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large_stringclasses
414 values
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large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
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14
3.37k
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large_stringlengths
1
581
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large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
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large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-499c1cc00a404c2bb82dd402c8304336
COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2OCc1ccc(OC)cc1>>COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2O
C(=O)(O)[O-].[Na+].C(#N)C1=C(C(=O)C(=C(C1=O)Cl)Cl)C#N.COC(CCC\C=C/C[C@@H]1[C@H]([C@@H](CC1=O)O)C=1C=C2CCC(C2=CC1)OCC1=CC=C(C=C1)OC)=O.O>>COC(CCC\C=C/C[C@@H]1[C@H]([C@@H](CC1=O)O)C=1C=C2CCC(C2=CC1)O)=O
COc1ccc(C[O:27][CH:26]2[c:21]3[cH:20][cH:19][c:18]([C@@H:17]4[C@@H:11]([CH2:10]/[CH:9]=[CH:8]\[CH2:7][CH2:6][CH2:5][C:3]([O:2][CH3:1])=[O:4])[C:12](=[O:13])[CH2:14][C@H:15]4[OH:16])[cH:23][c:22]3[CH2:24][CH2:25]2)cc1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][CH2:7]/[CH:8]=[CH:9]\[CH2:10][C@H:11]1[C:12](=[O:13])[CH2:14][...
COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2OCc1ccc(OC)cc1
COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2O
null
null
ClCCl
Reduction
OtherReaction
c90596e654e5d1e77e11d554a977c19dbfd45f761dbcb2a67a22a5f8c8ab1ef2
628b56b3f4fed40b9cc8e2f7565bcae98d5e36a3f75394461dabd987fb619482
O=C1CC[C@H](c2ccc3c(c2)CCC3)C1
C-O-c1:c:c:c(-C-[O;H0;D2;+0:1]-[C:2](-[C:3])-[c:4]):c:c:1>>[C:3]-[C:2](-[OH;D1;+0:1])-[c:4]
434.7
[{"value": 60.0, "product": "COC(CCC\\C=C/C[C@@H]1[C@H]([C@@H](CC1=O)O)C=1C=C2CCC(C2=CC1)O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 434.7, "product": "COC(CCC\\C=C/C[C@@H]1[C@H]([C@@H](CC1=O)O)C=1C=C2CCC(C2=CC1)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
55
MINUTE
DDQ (41 mg, 0.18 mmol) was added to a mixture of 15-5 (11 mg, 0.021 mmol) in dichloromethane (3.5 mL)/water (175 μL). After 55 min., saturated NaHCO3 solution was added and the resulting mixture was extracted with dichloromethane (3×50 mL). The combined dichloromethane solution was washed with brine and then was dried ...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Secondary alcohol
c1ccccc1
null
C1CCCC1.c1ccc2c(c1)CCC2
HO-
ClCCl
null
0.916667
COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2OCc1ccc(OC)cc1>ClCCl>COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-aab96c42632a4a4890d68c2d0cb345b0
COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2OCc1ccc(OC)cc1>>COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2=O
C(=O)(O)[O-].[Na+].C(#N)C1=C(C(=O)C(=C(C1=O)Cl)Cl)C#N.COC(CCC\C=C/C[C@@H]1[C@H]([C@@H](CC1=O)O)C=1C=C2CCC(C2=CC1)OCC1=CC=C(C=C1)OC)=O.ClC(C)Cl>>COC(CCC\C=C/C[C@@H]1[C@H]([C@@H](CC1=O)O)C=1C=C2CCC(C2=CC1)=O)=O
COc1ccc(C[O:27][CH:26]2[c:21]3[cH:20][cH:19][c:18]([C@@H:17]4[C@@H:11]([CH2:10]/[CH:9]=[CH:8]\[CH2:7][CH2:6][CH2:5][C:3]([O:2][CH3:1])=[O:4])[C:12](=[O:13])[CH2:14][C@H:15]4[OH:16])[cH:23][c:22]3[CH2:24][CH2:25]2)cc1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][CH2:7]/[CH:8]=[CH:9]\[CH2:10][C@H:11]1[C:12](=[O:13])[CH2:14][...
COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2OCc1ccc(OC)cc1
COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2=O
null
null
ClCCl.O
Functional Group Interconversion
OtherReaction
d0dadbf1f41df81e42cc1b06e031cd4ce01cda1b95de9701c7b81cc85175e3d5
ff3c0d456b2d4191efb7126f02d8b343330f99a5bd55cfc08cd94367187e2524
O=C1CC[C@H](c2ccc3c(c2)CCC3=O)C1
C-O-c1:c:c:c(-C-[O;H0;D2;+0:1]-[CH;D3;+0:2]2-[C:3]-[C:4]-[c:5]:[c:6]-2:[c:7]):c:c:1>>[O;H0;D1;+0:1]=[C;H0;D3;+0:2]1-[C:3]-[C:4]-[c:5]:[c:6]-1:[c:7]
64.3
[{"value": 59.0, "product": "COC(CCC\\C=C/C[C@@H]1[C@H]([C@@H](CC1=O)O)C=1C=C2CCC(C2=CC1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 64.3, "product": "COC(CCC\\C=C/C[C@@H]1[C@H]([C@@H](CC1=O)O)C=1C=C2CCC(C2=CC1)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
DDQ (10 mg, 0.041 mmol) was added to a mixture of 15-5 (11 mg, 0.021 mmol) in dichloromethane (0.5 mL)/water (25 μL). After 1 h, dichloroethane (0.5 mL) was added and the reaction was stirred overnight. Saturated NaHCO3 solution was added and the resulting mixture was extracted with dichloromethane (3×20 mL). The combi...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Ketone
c1ccccc1.c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
C1CCCC1.c1ccc2c(c1)CCC2
HO-
ClCCl.O
null
1
COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2OCc1ccc(OC)cc1>ClCCl.O>COC(=O)CCC/C=C\C[C@H]1C(=O)C[C@@H](O)[C@@H]1c1ccc2c(c1)CCC2=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2bfb2671409546e88e8771b6b2fea5b7
C=CCc1ccc(O)c(CC=C)c1O>>CCCc1ccc(O)c(CCC)c1O
C(C=C)C1=C(O)C(=CC=C1O)CC=C>>C(CC)C1=C(O)C=CC(=C1O)CCC
[CH2:1]=[CH:2][CH2:3][c:4]1[cH:5][cH:6][c:7]([OH:8])[c:9]([CH2:10][CH:11]=[CH2:12])[c:13]1[OH:14]>>[CH3:1][CH2:2][CH2:3][c:4]1[cH:5][cH:6][c:7]([OH:8])[c:9]([CH2:10][CH2:11][CH3:12])[c:13]1[OH:14]
C=CCc1ccc(O)c(CC=C)c1O
CCCc1ccc(O)c(CCC)c1O
null
[Pd]
CO
Reduction
OtherReaction
f69b32ec19736437d6567a39731061f512e8e67ea9301cdcf93f07d7793003c3
d69deccbf6585965088073408ee5be8b8c3152f4b9c3604883a5d86aa3bdd693
c1ccccc1
[CH2;D1;+0:1]=[CH;D2;+0:2]-[C:3]-[c:4].[CH2;D1;+0:5]=[CH;D2;+0:6]-[C:7]-[c:8]>>[CH3;D1;+0:1]-[CH2;D2;+0:2]-[C:3]-[c:4].[CH3;D1;+0:5]-[CH2;D2;+0:6]-[C:7]-[c:8]
null
[]
null
null
null
null
The product 2,6-bis-allylresorcinol (33.5 gm) was dissolved in methanol and hydrogenated under H2 Pressure (initial pressure 45 psig) over 10% Pd on carbon (300 mg). The reaction mixture was filtered through celite and reduced i. vac. The crude oil was flushed through a short SiO2 gel column eluting with ethyl ether. T...
10.6084/m9.figshare.5104873.v1
null
Allyl.Allyl
null
null
null
c1ccccc1
null
[Pd].CO
null
null
C=CCc1ccc(O)c(CC=C)c1O>[Pd].CO>CCCc1ccc(O)c(CCC)c1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-07cdbdf55f0e4eb6803123ffb55d89c6
CCCc1c(O)ccc2c(C(F)(F)F)noc12.O=S(=O)(Cl)Cl>>CCCc1c(O)c(Cl)cc2c(C(F)(F)F)noc12
C(C(C)C)NCC(C)C.C(C(C)C)NCC(C)C.OC1=C(C2=C(C(=NO2)C(F)(F)F)C=C1)CCC.S([O-])(O)=O.[Na+].O1N=CC2=C1C=CC=C2.S(=O)(=O)(Cl)Cl>>ClC=1C(=C(C2=C(C(=NO2)C(F)(F)F)C1)CCC)O
[CH3:1][CH2:2][CH2:3][c:4]1[c:5]([OH:6])[cH:7][cH:9][c:10]2[c:11]([C:12]([F:13])([F:14])[F:15])[n:16][o:17][c:18]12.O=S(=O)(Cl)[Cl:8]>>[CH3:1][CH2:2][CH2:3][c:4]1[c:5]([OH:6])[c:7]([Cl:8])[cH:9][c:10]2[c:11]([C:12]([F:13])([F:14])[F:15])[n:16][o:17][c:18]12
CCCc1c(O)ccc2c(C(F)(F)F)noc12.O=S(=O)(Cl)Cl
CCCc1c(O)c(Cl)cc2c(C(F)(F)F)noc12
null
null
C(C)OCC.C1(=CC=CC=C1)C
Functional Group Interconversion
Chlorination
b7992ebb52d63e770c64ca0975a9b9bafbd1dbe31ad0828e52b61c031d34db6c
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc2oncc2c1
Cl-S(=O)(=O)-[Cl;H0;D1;+0:1].[O;D1;H1:2]-[c:3]1:[c:4]:[c:5]2:[#8;a:6]:[#7;a:7]:[c:8]:[c:9]:2:[c:10]:[cH;D2;+0:11]:1>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:11]1:[c:10]:[c:9]2:[c:8]:[#7;a:7]:[#8;a:6]:[c:5]:2:[c:4]:[c:3]:1-[O;D1;H1:2]
null
[]
null
null
8
HOUR
Diisobutylamine (0.8 ml, 0.10 eq) and 6-hydroxy-7-propyl-3-trifluoromethylbenzisoxazole (11 gm, 1.0 eq) were dissolved in toluene (275 ml) at room temperature. Slow addition of sulfuryl chloride (4.20 ml, 1.15 eq) results in a suspension which was stirred overnight. Additional diisobutylamine (total 1.6 ml, 0.4 eq) was...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2oncc2c1
c1ccc2oncc2c1
c1ccc2oncc2c1
HCl
C(C)OCC.C1(=CC=CC=C1)C
null
8
CCCc1c(O)ccc2c(C(F)(F)F)noc12.O=S(=O)(Cl)Cl>C(C)OCC.C1(=CC=CC=C1)C>CCCc1c(O)c(Cl)cc2c(C(F)(F)F)noc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-83d069dc05c04271afbe84952104b3b2
C=CCOc1ccc(C(=O)c2ccccc2)c(O)c1>>C=CCc1c(O)ccc(C(=O)c2ccccc2)c1O
C(C=C)OC1=CC(=C(C(=O)C2=CC=CC=C2)C=C1)O.ClC1=C(C=CC=C1)Cl>>OC1=C(C(=O)C2=CC=CC=C2)C=CC(=C1CC=C)O
[CH2:1]=[CH:2][CH2:3][O:6][c:5]1[cH:4][c:18]([OH:19])[c:9]([C:10](=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:8][cH:7]1>>[CH2:1]=[CH:2][CH2:3][c:4]1[c:5]([OH:6])[cH:7][cH:8][c:9]([C:10](=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[c:18]1[OH:19]
C=CCOc1ccc(C(=O)c2ccccc2)c(O)c1
C=CCc1c(O)ccc(C(=O)c2ccccc2)c1O
null
null
null
Miscellaneous
OtherReaction
f9046ab8287acad6d9b914f5f533866252d6845a323cc2516eb4a5b1de541a76
58578155da4647eafb0f18a2061753170490dc4f2b17890a513522e28d385731
O=C(c1ccccc1)c1ccccc1
[C;D1;H2:1]=[C:2]-[CH2;D2;+0:3]-[O;H0;D2;+0:4]-[c:5](:[c:6]):[cH;D2;+0:7]:[c:8](-[O;D1;H1:9]):[c:10]-[C:11]=[O;D1;H0:12]>>[C;D1;H2:1]=[C:2]-[CH2;D2;+0:3]-[c;H0;D3;+0:7](:[c:8](-[O;D1;H1:9]):[c:10]-[C:11]=[O;D1;H0:12]):[c:5](-[OH;D1;+0:4]):[c:6]
null
[]
null
null
null
null
Commercially available 4-allyloxy-2-hydroxybenzophenone (15 g) was rearranged by heating under reflux in ortho-dichlorobenzene (60 mL) for 26 hours. The product was isolated by dilution of the reaction mixture with 5 volumes hexanes to give a crystalline product as fine needles. Conditions: See reaction.notes.procedure...
10.6084/m9.figshare.5104873.v1
null
Ether.Allyl
Aromatic alcohol.Allyl
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
null
null
null
null
C=CCOc1ccc(C(=O)c2ccccc2)c(O)c1>>C=CCc1c(O)ccc(C(=O)c2ccccc2)c1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-dae0fbb51a884e2aa48fba735687cadc
C=CCc1c(O)ccc(C(=O)c2ccccc2)c1O>>CCCc1c(O)ccc(C(=O)c2ccccc2)c1O
OC1=C(C(=O)C2=CC=CC=C2)C=CC(=C1CC=C)O>>OC1=C(C(=O)C2=CC=CC=C2)C=CC(=C1CCC)O
[CH2:1]=[CH:2][CH2:3][c:4]1[c:5]([OH:6])[cH:7][cH:8][c:9]([C:10](=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[c:18]1[OH:19]>>[CH3:1][CH2:2][CH2:3][c:4]1[c:5]([OH:6])[cH:7][cH:8][c:9]([C:10](=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[c:18]1[OH:19]
C=CCc1c(O)ccc(C(=O)c2ccccc2)c1O
CCCc1c(O)ccc(C(=O)c2ccccc2)c1O
null
[Pd]
C(C)(=O)OCC
Reduction
Hydrogenation (double to single)
bc16a674f12262641e5cd54edc2026446c884c0ddcda2374dddc2ac4d3dae2ab
6afc5b4ad7d0f8b85f89bd805881fd9206fc3da38639abfb1c97bb82ede31c54
O=C(c1ccccc1)c1ccccc1
[CH2;D1;+0:1]=[CH;D2;+0:2]-[C:3]-[c:4]>>[CH3;D1;+0:1]-[CH2;D2;+0:2]-[C:3]-[c:4]
null
[]
null
null
null
null
A solution of 2,4-dihydroxy-3-(2-propenyl)benzophenone (3 g) was reduced under ˜1 atm H2 in ethyl acetate (100 mL) over 10% Pd/C catalyst (0.3 grams) for 3 hours. The product was purified by crystallization from methanol/water. The product is obtained as small yellow plates. Conditions: See reaction.notes.procedure_det...
10.6084/m9.figshare.5104873.v1
null
Allyl
null
null
null
c1ccccc1.c1ccccc1
null
[Pd].C(C)(=O)OCC
null
null
C=CCc1c(O)ccc(C(=O)c2ccccc2)c1O>[Pd].C(C)(=O)OCC>CCCc1c(O)ccc(C(=O)c2ccccc2)c1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9c83a6e508cf40888e8a12369cb3ade0
CCCc1cc(C(=O)CC)c(O)c(CCC)c1OC(C(=O)OC)c1ccccc1>>CCCc1cc(C(=O)CC)c(O)c(CCC)c1OC(C(=O)O)c1ccccc1
OC=1C(=C(OC(C(=O)OC)C2=CC=CC=C2)C(=CC1C(CC)=O)CCC)CCC.[OH-].[Na+]>>OC=1C(=C(OC(C(=O)O)C2=CC=CC=C2)C(=CC1C(CC)=O)CCC)CCC
C[O:22][C:20]([CH:19]([O:18][c:17]1[c:4]([CH2:3][CH2:2][CH3:1])[cH:5][c:6]([C:7](=[O:8])[CH2:9][CH3:10])[c:11]([OH:12])[c:13]1[CH2:14][CH2:15][CH3:16])[c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1)=[O:21]>>[CH3:1][CH2:2][CH2:3][c:4]1[cH:5][c:6]([C:7](=[O:8])[CH2:9][CH3:10])[c:11]([OH:12])[c:13]([CH2:14][CH2:15][CH3:16])[...
CCCc1cc(C(=O)CC)c(O)c(CCC)c1OC(C(=O)OC)c1ccccc1
CCCc1cc(C(=O)CC)c(O)c(CCC)c1OC(C(=O)O)c1ccccc1
null
null
null
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(COc2ccccc2)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
The ester of step 2 (18.6 gm) was hydrolyzed with NaOH (98 ml) as for example 1, step 5. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1
Other
null
null
null
CCCc1cc(C(=O)CC)c(O)c(CCC)c1OC(C(=O)OC)c1ccccc1>>CCCc1cc(C(=O)CC)c(O)c(CCC)c1OC(C(=O)O)c1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ec11d9e4f3f449f6a915145c8ea66bec
CCC(=O)[O-].CCCc1cccc(CCC)c1O>>CCCc1cc(C(=O)CC)cc(CCC)c1O
C(CC)(=O)[O-].[Na+].C(CC)C1=C(C(=CC=C1)CCC)O>>C(CC)C1=C(C(=CC(=C1)C(CC)=O)CCC)O
[O-][C:7](=[O:8])[CH2:9][CH3:10].[CH3:1][CH2:2][CH2:3][c:4]1[cH:5][cH:6][cH:11][c:12]([CH2:13][CH2:14][CH3:15])[c:16]1[OH:17]>>[CH3:1][CH2:2][CH2:3][c:4]1[cH:5][c:6]([C:7](=[O:8])[CH2:9][CH3:10])[cH:11][c:12]([CH2:13][CH2:14][CH3:15])[c:16]1[OH:17]
CCC(=O)[O-].CCCc1cccc(CCC)c1O
CCCc1cc(C(=O)CC)cc(CCC)c1O
null
null
OS(=O)(=O)C(F)(F)F
C-C Coupling
OtherReaction
e5396060890e7063846e7fb4a7b028009286093e3288e682a220bc78c8f51cd3
f600e7da43691f6eafd7566c832dd1dfb3eebdf72a39a998750efa402a8f7cf6
c1ccccc1
[C;D1;H3:1]-[C:2]-[C;H0;D3;+0:3](-[O-])=[O;D1;H0:4].[c:5]:[c:6]:[cH;D2;+0:7]:[c:8]:[c:9]>>[C;D1;H3:1]-[C:2]-[C;H0;D3;+0:3](=[O;D1;H0:4])-[c;H0;D3;+0:7](:[c:6]:[c:5]):[c:8]:[c:9]
null
[]
null
null
null
null
Sodium propanoate (0.88 g, 1.5 eq) and 2,6-dipropylphenol (1.09 g, 1.0 eq) were combined in Triflic Acid (5.0 g) as in Example 13, step 1. The resulting waxy solid was purified by chromatography on silica gel using ethyl acetate:hexanes:acetic acid (10:90:1) to give the titled phenol. Conditions: See reaction.notes.pro...
10.6084/m9.figshare.5104873.v1
null
null
Ketone
c1ccccc1
c1ccccc1
c1ccccc1
HO-
OS(=O)(=O)C(F)(F)F
null
null
CCC(=O)[O-].CCCc1cccc(CCC)c1O>OS(=O)(=O)C(F)(F)F>CCCc1cc(C(=O)CC)cc(CCC)c1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7592862b4de4400099977859206fead8
CC(C)Br.COC(=O)Cc1ccc(O)cc1>>COC(=O)Cc1ccc(OC(C)C)cc1
Cl.OC1=CC=C(C=C1)CC(=O)OC.C(=O)([O-])[O-].[Cs+].[Cs+].BrC(C)C>>CC(C)OC1=CC=C(C=C1)CC(=O)OC
Br[CH:11]([CH3:12])[CH3:13].[CH3:1][O:2][C:3](=[O:4])[CH2:5][c:6]1[cH:7][cH:8][c:9]([OH:10])[cH:14][cH:15]1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH:11]([CH3:12])[CH3:13])[cH:14][cH:15]1
CC(C)Br.COC(=O)Cc1ccc(O)cc1
COC(=O)Cc1ccc(OC(C)C)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
bff4876be49b448135c783dd3eeeb68ab3cc5bdc91beadda8a9095106cd5c747
cf768afb66ed5041aefdce1fa6d1e40995a1ab7c4b4a4ca47544fe49ee1e629f
c1ccccc1
Br-[CH;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3].[OH;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C;D1;H3:2]-[CH;D3;+0:1](-[C;D1;H3:3])-[O;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]
null
[]
null
null
8
HOUR
Methyl (4-hydroxyphenyl)acetate (1.0 g, 1.0 eq), Cs2CO3 (2.15 g, 1.1 eq) and 2-bromopropane (0.565 mL. 1.0 eq) were combined in 100 ml DMF at room temperature. The mixture was stirred overnight. The suspension was poured into 50 mL 1 N HCl and extracted with ethyl acetate. The organic phase was separated and washed wit...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HBr
CN(C)C=O
null
8
CC(C)Br.COC(=O)Cc1ccc(O)cc1>CN(C)C=O>COC(=O)Cc1ccc(OC(C)C)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f951ff6e45a44e29983784a13e42f834
CCC(=O)O.CCCc1ccc(O)c(CCC)c1F>>CCCc1cc(C(=O)CC)c(F)c(CCC)c1O
C(CC)(=O)O.FC=1C(=C(C=CC1CCC)O)CCC.FC(S(=O)(=O)O)(F)F>>FC=1C(=C(C(=CC1C(CC)=O)CCC)O)CCC
O[C:7](=[O:8])[CH2:9][CH3:10].[CH3:1][CH2:2][CH2:3][c:4]1[cH:5][cH:6][c:11]([OH:18])[c:13]([CH2:14][CH2:15][CH3:16])[c:17]1[F:12]>>[CH3:1][CH2:2][CH2:3][c:4]1[cH:5][c:6]([C:7](=[O:8])[CH2:9][CH3:10])[c:11]([F:12])[c:13]([CH2:14][CH2:15][CH3:16])[c:17]1[OH:18]
CCC(=O)O.CCCc1ccc(O)c(CCC)c1F
CCCc1cc(C(=O)CC)c(F)c(CCC)c1O
null
null
null
Functional Group Interconversion
OtherReaction
226287c5381c26952dfe91dfeb9f272de32d3e5724429362f80e36413cbcbe19
fdd617d504c91eca46103a55d487a57bf4aee64556f8d813b4f116bc72575b31
c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C;D1;H3:4].[C:5]-[c:6]1:[c;H0;D3;+0:7](-[OH;D1;+0:8]):[cH;D2;+0:9]:[c:10]:[c:11](-[C:12]):[c;H0;D3;+0:13]:1-[F;H0;D1;+0:14]>>[C:5]-[c:6]1:[c;H0;D3;+0:7](-[F;H0;D1;+0:14]):[c;H0;D3;+0:9](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C;D1;H3:4]):[c:10]:[c:11](-[C:12]):[c;H0;D3;+0:13]:1-[OH;D1...
null
[]
null
null
null
null
Propionic acid (9.07 g, 123 mmol) and 3-fluoro-2,4-dipropylphenol (9.60 g, 49.0 mmol) were mixed in trifluoromethanesulfonic acid (50 mL) as in Example 13, step 1. Purification by chramotography on silica gel using ethyl acetate:hexane (10:90) gave the title compound as a white solid. Conditions: See reaction.notes.pro...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carboxylic acid.Aromatic alcohol
Aromatic halide.Ketone.Aromatic alcohol
c1ccccc1
c1ccccc1
c1ccccc1
HO-
null
null
null
CCC(=O)O.CCCc1ccc(O)c(CCC)c1F>>CCCc1cc(C(=O)CC)c(F)c(CCC)c1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e82600096dac46b5b34ea78698e65332
O=S(=O)(Cl)CC(F)(F)F.[NH4+]>>NS(=O)(=O)CC(F)(F)F
C(F)(F)(F)CS(=O)(=O)Cl.[NH4+].[OH-]>>C(F)(F)(F)CS(=O)(=O)N
Cl[S:2](=[O:3])(=[O:4])[CH2:5][C:6]([F:7])([F:8])[F:9].[NH4+:1]>>[NH2:1][S:2](=[O:3])(=[O:4])[CH2:5][C:6]([F:7])([F:8])[F:9]
O=S(=O)(Cl)CC(F)(F)F.[NH4+]
NS(=O)(=O)CC(F)(F)F
null
null
O.C(Cl)Cl
Functional Group Interconversion
OtherReaction
76fbc3582e2f63736dd65176b79ffad31881adfa34415872457e21307ad3c8dc
8d9fe3486c870d18f12e4e21ee2410d7c9641745d38b34bc61fa11f384cef528
null
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[C:4]-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[F;D1;H0:8].[NH4+;D0:9]>>[F;D1;H0:6]-[C:5](-[F;D1;H0:7])(-[F;D1;H0:8])-[C:4]-[S;H0;D4;+0:1](-[NH2;D1;+0:9])(=[O;D1;H0:2])=[O;D1;H0:3]
null
[]
null
null
null
null
The CF3CH2SO2NH2 was prepared by cooling a solution of commercially available CF3CH2SO2Cl (0.6 ml, 1 eq) in CH2Cl2 to 0° C. NH4OH (0.75 ml, 14.8 N, 2 eq) was then added dropwise. The mixture was allowed to warm to room temperature overnight. The reaction was diluted with water and extracted three times with CH2Cl2. The...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
Sulfonamide
null
null
null
HCl
O.C(Cl)Cl
null
null
O=S(=O)(Cl)CC(F)(F)F.[NH4+]>O.C(Cl)Cl>NS(=O)(=O)CC(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-38a9717950d0440ea0c81b2cb1362db2
CCOC(=O)Cc1cccnc1.O=C1CCC(=O)N1Br>>CCOC(=O)C(Br)c1cccnc1
BrN1C(CCC1=O)=O.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].N1=CC(=CC=C1)CC(=O)OCC.Cl[Si](C)(C)C>>BrC(C(=O)OCC)C=1C=NC=CC1
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][c:8]1[cH:9][cH:10][cH:11][n:12][cH:13]1.O=C1CCC(=O)N1[Br:7]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]([Br:7])[c:8]1[cH:9][cH:10][cH:11][n:12][cH:13]1
CCOC(=O)Cc1cccnc1.O=C1CCC(=O)N1Br
CCOC(=O)C(Br)c1cccnc1
null
null
C1CCOC1.O
Functional Group Interconversion
Wohl-Ziegler bromination benzyl secondary
3f38b5884dced4ec8dd37f9fecb8c81145add99f2a1017bd9519b1712776da1f
9deb701e8012c4f1578ccc05651bfed620e4410cab5fedb649aa1ac30c26adec
c1ccncc1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[C:2]-[#8:3]-[C:4](=[O;D1;H0:5])-[CH2;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]>>[Br;H0;D1;+0:1]-[CH;D3;+0:6](-[C:4](=[O;D1;H0:5])-[#8:3]-[C:2])-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]
null
[]
-78
CELSIUS
20
MINUTE
Ethyl 3-pyridylacetate (1.0 g, 1.0 eq) was dissolved in THF (50 mL) and cooled to −78° C. Lithium bis (trimethylsilyl) amide (6.66 mL, 1.1 eq) was added to the reaction and stirred for 20 minutes. Chlorotrimethylsilane (1.44 mL, 1.875 eq) was added at −78° C. and stirred for 20 minutes. N-bromosuccinimide (1.09 g, 1.01...
10.6084/m9.figshare.5104873.v1
null
Ester.Tertiary amide.Tertiary amide
Secondary halide
C1CCNC1
null
c1ccncc1
HO-
C1CCOC1.O
-78
0.333333
CCOC(=O)Cc1cccnc1.O=C1CCC(=O)N1Br>C1CCOC1.O>CCOC(=O)C(Br)c1cccnc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1782f4c6e18d44388356e24fbc39135b
C=CCBr.CC(C)=O.Oc1ccc(OCc2ccccc2)cc1>>C=CCc1cc(OCc2ccccc2)cc(CC=C)c1O
C(C1=CC=CC=C1)OC1=CC=C(C=C1)O.C(C=C)Br.C(=O)([O-])[O-].[K+].[K+].CC(=O)C>>C(C=C)C1=C(C(=CC(=C1)OCC1=CC=CC=C1)CC=C)O
Br[CH2:17][CH:18]=[CH2:19].O=[C:2]([CH3:1])[CH3:3].[cH:4]1[cH:5][c:6]([O:7][CH2:8][c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[cH:15][cH:16][c:20]1[OH:21]>>[CH2:1]=[CH:2][CH2:3][c:4]1[cH:5][c:6]([O:7][CH2:8][c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[cH:15][c:16]([CH2:17][CH:18]=[CH2:19])[c:20]1[OH:21]
C=CCBr.CC(C)=O.Oc1ccc(OCc2ccccc2)cc1
C=CCc1cc(OCc2ccccc2)cc(CC=C)c1O
null
null
null
C-C Coupling
OtherReaction
c5e563466469107a02e912fa2c3d047d92bc0bea0e97fbdca3bf7287a82c7c13
e47cdb53db8bcaa27a4325516a44570d192da6f35ef9365fa43284d4b56f7d79
c1ccc(COc2ccccc2)cc1
Br-[CH2;D2;+0:1]-[C:2]=[C;D1;H2:3].O=[C;H0;D3;+0:4](-[CH3;D1;+0:5])-[CH3;D1;+0:6].[O;D1;H1:7]-[c:8]1:[cH;D2;+0:9]:[c:10]:[c:11]:[c:12]:[cH;D2;+0:13]:1>>[C;D1;H2:3]=[C:2]-[CH2;D2;+0:1]-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[c:12]:[c;H0;D3;+0:13](-[CH2;D2;+0:6]-[CH;D2;+0:4]=[CH2;D1;+0:5]):[c:8]:1-[O;D1;H1:7]
null
[]
null
null
null
null
To a solution of starting 4-benzyloxyphenol (20 g) in acetone (800 mL) were added allylbromide (50 mL) and K2CO3 (60 g). The reaction mixture was refluxed overnight. After cooling to the room temperature, the insoluble materials were removed by filtration. The filtrate was concentrated in vac. The residue was partition...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Allyl
Allyl.Allyl
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HBr
null
null
null
C=CCBr.CC(C)=O.Oc1ccc(OCc2ccccc2)cc1>>C=CCc1cc(OCc2ccccc2)cc(CC=C)c1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cbe90fa9d62e4ab79ebe977953f20624
C=CCc1cc(OCc2ccccc2)cc(CC=C)c1O.COC(=O)C(Br)c1ccc(Cl)cc1>>C=CCc1cc(O)cc(CC=C)c1OC(C(=O)OC)c1ccc(Cl)cc1
CCOCC.C(C=C)C1=C(C(=CC(=C1)OCC1=CC=CC=C1)CC=C)O.BrC(C(=O)OC)C1=CC=C(C=C1)Cl.C(=O)([O-])[O-].[Cs+].[Cs+]>>C(C=C)C1=C(OC(C(=O)OC)C2=CC=C(C=C2)Cl)C(=CC(=C1)O)CC=C
c1ccc(C[O:7][c:6]2[cH:5][c:4]([CH2:3][CH:2]=[CH2:1])[c:13]([OH:14])[c:9]([CH2:10][CH:11]=[CH2:12])[cH:8]2)cc1.Br[CH:15]([C:16](=[O:17])[O:18][CH3:19])[c:20]1[cH:21][cH:22][c:23]([Cl:24])[cH:25][cH:26]1>>[CH2:1]=[CH:2][CH2:3][c:4]1[cH:5][c:6]([OH:7])[cH:8][c:9]([CH2:10][CH:11]=[CH2:12])[c:13]1[O:14][CH:15]([C:16](=[O:17...
C=CCc1cc(OCc2ccccc2)cc(CC=C)c1O.COC(=O)C(Br)c1ccc(Cl)cc1
C=CCc1cc(O)cc(CC=C)c1OC(C(=O)OC)c1ccc(Cl)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
53f85fb4df1ea6f44f3a294e10703f62f089f6e01b80df7715f3e9b212492d83
548bf445f48f5c4b6c7dcf37d92ce8ff2e6db460b8f4bcaf9e4dc8979044834f
c1ccc(COc2ccccc2)cc1
Br-[CH;D3;+0:1](-[C:2](=[O;D1;H0:3])-[#8:4]-[C;D1;H3:5])-[c:6](:[c:7]):[c:8].[OH;D1;+0:9]-[c:10]1:[c:11]:[c:12]:[c:13](-[O;H0;D2;+0:14]-C-c2:c:c:c:c:c:2):[c:15]:[c:16]:1>>[C;D1;H3:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[CH;D3;+0:1](-[O;H0;D2;+0:9]-[c:10]1:[c:11]:[c:12]:[c:13](-[OH;D1;+0:14]):[c:15]:[c:16]:1)-[c:6](:[c:7]):[c:8]
null
[]
null
null
15
HOUR
To a solution of 2,6-diallyl-4-benzyloxyphenol (200 mg, 1.0 eq) in DMF (8 mL) were added methyl α-bromo-4-chlorobenzeneacetate (190 mg, 1.0 eq) and Cs2CO3 (285 mg, 1.2 eq). The reaction mixture was stirred at room temperature for 15 h, poured into ether, washed with water and brine, dried over MgSO4, filtered, and conc...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ester.Ether.Aromatic alcohol
Ester.Ether.Aromatic alcohol
c1ccccc1
null
c1ccccc1.c1ccccc1
HBr
CN(C)C=O
null
15
C=CCc1cc(OCc2ccccc2)cc(CC=C)c1O.COC(=O)C(Br)c1ccc(Cl)cc1>CN(C)C=O>C=CCc1cc(O)cc(CC=C)c1OC(C(=O)OC)c1ccc(Cl)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-de8f73a85c194ba78978de97959b81eb
CC(=O)c1ccc(F)cc1O.O=C(O)Cc1ccc(Cl)cc1>>O=c1ccc2ccccc2o1
C([O-])([O-])=O.[K+].[K+].CC(=O)C1=C(C=C(C=C1)F)O.ClC1=CC=C(C=C1)CC(=O)O.C1=CN(C=N1)C(=O)N2C=CN=C2>>O1C(C=CC2=C1C=CC=C2)=O
O=[C:4]([CH3:3])[c:5]1[cH:6][cH:7][c:8](F)[cH:9][c:10]1[OH:11].O[C:2](Cc1ccc(Cl)cc1)=[O:1]>>[O:1]=[c:2]1[cH:3][cH:4][c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[o:11]1
CC(=O)c1ccc(F)cc1O.O=C(O)Cc1ccc(Cl)cc1
O=c1ccc2ccccc2o1
null
CN(C)C=1C=CN=CC1
O.CN(C)C=O
Miscellaneous
OtherReaction
4e101e46a19ea3ee90b3fc9c267be5b135c81127def38ae3bbc651741dd6f969
d0c273f5c25e93056ec27ba8a414d05032b56c89b0bcca1a7efb3a560218b0dc
O=c1ccc2ccccc2o1
Cl-c1:c:c:c(-C-[C;H0;D3;+0:1](-O)=[O;D1;H0:2]):c:c:1.F-[c;H0;D3;+0:3]1:[c:4]:[c:5]:[c:6](-[C;H0;D3;+0:7](=O)-[CH3;D1;+0:8]):[c:9](-[OH;D1;+0:10]):[c:11]:1>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[cH;D2;+0:8]:[cH;D2;+0:7]:[c:6]2:[c:5]:[c:4]:[cH;D2;+0:3]:[c:11]:[c:9]:2:[o;H0;D2;+0:10]:1
38
[{"value": 38.0, "product": "O1C(C=CC2=C1C=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 37.0, "product": "O1C(C=CC2=C1C=CC=C2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
A solution of 4-chlorophenylacetic acid (11.05 g, 64.8 mmol) in DMF (100 mL) was treated with CDI (13.13 g, 81 mmol) in several portions over about 15 minutes and the mixture was stirred until gas evolution had ceased. 4-Fluoro-2-hydroxyacetophenone (5.0 g, 32.4 mmol) was added followed by potassium carbonate (15.7 g, ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Carboxylic acid.Ketone.Aromatic alcohol
null
c1ccccc1.c1ccccc1
c1ccc2ccccc2o1
c1ccc2ccccc2o1
HF
CN(C)C=1C=CN=CC1.O.CN(C)C=O
80
null
CC(=O)c1ccc(F)cc1O.O=C(O)Cc1ccc(Cl)cc1>CN(C)C=1C=CN=CC1.O.CN(C)C=O>O=c1ccc2ccccc2o1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-61a939bb8ae141e4bb2ed9c3a947327d
CC(C)[CH2][Mg][Br].OC1CCC=C1Br>>CC(C)CC1=CCCC1O
BrC=1C(CCC1)O.BrC=1C(CCC1)O.C(C(C)C)[Mg]Br>>C(C(C)C)C=1C(CCC1)O
[Br][Mg][CH2:4][CH:2]([CH3:1])[CH3:3].Br[C:5]1=[CH:6][CH2:7][CH2:8][CH:9]1[OH:10]>>[CH3:1][CH:2]([CH3:3])[CH2:4][C:5]1=[CH:6][CH2:7][CH2:8][CH:9]1[OH:10]
CC(C)[CH2][Mg][Br].OC1CCC=C1Br
CC(C)CC1=CCCC1O
null
[Ni](Cl)Cl.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1
C1CCOC1
C-C Coupling
OtherReaction
db82bbef8df76a2432f2b7b688121f836580d3a5c6da8087deb078cabef2b073
25890778c2a34dbd8a57fb42f469f5e416c2ea4b1399554507deb7ca9b3263b7
C1=CCCC1
Br-[C;H0;D3;+0:1]1=[C:2]-[C:3]-[C:4]-[C:5]-1-[O;D1;H1:6].[Br]-[Mg]-[CH2;D2;+0:7]-[C:8](-[C;D1;H3:9])-[C;D1;H3:10]>>[C;D1;H3:9]-[C:8](-[C;D1;H3:10])-[CH2;D2;+0:7]-[C;H0;D3;+0:1]1=[C:2]-[C:3]-[C:4]-[C:5]-1-[O;D1;H1:6]
null
[]
null
null
null
null
The alcohol (Intermediate D3, 16 mmol) in THF (30 mL) at 0° C. was treated with isobutyl magnesium bromide (40 mmol). The catalyst, 1,3-bis(diphenylphosphino)propane nickel (II) chloride (0.75 mmol) (NiCl2dppp) was added in one portion and the mixture was heated to reflux for 3 h. (see: Organ et al. J. Org. Chem. 1997,...
10.6084/m9.figshare.5104873.v1
null
Magnesium halide.Alkenyl halide
null
C1=CCCC1
C1=CCCC1
C1=CCCC1
Br-.Mg
[Ni](Cl)Cl.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1
null
null
CC(C)[CH2][Mg][Br].OC1CCC=C1Br>[Ni](Cl)Cl.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1>CC(C)CC1=CCCC1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c6bac18ad000457ea6e76f93c42ca587
C1=COCCC1.Cc1ccc(S(=O)(=O)[O-])cc1.[O]=[Cr](=[O])([O-])[Cl].c1cc[nH+]cc1>>O=C1CCCc2cccc(COC3CCCCO3)c21
O1CCCC=C1.C1(=CC=C(C=C1)S(=O)(=O)[O-])C.[NH+]1=CC=CC=C1.[Cr](=O)(=O)([O-])Cl.[NH+]1=CC=CC=C1.C(C)(=O)[O-].[Na+]>>O1C(CCCC1)OCC=1C=CC=C2CCCC(C12)=O
[CH:13]1=[CH:14][CH2:15][CH2:16][CH2:17][O:18]1.O=S(=O)([O-:1])[c:2]1[cH:3]c[c:5]([CH3:4])[cH:6][cH:19]1.[O]=[Cr](=[O])([Cl])[O-:12].[nH+]1[cH:7][cH:8][cH:9][cH:10][cH:11]1>>[O:1]=[C:2]1[CH2:3][CH2:4][CH2:5][c:6]2[cH:7][cH:8][cH:9][c:10]([CH2:11][O:12][CH:13]3[CH2:14][CH2:15][CH2:16][CH2:17][O:18]3)[c:19]21
C1=COCCC1.Cc1ccc(S(=O)(=O)[O-])cc1.[O]=[Cr](=[O])([O-])[Cl].c1cc[nH+]cc1
O=C1CCCc2cccc(COC3CCCCO3)c21
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
7601df4ebe7c8306f678a974b9a4f6c9dd5bbe853665a3a426ff89543189bf7c
28bca55dec68c7a0c75759f892decdd5bb046fceea560a720b79b673ac13228a
O=C1CCCc2cccc(COC3CCCCO3)c21
O=S(=O)(-[O-;H0;D1:1])-[c;H0;D3;+0:2]1:[cH;D2;+0:3]:[cH;D2;+0:4]:[c;H0;D3;+0:5](-[CH3;D1;+0:6]):c:[cH;D2;+0:7]:1.[#8:8]1-[C:9]-[C:10]-[C:11]-[CH;D2;+0:12]=[CH;D2;+0:13]-1.[Cl]-[Cr](-[O-;H0;D1:14])(=[O])=[O].[c:15]1:[c:16]:[cH;D2;+0:17]:[cH;D2;+0:18]:[nH+]:[cH;D2;+0:19]:1>>[O;H0;D1;+0:1]=[C;H0;D3;+0:2]1-[CH2;D2;+0:7]-[C...
55
[{"value": 55.0, "product": "O1C(CCCC1)OCC=1C=CC=C2CCCC(C12)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The diol (Intermediate H3) (2.42 g, 13.5 mmol) was dissolved in CH2Cl2 (75 mL) and reacted with dihydropyran (1.3 mL, 13.8 mmol) and pyridinium para-toluene sulfonate (PPTS) (350 mg, 1.36 mmol) at rt for 18 h. The mixture was concentrated onto SiO2 and purified by chromatography with 10% EtOAc:Hx. The tetrahydropyranyl...
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null
Tosylate.Ether
Ketone.Ether.Ether
C1=COCCC1.c1ccccc1.c1cc[n+]cc1
c1ccc2c(c1)CCCC2.C1CCOCC1
c1ccc2c(c1)CCCC2.C1CCOCC1
TsOH.HCl
C(Cl)Cl
null
null
C1=COCCC1.Cc1ccc(S(=O)(=O)[O-])cc1.[O]=[Cr](=[O])([O-])[Cl].c1cc[nH+]cc1>C(Cl)Cl>O=C1CCCc2cccc(COC3CCCCO3)c21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5a9e347455ad418da520a0da2e094ddc
CC(=O)Cl.Nc1cccc2c1CCCC2.[O]=[Mn](=[O])(=[O])[O-]>>CC(=O)Nc1cccc2c1C(=O)CCC2
[NH4+].[Cl-].C(C)(=O)Cl.[O-]S(=O)(=O)[O-].[Mg+2].[O-][Mn](=O)(=O)=O.[K+].C1(=CC=CC=2CCCCC12)N>>O=C1CCCC=2C=CC=C(C12)NC(C)=O
Cl[C:2]([CH3:1])=[O:3].[NH2:4][c:5]1[cH:6][cH:7][cH:8][c:9]2[c:10]1[CH2:11][CH2:13][CH2:14][CH2:15]2.[O]=[Mn](=[O])([O-])=[O:12]>>[CH3:1][C:2](=[O:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][c:9]2[c:10]1[C:11](=[O:12])[CH2:13][CH2:14][CH2:15]2
CC(=O)Cl.Nc1cccc2c1CCCC2.[O]=[Mn](=[O])(=[O])[O-]
CC(=O)Nc1cccc2c1C(=O)CCC2
null
null
CC(=O)C.O.CCN(CC)CC.C(Cl)(Cl)Cl.C(Cl)Cl
Protection
OtherReaction
767d72dbcbd04e343c1d04bfc4316ff2bb75efa0566f9b21c8dfa71cf6c6a001
89aefbfb6f78410748f2a731669640d685ca87237e823b898811a79392e6c255
O=C1CCCc2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5]-[CH2;D2;+0:6]-[c:7](:[c:8]):[c:9](-[NH2;D1;+0:10]):[c:11].[O-]-[Mn](=[O;H0;D1;+0:12])(=[O])=[O]>>[C:4]-[C:5]-[C;H0;D3;+0:6](=[O;H0;D1;+0:12])-[c:7](:[c:8]):[c:9](-[NH;D2;+0:10]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]):[c:11]
null
[]
0
CELSIUS
2
HOUR
5,6,7,8-Tetrahydro-naphthalen-1-ylamine (Intermediate J1, commercially available from Aldrich) (5 mL, 35.3 mmol) was dissolved in CH2Cl2 (40 mL) and treated with NEt3 (10 mL) and acetyl chloride (3.8 mL, 53 mmol) at rt for 1 h. The mixture was diluted in CHCl3 and acidified with sat NH4Cl. The aqueous layer was extract...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Ketone.Secondary amide
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
HCl
CC(=O)C.O.CCN(CC)CC.C(Cl)(Cl)Cl.C(Cl)Cl
0
2
CC(=O)Cl.Nc1cccc2c1CCCC2.[O]=[Mn](=[O])(=[O])[O-]>CC(=O)C.O.CCN(CC)CC.C(Cl)(Cl)Cl.C(Cl)Cl>CC(=O)Nc1cccc2c1C(=O)CCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cb8706557d35427e999736d01fcd803a
CC(=O)Nc1cccc2c1C(=O)CCC2>>Nc1cccc2c1C(=O)CCC2
O=C1CCCC=2C=CC=C(C12)NC(C)=O.C(=O)([O-])[O-].[Na+].[Na+].[OH-].[Na+]>>NC=1C=CC=C2CCCC(C12)=O
CC(=O)[NH:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[C:8](=[O:9])[CH2:10][CH2:11][CH2:12]2>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[C:8](=[O:9])[CH2:10][CH2:11][CH2:12]2
CC(=O)Nc1cccc2c1C(=O)CCC2
Nc1cccc2c1C(=O)CCC2
null
null
Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
755df58c254dea764fdda078ffd678ec540bba057c83683be04c253f1270ac7b
025f7cefe51e71668ad5d09fca32df168e9b538347403e4d5c1748073e538adc
O=C1CCCc2ccccc21
C-C(=O)-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5]=[O;D1;H0:6]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]-[C:5]=[O;D1;H0:6]
56
[{"value": 56.0, "product": "NC=1C=CC=C2CCCC(C12)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 55.6, "product": "NC=1C=CC=C2CCCC(C12)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The amide (Intermediate J2, 4.12 g, 20.3 mmol) was heated at 90° C. in 6N HCl (140 mL) for 3 h. The mixture was cooled to rt and Na2CO3 was added in small portions followed by addition of 2N NaOH until the mixture was at pH 8. The aqueous layer was extracted with EtOAc and the organic fractions were combined, washed wi...
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null
Secondary amide
Primary amine
null
null
c1ccc2c(c1)CCCC2
HO-
Cl
null
null
CC(=O)Nc1cccc2c1C(=O)CCC2>Cl>Nc1cccc2c1C(=O)CCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a8ca59da901b4226a81b5c7540f40e6a
FB(F)F.Nc1cccc2c1C(=O)CCC2>>O=C1CCCc2cccc(F)c21
N(=O)OC(C)(C)C.NC=1C=CC=C2CCCC(C12)=O.B(F)(F)F.CCOCC>>FC=1C=CC=C2CCCC(C12)=O
FB(F)[F:11].N[c:10]1[cH:9][cH:8][cH:7][c:6]2[c:12]1[C:2](=[O:1])[CH2:3][CH2:4][CH2:5]2>>[O:1]=[C:2]1[CH2:3][CH2:4][CH2:5][c:6]2[cH:7][cH:8][cH:9][c:10]([F:11])[c:12]21
FB(F)F.Nc1cccc2c1C(=O)CCC2
O=C1CCCc2cccc(F)c21
null
null
C(Cl)Cl.CCCCC
Functional Group Interconversion
OtherReaction
3ef279fffa325c85794079ae07ad71ae4cf8f50c0b924a8c49d6ef3025178107
9c224743a26d9e1c3135e4817dd611aec414d8ea156f02200a3aef865be78b01
O=C1CCCc2ccccc21
F-B(-F)-[F;H0;D1;+0:1].N-[c;H0;D3;+0:2](:[c:3]:[c:4]):[c:5](:[c:6])-[C:7](=[O;D1;H0:8])-[C:9]>>[C:9]-[C:7](=[O;D1;H0:8])-[c:5](:[c:6]):[c;H0;D3;+0:2](-[F;H0;D1;+0:1]):[c:3]:[c:4]
null
[]
0
CELSIUS
10
MINUTE
The amine (Intermediate J3, 1.83 g, 11.3 mmol) in CH2Cl2 (17 mL) was added to BF3.OEt2 (2.80 mL, 22.1 mmol) at −15° C. More CH2Cl2 (20 mL) was added to the precipitate. Next, t-butyl nitrite (1.8 mL, 12.9 mmol) in CH2Cl2 (20 mL) was added at −15° C. and stirred for 10 min. and at 0° C. for 20 m. The mixture was diluted...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Aromatic halide
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
HF.B
C(Cl)Cl.CCCCC
0
0.166667
FB(F)F.Nc1cccc2c1C(=O)CCC2>C(Cl)Cl.CCCCC>O=C1CCCc2cccc(F)c21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2e74f4b9a84246f1b5d7ef55e09714c0
c1ccc(COCCC2CCC3(CC2)OCCO3)cc1>>O=C1CCC(CCOCc2ccccc2)CC1
C(C1=CC=CC=C1)OCCC1CCC2(OCCO2)CC1.O.CC=1C=CC(=CC1)S(=O)(=O)O>>C(C1=CC=CC=C1)OCCC1CCC(CC1)=O
C1C[O:1][C:2]2(O1)[CH2:3][CH2:4][CH:5]([CH2:6][CH2:7][O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)[CH2:16][CH2:17]2>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([CH2:6][CH2:7][O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[CH2:16][CH2:17]1
c1ccc(COCCC2CCC3(CC2)OCCO3)cc1
O=C1CCC(CCOCc2ccccc2)CC1
null
null
CC(=O)C
Miscellaneous
Ketal hydrolysis to ketone
7165849453c1f3f22c37497ec202aa2a6a319b018b3ae9fffa16fa9182ebd128
547697208447432e865290cf95eed8e4fcddc12f59856b7ddbf24dc1accb1210
O=C1CCC(CCOCc2ccccc2)CC1
[C:1]-[C:2]-[C;H0;D4;+0:3]1(-O-C-C-[O;H0;D2;+0:4]-1)-[C:5]-[C:6]>>[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[C:5]-[C:6]
97
[{"value": 97.0, "product": "C(C1=CC=CC=C1)OCCC1CCC(CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
8-(2-Benzyloxy-ethyl)-1,4-dioxa-spiro[4.5]decane (Intermediate K1, 1.02 g, 3.70 mmol) (prepared in accordance with the publication Ciufolini et. al. J. Amer. Chem. Soc. 1991, 113, 8016, incorporated herein by reference) was dissolved in acetone (100 mL): H2O (5 mL) and reacted with TsOH (140 mg, 0.74 mmol) at 45° C. fo...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Ketone
C1CCC2(CC1)OCCO2
C1CCCCC1
C1CCCCC1.c1ccccc1
HO-
CC(=O)C
null
null
c1ccc(COCCC2CCC3(CC2)OCCO3)cc1>CC(=O)C>O=C1CCC(CCOCc2ccccc2)CC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-37e41d6c8bde4a8c90ee4691de966a73
COC(=O)C#N.O=C1CCC(CCOCc2ccccc2)CC1>>COC(=O)C1CCCCC1
C(#N)C(=O)OC.CN(C)P(=O)(N(C)C)N(C)C.[Li+].CC(C)[N-]C(C)C.C(C1=CC=CC=C1)OCCC1CCC(CC1)=O>>COC(=O)C1CCCCC1
N#C[C:3]([O:2][CH3:1])=[O:4].O=[C:8]1[CH2:7][CH2:6][CH:5](CCOCc2ccccc2)[CH2:10][CH2:9]1>>[CH3:1][O:2][C:3](=[O:4])[CH:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1
COC(=O)C#N.O=C1CCC(CCOCc2ccccc2)CC1
COC(=O)C1CCCCC1
null
null
C1CCOC1
C-C Coupling
OtherReaction
928e825e225c84955bd59aed5069293c703110ef34100e7e6a88abac42c39cf7
e6602ab2673207a87d130997833085ef464dfa62e8dfa722678056077bfe8908
C1CCCCC1
N#C-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].O=[C;H0;D3;+0:5]1-[C:6]-[C:7]-[CH;D3;+0:8](-C-C-O-C-c2:c:c:c:c:c:2)-[C:9]-[C:10]-1>>[C;D1;H3:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH;D3;+0:8]1-[C:9]-[C:10]-[CH2;D2;+0:5]-[C:6]-[C:7]-1
null
[]
0
CELSIUS
null
null
A solution of LDA (33 ml, 1.5 M in Et2O) in THF (50 mL) at −78° C. was treated with 4-(2-benzyloxy-ethyl)-cyclohexanone (9.5 g, 40.2 mmol). The mixture was warmed to 0° C. over 30 min. before re-cooling to −78° C. and adding HMPA (7 mL). Methyl cyanoformate (CNCO2Me, 4.1 mL, 85 mmol) was added and the mixture was stirr...
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null
Ketone.Ester.Ether.Nitrile
Ester
C1CCCCC1.c1ccccc1
C1CCCCC1
C1CCCCC1
HO-
C1CCOC1
0
null
COC(=O)C#N.O=C1CCC(CCOCc2ccccc2)CC1>C1CCOC1>COC(=O)C1CCCCC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-16fa2f13876a42159089e1648883c1e5
CCI.COC(=O)C1CC(CCOCc2ccccc2)CCC1=O>>CCC1(C(=O)OC)CC(CCOCc2ccccc2)CCC1=O
COC(=O)C1C(CCC(C1)CCOCC1=CC=CC=C1)=O.C[O-].[Na+].C[O-].[Na+].C(C)I.ICC>>COC(=O)C1(C(CCC(C1)CCOCC1=CC=CC=C1)=O)CC
I[CH2:2][CH3:1].[CH:3]1([C:4](=[O:5])[O:6][CH3:7])[CH2:8][CH:9]([CH2:10][CH2:11][O:12][CH2:13][c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[CH2:20][CH2:21][C:22]1=[O:23]>>[CH3:1][CH2:2][C:3]1([C:4](=[O:5])[O:6][CH3:7])[CH2:8][CH:9]([CH2:10][CH2:11][O:12][CH2:13][c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[CH2:20][CH2:21...
CCI.COC(=O)C1CC(CCOCc2ccccc2)CCC1=O
CCC1(C(=O)OC)CC(CCOCc2ccccc2)CCC1=O
null
null
CO
C-C Coupling
OtherReaction
deecb6e0e045bc39174217ca5e58aac9964e4446522d6e6b0f2101d43cb988e9
61bad66347ae366bfd0a2cd3779dd3d0c29125e97564b97243e11258be3b2a9f
O=C1CCC(CCOCc2ccccc2)CC1
I-[CH2;D2;+0:1]-[C;D1;H3:2].[C:3]-[C:4](=[O;D1;H0:5])-[CH;D3;+0:6](-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10])-[C:11]-[C:12]>>[C:3]-[C:4](=[O;D1;H0:5])-[C;H0;D4;+0:6](-[CH2;D2;+0:1]-[C;D1;H3:2])(-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10])-[C:11]-[C:12]
null
[]
null
null
48
HOUR
A mixture of 5-(2-benzyloxy-ethyl)-2-oxo-cyclohexanecarboxylic acid methyl ester in anhydrous MeOH (10 mL) was reacted with NaOMe solution (16.6 mL, 8.28 mmol) at rt for 15 min. Iodoethane (2.76 mL, 34.5 mmol) was added via syringe and the mixture was stored at rt for 48 h. Another portion of NaOMe (8.3 mmol) and EtI (...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone
Ketone.Ester
C1CCCCC1
C1CCCCC1
C1CCCCC1.c1ccccc1
HI
CO
null
48
CCI.COC(=O)C1CC(CCOCc2ccccc2)CCC1=O>CO>CCC1(C(=O)OC)CC(CCOCc2ccccc2)CCC1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a5132735e67540d7a278e6269fdf07ee
CCC1CC(CCOCc2ccccc2)CCC1(C)O>>CCC1=C(C)CCC(CCOCc2ccccc2)C1
C(C1=CC=CC=C1)OCCC1CC(C(CC1)(O)C)CC.S(=O)(=O)(C1=CC=C(C)C=C1)O.O.[O-]S(=O)(=O)[O-].[Mg+2]>>C(C)C=1CC(CCC1C)CCOCC1=CC=CC=C1
O[C:4]1([CH3:5])[CH:3]([CH2:2][CH3:1])[CH2:19][CH:8]([CH2:9][CH2:10][O:11][CH2:12][c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[CH2:7][CH2:6]1>>[CH3:1][CH2:2][C:3]1=[C:4]([CH3:5])[CH2:6][CH2:7][CH:8]([CH2:9][CH2:10][O:11][CH2:12][c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[CH2:19]1
CCC1CC(CCOCc2ccccc2)CCC1(C)O
CCC1=C(C)CCC(CCOCc2ccccc2)C1
null
null
C1=CC=CC=C1
Functional Group Interconversion
OtherReaction
bb751e8d8bac081516d1433e6fec088b316018c4b9e2465f1f9c878bad0b1e7c
63e4ba80024292782b5f87f96975225484dff39f49e96eea21874ac0cd9091a0
C1=CCC(CCOCc2ccccc2)CC1
O-[C;H0;D4;+0:1]1(-[C;D1;H3:2])-[C:3]-[C:4]-[C:5]-[C:6]-[CH;D3;+0:7]-1-[C:8]-[C;D1;H3:9]>>[C;D1;H3:9]-[C:8]-[C;H0;D3;+0:7]1=[C;H0;D3;+0:1](-[C;D1;H3:2])-[C:3]-[C:4]-[C:5]-[C:6]-1
71
[{"value": 71.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 5-(2-benzyloxy-ethyl)-2-oxo-cyclohexanecarboxylic acid methyl ester in anhydrous MeOH (10 mL) was reacted with NaOMe solution (16.6 mL, 8.28 mmol) at rt for 15 min. Iodoethane (2.76 mL, 34.5 mmol) was added via syringe and the mixture was stored at rt for 48 h. Another portion of NaOMe (8.3 mmol) and EtI (...
10.6084/m9.figshare.5104873.v1
null
Tertiary alcohol
null
C1CCCCC1
C1=CCCCC1
C1=CCCCC1.c1ccccc1
HO-
C1=CC=CC=C1
null
null
CCC1CC(CCOCc2ccccc2)CCC1(C)O>C1=CC=CC=C1>CCC1=C(C)CCC(CCOCc2ccccc2)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-453edea139244baf9c9ab10628a42515
CCC1CC(CCOCc2ccccc2)CCC1(C)O>>CCC1=C(C)CCC(CC=O)C1
C(C1=CC=CC=C1)OCCC1CC(C(CC1)(O)C)CC.CCN(CC)CC.C(C1=CC=CC=C1)OCCC1CC(C(CC1)(O)C)CC.C(C(=O)Cl)(=O)Cl.CS(=O)C>>C(C)C=1CC(CCC1C)CC=O
O[C:4]1([CH3:5])[CH:3]([CH2:2][CH3:1])[CH2:12][CH:8]([CH2:9][CH2:10][O:11]Cc2ccccc2)[CH2:7][CH2:6]1>>[CH3:1][CH2:2][C:3]1=[C:4]([CH3:5])[CH2:6][CH2:7][CH:8]([CH2:9][CH:10]=[O:11])[CH2:12]1
CCC1CC(CCOCc2ccccc2)CCC1(C)O
CCC1=C(C)CCC(CC=O)C1
null
null
C(Cl)Cl
Functional Group Interconversion
OtherReaction
be4941a18e7a4255bfefcc67f8959fb712bcee80410bba3c57cbe2980db0414f
4426f7f4a41437378342710cbad6905f9467a7d2ab3100172eaffaec02d8e0f9
C1=CCCCC1
O-[C;H0;D4;+0:1]1(-[C;D1;H3:2])-[C:3]-[C:4]-[C:5](-[C:6]-[CH2;D2;+0:7]-[O;H0;D2;+0:8]-C-c2:c:c:c:c:c:2)-[C:9]-[CH;D3;+0:10]-1-[C:11]-[C;D1;H3:12]>>[C;D1;H3:12]-[C:11]-[C;H0;D3;+0:10]1=[C;H0;D3;+0:1](-[C;D1;H3:2])-[C:3]-[C:4]-[C:5](-[C:6]-[CH;D2;+0:7]=[O;H0;D1;+0:8])-[C:9]-1
null
[]
null
null
40
MINUTE
The deprotected alcohol was oxidized by the standard “Swern” procedure (Mancuso, Synthesis 1981 p165, incorporated herein by reference) as follows: The alcohol (5 mmol) was added to a solution of oxalyl chloride (3.5 mL, 7.0 mmol) in CH2Cl2 (30 mL) with DMSO (0.64 mL, 9.0 mmol) at −78° C. After 40 min., NEt3 (2.50 mL) ...
10.6084/m9.figshare.5104873.v1
null
Ether.Tertiary alcohol
Aldehyde
C1CCCCC1.c1ccccc1
C1=CCCCC1
C1=CCCCC1
HO-
C(Cl)Cl
null
0.666667
CCC1CC(CCOCc2ccccc2)CCC1(C)O>C(Cl)Cl>CCC1=C(C)CCC(CC=O)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d2ed4b52ee0845be8a8cce8c441467cb
CC(C)(C)[Si](C)(C)Cl.CN(C)S(=O)(=O)n1ccnc1>>CN(C)S(=O)(=O)n1ccnc1[Si](C)(C)C(C)(C)C
CN(S(=O)(=O)N1C=NC=C1)C.[Li]CCCC.[Si](C)(C)(C(C)(C)C)Cl>>CN(S(=O)(=O)N1C(=NC=C1)[Si](C)(C)C(C)(C)C)C
Cl[Si:12]([CH3:13])([CH3:14])[C:15]([CH3:16])([CH3:17])[CH3:18].[CH3:1][N:2]([CH3:3])[S:4](=[O:5])(=[O:6])[n:7]1[cH:8][cH:9][n:10][cH:11]1>>[CH3:1][N:2]([CH3:3])[S:4](=[O:5])(=[O:6])[n:7]1[cH:8][cH:9][n:10][c:11]1[Si:12]([CH3:13])([CH3:14])[C:15]([CH3:16])([CH3:17])[CH3:18]
CC(C)(C)[Si](C)(C)Cl.CN(C)S(=O)(=O)n1ccnc1
CN(C)S(=O)(=O)n1ccnc1[Si](C)(C)C(C)(C)C
null
null
C1CCOC1.O
Functional Group Interconversion
OtherReaction
2a4b40f1b9ebeb08c29f68284298974d85bccd40abdd83eda0860c5d43fa28d0
62b25486659a0c3b8981491307676661488416039e4a601c8996c7216be92cf1
c1c[nH]cn1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[#16:8]-[#7;a:9]1:[c:10]:[c:11]:[#7;a:12]:[cH;D2;+0:13]:1>>[#16:8]-[#7;a:9]1:[c:10]:[c:11]:[#7;a:12]:[c;H0;D3;+0:13]:1-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7]
null
[]
-78
CELSIUS
24
HOUR
Imidazole (Intermediate L1, available from Aldrich, 20.0 g, 0.29 mol), triethylamine (41.0 mL, 0.29 mol) and N,N-dimethylsulfamoyl chloride (31.6 mL, 0.29 mol) were added to benzene (320 mL). The reaction was stirred for 48 h at rt and then filtered. The filtrate was collected and concentrated under reduced pressure. V...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
Silyl protective group
c1c[nH]cn1
c1ncc[nH]1
c1ncc[nH]1
HCl
C1CCOC1.O
-78
24
CC(C)(C)[Si](C)(C)Cl.CN(C)S(=O)(=O)n1ccnc1>C1CCOC1.O>CN(C)S(=O)(=O)n1ccnc1[Si](C)(C)C(C)(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-34d736d2a0ea4ad099e56c5998df35eb
C=COCC.OC1CCC=C1Br>>C=COC1CCC=C1Br
BrC=1C(CCC1)O.BrC=1C(CCC1)O.C(=C)OCC>>BrC1=CCCC1OC=C
CCO[CH:2]=[CH2:1].[OH:3][CH:4]1[CH2:5][CH2:6][CH:7]=[C:8]1[Br:9]>>[CH2:1]=[CH:2][O:3][CH:4]1[CH2:5][CH2:6][CH:7]=[C:8]1[Br:9]
C=COCC.OC1CCC=C1Br
C=COC1CCC=C1Br
null
[Hg](OC(=O)C)OC(=O)C
null
Acylation
OtherReaction
9f1a8de39cf5a08a1f44abee84b9664c807b2fd8724957eb8629cb322ac3bf03
60fd153f0b02c0d51bbf266782eeb8125a802a18d05f2f324ecdcbf97326001e
C1=CCCC1
C-C-O-[CH;D2;+0:1]=[C;D1;H2:2].[Br;D1;H0:3]-[C:4]1=[C:5]-[C:6]-[C:7]-[C:8]-1-[OH;D1;+0:9]>>[Br;D1;H0:3]-[C:4]1=[C:5]-[C:6]-[C:7]-[C:8]-1-[O;H0;D2;+0:9]-[CH;D2;+0:1]=[C;D1;H2:2]
null
[]
null
null
null
null
A solution of 2-bromo-cyclopent-2-enol (Intermediate D3) (21.7 g, 133.1 mmol) in ethyl vinyl ether (300 mL) was treated with Hg(OAc)2 (31.8 g, 99 mmol) at rt for 60 h. The mixture was quenched with 5% NaOH (150 mL) and filtered through celite. The residue was concentrated to yield 1-bromo-5-vinyloxy-cyclopentene as a p...
10.6084/m9.figshare.5104873.v1
null
Ether.Secondary alcohol.Vinyl
Ether
null
null
C1=CCCC1
HO-
[Hg](OC(=O)C)OC(=O)C
null
null
C=COCC.OC1CCC=C1Br>[Hg](OC(=O)C)OC(=O)C>C=COC1CCC=C1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b08eddab25a944edabedd2575e1e1f78
COC(C)(OC)N(C)C.OC1CCC=C1Br>>CN(C)C(=O)CC1CCC=C1Br
BrC=1C(CCC1)O.BrC=1C(CCC1)O.COC(C)(N(C)C)OC>>BrC=1C(CCC1)CC(=O)N(C)C
CO[C:4]([N:2]([CH3:1])[CH3:3])([O:5]C)[CH3:6].O[CH:7]1[CH2:8][CH2:9][CH:10]=[C:11]1[Br:12]>>[CH3:1][N:2]([CH3:3])[C:4](=[O:5])[CH2:6][CH:7]1[CH2:8][CH2:9][CH:10]=[C:11]1[Br:12]
COC(C)(OC)N(C)C.OC1CCC=C1Br
CN(C)C(=O)CC1CCC=C1Br
null
null
C1(=CC(=CC=C1)C)C
Acylation
OtherReaction
472efbd11bccde21c77e60699870409b373bfa9a687d07c8eab1af485f3a91e4
af349c417be477b4d858dc01708167320fccf28f33d370d57c6d20ba9e230b4c
C1=CCCC1
C-O-[C;H0;D4;+0:1](-[CH3;D1;+0:2])(-[O;H0;D2;+0:3]-C)-[#7:4](-[C;D1;H3:5])-[C;D1;H3:6].O-[CH;D3;+0:7]1-[C:8]-[C:9]-[C:10]=[C:11]-1-[Br;D1;H0:12]>>[Br;D1;H0:12]-[C:11]1=[C:10]-[C:9]-[C:8]-[CH;D3;+0:7]-1-[CH2;D2;+0:2]-[C;H0;D3;+0:1](=[O;H0;D1;+0:3])-[#7:4](-[C;D1;H3:5])-[C;D1;H3:6]
63
[{"value": 63.0, "product": "BrC=1C(CCC1)CC(=O)N(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 62.7, "product": "BrC=1C(CCC1)CC(=O)N(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2-Bromo-cyclopent-2-enol (Intermediate D3) (2.18 g, 13.4 mmol) and N,N-dimethylacetamide dimethyl acetal (3.5 mL, 21.5 mmol) in m-xylene (˜20 mL) were heated to 140° C. for 14 h. The mixture was freed of solvent and the residue was purified on a column of silica gel with 30% to 50% EtOAc:hexanes to give 2-(2-bromo-cycl...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary alcohol
Tertiary amide
C1=CCCC1
C1=CCCC1
C1=CCCC1
HO-
C1(=CC(=CC=C1)C)C
null
null
COC(C)(OC)N(C)C.OC1CCC=C1Br>C1(=CC(=CC=C1)C)C>CN(C)C(=O)CC1CCC=C1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-08e867a4674e4c02a3f0795e25c3850a
CN(C)C(=O)CC1CCC=C1Br>>OCCC1CCC=C1Br
BrC=1C(CCC1)CC(=O)N(C)C.C(C)[BH-](CC)CC.[Li+]>>BrC=1C(CCC1)CCO
CN(C)[C:2](=[O:1])[CH2:3][CH:4]1[CH2:5][CH2:6][CH:7]=[C:8]1[Br:9]>>[OH:1][CH2:2][CH2:3][CH:4]1[CH2:5][CH2:6][CH:7]=[C:8]1[Br:9]
CN(C)C(=O)CC1CCC=C1Br
OCCC1CCC=C1Br
null
null
C1CCOC1
Miscellaneous
OtherReaction
0c75196bc326a5f4df5281c5aa6ae5cdc4819d93f21e68fb7ca3f026ca65886c
cfd0fcbb4b1cf020b5a9adf1c1aee54d845237b6f4e1af15a68ce24628b71452
C1=CCCC1
C-N(-C)-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3]-[C:4]-[C:5]=[C:6]>>[C:6]=[C:5]-[C:4]-[C:3]-[CH2;D2;+0:1]-[OH;D1;+0:2]
58
[{"value": 58.0, "product": "BrC=1C(CCC1)CCO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2-(2-Bromo-cyclopent-2-enyl)-N,N-dimethyl-acetamide (Intermediate FOUR1) (1.93 g, 8.3 mmol) in THF (50 mL) was reacted with lithium triethylborohydride (19 mL, 1 M in THF) at 0° C. for 1 h. The mixture was treated with an aqueous work-up and the resultant alcohol was purified by column chromatography to give 0.92 g of ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide
Primary alcohol
null
null
C1=CCCC1
Other
C1CCOC1
null
null
CN(C)C(=O)CC1CCC=C1Br>C1CCOC1>OCCC1CCC=C1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5ee325071a0d46e99c30139f1c8099af
OB(O)c1ccccc1F.OCCC1CCC=C1Br>>OCCC1CCC=C1c1ccccc1F
BrC=1C(CCC1)CCO.C(=O)([O-])[O-].[Na+].[Na+].FC1=C(C=CC=C1)B(O)O>>FC1=C(C=CC=C1)C=1C(CCC1)CCO
OB(O)[c:9]1[cH:10][cH:11][cH:12][cH:13][c:14]1[F:15].Br[C:8]1=[CH:7][CH2:6][CH2:5][CH:4]1[CH2:3][CH2:2][OH:1]>>[OH:1][CH2:2][CH2:3][CH:4]1[CH2:5][CH2:6][CH:7]=[C:8]1[c:9]1[cH:10][cH:11][cH:12][cH:13][c:14]1[F:15]
OB(O)c1ccccc1F.OCCC1CCC=C1Br
OCCC1CCC=C1c1ccccc1F
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=...
CCO.O.C1=CC=CC=C1
C-C Coupling
Suzuki coupling with boronic acids
8b39a68e12ea3ce139cd616a612024de0f2d741f1d7eb710bb082906f1f12f29
5a0296c84d2188f496a7851efee830bbda9aa21de5f6b9e031f92f0a517689c7
C1=C(c2ccccc2)CCC1
Br-[C;H0;D3;+0:1]1=[C:2]-[C:3]-[C:4]-[C:5]-1-[C:6].O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[F;D1;H0:11]):[c:12]>>[C:6]-[C:5]1-[C:4]-[C:3]-[C:2]=[C;H0;D3;+0:1]-1-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[F;D1;H0:11]):[c:12]
null
[]
80
CELSIUS
null
null
2-(2-Bromo-cyclopent-2-enyl)-ethanol Intermediate FIVE1 (1.21 g, 6.33 mmol) in benzene (40 mL), and Na2CO3 (7 mL, 2M) was treated with a solution of 2-fluorophenylboronic acid (1.08 g, 7.72 mmol) in EtOH (28 mL). Tetrakis(triphenylphosphine)palladium(0), Pd(PPh3)4 (0.38 g, 5 mol %) was added and the mixture was heated ...
10.6084/m9.figshare.5104873.v1
null
Alkenyl halide.Boronic acid
null
c1ccccc1.C1=CCCC1
C1=CCCC1.c1ccccc1
C1=CCCC1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=...
80
null
OB(O)c1ccccc1F.OCCC1CCC=C1Br>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=...
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-dbc0d9ebb62a4b7f88776da007ed6142
CCOC1=CC(=O)CC1.O=C1CCC(=O)N1Br>>CCOC1=C(Br)C(=O)CC1
C(C)OC1=CC(CC1)=O.C1CC(=O)N(C1=O)Br>>BrC=1C(CCC1OCC)=O
[CH3:1][CH2:2][O:3][C:4]1=[CH:5][C:7](=[O:8])[CH2:9][CH2:10]1.O=C1CCC(=O)N1[Br:6]>>[CH3:1][CH2:2][O:3][C:4]1=[C:5]([Br:6])[C:7](=[O:8])[CH2:9][CH2:10]1
CCOC1=CC(=O)CC1.O=C1CCC(=O)N1Br
CCOC1=C(Br)C(=O)CC1
null
null
C(Cl)(Cl)(Cl)Cl
Functional Group Interconversion
Bromination
9e1015dee387752fede3530dfce87ae0ed0bc8bdfc02d155d60141e6bf3e07a5
91b04554311f4a27d2463e6f0477568ffd575c02d8acaa1ad2eb9195fa41deab
O=C1C=CCC1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#8:2]-[C:3]1=[CH;D2;+0:4]-[C:5](=[O;D1;H0:6])-[C:7]-[C:8]-1>>[#8:2]-[C:3]1=[C;H0;D3;+0:4](-[Br;H0;D1;+0:1])-[C:5](=[O;D1;H0:6])-[C:7]-[C:8]-1
null
[]
null
null
null
null
3-Ethoxy-cyclopent-2-enone (Intermediate NINE1) (commercially available from Aldrich) (10.0 g, 77.6 mmol) in carbon tetrachloride (15 mL) at 0° C. was treated with NBS (15.3 g, ˜85 mmol) added portion-wise over 30 m. After 1 h at 0° C. the mixture was partitioned between CH2Cl2 and saturated NaHCO3. The aqueous layer w...
10.6084/m9.figshare.5104873.v1
null
Ketone.Tertiary amide.Tertiary amide
Alkenyl halide
C1=CCCC1.C1CCNC1
C1=CCCC1
C1=CCCC1
HO-
C(Cl)(Cl)(Cl)Cl
null
null
CCOC1=CC(=O)CC1.O=C1CCC(=O)N1Br>C(Cl)(Cl)(Cl)Cl>CCOC1=C(Br)C(=O)CC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1b99ecc263fc43ae8cb7d0f030d361c9
CCOC1=C(Br)C(=O)CC1.OB(O)c1ccc(F)cc1>>CCOC1=C(c2ccc(F)cc2)C(=O)CC1
BrC=1C(CCC1OCC)=O.C(=O)([O-])[O-].[K+].[K+].FC1=CC=C(C=C1)B(O)O>>C(C)OC1=C(C(CC1)=O)C1=CC=C(C=C1)F
Br[C:5]1=[C:4]([O:3][CH2:2][CH3:1])[CH2:16][CH2:15][C:13]1=[O:14].OB(O)[c:6]1[cH:7][cH:8][c:9]([F:10])[cH:11][cH:12]1>>[CH3:1][CH2:2][O:3][C:4]1=[C:5]([c:6]2[cH:7][cH:8][c:9]([F:10])[cH:11][cH:12]2)[C:13](=[O:14])[CH2:15][CH2:16]1
CCOC1=C(Br)C(=O)CC1.OB(O)c1ccc(F)cc1
CCOC1=C(c2ccc(F)cc2)C(=O)CC1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=...
CCO.O.C1=CC=CC=C1.C1(=CC=CC=C1)C
C-C Coupling
Suzuki coupling with boronic acids
f7bba2cceceb9f43c641f927a7f9afed99196e4de44cb21ace80bae0c7d3e127
8b2fd2c710285a8e42ec4e306f128a23a05d3000a0fcad7f4f9c1377cd9b6157
O=C1CCC=C1c1ccccc1
Br-[C;H0;D3;+0:1]1=[C:2](-[#8:3])-[C:4]-[C:5]-[C:6]-1=[O;D1;H0:7].O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#8:3]-[C:2]1=[C;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12])-[C:6](=[O;D1;H0:7])-[C:5]-[C:4]-1
70
[{"value": 70.0, "product": "C(C)OC1=C(C(CC1)=O)C1=CC=C(C=C1)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.6, "product": "C(C)OC1=C(C(CC1)=O)C1=CC=C(C=C1)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
2-Bromo-3-ethoxy-cyclopent-2-enone (Intermediate NINE2) (10.5 g, 51.2 mmol) and K2CO3 (14.2 g, 102 mmol) in toluene (100 mL), benzene (100 mL) and H2O (50 mL) was treated with a solution of 4-fluorophenylboronic acid (9.31 g, 66.5) in EtOH (100 mL). Tetrakis(triphenylphosphine)palladium(0) Pd(PPh3)4 (3 g, 2.6 mmol), bi...
10.6084/m9.figshare.5104873.v1
null
Alkenyl halide.Ketone.Boronic acid
Ketone
C1=CCCC1.c1ccccc1
C1=CCCC1.c1ccccc1
C1=CCCC1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=...
100
null
CCOC1=C(Br)C(=O)CC1.OB(O)c1ccc(F)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=C...
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f410f80b3f0a4b32a915abb183781321
CC1=C(Br)C(=O)CC1.N#Cc1ccc(B(O)O)cc1>>CC1=C(c2ccc(C#N)cc2)C(=O)CC1
BrC=1C(CCC1C)=O.C(=O)([O-])[O-].[K+].[K+].C(#N)C1=CC=C(C=C1)B(O)O.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>CC1=C(C(CC1)=O)C1=CC=C(C#N)C=C1
Br[C:3]1=[C:2]([CH3:1])[CH2:15][CH2:14][C:12]1=[O:13].OB(O)[c:4]1[cH:5][cH:6][c:7]([C:8]#[N:9])[cH:10][cH:11]1>>[CH3:1][C:2]1=[C:3]([c:4]2[cH:5][cH:6][c:7]([C:8]#[N:9])[cH:10][cH:11]2)[C:12](=[O:13])[CH2:14][CH2:15]1
CC1=C(Br)C(=O)CC1.N#Cc1ccc(B(O)O)cc1
CC1=C(c2ccc(C#N)cc2)C(=O)CC1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=...
CCO.C1(=CC=CC=C1)C
C-C Coupling
Suzuki coupling with boronic acids
f7bba2cceceb9f43c641f927a7f9afed99196e4de44cb21ace80bae0c7d3e127
8b2fd2c710285a8e42ec4e306f128a23a05d3000a0fcad7f4f9c1377cd9b6157
O=C1CCC=C1c1ccccc1
Br-[C;H0;D3;+0:1]1=[C:2](-[C;D1;H3:3])-[C:4]-[C:5]-[C:6]-1=[O;D1;H0:7].O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[C;D1;H3:3]-[C:2]1=[C;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12])-[C:6](=[O;D1;H0:7])-[C:5]-[C:4]-1
null
[]
80
CELSIUS
null
null
2-Bromo-3-methyl-cyclopent-2-enone (Intermediate TEN1) (commercially available from Aldrich) (2.04 g, 11.4 mmol) and K2CO3 (3.16 g in 11 mL H2O) in toluene (45 mL) was treated with a solution 4-cyanophenylboronic acid (commercially available from Aldrich) (2.2 g, 15 mmol) in EtOH (27 mL). Tetrakis(triphenylphosphine)pa...
10.6084/m9.figshare.5104873.v1
null
Alkenyl halide.Ketone.Boronic acid
Ketone
C1=CCCC1.c1ccccc1
C1=CCCC1.c1ccccc1
C1=CCCC1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=...
80
null
CC1=C(Br)C(=O)CC1.N#Cc1ccc(B(O)O)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=C...
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5cb5054aa9ad4c07b38d5b7d2bbe5aca
OCCC1Cc2ccccc2C1>>O=CCC1Cc2ccccc2C1
C1C(CC2=CC=CC=C12)CCO.C[N+]1(CCOCC1)[O-].C1C(CC2=CC=CC=C12)CC(=O)O.[H-].[H-].[H-].[H-].[Li+].[Al+3]>>C1C(CC2=CC=CC=C12)CC=O
[OH:1][CH2:2][CH2:3][CH:4]1[CH2:5][c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[CH2:12]1>>[O:1]=[CH:2][CH2:3][CH:4]1[CH2:5][c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[CH2:12]1
OCCC1Cc2ccccc2C1
O=CCC1Cc2ccccc2C1
null
CCC[N+](CCC)(CCC)CCC.[O-][Ru](=O)(=O)=O.[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC
CC#N.C1CCOC1.C(Cl)Cl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccc2c(c1)CCC2
[C:1]-[C:2]-[CH2;D2;+0:3]-[OH;D1;+0:4]>>[C:1]-[C:2]-[CH;D2;+0:3]=[O;H0;D1;+0:4]
null
[]
null
null
16
HOUR
Use of indan-2-yl-acetic acid (commercially available from Lancaster) (Intermediate SEVENTEEN-1) (1.58 g, 8.88 mmol) in THF (15 mL) was added dropwise to a solution of LiAlH4 (9 mL, 1M in Et2O) in THF (10 mL) at 0° C. The mixture was reacted for 2 h at rt and quenched with Rochelle's salt solution and extracted with Et...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccc2c(c1)CCC2
null
CCC[N+](CCC)(CCC)CCC.[O-][Ru](=O)(=O)=O.[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.CC#N.C1CCOC1.C(Cl)Cl
null
16
OCCC1Cc2ccccc2C1>CCC[N+](CCC)(CCC)CCC.[O-][Ru](=O)(=O)=O.[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.CC#N.C1CCOC1.C(Cl)Cl>O=CCC1Cc2ccccc2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-21761f62448e4eaeb88a57c0e17395ff
COC(=O)OC.O=C1CCc2cc(F)ccc21>>COC(=O)C1Cc2ccc(F)cc2C1
Cl.[H-].[Na+].COC(OC)=O.FC=1C=C2CCC(C2=CC1)=O>>COC(=O)C1CC2=CC=C(C=C2C1)F
CO[C:3]([O:2][CH3:1])=[O:4].O=[C:6]1[CH2:5][CH2:14][c:13]2[c:7]1[cH:8][cH:9][c:10]([F:11])[cH:12]2>>[CH3:1][O:2][C:3](=[O:4])[CH:5]1[CH2:6][c:7]2[cH:8][cH:9][c:10]([F:11])[cH:12][c:13]2[CH2:14]1
COC(=O)OC.O=C1CCc2cc(F)ccc21
COC(=O)C1Cc2ccc(F)cc2C1
null
null
C1CCOC1
C-C Coupling
OtherReaction
2890360cfb4b3d777952995f9ea6fb59f6a398984fc169af8dcfcef1a3752370
fa68f4aa0d3109d3a74ccba0f7352d8a6ecbc181d17439eb72406023cade9696
c1ccc2c(c1)CCC2
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].O=[C;H0;D3;+0:5]1-[CH2;D2;+0:6]-[C:7]-[c:8]:[c:9]-1:[c:10]>>[C;D1;H3:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH;D3;+0:6]1-[C:7]-[c:8]:[c:9](:[c:10])-[CH2;D2;+0:5]-1
null
[]
65
CELSIUS
18
HOUR
To a mixture of NaH (2.64 g, 66 mmol) in dimethylcarbonate (4.2 mL, 50 mmol) in THF (30 mL) was added a solution of 5-fluoroindanone (commercially available from Aldrich) (5 g, 33 mmol). After 30 m at 65° C. the mixture was cooled to rt, acidified with HCl (aq) and extracted with Et2O or EtOAc. The organic layers were ...
10.6084/m9.figshare.5104873.v1
null
Carbonic Ester.Ketone
Ester
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
HO-
C1CCOC1
65
18
COC(=O)OC.O=C1CCc2cc(F)ccc21>C1CCOC1>COC(=O)C1Cc2ccc(F)cc2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7bef4df5984842bd9e09da4202b7770b
COC(=O)OC.O=C1CCc2cc(Br)ccc21>>COC(=O)C1Cc2cc(Br)ccc2C1=O
BrC=1C=C2CCC(C2=CC1)=O.[H-].[Na+].COC(OC)=O>>COC(=O)C1C(C2=CC=C(C=C2C1)Br)=O
CO[C:3]([O:2][CH3:1])=[O:4].[CH2:5]1[CH2:6][c:7]2[cH:8][c:9]([Br:10])[cH:11][cH:12][c:13]2[C:14]1=[O:15]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]1[CH2:6][c:7]2[cH:8][c:9]([Br:10])[cH:11][cH:12][c:13]2[C:14]1=[O:15]
COC(=O)OC.O=C1CCc2cc(Br)ccc21
COC(=O)C1Cc2cc(Br)ccc2C1=O
null
null
null
C-C Coupling
OtherReaction
c2c31337dfb867d8c28bc65df0ad4496f817a712a58e176523b47d7fdb6e4f91
d76b6fc9d01d8258e5777a3b2326a8d78a9d9a55717b27736ba55600205f4ed0
O=C1CCc2ccccc21
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].[O;D1;H0:5]=[C:6]1-[CH2;D2;+0:7]-[C:8]-[c:9]:[c:10]-1>>[C;D1;H3:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH;D3;+0:7]1-[C:8]-[c:9]:[c:10]-[C:6]-1=[O;D1;H0:5]
null
[]
null
null
null
null
Use of 5-bromo-indan-1-one (Intermediate NINETEEN-1) in a reaction with NaH and dimethylcarbonate (refer to procedures in Method EIGHTEEN) produced 5-bromo-1-oxo-indan-2-carboxylic acid methyl ester (Intermediate NINETEEN-2). A solution of 5-bromo-1-oxo-indan-2-carboxylic acid methyl ester (4.75 g, 17.7 mmol) in TFA (8...
10.6084/m9.figshare.5104873.v1
null
Carbonic Ester.Ketone
Ketone.Ester
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
HO-
null
null
null
COC(=O)OC.O=C1CCc2cc(Br)ccc21>>COC(=O)C1Cc2cc(Br)ccc2C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-dcd109e13fcc40fbb23bd72b4524be9c
COC(=O)C1Cc2cc(Br)ccc2C1=O>>COC(=O)C1Cc2ccc(Br)cc2C1
COC(=O)C1C(C2=CC=C(C=C2C1)Br)=O.C(C)[SiH](CC)CC>>COC(=O)C1CC2=CC=C(C=C2C1)Br
O=[C:6]1[CH:5]([C:3]([O:2][CH3:1])=[O:4])[CH2:14][c:13]2[c:7]1[cH:8][cH:9][c:10]([Br:11])[cH:12]2>>[CH3:1][O:2][C:3](=[O:4])[CH:5]1[CH2:6][c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][c:13]2[CH2:14]1
COC(=O)C1Cc2cc(Br)ccc2C1=O
COC(=O)C1Cc2ccc(Br)cc2C1
null
null
C(=O)(C(F)(F)F)O
Reduction
OtherReaction
6a1c34e1ccacafe0bd80d1f5ae97146d791a381b1dfbf61349064f8e4b70bdd9
f9ba67182f94acd5fbe41487f8f71e26bccf898b8fc8091ef46f4363de5628d4
c1ccc2c(c1)CCC2
O=[C;H0;D3;+0:1]1-[C:2](-[C:3](=[O;D1;H0:4])-[#8:5]-[C;D1;H3:6])-[C:7]-[c:8]:[c:9]-1:[c:10]>>[C;D1;H3:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[C:2]1-[C:7]-[c:8]:[c:9](:[c:10])-[CH2;D2;+0:1]-1
null
[]
null
null
18
HOUR
Use of 5-bromo-indan-1-one (Intermediate NINETEEN-1) in a reaction with NaH and dimethylcarbonate (refer to procedures in Method EIGHTEEN) produced 5-bromo-1-oxo-indan-2-carboxylic acid methyl ester (Intermediate NINETEEN-2). A solution of 5-bromo-1-oxo-indan-2-carboxylic acid methyl ester (4.75 g, 17.7 mmol) in TFA (8...
10.6084/m9.figshare.5104873.v1
null
Ketone
null
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
Other
C(=O)(C(F)(F)F)O
null
18
COC(=O)C1Cc2cc(Br)ccc2C1=O>C(=O)(C(F)(F)F)O>COC(=O)C1Cc2ccc(Br)cc2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-467a0d7965df4e4793d80e95c83d1100
COC(=O)C1Cc2ccc(Br)cc2C1>>O=C(O)C1Cc2ccc(Br)cc2C1
COC(=O)C1CC2=CC=C(C=C2C1)Br>>BrC=1C=C2CC(CC2=CC1)C(=O)O
C[O:3][C:2](=[O:1])[CH:4]1[CH2:5][c:6]2[cH:7][cH:8][c:9]([Br:10])[cH:11][c:12]2[CH2:13]1>>[O:1]=[C:2]([OH:3])[CH:4]1[CH2:5][c:6]2[cH:7][cH:8][c:9]([Br:10])[cH:11][c:12]2[CH2:13]1
COC(=O)C1Cc2ccc(Br)cc2C1
O=C(O)C1Cc2ccc(Br)cc2C1
null
null
CC(=O)O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(c1)CCC2
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
Use of 5-bromo-indan-1-one (Intermediate NINETEEN-1) in a reaction with NaH and dimethylcarbonate (refer to procedures in Method EIGHTEEN) produced 5-bromo-1-oxo-indan-2-carboxylic acid methyl ester (Intermediate NINETEEN-2). A solution of 5-bromo-1-oxo-indan-2-carboxylic acid methyl ester (4.75 g, 17.7 mmol) in TFA (8...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2c(c1)CCC2
Other
CC(=O)O
null
null
COC(=O)C1Cc2ccc(Br)cc2C1>CC(=O)O>O=C(O)C1Cc2ccc(Br)cc2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-39187aa04b4741c7af65c404933627df
O=C(O)CCc1ccccc1Br>>O=C1CCc2c(Br)cccc21
[Al+3].[Cl-].[Cl-].[Cl-].BrC1=C(C=CC=C1)CCC(=O)O.C(C(=O)Cl)(=O)Cl>>BrC1=C2CCC(C2=CC=C1)=O
O[C:2](=[O:1])[CH2:3][CH2:4][c:5]1[c:6]([Br:7])[cH:8][cH:9][cH:10][cH:11]1>>[O:1]=[C:2]1[CH2:3][CH2:4][c:5]2[c:6]([Br:7])[cH:8][cH:9][cH:10][c:11]21
O=C(O)CCc1ccccc1Br
O=C1CCc2c(Br)cccc21
null
CN(C)C=O
C(Cl)Cl
Functional Group Interconversion
OtherReaction
5fa70460ed4c9b149f869ba1e1d7456e1bbb70fa33dd43785c52e9f0686f4e57
6a71bb5a71b59feeb4f6a39b1b66fa450a058b64b0a3909e1a51c22473a141c5
O=C1CCc2ccccc21
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]-[c:5](:[c:6]):[cH;D2;+0:7]:[c:8]:[c:9]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:3]-[C:4]-[c:5](:[c:6]):[c;H0;D3;+0:7]-1:[c:8]:[c:9]
null
[]
0
CELSIUS
null
null
4-Bromo-indan-1-one was obtained by the following procedure: A solution of 3-(2-bromo-phenyl)-propionic acid (commercially available from Oakwood Products) (15.0 g, 65.5 mmol) in CH2Cl2 at 0° C. was reacted with oxalyl chloride (7.2 mL, 1.5 eq) followed by 2–3 drops of DMF. The mixture was stirred until no more gas evo...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ketone
c1ccccc1
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
HO-
CN(C)C=O.C(Cl)Cl
0
null
O=C(O)CCc1ccccc1Br>CN(C)C=O.C(Cl)Cl>O=C1CCc2c(Br)cccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-37f646d79a3c49df86a5c25e5f201708
Cc1c(Cl)cccc1C(=O)O>>Cc1c(Cl)ccc2c1C(=O)CC2
[Al+3].[Cl-].[Cl-].[Cl-].S(=O)(Cl)Cl.ClC=1C(=C(C(=O)O)C=CC1)C.C1=CC=CC=C1>>ClC1=CC=C2CCC(C2=C1C)=O
O[C:9]([c:8]1[c:2]([CH3:1])[c:3]([Cl:4])[cH:5][cH:6][cH:7]1)=[O:10]>>[CH3:1][c:2]1[c:3]([Cl:4])[cH:5][cH:6][c:7]2[c:8]1[C:9](=[O:10])[CH2:11][CH2:12]2
Cc1c(Cl)cccc1C(=O)O
Cc1c(Cl)ccc2c1C(=O)CC2
null
null
ClC(C)Cl
Functional Group Interconversion
OtherReaction
5fa70460ed4c9b149f869ba1e1d7456e1bbb70fa33dd43785c52e9f0686f4e57
6a71bb5a71b59feeb4f6a39b1b66fa450a058b64b0a3909e1a51c22473a141c5
O=C1CCc2ccccc21
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[cH;D2;+0:5]:[c:6]:[c:7]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:8]-[C:9]-[c;H0;D3;+0:5](:[c:6]:[c:7]):[c:3]-1:[c:4]
72
[{"value": 72.0, "product": "ClC1=CC=C2CCC(C2=C1C)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Thionyl chloride (10.0 mL, 1.5 eq) and 3-chloro-2-methyl-benzoic acid (commercially available from Aldrich) (15.6 g, 91.4 mmol) in benzene was refluxed until no more gas evolution was observed. After cooling to rt the mixture was concentrated. The concentrate was diluted with dichloroethane and added to a solution of A...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ketone
c1ccccc1
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
null
ClC(C)Cl
null
8
Cc1c(Cl)cccc1C(=O)O>ClC(C)Cl>Cc1c(Cl)ccc2c1C(=O)CC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-395b0b58d94d4e89ade806c738c584d6
O=C(O)c1cccc(Cl)c1Cl>>O=C1CCc2ccc(Cl)c(Cl)c21
[Al+3].[Cl-].[Cl-].[Cl-].S(=O)(Cl)Cl.ClC1=C(C(=O)O)C=CC=C1Cl.C1=CC=CC=C1>>ClC1=CC=C2CCC(C2=C1Cl)=O
O[C:2](=[O:1])[c:12]1[cH:5][cH:6][cH:7][c:8]([Cl:9])[c:10]1[Cl:11]>>[O:1]=[C:2]1[CH2:3][CH2:4][c:5]2[cH:6][cH:7][c:8]([Cl:9])[c:10]([Cl:11])[c:12]21
O=C(O)c1cccc(Cl)c1Cl
O=C1CCc2ccc(Cl)c(Cl)c21
null
null
ClC(C)Cl
Functional Group Interconversion
OtherReaction
5fa70460ed4c9b149f869ba1e1d7456e1bbb70fa33dd43785c52e9f0686f4e57
6a71bb5a71b59feeb4f6a39b1b66fa450a058b64b0a3909e1a51c22473a141c5
O=C1CCc2ccccc21
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[cH;D2;+0:5]:[c:6]:[c:7]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:8]-[C:9]-[c;H0;D3;+0:5](:[c:6]:[c:7]):[c:3]-1:[c:4]
80
[{"value": 80.0, "product": "ClC1=CC=C2CCC(C2=C1Cl)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Thionyl chloride (5.73 mL, ˜79 mmol) and 2,3-dichloro-benzoic acid (commercially available from Aldrich) (10.0 g, 52.4 mmol) in benzene was heated to reflux until no more gas evolution was observed. After cooling to rt the mixture was concentrated. The concentrate was diluted with dichloroethane and added to AlCl3 (7.0...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ketone
c1ccccc1
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
null
ClC(C)Cl
null
8
O=C(O)c1cccc(Cl)c1Cl>ClC(C)Cl>O=C1CCc2ccc(Cl)c(Cl)c21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-63a36677e98d454d93144fbbcd713e23
O=C(O)C=Cc1cccc(F)c1F>>O=C(O)CCc1cccc(F)c1F
FC1=C(C=CC(=O)O)C=CC=C1F>>FC1=C(C=CC=C1F)CCC(=O)O
[O:1]=[C:2]([OH:3])[CH:4]=[CH:5][c:6]1[cH:7][cH:8][cH:9][c:10]([F:11])[c:12]1[F:13]>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][c:6]1[cH:7][cH:8][cH:9][c:10]([F:11])[c:12]1[F:13]
O=C(O)C=Cc1cccc(F)c1F
O=C(O)CCc1cccc(F)c1F
null
[Pd]
C(C)O
Reduction
Hydrogenation (double to single)
0bc3968b35f0839c230afb4215314da278abd4e1f10e42ec3012c5512de49ea5
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
c1ccccc1
[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[CH;D2;+0:4]=[CH;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[CH2;D2;+0:4]-[CH2;D2;+0:5]-[c:6](:[c:7]):[c:8]
null
[]
null
null
null
null
A solution of 2,3-difluorocinnamic acid (2.8 g, 15.2 mol) (commercially available from Lancaster) (Intermediate TWENTY-1) in ethanol (100 mL) was hydrogenated with H2 (balloon) and 10% Pd/C (0.3 g) at rt for 16 h. The mixture was filtered through Celite® and the solvent was evaporated to give 3-(2,3-difluoro-phenyl)-pr...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1
null
[Pd].C(C)O
null
null
O=C(O)C=Cc1cccc(F)c1F>[Pd].C(C)O>O=C(O)CCc1cccc(F)c1F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1e890937625b4be5ae684bf8922e4ae5
O=C(O)CCc1cccc(F)c1F>>O=C1CCc2c1ccc(F)c2F
[Al+3].[Cl-].[Cl-].[Cl-].FC1=C(C=CC=C1F)CCC(=O)O.C(C(=O)Cl)(=O)Cl>>FC1=C2CCC(C2=CC=C1F)=O
O[C:2](=[O:1])[CH2:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][c:9]([F:10])[c:11]1[F:12]>>[O:1]=[C:2]1[CH2:3][CH2:4][c:5]2[c:6]1[cH:7][cH:8][c:9]([F:10])[c:11]2[F:12]
O=C(O)CCc1cccc(F)c1F
O=C1CCc2c1ccc(F)c2F
null
CN(C)C=O
C(Cl)Cl
Functional Group Interconversion
OtherReaction
5fa70460ed4c9b149f869ba1e1d7456e1bbb70fa33dd43785c52e9f0686f4e57
6a71bb5a71b59feeb4f6a39b1b66fa450a058b64b0a3909e1a51c22473a141c5
O=C1CCc2ccccc21
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]-[c:5](:[c:6]):[cH;D2;+0:7]:[c:8]:[c:9]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:3]-[C:4]-[c:5](:[c:6]):[c;H0;D3;+0:7]-1:[c:8]:[c:9]
null
[]
null
null
2
HOUR
A solution of 2,3-difluorocinnamic acid (2.8 g, 15.2 mol) (commercially available from Lancaster) (Intermediate TWENTY-1) in ethanol (100 mL) was hydrogenated with H2 (balloon) and 10% Pd/C (0.3 g) at rt for 16 h. The mixture was filtered through Celite® and the solvent was evaporated to give 3-(2,3-difluoro-phenyl)-pr...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ketone
c1ccccc1
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
HO-
CN(C)C=O.C(Cl)Cl
null
2
O=C(O)CCc1cccc(F)c1F>CN(C)C=O.C(Cl)Cl>O=C1CCc2c1ccc(F)c2F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2bd0f005d77a4fd481fc55c63a23a3a2
CCOC(=O)CC1CCc2c1ccc(F)c2F>>OCCC1CCc2c1ccc(F)c2F
C(C)OC(CC1CCC2=C(C(=CC=C12)F)F)=O.[Li+].[BH4-]>>FC1=C2CCC(C2=CC=C1F)CCO
CCO[C:2](=[O:1])[CH2:3][CH:4]1[CH2:5][CH2:6][c:7]2[c:8]1[cH:9][cH:10][c:11]([F:12])[c:13]2[F:14]>>[OH:1][CH2:2][CH2:3][CH:4]1[CH2:5][CH2:6][c:7]2[c:8]1[cH:9][cH:10][c:11]([F:12])[c:13]2[F:14]
CCOC(=O)CC1CCc2c1ccc(F)c2F
OCCC1CCc2c1ccc(F)c2F
null
[Pd]
CO.C1CCOC1.CCOC(=O)C
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc2c(c1)CCC2
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3]-[C:4]>>[C:4]-[C:3]-[CH2;D2;+0:1]-[OH;D1;+0:2]
null
[]
null
null
null
null
A mixture of E- and Z-(4,5-difluoro-indan-1-ylidene)-acetic acid ethyl ester (Intermediate TWENTY-3) (1.1 g) in EtOAc (25 mL) was hydrogenated with 10% Pd/C (0.16 g) under H2 (balloon) at rt for 16 h. The mixture was filtered through a bed of Celite® and the filtrate was evaporated under vacuum. The ester, (4,5-difluor...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccc2c(c1)CCC2
HO-
[Pd].CO.C1CCOC1.CCOC(=O)C
null
null
CCOC(=O)CC1CCc2c1ccc(F)c2F>[Pd].CO.C1CCOC1.CCOC(=O)C>OCCC1CCc2c1ccc(F)c2F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9b9de1057bbe403baed0bb47fffa7c28
O=C1c2cccnc2CCC1Cc1c[nH]cn1>>c1cnc2c(c1)CC(Cc1c[nH]cn1)CC2
[OH-].[K+].N1C=NC(=C1)CC1C(C=2C=CC=NC2CC1)=O.NN>>N1C=NC(=C1)CC1CC=2C=CC=NC2CC1
O=[C:7]1[c:5]2[c:4]([n:3][cH:2][cH:1][cH:6]2)[CH2:16][CH2:15][CH:8]1[CH2:9][c:10]1[cH:11][nH:12][cH:13][n:14]1>>[cH:1]1[cH:2][n:3][c:4]2[c:5]([cH:6]1)[CH2:7][CH:8]([CH2:9][c:10]1[cH:11][nH:12][cH:13][n:14]1)[CH2:15][CH2:16]2
O=C1c2cccnc2CCC1Cc1c[nH]cn1
c1cnc2c(c1)CC(Cc1c[nH]cn1)CC2
null
null
C(=O)(O)[O-].[Na+].O.C(COCCO)O
Reduction
OtherReaction
c75925b35ee2d5552de19b47813876b5230d4b373c49e7a684e043aaa1cea5d6
f9ba67182f94acd5fbe41487f8f71e26bccf898b8fc8091ef46f4363de5628d4
c1cnc2c(c1)CC(Cc1c[nH]cn1)CC2
O=[C;H0;D3;+0:1]1-[C:2](-[C:3])-[C:4]-[C:5]-[c:6](:[#7;a:7]:[c:8]):[c:9]-1:[c:10]>>[C:3]-[C:2]1-[C:4]-[C:5]-[c:6](:[#7;a:7]:[c:8]):[c:9](:[c:10])-[CH2;D2;+0:1]-1
null
[]
170
CELSIUS
null
null
Use of 7,8-dihydro-6H-quinolin-5-one (Intermediate TWENTYTWO-1) (obtained as described in Molina, et. al. Tetrahedron 1995, 51, 1265, incorporated herein by reference) in Method E produced 6-(1H-imidazol-4-ylmethyl)-7,8-dihydro-6H-quinolin-5-one (Intermediate TWENTYTWO-2). To a solution of 6-(1H-imidazol-4-ylmethyl)-7,...
10.6084/m9.figshare.5104873.v1
null
Ketone
null
c1cnc2c(c1)CCCC2
c1cnc2c(c1)CCCC2
c1cnc2c(c1)CCCC2.c1c[nH]cn1
Other
C(=O)(O)[O-].[Na+].O.C(COCCO)O
170
null
O=C1c2cccnc2CCC1Cc1c[nH]cn1>C(=O)(O)[O-].[Na+].O.C(COCCO)O>c1cnc2c(c1)CC(Cc1c[nH]cn1)CC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-8c0c6bf75b19483c82a57fcb9c08452e
CCOC(C)=O.O=C1CCc2c(Cl)cccc21>>CCOC(=O)CC1CCc2c(Cl)cccc21
[H-].[Na+].ClC1=C2CCC(C2=CC=C1)=O.CCOC(=O)C>>C(C)OC(CC1CCC2=C(C=CC=C12)Cl)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH3:6].O=[C:7]1[CH2:8][CH2:9][c:10]2[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]21>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH:7]1[CH2:8][CH2:9][c:10]2[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]21
CCOC(C)=O.O=C1CCc2c(Cl)cccc21
CCOC(=O)CC1CCc2c(Cl)cccc21
null
[Rh]
C1CCOC1
C-C Coupling
OtherReaction
494b529c4b01bb0dca388321e034d6f4fb2fd91ad19b78524aceef0167199e0d
79a946b42eb7e7aee42e09efe41630192c1745e07085cd7f7f88cc7b599f9082
c1ccc2c(c1)CCC2
O=[C;H0;D3;+0:1]1-[C:2]-[C:3]-[c:4]:[c:5]-1:[c:6].[C:7]-[#8:8]-[C:9](-[CH3;D1;+0:10])=[O;D1;H0:11]>>[C:7]-[#8:8]-[C:9](=[O;D1;H0:11])-[CH2;D2;+0:10]-[CH;D3;+0:1]1-[C:2]-[C:3]-[c:4]:[c:5]-1:[c:6]
null
[]
null
null
16
HOUR
Use of 2-chlorocinnamic acid (Intermediate TWENTYTHREE-1) (commercially available from Aldrich) in the applicable process steps described in Method TWENTY produced 4-chloro-indan-1-one (Intermediate TWENTYFOUR-1). Triethylphosphonoacetate (3.5 mL, 17.2 mmol) was added to a mixture of NaH (0.69 g, 12.2 mmol) in THF (25 ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester
Ester
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
Other
[Rh].C1CCOC1
null
16
CCOC(C)=O.O=C1CCc2c(Cl)cccc21>[Rh].C1CCOC1>CCOC(=O)CC1CCc2c(Cl)cccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-3bd5b34b9668455190055c5e0f263011
O=C1CCc2c(Br)cccc21.S=c1[nH]cc(C2Cc3cccc(Br)c3C2)[nH]1>>S=c1[nH]cc(CC2CCc3c(Br)cccc32)[nH]1
BrC1=C2CCC(C2=CC=C1)=O.BrC1=C2CC(CC2=CC=C1)C=1NC(NC1)=S>>BrC1=C2CCC(C2=CC=C1)CC=1NC(NC1)=S
O=[C:7]1[CH2:8][CH2:9][c:10]2[c:11]([Br:12])[cH:13][cH:14][cH:15][c:16]21.Brc1cccc2c1C[CH:6]([c:5]1[cH:4][nH:3][c:2](=[S:1])[nH:17]1)C2>>[S:1]=[c:2]1[nH:3][cH:4][c:5]([CH2:6][CH:7]2[CH2:8][CH2:9][c:10]3[c:11]([Br:12])[cH:13][cH:14][cH:15][c:16]32)[nH:17]1
O=C1CCc2c(Br)cccc21.S=c1[nH]cc(C2Cc3cccc(Br)c3C2)[nH]1
S=c1[nH]cc(CC2CCc3c(Br)cccc32)[nH]1
null
null
null
C-C Coupling
OtherReaction
b7fea274054caafc7784f037120973a3c40d41ce02abedda9427ae073660400a
554b1bee1ccf92984990164979ec7aaf354dc2a70796dc88c3036796633e99e1
S=c1[nH]cc(CC2CCc3ccccc32)[nH]1
Br-c1:c:c:c:c2:c:1-C-[CH;D3;+0:1](-[c:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]:1)-C-2.O=[C;H0;D3;+0:7]1-[C:8]-[C:9]-[c:10]:[c:11]-1:[c:12]>>[c:12]:[c:11]1:[c:10]-[C:9]-[C:8]-[CH;D3;+0:7]-1-[CH2;D2;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]:1
null
[]
null
null
null
null
Use of 4-bromoindanone (obtained by the procedures in Example NINETEEN-1 (Compound 149) in Method TWENTYFOUR produced 4-(4-bromo-indan-1-ylmethyl)-1,3-dihydro-imidazole-2-thione (Compound 167). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ketone
null
c1ccc2c(c1)CCC2.c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
c1c[nH]cn1.c1ccc2c(c1)CCC2
HBr
null
null
null
O=C1CCc2c(Br)cccc21.S=c1[nH]cc(C2Cc3cccc(Br)c3C2)[nH]1>>S=c1[nH]cc(CC2CCc3c(Br)cccc32)[nH]1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f6d569a98bd045b096ff8164515028c3
ClC(c1ccccc1)(c1ccccc1)c1ccccc1.O=C1c2ccccc2CCC1Cc1c[nH]cn1>>O=C1c2ccccc2CCC1Cc1cn(C(c2ccccc2)(c2ccccc2)c2ccccc2)cn1
N1C=NC(=C1)CC1C(C2=CC=CC=C2CC1)=O.N1C=NC(=C1)CC1C(C2=CC=CC=C2CC1)=O.C(C)N(CC)CC.C1(=CC=CC=C1)C(C1=CC=CC=C1)(C1=CC=CC=C1)Cl>>C(C1=CC=CC=C1)(C1=CC=CC=C1)(C1=CC=CC=C1)N1C=NC(=C1)CC1C(C2=CC=CC=C2CC1)=O
Cl[C:16]([c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1)([c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1)[c:29]1[cH:30][cH:31][cH:32][cH:33][cH:34]1.[O:1]=[C:2]1[c:3]2[cH:4][cH:5][cH:6][cH:7][c:8]2[CH2:9][CH2:10][CH:11]1[CH2:12][c:13]1[cH:14][nH:15][cH:35][n:36]1>>[O:1]=[C:2]1[c:3]2[cH:4][cH:5][cH:6][cH:7][c:8]2[CH2:9][CH2:10...
ClC(c1ccccc1)(c1ccccc1)c1ccccc1.O=C1c2ccccc2CCC1Cc1c[nH]cn1
O=C1c2ccccc2CCC1Cc1cn(C(c2ccccc2)(c2ccccc2)c2ccccc2)cn1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
e11c706bbc4ed4c537e0a88a7bb26c47a17011e98b2e37f239a30e81d0496061
677f263b618a481bcdc02c85060e6c44b1f44f328207057cd4782b98754b7773
O=C1c2ccccc2CCC1Cc1cn(C(c2ccccc2)(c2ccccc2)c2ccccc2)cn1
Cl-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10].[C:11]-[c:12]1:[#7;a:13]:[c:14]:[nH;D2;+0:15]:[c:16]:1>>[C:11]-[c:12]1:[#7;a:13]:[c:14]:[n;H0;D3;+0:15](-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10]):[c:16]:1
null
[]
null
null
null
null
A solution of 2-(1H-imidazol-4-ylmethyl)-3,4-dihydro-2H-naphthalen-1-one (Intermediate E4) (2.11 g, 9.3 mmol) in DMF (25 mL) was treated with triethyl amine (1.9 mL, 13.6 mmol) and triphenylmethylchloride (tritylchloride) (2.74 g, 9.6 mmol, added dropwise in DMF (25 mL)). After 16 h at rt the mixture was partitioned be...
10.6084/m9.figshare.5104873.v1
null
Tertiary halide
null
c1c[nH]cn1
c1c[nH]cn1
c1ccc2c(c1)CCCC2.c1c[nH]cn1.c1ccccc1.c1ccccc1.c1ccccc1
HCl
CN(C)C=O
null
null
ClC(c1ccccc1)(c1ccccc1)c1ccccc1.O=C1c2ccccc2CCC1Cc1c[nH]cn1>CN(C)C=O>O=C1c2ccccc2CCC1Cc1cn(C(c2ccccc2)(c2ccccc2)c2ccccc2)cn1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-092c15c54f9544a98141d68f8848fcc2
CCOP(=O)(CC#N)OCC.O=C1c2ccccc2CCC1Cc1cn(C(c2ccccc2)(c2ccccc2)c2ccccc2)cn1>>N#CC=C1c2ccccc2CCC1Cc1c[nH]cn1
[H-].[Na+].C(C)OP(OCC)(=O)CC#N.[H-].[Na+].C(C)OP(OCC)(=O)CC#N.C(C1=CC=CC=C1)(C1=CC=CC=C1)(C1=CC=CC=C1)N1C=NC(=C1)CC1C(C2=CC=CC=C2CC1)=O>>N1C=NC(=C1)CC1C(C2=CC=CC=C2CC1)=CC#N
CCOP(=O)(OCC)[CH2:3][C:2]#[N:1].O=[C:4]1[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[CH2:11][CH2:12][CH:13]1[CH2:14][c:15]1[cH:16][n:17](C(c2ccccc2)(c2ccccc2)c2ccccc2)[cH:18][n:19]1>>[N:1]#[C:2][CH:3]=[C:4]1[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[CH2:11][CH2:12][CH:13]1[CH2:14][c:15]1[cH:16][nH:17][cH:18][n:19]1
CCOP(=O)(CC#N)OCC.O=C1c2ccccc2CCC1Cc1cn(C(c2ccccc2)(c2ccccc2)c2ccccc2)cn1
N#CC=C1c2ccccc2CCC1Cc1c[nH]cn1
null
null
CN(C)C=O
C-C Coupling
OtherReaction
47bf1c3aedd17a317c1f93fa6525c8e2e2ed528867ea5276a8a3dfc10d423ae4
06a42e352cf517302d592bf38a2fd11b220014e39071074dc7becb6ee0bee4b2
[CH]=C1c2ccccc2CCC1Cc1c[nH]cn1
C-C-O-P(=O)(-O-C-C)-[CH2;D2;+0:1]-[C:2]#[N;D1;H0:3].O=[C;H0;D3;+0:4](-[C:5](-[C:6]-[c:7]1:[#7;a:8]:[c:9]:[n;H0;D3;+0:10](-C(-c2:c:c:c:c:c:2)(-c2:c:c:c:c:c:2)-c2:c:c:c:c:c:2):[c:11]:1)-[C:12])-[c:13](:[c:14]):[c:15]>>[C:12]-[C:5](-[C:6]-[c:7]1:[#7;a:8]:[c:9]:[nH;D2;+0:10]:[c:11]:1)-[C;H0;D3;+0:4](=[CH;D2;+0:1]-[C:2]#[N;...
null
[]
null
null
16
HOUR
A solution of 2-(1H-imidazol-4-ylmethyl)-3,4-dihydro-2H-naphthalen-1-one (Intermediate E4) (2.11 g, 9.3 mmol) in DMF (25 mL) was treated with triethyl amine (1.9 mL, 13.6 mmol) and triphenylmethylchloride (tritylchloride) (2.74 g, 9.6 mmol, added dropwise in DMF (25 mL)). After 16 h at rt the mixture was partitioned be...
10.6084/m9.figshare.5104873.v1
null
Ketone
null
c1ccc2c(c1)CCCC2.c1c[nH]cn1.c1ccccc1.c1ccccc1.c1ccccc1
c1ccc2c(c1)CCCC2.c1c[nH]cn1
c1ccc2c(c1)CCCC2.c1c[nH]cn1
HO-
CN(C)C=O
null
16
CCOP(=O)(CC#N)OCC.O=C1c2ccccc2CCC1Cc1cn(C(c2ccccc2)(c2ccccc2)c2ccccc2)cn1>CN(C)C=O>N#CC=C1c2ccccc2CCC1Cc1c[nH]cn1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-099d9a9db3364adcb35165d5d1ed609e
O=C(Cl)Oc1ccccc1.c1nc(CC2CCC3=C2CCC3)c[nH]1>>O=c1[nH]cc(CC2CCC3=C2CCC3)[nH]1
ClC(=O)OC1=CC=CC=C1.C1(CCC=2CCCC12)CC=1N=CNC1.C(=O)(O)[O-].[Na+]>>C1(CCC=2CCCC12)CC=1NC(NC1)=O
ClC(Oc1ccccc1)=[O:1].[cH:2]1[nH:3][cH:4][c:5]([CH2:6][CH:7]2[CH2:8][CH2:9][C:10]3=[C:11]2[CH2:12][CH2:13][CH2:14]3)[n:15]1>>[O:1]=[c:2]1[nH:3][cH:4][c:5]([CH2:6][CH:7]2[CH2:8][CH2:9][C:10]3=[C:11]2[CH2:12][CH2:13][CH2:14]3)[nH:15]1
O=C(Cl)Oc1ccccc1.c1nc(CC2CCC3=C2CCC3)c[nH]1
O=c1[nH]cc(CC2CCC3=C2CCC3)[nH]1
null
null
C1CCOC1.O
Miscellaneous
OtherReaction
82d419be310f94e0fb372475936a7f6ca5545d4fb6630b253bc6e6c76775fdd0
11873959194d43f291af7fba282284829cc9317bd0f9101d9a22013c97d9b731
O=c1[nH]cc(CC2CCC3=C2CCC3)[nH]1
Cl-C(=[O;H0;D1;+0:1])-O-c1:c:c:c:c:c:1.[C:2]-[c:3]1:[c:4]:[#7;a:5]:[cH;D2;+0:6]:[n;H0;D2;+0:7]:1>>[C:2]-[c:3]1:[c:4]:[#7;a:5]:[c;H0;D3;+0:6](=[O;H0;D1;+0:1]):[nH;D2;+0:7]:1
50
[{"value": 50.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of 4-(1,2,3,4,5,6-hexahydro-pentalen-1-ylmethyl)-1H-imidazole; fumarate salt (Intermediate A5 as described in Example A, 340 mg, 1.81 mmol) in THF (15 mL) and water (15 mL) was treated with NaHCO3 (1.52 g, 18 mmol) at rt for 30 m. Phenyl chloroformate (600 mL, 4.7 mmol) was added and stirring was continued f...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether
null
c1ccccc1.c1c[nH]cn1
c1c[nH]cn1
c1c[nH]cn1.C1CC2=C(C1)CCC2
HCl
C1CCOC1.O
null
1
O=C(Cl)Oc1ccccc1.c1nc(CC2CCC3=C2CCC3)c[nH]1>C1CCOC1.O>O=c1[nH]cc(CC2CCC3=C2CCC3)[nH]1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b3d9b7426dec42f29bec9b8563dce9bd
c1ccc(COCCC2CCC3(CC2)OCCO3)cc1>>O=C1CCC(CCOCc2ccccc2)CC1
C(C1=CC=CC=C1)OCCC1CCC2(OCCO2)CC1.O.CC=1C=CC(=CC1)S(=O)(=O)O>>C(C1=CC=CC=C1)OCCC1CCC(CC1)=O
C1C[O:1][C:2]2(O1)[CH2:3][CH2:4][CH:5]([CH2:6][CH2:7][O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)[CH2:16][CH2:17]2>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([CH2:6][CH2:7][O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[CH2:16][CH2:17]1
c1ccc(COCCC2CCC3(CC2)OCCO3)cc1
O=C1CCC(CCOCc2ccccc2)CC1
null
null
CC(=O)C
Miscellaneous
Ketal hydrolysis to ketone
7165849453c1f3f22c37497ec202aa2a6a319b018b3ae9fffa16fa9182ebd128
547697208447432e865290cf95eed8e4fcddc12f59856b7ddbf24dc1accb1210
O=C1CCC(CCOCc2ccccc2)CC1
[C:1]-[C:2]-[C;H0;D4;+0:3]1(-O-C-C-[O;H0;D2;+0:4]-1)-[C:5]-[C:6]>>[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[C:5]-[C:6]
97
[{"value": 97.0, "product": "C(C1=CC=CC=C1)OCCC1CCC(CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
8-(2-Benzyloxy-ethyl)-1,4-dioxa-spiro[4.5]decane (Intermediate R1, 1.02 g, 3.70 mmol) (obtainable as described in the publication by Ciufolini et. al. J. Amer. Chem. Soc. 1991, 113, 8016, incorporated herein by reference) was dissolved in acetone (100 mL): H2O (5 mL) and reacted with TsOH (140 mg, 0.74 mmol) at 45° C. ...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Ketone
C1CCC2(CC1)OCCO2
C1CCCCC1
C1CCCCC1.c1ccccc1
HO-
CC(=O)C
null
null
c1ccc(COCCC2CCC3(CC2)OCCO3)cc1>CC(=O)C>O=C1CCC(CCOCc2ccccc2)CC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-36c0fb0cef9b4fd690399403bca865cf
COC(=O)C#N.O=C1CCC(CCOCc2ccccc2)CC1>>COC(=O)C1CC(CCOCc2ccccc2)CCC1=O
C(#N)C(=O)OC.CN(C)P(=O)(N(C)C)N(C)C.[Li+].CC(C)[N-]C(C)C.C(C1=CC=CC=C1)OCCC1CCC(CC1)=O>>COC(=O)C1C(CCC(C1)CCOCC1=CC=CC=C1)=O
N#C[C:3]([O:2][CH3:1])=[O:4].[CH2:5]1[CH2:6][CH:7]([CH2:8][CH2:9][O:10][CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[CH2:18][CH2:19][C:20]1=[O:21]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]1[CH2:6][CH:7]([CH2:8][CH2:9][O:10][CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[CH2:18][CH2:19][C:20]1=[O:21]
COC(=O)C#N.O=C1CCC(CCOCc2ccccc2)CC1
COC(=O)C1CC(CCOCc2ccccc2)CCC1=O
null
null
C1CCOC1
C-C Coupling
OtherReaction
6a637de02d731d3d400000ea4c333bde9eb2fe719003381bc70d0bd8f95d6bee
ea62efa90ef3cfb13125a23e62e9e1787aa2a0b0ee48c8a61b3326a3bda24134
O=C1CCC(CCOCc2ccccc2)CC1
N#C-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].[C:5]-[C:6](=[O;D1;H0:7])-[CH2;D2;+0:8]-[C:9]-[C:10]>>[C:5]-[C:6](=[O;D1;H0:7])-[CH;D3;+0:8](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4])-[C:9]-[C:10]
null
[]
0
CELSIUS
null
null
A solution of LDA (33 ml, 1.5 M in Et2O) in THF (50 mL) at −78° C. was treated with 4-(2-benzyloxy-ethyl)-cyclohexanone (9.5 g, 40.2 mmol). The mixture was warmed to 0° C. over 30 m before re-cooling to −78° C. and adding HMPA (7 mL). Methyl cyanoformate (4.1 mL, 85 mmol) was added and the mixture was stirred for 15 m ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Nitrile
Ketone.Ester
C1CCCCC1
C1CCCCC1
C1CCCCC1.c1ccccc1
Other
C1CCOC1
0
null
COC(=O)C#N.O=C1CCC(CCOCc2ccccc2)CC1>C1CCOC1>COC(=O)C1CC(CCOCc2ccccc2)CCC1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a212ef8076d6461486f10c4b5443e7f8
COC(=O)C1CC(CCOCc2ccccc2)CCC1O>>COC(=O)C1=CCCC(CCOCc2ccccc2)C1
C1CCC2=NCCCN2CC1.CCOC(=O)C.COC(=O)C1C(CCC(C1)CCOCC1=CC=CC=C1)O.O=S(Cl)Cl>>COC(=O)C1=CCCC(C1)CCOCC1=CC=CC=C1
O[CH:6]1[CH:5]([C:3]([O:2][CH3:1])=[O:4])[CH2:20][CH:9]([CH2:10][CH2:11][O:12][CH2:13][c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[CH2:8][CH2:7]1>>[CH3:1][O:2][C:3](=[O:4])[C:5]1=[CH:6][CH2:7][CH2:8][CH:9]([CH2:10][CH2:11][O:12][CH2:13][c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[CH2:20]1
COC(=O)C1CC(CCOCc2ccccc2)CCC1O
COC(=O)C1=CCCC(CCOCc2ccccc2)C1
null
null
N1=CC=CC=C1
Functional Group Interconversion
OtherReaction
579eaa370a2e820e4e797509751f1a267c4c2023a9c84c83636e14e9358f50f3
41a0f24bab2dd1842411d86540b9e431e13b91d9b083780e582360bedf475320
C1=CCC(CCOCc2ccccc2)CC1
O-[CH;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-[CH;D3;+0:6]-1-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10]>>[C;D1;H3:10]-[#8:9]-[C:7](=[O;D1;H0:8])-[C;H0;D3;+0:6]1=[CH;D2;+0:1]-[C:2]-[C:3]-[C:4]-[C:5]-1
null
[]
55
CELSIUS
null
null
A solution of 5-(2-benzyloxy-ethyl)-2-hydroxy-cyclohexanecarboxylic acid methyl ester (Intermediate R2, 0.72 g, 2.48 mmol) in pyridine (10 mL) was treated with SOCl2 (0.73 mL, 12.4 mmol) at −20° C. The mixture was allowed to react for 15 m and was then warmed to 55° C. for 16 h. The solvents were removed under vacuum a...
10.6084/m9.figshare.5104873.v1
null
Ester.Secondary alcohol
Ester
C1CCCCC1
C1=CCCCC1
C1=CCCCC1.c1ccccc1
HO-
N1=CC=CC=C1
55
null
COC(=O)C1CC(CCOCc2ccccc2)CCC1O>N1=CC=CC=C1>COC(=O)C1=CCCC(CCOCc2ccccc2)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-02c6ad70fe5f4ce699d15439da78968c
COC(=O)C1=CCCC(CCOCc2ccccc2)C1>>CC1=CCCC(CCOCc2ccccc2)C1
COC(=O)C1=CCCC(C1)CCOCC1=CC=CC=C1.CC(C)C[AlH]CC(C)C.N1=CC=CC=C1.S(=O)(=O)=O.[H-].[H-].[H-].[H-].[Li+].[Al+3]>>CC=1CC(CCC1)CCOCC1=CC=CC=C1
CO[C:1](=O)[C:2]1=[CH:3][CH2:4][CH2:5][CH:6]([CH2:7][CH2:8][O:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[CH2:17]1>>[CH3:1][C:2]1=[CH:3][CH2:4][CH2:5][CH:6]([CH2:7][CH2:8][O:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[CH2:17]1
COC(=O)C1=CCCC(CCOCc2ccccc2)C1
CC1=CCCC(CCOCc2ccccc2)C1
null
null
C1CCOC1
Reduction
OtherReaction
bbe4aa74424ca2aa68ccc284976164429303e3793b330c9b63e6e77a951d8d58
b8e5da8ea19c403a2e974791a9cf591400749acb6b71151717aaece4f3b22bef
C1=CCC(CCOCc2ccccc2)CC1
C-O-[C;H0;D3;+0:1](=O)-[C:2](=[C:3]-[C:4])-[C:5]>>[C:5]-[C:2](-[CH3;D1;+0:1])=[C:3]-[C:4]
82
[{"value": 82.0, "product": "CC=1CC(CCC1)CCOCC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
5-(2-Benzyloxy-ethyl)-cyclohex-1-enecarboxylic acid methyl ester (Intermediate R3 obtained above in Example R1 in accordance with Method R) was reduced with DIBAL. The resulting alcohol (Intermediate R7, 1.18 g, 4.81 mmol) in THF (20 mL) at 0° C. was treated with sulfur trioxide-pyridine. (1.15 g, 7.21 mmol) for 3 h. L...
10.6084/m9.figshare.5104873.v1
null
Ester
null
null
null
C1=CCCCC1.c1ccccc1
Other
C1CCOC1
null
3
COC(=O)C1=CCCC(CCOCc2ccccc2)C1>C1CCOC1>CC1=CCCC(CCOCc2ccccc2)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-470e70b40dd84612b6776db3961162df
CC(C)[Si](OS(=O)(=O)C(F)(F)F)(C(C)C)C(C)C.O=C1CCC(CCO)CC1>>CC(C)[Si](OCCC1CCC(=O)CC1)(C(C)C)C(C)C
OCCC1CCC(CC1)=O.C(C)(C)N(CC)C(C)C.FC(S(=O)(=O)O[Si](C(C)C)(C(C)C)C(C)C)(F)F>>C(C)(C)[Si](OCCC1CCC(CC1)=O)(C(C)C)C(C)C
O=S(=O)(O[Si:4]([CH:2]([CH3:1])[CH3:3])([CH:15]([CH3:16])[CH3:17])[CH:18]([CH3:19])[CH3:20])C(F)(F)F.[OH:5][CH2:6][CH2:7][CH:8]1[CH2:9][CH2:10][C:11](=[O:12])[CH2:13][CH2:14]1>>[CH3:1][CH:2]([CH3:3])[Si:4]([O:5][CH2:6][CH2:7][CH:8]1[CH2:9][CH2:10][C:11](=[O:12])[CH2:13][CH2:14]1)([CH:15]([CH3:16])[CH3:17])[CH:18]([CH3:...
CC(C)[Si](OS(=O)(=O)C(F)(F)F)(C(C)C)C(C)C.O=C1CCC(CCO)CC1
CC(C)[Si](OCCC1CCC(=O)CC1)(C(C)C)C(C)C
null
null
C(Cl)Cl
Functional Group Interconversion
OtherReaction
1e32bf15362f1db6caa13aeae0e4a2332995f251d0e7d3892b6ae595fa4cebef
6deb768ca6c69e1952bf0a14ab712bbae796f6fbf3723f779ccbc0662be93df5
O=C1CCCCC1
F-C(-F)(-F)-S(=O)(=O)-O-[Si;H0;D4;+0:1](-[C:2](-[C;D1;H3:3])-[C;D1;H3:4])(-[C:5](-[C;D1;H3:6])-[C;D1;H3:7])-[C:8](-[C;D1;H3:9])-[C;D1;H3:10].[C:11]-[C:12]-[OH;D1;+0:13]>>[C:11]-[C:12]-[O;H0;D2;+0:13]-[Si;H0;D4;+0:1](-[C:2](-[C;D1;H3:3])-[C;D1;H3:4])(-[C:5](-[C;D1;H3:6])-[C;D1;H3:7])-[C:8](-[C;D1;H3:9])-[C;D1;H3:10]
null
[]
0
CELSIUS
null
null
A solution of 4-(2-hydroxy-ethyl)-cyclohexanone (Intermediate R10, 6.8 g, 52.6 mmol, (obtainable as described in the publication by Ciufolini et. al. J. Amer. Chem. Soc. 1991, 113, 8016) was dissolved in CH2Cl2 (75 mL) and treated with diisopropylethylamine (9.2 mL, 52.6 mmol) followed by tri-isopropylsilyl trifluorome...
10.6084/m9.figshare.5104873.v1
null
Triflate.Primary alcohol.Silyl protective group
Silyl protective group
null
null
C1CCCCC1
TfOH.HO-
C(Cl)Cl
0
null
CC(C)[Si](OS(=O)(=O)C(F)(F)F)(C(C)C)C(C)C.O=C1CCC(CCO)CC1>C(Cl)Cl>CC(C)[Si](OCCC1CCC(=O)CC1)(C(C)C)C(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-4ddb018270b74e6f9303a922edff502b
CC(C)[Si](OCCC1CCC=C(C=O)C1)(C(C)C)C(C)C.C[Si](C)(C)C=[N+]=[N-]>>C#CC1=CCCC(CCO[Si](C(C)C)(C(C)C)C(C)C)C1
C(C)(C)[Si](OCCC1CCC=C(C1)C=O)(C(C)C)C(C)C.[Si](C)(C)(C)C=[N+]=[N-].[Li]CCCC>>C(#C)C=1CC(CCC1)CCO[Si](C(C)C)(C(C)C)C(C)C
O=[CH:2][C:3]1=[CH:4][CH2:5][CH2:6][CH:7]([CH2:8][CH2:9][O:10][Si:11]([CH:12]([CH3:13])[CH3:14])([CH:15]([CH3:16])[CH3:17])[CH:18]([CH3:19])[CH3:20])[CH2:21]1.C[Si](C)(C)[CH:1]=[N+]=[N-]>>[CH:1]#[C:2][C:3]1=[CH:4][CH2:5][CH2:6][CH:7]([CH2:8][CH2:9][O:10][Si:11]([CH:12]([CH3:13])[CH3:14])([CH:15]([CH3:16])[CH3:17])[CH:1...
CC(C)[Si](OCCC1CCC=C(C=O)C1)(C(C)C)C(C)C.C[Si](C)(C)C=[N+]=[N-]
C#CC1=CCCC(CCO[Si](C(C)C)(C(C)C)C(C)C)C1
null
null
C1CCOC1
Miscellaneous
OtherReaction
b4c50d40bd73f29fc59705faabbc29885d48952a3cd07fd1e79a6158348af59e
1cf50b336c146b01b0780412724e40fc1414b82a1d6078fe921f14b132744e18
C1=CCCCC1
C-[Si](-C)(-C)-[CH;D2;+0:1]=[N+]=[N-].O=[CH;D2;+0:2]-[C:3](=[C:4]-[C:5])-[C:6]>>[C:6]-[C:3](-[C;H0;D2;+0:2]#[CH;D1;+0:1])=[C:4]-[C:5]
null
[]
null
null
null
null
A solution of TMS-diazomethane (4.61 mL, 9.22 mmol) in THF (60 mL) was reacted with n-BuLi (5.0 mL, 7.99 mmol) at −78° C. for 0.5 h. 5-(2-triisopropylsilanyloxy-ethyl)-cyclohex-1-enecarbaldehyde (Intermediate R13) was added via cannula. The mixture was reacted at −78° C. for 1 h and at 0° C. for 1 h. After work-up and ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Diazo.Silyl protective group
Alkyne
null
null
C1=CCCCC1
HO-
C1CCOC1
null
null
CC(C)[Si](OCCC1CCC=C(C=O)C1)(C(C)C)C(C)C.C[Si](C)(C)C=[N+]=[N-]>C1CCOC1>C#CC1=CCCC(CCO[Si](C(C)C)(C(C)C)C(C)C)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-694fed7805bc4205a8b843e02f34766d
C=CC1=CCCC(Cc2c[nH]cn2)C1.OO>>CCC1=CCCC(Cc2c[nH]c(=O)[nH]2)C1
OO.C(=C)C=1CC(CCC1)CC=1N=CNC1.NN.O>>C(C)C=1CC(CCC1)CC=1NC(NC1)=O
[CH2:1]=[CH:2][C:3]1=[CH:4][CH2:5][CH2:6][CH:7]([CH2:8][c:9]2[cH:10][nH:11][cH:12][n:14]2)[CH2:15]1.O[OH:13]>>[CH3:1][CH2:2][C:3]1=[CH:4][CH2:5][CH2:6][CH:7]([CH2:8][c:9]2[cH:10][nH:11][c:12](=[O:13])[nH:14]2)[CH2:15]1
C=CC1=CCCC(Cc2c[nH]cn2)C1.OO
CCC1=CCCC(Cc2c[nH]c(=O)[nH]2)C1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
60747b62e45636256388d4dafb4e1c1823ad34aea5db13df35593c9678c13d9d
f31c628702cf0fcf5a903442a4ec25cb67ad0ae56b375a9a0f274c0dccf17a1c
O=c1[nH]cc(CC2CC=CCC2)[nH]1
O-[OH;D1;+0:1].[C:2]-[C:3](-[CH;D2;+0:4]=[CH2;D1;+0:5])=[C:6]-[C:7].[C:8]-[c:9]1:[c:10]:[#7;a:11]:[cH;D2;+0:12]:[n;H0;D2;+0:13]:1>>[C:2]-[C:3](-[CH2;D2;+0:4]-[CH3;D1;+0:5])=[C:6]-[C:7].[C:8]-[c:9]1:[c:10]:[#7;a:11]:[c;H0;D3;+0:12](=[O;H0;D1;+0:1]):[nH;D2;+0:13]:1
null
[]
0
CELSIUS
6
HOUR
A mixture of NiCl2 (0.364 g, 2.81 mmol) in EtOH (20 mL) was reacted with NaBH4 (0.053 mg, 1.40 mmol) at rt for 15 m after saturation of the solution with hydrogen gas. Ethylene diamine (0.17 g, 2.81 mmol) was added followed by the alkynyl imidazol (Intermediate R15, 0.26 g, 1.40 mmol) at rt for 45 m under an atmosphere...
10.6084/m9.figshare.5104873.v1
null
Peroxide.Vinyl
null
c1c[nH]cn1
c1c[nH]cn1
C1=CCCCC1.c1c[nH]cn1
Other
C(C)O
0
6
C=CC1=CCCC(Cc2c[nH]cn2)C1.OO>C(C)O>CCC1=CCCC(Cc2c[nH]c(=O)[nH]2)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bd97467992de4fa6b98437d8bbc8d45d
O=C(O)C1CCc2cc(F)ccc21>>O=C(O)[C@@H]1CCc2cc(F)ccc21
COC=1C=C2C(=CC1OC)N3[C@@H]4[C@]25CCN6[C@H]5C[C@@H]7[C@H]4[C@H](CC3=O)OCC=C7C6.FC=1C=C2CCC(C2=CC1)C(=O)O.FC=1C=C2CCC(C2=CC1)C(=O)O.FC=1C=C2CCC(C2=CC1)C(=O)O.Cl>>FC=1C=C2CC[C@H](C2=CC1)C(=O)O
[O:1]=[C:2]([OH:3])[CH:4]1[CH2:5][CH2:6][c:7]2[cH:8][c:9]([F:10])[cH:11][cH:12][c:13]21>>[O:1]=[C:2]([OH:3])[C@@H:4]1[CH2:5][CH2:6][c:7]2[cH:8][c:9]([F:10])[cH:11][cH:12][c:13]21
O=C(O)C1CCc2cc(F)ccc21
O=C(O)[C@@H]1CCc2cc(F)ccc21
null
null
CC(=O)C
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
c1ccc2c(c1)CCC2
null
10.5
[{"value": 10.5, "product": "FC=1C=C2CC[C@H](C2=CC1)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The combined mother liquors from the resolution of Intermediate T3 were concentrated under reduced pressure until no acetone remained and acidified to pH 3 with 0° C. 5N HCl. This solution was extracted 3 times with Et2O (200 ml portions) and the combined Et2O portions were washed successively with 1N HCl, H2O and brin...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccc2c(c1)CCC2
null
CC(=O)C
null
null
O=C(O)C1CCc2cc(F)ccc21>CC(=O)C>O=C(O)[C@@H]1CCc2cc(F)ccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bfaeb299ce614cc1b00cd1c3898b5524
CC1=C(Br)C(O)CC1>>CCC1=C(C)CCC1O
BrC=1C(CCC1C)O.C(C)[Mg]Br>>C(C)C=1C(CCC1C)O
Br[C:3]1=[C:4]([CH3:5])[CH2:6][CH2:7][CH:8]1[OH:9]>>[CH3:1][CH2:2][C:3]1=[C:4]([CH3:5])[CH2:6][CH2:7][CH:8]1[OH:9]
CC1=C(Br)C(O)CC1
CCC1=C(C)CCC1O
null
[Ni](Cl)Cl.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1
C1CCOC1
Functional Group Interconversion
OtherReaction
a82332ed27065c9fa7794673a8ff03debc03a422dc5d86bfdfdaf348f60818d9
ec7c8e18578a00f3028f55e642ee15a34a79a79f174afac37d3207d26250efd7
C1=CCCC1
Br-[C;H0;D3;+0:1]1=[C:2](-[C;D1;H3:3])-[C:4]-[C:5]-[C:6]-1-[O;D1;H1:7]>>[C;D1;H3:8]-[C:9]-[C;H0;D3;+0:1]1=[C:2](-[C;D1;H3:3])-[C:4]-[C:5]-[C:6]-1-[O;D1;H1:7]
null
[]
null
null
null
null
The alcohol (Intermediate V2, 16 mmol) in THF (30 mL) at 0° C. was treated with ethyl magnesium bromide (40 mmol). The catalyst, 1,3-bis(diphenylphosphino)propane nickel (11) chloride (0.75 mmol) (NiCl2dppp) was added in one portion and the mixture was heated to reflux for 3 hours following the procedure of Organ et al...
10.6084/m9.figshare.5104873.v1
null
Alkenyl halide
null
C1=CCCC1
C1=CCCC1
C1=CCCC1
Br-
[Ni](Cl)Cl.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1
null
null
CC1=C(Br)C(O)CC1>[Ni](Cl)Cl.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1>CCC1=C(C)CCC1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-edb19e9ecf824c87ace7643d36df2462
C=CCc1ccc2c(c1)OCO2>>CC=Cc1ccc2c(c1)OCO2
O1COC2=CC(CC=C)=CC=C12.[OH-].[K+].Cl>>O1COC2=CC(C=CC)=CC=C12
[CH2:1]=[CH:2][CH2:3][c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[O:10][CH2:11][O:12]2>>[CH3:1][CH:2]=[CH:3][c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[O:10][CH2:11][O:12]2
C=CCc1ccc2c(c1)OCO2
CC=Cc1ccc2c(c1)OCO2
null
null
C(CCC)O
Miscellaneous
OtherReaction
57a64b6b42d462fe8276aa79a48b5b98ebab75830adad1905b3795c71ea65b06
b53d8f361e43dc967c3023dcafe218466acf623d0cf729a1557a2a80217926eb
c1ccc2c(c1)OCO2
[CH2;D1;+0:1]=[CH;D2;+0:2]-[CH2;D2;+0:3]-[c:4](:[c:5]):[c:6]>>[CH3;D1;+0:1]-[CH;D2;+0:2]=[CH;D2;+0:3]-[c:4](:[c:5]):[c:6]
98,652.6
[{"value": 97.0, "product": "O1COC2=CC(C=CC)=CC=C12", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98652.6, "product": "O1COC2=CC(C=CC)=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
Synthesis of isosafrale To 80 g (0.49 mmol) of safrole was added 100 ml of a 3N solution of potassium hydroxide (KOH) in n-butyl alcohol and the reaction mixture was stirred at room temperature for 3 h. The mixture was poured into a solution of 12 ml of concentrated hydrochloric acid (HCl), and 52 ml of ice water. Afte...
10.6084/m9.figshare.5104873.v1
null
Allyl
null
null
null
c1ccc2c(c1)OCO2
null
C(CCC)O
null
3
C=CCc1ccc2c(c1)OCO2>C(CCC)O>CC=Cc1ccc2c(c1)OCO2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-386fea515fe549098d963803cb3d34d0
CC(C)(C)OC(=O)NCc1ccc(N)cc1.Cc1ccccc1N=C=O>>Cc1ccccc1NC(=O)Nc1ccc(CNC(=O)OC(C)(C)C)cc1
CC1=C(C=CC=C1)N=C=O.C(C)(C)(C)OC(NCC1=CC=C(C=C1)N)=O>>CC1=C(C=CC=C1)NC(=O)NC1=CC=C(CNC(OC(C)(C)C)=O)C=C1
[NH2:11][c:12]1[cH:13][cH:14][c:15]([CH2:16][NH:17][C:18](=[O:19])[O:20][C:21]([CH3:22])([CH3:23])[CH3:24])[cH:25][cH:26]1.[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[N:8]=[C:9]=[O:10]>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[NH:8][C:9](=[O:10])[NH:11][c:12]1[cH:13][cH:14][c:15]([CH2:16][NH:17][C:18](=[O:19])[O:20]...
CC(C)(C)OC(=O)NCc1ccc(N)cc1.Cc1ccccc1N=C=O
Cc1ccccc1NC(=O)Nc1ccc(CNC(=O)OC(C)(C)C)cc1
null
null
C(Cl)Cl
Acylation
Urea synthesis via isocyanate and primary amine
d39cd7dc52a79bb265ff8ef61ef7bf9dc7f7b5fb0150fcb4881bdfb18ab9c380
a5dc801930c765d2a435a0a2973e50163c305ba8e7641d6adbcc1550b7b96de7
O=C(Nc1ccccc1)Nc1ccccc1
[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H0:5]=[C;H0;D2;+0:6]=[N;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]>>[O;D1;H0:5]=[C;H0;D3;+0:6](-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4])-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]
null
[]
null
null
null
null
2-Methylphenylisocyanate (7.57 g, 59.83 mmol) was added dropwise at 0° C. to a solution of (4-amino-benzyl)-carbamic acid tert-butyl ester (13.30 g, 59.83 mmol, prepared analoguous to: Moloney, Gerard P.; Martin, Graeme R.; Mathews, Neil; Milne, Aynsley; Hobbs, Heather; et al. J Med. Chem. 1999, 42, 2504–2526) in 120 m...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Primary amine
Urea
null
null
c1ccccc1.c1ccccc1
null
C(Cl)Cl
null
null
CC(C)(C)OC(=O)NCc1ccc(N)cc1.Cc1ccccc1N=C=O>C(Cl)Cl>Cc1ccccc1NC(=O)Nc1ccc(CNC(=O)OC(C)(C)C)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b7df99201e2a45bfaa337e797e30760b
Cc1ccccc1NC(=O)Nc1ccc(CNC(=O)OC(C)(C)C)cc1>>Cc1ccccc1NC(=O)Nc1ccc(CN)cc1
CC1=C(C=CC=C1)NC(=O)NC1=CC=C(CNC(OC(C)(C)C)=O)C=C1>>NCC1=CC=C(C=C1)NC(=O)NC1=C(C=CC=C1)C
CC(C)(C)OC(=O)[NH:17][CH2:16][c:15]1[cH:14][cH:13][c:12]([NH:11][C:9]([NH:8][c:7]2[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]2)=[O:10])[cH:19][cH:18]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[NH:8][C:9](=[O:10])[NH:11][c:12]1[cH:13][cH:14][c:15]([CH2:16][NH2:17])[cH:18][cH:19]1
Cc1ccccc1NC(=O)Nc1ccc(CNC(=O)OC(C)(C)C)cc1
Cc1ccccc1NC(=O)Nc1ccc(CN)cc1
null
null
C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=C(Nc1ccccc1)Nc1ccccc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]-[c:3]>>[NH2;D1;+0:1]-[C:2]-[c:3]
null
[]
null
null
2
HOUR
To a solution of tert-butyl 4-({[(2-methylphenyl)amino]carbonyl}amino)benzylcarbamate (2.00 g, 5.63 mmol) in CH2Cl2 (120 mL) TFA (36 mL) was added at 0° C. and stirred for 2 h at r.t.. The reaction mixture was evaporated and the product was collected (2.72 g, TFA salt). M.p. 142–143° C.; TLC (PE/EtOAc 3/2) Rf 0.14; 1H ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccccc1.c1ccccc1
HO-
C(Cl)Cl
null
2
Cc1ccccc1NC(=O)Nc1ccc(CNC(=O)OC(C)(C)C)cc1>C(Cl)Cl>Cc1ccccc1NC(=O)Nc1ccc(CN)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b8003c8aab514e7886d4813c31252eda
COc1ccc(C(CC(=O)Nc2ccc(NC(=O)Nc3ccccc3C)cc2)NC(=O)c2ccc(C(=O)OC(C)(C)C)cc2)cc1OC>>COc1ccc(C(CC(=O)Nc2ccc(NC(=O)Nc3ccccc3C)cc2)NC(=O)c2ccc(C(=O)O)cc2)cc1OC
C(C)(C)(C)OC(C1=CC=C(C=C1)C(=O)NC(CC(=O)NC1=CC=C(C=C1)NC(=O)NC1=C(C=CC=C1)C)C1=CC(=C(C=C1)OC)OC)=O.C(=O)(C(F)(F)F)O>>COC=1C=C(C=CC1OC)C(CC(=O)NC1=CC=C(C=C1)NC(=O)NC1=C(C=CC=C1)C)NC(=O)C1=CC=C(C(=O)O)C=C1
CC(C)(C)[O:38][C:36]([c:35]1[cH:34][cH:33][c:32]([C:30]([NH:29][CH:7]([c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[c:42]([O:43][CH3:44])[cH:41]2)[CH2:8][C:9](=[O:10])[NH:11][c:12]2[cH:13][cH:14][c:15]([NH:16][C:17](=[O:18])[NH:19][c:20]3[cH:21][cH:22][cH:23][cH:24][c:25]3[CH3:26])[cH:27][cH:28]2)=[O:31])[cH:40][cH:39]1)=[O:37...
COc1ccc(C(CC(=O)Nc2ccc(NC(=O)Nc3ccccc3C)cc2)NC(=O)c2ccc(C(=O)OC(C)(C)C)cc2)cc1OC
COc1ccc(C(CC(=O)Nc2ccc(NC(=O)Nc3ccccc3C)cc2)NC(=O)c2ccc(C(=O)O)cc2)cc1OC
null
null
C(Cl)Cl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C(CC(NC(=O)c1ccccc1)c1ccccc1)Nc1ccc(NC(=O)Nc2ccccc2)cc1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
null
null
24
HOUR
tert-Butyl-4-{[(1-(3,4-dimethoxyphenyl)-3-{[4-({[(2-methylphenyl)amino]carbonyl}amino) phenyl]amino}-3-oxopropyl)amino]carbonyl}benzoate (30 mg, 0.05 mmol) was dissolved in DCM (10 mL) and TFA (0.18 mL, 2.30 mmol) was added at 0° C. and the reaction mixture was stirred at r.t. for 24 h. The solvent was removed in vacuu...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
Other
C(Cl)Cl
null
24
COc1ccc(C(CC(=O)Nc2ccc(NC(=O)Nc3ccccc3C)cc2)NC(=O)c2ccc(C(=O)OC(C)(C)C)cc2)cc1OC>C(Cl)Cl>COc1ccc(C(CC(=O)Nc2ccc(NC(=O)Nc3ccccc3C)cc2)NC(=O)c2ccc(C(=O)O)cc2)cc1OC
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d172a1b84e4647bc9c8687f1cd8f5dda
CC(C)(C)[Si](C)(C)Cl.COc1ccc2c(-c3ccc(OC)c(O)c3)coc2c1>>COc1ccc2c(-c3ccc(OC)c(O[Si](C)(C)C(C)(C)C)c3)coc2c1
CC(C)(C)[Si](C)(C)Cl.OC=1C=C(C=CC1OC)C=1C2=C(OC1)C=C(C=C2)OC.CCN(CC)CC>>[Si](C)(C)(C(C)(C)C)OC=1C=C(C=CC1OC)C=1C2=C(OC1)C=C(C=C2)OC
Cl[Si:16]([CH3:17])([CH3:18])[C:19]([CH3:20])([CH3:21])[CH3:22].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7](-[c:8]3[cH:9][cH:10][c:11]([O:12][CH3:13])[c:14]([OH:15])[cH:23]3)[cH:24][o:25][c:26]2[cH:27]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7](-[c:8]3[cH:9][cH:10][c:11]([O:12][CH3:13])[c:14]([O:15][Si:16]([CH3:17])([CH...
CC(C)(C)[Si](C)(C)Cl.COc1ccc2c(-c3ccc(OC)c(O)c3)coc2c1
COc1ccc2c(-c3ccc(OC)c(O[Si](C)(C)C(C)(C)C)c3)coc2c1
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Protection
Alcohol protection with silyl ethers
91043baed1393f1ecd2302d7d0b31c01cf171d3977dd7c70afa1da52fa298c73
4a917c959d011f885a1269fa3c1f022ee5e09144996246d24e42e65634a451ac
c1ccc(-c2coc3ccccc23)cc1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[OH;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[C;D1;H3:2]-[Si;H0;D4;+0:1](-[C;D1;H3:3])(-[O;H0;D2;+0:8]-[c:9](:[c:10]):[c:11])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7]
92.2
[{"value": 92.0, "product": "[Si](C)(C)(C(C)(C)C)OC=1C=C(C=CC1OC)C=1C2=C(OC1)C=C(C=C2)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.2, "product": "[Si](C)(C)(C(C)(C)C)OC=1C=C(C=CC1OC)C=1C2=C(OC1)C=C(C=C2)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
To a solution of 14 (3.51 g, 12.9 mmol) in CH2Cl2 (30 mL), under nitrogen, was added Et3N (1.98 mL, 14.2 mmol) followed by DMAP (0.162 g, 14.2 mmol) and TBSCl (2.4 g, 14.2 mmol) at 0° C. The reaction mixture was stirred for 12 h allowing too reach room temperature. The reaction was quenched with water, the phases separ...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol.Silyl protective group
TMS ether protective group
null
null
c1ccccc1.c1ccc2occc2c1
HCl
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
12
CC(C)(C)[Si](C)(C)Cl.COc1ccc2c(-c3ccc(OC)c(O)c3)coc2c1>CN(C)C=1C=CN=CC1.C(Cl)Cl>COc1ccc2c(-c3ccc(OC)c(O[Si](C)(C)C(C)(C)C)c3)coc2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9c5bd52821714c9bb9e8153a9d33262f
COc1ccc(C=O)c(OC)c1OC>>COc1ccc(C=O)c(O)c1O
Cl.COC1=C(C=O)C=CC(=C1OC)OC.B(Cl)(Cl)Cl.C([O-])(O)=O.[Na+]>>OC1=C(C=O)C=CC(=C1O)OC
C[O:10][c:9]1[c:6]([CH:7]=[O:8])[cH:5][cH:4][c:3]([O:2][CH3:1])[c:11]1[O:12]C>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH:7]=[O:8])[c:9]([OH:10])[c:11]1[OH:12]
COc1ccc(C=O)c(OC)c1OC
COc1ccc(C=O)c(O)c1O
null
null
C(Cl)Cl
Deprotection
OtherReaction
a0f05885bbc65ae2846cad0ac34029941211b2ef3a426958b0c8aa83bb16fe86
9df751cd682ad9d54ed75d7313aaead6a019c5d37ede15c4672866d319b900ff
c1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]-[C:4]=[O;D1;H0:5]):[c:6](-[O;H0;D2;+0:7]-C):[c:8]>>[O;D1;H0:5]=[C:4]-[c:3]:[c:2](-[OH;D1;+0:1]):[c:6](-[OH;D1;+0:7]):[c:8]
73
[{"value": 73.0, "product": "OC1=C(C=O)C=CC(=C1O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.6, "product": "OC1=C(C=O)C=CC(=C1O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
A dry CH2Cl2 (200 mL) solution of 2,3,4-trimethoxybenzaldehyde (19.6 g, 100 mmol), under nitrogen, was stirred for 10 min and BCl3 (1.0M solution in CH2Cl2, 200 mL) was added. The reaction was stirred for 24 hours and a 10% sodium bicarbonate solution (40 g/360 mL) was added. The resulting solution was acidified with c...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Aromatic alcohol.Aromatic alcohol
null
null
c1ccccc1
Other
C(Cl)Cl
null
24
COc1ccc(C=O)c(OC)c1OC>C(Cl)Cl>COc1ccc(C=O)c(O)c1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-fcacfd8cbe564e93b9260f019b289944
CC(C)Br.CCOC(C)=O.COc1ccc(C=O)c(O)c1O>>COc1ccc(C=O)c(OC(C)C)c1OC(C)C
OC1=C(C=O)C=CC(=C1O)OC.C(=O)([O-])[O-].[K+].[K+].O.CCOC(=O)C.BrC(C)C>>C(C)(C)OC1=C(C=O)C=CC(=C1OC(C)C)OC
Br[CH:16]([CH3:13])[CH3:17].O=[C:11](OC[CH3:18])[CH3:12].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH:7]=[O:8])[c:9]([OH:10])[c:14]1[OH:15]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH:7]=[O:8])[c:9]([O:10][CH:11]([CH3:12])[CH3:13])[c:14]1[O:15][CH:16]([CH3:17])[CH3:18]
CC(C)Br.CCOC(C)=O.COc1ccc(C=O)c(O)c1O
COc1ccc(C=O)c(OC(C)C)c1OC(C)C
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
684858b2c020d9d6d36d1825ea5e12be6ae3975f64a028f56fa8e97d882f6a1c
88ed51cd3eddf51d88767b8d4e94bf799aa7e96d44010d584a877b7adf2bfc8a
c1ccccc1
Br-[CH;D3;+0:1](-[C;D1;H3:2])-[CH3;D1;+0:3].O=[C;H0;D3;+0:4](-[C;D1;H3:5])-O-C-[CH3;D1;+0:6].[O;D1;H0:7]=[C:8]-[c:9]:[c:10](-[OH;D1;+0:11]):[c:12](-[OH;D1;+0:13]):[c:14]>>[C;D1;H3:5]-[CH;D3;+0:4](-[CH3;D1;+0:3])-[O;H0;D2;+0:11]-[c:10](:[c:9]-[C:8]=[O;D1;H0:7]):[c:12](-[O;H0;D2;+0:13]-[CH;D3;+0:1](-[C;D1;H3:2])-[CH3;D1;...
82
[{"value": 82.0, "product": "C(C)(C)OC1=C(C=O)C=CC(=C1OC(C)C)OC", "details": "PERCENTYIELD", "is_desired": false}]
90
CELSIUS
null
null
To a solution of 21 (26.70 g, 158.7 mmol) in DMF (150 mL) under nitrogen, was added K2CO3 (65.84 g, 476.3 mmol) followed by 2-bromopropane (44.72 mL, 476.3 mmol) and heated to reflux (90° C.) for 12 hours. Water (200 mL) and EtOAc (200 mL) were added to the reaction mixture, the phases were separated, and the aqueous p...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ester.Aromatic alcohol.Aromatic alcohol
Ether.Ether
null
null
c1ccccc1
HBr
CN(C)C=O
90
null
CC(C)Br.CCOC(C)=O.COc1ccc(C=O)c(O)c1O>CN(C)C=O>COc1ccc(C=O)c(OC(C)C)c1OC(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-984178fe26d140788905778d11aa6935
COc1ccc(C=O)c(OC(C)C)c1OC(C)C>>COc1ccc(C(C)O)c(OC(C)C)c1OC(C)C
C(C)(C)OC1=C(C=O)C=CC(=C1OC(C)C)OC.C[Li]>>C(C)(C)OC1=C(C=CC(=C1OC(C)C)OC)C(C)O
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH:7]=[O:9])[c:10]([O:11][CH:12]([CH3:13])[CH3:14])[c:15]1[O:16][CH:17]([CH3:18])[CH3:19]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH:7]([CH3:8])[OH:9])[c:10]([O:11][CH:12]([CH3:13])[CH3:14])[c:15]1[O:16][CH:17]([CH3:18])[CH3:19]
COc1ccc(C=O)c(OC(C)C)c1OC(C)C
COc1ccc(C(C)O)c(OC(C)C)c1OC(C)C
null
null
C(C)OCC
Miscellaneous
OtherReaction
1ffaf80f172e20da969364a5d2977299bc51b204f2262675c45c8ec58ff36ac0
e005d650d08e61fc67b766830eb53235a9bc084cc3667d2f8a73c2fb8bb34277
c1ccccc1
[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[C;D1;H3:6]-[CH;D3;+0:2](-[OH;D1;+0:1])-[c:3](:[c:4]):[c:5]
84
[{"value": 84.0, "product": "C(C)(C)OC1=C(C=CC(=C1OC(C)C)OC)C(C)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 22 (23.10 g, 91.56 mmol) in dry ethyl ether (150 mL) was added dropwise methyllithium (98.10 mL, 1.4 M in EtO2, 1.37.3 mmol) at 0° C. under nitrogen. The reaction mixture was stirred for 2 h allowing too reach room temperature. The reaction was slowly quenched with water, the phases were separated, and...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Secondary alcohol
null
null
c1ccccc1
Other
C(C)OCC
null
2
COc1ccc(C=O)c(OC(C)C)c1OC(C)C>C(C)OCC>COc1ccc(C(C)O)c(OC(C)C)c1OC(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-44b54a3e212a410d8860722b1d5535c3
COc1cc(Br)cc(OC)c1OC>>[Li][c]1cc(OC)c(OC)c(OC)c1
C(CCC)[Li].COC=1C=C(C=C(C1OC)OC)Br>>COC=1C=C(C=C(C1OC)OC)[Li]
Br[c:2]1[cH:3][c:4]([O:5][CH3:6])[c:7]([O:8][CH3:9])[c:10]([O:11][CH3:12])[cH:13]1>>[Li:1][c:2]1[cH:3][c:4]([O:5][CH3:6])[c:7]([O:8][CH3:9])[c:10]([O:11][CH3:12])[cH:13]1
COc1cc(Br)cc(OC)c1OC
[Li][c]1cc(OC)c(OC)c(OC)c1
null
null
CCOCC
Miscellaneous
Preparation of organolithium compounds
09779d25a04d5c0f9dabfacc40aa046c53f91c14a1d59b1794183fd92ad3e2b7
b74e09b9a6bbb0311fc1db764a25c5a719efefaac386e11fdf0023b3ff360a3e
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]>>[Li;D1;H0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
null
null
1
HOUR
To a stirred solution of n-butyllithium (3.7 mL, 1.6 M in hexane solution,6.0 mol) in dry ether (40 mL), a solution of 3,4,5-trimethoxyphenylbromide (0.74 g, 3.0 mol) in ether (20 mL) was added under dry nitrogen at −78° C. The solution was stirred for 1 h in order to form 3,4,5-trimethoxyphenyllithum (“TPL”). Substitu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Aryl lithium
c1ccccc1
c1ccccc1
c1ccccc1
null
CCOCC
null
1
COc1cc(Br)cc(OC)c1OC>CCOCC>[Li][c]1cc(OC)c(OC)c(OC)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-36a01d141f4a4baca50a7e0cdac2419d
ICCCCCI.O=C1Cc2ccccc2N1>>O=C1Nc2ccccc2C12CCCCC2
ICCCCCI.N1C(CC2=CC=CC=C12)=O.C(CCC)[Li].[Cl-].[NH4+].CN(CCN(C)C)C>>N1C(C2(C3=CC=CC=C13)CCCCC2)=O
I[CH2:11][CH2:12][CH2:13][CH2:14][CH2:15]I.[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH2:10]1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH2:14][CH2:15]2
ICCCCCI.O=C1Cc2ccccc2N1
O=C1Nc2ccccc2C12CCCCC2
null
null
CCOC(=O)C.O1CCCC1
C-C Coupling
OtherReaction
579f0f36d3c1f227acfe012179441842108aef707a45bbf7908129260433618c
7b68950fc1047c59bb49c25e850f5a51cbe91a99bb87839c4547aec123110e4b
O=C1Nc2ccccc2C12CCCCC2
I-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4]-[CH2;D2;+0:5]-I.[O;D1;H0:6]=[C:7]1-[#7:8]-[c:9]:[c:10](:[c:11])-[CH2;D2;+0:12]-1>>[O;D1;H0:6]=[C:7]1-[#7:8]-[c:9]:[c:10](:[c:11])-[C;H0;D4;+0:12]-12-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4]-[CH2;D2;+0:5]-2
69.6
[{"value": 69.6, "product": "N1C(C2(C3=CC=CC=C13)CCCCC2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.8, "product": "N1C(C2(C3=CC=CC=C13)CCCCC2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A solution of oxindole (25 g, 0.19 mol) in anhydrous tetrahydrofuran (800 cm3) was cooled to −20° C., then n-butyllithium (2.5M in hexanes, 152 cm3, 0.38 mol) was added slowly followed by N,N,N′,N′-tetramethylethylenediamine (51 cm3, 0.38 mol,). After 15 min. 1,5-diiodopentane (174 g, 0.54 mol) was added slowly and the...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide
null
c1ccc2c(c1)CCN2
c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)NCC21CCCCC1
HI
CCOC(=O)C.O1CCCC1
null
0.25
ICCCCCI.O=C1Cc2ccccc2N1>CCOC(=O)C.O1CCCC1>O=C1Nc2ccccc2C12CCCCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-19435386e3f9410d97590e76cde4c6c3
BrBr.O=C1Nc2ccccc2C12CCCCC2>>O=C1Nc2ccc(Br)cc2C12CCCCC2
N1C(C2(C3=CC=CC=C13)CCCCC2)=O.C(C)(=O)[O-].[Na+].BrBr>>BrC=1C=C2C3(C(NC2=CC1)=O)CCCCC3
Br[Br:8].[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:9][c:10]2[C:11]12[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]2>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][c:7]([Br:8])[cH:9][c:10]2[C:11]12[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]2
BrBr.O=C1Nc2ccccc2C12CCCCC2
O=C1Nc2ccc(Br)cc2C12CCCCC2
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
b75a0cb1be6e87ac5ae2a0c4fc61b176231cdf76c6a5c5e00ef053906cd4efba
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1Nc2ccccc2C12CCCCC2
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]:[cH;D2;+0:4]:[c:5]:[c:6]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:3]:[c:2]
67
[{"value": 67.0, "product": "BrC=1C=C2C3(C(NC2=CC1)=O)CCCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.4, "product": "BrC=1C=C2C3(C(NC2=CC1)=O)CCCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of spiro[cyclohexane-1,3′-[3H]indol]-2′(1′H)-one (17.6 g, 0.09 mol) in acetic acid (300 cm3) was added sodium acetate (8.0 g, 0.1 mol) and bromine (14.6 g, 0.091 mol) with stirring. After 30 min. at room temperature, the reaction mixture was partitioned between water and EtOAc. The aqueous phase was extra...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)NCC21CCCCC1
HBr
C(C)(=O)O
null
0.5
BrBr.O=C1Nc2ccccc2C12CCCCC2>C(C)(=O)O>O=C1Nc2ccc(Br)cc2C12CCCCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a1716cb0b7ce4140b396a0bde09d0a6f
CN(C)C=O.Fc1cc(Br)cc(Br)c1>>O=Cc1cc(F)cc(Br)c1
CN(C)C=O.BrC=1C=C(C=C(C1)Br)F.C(CCC)[Li]>>FC=1C=C(C=O)C=C(C1)Br
CN(C)[CH:2]=[O:1].Br[c:3]1[cH:4][c:5]([F:6])[cH:7][c:8]([Br:9])[cH:10]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8]([Br:9])[cH:10]1
CN(C)C=O.Fc1cc(Br)cc(Br)c1
O=Cc1cc(F)cc(Br)c1
null
null
C(C)OCC
C-C Coupling
Bouveault aldehyde synthesis
4664d189e1ff40b394aee0a7d0943c7bfc06c1f81f238cff6865649dda594153
afd09ced98f25d311f21cc04ba6a50fe7e5516de47e17484683ded13d323b1b2
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].C-N(-C)-[CH;D2;+0:6]=[O;D1;H0:7]>>[O;D1;H0:7]=[CH;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
100
[{"value": 100.0, "product": "FC=1C=C(C=O)C=C(C1)Br", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 3,5-dibromofluorobenzene in diethyl ether (100 cm3) at −78° C. was added n-butyl lithium (2.5 M, 8 cm3, 20 mmol) dropwise. After 30 min. the mixture was treated with DMF (20 cm3 diethyl ether (10 cm3 stirring was continued at −78° C. After 30 min. the mixture was quenched with dilute HCl aq., separated...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tertiary amide
Aldehyde
c1ccccc1
c1ccccc1
c1ccccc1
HBr
C(C)OCC
null
null
CN(C)C=O.Fc1cc(Br)cc(Br)c1>C(C)OCC>O=Cc1cc(F)cc(Br)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-09c0fd12d8af423d9f04780d9705f1c8
ON=Cc1cc(F)cc(Br)c1>>N#Cc1cc(F)cc(Br)c1
FC=1C=C(C=NO)C=C(C1)Br>>FC=1C=C(C#N)C=C(C1)Br
O[N:1]=[CH:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8]([Br:9])[cH:10]1>>[N:1]#[C:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8]([Br:9])[cH:10]1
ON=Cc1cc(F)cc(Br)c1
N#Cc1cc(F)cc(Br)c1
null
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-]
C(C)#N
Functional Group Interconversion
OtherReaction
17f476cc256704e312f02cdb730538a4d2e78e129aaed9ef4aa555a9b052c890
9ad4e779dba60265752423413bc1b61ff9562539f91b24f3b3d9205e4bb46232
c1ccccc1
O-[N;H0;D2;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]
89.3
[{"value": 89.0, "product": "FC=1C=C(C#N)C=C(C1)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.3, "product": "FC=1C=C(C#N)C=C(C1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
The above oxime (3.76 g, 17.24 mmol) and copper (II) acetate (370 mg) were dissolved in acetonitrile (100 cm3) under nitrogen and heated under reflux. After 5 h, the mixture was evaporated, the residue taken into EtOAc, washed with sulfuric acid (1N), water, brine, dried (MgSO4) and evaporated to give 3-fluoro-5-bromob...
10.6084/m9.figshare.5104873.v1
null
Oxime
Nitrile
null
null
c1ccccc1
HO-
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].C(C)#N
null
5
ON=Cc1cc(F)cc(Br)c1>C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].C(C)#N>N#Cc1cc(F)cc(Br)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0b8a828b260f43bca10e9f199504f305
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCC2>>CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCC1)C(=O)N2
BrC=1C=C2C3(C(NC2=CC1)=O)CCCC3.C(C)(C)(C)OC(=O)N1C(=CC=C1)B(O)O.C([O-])([O-])=O.[K+].[K+]>>O=C1NC2=CC=C(C=C2C12CCCC2)C=2N(C=CC2)C(=O)OC(C)(C)C
OB(O)[c:12]1[n:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[cH:9][cH:10][cH:11]1.Br[c:13]1[cH:14][cH:15][c:16]2[c:17]([cH:18]1)[C:19]1([CH2:20][CH2:21][CH2:22][CH2:23]1)[C:24](=[O:25])[NH:26]2>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[n:8]1[cH:9][cH:10][cH:11][c:12]1-[c:13]1[cH:14][cH:15][c:16]2[c:17]([...
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCC2
CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCC1)C(=O)N2
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
Suzuki coupling with boronic acids
f4c0bb8a2ef20aeab29eef207992d304c861d6e70be458c5f816d6d34ebf1e84
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccc[nH]3)cc2C12CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6]1:[c:7]:[c:8]:[c:9]:[#7;a:10]:1-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C;D1;H3:15]-[C:14](-[C;D1;H3:16])(-[C;D1;H3:17])-[#8:13]-[C:11](=[O;D1;H0:12])-[#7;a:10]1:[c:9]:[c:8]:[c:7]:[c;H0;D3;+0:6]:1-[c;H0;D3;+0:1](...
83.2
[{"value": 83.0, "product": "O=C1NC2=CC=C(C=C2C12CCCC2)C=2N(C=CC2)C(=O)OC(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.2, "product": "O=C1NC2=CC=C(C=C2C12CCCC2)C=2N(C=CC2)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
5-(2′-Oxo-2′,3′-dihydrospiro[cyclopentane-1,3′-[3H]indol]-5′-yl-2-cyanopyrrole: A solution of 5′-bromospiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one (2.0 g, 7.5 mmol) and tetrakis(triphenylphosphine)palladium(0) (430 mg, 0.3 mmol) in ethylene glycol dimethyl ether (50 mL) was stirred under a flow of nitrogen for 15 min...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCC1
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCC1
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCC1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
80
null
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCC2>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCC1)C(=O)N2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-89b28dbe8cec44cf9b69ba8d95d0eaad
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCCC2>>CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
B(O)(O)C=1N(C=CC1)C(=O)OC(C)(C)C.C(=O)([O-])[O-].[K+].[K+].BrC=1C=C2C3(C(NC2=CC1)=O)CCCCC3>>O=C1NC2=CC=C(C=C2C12CCCCC2)C=2N(C=CC2)C(=O)OC(C)(C)C
OB(O)[c:12]1[n:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[cH:9][cH:10][cH:11]1.Br[c:13]1[cH:14][cH:15][c:16]2[c:17]([cH:18]1)[C:19]1([CH2:20][CH2:21][CH2:22][CH2:23][CH2:24]1)[C:25](=[O:26])[NH:27]2>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[n:8]1[cH:9][cH:10][cH:11][c:12]1-[c:13]1[cH:14][cH:15][c:16]2...
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCCC2
CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
null
null
O
C-C Coupling
Suzuki coupling with boronic acids
72cb0722e2dfbd8433f7f279041b17208e2a10c7d719ed09e6c4b6dd1c93185b
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccc[nH]3)cc2C12CCCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6]1:[c:7]:[c:8]:[c:9]:[#7;a:10]:1-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C;D1;H3:15]-[C:14](-[C;D1;H3:16])(-[C;D1;H3:17])-[#8:13]-[C:11](=[O;D1;H0:12])-[#7;a:10]1:[c:9]:[c:8]:[c:7]:[c;H0;D3;+0:6]:1-[c;H0;D3;+0:1](...
77.3
[{"value": 76.0, "product": "O=C1NC2=CC=C(C=C2C12CCCCC2)C=2N(C=CC2)C(=O)OC(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.3, "product": "O=C1NC2=CC=C(C=C2C12CCCCC2)C=2N(C=CC2)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
15
MINUTE
To a solution of 5′-bromo-spiro[cyclohexane-1,3′-indolin]-2′-one (3.4 g, 12 mmol) in 1,2-DME (100 mL) under a nitrogen atmosphere was added tetrakis(triphenylphospine)palladium(0) (70 mg, 5 mol %). After 15 min, 2-borono-1H-pyrrole-1-carboxylic acid, 1-tert butyl ester (1.3 eq, 3.31 g, 15.6 mmol) and a solution of K2CO...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCCC1
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCCC1
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
O
80
0.25
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCCC2>O>CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-70f66bc6736f4a80ac413ff2db27ac21
COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1.Cn1c(C#N)ccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2>>Cn1c(C#N)ccc1-c1ccc2c(c1)C1(CCCCC1)C(=S)N2
O.O=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC=C(N2C)C#N.COC=1C=CC(=CC1)P2(=S)SP(=S)(S2)C=3C=CC(=CC3)OC>>S=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC=C(N2C)C#N
COc1ccc(P2(=S)SP(c3ccc(OC)cc3)(=[S:22])S2)cc1.O=[C:21]1[C:15]2([c:13]3[c:12]([cH:11][cH:10][c:9](-[c:8]4[n:2]([CH3:1])[c:3]([C:4]#[N:5])[cH:6][cH:7]4)[cH:14]3)[NH:23]1)[CH2:16][CH2:17][CH2:18][CH2:19][CH2:20]2>>[CH3:1][n:2]1[c:3]([C:4]#[N:5])[cH:6][cH:7][c:8]1-[c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[C:15]1([CH2:16]...
COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1.Cn1c(C#N)ccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
Cn1c(C#N)ccc1-c1ccc2c(c1)C1(CCCCC1)C(=S)N2
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
ca3e51120f3a4b20097412f955afcc8b20206caa645bcb7aa2c74ea9fa008f79
558580c5823c2cfab2cae548a45ef991ba9b53d2e5812b481e23ff3540a5940e
S=C1Nc2ccc(-c3ccc[nH]3)cc2C12CCCCC2
C-O-c1:c:c:c(-P2(=S)-S-P(=[S;H0;D1;+0:1])(-c3:c:c:c(-O-C):c:c:3)-S-2):c:c:1.O=[C;H0;D3;+0:2]1-[#7:3]-[c:4]:[c:5]-[C:6]-1(-[C:7])-[C:8]>>[C:7]-[C:6]1(-[C:8])-[c:5]:[c:4]-[#7:3]-[C;H0;D3;+0:2]-1=[S;H0;D1;+0:1]
90.5
[{"value": 55.0, "product": "S=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC=C(N2C)C#N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.5, "product": "S=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC=C(N2C)C#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
To a solution of 5-(2′-oxospiro[cyclohexane-1,3′-[3H]indol]-5′-yl)-1-methyl-pyrrole-2-carbonitrile (0.55 g, 1.8 mmol, 1 eq) in toluene (50 mL) was added Lawesson's reagent (0.47 g, 1.1 mmol, 0.65 eq) and the reaction was heated to 80° C. for 1 hour. The reaction was cooled to room temperature, poured into water (100 mL...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary amide.Monosulfide.Monosulfide
Thioamide
c1ccccc1.P1SPS1.c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)NCC21CCCCC1
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCCC1
Other
C1(=CC=CC=C1)C
80
null
COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1.Cn1c(C#N)ccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2>C1(=CC=CC=C1)C>Cn1c(C#N)ccc1-c1ccc2c(c1)C1(CCCCC1)C(=S)N2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-70fbe5d426504ba9b0472297ac3af260
ICCCCI.O=C1Cc2ccccc2N1>>O=C1Nc2ccccc2C12CCCC2
N1C(CC2=CC=CC=C12)=O.C(CCC)[Li].ICCCCI.CN(CCN(C)C)C>>N1C(C2(C3=CC=CC=C13)CCCC2)=O
I[CH2:11][CH2:12][CH2:13][CH2:14]I.[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH2:10]1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH2:14]2
ICCCCI.O=C1Cc2ccccc2N1
O=C1Nc2ccccc2C12CCCC2
null
null
C1CCOC1.O
C-C Coupling
OtherReaction
da305b19e438cec6dd9ecd353ca3cd934886dd4c5b3846022dac2a623fceb79e
7b68950fc1047c59bb49c25e850f5a51cbe91a99bb87839c4547aec123110e4b
O=C1Nc2ccccc2C12CCCC2
I-[CH2;D2;+0:1]-[C:2]-[C:3]-[CH2;D2;+0:4]-I.[O;D1;H0:5]=[C:6]1-[#7:7]-[c:8]:[c:9](:[c:10])-[CH2;D2;+0:11]-1>>[O;D1;H0:5]=[C:6]1-[#7:7]-[c:8]:[c:9](:[c:10])-[C;H0;D4;+0:11]-12-[CH2;D2;+0:1]-[C:2]-[C:3]-[CH2;D2;+0:4]-2
50
[{"value": 50.0, "product": "N1C(C2(C3=CC=CC=C13)CCCC2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 50.0, "product": "N1C(C2(C3=CC=CC=C13)CCCC2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
To a −25° C. solution of oxindole (2.0 g, 15.0 mmol) in 40 (cm3) of anhydrous THF under N2 was added n-butyllithium (1.6 M in hexanes, 19.7 cm3, 31.5 mmol) drop-wise. To the resulting milky solution was added N,N,N′,N′-tetramethylethylenediamine (4.75 cm3, 31.5 mmol). After 30 min. a solution of 1,4-diiodobutane (21.9 ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide
null
c1ccc2c(c1)CCN2
c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)NCC21CCCC1
HI
C1CCOC1.O
null
14
ICCCCI.O=C1Cc2ccccc2N1>C1CCOC1.O>O=C1Nc2ccccc2C12CCCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f40b35095113458e955889004f700469
BrBr.O=C1Nc2ccccc2C12CCCC2>>O=C1Nc2ccccc2C12CCCC2Br
C(O)([O-])=O.[Na+].N1C(C2(C3=CC=CC=C13)CCCC2)=O.C(C)(=O)[O-].[Na+].BrBr>>BrC1CCCC12C(NC1=CC=CC=C21)=O
Br[Br:15].[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH2:14]2>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH:14]2[Br:15]
BrBr.O=C1Nc2ccccc2C12CCCC2
O=C1Nc2ccccc2C12CCCC2Br
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
5d1ae453742bff017caef24079c4e11e210e4fe7fcd315c0a1d757dce473ae36
0c353a1260488c22c3ffb72de5623420c3ec35470a0b3a2045b11c29224f458e
O=C1Nc2ccccc2C12CCCC2
Br-[Br;H0;D1;+0:1].[O;D1;H0:2]=[C:3]1-[#7:4]-[c:5]:[c:6]-[C:7]-12-[C:8]-[C:9]-[C:10]-[CH2;D2;+0:11]-2>>[Br;H0;D1;+0:1]-[CH;D3;+0:11]1-[C:10]-[C:9]-[C:8]-[C:7]-12-[c:6]:[c:5]-[#7:4]-[C:3]-2=[O;D1;H0:2]
105
[{"value": 96.0, "product": "BrC1CCCC12C(NC1=CC=CC=C21)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 105.0, "product": "BrC1CCCC12C(NC1=CC=CC=C21)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one (0.27 g, 1.4 mmol) and sodium acetate (0.12 g, 1.46 mmol) in acetic acid (10 cm3) was treated with bromine (0.24 g, 1.51 mmol) in acetic acid (2 cm3). After 30 min. the mixture was poured into sat. sodium hydrogen carbonate solution and extracted with EtOAc (...
10.6084/m9.figshare.5104873.v1
null
null
Secondary halide
c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)NCC21CCCC1
HBr
C(C)(=O)O
null
null
BrBr.O=C1Nc2ccccc2C12CCCC2>C(C)(=O)O>O=C1Nc2ccccc2C12CCCC2Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-00d03b2c1c3b4c2a908a9d526535d5cd
N#Cc1cc(F)cc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O>>N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
C([O-])([O-])=O.[Na+].[Na+].C(#N)C=1C=C(C=C(C1)F)Br.[OH-].[Na+].N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O>>C(#N)C=1C=C(C=C(C1)F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3
Br[c:8]1[cH:7][c:5]([F:6])[cH:4][c:3]([C:2]#[N:1])[cH:23]1.OB(O)[CH:19]1[C:15]2([c:13]3[c:12]([cH:11][cH:10][cH:9][cH:14]3)[NH:22][C:20]2=[O:21])[CH2:16][CH2:17][CH2:18]1>>[N:1]#[C:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[C:15]2([CH2:16][CH2:17][CH2:18][CH2:19]2)[C:20](=[O:21])...
N#Cc1cc(F)cc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O
N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
null
null
O.COCCOC
C-C Coupling
OtherReaction
730dcdc10a1abdabad91331a2b6e5cbbf0777aa3d68588c0d603eed6404753ea
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[CH;D3;+0:6]1-[C:7]-[C:8]-[C:9]-[C:10]-12-[C:11](=[O;D1;H0:12])-[#7:13]-[c:14]1:[c:15]:[c:16]:[cH;D2;+0:17]:[c:18]:[c:19]:1-2>>[O;D1;H0:12]=[C:11]1-[#7:13]-[c:14]2:[c:15]:[c:16]:[c;H0;D3;+0:17](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:18]:[c:19]:2-[C:10]-12-[C:9]...
44
[{"value": 44.0, "product": "C(#N)C=1C=C(C=C(C1)F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 43.9, "product": "C(#N)C=1C=C(C=C(C1)F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-cyano-5-fluoro-bromobenzene (0.5 g, 2.6 mmol), and tetrakis (triphenylphosphine)palladium(0) (0.2 g) in ethylene glycol dimethyl ether (20 cm3) was stirred under N2 for 20 minutes. To this mixture was then added (spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one-5-yl)boronic acid (0.9 g, 3.9 mmol) and sodi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
HBr.B
O.COCCOC
null
null
N#Cc1cc(F)cc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O>O.COCCOC>N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b9142de5693444da9440ade37d4c5c15
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>>CC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
BrC=1C=C2C(C(NC2=CC1)=O)(C)C.ClC=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[K+].[K+]>>ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C
Br[c:10]1[cH:9][cH:8][c:7]2[c:19]([cH:18]1)[C:2]([CH3:1])([CH3:3])[C:4](=[O:5])[NH:6]2.OB(O)[c:11]1[cH:12][cH:13][cH:14][c:15]([Cl:16])[cH:17]1>>[CH3:1][C:2]1([CH3:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][c:15]([Cl:16])[cH:17]3)[cH:18][c:19]21
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1
CC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C(OC)COC.[Cl-].[NH4+]
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
25
[{"value": 25.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 0.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
5-bromo-1,3-dihydro-3,3-dimethyl-2H-indol-2-one (0.98 g, 4.07 mol) and tetrakis(triphenylphosphine)palladium(0) (0.239 g) were stirred under an atmosphere of nitrogen in dimethoxyethane (35 cm3). After 15 min., 3-chlorophenylboronic acid (1.27 g, 8.13 mol) was added, followed by potassium carbonate (3.40 g, 45 mmol) in...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC.[Cl-].[NH4+]
null
0.25
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC.[Cl-].[NH4+]>CC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6c1602386b2f47d482b05454e4845707
CC1(Cc2ccccc2)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1>>CC1(Cc2ccccc2)C(=S)Nc2ccc(-c3cccc(Cl)c3)cc21
C(C1=CC=CC=C1)C1(C(NC2=CC=C(C=C12)C1=CC(=CC=C1)Cl)=O)C.COC=1C=CC(=CC1)P2(=S)SP(=S)(S2)C=3C=CC(=CC3)OC>>C(C1=CC=CC=C1)C1(C(NC2=CC=C(C=C12)C1=CC(=CC=C1)Cl)=S)C
O=[C:10]1[C:2]([CH3:1])([CH2:3][c:4]2[cH:5][cH:6][cH:7][cH:8][cH:9]2)[c:25]2[c:13]([cH:14][cH:15][c:16](-[c:17]3[cH:18][cH:19][cH:20][c:21]([Cl:22])[cH:23]3)[cH:24]2)[NH:12]1.COc1ccc(P2(=S)SP(c3ccc(OC)cc3)(=[S:11])S2)cc1>>[CH3:1][C:2]1([CH2:3][c:4]2[cH:5][cH:6][cH:7][cH:8][cH:9]2)[C:10](=[S:11])[NH:12][c:13]2[cH:14][cH...
CC1(Cc2ccccc2)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1
CC1(Cc2ccccc2)C(=S)Nc2ccc(-c3cccc(Cl)c3)cc21
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
5ed7a1677d229b16df832cbfd7a180a5851f4818c8175b9dd146291c84305872
558580c5823c2cfab2cae548a45ef991ba9b53d2e5812b481e23ff3540a5940e
S=C1Nc2ccc(-c3ccccc3)cc2C1Cc1ccccc1
C-O-c1:c:c:c(-P2(=S)-S-P(=[S;H0;D1;+0:1])(-c3:c:c:c(-O-C):c:c:3)-S-2):c:c:1.O=[C;H0;D3;+0:2]1-[#7:3]-[c:4]:[c:5]-[C:6]-1(-[C:7])-[C;D1;H3:8]>>[C:7]-[C:6]1(-[C;D1;H3:8])-[c:5]:[c:4]-[#7:3]-[C;H0;D3;+0:2]-1=[S;H0;D1;+0:1]
21
[{"value": 21.0, "product": "C(C1=CC=CC=C1)C1(C(NC2=CC=C(C=C12)C1=CC(=CC=C1)Cl)=S)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The title compound was prepared from 3-benzyl-5-(3-chloro-phenyl)-3-methyl-1,3-dihydro-indol-2-one (100 mg) and Lawesson's reagent (120 mg) in toluene (10 ml) at reflux, according to General Procedure A, to afford the title compound (0.022 g) as an off white solid: mp. 168–170° C.; 1H NMR (CDCl3) δ 9.23 (br s, 1H), 7.4...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary amide.Monosulfide.Monosulfide
Thioamide
c1ccc2c(c1)CCN2.c1ccccc1.P1SPS1.c1ccccc1
c1ccc2c(c1)CCN2
c1ccccc1.c1ccc2c(c1)CCN2.c1ccccc1
Other
C1(=CC=CC=C1)C
null
null
CC1(Cc2ccccc2)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1>C1(=CC=CC=C1)C>CC1(Cc2ccccc2)C(=S)Nc2ccc(-c3cccc(Cl)c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1410de5373474c20b5b594a894ba44f8
BrBr.CC1(C)C(=O)Nc2ccccc21>>CC1(C)C(=O)Nc2ccc(Br)cc21
C([O-])([O-])=O.[Na+].[Na+].CC1(C(NC2=CC=CC=C12)=O)C.C(C)(=O)[O-].[Na+].BrBr>>BrC=1C=C2C(C(NC2=CC1)=O)(C)C
Br[Br:11].[CH3:1][C:2]1([CH3:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][cH:10][cH:12][c:13]21>>[CH3:1][C:2]1([CH3:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][c:13]21
BrBr.CC1(C)C(=O)Nc2ccccc21
CC1(C)C(=O)Nc2ccc(Br)cc21
null
null
O.C(C)(=O)O
Functional Group Interconversion
Bromination
e5aad40fc3ec640bed45a7119ff569558b20c39979304f365dafdbc5ae4e4cd4
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1Cc2ccccc2N1
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]:[cH;D2;+0:4]:[c:5]:[c:6]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4](:[c:3]:[c:2]):[c:5]:[c:6]
92
[{"value": 92.0, "product": "BrC=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.0, "product": "BrC=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
50
MINUTE
3,3-dimethyl-indol-2-one (0.65 g, 4.03 mmol) and sodium acetate (0.33 g, 4.07 mmol) were stirred in acetic acid (5 cm3) then bromine (0.66 g, 4.13 mmol) in acetic acid (5 cm3) was added drop-wise to the reaction mixture. The reaction was stirred for 50 min., then poured into water. The mixture was basified with sodium ...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
HBr
O.C(C)(=O)O
null
0.833333
BrBr.CC1(C)C(=O)Nc2ccccc21>O.C(C)(=O)O>CC1(C)C(=O)Nc2ccc(Br)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-50462c2ef19b45b9985f6de89953a1bc
CC1(C)C(=O)Nc2ccc(Br)cc21.COc1cccc(B(O)O)c1>>COc1cccc(-c2ccc3c(c2)C(C)(C)C(=O)N3)c1
[Cl-].[NH4+].BrC=1C=C2C(C(NC2=CC1)=O)(C)C.COC=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[K+].[K+]>>COC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C
Br[c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[C:14]([CH3:15])([CH3:16])[C:17](=[O:18])[NH:19]2.OB(O)[c:7]1[cH:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:20]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13]2)[C:14]([CH3:15])([CH3:16])[C:17](=[O:18])[NH:19]3)[cH:20]1
CC1(C)C(=O)Nc2ccc(Br)cc21.COc1cccc(B(O)O)c1
COc1cccc(-c2ccc3c(c2)C(C)(C)C(=O)N3)c1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
CCOC(=O)C.O.C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:2]:[c:3]
31
[{"value": 31.0, "product": "COC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 29.8, "product": "COC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
5-bromo-1,3-dihydro-3,3-dimethyl-2H-indol-2-one (0.33 g, 1.38 mmol) and tetrakis(triphenylphosphine)palladium(0) (0.094 g) were stirred under an atmosphere of nitrogen in dimethoxyethane (12 cm3). After 15 minutes, 3-methoxyphenylboronic acid (0.42 g, 2.76 mmol) was added, followed by potassium carbonate (1.15 g, 8.34 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccccc1.c1ccc2c(c1)CCN2
c1ccccc1.c1ccc2c(c1)CCN2
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CCOC(=O)C.O.C(OC)COC
null
0.25
CC1(C)C(=O)Nc2ccc(Br)cc21.COc1cccc(B(O)O)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CCOC(=O)C.O.C(OC)COC>COc1cccc(-c2ccc3c(c2)C(C)(C)C(=O)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-89c517760b0f47fbbd4ca1ae0d7c1d26
CN(C)C=O.Cc1ccsc1Br>>Cc1cc(C=O)sc1Br
BrC=1SC=CC1C.C(C)NCC.[Li]CCCC.CN(C)C=O>>BrC1=C(C=C(S1)C=O)C
CN(C)[CH:5]=[O:6].[CH3:1][c:2]1[cH:3][cH:4][s:7][c:8]1[Br:9]>>[CH3:1][c:2]1[cH:3][c:4]([CH:5]=[O:6])[s:7][c:8]1[Br:9]
CN(C)C=O.Cc1ccsc1Br
Cc1cc(C=O)sc1Br
null
null
C1CCOC1.CCCCCC
C-C Coupling
OtherReaction
77a8917ac8ed8f2ad464b767187c983c24a719c711c4936bfe09b270792882f5
f0bd75a0630092c31f21f61f4a015c77ae0dff14a0b742b4370d7a38fda490f7
c1ccsc1
C-N(-C)-[CH;D2;+0:1]=[O;D1;H0:2].[#16;a:3]1:[c:4]:[c:5]:[c:6]:[cH;D2;+0:7]:1>>[O;D1;H0:2]=[CH;D2;+0:1]-[c;H0;D3;+0:7]1:[#16;a:3]:[c:4]:[c:5]:[c:6]:1
88.3
[{"value": 88.3, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
-40
CELSIUS
30
MINUTE
To a solution of diethylamine (28 g, 0.383 mol) in anhydrous THF (400 mL) was added at −40° C. under nitrogen a solution of n-BuLi (2.5 M, 153 mL, 0.383 mol) in hexane. After addition, the solution was stirred at −40° C. under nitrogen for 30 minutes, cooled to −78° C. and treated dropwise with a solution of 2-bromo-3-...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide
Aldehyde
c1ccsc1
c1ccsc1
c1ccsc1
Other
C1CCOC1.CCCCCC
-40
0.5
CN(C)C=O.Cc1ccsc1Br>C1CCOC1.CCCCCC>Cc1cc(C=O)sc1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-919f5637e2fc42948973a9ffeda0599d
CCI.O=C1Cc2ccccc2N1>>CCC1=c2ccccc2=NC1=O
ICC.N1C(CC2=CC=CC=C12)=O.C(CCC)[Li].[NH4+].[Cl-].CN(CCN(C)C)C>>C(C)C=1C(N=C2C=CC=CC12)=O
I[CH2:2][CH3:1].[CH2:3]1[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[NH:10][C:11]1=[O:12]>>[CH3:1][CH2:2][C:3]1=[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2=[N:10][C:11]1=[O:12]
CCI.O=C1Cc2ccccc2N1
CCC1=c2ccccc2=NC1=O
null
null
C1CCOC1
C-C Coupling
OtherReaction
7f8efd166912a03506850ad77dd8b310e9bbf110f40dc0aa3466aad53303d70b
9795126e672adf3dfeb9ebcd165d02e10eb1b4ac31d83997fdca7c7a739d39dc
O=C1C=c2ccccc2=N1
I-[CH2;D2;+0:1]-[C;D1;H3:2].[O;D1;H0:3]=[C:4]1-[CH2;D2;+0:5]-[c;H0;D3;+0:6]2:[c:7]:[c:8]:[c:9]:[c:10]:[c;H0;D3;+0:11]:2-[NH;D2;+0:12]-1>>[C;D1;H3:2]-[CH2;D2;+0:1]-[C;H0;D3;+0:5]1=[c;H0;D3;+0:6]2:[c:7]:[c:8]:[c:9]:[c:10]:[c;H0;D3;+0:11]:2=[N;H0;D2;+0:12]-[C:4]-1=[O;D1;H0:3]
2.9
[{"value": 2.9, "product": "C(C)C=1C(N=C2C=CC=CC12)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of oxindole (40 g, 0.3 mol) in dry THF (400 ml) under N2 was cooled to −25° C. and treated drop wise with n-butyl lithium (2.5M in hexanes, 240 ml, 0.6 mol). To the resulting solution was added N,N,N′,N′-tetramethylethylenediamine (90.4 ml, 0.6 mol). After 30 min. iodoethane (48 ml, 0.6 mol) was added and th...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amide
null
c1ccc2c(c1)CCN2
C1=c2ccccc2=NC1
C1=c2ccccc2=NC1
HI
C1CCOC1
null
null
CCI.O=C1Cc2ccccc2N1>C1CCOC1>CCC1=c2ccccc2=NC1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2b44cd7d278c4cc8bad2b58a6a049672
CCC1=c2ccccc2=NC1=O.CCI>>CCC1(CC)C(=O)Nc2ccccc21
ICC.C(C)C=1C(N=C2C=CC=CC12)=O.C(CCC)[Li].[NH4+].[Cl-].CN(CCN(C)C)C>>C(C)C1(C(NC2=CC=CC=C12)=O)CC
[C:3]1([CH2:4][CH3:5])=[c:14]2[c:9]([cH:10][cH:11][cH:12][cH:13]2)=[N:8][C:6]1=[O:7].I[CH2:2][CH3:1]>>[CH3:1][CH2:2][C:3]1([CH2:4][CH3:5])[C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]21
CCC1=c2ccccc2=NC1=O.CCI
CCC1(CC)C(=O)Nc2ccccc21
null
null
C1CCOC1
C-C Coupling
OtherReaction
f15f58906703f12b51d1da977226590dc73f51d4fa9868a7b3d7ebfdcc2201e7
53812deded8d8876ba2f198bf967d0e3a8cebb6ae8cbe5dd02b6ae90ad0b6669
O=C1Cc2ccccc2N1
I-[CH2;D2;+0:1]-[C;D1;H3:2].[C;D1;H3:3]-[C:4]-[C;H0;D3;+0:5]1=[c;H0;D3;+0:6]2:[c:7]:[c:8]:[c:9]:[c:10]:[c;H0;D3;+0:11]:2=[N;H0;D2;+0:12]-[C:13]-1=[O;D1;H0:14]>>[C;D1;H3:2]-[CH2;D2;+0:1]-[C;H0;D4;+0:5]1(-[C:4]-[C;D1;H3:3])-[C:13](=[O;D1;H0:14])-[NH;D2;+0:12]-[c;H0;D3;+0:11]2:[c:10]:[c:9]:[c:8]:[c:7]:[c;H0;D3;+0:6]:2-1
47.6
[{"value": 45.0, "product": "C(C)C1(C(NC2=CC=CC=C12)=O)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 47.6, "product": "C(C)C1(C(NC2=CC=CC=C12)=O)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-ethyl-indol-2-one (16 g, 0.1 mol) in dry THF (200 ml) under N2 was cooled to −25° C. and treated drop wise with n-butyllithium (2.5M in hexanes, 80 ml, 0.2 mol). To the resulting solution was added N,N,N′,N′-tetramethylethylenediamine (30 ml, 0.2 mol). After 30 min. iodoethane (8 ml, 0.1 mol) was added ...
10.6084/m9.figshare.5104873.v1
null
Primary halide
Secondary amide
C1=c2ccccc2=NC1
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
I-
C1CCOC1
null
null
CCC1=c2ccccc2=NC1=O.CCI>C1CCOC1>CCC1(CC)C(=O)Nc2ccccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-556c1aea34984edebf71a28e879e10a3
BrBr.CCC1(CC)C(=O)Nc2ccccc21>>CCC1(CC)C(=O)Nc2ccc(Br)cc21
C(C)C1(C(NC2=CC=CC=C12)=O)CC.C(C)(=O)[O-].[Na+].BrBr>>BrC=1C=C2C(C(NC2=CC1)=O)(CC)CC
Br[Br:13].[CH3:1][CH2:2][C:3]1([CH2:4][CH3:5])[C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][cH:12][cH:14][c:15]21>>[CH3:1][CH2:2][C:3]1([CH2:4][CH3:5])[C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][c:15]21
BrBr.CCC1(CC)C(=O)Nc2ccccc21
CCC1(CC)C(=O)Nc2ccc(Br)cc21
null
null
O.C(C)(=O)O
Functional Group Interconversion
Bromination
e5aad40fc3ec640bed45a7119ff569558b20c39979304f365dafdbc5ae4e4cd4
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1Cc2ccccc2N1
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]:[cH;D2;+0:4]:[c:5]:[c:6]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4](:[c:3]:[c:2]):[c:5]:[c:6]
null
[]
null
null
null
null
A solution of 3,3-diethylindol-2-one (8 g, 40 mmol) and sodium acetate (4 g, 48 mmol) in acetic acid (100 ml) was treated with bromine (6.4 g, 40 mmol). After 30 min. the mixture was diluted with water and extracted with EtOAc (2×); the combined organic layers were washed with water, sat. sodium hydrogen carbonate solu...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
HBr
O.C(C)(=O)O
null
null
BrBr.CCC1(CC)C(=O)Nc2ccccc21>O.C(C)(=O)O>CCC1(CC)C(=O)Nc2ccc(Br)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6ee58afad1c54d4ca431da562fb42f20
CCC1(CC)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>>CCC1(CC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
BrC=1C=C2C(C(NC2=CC1)=O)(CC)CC.ClC=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[K+].[K+]>>ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(CC)CC
Br[c:12]1[cH:11][cH:10][c:9]2[c:21]([cH:20]1)[C:3]([CH2:2][CH3:1])([CH2:4][CH3:5])[C:6](=[O:7])[NH:8]2.OB(O)[c:13]1[cH:14][cH:15][cH:16][c:17]([Cl:18])[cH:19]1>>[CH3:1][CH2:2][C:3]1([CH2:4][CH3:5])[C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12](-[c:13]3[cH:14][cH:15][cH:16][c:17]([Cl:18])[cH:19]3)[cH:20][c:21]21
CCC1(CC)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1
CCC1(CC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C(OC)COC.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
27
[{"value": 27.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(CC)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 26.7, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(CC)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-bromo-1,3-dihydro-3,3-diethyl-[2H]-indol-2-one (2.7 g, 10 mmol), 3-chlorophenylboronic acid (1.6 g, 10 mmol), potassium carbonate (4 g, 30 mmol) and tetrakis(triphenylphosphine)palladium(0) (0.5 g, 0.4 mmol) in dimethoxyethane (100 ml), ethanol (25 ml), and water (25 ml) was heated to reflux for 6 hours...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC.C(C)O
null
null
CCC1(CC)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC.C(C)O>CCC1(CC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b2ba3a136dae496caa6ed5d95948979f
CCC1(CC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1>>CCC1(CC)C(=S)Nc2ccc(-c3cccc(Cl)c3)cc21
ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(CC)CC.COC=1C=CC(=CC1)P2(=S)SP(=S)(S2)C=3C=CC(=CC3)OC>>ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=S)(CC)CC
O=[C:6]1[C:3]([CH2:2][CH3:1])([CH2:4][CH3:5])[c:21]2[c:9]([cH:10][cH:11][c:12](-[c:13]3[cH:14][cH:15][cH:16][c:17]([Cl:18])[cH:19]3)[cH:20]2)[NH:8]1.COc1ccc(P2(=S)SP(c3ccc(OC)cc3)(=[S:7])S2)cc1>>[CH3:1][CH2:2][C:3]1([CH2:4][CH3:5])[C:6](=[S:7])[NH:8][c:9]2[cH:10][cH:11][c:12](-[c:13]3[cH:14][cH:15][cH:16][c:17]([Cl:18]...
CCC1(CC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1
CCC1(CC)C(=S)Nc2ccc(-c3cccc(Cl)c3)cc21
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
5ed7a1677d229b16df832cbfd7a180a5851f4818c8175b9dd146291c84305872
558580c5823c2cfab2cae548a45ef991ba9b53d2e5812b481e23ff3540a5940e
S=C1Cc2cc(-c3ccccc3)ccc2N1
C-O-c1:c:c:c(-P2(=S)-S-P(=[S;H0;D1;+0:1])(-c3:c:c:c(-O-C):c:c:3)-S-2):c:c:1.O=[C;H0;D3;+0:2]1-[#7:3]-[c:4]:[c:5]-[C:6]-1(-[C:7])-[C:8]>>[C:7]-[C:6]1(-[C:8])-[c:5]:[c:4]-[#7:3]-[C;H0;D3;+0:2]-1=[S;H0;D1;+0:1]
null
[]
null
null
null
null
The title compound was prepared from 5-(3-chloro-phenyl)-3,3-diethyl-1,3-dihydro-indol-2-one compound (100 mg) and Lawesson's reagent (100 mg) in toluene (10 ml) at reflux, according to General Procedure A, to afford the product (0.023 g) as a yellow solid: 1H NMR (DMSO-d6) δ 12.73 (br s, 1H), 7.77 (t, 1H, J=1.8 Hz), 7...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary amide.Monosulfide.Monosulfide
Thioamide
c1ccc2c(c1)CCN2.c1ccccc1.P1SPS1.c1ccccc1
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2.c1ccccc1
Other
C1(=CC=CC=C1)C
null
null
CCC1(CC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1>C1(=CC=CC=C1)C>CCC1(CC)C(=S)Nc2ccc(-c3cccc(Cl)c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2a5db7c4f64e47bcb8b812a4d9f7db0b
CSC1=Nc2ccc(Br)cc2C12CCCCC2.NOCc1ccccc1>>Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2
BrC=1C=C2C3(C(=NC2=CC1)SC)CCCCC3.Cl.C(C1=CC=CC=C1)ON>>C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)Br
CS[C:14]1=[N:24][c:5]2[cH:4][cH:3][c:2]([Br:1])[cH:7][c:6]2[C:8]12[CH2:9][CH2:10][CH2:11][CH2:12][CH2:13]2.[NH2:15][O:16][CH2:17][c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[Br:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[C:8]1([CH2:9][CH2:10][CH2:11][CH2:12][CH2:13]1)[C:14](=[N:15][O:16][CH2:17][c:18]1[cH:19][cH:20][cH:2...
CSC1=Nc2ccc(Br)cc2C12CCCCC2.NOCc1ccccc1
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2
null
null
CO
Heteroatom Alkylation and Arylation
OtherReaction
b7e408d847daf7a54697e7f466696f5de562d32f1fb12304c1fd1aaf97ca6430
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
c1ccc(CON=C2Nc3ccccc3C23CCCCC3)cc1
C-S-[C;H0;D3;+0:1]1=[N;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]-[C:6]-1(-[C:7])-[C:8].[C:9]-[#8:10]-[NH2;D1;+0:11]>>[C:7]-[C:6]1(-[C:8])-[c:5]:[c:3](:[c:4])-[NH;D2;+0:2]-[C;H0;D3;+0:1]-1=[N;H0;D2;+0:11]-[#8:10]-[C:9]
null
[]
45
CELSIUS
null
null
5′-Bromo-2′-(methylthio)spiro[cyclohexane-1,3′-[3H]indole] (9.0 g, 28.98 mmol) and O-benzylhydroxylamine hydrochloride (13.8 g, 86.9 mmol) were combined in methanol (150 mL) and heated to 45° C. for 6 hours. Methanol was evaporated in vacuo. Ethyl acetate was added to the residue and this mixture was washed with ammoni...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
C1=Nc2ccccc2C12CCCCC2
c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
Other
CO
45
null
CSC1=Nc2ccc(Br)cc2C12CCCCC2.NOCc1ccccc1>CO>Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6a3ce03affcd467280633224e16787b9
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.OB(O)c1ccc(F)cc1>>Fc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)cc1
CCCCCC.C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)Br.FC1=CC=C(C=C1)B(O)O>>C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC=C(C=C2)F
Br[c:6]1[cH:7][cH:8][c:9]2[c:10]([cH:11]1)[C:12]1([CH2:13][CH2:14][CH2:15][CH2:16][CH2:17]1)[C:18](=[N:19][O:20][CH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1)[NH:28]2.OB(O)[c:5]1[cH:4][cH:3][c:2]([F:1])[cH:30][cH:29]1>>[F:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]3[c:10]([cH:11]2)[C:12]2([CH2:13][CH2:14][...
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.OB(O)c1ccc(F)cc1
Fc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)cc1
null
null
C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
8734c5dd9f1a6e6409bcbbc53c99a0241dd1b8ab9806eccd050fa6b5202b7ad6
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(CON=C2Nc3ccc(-c4ccccc4)cc3C23CCCCC3)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
67
[{"value": 67.0, "product": "C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC=C(C=C2)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.4, "product": "C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC=C(C=C2)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Prepared from 5′-bromospiro{cyclohexane-1,3′-[3H]indol}-2′(1′H)-one 2′(O-benzyloxime) (1.0 g, 2.6 mmol), and 4-fluorophenyl boronic acid (0.72 g, 5.2 mmol) according to Example 45 procedure A. The product was purified by flash silica gel chromatography; (eluant: 10:0.5 hexane:ethyl acetate) to give the desired product ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)NCC21CCCCC1.c1ccccc1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
C(C)(=O)OCC
null
null
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.OB(O)c1ccc(F)cc1>C(C)(=O)OCC>Fc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a7b50e2533454ec0abc01181cf564b57
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.OB(O)c1ccc(F)c(F)c1>>Fc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)cc1F
C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)Br.FC=1C=C(C=CC1F)B(O)O>>C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC(=C(C=C2)F)F
Br[c:6]1[cH:7][cH:8][c:9]2[c:10]([cH:11]1)[C:12]1([CH2:13][CH2:14][CH2:15][CH2:16][CH2:17]1)[C:18](=[N:19][O:20][CH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1)[NH:28]2.OB(O)[c:5]1[cH:4][cH:3][c:2]([F:1])[c:30]([F:31])[cH:29]1>>[F:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]3[c:10]([cH:11]2)[C:12]2([CH2:13][C...
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.OB(O)c1ccc(F)c(F)c1
Fc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)cc1F
null
null
C1CCOC1.O
C-C Coupling
Suzuki coupling with boronic acids
8734c5dd9f1a6e6409bcbbc53c99a0241dd1b8ab9806eccd050fa6b5202b7ad6
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(CON=C2Nc3ccc(-c4ccccc4)cc3C23CCCCC3)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
69
[{"value": 69.0, "product": "C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC(=C(C=C2)F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Prepared from 5′-bromospiro{cyclohexane-1,3′-[3H]indol}-2′(1′H)-one 2′(O-benzyloxime) (1.0 g, 2.6 mmol) and 3,4-diflurophenyl boronic acid (1.6 g, 5.2 mmol of a 50% solution of acid in THF/water) according to Example 45 procedure A. The product was purified by flash silica gel chromatography (eluant: 10:0.5 hexane:ethy...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)NCC21CCCCC1.c1ccccc1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
C1CCOC1.O
null
null
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.OB(O)c1ccc(F)c(F)c1>C1CCOC1.O>Fc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)cc1F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-505d378986564b289b6586ca9291e8b6
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.COc1cccc(B(O)O)c1>>COc1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)c1
CCCCCC.C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)Br.COC=1C=C(C=CC1)B(O)O>>C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC(=CC=C2)OC
Br[c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[C:14]1([CH2:15][CH2:16][CH2:17][CH2:18][CH2:19]1)[C:20](=[N:21][O:22][CH2:23][c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1)[NH:30]2.OB(O)[c:7]1[cH:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:31]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13]2)[C...
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.COc1cccc(B(O)O)c1
COc1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)c1
null
null
C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
8734c5dd9f1a6e6409bcbbc53c99a0241dd1b8ab9806eccd050fa6b5202b7ad6
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(CON=C2Nc3ccc(-c4ccccc4)cc3C23CCCCC3)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:2]:[c:3]
75
[{"value": 75.0, "product": "C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC(=CC=C2)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.1, "product": "C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC(=CC=C2)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Prepared from 5′-bromospiro{cyclohexane-1,3′-[3H]indol}-2′(1′H)-one 2′(O-benzyloxime) (1.0 g, 2.6 mmol) and 3-methoxyphenyl boronic acid (0.79 g, 5.2 mmol) according to Example 45 procedure A. The product was purified by flash silica gel chromatography; (eluant: 10:0.5 hexane:ethyl acetate) to give the desired product ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)NCC21CCCCC1.c1ccccc1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
C(C)(=O)OCC
null
null
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.COc1cccc(B(O)O)c1>C(C)(=O)OCC>COc1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0339de4b5b6c487c862e7caab6206f02
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.O=[N+]([O-])c1cccc(B(O)O)c1>>O=[N+]([O-])c1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)c1
C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)Br.[N+](=O)([O-])C=1C=C(C=CC1)B(O)O>>C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC(=CC=C2)[N+](=O)[O-]
Br[c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[C:15]1([CH2:16][CH2:17][CH2:18][CH2:19][CH2:20]1)[C:21](=[N:22][O:23][CH2:24][c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1)[NH:31]2.OB(O)[c:8]1[cH:7][cH:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:32]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]3...
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.O=[N+]([O-])c1cccc(B(O)O)c1
O=[N+]([O-])c1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
8734c5dd9f1a6e6409bcbbc53c99a0241dd1b8ab9806eccd050fa6b5202b7ad6
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(CON=C2Nc3ccc(-c4ccccc4)cc3C23CCCCC3)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
55
[{"value": 55.0, "product": "C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC(=CC=C2)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 53.8, "product": "C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)C2=CC(=CC=C2)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Prepared from 5′-bromospiro{cyclohexane-1,3′-[3H]indol}-2′(1′H)-one 2′(O-benzyloxime) (1.0 g, 2.6 mmol) and 3-Nitrophenyl boronic acid (0.86 g, 5.2 mmol) according to Example 45 procedure A. Purification by flash silica gel chromatography (eluant: 10:0.5 hexane:ethyl acetate) afforded the desired compound (0.60 g, 1.4 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)NCC21CCCCC1.c1ccccc1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
null
null
null
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.O=[N+]([O-])c1cccc(B(O)O)c1>>O=[N+]([O-])c1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NOCc2ccccc2)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0c8aec81ccc749b5850d7d06995e26e2
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.N#Cc1cccc(B(O)O)c1>>N#Cc1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NO)N3)c1
C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)Br.C(#N)C=1C=C(C=CC1)B(O)O>>C(#N)C=1C=C(C=CC1)C=1C=C2C3(C(NC2=CC1)=NO)CCCCC3
Br[c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[C:14]1([CH2:15][CH2:16][CH2:17][CH2:18][CH2:19]1)[C:20](=[N:21][O:22]Cc1ccccc1)[NH:23]2.OB(O)[c:7]1[cH:6][cH:5][cH:4][c:3]([C:2]#[N:1])[cH:24]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13]2)[C:14]2([CH2:15][CH2:16][CH2:17][CH2:18][CH2:1...
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.N#Cc1cccc(B(O)O)c1
N#Cc1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NO)N3)c1
null
null
C(C1=CC=CC=C1)#N
C-C Coupling
OtherReaction
07b6e6d68ffe0d8fe0c6094199408af1101acbbbfc3a96507d90206e95662212
e4b7a679ed09f6e9e384aa87a819f1defd661035a1c737866741e2bca62ab2cd
N=C1Nc2ccc(-c3ccccc3)cc2C12CCCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]-[C:4]-[C:5](=[#7:6]-[O;H0;D2;+0:7]-C-c1:c:c:c:c:c:1)-[#7:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]>>[#7:8]-[C:5](=[#7:6]-[OH;D1;+0:7])-[C:4]-[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]):[c:9]:[c:10]
71
[{"value": 71.0, "product": "C(#N)C=1C=C(C=CC1)C=1C=C2C3(C(NC2=CC1)=NO)CCCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.2, "product": "C(#N)C=1C=C(C=CC1)C=1C=C2C3(C(NC2=CC1)=NO)CCCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
3-[Spiro[cyclohexane-1,3′-[3H]indol]-(1′H)-one-2′-(O-benzyloxime)]benzonitrile[3H]indol]-5-yl]benzonitrile. Prepared from 5′-bromospiro{cyclohexane-1,3′-[3H]indol}-2′(1′H)-one 2′(O-benzyloxime) (1.0 g, 2.6 mmol) and 3-cyanophenyl boronic acid (0.76 g, 5.2 mmol) according to Example 45 procedure A. The product was purif...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
Oxime
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1.c1ccccc1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
C(C1=CC=CC=C1)#N
null
null
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.N#Cc1cccc(B(O)O)c1>C(C1=CC=CC=C1)#N>N#Cc1cccc(-c2ccc3c(c2)C2(CCCCC2)C(=NO)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-542e11faf0c04255953d092e54cc0035
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.N#Cc1cc(F)cc(Br)c1>>N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=NO)N3)c1
C(C1=CC=CC=C1)ON=C1NC2=CC=C(C=C2C12CCCCC2)Br.C([O-])([O-])=O.[Na+].[Na+].FC=1C=C(C=C(C1)C#N)Br.C(C)(=O)[O-].[K+]>>ON=C1NC2=CC=C(C=C2C12CCCCC2)C=2C=C(C#N)C=C(C2)F
Br[c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[C:15]1([CH2:16][CH2:17][CH2:18][CH2:19][CH2:20]1)[C:21](=[N:22][O:23]Cc1ccccc1)[NH:24]2.Br[c:8]1[cH:7][c:5]([F:6])[cH:4][c:3]([C:2]#[N:1])[cH:25]1>>[N:1]#[C:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[C:15]2([CH2:16][CH2:17][CH2:18][CH...
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.N#Cc1cc(F)cc(Br)c1
N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=NO)N3)c1
null
Cl[Pd]Cl.Cl[Pd]Cl
CN(C)C=O
C-C Coupling
OtherReaction
ef2298fe43b7ac763c63c8842faa33441ac9511774f9ae9610bb64b322049b00
c817a1ff3d935ee2a58f4808dfe267bc36b8ffa48b144e313e0aa8a164a83fc5
N=C1Nc2ccc(-c3ccccc3)cc2C12CCCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].Br-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]-[C:11]-[C:12](=[#7:13]-[O;H0;D2;+0:14]-C-c1:c:c:c:c:c:1)-[#7:15]>>[#7:15]-[C:12](=[#7:13]-[OH;D1;+0:14])-[C:11]-[c:10]:[c:9]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:7]:[c:8]
66
[{"value": 66.0, "product": "ON=C1NC2=CC=C(C=C2C12CCCCC2)C=2C=C(C#N)C=C(C2)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.0, "product": "ON=C1NC2=CC=C(C=C2C12CCCCC2)C=2C=C(C#N)C=C(C2)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
8
HOUR
To a solution of 3-fluoro-5-cyano-bromobenzene (0.4 g, 2.0 mmol) in dry DMF (10 ml) was added diboron pinacolate ester (0.63 g, 2.5 mmol), potassium acetate (0.65 g, 6.7 mmol) and PdCl2 (dppf) (0.2 g) and the reaction was heated to 80° C. under a nitrogen atmosphere. After 8 h. from 5′-bromospiro{cyclohexane-1,3′-[3H]i...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide
Oxime
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1.c1ccccc1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr
Cl[Pd]Cl.Cl[Pd]Cl.CN(C)C=O
80
8
Brc1ccc2c(c1)C1(CCCCC1)C(=NOCc1ccccc1)N2.N#Cc1cc(F)cc(Br)c1>Cl[Pd]Cl.Cl[Pd]Cl.CN(C)C=O>N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=NO)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a9e750599b754d7482e18a1d5914ad02
NN.O.ONC1CCCCC12C=Nc1ccc(-c3cccc(Cl)c3)cc12>>NC1=Nc2ccc(-c3cccc(Cl)c3)cc2C12CCCCC2.[NH4+].[OH-]
ClC=1C=C(C=CC1)C=1C=C2C3(C=NC2=CC1)C(CCCC3)NO.O.NN>>[OH-].[NH4+].ClC=1C=C(C=CC1)C=1C=C2C3(C(=NC2=CC1)N)CCCCC3
[NH2:1][NH2:23].[OH2:24].ON[CH:22]1[C:17]2([CH:2]=[N:3][c:4]3[cH:5][cH:6][c:7](-[c:8]4[cH:9][cH:10][cH:11][c:12]([Cl:13])[cH:14]4)[cH:15][c:16]32)[CH2:18][CH2:19][CH2:20][CH2:21]1>>[NH2:1][C:2]1=[N:3][c:4]2[cH:5][cH:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][c:12]([Cl:13])[cH:14]3)[cH:15][c:16]2[C:17]12[CH2:18][CH2:19][CH2:20...
NN.O.ONC1CCCCC12C=Nc1ccc(-c3cccc(Cl)c3)cc12
NC1=Nc2ccc(-c3cccc(Cl)c3)cc2C12CCCCC2.[NH4+].[OH-]
null
[Ni]
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
4b8d9cea12497294d88671b36f0603d21a5cc32675f08f66455fb407789c7e10
247f27afc29ce267bfe640918462fc5d7b8113f354fd4db111896ba3ae4e0a45
C1=Nc2ccc(-c3ccccc3)cc2C12CCCCC2
O-N-[CH;D3;+0:1](-[C:2]-[C:3])-[C:4]1(-[C:5])-[CH;D2;+0:6]=[#7:7]-[c:8]:[c:9]-1.[NH2;D1;+0:10]-[NH2;D1;+0:11].[OH2;D0;+0:12]>>[C:5]-[C:4]1(-[CH2;D2;+0:1]-[C:2]-[C:3])-[c:9]:[c:8]-[#7:7]=[C;H0;D3;+0:6]-1-[NH2;D1;+0:10].[NH4+;D0:11].[OH-;D0:12]
130.4
[{"value": 0.1, "product": "[OH-].[NH4+]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C3(C(=NC2=CC1)N)CCCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 130.4, "product": "ClC=1C=C(C=CC1)C=1C=C2C3(C(=NC2=CC1)N)CCCCC3", "details": "CALCULATEDPERCEN...
55
CELSIUS
45
MINUTE
To a turbid solution of 5′-(3-Chlorophenyl)-N-hydroxyspiro[cyclohexane-1,3-[3H]indol]-2-amine (0.500 g; 1.53 mmol) in 25 mL of ethanol was added hydrazine hydrate (0.600 mL; 12.24 mmol). The solution was warmed to 55° C., where Raney-nickel (50% in water) was added to the reaction to keep a constant evolution of gas. A...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Substituted imine.Secondary amine
Primary amine
C1=Nc2ccccc2C12CCCCC2
C1=Nc2ccccc2C12CCCCC2
c1ccccc1.C1=Nc2ccccc2C12CCCCC2
HO-
[Ni].C(C)O
55
0.75
NN.O.ONC1CCCCC12C=Nc1ccc(-c3cccc(Cl)c3)cc12>[Ni].C(C)O>NC1=Nc2ccc(-c3cccc(Cl)c3)cc2C12CCCCC2.[NH4+].[OH-]
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-dd39daf5a58f4d5c9e45cf979091f75a
COC(=O)COc1ccc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)cc1C>>Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O
O.Cl.COC(COC1=C(C=C(C=C1)SCC=C(C1=CC=C(C=C1)Br)C1=CC=C(C=C1)Br)C)=O.[OH-].[Na+]>>BrC1=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)Br
C[O:30][C:28]([CH2:27][O:26][c:25]1[c:2]([CH3:1])[cH:3][c:4]([S:5][CH2:6][CH:7]=[C:8]([c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]2)[c:16]2[cH:17][cH:18][c:19]([Br:20])[cH:21][cH:22]2)[cH:23][cH:24]1)=[O:29]>>[CH3:1][c:2]1[cH:3][c:4]([S:5][CH2:6][CH:7]=[C:8]([c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]2)[c:16...
COC(=O)COc1ccc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)cc1C
Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O
null
null
C(C)O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
C(CSc1ccccc1)=C(c1ccccc1)c1ccccc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
93.5
[{"value": 93.0, "product": "BrC1=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.5, "product": "BrC1=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of {4-[3,3-bis-(4-bromo-phenyl)-allylsulfanyl]-2-methyl-phenoxy}-acetic acid methyl ester (530 mg, 0.94 mmol) in ethanol (20 ml) and 1M NaOH (2.0 ml, 2.0 mmol) was stirred at room temp. for 2 h. The reaction mixture added water (20 ml) and 1N HCl (3.0 ml). The water phase was extracted with dichloromethane (...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccccc1
Other
C(C)O
null
null
COC(=O)COc1ccc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)cc1C>C(C)O>Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-98105445b39e4979b24da4a8f78d2882
Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O.OB(O)c1ccccc1>>Cc1cc(SCC=C(c2ccc(-c3ccccc3)cc2)c2ccc(-c3ccccc3)cc2)ccc1OCC(=O)O
BrC1=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)Br.C1(=CC=CC=C1)B(O)O.[F-].[K+].[Cl-].[NH4+]>>C1(=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)C1=CC=CC=C1)C1=CC=CC=C1
Br[c:12]1[cH:11][cH:10][c:9]([C:8](=[CH:7][CH2:6][S:5][c:4]2[cH:3][c:2]([CH3:1])[c:35]([O:36][CH2:37][C:38](=[O:39])[OH:40])[cH:34][cH:33]2)[c:21]2[cH:13][cH:23][c:24](Br)[cH:31][cH:32]2)[cH:20][cH:19]1.OB(O)[c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1>>[CH3:1][c:2]1[cH:3][c:4]([S:5][CH2:6][CH:7]=[C:8]([c:9]2[cH:10][cH:...
Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O.OB(O)c1ccccc1
Cc1cc(SCC=C(c2ccc(-c3ccccc3)cc2)c2ccc(-c3ccccc3)cc2)ccc1OCC(=O)O
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].CC(C)([P](C(C)(C)C)([Pd][P](C(C)(C)C)(C(C)(C)C)C(C)(C)C)C(C)(C)C)C
C1CCOC1
C-C Coupling
OtherReaction
f401823538ae6a41b0707d4f934f9582ed0798088e8db44163a0909a254467ad
b431b00445693c7ae33759145152dfe407ee85c3562148bfc9cb7e8a06213bb6
C(CSc1ccccc1)=C(c1ccc(-c2ccccc2)cc1)c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[C:5](=[C:6]-[C:7])-[c;H0;D3;+0:8]2:[c:9]:[c:10]:[c;H0;D3;+0:11](-Br):[cH;D2;+0:12]:[cH;D2;+0:13]:2):[c:14]:[c:15]:1.O-B(-O)-[c;H0;D3;+0:16](:[c:17]:[c:18]):[c:19]:[c:20]>>[C:7]-[C:6]=[C:5](-[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:13](:[c:21]:[c:22]):[c:23]:[c:24]):[c:15]:[c...
null
[]
null
null
1
HOUR
In an evaporated schlenk flask kept under nitrogen atmosphere were added {4-[3,3-bis-(4-bromo-phenyl)-allylsulfanyl]-2-methyl-phenoxy}-acetic acid (297 mg, 0.54 mmol), phenylboronic acid (152 mg, 1.2 mmol), KF (104 mg, 1.79 mmol), Pd2(dba)3 (30 mg, 33 mmol) and Pd(P(t-Bu)3)2 (33 mg, 65 mmol). THF (6 ml) was added to th...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
Br-.B
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].CC(C)([P](C(C)(C)C)([Pd][P](C(C)(C)C)(C(C)(C)C)C(C)(C)C)C(C)(C)C)C.C1CCOC1
null
1
Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O.OB(O)c1ccccc1>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].CC(C)([P](C(C)(C)C)([Pd][P](C(C)(C)C)(C(C)(C)C)C(C)(C)C)C(C)(C)C)C.C1CCOC1>Cc1cc(SCC=C(c2ccc(-c3ccccc3)cc2)c2ccc(-c3ccccc3)cc...
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b3d87d56f4e042bca847751840000337
CS(=O)(=O)c1ccc(B(O)O)cc1.Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O>>Cc1cc(SCC=C(c2ccc(-c3ccc(S(C)(=O)=O)cc3)cc2)c2ccc(-c3ccc(S(C)(=O)=O)cc3)cc2)ccc1OCC(=O)O
BrC1=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)Br.CS(=O)(=O)C1=CC=C(C=C1)B(O)O.[F-].[K+].[Cl-].[NH4+]>>CS(=O)(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)C1=CC=C(C=C1)S(=O)(=O)C
B([OH:19])([OH:20])[c:29]1[cH:30][cH:31][c:32]([S:33]([CH3:34])(=[O:35])=[O:36])[cH:37][cH:38]1.Br[c:12]1[cH:11][cH:10][c:9]([C:8](=[CH:7][CH2:6][S:5][c:4]2[cH:3][c:2]([CH3:1])[c:43]([O:44][CH2:45][C:46](=[O:47])[OH:48])[cH:42][cH:41]2)[c:25]2[cH:13][cH:39][c:28](Br)[cH:27][cH:26]2)[cH:24][cH:23]1>>[CH3:1][c:2]1[cH:3][...
CS(=O)(=O)c1ccc(B(O)O)cc1.Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O
Cc1cc(SCC=C(c2ccc(-c3ccc(S(C)(=O)=O)cc3)cc2)c2ccc(-c3ccc(S(C)(=O)=O)cc3)cc2)ccc1OCC(=O)O
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd]
C1CCOC1
Aromatic Heterocycle Formation
OtherReaction
ce56a450dd6b8f96deb02dac9a10e8b4c15b39e33b79e30a389dd2b31b0d3aa4
996ce2d4d4695a5c5f5489bc18374e40992c567a4c050b6407b43ea3455965ab
C(CSc1ccccc1)=C(c1ccc(-c2ccccc2)cc1)c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[C:5](=[C:6]-[C:7])-[c;H0;D3;+0:8]2:[c:9]:[c:10]:[c;H0;D3;+0:11](-Br):[cH;D2;+0:12]:[cH;D2;+0:13]:2):[c:14]:[c:15]:1.[OH;D1;+0:16]-B(-[OH;D1;+0:17])-[c;H0;D3;+0:18](:[c:19]:[c:20]):[c:21]:[c:22]>>[C:7]-[C:6]=[C:5](-[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:13]2:[c:23]:[c:24]:[...
null
[]
null
null
1
HOUR
In an evaporated schlenk flask kept under nitrogen atmosphere were added {4-[3,3-bis-(4-bromo-phenyl)-allylsulfanyl]-2-methyl-phenoxy}-acetic acid (208 mg, 0.38 mmol, example 1, step A–B), 4-(methansulfonyl)phenylboronic acid (280 mg, 1.4 mmol), KF (77 mg, 1.33 mmol), Pd2(dba)3 (21 mg, 23 mmol) and Pd(P(t-BU)3)2 (23 mg...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Boronic acid
Sulfone
c1ccccc1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
Br-.B
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C1CCOC1
null
1
CS(=O)(=O)c1ccc(B(O)O)cc1.Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C1CCOC1>Cc1cc(SCC=C(c2ccc(-c3ccc(S(C)(=O)=O)cc3)cc2)c2ccc(-c3ccc(S(C)(=O)=O)cc3)cc2)ccc1OCC(=O)O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bb4c73dfe7584f60933d4cf801180706
Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O.OB(O)c1cccc(C(F)(F)F)c1.[F-]>>Cc1cc(SCC=C(c2ccc(-c3cccc(C(F)(F)F)c3)cc2)c2ccc(-c3cccc(C(F)(F)F)c3)cc2)ccc1OCC(=O)O
BrC1=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)Br.FC(C=1C=C(C=CC1)B(O)O)(F)F.[F-].[K+].[Cl-].[NH4+]>>FC(C=1C=C(C=CC1)C1=CC=C(C=C1)C(=CCSC1=CC(=C(OCC(=O)O)C=C1)C)C1=CC=C(C=C1)C1=CC(=CC=C1)C(F)(F)F)(F)F
Br[c:12]1[cH:11][cH:10][c:9]([C:8](=[CH:7][CH2:6][S:5][c:4]2[cH:3][c:2]([CH3:1])[c:43]([O:44][CH2:45][C:46](=[O:47])[OH:48])[cH:42][cH:41]2)[c:25]2[cH:13][cH:27][c:28](Br)[cH:39][cH:40]2)[cH:24][cH:23]1.OB(O)[c:29]1[cH:30][cH:31][cH:32][c:17]([C:18]([F:19])([F:21])[F:37])[cH:38]1.[F-:20]>>[CH3:1][c:2]1[cH:3][c:4]([S:5]...
Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O.OB(O)c1cccc(C(F)(F)F)c1.[F-]
Cc1cc(SCC=C(c2ccc(-c3cccc(C(F)(F)F)c3)cc2)c2ccc(-c3cccc(C(F)(F)F)c3)cc2)ccc1OCC(=O)O
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].CC(C)([P](C(C)(C)C)([Pd][P](C(C)(C)C)(C(C)(C)C)C(C)(C)C)C(C)(C)C)C
C1CCOC1
C-C Coupling
OtherReaction
02c971e011cd5a0ccf33bf84d311b8c23ca02678739a7920a6f5e84c4eebcdcd
bbcf2f366e45954510b4dc1e8f94176f116ad3092cd1991a9da7890495c35b5d
C(CSc1ccccc1)=C(c1ccc(-c2ccccc2)cc1)c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[C:5](=[C:6]-[C:7])-[c;H0;D3;+0:8]2:[c:9]:[c:10]:[c;H0;D3;+0:11](-Br):[cH;D2;+0:12]:[cH;D2;+0:13]:2):[c:14]:[c:15]:1.O-B(-O)-[c;H0;D3;+0:16]1:[c:17]:[c:18]:[cH;D2;+0:19]:[c;H0;D3;+0:20](-[C;H0;D4;+0:21](-[F;D1;H0:22])(-[F;D1;H0:23])-[F;H0;D1;+0:24]):[cH;D2;+0:25]:1.[F-;H0;D0:26]>>[...
null
[]
null
null
1
HOUR
In an evaporated schlenk flask kept under nitrogen atmosphere were added {4-[3,3-bis-(4-bromo-phenyl)-allylsulfanyl]-2-methyl-phenoxy}-acetic acid (231 mg, 0.42 mmol, example 1, step A–B), 3-(trifluoromethyl)phenylboronic acid (203 mg, 1.1 mmol), KF (81 mg, 1.39 mmol), Pd2(dba)3 (23 mg, 25 mmol) and Pd(P(t-Bu)3)2 (26 m...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Aromatic halide.Aromatic halide.Boronic acid
Trifluoro group.Trifluoro group
c1ccccc1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
Br-.B
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].CC(C)([P](C(C)(C)C)([Pd][P](C(C)(C)C)(C(C)(C)C)C(C)(C)C)C(C)(C)C)C.C1CCOC1
null
1
Cc1cc(SCC=C(c2ccc(Br)cc2)c2ccc(Br)cc2)ccc1OCC(=O)O.OB(O)c1cccc(C(F)(F)F)c1.[F-]>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].CC(C)([P](C(C)(C)C)([Pd][P](C(C)(C)C)(C(C)(C)C)C(C)(C)C)C(C)(C)C)C.C1CCOC1>Cc1cc(SCC=C(c2ccc(-c3cccc(C(F)(F)F)...