 mmol) (Aldrich) and cyanuric fluoride (1.58 g, 11.72 mmol) (Aldrich) were successively added at room temperature and the mixture was stirred for 6.5 hours. Ice cold water (100 mL) was added and the resulting ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1ccc2[nH]ccc2c1.c1ccc2c(c1)Cc1ccccc12
null
ClCCl
null
6.5
O=C(N[C@@H](Cc1c[nH]c2ccccc12)C(=O)O)OCC1c2ccccc2-c2ccccc21>ClCCl>O=C(N[C@@H](Cc1c[nH]c2ccccc12)C(=O)F)OCC1c2ccccc2-c2ccccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7e467cb3ee834f5c8c6a348a4e446e43
CC(C)(C)OC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O>>CC(C)(C)OC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)F
N1=CC=CC=C1.N1=C(F)N=C(F)N=C1F.C(=O)(OCC1C2=CC=CC=C2C2=CC=CC=C12)N[C@@H](COC(C)(C)C)C(=O)O>>C(=O)(OCC1C2=CC=CC=C2C2=CC=CC=C12)N[C@@H](COC(C)(C)C)C(=O)F
O[C:26]([C@H:7]([CH2:6][O:5][C:2]([CH3:1])([CH3:3])[CH3:4])[NH:8][C:9](=[O:10])[O:11][CH2:12][CH:13]1[c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]2-[c:20]2[cH:21][cH:22][cH:23][cH:24][c:25]21)=[O:27]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][CH2:6][C@H:7]([NH:8][C:9](=[O:10])[O:11][CH2:12][CH:13]1[c:14]2[cH:15][cH:16][cH:17][cH...
CC(C)(C)OC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O
CC(C)(C)OC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)F
null
null
ClCCl
Functional Group Interconversion
OtherReaction
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1ccc2c(c1)Cc1ccccc1-2
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7]>>[C:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](-[F;D1;H0:8])=[O;D1;H0:2]
null
[]
null
null
8
HOUR
N-FMOC-O-t-Butyl-L-serine (10 g, 26.07 mmol) (Bachem) was dissolved in dichloromethane (135 mL). Pyridine (2.11 mL, 26.07 mmol) (Aldrich) and cyanuric fluoride (3.52 g, 26.07 mmol) (Aldrich) were successively added at room temperature and the mixture was stirred overnight. Ice cold water (100 mL) was added and the resu...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1ccc2c(c1)Cc1ccccc12
null
ClCCl
null
8
CC(C)(C)OC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O>ClCCl>CC(C)(C)OC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ff701405dbdb4c8d96cc24948af218ae
CSCC[C@@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O>>CSCC[C@@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)F
N1=CC=CC=C1.N1=C(F)N=C(F)N=C1F.C(=O)(OCC1C2=CC=CC=C2C2=CC=CC=C12)N[C@H](CCSC)C(=O)O>>C(=O)(OCC1C2=CC=CC=C2C2=CC=CC=C12)N[C@H](CCSC)C(=O)F
O[C:24]([C@@H:5]([CH2:4][CH2:3][S:2][CH3:1])[NH:6][C:7](=[O:8])[O:9][CH2:10][CH:11]1[c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2-[c:18]2[cH:19][cH:20][cH:21][cH:22][c:23]21)=[O:25]>>[CH3:1][S:2][CH2:3][CH2:4][C@@H:5]([NH:6][C:7](=[O:8])[O:9][CH2:10][CH:11]1[c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2-[c:18]2[cH:19][cH:20][...
CSCC[C@@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O
CSCC[C@@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)F
null
null
ClCCl
Functional Group Interconversion
OtherReaction
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1ccc2c(c1)Cc1ccccc1-2
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7]>>[C:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](-[F;D1;H0:8])=[O;D1;H0:2]
null
[]
null
null
4
HOUR
FMOC-D-Methionine (5.00 g, 13.46 mmol) (Bachem) was dissolved in dichloromethane (70 mL). Pyridine (1.09 mL, 13.46 mmol) (Aldrich) and cyanuric fluoride (1.82 g, 13.46 mmol) (Aldrich) were successively added at room temperature and the mixture was stirred for 4 hours. Ice cold water (100 mL) was added and the resulting...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1ccc2c(c1)Cc1ccccc12
null
ClCCl
null
4
CSCC[C@@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O>ClCCl>CSCC[C@@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-fdb8a9152bfd4faca050f70d5c0c0d5b
CC(C)(C)[Si](C)(C)Cl.O=[N+]([O-])c1ccc(O)cc1>>CC(C)(C)[Si](C)(C)Oc1ccc([N+](=O)[O-])cc1
[Si](C)(C)(C(C)(C)C)Cl.[N+](=O)([O-])C1=CC=C(C=C1)O.N1C=NC=C1.[Si](C)(C)(C(C)(C)C)Cl>>[N+](=O)([O-])C1=CC=C(C=C1)O[Si](C(C)(C)C)(C)C
Cl[Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7].[OH:8][c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[cH:16][cH:17]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[cH:16][cH:17]1
CC(C)(C)[Si](C)(C)Cl.O=[N+]([O-])c1ccc(O)cc1
CC(C)(C)[Si](C)(C)Oc1ccc([N+](=O)[O-])cc1
null
null
CN(C=O)C
Protection
Alcohol protection with silyl ethers
91043baed1393f1ecd2302d7d0b31c01cf171d3977dd7c70afa1da52fa298c73
4a917c959d011f885a1269fa3c1f022ee5e09144996246d24e42e65634a451ac
c1ccccc1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[OH;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[C;D1;H3:5]-[C:4](-[C;D1;H3:6])(-[C;D1;H3:7])-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[O;H0;D2;+0:8]-[c:9](:[c:10]):[c:11]
null
[]
null
null
1
DAY
To a solution of 4-nitrophenol (5.0 g, 35.9 mmol) (Aldrich) in dimethylformamide (50 mL) was added imidazole (3.18 g, 46.7 mmol) (Aldrich) and t-butyldimethylsilyl chloride (6.49 g, 43.1 mmol) (Avocado Research Chemicals Ltd.). The reaction mixture was stirred at room temperature for 1 day. TLC analysis showed starting...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol.Silyl protective group
TMS ether protective group
null
null
c1ccccc1
HCl
CN(C=O)C
null
24
CC(C)(C)[Si](C)(C)Cl.O=[N+]([O-])c1ccc(O)cc1>CN(C=O)C>CC(C)(C)[Si](C)(C)Oc1ccc([N+](=O)[O-])cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a803ccb62a404612ad797f6d240d47bb
CC(C)(C)[Si](C)(C)Oc1ccc([N+](=O)[O-])cc1>>CC(C)(C)[Si](C)(C)Oc1ccc(N)cc1
[N+](=O)([O-])C1=CC=C(C=C1)O[Si](C(C)(C)C)(C)C>>C[Si](C(C)(C)C)(OC1=CC=C(C=C1)N)C
O=[N+:13]([O-])[c:12]1[cH:11][cH:10][c:9]([O:8][Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7])[cH:15][cH:14]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][c:9]1[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]1
CC(C)(C)[Si](C)(C)Oc1ccc([N+](=O)[O-])cc1
CC(C)(C)[Si](C)(C)Oc1ccc(N)cc1
null
[Pd]
C(C)(=O)OCC
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
A solution of 1-nitro4-(1,1,2,2-tetramethyl-1-silapropoxy)benzene (7.8 g, 30.8 mmol) (from Example 19a supra) and 10% Pd/C (0.70 g) (Aldrich) in ethyl acetate (100 mL) was hydrogenated for 1 day. The reaction mixture was filtered though Celite® and concentrated. The residue was purified by flash chromatography eluting ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
[Pd].C(C)(=O)OCC
null
null
CC(C)(C)[Si](C)(C)Oc1ccc([N+](=O)[O-])cc1>[Pd].C(C)(=O)OCC>CC(C)(C)[Si](C)(C)Oc1ccc(N)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-08b42f333f054ad0a9ab1a2e5240f66b
COC(=O)OC.COc1c(F)cc(C(C)=O)cc1F>>COC(=O)CC(=O)c1cc(F)c(OC)c(F)c1
CC(=O)C1=CC(=C(C(=C1)F)OC)F.C(OC)(OC)=O>>FC=1C=C(C(=O)CC(=O)OC)C=C(C1OC)F
CO[C:3]([O:2][CH3:1])=[O:4].[CH3:5][C:6](=[O:7])[c:8]1[cH:9][c:10]([F:11])[c:12]([O:13][CH3:14])[c:15]([F:16])[cH:17]1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][C:6](=[O:7])[c:8]1[cH:9][c:10]([F:11])[c:12]([O:13][CH3:14])[c:15]([F:16])[cH:17]1
COC(=O)OC.COc1c(F)cc(C(C)=O)cc1F
COC(=O)CC(=O)c1cc(F)c(OC)c(F)c1
null
null
null
C-C Coupling
OtherReaction
984c35cff4b3f334715b1696c3f8f2fb17ccd67fc374fcef5afdd55b5aabecf9
d76b6fc9d01d8258e5777a3b2326a8d78a9d9a55717b27736ba55600205f4ed0
c1ccccc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].[CH3;D1;+0:5]-[C:6](=[O;D1;H0:7])-[c:8]>>[C;D1;H3:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH2;D2;+0:5]-[C:6](=[O;D1;H0:7])-[c:8]
97
[{"value": 97.0, "product": "FC=1C=C(C(=O)CC(=O)OC)C=C(C1OC)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 3,5-difluoro-4-methoxyacetophenone and dimethyl carbonate according to method A. Yellow solid; Yield: 97%; mp 64–67° C.; 1H-NMR (300 MHz, CDCl3) δ 3.77 (s, 3H), 3.93 (s, 2H), 4.13 (t, J=1.7 Hz, 3H), 7.52 (m, 2H). Minor tautomer: 3.81 (s, 3H), 4.06 (m, 3H), 5.58 (s, 1H), 7.34 (m, 2H), 12....
10.6084/m9.figshare.5104873.v1
null
Carbonic Ester.Ketone
Ketone.Ester
null
null
c1ccccc1
HO-
null
null
null
COC(=O)OC.COc1c(F)cc(C(C)=O)cc1F>>COC(=O)CC(=O)c1cc(F)c(OC)c(F)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bebeddd30f25409fb8a19ebf0a18be6c
COc1ccc(-c2cc(C#N)c3cc(OC)ccc3n2)cc1>>N#Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
C(#N)C1=CC(=NC2=CC=C(C=C12)OC)C1=CC=C(C=C1)OC.N1[C@@H](CCC1=O)C(=O)O.Br>>C(#N)C1=CC(=NC2=CC=C(C=C12)O)C1=CC=C(C=C1)O
C[O:10][c:9]1[cH:8][cH:7][c:6](-[c:5]2[cH:4][c:3]([C:2]#[N:1])[c:20]3[c:14]([n:13]2)[cH:15][cH:16][c:17]([O:18]C)[cH:19]3)[cH:12][cH:11]1>>[N:1]#[C:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([OH:10])[cH:11][cH:12]2)[n:13][c:14]2[cH:15][cH:16][c:17]([OH:18])[cH:19][c:20]12
COc1ccc(-c2cc(C#N)c3cc(OC)ccc3n2)cc1
N#Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
null
null
null
Deprotection
OtherReaction
a0f05885bbc65ae2846cad0ac34029941211b2ef3a426958b0c8aa83bb16fe86
9df751cd682ad9d54ed75d7313aaead6a019c5d37ede15c4672866d319b900ff
c1ccc(-c2ccc3ccccc3n2)cc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4].C-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4].[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]
89
[{"value": 89.0, "product": "C(#N)C1=CC(=NC2=CC=C(C=C12)O)C1=CC=C(C=C1)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 9a using Pyr./HBr according to method I. Yellow solid; Yield: 89%; mp>240° C. (dec.); 1H-NMR (300 MHz, DMSO-d6) δ 6.92 (d, J=8.7 Hz, 2H), 7.30 (d, J=2.6 Hz, 1H), 7.45 (dd, J=9.1, 2.6 Hz, 1H), 8.02 (d, J=9.1 Hz, 1H), 8.13 (d, J=8.7 Hz, 2H), 8.58 (s, 1H), 9.93 (s, 1H), 10.64 (s, 1H); MS (E...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Aromatic alcohol.Aromatic alcohol
null
null
c1ccccc1.c1ccc2ncccc2c1
Other
null
null
null
COc1ccc(-c2cc(C#N)c3cc(OC)ccc3n2)cc1>>N#Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-61a03d10d06c4d8fafd1f62dfc401067
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.Oc1ccc(-c2cc(Br)c3cc(O)ccc3n2)cc1>>C=Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC=C(C=C1)O.C(CCC)[Sn](C=C)(CCCC)CCCC>>OC1=CC=C(C=C1)C1=NC2=CC=C(C=C2C(=C1)C=C)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[CH:2]=[CH2:1].Br[c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([OH:10])[cH:11][cH:12]2)[n:13][c:14]2[cH:15][cH:16][c:17]([OH:18])[cH:19][c:20]12>>[CH2:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([OH:10])[cH:11][cH:12]2)[n:13][c:14]2[cH:15][cH:16][c:17]([OH:18])[cH:19][c:20]12
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.Oc1ccc(-c2cc(Br)c3cc(O)ccc3n2)cc1
C=Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
null
null
null
C-C Coupling
Stille reaction_vinyl
b76d02284eab1606d02e43e8d6b217f827d8bc76b0b2203ccf942abed5fcc5b2
ec03c739f58696d2a3659a73884744e1a490a20a587da6f115be382b663cf23d
c1ccc(-c2ccc3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[CH;D2;+0:10]=[C;D1;H2:11]>>[C;D1;H2:11]=[CH;D2;+0:10]-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
69
[{"value": 69.0, "product": "OC1=CC=C(C=C1)C1=NC2=CC=C(C=C2C(=C1)C=C)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6a and tributyl(vinyl)tin according to method J. Yellow solid; Yield: 69%; mp>200° C. (dec.); 1H-NMR (400 MHz, DMSO-d6) δ 5.69 (d, J=11.7 Hz, 1H), 6.23 (dd, J=18.3, 1.0 Hz, 1H), 6.90 (d, J=8.5 Hz, 2H), 7.31 (dd, J=9.0, 2.7 Hz, 1H), 7.35 (d, J=2.2 Hz, 1H), 7.40 (dd, J=17.3, 11.0 Hz, 1H), ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl.Tin
Vinyl
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
HBr.Sn
null
null
null
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.Oc1ccc(-c2cc(Br)c3cc(O)ccc3n2)cc1>>C=Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-4c803b350ae34937859e5cb419f1475d
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc(-c2cc(Br)c3cc(O)ccc3n2)cc1>>C[Si](C)(C)C#Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC=C(C=C1)O.C[Si](C)(C)C#C[Sn](CCCC)(CCCC)CCCC>>OC1=CC=C(C=C1)C1=NC2=CC=C(C=C2C(=C1)C#C[Si](C)(C)C)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[C:6]#[C:5][Si:2]([CH3:1])([CH3:3])[CH3:4].Br[c:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][c:13]([OH:14])[cH:15][cH:16]2)[n:17][c:18]2[cH:19][cH:20][c:21]([OH:22])[cH:23][c:24]12>>[CH3:1][Si:2]([CH3:3])([CH3:4])[C:5]#[C:6][c:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][c:13]([OH:14])[cH:15][cH:16]2)...
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc(-c2cc(Br)c3cc(O)ccc3n2)cc1
C[Si](C)(C)C#Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
null
null
null
C-C Coupling
Stille reaction_other
5b7d122d5cbf3feee31209339c4cd554facd746c4b7c95e3041c641d09f4e525
84197a108c0019520f13001872ce55981c95862f930591903269e152b52aac86
c1ccc(-c2ccc3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].C-C-C-[CH2]-[Sn](-[C;H0;D2;+0:10]#[C:11]-[#14:12](-[C;D1;H3:13])(-[C;D1;H3:14])-[C;D1;H3:15])(-[CH2]-C-C-C)-[CH2]-C-C-C>>[C;D1;H3:13]-[#14:12](-[C;D1;H3:14])(-[C;D1;H3:15])-[C:11]#[C;H0;D2;+0:10]-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:...
83
[{"value": 83.0, "product": "OC1=CC=C(C=C1)C1=NC2=CC=C(C=C2C(=C1)C#C[Si](C)(C)C)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6a and (trimethylsilylethynyl)tributyltin according to method J. Yellow powder; Yield: 83%; mp 210° C. (dec.); 1H-NMR (300 MHz, acetone-d6) δ 0.38 (s, 9H), 7.02 (d, J=8.7 Hz, 2H), 7.44 (dd, J=9.1, 2.7 Hz, 1H), 7.63 (d, J=2.7 Hz, 1H), 7.99 (d, J=9.1 Hz, 1H), 8.05 (s, 1H), 8.18 (d, J=8.7 H...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne.Tin
Alkyne
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
HBr.Sn
null
null
null
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc(-c2cc(Br)c3cc(O)ccc3n2)cc1>>C[Si](C)(C)C#Cc1cc(-c2ccc(O)cc2)nc2ccc(O)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9fbcc659dc29475ebabf18f9a67dbd15
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>C[Si](C)(C)C#Cc1cc(-c2ccc(O)c(F)c2)nc2ccc(O)cc12
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.C[Si](C)(C)C#C[Sn](CCCC)(CCCC)CCCC>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C#C[Si](C)(C)C)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[C:6]#[C:5][Si:2]([CH3:1])([CH3:3])[CH3:4].Br[c:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][c:13]([OH:14])[c:15]([F:16])[cH:17]2)[n:18][c:19]2[cH:20][cH:21][c:22]([OH:23])[cH:24][c:25]12>>[CH3:1][Si:2]([CH3:3])([CH3:4])[C:5]#[C:6][c:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][c:13]([OH:14])[c:15]([F...
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
C[Si](C)(C)C#Cc1cc(-c2ccc(O)c(F)c2)nc2ccc(O)cc12
null
null
null
C-C Coupling
Stille reaction_other
5b7d122d5cbf3feee31209339c4cd554facd746c4b7c95e3041c641d09f4e525
84197a108c0019520f13001872ce55981c95862f930591903269e152b52aac86
c1ccc(-c2ccc3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].C-C-C-[CH2]-[Sn](-[C;H0;D2;+0:10]#[C:11]-[#14:12](-[C;D1;H3:13])(-[C;D1;H3:14])-[C;D1;H3:15])(-[CH2]-C-C-C)-[CH2]-C-C-C>>[C;D1;H3:13]-[#14:12](-[C;D1;H3:14])(-[C;D1;H3:15])-[C:11]#[C;H0;D2;+0:10]-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:...
94
[{"value": 94.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C#C[Si](C)(C)C)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b and (trimethylsilylethynyl)tributyltin according to method J. Red powder; Yield: 94%; 1H-NMR (300 MHz, acetone-d6) δ 0.43 (s, 9H), 7.21 (dd, J=8.8, 8.8 Hz, 1H), 7.51 (dd, J=9.1, 2.7 Hz, 1H), 7.68 (d, J=2.7 Hz, 1H), 8.05 (m, 1H), 8.07 (d, J=9.0 Hz, 1H), 8.13 (s, 1H), 8.18 (dd, J=12.8, ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne.Tin
Alkyne
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
HBr.Sn
null
null
null
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>C[Si](C)(C)C#Cc1cc(-c2ccc(O)c(F)c2)nc2ccc(O)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-03fd43b53d484816aceded56c9677dc8
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3cc(F)c(O)c(F)c3)cc(Br)c2c1>>C#Cc1cc(-c2cc(F)c(O)c(F)c2)nc2ccc(O)cc12
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C(=C1)F)O)F.C[Si](C)(C)C#C[Sn](CCCC)(CCCC)CCCC>>FC=1C=C(C=C(C1O)F)C1=NC2=CC=C(C=C2C(=C1)C#C)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[C:2]#[C:1][Si](C)(C)C.Br[c:3]1[cH:4][c:5](-[c:6]2[cH:7][c:8]([F:9])[c:10]([OH:11])[c:12]([F:13])[cH:14]2)[n:15][c:16]2[cH:17][cH:18][c:19]([OH:20])[cH:21][c:22]12>>[CH:1]#[C:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][c:8]([F:9])[c:10]([OH:11])[c:12]([F:13])[cH:14]2)[n:15][c:16]2[cH:17][cH:18][c:...
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3cc(F)c(O)c(F)c3)cc(Br)c2c1
C#Cc1cc(-c2cc(F)c(O)c(F)c2)nc2ccc(O)cc12
null
null
null
C-C Coupling
OtherReaction
519663089044573005838583055d682ebb55d07ad1272ec0cac80bd42ad98882
42261e6f5c424e854c8a54f17242936ae7e106b9527e439abf449ecc45648867
c1ccc(-c2ccc3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].C-C-C-[CH2]-[Sn](-[C;H0;D2;+0:10]#[C;H0;D2;+0:11]-[Si](-C)(-C)-C)(-[CH2]-C-C-C)-[CH2]-C-C-C>>[CH;D1;+0:11]#[C;H0;D2;+0:10]-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
87
[{"value": 87.0, "product": "FC=1C=C(C=C(C1O)F)C1=NC2=CC=C(C=C2C(=C1)C#C)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6c following a combination of method J using (trimethylsilylethynyl)tributyltin and method L. Yellow solid; Yield: 87%; mp 220° C. (dec.); 1H-NMR (300 MHz, acetone-d6) δ 4.39 (s, 1H), 7.45 (dd, J=9.1, 2.7 Hz, 1H), 7.60 (d, J=2.7 Hz, 1H), 7.95 (d, J=10.1 Hz, 1H), 7.96 (d, J=7.1 Hz, 1H), 8...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne.Silyl protective group.Tin
Alkyne
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
HBr.Sn
null
null
null
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3cc(F)c(O)c(F)c3)cc(Br)c2c1>>C#Cc1cc(-c2cc(F)c(O)c(F)c2)nc2ccc(O)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-61877ec17af6430e864c5fb131b6cb2a
CCC[CH2][Sn]([C]#Cc1ccccc1)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(C#Cc3ccccc3)c2c1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.C(CCC)[Sn](C#CC1=CC=CC=C1)(CCCC)CCCC>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C#CC1=CC=CC=C1)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[C:18]#[C:19][c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1.Br[c:17]1[cH:16][c:7](-[c:8]2[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]2)[n:6][c:5]2[cH:4][cH:3][c:2]([OH:1])[cH:27][c:26]21>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]3...
CCC[CH2][Sn]([C]#Cc1ccccc1)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(C#Cc3ccccc3)c2c1
null
null
null
C-C Coupling
Stille reaction_other
5b7d122d5cbf3feee31209339c4cd554facd746c4b7c95e3041c641d09f4e525
84197a108c0019520f13001872ce55981c95862f930591903269e152b52aac86
C(#Cc1cc(-c2ccccc2)nc2ccccc12)c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].C-C-C-[CH2]-[Sn](-[C;H0;D2;+0:10]#[C:11]-[c:12])(-[CH2]-C-C-C)-[CH2]-C-C-C>>[c:12]-[C:11]#[C;H0;D2;+0:10]-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
92
[{"value": 92.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C#CC1=CC=CC=C1)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b and tributyl(phenylethynyl)tin according to method J. Orange powder; Yield: 92%; mp 125–129° C; 1H-NMR (300 MHz, DMSO-d6) δ 7.08 (dd, J=8.8, 8.8 Hz, 1H), 7.36 (dd, J=9.0, 2.6 Hz, 1H), 7.53 (m, 3H), 7.59 (d, J=2.6 Hz, 1H), 7.74 (m, 2H), 7.94 (d, J=9.1 Hz, 2H), 8.05 (dd, J=13.0, 1.8 Hz,...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne.Tin
Alkyne
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1ccccc1.c1ccccc1
HBr.Sn
null
null
null
CCC[CH2][Sn]([C]#Cc1ccccc1)([CH2]CCC)[CH2]CCC.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(C#Cc3ccccc3)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-51161c16317b4c838a8ed98ea6f53449
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1nccs1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3nccs3)c2c1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.C(CCC)[Sn](C=1SC=CN1)(CCCC)CCCC>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C=1SC=CN1)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c:18]1[n:19][cH:20][cH:21][s:22]1.Br[c:17]1[cH:16][c:7](-[c:8]2[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]2)[n:6][c:5]2[cH:4][cH:3][c:2]([OH:1])[cH:24][c:23]21>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]3)[cH:16][c:17](-[c:18]...
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1nccs1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3nccs3)c2c1
null
null
null
C-C Coupling
Stille reaction_aryl
fc253538fac18be712decdf7e55d082e5584b30a027de13d08589650e0a5abd9
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
c1ccc(-c2cc(-c3nccs3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[c;H0;D3;+0:10]1:[#16;a:11]:[c:12]:[c:13]:[#7;a:14]:1>>[c:9]:[c:8]1:[c:6](:[c:7]):[#7;a:5]:[c:3](-[c:4]):[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:10]1:[#16;a:11]:[c:12]:[c:13]:[#7;a:14]:1
56
[{"value": 56.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C=1SC=CN1)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b and 2-tributylstannylthiazole according to method J. Yellow powder; Yield: 56%; mp>280° C. (dec.); 1H-NMR (400 MHz, DMSO-d6) δ 7.10 (t, J=8.8 Hz, 1H), 7.38 (dd, J=9.1, 2.7 Hz, 1H), 7.95–8.00 (m, 2H), 8.07–8.12 (m, 3H), 8.21 (m, 2H), 10.18 (s, 1H), 10.26 (s, 1H); MS (ESI) m/z 337 ([M−H...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1cscn1.c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1cscn1
c1ccc2ncccc2c1.c1ccccc1.c1cscn1
HBr.Sn
null
null
null
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1nccs1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3nccs3)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-04c274e7ad19452d83077b67cba5d514
Cc1ccc(B(O)O)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3ccc(O)cc23)cc1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.B(C=1C=CC(=CC1)C)(O)O>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CC=C(C=C1)C)O
OB(O)[c:5]1[cH:4][cH:3][c:2]([CH3:1])[cH:26][cH:25]1.Br[c:6]1[cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([OH:13])[c:14]([F:15])[cH:16]2)[n:17][c:18]2[cH:19][cH:20][c:21]([OH:22])[cH:23][c:24]12>>[CH3:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][c:8](-[c:9]3[cH:10][cH:11][c:12]([OH:13])[c:14]([F:15])[cH:16]3)[n:17][c:18]3[cH:19]...
Cc1ccc(B(O)O)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3ccc(O)cc23)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccccc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[c:7]:[c:6]1:[#7;a:5]:[c:3](-[c:4]):[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:8]:1:[c:9]
85
[{"value": 85.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CC=C(C=C1)C)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b using p-tolylboronic acid according to method P. Orange powder; Yield: 85%; mp 184–188° C.; 1H-NMR (300 MHz, DMSO-d6) δ 2.44 (s, 3H), 7.07 (dd, J=8.8, 8.8 Hz, 1H), 7.12 (d, J=2.6 Hz, 1H), 7.31 (dd, J=9.1, 2.6 Hz, 1H), 7.40 (d, J=8.0 Hz, 2H), 7.49 (d, J=8.0 Hz, 2H), 7.82 (s, 1H), 7.94 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccccc1.c1ccc2ncccc2c1
HBr.B
null
null
null
Cc1ccc(B(O)O)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3ccc(O)cc23)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2fa5700fd5364c35af981aebf453db3e
OB(O)c1ccc(F)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(F)cc3)c2c1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.FC1=CC=C(C=C1)B(O)O>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CC=C(C=C1)F)O
OB(O)[c:18]1[cH:19][cH:20][c:21]([F:22])[cH:23][cH:24]1.Br[c:17]1[cH:16][c:7](-[c:8]2[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]2)[n:6][c:5]2[cH:4][cH:3][c:2]([OH:1])[cH:26][c:25]21>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]3)[cH:16][c:17](-[c:18]3[cH:19][cH...
OB(O)c1ccc(F)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(F)cc3)c2c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccccc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]):[c:13]:[c:14]
90
[{"value": 90.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CC=C(C=C1)F)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b using 4-fluorophenylboronic acid according to method P. Orange powder; Yield: 90%; mp 240–243° C.; 1H-NMR (300 MHz, DMSO-d6) δ 7.05 (d, J=2.6 Hz, 1H), 7.07 (dd, J=8.9, 8.7 Hz, 1H), 7.32 (dd, J=9.0, 2.6 Hz, 1H), 7.44 (dd, J=8.9, 8.9 Hz, 2H), 7.63 (m, 2H), 7.86 (s, 1H), 7.95 (dd, J=8.4,...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1ccccc1
c1ccc2ncccc2c1.c1ccccc1.c1ccccc1
HBr.B
null
null
null
OB(O)c1ccc(F)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(F)cc3)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2e87ef03d13944988967e1bb4dcac910
OB(O)c1ccc(Cl)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(Cl)cc3)c2c1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.ClC1=CC=C(C=C1)B(O)O>>ClC1=CC=C(C=C1)C1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F
OB(O)[c:18]1[cH:19][cH:20][c:21]([Cl:22])[cH:23][cH:24]1.Br[c:17]1[cH:16][c:7](-[c:8]2[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]2)[n:6][c:5]2[cH:4][cH:3][c:2]([OH:1])[cH:26][c:25]21>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]3)[cH:16][c:17](-[c:18]3[cH:19][c...
OB(O)c1ccc(Cl)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(Cl)cc3)c2c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccccc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]):[c:13]:[c:14]
87
[{"value": 87.0, "product": "ClC1=CC=C(C=C1)C1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b using 4-chlorophenylboronic acid according to method P. Orange powder; Yield: 87%; mp 140–147° C.; 1H-NMR (400 MHz, DMSO-d6) δ 7.03 (d, J=2.7 Hz, 1H), 7.06 (t, J=8.8 Hz, 1H), 7.32 (dd, J=9.1, 2.7 Hz, 1H), 7.63 (d, J=8.8 Hz, 2H), 7.67 (d, J=8.7 Hz, 2H), 7.87 (s, 1H), 7.93–7.98 (m, 2H),...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1ccccc1
c1ccc2ncccc2c1.c1ccccc1.c1ccccc1
HBr.B
null
null
null
OB(O)c1ccc(Cl)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(Cl)cc3)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-abdf39d15bf8495fba05b5d7db69b61a
N#Cc1ccc(B(O)O)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>N#Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3ccc(O)cc23)cc1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.C(#N)C1=CC=C(C=C1)B(O)O>>C(#N)C1=CC=C(C=C1)C1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F
OB(O)[c:6]1[cH:5][cH:4][c:3]([C:2]#[N:1])[cH:27][cH:26]1.Br[c:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][c:13]([OH:14])[c:15]([F:16])[cH:17]2)[n:18][c:19]2[cH:20][cH:21][c:22]([OH:23])[cH:24][c:25]12>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][c:9](-[c:10]3[cH:11][cH:12][c:13]([OH:14])[c:15]([F:16])[cH:17]3)[n:18][c:1...
N#Cc1ccc(B(O)O)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
N#Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3ccc(O)cc23)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccccc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[c:4]-[c:3]1:[#7;a:5]:[c:6](:[c:7]):[c:8](:[c:9]):[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:2]:1
52
[{"value": 52.0, "product": "C(#N)C1=CC=C(C=C1)C1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b using 4-cyanophenylboronic acid according to method P. Yellow powder; Yield: 52%; mp 266–267° C.; 1H-NMR (400 MHz, DMSO-d6) δ 6.97 (d, J=2.7 Hz, 1H), 7.07 (t, J=8.8 Hz, 1H), 7.34 (dd, J=9.0, 2.6 Hz, 1H), 7.82 (d, J=8.5 Hz, 2H), 7.92 (s, 1H), 7.95–8.00 (m, 2H), 8.07–8.10 (m, 3H), 10.00...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccccc1.c1ccc2ncccc2c1
HBr.B
null
null
null
N#Cc1ccc(B(O)O)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>N#Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3ccc(O)cc23)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-3b1a5620622c48788ea58af1537cfdc0
OB(O)c1ccc(C(F)(F)F)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(C(F)(F)F)cc3)c2c1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.FC(C1=CC=C(C=C1)B(O)O)(F)F>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CC=C(C=C1)C(F)(F)F)O
OB(O)[c:18]1[cH:19][cH:20][c:21]([C:22]([F:23])([F:24])[F:25])[cH:26][cH:27]1.Br[c:17]1[cH:16][c:7](-[c:8]2[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]2)[n:6][c:5]2[cH:4][cH:3][c:2]([OH:1])[cH:29][c:28]21>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]3)[cH:16][c:...
OB(O)c1ccc(C(F)(F)F)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(C(F)(F)F)cc3)c2c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccccc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]):[c:13]:[c:14]
76
[{"value": 76.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CC=C(C=C1)C(F)(F)F)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b using 4-trifluoromethylphenylboronic acid according to method P. Yellow crystals; Yield: 76%; mp 299–300° C.; 1H-NMR (400 MHz, DMSO-d6) δ 7.07 (dd, J=8.8, 8.8 Hz, 1H), 7.12 (d, J=2.6 Hz, 1H), 7.31 (dd, J=9.1, 2.6 Hz, 1H), 7.40 (d, J=8.0 Hz, 2H), 7.49 (d, J=8.0 Hz, 2H), 7.82 (s, 1H), 7...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1ccccc1
c1ccc2ncccc2c1.c1ccccc1.c1ccccc1
HBr.B
null
null
null
OB(O)c1ccc(C(F)(F)F)cc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccc(C(F)(F)F)cc3)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0e818c8419c54a7fac724398d987ee72
OB(O)c1ccsc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccsc3)c2c1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.S1C=C(C=C1)B(O)O>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CSC=C1)O
OB(O)[c:18]1[cH:19][cH:20][s:21][cH:22]1.Br[c:17]1[cH:16][c:7](-[c:8]2[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]2)[n:6][c:5]2[cH:4][cH:3][c:2]([OH:1])[cH:24][c:23]21>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]3)[cH:16][c:17](-[c:18]3[cH:19][cH:20][s:21][cH:2...
OB(O)c1ccsc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccsc3)c2c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
7ec2bb10523ea4edebf661f837af8541c569fb5ea40337ce1dd151fc4300fa1e
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccsc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10]1:[c:11]:[c:12]:[#16;a:13]:[c:14]:1>>[c:9]:[c:8]1:[c:6](:[c:7]):[#7;a:5]:[c:3](-[c:4]):[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:10]1:[c:11]:[c:12]:[#16;a:13]:[c:14]:1
95
[{"value": 95.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CSC=C1)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b using 3-thiopheneboronic acid according to method P. Orange powder; Yield: 95%; mp>160° C. (dec.); 1H-NMR (400 MHz, DMSO-d6) δ 7.06 (t, J=8.8 Hz, 1H), 7.30–7.33 (m, 2H), 7.50 (dd, J=4.9, 1.2 Hz, 1H), 7.82 (dd, J=4.9, 3.0 Hz, 1H), 7.90–7.95 (m, 4H), 8.06 (dd, J=13.0, 2.1 Hz, 1H), 9.97 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccsc1.c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1ccsc1
c1ccc2ncccc2c1.c1ccccc1.c1ccsc1
HBr.B
null
null
null
OB(O)c1ccsc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccsc3)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2462d807654541a2a1bf0f369b69e9aa
OB(O)c1ccncc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccncc3)c2c1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.N1=CC=C(C=C1)B(O)O>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CC=NC=C1)O
OB(O)[c:18]1[cH:19][cH:20][n:21][cH:22][cH:23]1.Br[c:17]1[cH:16][c:7](-[c:8]2[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]2)[n:6][c:5]2[cH:4][cH:3][c:2]([OH:1])[cH:25][c:24]21>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]3)[cH:16][c:17](-[c:18]3[cH:19][cH:20][n:2...
OB(O)c1ccncc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccncc3)c2c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
65c50f146f4e013debcd45594af7db1f345f787e9158328ac1b943e3b140f8c7
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccncc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:[c:15]:1>>[c:9]:[c:8]1:[c:6](:[c:7]):[#7;a:5]:[c:3](-[c:4]):[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:[c:15]:1
20
[{"value": 20.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C1=CC=NC=C1)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b using 4-pyridinylboronic acid according to method P. Yellow powder; Yield: 20%; mp>350° C. (dec.); 1H-NMR (400 MHz, DMSO-d6) δ 7.02 (d, J=2.6 Hz, 1H), 7.07 (t, J=8.8 Hz, 1H), 7.34 (dd, J=9.0, 2.6 Hz, 1H), 7.64 (d, J=5.9 Hz, 2H), 7.93 (s, 1H), 7.95–8.00 (m, 2H), 8.08 (dd, J=13.0, 2.1 H...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1ccncc1
c1ccc2ncccc2c1.c1ccccc1.c1ccncc1
HBr.B
null
null
null
OB(O)c1ccncc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3ccncc3)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bf76c2d6b3c04c949b881161cb4b3370
OB(O)c1cncnc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3cncnc3)c2c1
BrC1=CC(=NC2=CC=C(C=C12)O)C1=CC(=C(C=C1)O)F.N1=CN=CC(=C1)B(O)O>>FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C=1C=NC=NC1)O
OB(O)[c:18]1[cH:19][n:20][cH:21][n:22][cH:23]1.Br[c:17]1[cH:16][c:7](-[c:8]2[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]2)[n:6][c:5]2[cH:4][cH:3][c:2]([OH:1])[cH:25][c:24]21>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([OH:12])[c:13]([F:14])[cH:15]3)[cH:16][c:17](-[c:18]3[cH:19][n:20][cH:21...
OB(O)c1cncnc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3cncnc3)c2c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
0d1faee6975c7818135cd293769cc69788382bc29eaa2ec7b2053932304d61e3
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3cncnc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10]1:[c:11]:[#7;a:12]:[c:13]:[#7;a:14]:[c:15]:1>>[c:9]:[c:8]1:[c:6](:[c:7]):[#7;a:5]:[c:3](-[c:4]):[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:10]1:[c:11]:[#7;a:12]:[c:13]:[#7;a:14]:[c:15]:1
34
[{"value": 34.0, "product": "FC=1C=C(C=CC1O)C1=NC2=CC=C(C=C2C(=C1)C=1C=NC=NC1)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 6b using 5-pyrimidinylboronic acid according to method P. Yellow powder; Yield: 34%; mp>340° C. (dec.); 1H-NMR (400 MHz, DMSO-d6) δ 7.00 (d, J=2.6 Hz, 1H), 7.08 (t, J=8.8 Hz, 1H), 7.36 (dd, J=9.0, 2.6 Hz, 1 H), 7.98–8.02 (m, 2H), 8.08 (s, 1H), 8.11 (dd, J=13.1, 2.2 Hz, 1H), 9.11 (s, 2H),...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cncnc1.c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1cncnc1
c1ccc2ncccc2c1.c1ccccc1.c1cncnc1
HBr.B
null
null
null
OB(O)c1cncnc1.Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>Oc1ccc2nc(-c3ccc(O)c(F)c3)cc(-c3cncnc3)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-24f6748ad3254b64b7ff404d539083cd
OB(O)c1ccc(F)cc1.Oc1ccc(-c2nc3ccc(O)cc3c(Br)c2Cl)cc1>>Oc1ccc(-c2nc3ccc(O)cc3c(-c3ccc(F)cc3)c2Cl)cc1
BrC1=C(C(=NC2=CC=C(C=C12)O)C1=CC=C(C=C1)O)Cl.FC1=CC=C(C=C1)B(O)O>>ClC=1C(=NC2=CC=C(C=C2C1C1=CC=C(C=C1)F)O)C1=CC=C(C=C1)O
OB(O)[c:16]1[cH:17][cH:18][c:19]([F:20])[cH:21][cH:22]1.Br[c:15]1[c:14]2[c:8]([n:7][c:6](-[c:5]3[cH:4][cH:3][c:2]([OH:1])[cH:26][cH:25]3)[c:23]1[Cl:24])[cH:9][cH:10][c:11]([OH:12])[cH:13]2>>[OH:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[n:7][c:8]3[cH:9][cH:10][c:11]([OH:12])[cH:13][c:14]3[c:15](-[c:16]3[cH:17][cH:18][c:19]([F:2...
OB(O)c1ccc(F)cc1.Oc1ccc(-c2nc3ccc(O)cc3c(Br)c2Cl)cc1
Oc1ccc(-c2nc3ccc(O)cc3c(-c3ccc(F)cc3)c2Cl)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccccc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7](-[c:8]):[c:9]:1-[Cl;D1;H0:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]>>[Cl;D1;H0:10]-[c:9]1:[c:7](-[c:8]):[#7;a:6]:[c:4](:[c:5]):[c:2](:[c:3]):[c;H0;D3;+0:1]:1-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]
95
[{"value": 95.0, "product": "ClC=1C(=NC2=CC=C(C=C2C1C1=CC=C(C=C1)F)O)C1=CC=C(C=C1)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 35a and 4-fluorophenylboronic acid according to method P. White solid; Yield: 95%; mp 295–296° C.; 1H-NMR (300 MHz, DMSO-d6) δ 6.55 (d, J=2.6 Hz, 1H), 6.87 (d, J=8.6 Hz, 2H), 7.31 (dd, J=9.1, 2.6 Hz, 1H), 7.45 (m, 4H), 7.57 (d, J=8.6 Hz, 2H), 7.92 (d, J=9.1 Hz, 1H), 9.73 (s, 1H), 10.07 (...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1ccccc1
c1ccccc1.c1ccc2ncccc2c1.c1ccccc1
HBr.B
null
null
null
OB(O)c1ccc(F)cc1.Oc1ccc(-c2nc3ccc(O)cc3c(Br)c2Cl)cc1>>Oc1ccc(-c2nc3ccc(O)cc3c(-c3ccc(F)cc3)c2Cl)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2b0d9ce6dac1428494fdac9548bda8fb
COc1ccc2nc(-c3ccc(OC)c(F)c3)c(Cl)c(Br)c2c1.O=C1CC[C@@H](C(=O)O)N1>>N#Cc1c(Cl)c(-c2ccc(O)c(F)c2)nc2ccc(O)cc12
BrC1=C(C(=NC2=CC=C(C=C12)OC)C1=CC(=C(C=C1)OC)F)Cl.N1[C@@H](CCC1=O)C(=O)O.Cl>>ClC=1C(=NC2=CC=C(C=C2C1C#N)O)C1=CC(=C(C=C1)O)F
C[O:11][c:10]1[cH:9][cH:8][c:7](-[c:6]2[c:4]([Cl:5])[c:3](Br)[c:22]3[c:16]([n:15]2)[cH:17][cH:18][c:19]([O:20]C)[cH:21]3)[cH:14][c:12]1[F:13].O=C(O)[C@@H]1CC[C:2](=O)[NH:1]1>>[N:1]#[C:2][c:3]1[c:4]([Cl:5])[c:6](-[c:7]2[cH:8][cH:9][c:10]([OH:11])[c:12]([F:13])[cH:14]2)[n:15][c:16]2[cH:17][cH:18][c:19]([OH:20])[cH:21][c:...
COc1ccc2nc(-c3ccc(OC)c(F)c3)c(Cl)c(Br)c2c1.O=C1CC[C@@H](C(=O)O)N1
N#Cc1c(Cl)c(-c2ccc(O)c(F)c2)nc2ccc(O)cc12
null
null
null
C-C Coupling
OtherReaction
e0141a8a25f67f65ff4a531b5b01a33f09546dbc4f21eaf313e861d84a1da590
84342470fb695059ed8ce211dd27ea5e5a1d7559cdd73a98a0caf487589adb38
c1ccc(-c2ccc3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]2:[c:3]:[c:4](-[O;H0;D2;+0:5]-C):[c:6]:[c:7]:[c:8]:2:[#7;a:9]:[c:10](-[c:11]):[c:12]:1-[Cl;D1;H0:13].C-[O;H0;D2;+0:14]-[c:15](:[c:16]):[c:17].O-C(=O)-[C@H]1-C-C-[C;H0;D3;+0:18](=O)-[NH;D2;+0:19]-1>>[Cl;D1;H0:13]-[c:12]1:[c:10](-[c:11]):[#7;a:9]:[c:8]2:[c:7]:[c:6]:[c:4](-[OH;D1;+0:5]):[c:3]:[c:2]...
41
[{"value": 41.0, "product": "ClC=1C(=NC2=CC=C(C=C2C1C#N)O)C1=CC(=C(C=C1)O)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 34b according to method F and method G (using Pyr./HCl). Yellow solid; Yield: 41% (for two steps); mp 325–328° C. (dec.); 1H-NMR (300 MHz, DMSO-d6) δ 7.10 (dd, J=8.8, 8.7 Hz, 1H), 7.27 (d, J=2.5 Hz, 1H), 7.43 (dd, J=8.4, 1.4 Hz, 1H), 7.49 (dd, J=9.2, 2.5 Hz, 1H), 7.55 (dd, J=12.2, 2.0 Hz...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carboxylic acid.Ether.Ether.Secondary amide
Nitrile.Aromatic alcohol.Aromatic alcohol
c1ccc2ncccc2c1.C1CCNC1
c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
HBr
null
null
null
COc1ccc2nc(-c3ccc(OC)c(F)c3)c(Cl)c(Br)c2c1.O=C1CC[C@@H](C(=O)O)N1>>N#Cc1c(Cl)c(-c2ccc(O)c(F)c2)nc2ccc(O)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-33d7c3429b6b44bb87a813f255e9b2cc
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>C#Cc1cc(-c2ccc(O)c(F)c2)nc2c(Cl)cc(O)cc12
BrC1=CC(=NC2=C(C=C(C=C12)O)Cl)C1=CC(=C(C=C1)O)F.C[Si](C)(C)C#C[Sn](CCCC)(CCCC)CCCC>>ClC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)O)F)C#C)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[C:2]#[C:1][Si](C)(C)C.Br[c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([OH:10])[c:11]([F:12])[cH:13]2)[n:14][c:15]2[c:16]([Cl:17])[cH:18][c:19]([OH:20])[cH:21][c:22]12>>[CH:1]#[C:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([OH:10])[c:11]([F:12])[cH:13]2)[n:14][c:15]2[c:16]([Cl:17])[cH:18][...
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
C#Cc1cc(-c2ccc(O)c(F)c2)nc2c(Cl)cc(O)cc12
null
null
null
C-C Coupling
OtherReaction
519663089044573005838583055d682ebb55d07ad1272ec0cac80bd42ad98882
42261e6f5c424e854c8a54f17242936ae7e106b9527e439abf449ecc45648867
c1ccc(-c2ccc3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].C-C-C-[CH2]-[Sn](-[C;H0;D2;+0:10]#[C;H0;D2;+0:11]-[Si](-C)(-C)-C)(-[CH2]-C-C-C)-[CH2]-C-C-C>>[CH;D1;+0:11]#[C;H0;D2;+0:10]-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
73
[{"value": 73.0, "product": "ClC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)O)F)C#C)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 45a following a combination of method J using (trimethylsilylethynyl)tributyltin and method L. Yellow solid; Yield: 73%; mp 210° C. (dec.); 1H-NMR (400 MHz, DMSO-d6) δ 5.06 (s, 1H), 7.09 (dd, J=8.9, 8.8 Hz, 1H), 7.45 (d, J=2.6 Hz, 1H), 7.56 (d, J=2.6 Hz, 1H), 8.00 (dd, J=8.5, 1.7 Hz, 1H)...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne.Silyl protective group.Tin
Alkyne
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
HBr.Sn
null
null
null
CCC[CH2][Sn]([C]#C[Si](C)(C)C)([CH2]CCC)[CH2]CCC.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>C#Cc1cc(-c2ccc(O)c(F)c2)nc2c(Cl)cc(O)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d2ccbacffcae40e28a57686d20464e40
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>C=Cc1cc(-c2ccc(O)c(F)c2)nc2c(Cl)cc(O)cc12
BrC1=CC(=NC2=C(C=C(C=C12)O)Cl)C1=CC(=C(C=C1)O)F.C(CCC)[Sn](C=C)(CCCC)CCCC>>ClC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)O)F)C=C)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[CH:2]=[CH2:1].Br[c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([OH:10])[c:11]([F:12])[cH:13]2)[n:14][c:15]2[c:16]([Cl:17])[cH:18][c:19]([OH:20])[cH:21][c:22]12>>[CH2:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([OH:10])[c:11]([F:12])[cH:13]2)[n:14][c:15]2[c:16]([Cl:17])[cH:18][c:19](...
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
C=Cc1cc(-c2ccc(O)c(F)c2)nc2c(Cl)cc(O)cc12
null
null
null
C-C Coupling
Stille reaction_vinyl
b76d02284eab1606d02e43e8d6b217f827d8bc76b0b2203ccf942abed5fcc5b2
ec03c739f58696d2a3659a73884744e1a490a20a587da6f115be382b663cf23d
c1ccc(-c2ccc3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[CH;D2;+0:10]=[C;D1;H2:11]>>[C;D1;H2:11]=[CH;D2;+0:10]-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
84
[{"value": 84.0, "product": "ClC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)O)F)C=C)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 45a based on method J using 1.1 equiv. of tributyl(vinyl)tin at 90° C. Red solid; Yield: 84%; mp 225° C. (dec.); 1H-NMR (400 MHz, DMSO-d6) δ 5.74 (dd, J=11.1, 1.0 Hz, 1H), 6.30 (dd, J=17.3, 1.1 Hz, 1H), 7.10 (dd, J=8.8, 8.8 Hz, 1H), 7.35 (d, J=2.6 Hz, 1H), 7.38 (dd, J=17.3, 11.1 Hz, 1H),...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl.Tin
Vinyl
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
HBr.Sn
null
null
null
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>C=Cc1cc(-c2ccc(O)c(F)c2)nc2c(Cl)cc(O)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-22992e010418414795f879d0f01603fc
N#Cc1ccc(B(O)O)cc1.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>N#Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3c(Cl)cc(O)cc23)cc1
BrC1=CC(=NC2=C(C=C(C=C12)O)Cl)C1=CC(=C(C=C1)O)F.C(#N)C1=CC=C(C=C1)B(O)O>>ClC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)O)F)C1=CC=C(C=C1)C#N)O
OB(O)[c:6]1[cH:5][cH:4][c:3]([C:2]#[N:1])[cH:28][cH:27]1.Br[c:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][c:13]([OH:14])[c:15]([F:16])[cH:17]2)[n:18][c:19]2[c:20]([Cl:21])[cH:22][c:23]([OH:24])[cH:25][c:26]12>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][c:9](-[c:10]3[cH:11][cH:12][c:13]([OH:14])[c:15]([F:16])[cH:17]3)[n...
N#Cc1ccc(B(O)O)cc1.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
N#Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3c(Cl)cc(O)cc23)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccccc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[c:4]-[c:3]1:[#7;a:5]:[c:6](:[c:7]):[c:8](:[c:9]):[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:2]:1
94
[{"value": 94.0, "product": "ClC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)O)F)C1=CC=C(C=C1)C#N)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 45a using 4-cyanophenylboronic acid according to method P. Yellow solid; Yield: 94%; mp 324° C. (dec.); 1H-NMR (400 MHz, DMSO-d6) δ 6.93 (d, J=2.5 Hz, 1H), 7.09 (dd, J=8.8, 8.8 Hz, 1H), 7.54 (d, J=2.6 Hz, 1H), 7.81 (d, J=8.4 Hz, 2H), 8.03 (s, 1H), 8.04 (dd, J=8.5, 1.6 Hz, 1H), 8.09 (d, J...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccccc1.c1ccc2ncccc2c1
HBr.B
null
null
null
N#Cc1ccc(B(O)O)cc1.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>N#Cc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3c(Cl)cc(O)cc23)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-81279442efa746b7a617ec2073a76c32
COc1ccc(B(O)O)cc1.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>COc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3c(Cl)cc(O)cc23)cc1
BrC1=CC(=NC2=C(C=C(C=C12)O)Cl)C1=CC(=C(C=C1)O)F.COC1=CC=C(C=C1)B(O)O>>ClC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)O)F)C1=CC=C(C=C1)OC)O
OB(O)[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:28][cH:27]1.Br[c:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][c:13]([OH:14])[c:15]([F:16])[cH:17]2)[n:18][c:19]2[c:20]([Cl:21])[cH:22][c:23]([OH:24])[cH:25][c:26]12>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][c:9](-[c:10]3[cH:11][cH:12][c:13]([OH:14])[c:15]([F:16])[cH:17]3)...
COc1ccc(B(O)O)cc1.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1
COc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3c(Cl)cc(O)cc23)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cc(-c3ccccc3)c3ccccc3n2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[c:4]-[c:3]1:[#7;a:5]:[c:6](:[c:7]):[c:8](:[c:9]):[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:2]:1
97
[{"value": 97.0, "product": "ClC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)O)F)C1=CC=C(C=C1)OC)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 45a using 4-methoxyphenylboronic acid according to method P. Orange solid; Yield: 97%; mp 140–142° C.; 1H-NMR (400 MHz, DMSO-d6) δ 3.87 (s, 3H), 7.09 (dd, J=8.8, 8.8 Hz, 1H), 7.11 (d, J=2.7 Hz, 1H), 7.16 (d, J=8.8 Hz, 2H), 7.51 (d, J=2.6 Hz, 1H), 7.53 (d, J=8.8 Hz, 2H), 7.93(s, 1H), 8.02...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccccc1.c1ccc2ncccc2c1
HBr.B
null
null
null
COc1ccc(B(O)O)cc1.Oc1cc(Cl)c2nc(-c3ccc(O)c(F)c3)cc(Br)c2c1>>COc1ccc(-c2cc(-c3ccc(O)c(F)c3)nc3c(Cl)cc(O)cc23)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5ba227c56f3a4e9babf17bf816fa60e1
COc1cc(Br)c2nc(-c3ccc(OC)c(F)c3)cc(O)c2c1.N#Cc1ccc(B(O)O)cc1>>COc1cc(-c2ccc(C#N)cc2)c2nc(-c3ccc(OC)c(F)c3)cc(O)c2c1
BrC=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)OC)F)O)OC.C(#N)C1=CC=C(C=C1)B(O)O>>C(#N)C1=CC=C(C=C1)C=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)OC)F)O)OC
Br[c:5]1[cH:4][c:3]([O:2][CH3:1])[cH:30][c:29]2[c:14]1[n:15][c:16](-[c:17]1[cH:18][cH:19][c:20]([O:21][CH3:22])[c:23]([F:24])[cH:25]1)[cH:26][c:27]2[OH:28].OB(O)[c:6]1[cH:7][cH:8][c:9]([C:10]#[N:11])[cH:12][cH:13]1>>[CH3:1][O:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([C:10]#[N:11])[cH:12][cH:13]2)[c:14]2[n:15][c:16]...
COc1cc(Br)c2nc(-c3ccc(OC)c(F)c3)cc(O)c2c1.N#Cc1ccc(B(O)O)cc1
COc1cc(-c2ccc(C#N)cc2)c2nc(-c3ccc(OC)c(F)c3)cc(O)c2c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
73d3d45d842e591351c81053feb1b3096820b80e5a86db47217e78e2a9707cc8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3cccc(-c4ccccc4)c3n2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7].O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[c:10]:[c:9]:[c;H0;D3;+0:8](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]):[c:11]:[c:12]
56
[{"value": 56.0, "product": "C(#N)C1=CC=C(C=C1)C=1C=C(C=C2C(=CC(=NC12)C1=CC(=C(C=C1)OC)F)O)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound was prepared from 41b using 4-cyanophenylboronic acid according to method P. Orange solid; Yield: 56%; mp 248–250° C.; 1H NMR (300 MHz, DMSO-d6) δ 3.89 (s, 3H), 3.94 (s, 3H), 7.28 (t, J=8.8 Hz, 1H), 7.36 (s, 1H), 7.44 (d, J=2.9 Hz, 1H), 7.53 (d, J=2.9 Hz, 1H), 7.75–7.79 (m, 2H), 7.97 (br s, 4H), 11.50 (s,...
10.6084/m9.figshare.5104873.v1
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Aromatic halide.Boronic acid
null
c1ccc2ncccc2c1.c1ccccc1
c1ccccc1.c1ccc2ncccc2c1
c1ccccc1.c1ccc2ncccc2c1.c1ccccc1
HBr.B
null
null
null
COc1cc(Br)c2nc(-c3ccc(OC)c(F)c3)cc(O)c2c1.N#Cc1ccc(B(O)O)cc1>>COc1cc(-c2ccc(C#N)cc2)c2nc(-c3ccc(OC)c(F)c3)cc(O)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-3b6de8a0b0db409880422faff950189b
Nc1ccccc1.O=[N+]([O-])c1ccc(Cl)cc1>>O=[N+]([O-])c1ccc(Nc2ccccc2)cc1
NC1=CC=CC=C1.[N+](=O)([O-])C1=CC=C(C=C1)Cl.NC1=CC=CC=C1>>C1=CC=C(C=C1)NC2=CC=C(C=C2)[N+](=O)[O-]
[NH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1.Cl[c:7]1[cH:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:16][cH:15]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([NH:8][c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[cH:15][cH:16]1
Nc1ccccc1.O=[N+]([O-])c1ccc(Cl)cc1
O=[N+]([O-])c1ccc(Nc2ccccc2)cc1
null
null
null
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
da9dae6a655c4bd18887b692f91621e77027436294d6e1fc7be7295afb364796
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2ccccc2)cc1
Cl-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:8]:[c:7](-[NH;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]
null
[]
null
null
null
null
aniline method, where p-nitro-chlorobenzene and aniline as raw materials react in the presence of a catalyst to produce 4-nitrodiphenylamine, then, 4-nitrodiphenylamine is reduced by sodium sulfide to form 4-aminodiphenylamine; Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HCl
null
null
null
Nc1ccccc1.O=[N+]([O-])c1ccc(Cl)cc1>>O=[N+]([O-])c1ccc(Nc2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-34bb9f2f23f345d6881cdbdf4c474d23
O=[N+]([O-])c1ccc(Nc2ccccc2)cc1>>Nc1ccc(Nc2ccccc2)cc1
C1=CC=C(C=C1)NC2=CC=C(C=C2)[N+](=O)[O-].[S-2].[Na+].[Na+]>>C1=CC=C(C=C1)NC2=CC=C(C=C2)N
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]([NH:6][c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][cH:14]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([NH:6][c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][cH:14]1
O=[N+]([O-])c1ccc(Nc2ccccc2)cc1
Nc1ccc(Nc2ccccc2)cc1
null
null
null
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Nc2ccccc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
aniline method, where p-nitro-chlorobenzene and aniline as raw materials react in the presence of a catalyst to produce 4-nitrodiphenylamine, then, 4-nitrodiphenylamine is reduced by sodium sulfide to form 4-aminodiphenylamine; Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
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Nitro group
Primary amine
null
null
c1ccccc1.c1ccccc1
Other
null
null
null
O=[N+]([O-])c1ccc(Nc2ccccc2)cc1>>Nc1ccc(Nc2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7a9eeef338d34ed09b7439bf73611b0e
Nc1ccccc1.O=[N+]([O-])c1ccc(Cl)cc1>>O=[N+]([O-])c1ccc(Nc2ccccc2)cc1
C(=O)NC1=CC=CC=C1.NC1=CC=CC=C1.[N+](=O)([O-])C1=CC=C(C=C1)Cl.C([O-])([O-])=O.[K+].[K+].C(=O)NC1=CC=CC=C1>>C1=CC=C(C=C1)NC2=CC=C(C=C2)[N+](=O)[O-]
[NH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1.Cl[c:7]1[cH:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:16][cH:15]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([NH:8][c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[cH:15][cH:16]1
Nc1ccccc1.O=[N+]([O-])c1ccc(Cl)cc1
O=[N+]([O-])c1ccc(Nc2ccccc2)cc1
null
null
C(=O)O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
da9dae6a655c4bd18887b692f91621e77027436294d6e1fc7be7295afb364796
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2ccccc2)cc1
Cl-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:8]:[c:7](-[NH;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]
null
[]
null
null
null
null
formanilide method, where formic acid and aniline are used as starting materials to prepare formanilide, which in turn reacts with p-nitro-chlorobenzene in the presence of an acid-binding agent such as potassium carbonate, to produce 4-nitrodiphenylamine, and then, 4-nitrodiphenylamine is reduced by sodium sulfide to f...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HCl
C(=O)O
null
null
Nc1ccccc1.O=[N+]([O-])c1ccc(Cl)cc1>C(=O)O>O=[N+]([O-])c1ccc(Nc2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-fb202ce28fce4b4aa4357668711c12d9
O=[N+]([O-])c1ccc(Nc2ccccc2)cc1>>Nc1ccc(Nc2ccccc2)cc1
C1=CC=C(C=C1)NC2=CC=C(C=C2)[N+](=O)[O-].[S-2].[Na+].[Na+]>>C1=CC=C(C=C1)NC2=CC=C(C=C2)N
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]([NH:6][c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][cH:14]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([NH:6][c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][cH:14]1
O=[N+]([O-])c1ccc(Nc2ccccc2)cc1
Nc1ccc(Nc2ccccc2)cc1
null
null
null
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Nc2ccccc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
formanilide method, where formic acid and aniline are used as starting materials to prepare formanilide, which in turn reacts with p-nitro-chlorobenzene in the presence of an acid-binding agent such as potassium carbonate, to produce 4-nitrodiphenylamine, and then, 4-nitrodiphenylamine is reduced by sodium sulfide to f...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccccc1
Other
null
null
null
O=[N+]([O-])c1ccc(Nc2ccccc2)cc1>>Nc1ccc(Nc2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e70b01ed6e6a4bcc904277bc74d3110e
c1ccc(Nc2ccccc2)cc1>>O=NN(c1ccccc1)c1ccccc1
C1(=CC=CC=C1)NC1=CC=CC=C1.C1(=CC=CC=C1)NC1=CC=CC=C1.N(=O)[O-]>>N(=O)N(C1=CC=CC=C1)C1=CC=CC=C1
[NH:3]([c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1)[c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1>>[O:1]=[N:2][N:3]([c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1)[c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1
c1ccc(Nc2ccccc2)cc1
O=NN(c1ccccc1)c1ccccc1
null
null
null
Miscellaneous
OtherReaction
97abfb757cd7a417aa05bf509390cc1dd42c2b1a0c96b91f95f5f6968df59ae4
797765290ff12ff8fc5d8a85352c4763898223fe8d7887a890f0208d031bd39f
c1ccc(Nc2ccccc2)cc1
[c:1]:[c:2](-[NH;D2;+0:3]-[c:4](:[c:5]):[c:6]):[c:7]>>[O;D1;H0:8]=[#7:9]-[N;H0;D3;+0:3](-[c:2](:[c:1]):[c:7])-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
diphenylamine method, where diphenylamine as raw material is nitrosated using a nitrite in an organic solvent to produce N-nitrosodiphenylamine, which is rearranged to 4-nitrosodiphenylamine hydrochloride under the action of anhydrous hydrogen chloride, and then, 4-nitrosodiphenylamine hydrochloride is neutralized with...
10.6084/m9.figshare.5104873.v1
null
Secondary amine
Hydrazone
null
null
c1ccccc1.c1ccccc1
Other
null
null
null
c1ccc(Nc2ccccc2)cc1>>O=NN(c1ccccc1)c1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0cb97dc9f2f146dc81187fbd22e6bbc9
CN(C)C.CO.COC(=O)OC>>COC(=O)[O-].C[N+](C)(C)C
C(OC)(OC)=O.CN(C)C.CO>>COC([O-])=O.C[N+](C)(C)C
[CH3:6][N:7]([CH3:8])[CH3:10].O[CH3:9].C[O:5][C:3]([O:2][CH3:1])=[O:4]>>[CH3:1][O:2][C:3](=[O:4])[O-:5].[CH3:6][N+:7]([CH3:8])([CH3:9])[CH3:10]
CN(C)C.CO.COC(=O)OC
COC(=O)[O-].C[N+](C)(C)C
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
3efa28bb7da20a8af742e588325974a8592b70db1c0bb0a9fae065dded35e252
607e925a6fd3c9c7471bcd5f5d75e257a9747db166c67a5d6c2c89cac4bbbe92
null
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C;D1;H3:5].O-[CH3;D1;+0:6].[C;D1;H3:7]-[N;H0;D3;+0:8](-[C;D1;H3:9])-[C;D1;H3:10]>>[C;D1;H3:5]-[#8:4]-[C:2](-[O-;H0;D1:1])=[O;D1;H0:3].[C;D1;H3:7]-[N+;H0;D4:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[CH3;D1;+0:6]
80.2
[{"value": 80.2, "product": "COC([O-])=O.C[N+](C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.1, "product": "COC([O-])=O.C[N+](C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
4
HOUR
To a 1.5 L autoclave equipped with a stirrer and a heating means were added 90 g (11.0 mol) of dimethyl carbonate, 59 g (1.0 mol) of trimethyl amine and 510 g (15 mol) of methanol. Stirring was initiated after the autoclave was sealed. The autoclave was heat to 140° C., and pressure was 1.5 MPa. The reaction was kept a...
10.6084/m9.figshare.5104873.v1
null
Carbonic Ester.Tertiary amine.Methanol
Carbonic Acid
null
null
null
HO-
null
140
4
CN(C)C.CO.COC(=O)OC>>COC(=O)[O-].C[N+](C)(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e695220a42e7464caba10ab706dbb1bd
CCN(CC)CC.CCOS(=O)(=O)OCC>>CC[N+](CC)(CC)CC
[OH-].[Na+].S(=O)(=O)(OCC)OCC.C(C)N(CC)CC.C(C)O>>[OH-].C(C)[N+](CC)(CC)CC
[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[CH2:8][CH3:9].CCOS(=O)(=O)O[CH2:6][CH3:7]>>[CH3:1][CH2:2][N+:3]([CH2:4][CH3:5])([CH2:6][CH3:7])[CH2:8][CH3:9]
CCN(CC)CC.CCOS(=O)(=O)OCC
CC[N+](CC)(CC)CC
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4fb461fd1d845eeffcd721907fb84dda2a83d6f16d6187a0c591ac1d342a1cfa
7c33147a6170e63e1fbe1110c4ce069481be57a96b70c4a5a6d7e8253f321bd2
null
C-C-O-S(=O)(=O)-O-[CH2;D2;+0:1]-[C;D1;H3:2].[C;D1;H3:3]-[C:4]-[N;H0;D3;+0:5](-[C:6]-[C;D1;H3:7])-[C:8]-[C;D1;H3:9]>>[C;D1;H3:3]-[C:4]-[N+;H0;D4:5](-[C:6]-[C;D1;H3:7])(-[C:8]-[C;D1;H3:9])-[CH2;D2;+0:1]-[C;D1;H3:2]
410.2
[{"value": 95.7, "product": "[OH-].C(C)[N+](CC)(CC)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 410.2, "product": "[OH-].C(C)[N+](CC)(CC)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
4
HOUR
To a 1.5 L autoclave equipped with a stirrer and a heating means were added 154 g (1.0 mol) of diethyl sulfate, 101 g (1.0 mol) of triethyl amine and 690 g (15 mol) of ethanol. Stirring was initiated after the autoclave was sealed. The autoclave was heat to 140° C., and pressure was 1.0 MPa. The reaction was kept at 14...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
null
null
null
null
HO-
null
140
4
CCN(CC)CC.CCOS(=O)(=O)OCC>>CC[N+](CC)(CC)CC
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d031c2a1d4404c0f8c49a7f6d73e8050
CC(C)(C)C(=O)CC(=O)C(C)(C)C.O.[OH-].[Zr+4]>>CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.[Zr]
[OH-].[Na+].[Cl-].[Cl-].[Cl-].[Cl-].[Zr+4].CC(C)(C(CC(C(C)(C)C)=O)=O)C.O>>CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.[Zr]
[CH3:1][C:2]([CH3:3])([CH3:21])[C:31](=[O:32])[CH2:33][C:34](=[O:35])[C:36]([CH3:37])([CH3:38])[CH3:39].[OH2:19].[OH-:6].[Zr+4:53]>>[CH3:1][C:2]([CH3:3])([CH3:4])[C:5](=[O:6])/[CH:7]=[C:8](\[OH:9])[C:10]([CH3:11])([CH3:12])[CH3:13].[CH3:14][C:15]([CH3:16])([CH3:17])[C:18](=[O:19])/[CH:20]=[C:21](\[OH:22])[C:23]([CH3:24...
CC(C)(C)C(=O)CC(=O)C(C)(C)C.O.[OH-].[Zr+4]
CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.[Zr]
null
null
CO
Acylation
OtherReaction
c22a721143f01f2466799be601772121394a32f25a80d253214aff053096e802
8d45196a57eebe875f9534d6f941f1cdc4cbacb7d09ae2588ed02920a79b77f0
null
[C;D1;H3:1]-[C;H0;D4;+0:2](-[C;D1;H3:3])(-[CH3;D1;+0:4])-[C;H0;D3;+0:5](=[O;D1;H0:6])-[CH2;D2;+0:7]-[C;H0;D3;+0:8](=[O;H0;D1;+0:9])-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13].[OH-;D0:14].[OH2;D0;+0:15].[Zr+4;H0;D0:16]>>[C;D1;H3:17]-[C:18](-[C;D1;H3:19])(-[C;D1;H3:20])-[C;H0;D3;+0:5](=[O;D1;H0:6])/[CH;D2;+0:7]=[C...
98.2
[{"value": 98.2, "product": "CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.[Zr]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.1, "product": "CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.CC(/C(=C/C(=O)C(C)(C)C)/O)(C)C.CC(/C(=C/C(=O)C(C)(C)...
null
null
1
HOUR
To 177 g of methanol, 43.7 g (0.216 mol) of 2,2,6,6-tetramethyl-3,5-heptanedione of 91% purity was dropwise added with stirring. To the resulting solution, a solution, which had been obtained by dissolving 12.7 g (0.054 mol) of ZrCl4 of 99% purity in 218 g of methanol and cooled to room temperature, was added over a pe...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone
Ketone.Ketone.Ketone.Ketone.Enol.Enol.Enol.Enol
null
null
null
null
CO
null
1
CC(C)(C)C(=O)CC(=O)C(C)(C)C.O.[OH-].[Zr+4]>CO>CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.CC(C)(C)C(=O)/C=C(\O)C(C)(C)C.[Zr]
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-dc825329a9534658b229511a87c5a84d
C1=CC2CCC1C2.C1=CC2CCC1C2>>C1=C2C3CCC(C3)C2CCC1
C1CC2CC1C=C2.C1CC2CC1C=C2.C=CC=C>>C12CCC(C3CCCC=C13)C2
[CH:2]1=[CH:8][CH:6]2[CH2:5][CH2:4][CH:3]1[CH2:7]2.C1=[CH:1][CH:11]2CC1[CH2:9][CH2:10]2>>[CH:1]1=[C:2]2[CH:3]3[CH2:4][CH2:5][CH:6]([CH2:7]3)[CH:8]2[CH2:9][CH2:10][CH2:11]1
C1=CC2CCC1C2.C1=CC2CCC1C2
C1=C2C3CCC(C3)C2CCC1
null
CC1=CC=C(C=C1)O
null
Functional Group Interconversion
OtherReaction
4ea1134b1431d680e613361a257dab0dc489a867ad8d3f93cf902a03efa8b1be
f1bbf9aa3c82f5e49be9f6d53533b6bb152f359232b6d32090c168949766aa71
C1=C2C3CCC(C3)C2CCC1
C1-C2-C=[CH;D2;+0:1]-[CH;D3;+0:2]-1-[C:3]-[CH2;D2;+0:4]-2.[C:5]1-[C:6]-[C:7]2-[C:8]-[C:9]-1-[CH;D2;+0:10]=[CH;D2;+0:11]-2>>[C:3]1-[CH2;D2;+0:2]-[CH;D2;+0:1]=[C;H0;D3;+0:10]2-[C:9]3-[C:5]-[C:6]-[C:7](-[C:8]-3)-[CH;D3;+0:11]-2-[CH2;D2;+0:4]-1
145.8
[{"value": 73.0, "product": "C12CCC(C3CCCC=C13)C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 145.8, "product": "C12CCC(C3CCCC=C13)C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
200
CELSIUS
null
null
A 400 ml autoclave was charged with bicyclo[2,2,1]-2-heptene (152 g, Aldrich), 4-methylphenol (1 g, Aldrich), and butadiene (110 g). The mixture was heated at 200° C. for 10 hours. The reaction mixtures from four identical reactions were combined and distilled at atmosphere to give starting bicyclo[2,2,1]-2-heptene (30...
10.6084/m9.figshare.5104873.v1
null
null
null
C1=CC2CCC1C2.C1=CC2CCC1C2
C1=C2C3CCC(C3)C2CCC1
C1=C2C3CCC(C3)C2CCC1
Other
CC1=CC=C(C=C1)O
200
null
C1=CC2CCC1C2.C1=CC2CCC1C2>CC1=CC=C(C=C1)O>C1=C2C3CCC(C3)C2CCC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-76944fac672d4c29a68933501960dba5
C1=C2C3CCC(C3)C2CCC1>>C1CCC2C3CCC(C3)C2C1
[H][H].C12CCC(C3CCCC=C13)C2.[H][H]>>C12CCC(C3CCCCC13)C2
[CH2:1]1[CH2:2][CH:3]=[C:4]2[CH:5]3[CH2:6][CH2:7][CH:8]([CH2:9]3)[CH:10]2[CH2:11]1>>[CH2:1]1[CH2:2][CH2:3][CH:4]2[CH:5]3[CH2:6][CH2:7][CH:8]([CH2:9]3)[CH:10]2[CH2:11]1
C1=C2C3CCC(C3)C2CCC1
C1CCC2C3CCC(C3)C2C1
null
[Pd]
CO
Reduction
Hydrogenation (double to single)
417c0c693fb009b1a7c8e162fdb847862fb77f86e94f4c844a69fd0bd6589a7c
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
C1CCC2C3CCC(C3)C2C1
[C:1]-[C:2]1-[C:3]-[C:4]-[C:5]2-[C:6]-[C:7]-[C:8]-[CH;D2;+0:9]=[C;H0;D3;+0:10]-2-1>>[C:1]-[C:2]1-[C:3]-[C:4]-[C:5]2-[C:6]-[C:7]-[C:8]-[CH2;D2;+0:9]-[CH;D3;+0:10]-2-1
257.6
[{"value": 86.0, "product": "C12CCC(C3CCCCC13)C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 257.6, "product": "C12CCC(C3CCCCC13)C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
45
MINUTE
A 400 ml autoclave was charged with octahydro-1,4-methanonaphthalene (122 g, prepared as described above), methanol (100 ml, Burdick & Jackson, HPLC grade), and palladium on activated carbon (1.5 g containing 10% Pd, Alfa products, powder). The autoclave was closed and sealed, then shaken under 50 psig hydrogen pressur...
10.6084/m9.figshare.5104873.v1
null
null
null
C1=C2C3CCC(C3)C2CCC1
C1CCC2C3CCC(C3)C2C1
C1CCC2C3CCC(C3)C2C1
null
[Pd].CO
null
0.75
C1=C2C3CCC(C3)C2CCC1>[Pd].CO>C1CCC2C3CCC(C3)C2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-3bf2e6545296467986cc10fd18ef8ea4
FC(F)(F)C1CC2CC1C1=CCCCC12>>FC(F)(F)C1CC2CC1C1CCCCC21
[H][H].FC(C1C2C3=CCCCC3C(C1)C2)(F)F.[H][H]>>FC(C1C2C3CCCCC3C(C1)C2)(F)F
[F:1][C:2]([F:3])([F:4])[CH:5]1[CH2:6][CH:7]2[CH2:8][CH:9]1[C:10]1=[CH:11][CH2:12][CH2:13][CH2:14][CH:15]21>>[F:1][C:2]([F:3])([F:4])[CH:5]1[CH2:6][CH:7]2[CH2:8][CH:9]1[CH:10]1[CH2:11][CH2:12][CH2:13][CH2:14][CH:15]21
FC(F)(F)C1CC2CC1C1=CCCCC12
FC(F)(F)C1CC2CC1C1CCCCC21
null
[Pd]
CO
Reduction
Hydrogenation (double to single)
417c0c693fb009b1a7c8e162fdb847862fb77f86e94f4c844a69fd0bd6589a7c
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
C1CCC2C3CCC(C3)C2C1
[C:1]-[C:2]1-[C:3]-[C:4]-[C:5]2-[C:6]-[C:7]-[C:8]-[CH;D2;+0:9]=[C;H0;D3;+0:10]-2-1>>[C:1]-[C:2]1-[C:3]-[C:4]-[C:5]2-[C:6]-[C:7]-[C:8]-[CH2;D2;+0:9]-[CH;D3;+0:10]-2-1
null
[]
null
null
45
MINUTE
A 400 ml autoclave is charged with 177 g of the thus purified octahydro-2-trifluormethyl-1,4-methanonaphthalene, methanol (100 ml, Burdick & Jackson, HPLC grade), and palladium on activated carbon (1.5 g containing 10% Pd, Alfa products, powder). The autoclave is closed and sealed, then it is shaken under 50 psig hydro...
10.6084/m9.figshare.5104873.v1
null
null
null
C1=C2C3CCC(C3)C2CCC1
C1CCC2C3CCC(C3)C2C1
C1CCC2C3CCC(C3)C2C1
null
[Pd].CO
null
0.75
FC(F)(F)C1CC2CC1C1=CCCCC12>[Pd].CO>FC(F)(F)C1CC2CC1C1CCCCC21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-acb43fa5eb1b42d09e33b5d59c24f091
CCN=C=NCCCN(C)C.CSCC[C@H](N)C(=O)O.C[C@H](N)C(=O)OC(C)(C)C.On1nnc2ccccc21>>CSCC[C@H](NC(=O)OCc1ccccc1)C(=O)N[C@@H](C)C(=O)OC(C)(C)C
C(C)(C)(C)OC([C@@H](N)C)=O.Cl.CN(CCCN=C=NCC)C.N[C@@H](CCSC)C(=O)O.C=1C=CC2=C(C1)N=NN2O>>C(C1=CC=CC=C1)OC(=O)N[C@@H](CCSC)C(=O)N[C@@H](C)C(=O)OC(C)(C)C
CN(C)CCCN=[C:7]=N[CH2:10][CH3:15].[CH3:1][S:2][CH2:3][CH2:4][C@H:5]([NH2:6])[C:17]([OH:8])=[O:18].[NH2:19][C@@H:20]([CH3:21])[C:22](=[O:23])[O:24][C:25]([CH3:26])([CH3:27])[CH3:28].n1nn([OH:9])[c:11]2c1[cH:12][cH:13][cH:14][cH:16]2>>[CH3:1][S:2][CH2:3][CH2:4][C@H:5]([NH:6][C:7](=[O:8])[O:9][CH2:10][c:11]1[cH:12][cH:13]...
CCN=C=NCCCN(C)C.CSCC[C@H](N)C(=O)O.C[C@H](N)C(=O)OC(C)(C)C.On1nnc2ccccc21
CSCC[C@H](NC(=O)OCc1ccccc1)C(=O)N[C@@H](C)C(=O)OC(C)(C)C
null
null
CN(C)C=O.C(C)N(CC)CC
C-C Coupling
OtherReaction
6d620ff54c8c76eb4d36b8abf9fffc2c5f76c8423bbc100610eca837575e5129
8df2b912fdba47beb0926dfbece6afe0e78922d84c3228bfea7a541631ccb925
c1ccccc1
C-N(-C)-C-C-C-N=[C;H0;D2;+0:1]=N-[CH2;D2;+0:2]-[CH3;D1;+0:3].[C;D1;H3:4]-[C:5](-[NH2;D1;+0:6])-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13].[C:14]-[C:15](-[NH2;D1;+0:16])-[C;H0;D3;+0:17](=[O;D1;H0:18])-[OH;D1;+0:19].[OH;D1;+0:20]-n1:n:n:c2:[cH;D2;+0:21]:[c:22]:[cH;D2;+0:23]:[cH;D2;+0:24]...
109.3
[{"value": 109.3, "product": "C(C1=CC=CC=C1)OC(=O)N[C@@H](CCSC)C(=O)N[C@@H](C)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Z-Protected L-methionine (10 g) was dissolved in DMF (200 ml) and 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (8.13 g) was added followed by HOBT (5.72 g) and triethylamine (19.7 ml). The mixture was stirred for 1 h then L-alanine tert-butyl ester (7.7 g) was added and stirring continued for 18 h. The...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine.Primary amine.Tertiary amine
Carbamic ester.Ether.Secondary amide
c1ccc2[nH]nnc2c1
c1ccccc1
c1ccccc1
Other
CN(C)C=O.C(C)N(CC)CC
null
1
CCN=C=NCCCN(C)C.CSCC[C@H](N)C(=O)O.C[C@H](N)C(=O)OC(C)(C)C.On1nnc2ccccc21>CN(C)C=O.C(C)N(CC)CC>CSCC[C@H](NC(=O)OCc1ccccc1)C(=O)N[C@@H](C)C(=O)OC(C)(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-4bd47d9e549343d0b97d459c637f4d5c
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O>>C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
C(C1=CC=CC=C1)OC(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O.FC(C(=O)O)(F)F>>C(C1=CC=CC=C1)OC(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O
CC(C)(C)[O:5][C:3]([C@H:2]([CH3:1])[N:6]1[CH2:7][CH2:8][C@H:9]([NH:10][C:11](=[O:12])[O:13][CH2:14][c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[C:21]1=[O:22])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[OH:5])[N:6]1[CH2:7][CH2:8][C@H:9]([NH:10][C:11](=[O:12])[O:13][CH2:14][c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[C:21]1=[O...
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
null
null
C(Cl)Cl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C(N[C@H]1CCNC1=O)OCc1ccccc1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
100.1
[{"value": 100.1, "product": "C(C1=CC=CC=C1)OC(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
tert-Butyl (2S)-2-((3S)-3-{[(benzyloxy)carbonyl]amino}-2-oxopyrrolidin-1-yl)propanoate (0.5 g) was dissolved in DCM (7 ml), and trifluoroacetic acid (4.7 ml) was added. The mixture was stirred at room temperature for 1.5 h and then concentrated under reduced pressure to give the title compound (0.423 g) as a colourless...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
C1CC[NH]C1.c1ccccc1
Other
C(Cl)Cl
null
1.5
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O>C(Cl)Cl>C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f3a66bbcb3f94cea9e8f39b795a686a8
C1CCNCC1.C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O>>C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
N1CCCCC1.C(C1=CC=CC=C1)OC(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O>>C[C@@H](C(N1CCCCC1)=O)N1C([C@H](CC1)NC(OCC1=CC=CC=C1)=O)=O
[NH:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1.O[C:3]([C@H:2]([CH3:1])[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][C:16](=[O:17])[O:18][CH2:19][c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[C:26]1=[O:27])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][C:16...
C1CCNCC1.C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(N[C@H]1CCN(CC(=O)N2CCCCC2)C1=O)OCc1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
68.8
[{"value": 68.8, "product": "C[C@@H](C(N1CCCCC1)=O)N1C([C@H](CC1)NC(OCC1=CC=CC=C1)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
To a solution of (2S)-2-((3S)-3-{[(benzyloxy)carbonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid (3.1 g) in DCM (30 ml) were added 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (4.6 g), HOBT (3.2 g) and triethylamine (2.5 ml) and the mixture was stirred at room temperature for 5 min. Piperidine (2.9 ml)...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]C1.c1ccccc1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
0.083333
C1CCNCC1.C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O>C(Cl)Cl.C(C)N(CC)CC>C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0e293147cef644178865951b6e7d89d5
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O.FC(C(=O)O)(F)F>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O
CC(C)(C)[O:5][C:3]([C@H:2]([CH3:1])[N:6]1[CH2:7][CH2:8][C@H:9]([NH:10][S:11](=[O:12])(=[O:13])[c:14]2[cH:15][cH:16][c:17]3[cH:18][c:19]([Cl:20])[cH:21][cH:22][c:23]3[cH:24]2)[C:25]1=[O:26])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[OH:5])[N:6]1[CH2:7][CH2:8][C@H:9]([NH:10][S:11](=[O:12])(=[O:13])[c:14]2[cH:15][cH:16][c:17]3...
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C1NCC[C@@H]1NS(=O)(=O)c1ccc2ccccc2c1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
99.4
[{"value": 99.4, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2.5
HOUR
tert-Butyl (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoate (0.643 g) was dissolved in DCM (19 ml), and trifluoroacetic acid (19 ml) was added. The mixture was stirred at room temperature for 2.5 h and then concentrated under reduced pressure. Anhydrous DCM (4 ml) was added and the ...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
C1CC[NH]C1.c1ccc2ccccc2c1
Other
C(Cl)Cl
null
2.5
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl>C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ccc78d613f444ad6b89c8dad33303608
CCOC(=O)C(CCBr)N=[N+]=[N-].C[C@@H](N)C(=O)OC(C)(C)C>>C[C@H](C(=O)OC(C)(C)C)N1CCC(N=[N+]=[N-])C1=O
C(C)(C)(C)OC([C@H](N)C)=O.C(C)(C)N(C(C)C)CC.N(=[N+]=[N-])C(C(=O)OCC)CCBr.[I-].[Na+]>>N(=[N+]=[N-])C1C(N(CC1)[C@@H](C(=O)OC(C)(C)C)C)=O
CCO[C:17]([CH:13]([CH2:12][CH2:11]Br)[N:14]=[N+:15]=[N-:16])=[O:18].[CH3:1][C@H:2]([C:3](=[O:4])[O:5][C:6]([CH3:7])([CH3:8])[CH3:9])[NH2:10]>>[CH3:1][C@H:2]([C:3](=[O:4])[O:5][C:6]([CH3:7])([CH3:8])[CH3:9])[N:10]1[CH2:11][CH2:12][CH:13]([N:14]=[N+:15]=[N-:16])[C:17]1=[O:18]
CCOC(=O)C(CCBr)N=[N+]=[N-].C[C@@H](N)C(=O)OC(C)(C)C
C[C@H](C(=O)OC(C)(C)C)N1CCC(N=[N+]=[N-])C1=O
null
null
C(C)#N
Acylation
OtherReaction
819e3f2b7868adc1c1b9de9bb195abc43156b28c3cf194597f96cec7ac859f91
0eb062b0407fca631aebf8550994dc507c145d19ea7e1f961f104337865aa8f4
O=C1CCCN1
Br-[CH2;D2;+0:1]-[C:2]-[C:3](-[#7:4]=[#7;+:5]=[N;-;D1;H0:6])-[C;H0;D3;+0:7](=[O;D1;H0:8])-O-C-C.[C;D1;H3:9]-[C:10](-[NH2;D1;+0:11])-[C:12](=[O;D1;H0:13])-[#8:14]-[C:15](-[C;D1;H3:16])(-[C;D1;H3:17])-[C;D1;H3:18]>>[C;D1;H3:9]-[C:10](-[C:12](=[O;D1;H0:13])-[#8:14]-[C:15](-[C;D1;H3:16])(-[C;D1;H3:17])-[C;D1;H3:18])-[N;H0;...
18.9
[{"value": 18.9, "product": "N(=[N+]=[N-])C1C(N(CC1)[C@@H](C(=O)OC(C)(C)C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
To a solution of D-alanine tert-butylester (1.28 g) and N,N-diisopropylethyamine (1.22 ml) in acetonitrile (15 ml), was added a solution of ethyl 2-azido-4-bromobutanoate (1 g) and sodium iodide (0.02 g) in acetonitrile (5 ml). The mixture was heated at 60° C. for 60 h and then concentrated under pressure to give a bro...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Primary amine
Tertiary amide
null
C1CC[NH]C1
C1CC[NH]C1
HBr
C(C)#N
60
null
CCOC(=O)C(CCBr)N=[N+]=[N-].C[C@@H](N)C(=O)OC(C)(C)C>C(C)#N>C[C@H](C(=O)OC(C)(C)C)N1CCC(N=[N+]=[N-])C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e844e5c076c84bcdb7aca1ff5d4592b9
CCOC(=O)C(CCI)N=[N+]=[N-].C[C@H](N)C(=O)OC(C)(C)C>>C[C@@H](C(=O)OC(C)(C)C)N1CCC(N=[N+]=[N-])C1=O
N(=[N+]=[N-])C(C(=O)OCC)CCI.C(C)(C)(C)OC([C@@H](N)C)=O>>N(=[N+]=[N-])C1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O
CCO[C:17]([CH:13]([CH2:12][CH2:11]I)[N:14]=[N+:15]=[N-:16])=[O:18].[CH3:1][C@@H:2]([C:3](=[O:4])[O:5][C:6]([CH3:7])([CH3:8])[CH3:9])[NH2:10]>>[CH3:1][C@@H:2]([C:3](=[O:4])[O:5][C:6]([CH3:7])([CH3:8])[CH3:9])[N:10]1[CH2:11][CH2:12][CH:13]([N:14]=[N+:15]=[N-:16])[C:17]1=[O:18]
CCOC(=O)C(CCI)N=[N+]=[N-].C[C@H](N)C(=O)OC(C)(C)C
C[C@@H](C(=O)OC(C)(C)C)N1CCC(N=[N+]=[N-])C1=O
null
null
null
Acylation
OtherReaction
819e3f2b7868adc1c1b9de9bb195abc43156b28c3cf194597f96cec7ac859f91
0eb062b0407fca631aebf8550994dc507c145d19ea7e1f961f104337865aa8f4
O=C1CCCN1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[#7:4]=[#7;+:5]=[N;-;D1;H0:6])-[C:7]-[CH2;D2;+0:8]-I.[C;D1;H3:9]-[C:10](-[NH2;D1;+0:11])-[C:12](=[O;D1;H0:13])-[#8:14]-[C:15](-[C;D1;H3:16])(-[C;D1;H3:17])-[C;D1;H3:18]>>[C;D1;H3:9]-[C:10](-[C:12](=[O;D1;H0:13])-[#8:14]-[C:15](-[C;D1;H3:16])(-[C;D1;H3:17])-[C;D1;H3:18])-[N;H0;D...
null
[]
null
null
null
null
Using ethyl 2-azido-4-iodobutanoate and L-alanine tert-butyl ester, and the procedure described for Intermediate 33, the title compound was prepared as a mixture of two diastereoisomers. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Primary amine
Tertiary amide
null
C1CC[NH]C1
C1CC[NH]C1
HI
null
null
null
CCOC(=O)C(CCI)N=[N+]=[N-].C[C@H](N)C(=O)OC(C)(C)C>>C[C@@H](C(=O)OC(C)(C)C)N1CCC(N=[N+]=[N-])C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2e791d8ad3284a08bf77aa27bde8bef4
CCC(=O)CBr.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)OC(C)(C)C)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].CO.BrCC(CC)=O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O)CC(CC)=O
Br[CH2:5][C:3]([CH2:2][CH3:1])=[O:4].[NH:6]([C@H:7]1[CH2:8][CH2:9][N:10]([C@@H:11]([CH3:12])[C:13](=[O:14])[O:15][C:16]([CH3:17])([CH3:18])[CH3:19])[C:20]1=[O:21])[S:22](=[O:23])(=[O:24])[c:25]1[cH:26][cH:27][c:28]2[cH:29][c:30]([Cl:31])[cH:32][cH:33][c:34]2[cH:35]1>>[CH3:1][CH2:2][C:3](=[O:4])[CH2:5][N:6]([C@H:7]1[CH2...
CCC(=O)CBr.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)OC(C)(C)C)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
3e42d5bcca7444f83191a46ba1444dcefee0e07920df674140f242a2d256ea8d
73633c824b1cf45c7f3d2af586c5778a55c8407a45442da8b8f942e0aebaa600
O=C1NCC[C@@H]1NS(=O)(=O)c1ccc2ccccc2c1
Br-[CH2;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4].[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[#7:9]1-[C:10]-[C:11]-[C:12](-[NH;D2;+0:13]-[#16:14](=[O;D1;H0:15])(=[O;D1;H0:16])-[c:17])-[C:18]-1=[O;D1;H0:19]>>[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[#7:9]1-[C:10]-[C:11]-[C:12](-[N;H0;D3;+0:13](-[CH2;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4])-[#16:14](...
null
[]
null
null
72
HOUR
A solution of tert-butyl (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoate (0.07 g) in THF (2 ml) was cooled to −78° C. under nitrogen, and treated with lithium bis(trimethylsilyl) amide (1.0M solution in THF; 0.186 ml), followed by 1-bromo-2-butanone (0.08 ml). The resultant solutio...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Primary halide
Ketone.Tertiary amine
null
null
C1CC[NH]C1.c1ccc2ccccc2c1
HBr
C1CCOC1
null
72
CCC(=O)CBr.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C1CCOC1>CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)OC(C)(C)C)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-43b9e540a68748f4a883cdf2e800a1a2
CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)OC(C)(C)C)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1>>CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O)CC(CC)=O.FC(C(=O)O)(F)F>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)CC(CC)=O
CC(C)(C)[O:15][C:13]([C@@H:11]([N:10]1[CH2:9][CH2:8][C@H:7]([N:6]([CH2:5][C:3]([CH2:2][CH3:1])=[O:4])[S:18](=[O:19])(=[O:20])[c:21]2[cH:22][cH:23][c:24]3[cH:25][c:26]([Cl:27])[cH:28][cH:29][c:30]3[cH:31]2)[C:16]1=[O:17])[CH3:12])=[O:14]>>[CH3:1][CH2:2][C:3](=[O:4])[CH2:5][N:6]([C@H:7]1[CH2:8][CH2:9][N:10]([C@@H:11]([CH...
CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)OC(C)(C)C)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
null
null
C(Cl)Cl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C1NCC[C@@H]1NS(=O)(=O)c1ccc2ccccc2c1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
100.8
[{"value": 100.8, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)CC(CC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
tert-Butyl (2S)-2-{(3S)-3-[[(6-chloro-2-naphthyl)sulfonyl](2-oxobutyl)amino]-2-oxopyrrolidin-1-yl}propanoate (0.07 g) was dissolved in DCM (2 ml), and trifluoroacetic acid (2 ml) was added. The mixture was stirred at room temperature for 1.5 h and then partitioned between water and DCM. The organic layer was separated,...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
C1CC[NH]C1.c1ccc2ccccc2c1
Other
C(Cl)Cl
null
1.5
CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)OC(C)(C)C)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1>C(Cl)Cl>CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-45ff7524fc5340a38581577b0a458e5b
COS(=O)(=O)c1ccc(C)cc1.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[Si](C)(C)[N-][Si](C)(C)C.[Li+].ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O.S(=O)(=O)(OC)C1=CC=C(C)C=C1>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O)C
Cc1ccc(S(=O)(=O)O[CH3:15])cc1.[CH3:1][C@@H:2]([C:3](=[O:4])[O:5][C:6]([CH3:7])([CH3:8])[CH3:9])[N:10]1[CH2:11][CH2:12][C@H:13]([NH:14][S:16](=[O:17])(=[O:18])[c:19]2[cH:20][cH:21][c:22]3[cH:23][c:24]([Cl:25])[cH:26][cH:27][c:28]3[cH:29]2)[C:30]1=[O:31]>>[CH3:1][C@@H:2]([C:3](=[O:4])[O:5][C:6]([CH3:7])([CH3:8])[CH3:9])[...
COS(=O)(=O)c1ccc(C)cc1.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
N-methylation
1e744aaec43d4cae0f62ffc033588ec8c1162aa614027d68ba7b84bcec4663fb
67298390bbcc11d70c41987c4ac06c2607123196b8179aab003bf84a312a9881
O=C1NCC[C@@H]1NS(=O)(=O)c1ccc2ccccc2c1
C-c1:c:c:c(-S(=O)(=O)-O-[CH3;D1;+0:1]):c:c:1.[#8:2]-[C:3](=[O;D1;H0:4])-[C:5]-[#7:6]1-[C:7]-[C:8]-[C:9](-[NH;D2;+0:10]-[#16:11](=[O;D1;H0:12])(=[O;D1;H0:13])-[c:14])-[C:15]-1=[O;D1;H0:16]>>[#8:2]-[C:3](=[O;D1;H0:4])-[C:5]-[#7:6]1-[C:7]-[C:8]-[C:9](-[N;H0;D3;+0:10](-[CH3;D1;+0:1])-[#16:11](=[O;D1;H0:12])(=[O;D1;H0:13])-...
null
[]
null
null
16
HOUR
A solution of tert-butyl (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoate (0.1 g) in THF (5 ml) was cooled to −78° C. under nitrogen, and treated with lithium bis(trimethylsilyl) amide (1.0M solution in THF; 0.23 ml), followed by methyl tosylate (0.206 g). The resultant solution was...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Tosylate
Tertiary amine
c1ccccc1
null
C1CC[NH]C1.c1ccc2ccccc2c1
TsOH.HO-
C1CCOC1
null
16
COS(=O)(=O)c1ccc(C)cc1.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C1CCOC1>C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-afe77ad6405b44e491a4a99117a535e9
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)O)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O)C.FC(C(=O)O)(F)F>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)C
CC(C)(C)[O:5][C:3]([C@H:2]([CH3:1])[N:6]1[CH2:7][CH2:8][C@H:9]([N:10]([CH3:11])[S:12](=[O:13])(=[O:14])[c:15]2[cH:16][cH:17][c:18]3[cH:19][c:20]([Cl:21])[cH:22][cH:23][c:24]3[cH:25]2)[C:26]1=[O:27])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[OH:5])[N:6]1[CH2:7][CH2:8][C@H:9]([N:10]([CH3:11])[S:12](=[O:13])(=[O:14])[c:15]2[cH...
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)O)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C1NCC[C@@H]1NS(=O)(=O)c1ccc2ccccc2c1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
102.3
[{"value": 102.3, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
tert-Butyl (2S)-2-{(3S)-3-[[(6-chloro-2-naphthyl)sulfonyl](methyl)amino]-2-oxopyrrolidin-1-yl}propanoate (0.1 g) was dissolved in DCM (2 ml), and trifluoroacetic acid (2 ml) was added. The mixture was stirred at room temperature for 1.5 h and then partitioned between water and DCM. The organic layer was separated, drie...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
C1CC[NH]C1.c1ccc2ccccc2c1
Other
C(Cl)Cl
null
1.5
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl>C[C@@H](C(=O)O)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e1e715609e01411ba597fa73de2bd029
CC(C)(C)OC(=O)N1CCCC(N)C1.CN(C)C=O.On1nnc2ccccc21>>CC(C)(C)OC(=O)N1CCCC(NC(=O)c2ccccc2)C1
Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O.C(C)N(CC)CC.NC1CN(CCC1)C(=O)OC(C)(C)C.CN(C)C=O.CN(C)C=O>>C(C1=CC=CC=C1)(=O)NC1CN(CCC1)C(=O)OC(C)(C)C
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][CH2:11][CH:12]([NH2:13])[CH2:22]1.CN(C)[CH:14]=[O:15].On1nn[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]12>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][CH2:11][CH:12]([NH:13][C:14](=[O:15])[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:...
CC(C)(C)OC(=O)N1CCCC(N)C1.CN(C)C=O.On1nnc2ccccc21
CC(C)(C)OC(=O)N1CCCC(NC(=O)c2ccccc2)C1
null
null
null
Acylation
OtherReaction
eb7fb864e129846ce9d20c39f662befcabafa5211a5b135db173c20539cde95a
d0f759e36e4db8bedafa647876c8fc5b29c30b781d9a211c65bebd3576e0d0b4
O=C(NC1CCCNC1)c1ccccc1
C-N(-C)-[CH;D2;+0:1]=[O;D1;H0:2].O-n1:n:n:[c;H0;D3;+0:3]2:[c:4]:[c:5]:[c:6]:[c:7]:[c;H0;D3;+0:8]:2:1.[#7:9]-[C:10]-[C:11](-[NH2;D1;+0:12])-[C:13]>>[#7:9]-[C:10]-[C:11](-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c;H0;D3;+0:3]1:[c:4]:[c:5]:[c:6]:[c:7]:[cH;D2;+0:8]:1)-[C:13]
null
[]
null
null
1
HOUR
A solution of benzoic add (0.123 g) in DMF (5 ml) was treated with 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.231 g), HOBT (0.163 g) and triethylamine (0.56 ml) and stirred at room temperature for 1 h. A solution of 3-amino-1-N-Boc-piperidine (0.3 g) in DMF (1 ml) was then added and stirring conti...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Primary amine
Secondary amide
c1ccc2[nH]nnc2c1
c1ccccc1
C1CC[NH]CC1.c1ccccc1
HO-
null
null
1
CC(C)(C)OC(=O)N1CCCC(N)C1.CN(C)C=O.On1nnc2ccccc21>>CC(C)(C)OC(=O)N1CCCC(NC(=O)c2ccccc2)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c3bcead969a34b93b1d3e7c8a3b42396
CC(C)(C)OC(=O)N1CCCC(NC(=O)c2ccccc2)C1>>O=C(NC1CCCNC1)c1ccccc1
N.C(C1=CC=CC=C1)(=O)NC1CN(CCC1)C(=O)OC(C)(C)C.FC(C(=O)O)(F)F>>N1CC(CCC1)NC(C1=CC=CC=C1)=O
CC(C)(C)OC(=O)[N:8]1[CH2:7][CH2:6][CH2:5][CH:4]([NH:3][C:2](=[O:1])[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[CH2:9]1>>[O:1]=[C:2]([NH:3][CH:4]1[CH2:5][CH2:6][CH2:7][NH:8][CH2:9]1)[c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1
CC(C)(C)OC(=O)N1CCCC(NC(=O)c2ccccc2)C1
O=C(NC1CCCNC1)c1ccccc1
null
null
C(Cl)Cl
Reduction
Boc amine deprotection
bf3cd5dc3e17e694d8665c89f5d7e08e8763b18436a633eb66e9bf530b8b0316
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=C(NC1CCCNC1)c1ccccc1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:5]-[C:4]-[NH;D2;+0:1]-[C:2]-[C:3]
105.6
[{"value": 105.6, "product": "N1CC(CCC1)NC(C1=CC=CC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
6
HOUR
A solution of tert-butyl 3-(benzoylamino)piperidine-1-carboxylate (0.120 g) in DCM (5 ml) was treated with trifluoroacetic acid (5 ml) and stirred at room temperature for 6 h. The mixture was concentrated under reduced pressure to give a yellow oil which following neutralisation with aqueous ammonia solution, was purif...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1CC[NH]CC1
C1CCNCC1
C1CCNCC1.c1ccccc1
HO-
C(Cl)Cl
null
6
CC(C)(C)OC(=O)N1CCCC(NC(=O)c2ccccc2)C1>C(Cl)Cl>O=C(NC1CCCNC1)c1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cef424cf0bb042ad81892277b4dd1e2e
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(Cc2nccs2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)O)N1CC[C@H](N(Cc2nccs2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O)CC=1SC=CN1.FC(C(=O)O)(F)F>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)CC=1SC=CN1
CC(C)(C)[O:5][C:3]([C@H:2]([CH3:1])[N:6]1[CH2:7][CH2:8][C@H:9]([N:10]([CH2:11][c:12]2[n:13][cH:14][cH:15][s:16]2)[S:17](=[O:18])(=[O:19])[c:20]2[cH:21][cH:22][c:23]3[cH:24][c:25]([Cl:26])[cH:27][cH:28][c:29]3[cH:30]2)[C:31]1=[O:32])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[OH:5])[N:6]1[CH2:7][CH2:8][C@H:9]([N:10]([CH2:11][...
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(Cc2nccs2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)O)N1CC[C@H](N(Cc2nccs2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C1NCC[C@@H]1N(Cc1nccs1)S(=O)(=O)c1ccc2ccccc2c1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
70.5
[{"value": 70.5, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)CC=1SC=CN1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of tert-butyl (2S)-2-{(3S)-3-[[(6-chloro-2-naphthyl)sulfonyl](1,3-thiazol-2-ylmethyl)amino]-2-oxopyrrolidin-1-yl}propanoate (0.03 g) in DCM (1 ml) was treated with trifluoroacetic acid (1 ml) and stirred at room temperature for 1 h. The solution was then concentrated under reduced pressure to give the title ...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
C1CC[NH]C1.c1cscn1.c1ccc2ccccc2c1
Other
C(Cl)Cl
null
1
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(Cc2nccs2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl>C[C@@H](C(=O)O)N1CC[C@H](N(Cc2nccs2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0d66f2913bdf4cf684ad6583f5f27c4b
CCOC(C)=O.N[C@H](CCC(=O)O)C(=O)O.O=C(Cl)OCc1ccccc1>>COC(=O)CC[C@@H](NC(=O)OCc1ccccc1)C(=O)OC
S(=O)(Cl)Cl.N[C@H](CCC(=O)O)C(=O)O.C(O)([O-])=O.[K+].ClC(=O)OCC1=CC=CC=C1.C(C)(=O)OCC>>C(C1=CC=CC=C1)OC(=O)N[C@@H](C(=O)OC)CCC(=O)OC
CC(=O)O[CH2:1][CH3:22].[OH:2][C:3](=[O:4])[CH2:5][CH2:6][C@@H:7]([NH2:8])[C:19](=[O:20])[OH:21].Cl[C:9](=[O:10])[O:11][CH2:12][c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][C@@H:7]([NH:8][C:9](=[O:10])[O:11][CH2:12][c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[C:19](=[O:20])[O:21][C...
CCOC(C)=O.N[C@H](CCC(=O)O)C(=O)O.O=C(Cl)OCc1ccccc1
COC(=O)CC[C@@H](NC(=O)OCc1ccccc1)C(=O)OC
null
null
CO.O
Protection
OtherReaction
0f9327ec2e19bacfcf1a90db37669b7bebdc518f6ed740ed1723aab5a8fa05e0
388ff98aac8b3e1f916bc2d53b085f5ef557692d32ded4c7247c38bc8fd0411b
c1ccccc1
C-C(=O)-O-[CH2;D2;+0:1]-[CH3;D1;+0:2].Cl-[C;H0;D3;+0:3](=[O;D1;H0:4])-[#8:5]-[C:6].[NH2;D1;+0:7]-[C:8](-[C:9]-[C:10]-[C:11](=[O;D1;H0:12])-[OH;D1;+0:13])-[C:14](=[O;D1;H0:15])-[OH;D1;+0:16]>>[C:6]-[#8:5]-[C;H0;D3;+0:3](=[O;D1;H0:4])-[NH;D2;+0:7]-[C:8](-[C:9]-[C:10]-[C:11](=[O;D1;H0:12])-[O;H0;D2;+0:13]-[CH3;D1;+0:1])-[...
null
[]
null
null
5
HOUR
Thionyl chloride (30 ml) was added to a cooled solution of D-glutamic acid (33.2 g) in methanol (250 ml) and the mixture subsequently heated under reflux for 16 h. On cooling, the mixture was concentrated under reduced pressure and the residue azeotroped with toluene to give a white solid. This was stirred with ethyl a...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Carboxylic acid.Carboxylic acid.Ester.Ether.Primary amine
Carbamic ester.Ester.Ester
null
null
c1ccccc1
HCl
CO.O
null
5
CCOC(C)=O.N[C@H](CCC(=O)O)C(=O)O.O=C(Cl)OCc1ccccc1>CO.O>COC(=O)CC[C@@H](NC(=O)OCc1ccccc1)C(=O)OC
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0716b8127315465ca5bb1dda1907bd78
O=C([O-])CCC(NC(=O)OCc1ccccc1)C(=O)[O-]>>O=C(N[C@@H](CO)CCCO)OCc1ccccc1
C(C1=CC=CC=C1)OC(=O)NC(C(=O)[O-])CCC(=O)[O-].[BH4-].[Li+]>>OCCC[C@H](CO)NC(OCC1=CC=CC=C1)=O
O=[C:9]([CH2:8][CH2:7][CH:4]([NH:3][C:2](=[O:1])[O:11][CH2:12][c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[C:5]([O-])=[O:6])[O-:10]>>[O:1]=[C:2]([NH:3][C@@H:4]([CH2:5][OH:6])[CH2:7][CH2:8][CH2:9][OH:10])[O:11][CH2:12][c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1
O=C([O-])CCC(NC(=O)OCc1ccccc1)C(=O)[O-]
O=C(N[C@@H](CO)CCCO)OCc1ccccc1
null
null
C1CCOC1.O.[Cl-].[Na+].O
Reduction
OtherReaction
c387793b491dae4262adcc791c73ba45fdff80869e7dcc0bd64fdd10818b0c85
44678ab29171bc4545e94bd412bac5255e3f987f15856a5641a6790aa4279e90
c1ccccc1
O=[C;H0;D3;+0:1](-[O-;H0;D1:2])-[C:3]-[C:4]-[CH;D3;+0:5](-[#7:6]-[C:7](-[#8:8])=[O;D1;H0:9])-[C;H0;D3;+0:10](-[O-])=[O;H0;D1;+0:11]>>[#8:8]-[C:7](=[O;D1;H0:9])-[#7:6]-[C@H;D3;+0:5](-[C:4]-[C:3]-[CH2;D2;+0:1]-[OH;D1;+0:2])-[CH2;D2;+0:10]-[OH;D1;+0:11]
81.2
[{"value": 81.2, "product": "OCCC[C@H](CO)NC(OCC1=CC=CC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
DAY
A solution of dimethyl (2R)-2-{[((benzyloxy)carbonyl]amino}pentanedioate (22.4 g) in dry THF (74 ml) was added dropwise over 1 h to a stirred mixture of lithium borohydride (4.5 g) in THF (200 ml) at room temperature, under nitrogen. Stirring at room temperature was continued for 3 days. The reaction mixture was dilute...
10.6084/m9.figshare.5104873.v1
null
null
Primary alcohol.Primary alcohol
null
null
c1ccccc1
Other
C1CCOC1.O.[Cl-].[Na+].O
null
72
O=C([O-])CCC(NC(=O)OCc1ccccc1)C(=O)[O-]>C1CCOC1.O.[Cl-].[Na+].O>O=C(N[C@@H](CO)CCCO)OCc1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f0d992a9a8f14e6b9e4f8b4467f7e8d6
CS(=O)(=O)Cl.O=C(N[C@@H](CO)CCCO)OCc1ccccc1.O=C([O-])O>>CS(=O)(=O)OCCC[C@H](COS(C)(=O)=O)NC(=O)OCc1ccccc1
OCCC[C@H](CO)NC(OCC1=CC=CC=C1)=O.C(C)N(CC)CC.C([O-])(O)=O.[Na+].CS(=O)(=O)Cl>>CS(=O)(=O)OC[C@@H](CCCOS(=O)(=O)C)NC(=O)OCC1=CC=CC=C1
Cl[S:2]([CH3:1])(=[O:3])=[O:4].[OH:5][CH2:6][CH2:7][CH2:8][C@H:9]([CH2:10][OH:11])[NH:16][C:17](=[O:18])[O:19][CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1.[O-][C:13]([OH:14])=[O:15]>>[CH3:1][S:2](=[O:3])(=[O:4])[O:5][CH2:6][CH2:7][CH2:8][C@H:9]([CH2:10][O:11][S:12]([CH3:13])(=[O:14])=[O:15])[NH:16][C:17](=[O:18]...
CS(=O)(=O)Cl.O=C(N[C@@H](CO)CCCO)OCc1ccccc1.O=C([O-])O
CS(=O)(=O)OCCC[C@H](COS(C)(=O)=O)NC(=O)OCc1ccccc1
null
null
C(Cl)Cl
Oxidation
OtherReaction
9d4d934bcbeb2d0c12301956d4f6b3081ef6785a160067cffd9435031b1840c5
7b7a07a5549da95bb7017f46e245561bcc3563036e9e87ce717294d15e35b2cc
c1ccccc1
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].[C:5]-[C:6]-[OH;D1;+0:7].[C:8]-[C:9]-[OH;D1;+0:10].[O-]-[C;H0;D3;+0:11](=[O;H0;D1;+0:12])-[OH;D1;+0:13]>>[C:8]-[C:9]-[O;H0;D2;+0:10]-[#16:14](-[CH3;D1;+0:11])(=[O;H0;D1;+0:13])=[O;H0;D1;+0:12].[C:5]-[C:6]-[O;H0;D2;+0:7]-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])...
null
[]
null
null
10
MINUTE
A solution of benzyl (1R)-4-hydroxy-1-(hydroxymethyl)butylcarbamate (1.5 g) in DCM (60 ml) was treated with triethylamine (3.3 ml) and stirred at room temperature for 10 min. Methanesulphonyl chloride (1.34 ml) was then added dropwise and the resultant mixture stirred at 0° C. for 75 min. Sodium bicarbonate solution wa...
10.6084/m9.figshare.5104873.v1
null
Carbonic Acid.Primary alcohol.Primary alcohol.Sulfonyl halide
Mesylate.Mesylate
null
null
c1ccccc1
Other
C(Cl)Cl
null
0.166667
CS(=O)(=O)Cl.O=C(N[C@@H](CO)CCCO)OCc1ccccc1.O=C([O-])O>C(Cl)Cl>CS(=O)(=O)OCCC[C@H](COS(C)(=O)=O)NC(=O)OCc1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d7f656c0db30491b9bd260da1a6f071a
CS(=O)(=O)OCCC[C@H](COS(C)(=O)=O)NC(=O)OCc1ccccc1.N>>O=C(N[C@@H]1CCCNC1)OCc1ccccc1
N.CS(=O)(=O)OC[C@@H](CCCOS(=O)(=O)C)NC(=O)OCC1=CC=CC=C1>>N1C[C@@H](CCC1)NC(OCC1=CC=CC=C1)=O
CS(=O)(=O)O[CH2:7][CH2:6][CH2:5][C@@H:4]([NH:3][C:2](=[O:1])[O:10][CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)[CH2:9]OS(C)(=O)=O.[NH3:8]>>[O:1]=[C:2]([NH:3][C@@H:4]1[CH2:5][CH2:6][CH2:7][NH:8][CH2:9]1)[O:10][CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1
CS(=O)(=O)OCCC[C@H](COS(C)(=O)=O)NC(=O)OCc1ccccc1.N
O=C(N[C@@H]1CCCNC1)OCc1ccccc1
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
0e1938088af445a4e2d42a1889b47fa5020ec9c67bd21c065d2bda8123847234
02cf7cdaee4e88b5c5cc4f98c273950b8431482c5462982230888681be2f5507
O=C(N[C@@H]1CCCNC1)OCc1ccccc1
C-S(=O)(=O)-O-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4](-[#7:5]-[C:6]=[O;D1;H0:7])-[CH2;D2;+0:8]-O-S(-C)(=O)=O.[NH3;D0;+0:9]>>[O;D1;H0:7]=[C:6]-[#7:5]-[C:4]1-[C:3]-[C:2]-[CH2;D2;+0:1]-[NH;D2;+0:9]-[CH2;D2;+0:8]-1
null
[]
null
null
46
HOUR
Liquid ammonia (ca. 30 ml) was added to a solution of (2R)-2-{[(benzyloxy)carbonyl]amino}-5-[(methylsulfonyl)oxy]pentyl methanesulfonate (1 g) in THF (15 ml) at −78° C. in a bomb reaction vessel and then the resultant mixture was allowed to reach room temperature. After 46 h, the solution was concentrated under reduced...
10.6084/m9.figshare.5104873.v1
null
Mesylate.Mesylate
Secondary amine
null
C1CCNCC1
C1CCNCC1.c1ccccc1
MsOH.HO-
C1CCOC1
null
46
CS(=O)(=O)OCCC[C@H](COS(C)(=O)=O)NC(=O)OCc1ccccc1.N>C1CCOC1>O=C(N[C@@H]1CCCNC1)OCc1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6537f41a60ef4c66bb92600fe8b85d0b
C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(N[C@H]1CCCNC1)OCc1ccccc1>>C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O.N1C[C@H](CCC1)NC(OCC1=CC=CC=C1)=O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@H](CCC1)NC(OCC1=CC=CC=C1)=O)C)=O
O[C:3]([C@H:2]([CH3:1])[N:22]1[CH2:23][CH2:24][C@H:25]([NH:26][S:27](=[O:28])(=[O:29])[c:30]2[cH:31][cH:32][c:33]3[cH:34][c:35]([Cl:36])[cH:37][cH:38][c:39]3[cH:40]2)[C:41]1=[O:42])=[O:4].[NH:5]1[CH2:6][CH2:7][CH2:8][C@H:9]([NH:10][C:11](=[O:12])[O:13][CH2:14][c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[CH2:21]1>>[CH3:...
C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(N[C@H]1CCCNC1)OCc1ccccc1
C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(N[C@H]1CCCN(C(=O)CN2CC[C@H](NS(=O)(=O)c3ccc4ccccc4c3)C2=O)C1)OCc1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
42.5
[{"value": 42.5, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@H](CCC1)NC(OCC1=CC=CC=C1)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid (0.408 g) in DCM (21 ml) was treated with 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.394 g), HOBT (0.278 g) and triethylamine (0.286 ml) and stirred at room temperature for 1 h. A solution of be...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccccc1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
1
C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(N[C@H]1CCCNC1)OCc1ccccc1>C(Cl)Cl.C(C)N(CC)CC>C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-da9cd41501664b12815cadc2aacf7368
C1COCCN1.C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
N1CCOCC1.C(C1=CC=CC=C1)OC(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.F[B-](F)(F)F.N1(N=NC2=C1C=CC=C2)OC(=[N+](C)C)N(C)C.[Cl-].[NH4+].C(C)(C)N(C(C)C)CC>>C[C@@H](C(=O)N1CCOCC1)N1C([C@H](CC1)NC(OCC1=CC=CC=C1)=O)=O
[NH:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1.O[C:3]([C@H:2]([CH3:1])[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][C:16](=[O:17])[O:18][CH2:19][c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[C:26]1=[O:27])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][C:16](=[...
C1COCCN1.C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
null
null
CN(C)C=O
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
2ef483949e7ba3e5f888cf14cdce25fa611f75be09fdf1854a473be519821b59
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(N[C@H]1CCN(CC(=O)N2CCOCC2)C1=O)OCc1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[#8:8]1-[C:9]-[C:10]-[NH;D2;+0:11]-[C:12]-[C:13]-1>>[C;D1;H3:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:11]1-[C:12]-[C:13]-[#8:8]-[C:9]-[C:10]-1
null
[]
null
null
2.5
HOUR
(2S)-2-((3S)-3-{[(Benzyloxy)carbonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid (84.5 g) was dissolved in DMF (2I) and O-(benzotriazol-1-yl)-N,N,N′,N′-tetramethyluronium tetrafluoroborate (161 g) was added, followed by N,N-diisopropylethylamine (92 ml) and morpholine (46 ml). The mixture was stirred under nitrogen for ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1.C1CC[NH]C1.c1ccccc1
HO-
CN(C)C=O
null
2.5
C1COCCN1.C[C@@H](C(=O)O)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O>CN(C)C=O>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c54c7d41fb7c4d1fb6d25147d00d8589
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N)C1=O
C[C@@H](C(=O)N1CCOCC1)N1C([C@H](CC1)NC(OCC1=CC=CC=C1)=O)=O>>N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O
O=C(OCc1ccccc1)[NH:15][C@H:14]1[CH2:13][CH2:12][N:11]([C@@H:2]([CH3:1])[C:3](=[O:4])[N:5]2[CH2:6][CH2:7][O:8][CH2:9][CH2:10]2)[C:16]1=[O:17]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][CH2:13][C@H:14]([NH2:15])[C:16]1=[O:17]
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N)C1=O
null
[Pd]
C(C)O
Reduction
Hydrogenolysis of amides/imides/carbamates
087b6600ba91d3df931fe6979f2445c192cbfd59e04fd2d8a10f7c7573ac669f
4e549866ec1acadec4c84aaf8495992a28ec78d8ea5ef1b9f44dd843b0dcb7d4
O=C(CN1CCCC1=O)N1CCOCC1
O=C(-O-C-c1:c:c:c:c:c:1)-[NH;D2;+0:1]-[C:2]1-[C:3]-[C:4]-[#7:5](-[C:6]-[C:7](-[#7:8])=[O;D1;H0:9])-[C:10]-1=[O;D1;H0:11]>>[#7:8]-[C:7](=[O;D1;H0:9])-[C:6]-[#7:5]1-[C:4]-[C:3]-[C:2](-[NH2;D1;+0:1])-[C:10]-1=[O;D1;H0:11]
95.7
[{"value": 95.7, "product": "N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
A mixture of benzyl (3S)-1-[(1S)-1-methyl-2-morpholin-4-yl-2-oxoethyl]-2-oxopyrrolidin-3-ylcarbamate (20 g), 10% palladium on carbon (2 g) and ethanol (1.3 l) was stirred under an atmosphere of hydrogen for 16 h. The reaction mixture was filtered through Celite™ and the filtrate was concentrated under reduced pressure ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Primary amine
c1ccccc1
null
C1COCC[NH]1.C1CC[NH]C1
HO-
[Pd].C(C)O
null
16
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NC(=O)OCc2ccccc2)C1=O>[Pd].C(C)O>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-41adcde0d5054088a64cf77e9b050dd6
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(CBr)OCc1ccccc1>>C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(CC(=O)OCc2ccccc2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O.C([O-])([O-])=O.[K+].[K+].C(C1=CC=CC=C1)OC(CBr)=O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O)CC(=O)OCC1=CC=CC=C1
[CH3:1][C@@H:2]([C:3](=[O:4])[O:5][C:6]([CH3:7])([CH3:8])[CH3:9])[N:10]1[CH2:11][CH2:12][C@H:13]([NH:14][S:26](=[O:27])(=[O:28])[c:29]2[cH:30][cH:31][c:32]3[cH:33][c:34]([Cl:35])[cH:36][cH:37][c:38]3[cH:39]2)[C:40]1=[O:41].Br[CH2:15][C:16](=[O:17])[O:18][CH2:19][c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1>>[CH3:1][C@@H:...
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(CBr)OCc1ccccc1
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(CC(=O)OCc2ccccc2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
2f528facaf9aa1ab05620b510ae63e5e27715204b772ae8ea86d62f30b49e54b
dc829e3fdfa2d32260f0309a759a8629d6d95173de69dce05d7915b3a870e113
O=C(CN([C@H]1CCNC1=O)S(=O)(=O)c1ccc2ccccc2c1)OCc1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5].[#8:6]-[C:7](=[O;D1;H0:8])-[C:9]-[#7:10]1-[C:11]-[C:12]-[C:13](-[NH;D2;+0:14]-[#16:15](=[O;D1;H0:16])(=[O;D1;H0:17])-[c:18])-[C:19]-1=[O;D1;H0:20]>>[#8:6]-[C:7](=[O;D1;H0:8])-[C:9]-[#7:10]1-[C:11]-[C:12]-[C:13](-[N;H0;D3;+0:14](-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-...
115.5
[{"value": 115.5, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O)CC(=O)OCC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
72
HOUR
To a solution of tert-butyl (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoate (1 g) in DMF (20 ml) was added potassium carbonate (0.92 g) and benzyl-2-bromoacetate (0.33 g), and the mixture was stirred under nitrogen at room temperature for 72 h. The reaction mixture was filtered, co...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Primary halide
Ester.Tertiary amine
null
null
C1CC[NH]C1.c1ccccc1.c1ccc2ccccc2c1
HBr
CN(C)C=O
null
72
C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(CBr)OCc1ccccc1>CN(C)C=O>C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](N(CC(=O)OCc2ccccc2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a765f630bfcc4d368621ba25c966168e
O=C(O)c1cc2cc(Cl)ccc2o1>>Clc1ccc2occc2c1
ClC=1C=CC2=C(C=C(O2)C(=O)O)C1>>ClC=1C=CC2=C(C=CO2)C1
O=C(O)[c:7]1[o:6][c:5]2[cH:4][cH:3][c:2]([Cl:1])[cH:10][c:9]2[cH:8]1>>[Cl:1][c:2]1[cH:3][cH:4][c:5]2[o:6][cH:7][cH:8][c:9]2[cH:10]1
O=C(O)c1cc2cc(Cl)ccc2o1
Clc1ccc2occc2c1
null
[Cu]
CN1C(CCC1)=O
Reduction
Decarboxylation
1e06ee8694605f99df1524a985cad3553546b6740d6b4031e52d0cb2491b70c3
292164ffdf89eeb341ee9424f24084b252a703a26bb77721b558b0f8a8528c45
c1ccc2occc2c1
O-C(=O)-[c;H0;D3;+0:1]1:[#8;a:2]:[c:3]:[c:4]:[c:5]:1>>[#8;a:2]1:[c:3]:[c:4]:[c:5]:[cH;D2;+0:1]:1
418.7
[{"value": 418.7, "product": "ClC=1C=CC2=C(C=CO2)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
250
CELSIUS
null
null
To a solution of 5-chloro-1-benzofuran-2-carboxylic acid (0.2 g) in 1-methyl-2-pyrrolidinone (2 ml) was added copper granules (0.2 g). The reaction mixture was heated at 250° C. for 3.5 min in a microwave. The reaction vessel was cooled to room temperature and the mixture combined with four other similar mixtures and t...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
null
c1ccc2occc2c1
c1ccc2occc2c1
c1ccc2occc2c1
Other
[Cu].CN1C(CCC1)=O
250
null
O=C(O)c1cc2cc(Cl)ccc2o1>[Cu].CN1C(CCC1)=O>Clc1ccc2occc2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ae0f49a59f394151a37927a4235f4ff1
CC(C)(C)[Si](C)(C)Oc1ccc(C=O)cc1Cl>>C=Cc1ccc(O)c(Cl)c1
ClC=1C=C(C=O)C=CC1O[Si](C)(C)C(C)(C)C.C(CCC)[Li]>>ClC1=C(C=CC(=C1)C=C)O
CC(C)(C)[Si](C)(C)[O:7][c:6]1[cH:5][cH:4][c:3]([CH:2]=O)[cH:10][c:8]1[Cl:9]>>[CH2:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]([OH:7])[c:8]([Cl:9])[cH:10]1
CC(C)(C)[Si](C)(C)Oc1ccc(C=O)cc1Cl
C=Cc1ccc(O)c(Cl)c1
null
[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1
C1CCOC1
Functional Group Interconversion
OtherReaction
2e8f050b566a6b6ad6c7b65706622195f93eadf1eda7a7bb5d8cc2e9f4ca6ccf
2005cf38c32b3fecba26a2825de56bb6eb2bc7995e575116f2f19492ff2fec94
c1ccccc1
C-C(-C)(-C)-[Si](-C)(-C)-[O;H0;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[c:5](-[CH;D2;+0:6]=O):[c:7]:[c:8]:1>>[C;D1;H2:9]=[CH;D2;+0:6]-[c:5]1:[c:7]:[c:8]:[c:2](-[OH;D1;+0:1]):[c:3]:[c:4]:1
null
[]
0
CELSIUS
20
MINUTE
To a slurry of methyltriphenylphosphonium bromide (0.23 g) in dry THF (5 ml) under nitrogen at −78° C., n-butyl lithium (1.6M in hexanes, 0.37 ml) was added dropwise over 2 min. The mixture was allowed to warm to 0° C., stirred for 20 min, cooled to −78° C. and a solution of 3-chloro-4-[[(1,1-dimethylethyl)dimethylsily...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.TMS ether protective group
Aromatic alcohol.Vinyl
null
null
c1ccccc1
HO-
[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1
0
0.333333
CC(C)(C)[Si](C)(C)Oc1ccc(C=O)cc1Cl>[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1>C=Cc1ccc(O)c(Cl)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c90cb717958747869b5e662292221011
CC(C)(C)[Si](C)(C)Cl.O=Cc1ccc(Cl)c(O)c1>>CC(C)(C)[Si](C)(C)Oc1cc(C=O)ccc1Cl
ClC1=C(C=C(C=O)C=C1)O.[Si](C)(C)(C(C)(C)C)Cl.C(C)N(CC)CC>>[Si](C)(C)(C(C)(C)C)OC=1C=C(C=O)C=CC1Cl
Cl[Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7].[OH:8][c:9]1[cH:10][c:11]([CH:12]=[O:13])[cH:14][cH:15][c:16]1[Cl:17]>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][c:9]1[cH:10][c:11]([CH:12]=[O:13])[cH:14][cH:15][c:16]1[Cl:17]
CC(C)(C)[Si](C)(C)Cl.O=Cc1ccc(Cl)c(O)c1
CC(C)(C)[Si](C)(C)Oc1cc(C=O)ccc1Cl
null
null
C(Cl)Cl
Protection
Alcohol protection with silyl ethers
91043baed1393f1ecd2302d7d0b31c01cf171d3977dd7c70afa1da52fa298c73
4a917c959d011f885a1269fa3c1f022ee5e09144996246d24e42e65634a451ac
c1ccccc1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[OH;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[C;D1;H3:5]-[C:4](-[C;D1;H3:6])(-[C;D1;H3:7])-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[O;H0;D2;+0:8]-[c:9](:[c:10]):[c:11]
null
[]
null
null
19
HOUR
A mixture of 4-chloro-3-hydroxy-benzaldehyde* (0.354 g), 4-N,N-dimethylaminopyridine (0.028 g), tert-butyldimethylsilyl chloride (0.409 g) and triethylamine (0.473 ml) in DCM (15 ml) was stirred at room temperature under nitrogen for 19 h. The mixture was quenched with saturated aqueous sodium bicarbonate and extracted...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol.Silyl protective group
TMS ether protective group
null
null
c1ccccc1
HCl
C(Cl)Cl
null
19
CC(C)(C)[Si](C)(C)Cl.O=Cc1ccc(Cl)c(O)c1>C(Cl)Cl>CC(C)(C)[Si](C)(C)Oc1cc(C=O)ccc1Cl
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-80dd5a41b73146389c0160db8e0b5bbb
CCC(N)C(=O)OC(C)(C)C.CCOC(=O)C(CCBr)N=[N+]=[N-]>>CCOC(=O)C(CCNC(CC)C(=O)OC(C)(C)C)N=[N+]=[N-]
NC(C(=O)OC(C)(C)C)CC.N(=[N+]=[N-])C(C(=O)OCC)CCBr.C(C)N(CC)CC>>N(=[N+]=[N-])C(C(=O)OCC)CCNC(CC)C(=O)OC(C)(C)C
[NH2:9][CH:10]([CH2:11][CH3:12])[C:13](=[O:14])[O:15][C:16]([CH3:17])([CH3:18])[CH3:19].Br[CH2:8][CH2:7][CH:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[N:20]=[N+:21]=[N-:22]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]([CH2:7][CH2:8][NH:9][CH:10]([CH2:11][CH3:12])[C:13](=[O:14])[O:15][C:16]([CH3:17])([CH3:18])[CH3:19])[N:20]=[N+:2...
CCC(N)C(=O)OC(C)(C)C.CCOC(=O)C(CCBr)N=[N+]=[N-]
CCOC(=O)C(CCNC(CC)C(=O)OC(C)(C)C)N=[N+]=[N-]
null
null
C(C)#N
Heteroatom Alkylation and Arylation
N-alkylation of primary amines with alkyl halides
fc19a1445ff204e66e51735d0191465bda3c6691fd233624a54742c9d4828411
0b1d32f56ad00f1e5bdae9390f9227bbea012fa2f8203aac34726b8a6761cc7c
null
Br-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4](-[#8:5])=[O;D1;H0:6].[C:7]-[C:8](-[NH2;D1;+0:9])-[C:10](=[O;D1;H0:11])-[#8:12]-[C:13](-[C;D1;H3:14])(-[C;D1;H3:15])-[C;D1;H3:16]>>[#8:5]-[C:4](=[O;D1;H0:6])-[C:3]-[C:2]-[CH2;D2;+0:1]-[NH;D2;+0:9]-[C:8](-[C:7])-[C:10](=[O;D1;H0:11])-[#8:12]-[C:13](-[C;D1;H3:14])(-[C;D1;H3:15])-[C;D1;H3...
52.5
[{"value": 52.5, "product": "N(=[N+]=[N-])C(C(=O)OCC)CCNC(CC)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
To a solution of tert-butyl 2-amino-butanoate (0.397 g) and ethyl 2-azido-4-bromo-butanoate (0.286 g) in acetonitrile (5 ml) was added triethylamine (0.347 ml). The mixture was heated at 50° C. for 18 h, cooled and evaporated onto silica gel (Merck.7734). The pre-absorbed material was purified by flash column chromatog...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary amine
Secondary amine
null
null
null
HBr
C(C)#N
50
null
CCC(N)C(=O)OC(C)(C)C.CCOC(=O)C(CCBr)N=[N+]=[N-]>C(C)#N>CCOC(=O)C(CCNC(CC)C(=O)OC(C)(C)C)N=[N+]=[N-]
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-11adef3129b84f0b94db91599fbd1023
CCO.C[C@H](C(=O)OC(C)(C)C)N1CC[C@@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>CCC(C(=O)OC(C)(C)C)N1CCC(NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C(C)(C)NC(C)C.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@H]1C(N(CC1)[C@@H](C(=O)OC(C)(C)C)C)=O.C(C)O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)NC1C(N(CC1)C(C(=O)OC(C)(C)C)CC)=O
OC[CH3:1].[CH3:2][C@H:3]([C:4](=[O:5])[O:6][C:7]([CH3:8])([CH3:9])[CH3:10])[N:11]1[CH2:12][CH2:13][C@@H:14]([NH:15][S:16](=[O:17])(=[O:18])[c:19]2[cH:20][cH:21][c:22]3[cH:23][c:24]([Cl:25])[cH:26][cH:27][c:28]3[cH:29]2)[C:30]1=[O:31]>>[CH3:1][CH2:2][CH:3]([C:4](=[O:5])[O:6][C:7]([CH3:8])([CH3:9])[CH3:10])[N:11]1[CH2:12...
CCO.C[C@H](C(=O)OC(C)(C)C)N1CC[C@@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
CCC(C(=O)OC(C)(C)C)N1CCC(NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
[Pd]
C(Cl)Cl
C-C Coupling
C-methylation
861590323101b9187e0da132999bd5db6e6f128995dfe411cf8248c6aee7d060
5086858461038ad8c4c4a388cee61b6d9e9118227e969bc00fcc5a7517669191
O=C1NCCC1NS(=O)(=O)c1ccc2ccccc2c1
O-C-[CH3;D1;+0:1].[C:2]-[#7:3](-[C@H;D3;+0:4](-[CH3;D1;+0:5])-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12])-[C:13](=[O;D1;H0:14])-[C:15]>>[C:2]-[#7:3](-[CH;D3;+0:4](-[CH2;D2;+0:5]-[CH3;D1;+0:1])-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12])-[C:13](=[O;D1;H0:...
null
[]
null
null
18
HOUR
A mixture of Intermediate 112 [Mixture 1] (0.051 g), 10% palladium on carbon (0.01 g) and ethanol (5 ml) was stirred under an atmosphere of hydrogen for 18 h. The reaction mixture was filtered through Celite™ and the filtrate was concentrated under reduced pressure to give a yellow gum. The gum (0.034 g) in DCM (2 ml) ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
null
null
null
C1CC[NH]C1.c1ccc2ccccc2c1
HO-
[Pd].C(Cl)Cl
null
18
CCO.C[C@H](C(=O)OC(C)(C)C)N1CC[C@@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>[Pd].C(Cl)Cl>CCC(C(=O)OC(C)(C)C)N1CCC(NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-18976329a6ca4e37a8fefcfba77a9493
C1COCCN1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
N1CCOCC1.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O
[NH:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1.O[C:3]([C@H:2]([CH3:1])[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][S:16](=[O:17])(=[O:18])[c:19]2[cH:20][cH:21][c:22]3[cH:23][c:24]([Cl:25])[cH:26][cH:27][c:28]3[cH:29]2)[C:30]1=[O:31])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][C...
C1COCCN1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
2ef483949e7ba3e5f888cf14cdce25fa611f75be09fdf1854a473be519821b59
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCOCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[#8:8]1-[C:9]-[C:10]-[NH;D2;+0:11]-[C:12]-[C:13]-1>>[C;D1;H3:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:11]1-[C:12]-[C:13]-[#8:8]-[C:9]-[C:10]-1
null
[]
null
null
30
MINUTE
To a solution of (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid [Intermediate 29] (0.105 g) in DCM (10 ml) were added 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.152 g), HOBT (0.107 g) and triethylamine (0.222 ml) and the mixture was stirred at room temper...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
0.5
C1COCCN1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl.C(C)N(CC)CC>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7fc146245d2646ceb6e43fdc8a567d2e
C1CCNCC1.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)cc2)C1=O>>C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)cc2)C1=O
Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O.FC(C(=O)O)(F)F.N1CCCCC1.ClC1=CC=C(C=C1)/C=C/S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)OC(C)(C)C)C)=O>>ClC1=CC=C(C=C1)/C=C/S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O
[NH:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1.CC(C)(C)O[C:3]([C@H:2]([CH3:1])[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][S:16](=[O:17])(=[O:18])/[CH:19]=[CH:20]/[c:21]2[cH:22][cH:23][c:24]([Cl:25])[cH:26][cH:27]2)[C:28]1=[O:29])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][...
C1CCNCC1.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)cc2)C1=O
C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)cc2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Aminolysis of esters
a20b0e549c926e15da0ab6c9f432f3e8da8a2d0c59e3c6d1c2419879bcd6ef9b
a230d8ef639419dcbb4a41f52df2a77ab969b1b79d00c9710330f813c3417267
O=C(CN1CC[C@H](NS(=O)(=O)/C=C/c2ccccc2)C1=O)N1CCCCC1
C-C(-C)(-C)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
21.3
[{"value": 21.3, "product": "ClC1=CC=C(C=C1)/C=C/S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
tert-Butyl (2S)-2-[(3S)-3-({[(E)-2-(4-chlorophenyl)ethenyl]sulfonyl}amino)-2-oxopyrrolidin-1-yl]propanoate (0.192 g) was dissolved in DCM (2 ml) and treated with trifluoroacetic acid (2 ml) and stirred at room temperature for 2 h. The mixture was then concentrated under reduced pressure to give an oil which was subsequ...
10.6084/m9.figshare.5104873.v1
null
Ester.Secondary amine.Boc
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]C1.c1ccccc1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
2
C1CCNCC1.C[C@@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)cc2)C1=O>C(Cl)Cl.C(C)N(CC)CC>C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)cc2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-eb3527bffa1344d285bd826e249706ce
C[C@@H](C(=O)N1CCCC(NC(=O)OC(C)(C)C)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CC(CCC1)NC(OC(C)(C)C)=O)C)=O.FC(C(=O)O)(F)F>>NC1CN(CCC1)C([C@H](C)N1C([C@H](CC1)NS(=O)(=O)C1=CC2=CC=C(C=C2C=C1)Cl)=O)=O
CC(C)(C)OC(=O)[NH:10][CH:9]1[CH2:8][CH2:7][CH2:6][N:5]([C:3]([C@H:2]([CH3:1])[N:12]2[CH2:13][CH2:14][C@H:15]([NH:16][S:17](=[O:18])(=[O:19])[c:20]3[cH:21][cH:22][c:23]4[cH:24][c:25]([Cl:26])[cH:27][cH:28][c:29]4[cH:30]3)[C:31]2=[O:32])=[O:4])[CH2:11]1>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][CH:9]([NH2...
C[C@@H](C(=O)N1CCCC(NC(=O)OC(C)(C)C)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4]-[#7:5]>>[#7:5]-[C:4]-[C:2](-[NH2;D1;+0:1])-[C:3]
76.6
[{"value": 76.6, "product": "NC1CN(CCC1)C([C@H](C)N1C([C@H](CC1)NS(=O)(=O)C1=CC2=CC=C(C=C2C=C1)Cl)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
tert-Butyl 1-[(2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoyl]piperidin-3-ylcarbamate (0.6 g) was dissolved in DCM (11 ml) and trifluoroacetic acid (11 ml) was added. The mixture was stirred at room temperature for 2 h and then concentrated under reduced pressure. The residue was di...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl
null
2
C[C@@H](C(=O)N1CCCC(NC(=O)OC(C)(C)C)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl>C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-3cee8656047a4293930211c443eeb1e4
CC1CCCNC1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>CC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.CC1CNCCC1>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CC(CCC1)C)C)=O
[CH3:1][CH:2]1[CH2:3][CH2:4][CH2:5][NH:6][CH2:32]1.O[C:7](=[O:8])[C@H:9]([CH3:10])[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][S:16](=[O:17])(=[O:18])[c:19]2[cH:20][cH:21][c:22]3[cH:23][c:24]([Cl:25])[cH:26][cH:27][c:28]3[cH:29]2)[C:30]1=[O:31]>>[CH3:1][CH:2]1[CH2:3][CH2:4][CH2:5][N:6]([C:7](=[O:8])[C@H:9]([CH3:10])[N:11]2[...
CC1CCCNC1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
CC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
null
null
CN(C)C=O.C(Cl)Cl.C(C)(C)N(C(C)C)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
27.3
[{"value": 27.3, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CC(CCC1)C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
DAY
To polymer N-cyclohexylcarbodiimide-N′-propyloxymethyl polystyrene (0.038 g) in an Alltech™ tube was added a solution of (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid (0.007 g) in DCM (0.9 ml) followed by 3-methylpiperidine (0.0025 g) in DMF (0.1 ml) and N,N-diisopropylethyla...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
CN(C)C=O.C(Cl)Cl.C(C)(C)N(C(C)C)CC
null
96
CC1CCCNC1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>CN(C)C=O.C(Cl)Cl.C(C)(C)N(C(C)C)CC>CC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f53b241f8dee44fe8e3b65a30b106c34
CC(C)(C)OC(=O)NC1CCCNC1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1CCCC(NC(=O)OC(C)(C)C)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.N1CC(CCC1)NC(OC(C)(C)C)=O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CC(CCC1)NC(OC(C)(C)C)=O)C)=O
[NH:5]1[CH2:6][CH2:7][CH2:8][CH:9]([NH:10][C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17])[CH2:18]1.O[C:3]([C@H:2]([CH3:1])[N:19]1[CH2:20][CH2:21][C@H:22]([NH:23][S:24](=[O:25])(=[O:26])[c:27]2[cH:28][cH:29][c:30]3[cH:31][c:32]([Cl:33])[cH:34][cH:35][c:36]3[cH:37]2)[C:38]1=[O:39])=[O:4]>>[CH3:1][C@@H:2]([C:3](=...
CC(C)(C)OC(=O)NC1CCCNC1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)N1CCCC(NC(=O)OC(C)(C)C)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
null
[]
null
null
null
null
The title compound was prepared using Intermediate 29 and tert-butyl piperidin-3-ylcarbamate, and the synthetic procedure described for Example 1. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
null
null
null
CC(C)(C)OC(=O)NC1CCCNC1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1CCCC(NC(=O)OC(C)(C)C)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-735af55b970e46e6a71764fc75e55f39
C#CC(=O)O.C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C#CC(=O)NC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
NC1CN(CCC1)C([C@H](C)N1C([C@H](CC1)NS(=O)(=O)C1=CC2=CC=C(C=C2C=C1)Cl)=O)=O.C(C#C)(=O)O.C(C)(C)N(C(C)C)CC.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=N2)N=N1.F[P-](F)(F)(F)(F)F>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CC(CCC1)NC(C#C)=O)C)=O
O[C:3]([C:2]#[CH:1])=[O:4].[NH2:5][CH:6]1[CH2:7][CH2:8][CH2:9][N:10]([C:11](=[O:12])[C@H:13]([CH3:14])[N:15]2[CH2:16][CH2:17][C@H:18]([NH:19][S:20](=[O:21])(=[O:22])[c:23]3[cH:24][cH:25][c:26]4[cH:27][c:28]([Cl:29])[cH:30][cH:31][c:32]4[cH:33]3)[C:34]2=[O:35])[CH2:36]1>>[CH:1]#[C:2][C:3](=[O:4])[NH:5][CH:6]1[CH2:7][CH2...
C#CC(=O)O.C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C#CC(=O)NC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
null
null
CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]#[C;D1;H1:4].[#7:5]-[C:6]-[C:7](-[NH2;D1;+0:8])-[C:9]>>[#7:5]-[C:6]-[C:7](-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]#[C;D1;H1:4])-[C:9]
115.5
[{"value": 115.5, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CC(CCC1)NC(C#C)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
To a solution of N-{(3S)-1-[(1S)-2-(3-aminopiperidin-1-yl)-1-methyl-2-oxoethyl]-2-oxopyrrolidin-3-yl}-6-chloronaphthalene-2-sulfonamide (0.005 g) in DMF (0.5 ml) were added propiolic acid (0.001 g), N,N-diisopropylethylamine (0.0044 ml) and o-(7-azabenzotriazol-1-yl)-N,N,N′,N′-tetramethyluronium hexafluorophosphate (0....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
CN(C)C=O
null
18
C#CC(=O)O.C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>CN(C)C=O>C#CC(=O)NC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f76981696ab54f1ea4848af4078fc098
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.OCc1ccoc1>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(Cc2ccoc2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O.N(=NC(=O)OC(C)C)C(=O)OC(C)C.O1C=C(C=C1)CO.C(CCC)P(CCCC)CCCC>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O)CC1=COC=C1
[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][S:22](=[O:23])(=[O:24])[c:25]2[cH:26][cH:27][c:28]3[cH:29][c:30]([Cl:31])[cH:32][cH:33][c:34]3[cH:35]2)[C:36]1=[O:37].O[CH2:16][c:17]1[cH:18][cH:19][o:20][cH:21]1>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH...
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.OCc1ccoc1
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(Cc2ccoc2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
Mitsunobu_sulfonamide
0bda68210bc1a4edc8064b140a39ccb3ef813b89c5267469bd545dded6906cd4
2497efd1dadfa61592e966deb414dc4463866875b7ffd693ba98c7592e2a7ec2
O=C(CN1CC[C@H](N(Cc2ccoc2)S(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCOCC1
O-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[#8;a:5]:[c:6]:1.[#7:7]-[C:8](=[O;D1;H0:9])-[C:10]-[#7:11]1-[C:12]-[C:13]-[C:14](-[NH;D2;+0:15]-[#16:16](=[O;D1;H0:17])(=[O;D1;H0:18])-[c:19])-[C:20]-1=[O;D1;H0:21]>>[#7:7]-[C:8](=[O;D1;H0:9])-[C:10]-[#7:11]1-[C:12]-[C:13]-[C:14](-[N;H0;D3;+0:15](-[CH2;D2;+0:1]-[c:2]2:[c:3]:[c:4]:[#8;...
null
[]
null
null
60
HOUR
A solution of 6-chloro-N-{(3S)-1-[(1S)-1-methyl-2-morpholin-4-yl-2-oxoethyl]-2-oxopyrrolidin-3-yl}naphthalene-2-sulfonamide (0.015 g) in THF (0.5 ml) was treated with diisopropyl azodicarboxylate (0.01 ml), 3-furanmethanol (0.004 ml) and tri-n-butylphosphine (0.008 ml) and shaken at room temperature for 60 h. The mixtu...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Primary alcohol
Tertiary amine
null
null
C1COCC[NH]1.C1CC[NH]C1.c1ccoc1.c1ccc2ccccc2c1
HO-
C1CCOC1
null
60
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.OCc1ccoc1>C1CCOC1>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(Cc2ccoc2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7a26f7ca820749cf8efbed27692d508a
C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(NC1CCCNC1)c1ccccc1>>C[C@H](C(=O)N1CCCC(NC(=O)c2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@@H](C(=O)OC(C)(C)C)C)=O.FC(C(=O)O)(F)F.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O.N1CC(CCC1)NC(C1=CC=CC=C1)=O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@@H](C(=O)N1CC(CCC1)NC(C1=CC=CC=C1)=O)C)=O
CC(C)(C)O[C:3]([C@@H:2]([CH3:1])[N:20]1[CH2:21][CH2:22][C@H:23]([NH:24][S:25](=[O:26])(=[O:27])[c:28]2[cH:29][cH:30][c:31]3[cH:32][c:33]([Cl:34])[cH:35][cH:36][c:37]3[cH:38]2)[C:39]1=[O:40])=[O:4].[NH:5]1[CH2:6][CH2:7][CH2:8][CH:9]([NH:10][C:11](=[O:12])[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[CH2:19]1>>[CH3:1][C@H...
C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(NC1CCCNC1)c1ccccc1
C[C@H](C(=O)N1CCCC(NC(=O)c2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Aminolysis of esters
a20b0e549c926e15da0ab6c9f432f3e8da8a2d0c59e3c6d1c2419879bcd6ef9b
a230d8ef639419dcbb4a41f52df2a77ab969b1b79d00c9710330f813c3417267
O=C(NC1CCCN(C(=O)CN2CC[C@H](NS(=O)(=O)c3ccc4ccccc4c3)C2=O)C1)c1ccccc1
C-C(-C)(-C)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
37.3
[{"value": 37.3, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@@H](C(=O)N1CC(CCC1)NC(C1=CC=CC=C1)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of tert-butyl (2R)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino)-2-oxopyrrolidin-1-yl)propanoate (0.025 g) in DCM (1 ml) was treated with trifluoroacetic acid (1 ml) and stirred at room temperature for 2 h. The mixture was then concentrated under reduced pressure to give an oil which was subsequently trea...
10.6084/m9.figshare.5104873.v1
null
Ester.Secondary amine.Boc
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccccc1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
2
C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(NC1CCCNC1)c1ccccc1>C(Cl)Cl.C(C)N(CC)CC>C[C@H](C(=O)N1CCCC(NC(=O)c2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2a63c23aabf6477a95f607a9610fff33
C1COCCN1.CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1>>CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCOCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
N1CCOCC1.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)CC(CC)=O.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(CC)=O)[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O
[NH:15]1[CH2:16][CH2:17][O:18][CH2:19][CH2:20]1.O[C:13]([C@@H:11]([N:10]1[CH2:9][CH2:8][C@H:7]([N:6]([CH2:5][C:3]([CH2:2][CH3:1])=[O:4])[S:23](=[O:24])(=[O:25])[c:26]2[cH:27][cH:28][c:29]3[cH:30][c:31]([Cl:32])[cH:33][cH:34][c:35]3[cH:36]2)[C:21]1=[O:22])[CH3:12])=[O:14]>>[CH3:1][CH2:2][C:3](=[O:4])[CH2:5][N:6]([C@H:7]...
C1COCCN1.CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCOCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
2ef483949e7ba3e5f888cf14cdce25fa611f75be09fdf1854a473be519821b59
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCOCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[#8:8]1-[C:9]-[C:10]-[NH;D2;+0:11]-[C:12]-[C:13]-1>>[C;D1;H3:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:11]1-[C:10]-[C:9]-[#8:8]-[C:13]-[C:12]-1
null
[]
null
null
30
MINUTE
To a solution of (2S)-2-{(3S)-3-[[(6-chloro-2-naphthyl)sulfonyl](2-oxobutyl)amino]-2-oxopyrrolidin-1-yl}propanoic acid (0.035 g) in DCM (2 ml) were added 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.044 g), HOBT (0.031 g) and triethylamine (0.064 ml) and the mixture was stirred at room temperature f...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1COCCN1
C1COCC[NH]1
C1CC[NH]C1.C1COCC[NH]1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
0.5
C1COCCN1.CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1>C(Cl)Cl.C(C)N(CC)CC>CCC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCOCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0d303d5cecda4a898a2f1582f72973c0
CC1CCCNC1.C[C@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>CC1CCCN(C(=O)[C@@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
CC1CNCCC1.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@@H](C(=O)O)C)=O.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@@H](C(=O)N1CC(CCC1)C)C)=O
[CH3:1][CH:2]1[CH2:3][CH2:4][CH2:5][NH:6][CH2:32]1.O[C:7](=[O:8])[C@@H:9]([CH3:10])[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][S:16](=[O:17])(=[O:18])[c:19]2[cH:20][cH:21][c:22]3[cH:23][c:24]([Cl:25])[cH:26][cH:27][c:28]3[cH:29]2)[C:30]1=[O:31]>>[CH3:1][CH:2]1[CH2:3][CH2:4][CH2:5][N:6]([C:7](=[O:8])[C@@H:9]([CH3:10])[N:11]...
CC1CCCNC1.C[C@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
CC1CCCN(C(=O)[C@@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
null
[]
null
null
75
MINUTE
To a solution of (2R)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid (0.018 g) in DCM (0.5 ml) were added 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.018 g), HOBT (0.013 g) and triethylamine (0.039 ml) and the mixture was stirred at room temperature for 75 min....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
1.25
CC1CCCNC1.C[C@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl.C(C)N(CC)CC>CC1CCCN(C(=O)[C@@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6f90fee4c2b2423b968f48b74db08314
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.N#CCBr>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CC#N)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].C[Si](C)(C)[N-][Si](C)(C)C.[Li+].BrCC#N>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O)CC#N
[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][S:19](=[O:20])(=[O:21])[c:22]2[cH:23][cH:24][c:25]3[cH:26][c:27]([Cl:28])[cH:29][cH:30][c:31]3[cH:32]2)[C:33]1=[O:34].Br[CH2:16][C:17]#[N:18]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:...
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.N#CCBr
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CC#N)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0fe6648877a29ae177a907a0d252f35d8beab440bf428116c5424a67bc0e72cd
0b054affe7e4bb904ceae512aabc19d89c93551cb46dfbc6f220fc85e5eeff75
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCOCC1
Br-[CH2;D2;+0:1]-[C:2]#[N;D1;H0:3].[#7:4]-[C:5](=[O;D1;H0:6])-[C:7]-[#7:8]1-[C:9]-[C:10]-[C:11](-[NH;D2;+0:12]-[#16:13](=[O;D1;H0:14])(=[O;D1;H0:15])-[c:16])-[C:17]-1=[O;D1;H0:18]>>[#7:4]-[C:5](=[O;D1;H0:6])-[C:7]-[#7:8]1-[C:9]-[C:10]-[C:11](-[N;H0;D3;+0:12](-[CH2;D2;+0:1]-[C:2]#[N;D1;H0:3])-[#16:13](=[O;D1;H0:14])(=[O...
27.7
[{"value": 27.7, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O)CC#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
16
HOUR
A solution of 6-chloro-N-{(3S)-1-[(1S)-1-methyl-2-morpholin-4-yl-2-oxoethyl]-2-oxopyrrolidin-3-yl}naphthalene-2-sulfonamide (0.01 g) in THF (2 ml) was cooled to −78° C. under nitrogen, and treated with lithium bis(trimethylsilyl) amide (1.0M solution in THF; 0.026 ml), followed by bromoacetonitrile (0.013 g). The resul...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Primary halide
Tertiary amine
null
null
C1COCC[NH]1.C1CC[NH]C1.c1ccc2ccccc2c1
HBr
C1CCOC1
-78
16
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.N#CCBr>C1CCOC1>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CC#N)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c3726134f7ce47758660d338cb2302ac
COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCOCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CC(=O)O)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
Cl.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(=O)OC)[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O.[OH-].[Li+]>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(=O)O)[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O
C[O:19][C:17]([CH2:16][N:15]([C@H:14]1[CH2:13][CH2:12][N:11]([C@@H:2]([CH3:1])[C:3](=[O:4])[N:5]2[CH2:6][CH2:7][O:8][CH2:9][CH2:10]2)[C:34]1=[O:35])[S:20](=[O:21])(=[O:22])[c:23]1[cH:24][cH:25][c:26]2[cH:27][c:28]([Cl:29])[cH:30][cH:31][c:32]2[cH:33]1)=[O:18]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:...
COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCOCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CC(=O)O)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C1CCOC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCOCC1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
61.6
[{"value": 61.6, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(=O)O)[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of methyl N-[(6-chloro-2-naphthyl)sulfonyl]-N-{(3S)-1-[(1S)-1-methyl-2-morpholin-4-yl-2-oxoethyl]-2-oxopyrrolidin-3-yl}glycinate (0.010 g) in THF (2 ml) was added lithium hydroxide (0.003 g) in water (2 ml), and the resultant solution stirred for 16 h. The mixture was acidified to pH5 using hydrochloric a...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
C1COCC[NH]1.C1CC[NH]C1.c1ccc2ccccc2c1
Other
C1CCOC1.O
null
null
COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCOCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1>C1CCOC1.O>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CC(=O)O)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c61282f557ce4c26a0dea4a210034ac1
CCOC(=O)C1CCCCN1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1CCCCC1C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
N1C(C(=O)OCC)CCCC1.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C(CCCC1)C(=O)O)C)=O
CC[O:13][C:11]([CH:10]1[NH:5][CH2:6][CH2:7][CH2:8][CH2:9]1)=[O:12].O[C:3]([C@H:2]([CH3:1])[N:14]1[CH2:15][CH2:16][C@H:17]([NH:18][S:19](=[O:20])(=[O:21])[c:22]2[cH:23][cH:24][c:25]3[cH:26][c:27]([Cl:28])[cH:29][cH:30][c:31]3[cH:32]2)[C:33]1=[O:34])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][...
CCOC(=O)C1CCCCN1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)N1CCCCC1C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Protection
OtherReaction
c14ebbb227134a7db53a92ba8c7e0f6e66e80fb137e8c94bc7392ee524bc2ca3
a9275dd4bfdd260ffab0c2af4db0d4d1bb31d9d460b4e9fcded21863ffc3ef53
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5])-[NH;D2;+0:6]-[C:7]-[C:8].O-[C;H0;D3;+0:9](=[O;D1;H0:10])-[C:11](-[C;D1;H3:12])-[#7:13]-[C:14]=[O;D1;H0:15]>>[C:8]-[C:7]-[N;H0;D3;+0:6](-[C;H0;D3;+0:9](=[O;D1;H0:10])-[C:11](-[C;D1;H3:12])-[#7:13]-[C:14]=[O;D1;H0:15])-[C:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1])-[C:5]
21.9
[{"value": 21.9, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C(CCCC1)C(=O)O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid (0.025 g) in DCM (10 ml) were added 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.036 g), HOBT (0.026 g) and triethylamine (0.026 ml) and the mixture was stirred at room temperature for 30 min. ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ester.Secondary amine
Carboxylic acid.Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
0.5
CCOC(=O)C1CCCCN1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl.C(C)N(CC)CC>C[C@@H](C(=O)N1CCCCC1C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ed4fcacec1d04b19971e56835f5b19ec
C1CCNCC1.C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@@H](C(=O)OC(C)(C)C)C)=O.FC(C(=O)O)(F)F.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O.N1CCCCC1>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@@H](C(N1CCCCC1)=O)C)=O
[NH:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1.CC(C)(C)O[C:3]([C@@H:2]([CH3:1])[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][S:16](=[O:17])(=[O:18])[c:19]2[cH:20][cH:21][c:22]3[cH:23][c:24]([Cl:25])[cH:26][cH:27][c:28]3[cH:29]2)[C:30]1=[O:31])=[O:4]>>[CH3:1][C@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1)[N:11...
C1CCNCC1.C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Aminolysis of esters
a20b0e549c926e15da0ab6c9f432f3e8da8a2d0c59e3c6d1c2419879bcd6ef9b
a230d8ef639419dcbb4a41f52df2a77ab969b1b79d00c9710330f813c3417267
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
C-C(-C)(-C)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
82
[{"value": 82.0, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@@H](C(N1CCCCC1)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of tert-butyl (2R)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoate (0.025 g) in DCM (3 ml) was treated with trifluoroacetic acid (3 ml) and stirred at room temperature for 2 h. The mixture was then concentrated under reduced pressure to give an oil which was subsequently trea...
10.6084/m9.figshare.5104873.v1
null
Ester.Secondary amine.Boc
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
2
C1CCNCC1.C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl.C(C)N(CC)CC>C[C@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-58e4412befac46d3ad1ca83cda34a7c0
C1CCNCC1.C[C@@H](C(=O)O)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
N1CCCCC1.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)C.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O)C
[NH:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1.O[C:3]([C@H:2]([CH3:1])[N:11]1[CH2:12][CH2:13][C@H:14]([N:15]([CH3:16])[S:17](=[O:18])(=[O:19])[c:20]2[cH:21][cH:22][c:23]3[cH:24][c:25]([Cl:26])[cH:27][cH:28][c:29]3[cH:30]2)[C:31]1=[O:32])=[O:4]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1)[N:1...
C1CCNCC1.C[C@@H](C(=O)O)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
8.6
[{"value": 8.6, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of (2S)-2{(3S)-3-[[(6-chloro-2-naphthyl)sulfonyl](methyl)amino]-2-oxopyrrolidin-1-yl}propanoic acid (0.020 g) in DCM (2 ml) were added 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.011 g), HOBT (0.007 g) and triethylamine (0.020 ml) and the mixture was stirred at room temperature for 30...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
0.5
C1CCNCC1.C[C@@H](C(=O)O)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl.C(C)N(CC)CC>C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bdf12c227e064ebabdacb44df1860c0a
C1CCNCC1.COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1>>COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCCCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
N1CCCCC1.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O)CC(=O)OC.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(=O)OC)[C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O
[NH:15]1[CH2:16][CH2:17][CH2:18][CH2:19][CH2:20]1.O[C:13]([C@@H:11]([N:10]1[CH2:9][CH2:8][C@H:7]([N:6]([CH2:5][C:3]([O:2][CH3:1])=[O:4])[S:23](=[O:24])(=[O:25])[c:26]2[cH:27][cH:28][c:29]3[cH:30][c:31]([Cl:32])[cH:33][cH:34][c:35]3[cH:36]2)[C:21]1=[O:22])[CH3:12])=[O:14]>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][N:6]([C@H:7]1[...
C1CCNCC1.COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCCCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
46.5
[{"value": 46.5, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(=O)OC)[C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of (2S)-2-{(3S)-3-[[(6-chloro-2-naphthyl)sulfonyl](2-methoxy-2-oxoethyl)amino]-2-oxopyrrolidin-1-yl}propanoic acid (0.032 g) in DCM (5 ml) were added 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.02 g), HOBT (0.014 g) and triethylamine (0.034 ml) and the mixture was stirred at room temp...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]C1.C1CC[NH]CC1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
1
C1CCNCC1.COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)O)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1>C(Cl)Cl.C(C)N(CC)CC>COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCCCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-49ce8660a0d44e569b4a46c3a121a7e7
COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCCCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1.[OH-]>>CO.C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(CC(=O)O)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(=O)OC)[C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O.[OH-].[Li+].Cl>>Cl.CO.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(=O)O)[C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O
[CH3:1][O:2][C:19]([CH2:18][N:17]([C@H:16]1[CH2:15][CH2:14][N:13]([C@@H:4]([CH3:3])[C:5](=[O:6])[N:7]2[CH2:8][CH2:9][CH2:10][CH2:11][CH2:12]2)[C:36]1=[O:37])[S:22](=[O:23])(=[O:24])[c:25]1[cH:26][cH:27][c:28]2[cH:29][c:30]([Cl:31])[cH:32][cH:33][c:34]2[cH:35]1)=[O:20].[OH-:21]>>[CH3:1][OH:2].[CH3:3][C@@H:4]([C:5](=[O:6...
COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCCCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1.[OH-]
CO.C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(CC(=O)O)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C1CCOC1.O
Acylation
OtherReaction
db9ee1d9bb846253c10c2f639d42c12d092d033c3651a71ea16dc0ecf4a55bdc
c5cee7247c9bd9461d9349ac8515839185f2e1daff3eef7b9c67c8b1310a1abe
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
[#7:1]-[C:2]-[C;H0;D3;+0:3](=[O;D1;H0:4])-[O;H0;D2;+0:5]-[C;D1;H3:6].[OH-;D0:7]>>[#7:1]-[C:2]-[C;H0;D3;+0:3](=[O;D1;H0:4])-[OH;D1;+0:7].[C;D1;H3:6]-[OH;D1;+0:5]
205.4
[{"value": 10.0, "product": "Cl.CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 205.4, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CC(=O)O)[C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of methyl N-[(6-chloro-2-naphthyl)sulfonyl]-N-{(3S)-1-[(1S)-1-methyl-2-oxo-2-piperidin-1-ylethyl]-2-oxopyrrolidin-3-yl}glycinate (0.010 g) in THF (1 ml) was added lithium hydroxide (0.005 g) in water (1 ml), and the resultant solution stirred for 16 h. The mixture was acidified to pH5 using hydrochloric a...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid.Methanol
null
null
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
null
C1CCOC1.O
null
null
COC(=O)CN([C@H]1CCN([C@@H](C)C(=O)N2CCCCC2)C1=O)S(=O)(=O)c1ccc2cc(Cl)ccc2c1.[OH-]>C1CCOC1.O>CO.C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(CC(=O)O)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-df5abb0d36a745ff964e2f8fa27724ba
C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.N#CCBr>>C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(CC#N)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].C[Si](C)(C)[N-][Si](C)(C)C.[Li+].BrCC#N>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O)CC#N
[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][CH2:13][C@H:14]([NH:15][S:19](=[O:20])(=[O:21])[c:22]2[cH:23][cH:24][c:25]3[cH:26][c:27]([Cl:28])[cH:29][cH:30][c:31]3[cH:32]2)[C:33]1=[O:34].Br[CH2:16][C:17]#[N:18]>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][...
C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.N#CCBr
C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(CC#N)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0fe6648877a29ae177a907a0d252f35d8beab440bf428116c5424a67bc0e72cd
0b054affe7e4bb904ceae512aabc19d89c93551cb46dfbc6f220fc85e5eeff75
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
Br-[CH2;D2;+0:1]-[C:2]#[N;D1;H0:3].[#7:4]-[C:5](=[O;D1;H0:6])-[C:7]-[#7:8]1-[C:9]-[C:10]-[C:11](-[NH;D2;+0:12]-[#16:13](=[O;D1;H0:14])(=[O;D1;H0:15])-[c:16])-[C:17]-1=[O;D1;H0:18]>>[#7:4]-[C:5](=[O;D1;H0:6])-[C:7]-[#7:8]1-[C:9]-[C:10]-[C:11](-[N;H0;D3;+0:12](-[CH2;D2;+0:1]-[C:2]#[N;D1;H0:3])-[#16:13](=[O;D1;H0:14])(=[O...
43
[{"value": 43.0, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@H](C(N1CCCCC1)=O)C)=O)CC#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
16
HOUR
A solution of 6-chloro-N-{(3S)-1-[(1S)-1-methyl-2-oxo-2-piperidin-1-ylethyl]-2-oxopyrrolidin-3-yl}naphthalene-2-sulfonamide (0.015 g) in THF (2 ml) was cooled to −78° C. under nitrogen, and treated with lithium bis(trimethylsilyl) amide (1.0M solution in THF; 0.042 ml), followed by bromoacetonitrile (0.019 g). The resu...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Primary halide
Tertiary amine
null
null
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HBr
C1CCOC1
-78
16
C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.N#CCBr>C1CCOC1>C[C@@H](C(=O)N1CCCCC1)N1CC[C@H](N(CC#N)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a3dd945734854eb2b4129c81254e1bbf
C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(NC1CCCNC1)c1ccccc1>>C[C@H](C(=O)N1CCCC(NC(=O)c2ccccc2)C1)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@@H](C(=O)OC(C)(C)C)C)=O)C.FC(C(=O)O)(F)F.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O.N1CC(CCC1)NC(C1=CC=CC=C1)=O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@@H](C(=O)N1CC(CCC1)NC(C1=CC=CC=C1)=O)C)=O)C
CC(C)(C)O[C:3]([C@@H:2]([CH3:1])[N:20]1[CH2:21][CH2:22][C@H:23]([N:24]([CH3:25])[S:26](=[O:27])(=[O:28])[c:29]2[cH:30][cH:31][c:32]3[cH:33][c:34]([Cl:35])[cH:36][cH:37][c:38]3[cH:39]2)[C:40]1=[O:41])=[O:4].[NH:5]1[CH2:6][CH2:7][CH2:8][CH:9]([NH:10][C:11](=[O:12])[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[CH2:19]1>>[C...
C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(NC1CCCNC1)c1ccccc1
C[C@H](C(=O)N1CCCC(NC(=O)c2ccccc2)C1)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Aminolysis of esters
a20b0e549c926e15da0ab6c9f432f3e8da8a2d0c59e3c6d1c2419879bcd6ef9b
a230d8ef639419dcbb4a41f52df2a77ab969b1b79d00c9710330f813c3417267
O=C(NC1CCCN(C(=O)CN2CC[C@H](NS(=O)(=O)c3ccc4ccccc4c3)C2=O)C1)c1ccccc1
C-C(-C)(-C)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
55.2
[{"value": 55.2, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N([C@@H]1C(N(CC1)[C@@H](C(=O)N1CC(CCC1)NC(C1=CC=CC=C1)=O)C)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of tert-butyl (2R)-2-{(3S)-3-[[(6-chloro-2-naphthyl)sulfonyl](methyl)amino]-2-oxopyrrolidin-1-yl}propanoate (0.017 g) in DCM (0.5 ml) was treated with trifluoroacetic acid (0.5 ml) and stirred at room temperature for 2 h. The mixture was then concentrated under reduced pressure to give an oil which was subse...
10.6084/m9.figshare.5104873.v1
null
Ester.Secondary amine.Boc
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccccc1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
2
C[C@H](C(=O)OC(C)(C)C)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(NC1CCCNC1)c1ccccc1>C(Cl)Cl.C(C)N(CC)CC>C[C@H](C(=O)N1CCCC(NC(=O)c2ccccc2)C1)N1CC[C@H](N(C)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-993085dca3ef4537b2715ac868b3332c
CC=O.C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>CCNC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
C(C)=O.NC1CN(CCC1)C([C@H](C)N1C([C@H](CC1)NS(=O)(=O)C1=CC2=CC=C(C=C2C=C1)Cl)=O)=O.C(C)(=O)O.C(C)(=O)O.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.C(C)[N+](CC)(CC)CC.C(C)=O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CC(CCC1)NCC)C)=O
O=[CH:2][CH3:1].[NH2:3][CH:4]1[CH2:5][CH2:6][CH2:7][N:8]([C:9](=[O:10])[C@H:11]([CH3:12])[N:13]2[CH2:14][CH2:15][C@H:16]([NH:17][S:18](=[O:19])(=[O:20])[c:21]3[cH:22][cH:23][c:24]4[cH:25][c:26]([Cl:27])[cH:28][cH:29][c:30]4[cH:31]3)[C:32]2=[O:33])[CH2:34]1>>[CH3:1][CH2:2][NH:3][CH:4]1[CH2:5][CH2:6][CH2:7][N:8]([C:9](=[...
CC=O.C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
CCNC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
O=[CH;D2;+0:1]-[C;D1;H3:2].[#7:3]-[C:4]-[C:5](-[NH2;D1;+0:6])-[C:7]>>[#7:3]-[C:4]-[C:5](-[NH;D2;+0:6]-[CH2;D2;+0:1]-[C;D1;H3:2])-[C:7]
null
[]
null
null
60
HOUR
To a solution of acetaldehyde (0.041 ml from a stock solution made up from 0.0127 l acetaldehyde dissolved in 1 ml DCM)) in dry DCM (0.4 ml) treated with acetic acid (0.1 ml from a stock solution made up from 0.0054 ml acetic acid dissolved in 1 ml DCM) was added N-{(3S)-1-[(1S)-2-(3-aminopiperidin-1-yl)-1-methyl-2-oxo...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
Other
C(Cl)Cl
null
60
CC=O.C[C@@H](C(=O)N1CCCC(N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl>CCNC1CCCN(C(=O)[C@H](C)N2CC[C@H](NS(=O)(=O)c3ccc4cc(Cl)ccc4c3)C2=O)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2092c867fb284e948b6e81396fe38769
C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(N[C@H]1CCCNC1)OCc1ccccc1>>C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.Cl.CN(CCCN=C=NCC)C.C=1C=CC2=C(C1)N=NN2O.N1C[C@H](CCC1)NC(OCC1=CC=CC=C1)=O>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@H](CCC1)NC(OCC1=CC=CC=C1)=O)C)=O
O[C:3]([C@H:2]([CH3:1])[N:22]1[CH2:23][CH2:24][C@H:25]([NH:26][S:27](=[O:28])(=[O:29])[c:30]2[cH:31][cH:32][c:33]3[cH:34][c:35]([Cl:36])[cH:37][cH:38][c:39]3[cH:40]2)[C:41]1=[O:42])=[O:4].[NH:5]1[CH2:6][CH2:7][CH2:8][C@H:9]([NH:10][C:11](=[O:12])[O:13][CH2:14][c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[CH2:21]1>>[CH3:...
C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(N[C@H]1CCCNC1)OCc1ccccc1
C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(N[C@H]1CCCN(C(=O)CN2CC[C@H](NS(=O)(=O)c3ccc4ccccc4c3)C2=O)C1)OCc1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
42.5
[{"value": 42.5, "product": "ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@H](CCC1)NC(OCC1=CC=CC=C1)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid (0.408 g) in DCM (21 ml) was treated with 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.394 g), HOBT (0.278 g) and triethylamine (0.286 ml) and stirred at room temperature for 1 h. A solution of be...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccccc1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl.C(C)N(CC)CC
null
1
C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=C(N[C@H]1CCCNC1)OCc1ccccc1>C(Cl)Cl.C(C)N(CC)CC>C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-81c46fc548a2432dba9495e6a550bdcd
C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1CCC[C@H](N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@H](CCC1)NC(OCC1=CC=CC=C1)=O)C)=O.FC(C(=O)O)(F)F>>N[C@@H]1CN(CCC1)C([C@H](C)N1C([C@H](CC1)NS(=O)(=O)C1=CC2=CC=C(C=C2C=C1)Cl)=O)=O
O=C(OCc1ccccc1)[NH:10][C@H:9]1[CH2:8][CH2:7][CH2:6][N:5]([C:3]([C@H:2]([CH3:1])[N:12]2[CH2:13][CH2:14][C@H:15]([NH:16][S:17](=[O:18])(=[O:19])[c:20]3[cH:21][cH:22][c:23]4[cH:24][c:25]([Cl:26])[cH:27][cH:28][c:29]4[cH:30]3)[C:31]2=[O:32])=[O:4])[CH2:11]1>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][CH2:8][C@H:9]([...
C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)N1CCC[C@H](N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
087b6600ba91d3df931fe6979f2445c192cbfd59e04fd2d8a10f7c7573ac669f
4e549866ec1acadec4c84aaf8495992a28ec78d8ea5ef1b9f44dd843b0dcb7d4
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCCCC1
O=C(-O-C-c1:c:c:c:c:c:1)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4]-[#7:5]>>[#7:5]-[C:4]-[C:2](-[NH2;D1;+0:1])-[C:3]
93
[{"value": 93.0, "product": "N[C@@H]1CN(CCC1)C([C@H](C)N1C([C@H](CC1)NS(=O)(=O)C1=CC2=CC=C(C=C2C=C1)Cl)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
6
HOUR
Benzyl (3S)-1-[(2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoyl]piperidin-3-ylcarbamate (0.128 g) was dissolved in DCM (3.5 ml) and treated with trifluoroacetic acid (10.5 ml) and stirred at room temperature for 6 h. The mixture was concentrated under reduced pressure and the residue...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Primary amine
c1ccccc1
null
C1CC[NH]CC1.C1CC[NH]C1.c1ccc2ccccc2c1
HO-
C(Cl)Cl
null
6
C[C@@H](C(=O)N1CCC[C@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>C(Cl)Cl>C[C@@H](C(=O)N1CCC[C@H](N)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-76208bbd205a40dfb12b242c62aea99a
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N)C1=O.O=S(=O)(Cl)c1cc2cc(Cl)ccc2o1>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2cc3cc(Cl)ccc3o2)C1=O
[Cl-].[NH4+].N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O.ClC=1C=CC2=C(C=C(O2)S(=O)(=O)Cl)C1>>ClC=1C=CC2=C(C=C(O2)S(=O)(=O)N[C@@H]2C(N(CC2)[C@H](C(=O)N2CCOCC2)C)=O)C1
[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][CH2:13][C@H:14]([NH2:15])[C:29]1=[O:30].Cl[S:16](=[O:17])(=[O:18])[c:19]1[cH:20][c:21]2[cH:22][c:23]([Cl:24])[cH:25][cH:26][c:27]2[o:28]1>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1)[N:11]1[CH2:12][CH2:13]...
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N)C1=O.O=S(=O)(Cl)c1cc2cc(Cl)ccc2o1
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2cc3cc(Cl)ccc3o2)C1=O
null
null
C(C)#N.N1=CC=CC=C1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C(CN1CC[C@H](NS(=O)(=O)c2cc3ccccc3o2)C1=O)N1CCOCC1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#8;a:6]:[c:7].[#7:8]-[C:9](=[O;D1;H0:10])-[C:11]-[#7:12]1-[C:13]-[C:14]-[C:15](-[NH2;D1;+0:16])-[C:17]-1=[O;D1;H0:18]>>[#7:8]-[C:9](=[O;D1;H0:10])-[C:11]-[#7:12]1-[C:13]-[C:14]-[C:15](-[NH;D2;+0:16]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#8...
55.1
[{"value": 55.1, "product": "ClC=1C=CC2=C(C=C(O2)S(=O)(=O)N[C@@H]2C(N(CC2)[C@H](C(=O)N2CCOCC2)C)=O)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
72
HOUR
To a solution of (3S)-3-amino-1-[(1S)-1-methyl-2-morpholin-4-yl-2-oxoethyl]pyrrolidin-2-one (0.077 g) in anhydrous acetonitrile (2ml) were added 5-chloro-1-benzofuran-2-sulfonyl chloride (0.043 g) in acetonitrile (2 ml) and pyridine (0.057 ml), and the mixture was stirred at room temperature for 72 h. Saturated ammoniu...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
C1COCC[NH]1.C1CC[NH]C1.c1ccc2occc2c1
HCl
C(C)#N.N1=CC=CC=C1
null
72
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N)C1=O.O=S(=O)(Cl)c1cc2cc(Cl)ccc2o1>C(C)#N.N1=CC=CC=C1>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)c2cc3cc(Cl)ccc3o2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-89d649d4b7be4c728ab42cad047e2397
C[C@@H](C(=O)N1CCC[C@@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1CCC[C@@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@@H](CCC1)NC(OCC1=CC=CC=C1)=O)C)=O>>C1=C(C=CC2=CC=CC=C12)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@@H](CCC1)NC(OCC1=CC=CC=C1)=O)C)=O
Cl[c:35]1[cH:34][c:33]2[cH:32][cH:31][c:30]([S:27]([NH:26][C@H:25]3[CH2:24][CH2:23][N:22]([C@@H:2]([CH3:1])[C:3](=[O:4])[N:5]4[CH2:6][CH2:7][CH2:8][C@@H:9]([NH:10][C:11](=[O:12])[O:13][CH2:14][c:15]5[cH:16][cH:17][cH:18][cH:19][cH:20]5)[CH2:21]4)[C:40]3=[O:41])(=[O:28])=[O:29])[cH:39][c:38]2[cH:37][cH:36]1>>[CH3:1][C@@...
C[C@@H](C(=O)N1CCC[C@@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)N1CCC[C@@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O
null
[Pd]
C(C)O
Functional Group Interconversion
Aromatic dehalogenation
b59c5c205c966b4215325ef1ee4f08427e93cdf8277de7587f9668b39e907bde
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
O=C(N[C@@H]1CCCN(C(=O)CN2CC[C@H](NS(=O)(=O)c3ccc4ccccc4c3)C2=O)C1)OCc1ccccc1
Cl-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]>>[c:3]:[c:2]:[cH;D2;+0:1]:[c:4]:[c:5]
3
[{"value": 3.0, "product": "C1=C(C=CC2=CC=CC=C12)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@@H](CCC1)NC(OCC1=CC=CC=C1)=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
17
HOUR
A mixture of benzyl (3R)-1-[(2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoyl]piperidin-3-ylcarbamate (0.350 g), 10% palladium on carbon (0.035 g) and ethanol (1000 ml) was stirred under an atmosphere of hydrogen for 17 h. The reaction mixture was filtered through Harbolite™ and the f...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccc2ccccc2c1
c1ccc2ccccc2c1
C1CC[NH]CC1.c1ccccc1.C1CC[NH]C1.c1ccc2ccccc2c1
Other
[Pd].C(C)O
null
17
C[C@@H](C(=O)N1CCC[C@@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>[Pd].C(C)O>C[C@@H](C(=O)N1CCC[C@@H](NC(=O)OCc2ccccc2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-42bdb3fb724a4485a85ae3d72f154c89
CC(C)(C)OC(=O)N1CC2CNCC(C2)C1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1C[C@@H]2C[C@@H](CN(C(=O)OC(C)(C)C)C2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)O)C)=O.C12CN(CC(CNC1)C2)C(=O)OC(C)(C)C.C12CN(CC(CNC1)C2)C(=O)OC(C)(C)C>>ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1C[C@H]2CN(C[C@@H](C1)C2)C(=O)OC(C)(C)C)C)=O
[NH:5]1[CH2:6][CH:7]2[CH2:8][CH:9]([CH2:10][N:11]([C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18])[CH2:19]2)[CH2:20]1.O[C:3]([C@H:2]([CH3:1])[N:21]1[CH2:22][CH2:23][C@H:24]([NH:25][S:26](=[O:27])(=[O:28])[c:29]2[cH:30][cH:31][c:32]3[cH:33][c:34]([Cl:35])[cH:36][cH:37][c:38]3[cH:39]2)[C:40]1=[O:41])=[O:4]>>[CH3:...
CC(C)(C)OC(=O)N1CC2CNCC(C2)C1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
C[C@@H](C(=O)N1C[C@@H]2C[C@@H](CN(C(=O)OC(C)(C)C)C2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
44fc7912ae653980c4958be1f5d66acd2f9ee13d2d0f8a1d50fa0b7e22c15fc8
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CN1CC[C@H](NS(=O)(=O)c2ccc3ccccc3c2)C1=O)N1C[C@@H]2CNC[C@@H](C2)C1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[#7:5]-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
null
[]
null
null
null
null
Using (2S)-2-((3S)-3-{[(6-chloro-2-naphthyl)sulfonyl]amino}-2-oxopyrrolidin-1-yl)propanoic acid and 3,7-diazabicyclo[3.3.1]nonane-3-carboxylic acid, 1,1-dimethylethyl ester* and the synthetic procedure described in Example 1, the title compound was prepared. * Reference for 3,7-Diazabicyclo[3.3.1]nonane-3-carboxylic ac...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1[NH]CC2CNCC1C2
C1[NH]C[C@H]2C[NH]C[C@@H]1C2
C1CC[NH]C1.C1[NH]C[C@H]2C[NH]C[C@@H]1C2.c1ccc2ccccc2c1
HO-
null
null
null
CC(C)(C)OC(=O)N1CC2CNCC(C2)C1.C[C@@H](C(=O)O)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O>>C[C@@H](C(=O)N1C[C@@H]2C[C@@H](CN(C(=O)OC(C)(C)C)C2)C1)N1CC[C@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bce6d1b0269345ada7d58941bda39329
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)c(O[Si](c3ccccc3)(c3ccccc3)C(C)(C)C)c2)C1=O>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)c(O)c2)C1=O
[Si](C1=CC=CC=C1)(C1=CC=CC=C1)(C(C)(C)C)OC=1C=C(C=CC1Cl)/C=C/S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC>>ClC1=C(C=C(C=C1)/C=C/S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O)O
CC(C)(C)[Si](c1ccccc1)(c1ccccc1)[O:27][c:26]1[c:24]([Cl:25])[cH:23][cH:22][c:21](/[CH:20]=[CH:19]/[S:16]([NH:15][C@H:14]2[CH2:13][CH2:12][N:11]([C@@H:2]([CH3:1])[C:3](=[O:4])[N:5]3[CH2:6][CH2:7][O:8][CH2:9][CH2:10]3)[C:29]2=[O:30])(=[O:17])=[O:18])[cH:28]1>>[CH3:1][C@@H:2]([C:3](=[O:4])[N:5]1[CH2:6][CH2:7][O:8][CH2:9][...
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)c(O[Si](c3ccccc3)(c3ccccc3)C(C)(C)C)c2)C1=O
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)c(O)c2)C1=O
null
null
C1CCOC1
Deprotection
Alcohol deprotection from silyl ethers
cb7a55bba7beea8afc666e12e8162e54d37a49e453e1640ce533ca6190b41190
bcb3a8510d04057b612b045a6ac632b147a7a112beeedd4cca92670e4d4c910b
O=C(CN1CC[C@H](NS(=O)(=O)/C=C/c2ccccc2)C1=O)N1CCOCC1
C-C(-C)(-C)-[Si](-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4])(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
83.8
[{"value": 83.8, "product": "ClC1=C(C=C(C=C1)/C=C/S(=O)(=O)N[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of (E)-2-(3-{[tert-butyl(diphenyl)silyl]oxy}-4-chlorophenyl)-N-{(3S)-1-[(1S)-1-methyl-2-morpholin-4-yl-2-oxoethyl]-2-oxopyrrolidin-3-yl}ethenesulfonamide (0.0078 g) in THF (0.3 ml) at −78° C. under nitrogen, tetra n-butylammonium fluoride (1M in THF, 0.014 ml) was added. The mixture was allowed to warm to...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
Aromatic alcohol
c1ccccc1.c1ccccc1
null
C1COCC[NH]1.C1CC[NH]C1.c1ccccc1
Other
C1CCOC1
null
null
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)c(O[Si](c3ccccc3)(c3ccccc3)C(C)(C)C)c2)C1=O>C1CCOC1>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](NS(=O)(=O)/C=C/c2ccc(Cl)c(O)c2)C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-68e91174ffe545608aa7ac5a653e7839
CCOC(C)=O.CN(C)C=O.C[C@H](C(=O)OC(C)(C)C)N1CC[C@@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.ClCCN1CCOCC1>>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CCN2CCOCC2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=CO
ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N[C@H]1C(N(CC1)[C@@H](C(=O)OC(C)(C)C)C)=O.Cl.ClCCN1CCOCC1.C([O-])([O-])=O.[K+].[K+].C(C)(=O)OCC.CN(C)C=O>>C(=O)O.ClC=1C=C2C=CC(=CC2=CC1)S(=O)(=O)N(CCN1CCOCC1)[C@@H]1C(N(CC1)[C@H](C(=O)N1CCOCC1)C)=O
CC(=O)OC[CH3:9].[N:5]([CH3:6])([CH3:10])[CH:41]=[O:40].CC(C)(C)[O:42][C:3]([C@@H:2]([CH3:1])[N:11]1[CH2:12][CH2:13][C@@H:14]([NH:15][S:24](=[O:25])(=[O:26])[c:27]2[cH:28][cH:29][c:30]3[cH:31][c:32]([Cl:33])[cH:34][cH:35][c:36]3[cH:37]2)[C:38]1=[O:39])=[O:4].Cl[CH2:16][CH2:17][N:18]1[CH2:19][CH2:20][O:21][CH2:22][CH2:23...
CCOC(C)=O.CN(C)C=O.C[C@H](C(=O)OC(C)(C)C)N1CC[C@@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.ClCCN1CCOCC1
C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CCN2CCOCC2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=CO
null
null
O
Acylation
OtherReaction
587a1834265d09e21c27d59c0e628af6623281afa9b3c943f1851b83330a735f
b845315bf5a7e52aca0797a39b510d29efd809527ec0cb2a85bae61afde03eff
O=C(CN1CC[C@H](N(CCN2CCOCC2)S(=O)(=O)c2ccc3ccccc3c2)C1=O)N1CCOCC1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C;H0;D3;+0:2](=[O;D1;H0:3])-[C:4](-[C;D1;H3:5])-[#7:6]1-[C:7]-[C:8]-[C:9](-[NH;D2;+0:10]-[#16:11](=[O;D1;H0:12])(=[O;D1;H0:13])-[c:14])-[C:15]-1=[O;D1;H0:16].C-C(=O)-O-C-[CH3;D1;+0:17].Cl-[CH2;D2;+0:18]-[C:19]-[#7:20].[CH3;D1;+0:21]-[N;H0;D3;+0:22](-[CH3;D1;+0:23])-[CH;D2;+0:24]=[O;D1;H0:25]...
null
[]
40
CELSIUS
2
HOUR
Example 1 (0.05 g) was dissolved in DMF (1 ml) and treated with chloroethylmorpholine hydrochloride (0.062 g) and potassium carbonate (0.093 g), and stirred at 40° C. for 2 h. The mixture was then heated at 80° C. for 8 h, cooled and treated with ethyl acetate and water. The organic extraxt was dried (over magnesium su...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Primary halide.Ester.Ester.Tertiary amide.Boc
Carboxylic acid.Ether.Tertiary amide.Tertiary amine
null
C1COCC[NH]1
C1COCC[NH]1.C1CC[NH]C1.C1COCC[NH]1.c1ccc2ccccc2c1
HCl
O
40
2
CCOC(C)=O.CN(C)C=O.C[C@H](C(=O)OC(C)(C)C)N1CC[C@@H](NS(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.ClCCN1CCOCC1>O>C[C@@H](C(=O)N1CCOCC1)N1CC[C@H](N(CCN2CCOCC2)S(=O)(=O)c2ccc3cc(Cl)ccc3c2)C1=O.O=CO
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1c85433b4ec64678bbc860768912d388
O=C(O)c1cccnc1-c1cccnc1>>OCc1cccnc1-c1cccnc1
CO.N1=C(C(=CC=C1)C(=O)O)C=1C=NC=CC1.C(C)N(CC)CC.Cl.[BH4-].[Na+]>>OCC=1C(=NC=CC1)C=1C=NC=CC1
O=[C:2]([OH:1])[c:3]1[cH:4][cH:5][cH:6][n:7][c:8]1-[c:9]1[cH:10][cH:11][cH:12][n:13][cH:14]1>>[OH:1][CH2:2][c:3]1[cH:4][cH:5][cH:6][n:7][c:8]1-[c:9]1[cH:10][cH:11][cH:12][n:13][cH:14]1
O=C(O)c1cccnc1-c1cccnc1
OCc1cccnc1-c1cccnc1
null
null
O1CCCC1
Reduction
Reduction of carboxylic acid to primary alcohol
0db83a5ebe1e318b78b55461cf7eb8f7c004eef0f9e3b6666d3df4c96b5f665e
93b4621647b04d2ad2f2825215b1567f171ba61fe10d136b5db6ea0470aa4932
c1ccc(-c2cccnc2)nc1
O=[C;H0;D3;+0:1](-[O;D1;H1:2])-[c:3](:[c:4]):[c:5](-[c:6]:[c:7]:[#7;a:8]):[#7;a:9]:[c:10]>>[#7;a:8]:[c:7]:[c:6]-[c:5](:[#7;a:9]:[c:10]):[c:3](-[CH2;D2;+0:1]-[O;D1;H1:2]):[c:4]
84.4
[{"value": 84.0, "product": "OCC=1C(=NC=CC1)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.4, "product": "OCC=1C(=NC=CC1)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
null
null
To a continually stirred, ice-cold solution of 2,3′-bipyridine-3-carboxylic acid (0.28 g, 1.40 mmole) in dry tetrahydrofuran (10 ml) and triethylamine (0.20 ml, 1.43 mmole) ethyl chloroformate (0.14 ml, 1.46 mmole) was added drop-by-drop over a 30 minute period. The precipitated product was then filtered and washed sev...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary alcohol
null
null
c1ccncc1.c1ccncc1
Other
O1CCCC1
20
null
O=C(O)c1cccnc1-c1cccnc1>O1CCCC1>OCc1cccnc1-c1cccnc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-522eee91ca144361b417e0fe45341314
OCc1cccnc1-c1cccnc1>>Cc1cccnc1-c1cccnc1
OCC=1C(=NC=CC1)C=1C=NC=CC1.Cl.O1CCOCC1>>CC=1C(=NC=CC1)C=1C=NC=CC1
O[CH2:1][c:2]1[cH:3][cH:4][cH:5][n:6][c:7]1-[c:8]1[cH:9][cH:10][cH:11][n:12][cH:13]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][n:6][c:7]1-[c:8]1[cH:9][cH:10][cH:11][n:12][cH:13]1
OCc1cccnc1-c1cccnc1
Cc1cccnc1-c1cccnc1
null
[Pd]
CO
Reduction
OtherReaction
1deafbccd34c1d747dea179c0b63e48cd7fc76936d377fecabe099ecef578991
0a2c8330040d049ae67653e1474aff520bf8a2d8c908ffd7076f536576936945
c1ccc(-c2cccnc2)nc1
O-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4](-[c:5]:[c:6]:[#7;a:7]):[#7;a:8]:[c:9]>>[#7;a:7]:[c:6]:[c:5]-[c:4](:[#7;a:8]:[c:9]):[c:2](-[CH3;D1;+0:1]):[c:3]
76.1
[{"value": 76.0, "product": "CC=1C(=NC=CC1)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.1, "product": "CC=1C(=NC=CC1)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A 3-hydroxymethyl-2,3′-bipyridyl (42.3 mg, 0.227 mmole) solution containing methanol (5 ml) and 4N solution of hydrogen chloride in dry 1,4-dioxane (0.57 ml, 2.3 mmole) was hydrogenated in the presence of palladium on activated carbon catalyst (10%, 40 mg) at room temperature and ambient pressure for 3 hours. The catal...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
null
null
null
c1ccncc1.c1ccncc1
Other
[Pd].CO
null
3
OCc1cccnc1-c1cccnc1>[Pd].CO>Cc1cccnc1-c1cccnc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b86fd53c2c1347ee8ef00fd260228086
CCO>>CCO.O.OCC(O)CO
C(C)O.C(CCCCCCC\C=C/CCCCCCCC)(=O)OCC(O)CO>>C(C)O.O.OCC(O)CO.C(CCCCCCC\C=C/CCCCCCCC)(=O)OCC(O)CO
[CH3:26][CH2:27][OH:28]>>[CH3:26][CH2:27][OH:28].[OH2:29].[OH:30][CH2:31][CH:32]([OH:33])[CH2:34][OH:35]
CCO
CCO.O.OCC(O)CO
null
null
O.OCC(O)CO
Miscellaneous
OtherReaction
a244f833733718b07f52109095aa98cd5943ebccc6e7556166190ea2fb1e9527
3886f50ccf014aba7d974a7f782a7e63fb3f50b880ebcf5701bc7ab1c8a8ad31
null
null
null
[]
null
null
null
null
95% ethanol (USP) was diluted with water (USP), glycerin (USP), and glycerol monooleate (Eastman Chemical, Kingsport N.Y.) to provide a final solution at ethanol/water/glycerin/glycerol monooleate percent ratios of 35/59/5/1, respectively. Oxybutynin free base was then dissolved into the above solution to a concentrati...
10.6084/m9.figshare.5104873.v1
null
null
Primary alcohol.Primary alcohol.Secondary alcohol
null
null
null
Other
O.OCC(O)CO
null
null
CCO>O.OCC(O)CO>CCO.O.OCC(O)CO
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-fe246bcbccfc45eab97f443429b20fe3
OCC1CC2C=CC1C2.Oc1ccc(I)cc1>>Ic1ccc(OCC2CC3C=CC2C3)cc1
CCOC(=O)/N=N/C(=O)OCC.C12C(CC(C=C1)C2)CO.IC1=CC=C(C=C1)O.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>IC1=CC=C(C=C1)OCC1C2C=CC(C1)C2
[OH:6][CH2:7][CH:8]1[CH2:9][CH:10]2[CH:11]=[CH:12][CH:13]1[CH2:14]2.O[c:5]1[cH:4][cH:3][c:2]([I:1])[cH:16][cH:15]1>>[I:1][c:2]1[cH:3][cH:4][c:5]([O:6][CH2:7][CH:8]2[CH2:9][CH:10]3[CH:11]=[CH:12][CH:13]2[CH2:14]3)[cH:15][cH:16]1
OCC1CC2C=CC1C2.Oc1ccc(I)cc1
Ic1ccc(OCC2CC3C=CC2C3)cc1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
8915084acbaaf997bf0f89ff5187cb2f89c25dc683fffc57b3391298c8430dd9
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
C1=CC2CC1CC2COc1ccccc1
O-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[C:7]-[OH;D1;+0:8]>>[C:6]-[C:7]-[O;H0;D2;+0:8]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
97
[{"value": 97.0, "product": "IC1=CC=C(C=C1)OCC1C2C=CC(C1)C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.0, "product": "IC1=CC=C(C=C1)OCC1C2C=CC(C1)C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
Diethylazodicarboxylate (8.7 g) was added dropwise to a solution of 5-norbornene-2-methanol (6.2 g, 0.05 mol), 4-iodophenol (11.0 g, 0.05 mol) and triphenylphosphine (13.1 g, 0.05 mol) in 100 mL of anhydrous tetrahydrofuran. After completion of the addition, the resulting solution was stirred for 18 h at room temperatu...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
C1=CC2CCC1C2.c1ccccc1
HO-
O1CCCC1
null
18
OCC1CC2C=CC1C2.Oc1ccc(I)cc1>O1CCCC1>Ic1ccc(OCC2CC3C=CC2C3)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9bdd41d1c9294f7b851c289c0070b4ce
BrCCCCBr.CCC1(CO)COC1>>CCC1(COCCCCBr)COC1
OCC1(COC1)CC.BrCCCCBr.CCCCCC.[OH-].[Na+]>>BrCCCCOCC1(COC1)CC
Br[CH2:6][CH2:7][CH2:8][CH2:9][Br:10].[CH3:1][CH2:2][C:3]1([CH2:4][OH:5])[CH2:11][O:12][CH2:13]1>>[CH3:1][CH2:2][C:3]1([CH2:4][O:5][CH2:6][CH2:7][CH2:8][CH2:9][Br:10])[CH2:11][O:12][CH2:13]1
BrCCCCBr.CCC1(CO)COC1
CCC1(COCCCCBr)COC1
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
dd3f9c60e1f90d961a7c01d970ae213561355ee1451f276a3b04696e4b6fae5c
46a6e883cf919b4006e69abfdfd883f458f55c08b3200960c6a5b57c4139fbca
C1COC1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]-[OH;D1;+0:6]>>[C:4]-[C:5]-[O;H0;D2;+0:6]-[CH2;D2;+0:1]-[C:2]-[C:3]
45
[{"value": 44.0, "product": "BrCCCCOCC1(COC1)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 45.0, "product": "BrCCCCOCC1(COC1)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
5
HOUR
Into a 2 L egg plant type flask were charged 46.3 g (0.40 mol) of 3-hydroxymethyl-3-ethyloxetane (product name: OXT-101 manufactured by Toagosei Co., Ltd.), 250.3 g (1.16 mol) of 1,4-dibromobutane (reagent, manufactured by Tokyo Kasei Kogyo Co., Ltd.), and 275 ml of hexane. 500 ml of a 33% sodium hydroxide aqueous solu...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary alcohol
Ether
null
null
C1COC1
HBr
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.O
80
5
BrCCCCBr.CCC1(CO)COC1>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.O>CCC1(COCCCCBr)COC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e20a963324004b499bf87587735aa884
CCC1(COCCCCBr)COC1.CCOC(=O)c1ccc(O)cc1>>CCC1(COCCCCOc2ccc(C(=O)O)cc2)COC1
OC1=CC=C(C(=O)OCC)C=C1.BrCCCCOCC1(COC1)CC>>C(C)C1(COC1)COCCCCOC1=CC=C(C(=O)O)C=C1
Br[CH2:9][CH2:8][CH2:7][CH2:6][O:5][CH2:4][C:3]1([CH2:2][CH3:1])[CH2:20][O:21][CH2:22]1.CC[O:17][C:15]([c:14]1[cH:13][cH:12][c:11]([OH:10])[cH:19][cH:18]1)=[O:16]>>[CH3:1][CH2:2][C:3]1([CH2:4][O:5][CH2:6][CH2:7][CH2:8][CH2:9][O:10][c:11]2[cH:12][cH:13][c:14]([C:15](=[O:16])[OH:17])[cH:18][cH:19]2)[CH2:20][O:21][CH2:22]...
CCC1(COCCCCBr)COC1.CCOC(=O)c1ccc(O)cc1
CCC1(COCCCCOc2ccc(C(=O)O)cc2)COC1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
c47049bacd28cc701f2e77df376a2fcefecd5392e081f9a62473cff265d23a8c
017337a0828c32d10d28543003ae15a8b492b5e2f69019c65a4461eabc617d95
c1ccc(OCCCCOCC2COC2)cc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].C-C-[O;H0;D2;+0:4]-[C:5](=[O;D1;H0:6])-[c:7].[OH;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:8]-[c:9](:[c:10]):[c:11].[O;D1;H0:6]=[C:5](-[OH;D1;+0:4])-[c:7]
90.3
[{"value": 89.0, "product": "C(C)C1(COC1)COCCCCOC1=CC=C(C(=O)O)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.3, "product": "C(C)C1(COC1)COCCCCOC1=CC=C(C(=O)O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
4
HOUR
In a 300 ml three neck flask, 5.2 g (31 mmol) of ethyl p-hydroxybenzoate, 4.7 g (34 mmol) of potassium carbonate anhydride, and 7.8 g (31 mmol) of the 3-[(4-bromobutoxy)methyl]-3-ethyloxetane were dissolved in 50 ml of dimethylformamide. After the solution remained turbid was heated to a temperature of 80° C. and stirr...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Aromatic alcohol
Carboxylic acid.Ether
null
null
c1ccccc1.C1COC1
HBr
CN(C=O)C
80
4
CCC1(COCCCCBr)COC1.CCOC(=O)c1ccc(O)cc1>CN(C=O)C>CCC1(COCCCCOc2ccc(C(=O)O)cc2)COC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1c09bba65c034d81b66bbb9495a49de8
C1=COCCC1.O=C(O)c1ccc(O)cc1>>O=C(O)c1ccc(OC2CCCCO2)cc1
O1CCCC=C1.OC1=CC=C(C(=O)O)C=C1.C(Cl)Cl>>O1C(CCCC1)OC1=CC=C(C(=O)O)C=C1
[CH:9]1=[CH:10][CH2:11][CH2:12][CH2:13][O:14]1.[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([OH:8])[cH:15][cH:16]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([O:8][CH:9]2[CH2:10][CH2:11][CH2:12][CH2:13][O:14]2)[cH:15][cH:16]1
C1=COCCC1.O=C(O)c1ccc(O)cc1
O=C(O)c1ccc(OC2CCCCO2)cc1
null
C1(=CC=C(C=C1)S(=O)(=O)[O-])C.[NH+]1=CC=CC=C1
CCOCC
Heteroatom Alkylation and Arylation
oxa-Michael addition
1c7c788bec8addec628516b12629525fab255984248a4af23c71106a7726e25d
da6d2e768f263ce18da31b53a21ee41abe25d00717257e942f83f912a04f86d8
c1ccc(OC2CCCCO2)cc1
[#8:1]1-[C:2]-[C:3]-[C:4]-[CH;D2;+0:5]=[CH;D2;+0:6]-1.[OH;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[c:9]:[c:8](-[O;H0;D2;+0:7]-[CH;D3;+0:6]1-[#8:1]-[C:2]-[C:3]-[C:4]-[CH2;D2;+0:5]-1):[c:10]
86.2
[{"value": 86.2, "product": "O1C(CCCC1)OC1=CC=C(C(=O)O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
Into a 300 ml three neck flask were charged 25.4 g of 2,3-dihydropyran (reagent, manufactured by Tokyo Kasei Kogyo Co., Ltd.), 41.4 g of p-hydroxybenzoic acid (reagent, manufactured by Tokyo Kasei Kogyo Co., Ltd.), and 3.7 g of pyridinium p-toluenesulfonate (reagent, manufactured by Tokyo Kasei Kogyo Co., Ltd.). The mi...
10.6084/m9.figshare.5104873.v1
null
Ether.Aromatic alcohol
Ether.Ether
C1=COCCC1
C1CCOCC1
c1ccccc1.C1CCOCC1
null
C1(=CC=C(C=C1)S(=O)(=O)[O-])C.[NH+]1=CC=CC=C1.CCOCC
null
3
C1=COCCC1.O=C(O)c1ccc(O)cc1>C1(=CC=C(C=C1)S(=O)(=O)[O-])C.[NH+]1=CC=CC=C1.CCOCC>O=C(O)c1ccc(OC2CCCCO2)cc1