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2010-04-26
Chemical Abundances for the Outer Halo Cluster Pal 4 from Co-added High-Resolution Spectroscopy
Context: Chemical element abundances for distant Galactic globular clusters (GCs) hold important clues to the origin of the Milky Way halo and its substructures. Aims: We study the chemical composition of red giant stars in Pal 4 - one of the most remote GCs in the Milky Way - and compare our abundance measurements to those for both low surface brightness dwarf galaxies, and GCs in the inner and the outer halo. Methods: By co-adding high-resolution, low-S/N Keck/HIRES spectra of 19 stars along the red giant branch, we estimate chemical abundance ratios of 20 alpha-, iron peak-, and neutron-capture elements. Our method gives total uncertainties on most element-to-iron ratios of typically 0.2 dex. Results: We measure [Fe/H] = -1.41 +- 0.04 (statistical) +- 0.17 (systematic) and an alpha-enhancement of [alpha/Fe] = +0.38 +- 0.11 dex, which is consistent with the canonical value of +0.4 dex found for Galactic halo field stars and most halo GCs at this metallicity. Although Pal 4 has higher enhancements in the heavier elements with respect to the halo, the majority of the element ratios are, within the measurement errors, consistent with those for local halo field stars. We find, however, evidence for a lower [Mg/Ca] ratio than in other halo clusters. Conclusions: Based on the available evidence, we conclude that the material from which Pal 4 and the Galactic halo formed experienced similar enrichment processes, despite the apparently younger age of this cluster. Within the limitations of our methodology we find no significant indication of an iron spread, as is typical of genuine GCs of the Milky Way. However, abundance ratios for individual stars in Pal 4 and other distant satellites are urgently needed to understand the relationship, if any, between remote GCs and other halo substructures (i.e., luminous and ultra-faint dwarf spheroidal galaxies).
1004.4625v1
2010-06-05
Variations in the X-ray eclipse transitions of Cen X-3
We report here an investigation of the X-ray eclipse transitions of the high mass X-ray binary pulsar Cen X-3 in different intensity states. Long term light curve of Cen X-3 obtained with RXTE-ASM spanning for more than 5000 days shows strong aperiodic flux variations with low and high states. We have investigated the eclipse transitions of Cen X-3 in different intensity states with data obtained from pointed observations with the more sensitive instruments on board ASCA, BeppoSAX, XMM-Newton, Chandra and RXTE. We found a very clear trend of sharp eclipse transitions in the high state and longer transitions in the low state. This is a confirmation of this feature first observed with the RXTE-ASM but now with much better clarity. From the light curves obtained from several missions, it is seen that the eclipse egress in the low state starts earlier by an orbital phase of 0.02 indicating that the observed X-rays originate from a much larger region. We have also performed spectral analysis of the post-eclipse part of each observations. From BeppoSAX observations, the out-of-eclipse X-ray fluxes is found to differ by a factor of ~ 26 during the high and low intensity states while the eclipse count rates differ by a factor of only ~ 4.7. This indicates that in the low state, there is an additional scattering medium which scatters some of the source photons towards the observer even when the neutron star is completely eclipsed. We could also resolve the three iron line components using XMM-Newton observation in the low state. By comparing the iron line equivalent width during the high and low states, it is seen that the width of iron line is relatively large during the low state which supports the fact that significant reprocessing and scattering of X-rays takes place in the low state.
1006.1035v1
2010-06-17
The supernova delay time distribution in galaxy clusters and implications for Type-Ia progenitors and metal enrichment
Knowledge of the supernova (SN) delay time distribution (DTD) - the SN rate versus time that would follow a hypothetical brief burst of star formation - can shed light on SN progenitors and physics. We compile recent measurements of the Type-Ia SN (SN Ia) rate in galaxy clusters at redshifts z=0-1.45. Together with the observed iron-to-stellar mass ratio in clusters, which constrains the time-integrated number of SN Ia events in clusters, we recover the DTD of SNe Ia in cluster environments. The DTD peaks at the shortest time-delay interval we probe, 0<t<2.2 Gyr, with a low tail out to delays of ~10 Gyr, and is remarkably consistent with several recent DTD reconstructions based on different methods, in different environments. We test DTD models from the literature, requiring that they simultaneously reproduce the observed cluster SN rates and the observed iron-to-stellar mass ratios. A power-law DTD of the form t^{-1.2+/-0.3}, extending to a Hubble time, can satisfy both constraints. Shallower power laws, such as t^{-1/2} cannot, assuming a single DTD, and a single star-formation burst (either brief or extended) at high z. This implies 50-85% of SNe Ia explode within 1 Gyr of star formation. DTDs from double-degenerate (DD) models, which generically have ~t^{-1} shapes over a wide range of timescales, match the data, but only if their predictions are scaled up by factors of 5-10. Single degenerate (SD) DTDs always give poor fits to the data, due to a lack of delayed SNe and overall low numbers of SNe. The observations also permit a combination of two SN Ia populations - prompt (e.g. SD) SNe Ia that explode within a few Gyr of star formation, and produce about 60% of the iron mass in clusters, and a DD population that contributes the events seen at z<1.4. Our results support the existence of a DD progenitor channel for SNe Ia, if the overall predicted numbers can be suitably increased.
1006.3576v3
2010-08-01
Chemical Enrichment in the Faintest Galaxies: the Carbon and Iron Abundance Spreads in the Boötes I Dwarf Spheroidal Galaxy and the Segue 1 System
We present an AAOmega spectroscopic study of red giant stars in Bootes I, which is an ultra-faint dwarf galaxy, and Segue 1, suggested to be either an extremely low-luminosity dwarf galaxy or a star cluster. Our focus is quantifying the mean abundance and abundance dispersion in iron and carbon, and searching for distant radial-velocity members, in these systems. The primary conclusion of our investigation is that the spread of carbon abundance in both Bootes I and Segue 1 is large. For Bootes I, 4 of our 16 velocity members have [C/H] < ~-3.1, while 2 have [C/H] > ~-2.3, suggesting a range of Delta[C/H] ~ 0.8. For Segue 1 there exists a range Delta[C/H] ~ 1.0, including our discovery of a star with [Fe/H] = -3.5 and [C/Fe] = +2.3, which is a radial velocity member at a distance of 4 half-light radii from the system center. The accompanying ranges in iron abundance are Delta[Fe/H] ~ 1.6 for both Bootes I and Segue 1. For [Fe/H] < -3.0, the Galaxy's dwarf galaxy satellites exhibit a dependence of [C/Fe] on [Fe/H] which is very similar to that observed in its halo populations. We find [C/Fe] ~ 0.3 for stars in the dwarf systems that we believe are the counterpart of the Spite et al. (2005) ``unmixed'' giants of the Galactic halo and for which they report [C/Fe] ~ 0.2, and which presumably represents the natal relative abundance of carbon for material with [Fe/H] = -3.0 to -4.0. We confirm the correlation between luminosity and both mean metallicity and abundance dispersion in the Galaxy's dwarf satellites, which extends to at least as faint as Mv = -5. The very low mean metallicity of Segue 1, and the high carbon dispersion in Bootes I, consistent with inhomogeneous chemical evolution in near zero-abundance gas, suggest these ultra-faint systems could be surviving examples of the very first bound systems.
1008.0137v1
2010-11-29
New Atomic Data for Trans-Iron Elements and Their Application to Abundance Determinations in Planetary Nebulae
[Abridged] Investigations of neutron(n)-capture element nucleosynthesis and chemical evolution have largely been based on stellar spectroscopy. However, the recent detection of these elements in several planetary nebulae (PNe) indicates that nebular spectroscopy is a promising new tool for such studies. In PNe, n-capture element abundance determinations reveal details of s-process nucleosynthesis and convective mixing in evolved low-mass stars, as well as the chemical evolution of elements that cannot be detected in stellar spectra. Only one or two ions of a given trans-iron element can typically be detected in individual nebulae. Elemental abundance determinations thus require corrections for the abundances of unobserved ions. Such corrections rely on the availability of atomic data for processes that control the ionization equilibrium of nebulae. Until recently, these data were unknown for virtually all n-capture element ions. For the first five ions of Se, Kr, and Xe -- the three most widely detected n-capture elements in PNe -- we are calculating photoionization cross sections and radiative and dielectronic recombination rate coefficients using the multi-configuration Breit-Pauli atomic structure code AUTOSTRUCTURE. Charge transfer rate coefficients are being determined with a multichannel Landau-Zener code. To calibrate these calculations, we have measured absolute photoionization cross sections of Se and Xe ions at the Advanced Light Source synchrotron radiation facility. These atomic data can be incorporated into photoionization codes, which we will use to derive ionization corrections (hence abundances) for Se, Kr, and Xe in ionized nebulae. These results are critical for honing nebular spectroscopy into a more effective tool for investigating the production and chemical evolution of trans-iron elements in the Universe.
1011.6311v1
2011-03-31
The metal contents of two groups of galaxies
The hot gas in clusters and groups of galaxies is continuously being enriched with metals from supernovae and stars. It is well established that the enrichment of the gas with elements from oxygen to iron is mainly caused by supernova explosions. The origins of nitrogen and carbon are still being debated. Possible candidates include massive, metal-rich stars, early generations of massive stars, intermediate or low mass stars and Asymptotic Giant Branch (AGB) stars. In this paper we accurately determine the metal abundances of the gas in the groups of galaxies NGC 5044 and NGC 5813, and discuss the nature of the objects that create these metals. We mainly focus on carbon and nitrogen. We use spatially-resolved high-resolution X-ray spectroscopy from XMM-Newton. For the spectral fitting, multi-temperature hot gas models are used. The abundance ratios of carbon over oxygen and nitrogen over oxygen that we find are high compared to the ratios in the stars in the disk of our Galaxy. The oxygen and nitrogen abundances we derive are similar to what was found in earlier work on other giant ellipticals in comparable environments. We show that the iron abundances in both our sources have a gradient along the cross-dispersion direction of the Reflection Grating Spectrometer (RGS). We conclude that it is unlikely that the creation of nitrogen and carbon takes place in massive stars, which end their lives as core-collapse supernovae, enriching the medium with oxygen because oxygen should then also be enhanced. Therefore we favour low-and intermediate mass stars as sources of these elements. The abundances in the hot gas can best be explained by a 30-40% contribution of type Ia supernovae based on the measured oxygen and iron abundances and under the assumption of a Salpeter Initial Mass Function (IMF).
1104.0001v1
2011-04-11
Self-consistent spin-wave theory for a frustrated Heisenberg model with biquadratic exchange in the columnar phase and its application to iron pnictides
Recent neutron scattering studies revealed the three dimensional character of the magnetism in the iron pnictides and a strong anisotropy between the exchange perpendicular and parallel to the spin stripes. We extend studies of the J1-J2-Jc Heisenberg model with S = 1 using self-consistent spin-wave theory. A discussion of two scenarios for the instability of the columnar phase is provided. The relevance of a biquadratic exchange term between in-plane nearest neighbors is discussed. We introduce mean-field decouplings for biquadratic terms using the Dyson-Maleev and the Schwinger boson representation. Remarkably their respective mean-field theories do not lead to the same results, even at zero temperature. They are gauged in the N'eel phase in comparison to exact diagonalization and series expansion. The J1-J2-Jc model is analyzed under the influence of the biquadratic exchange Jbq and a detailed description of the staggered magnetization and of the magnetic excitations is given. The biquadratic exchange increases the renormalization of the in-plane exchange constants which enhances the anisotropy between the exchange parallel and perpendicular to the spin stripes. Applying the model to iron pnictides, it is possible to reproduce the spin-wave dispersion for CaFe2As2 in the direction perpendicular to the spin stripes and perpendicular to the planes. Discrepancies remain in the direction parallel to the spin stripes which can be resolved by passing from S = 1 to S = 2. In addition, results for the dynamical structure factor within the self-consistent spin-wave theory are provided.
1104.1954v2
2011-04-22
K-shell Emission of Neutral Iron Line from Sgr B2 Excited by Subrelativistic Protons
We investigated the emission of K$\alpha$ iron line from the massive molecular clouds in the Galactic center (GC). We assume that at present the total flux of this emission consists of time variable component generated by primary X-ray photons ejected by Sagittarius A$^\ast$ (Sgr A$^\ast$) in the past and a relatively weak quasi-stationary component excited by impact of protons which were generated by star accretion onto the central black hole. The level of background emission was estimated from a rise of the 6.4 keV line intensity in the direction of several molecular clouds, that we interpreted as a stage when the X-ray front ejected by Sgr A$^\ast$ entered into these clouds. The 6.4 keV emission before this intensity jump we interpreted as emission generated by subrelativistic cosmic rays there. The cross-section of K$\alpha$ vacancies produced by protons differs from that of electrons or X-rays. Therefore, we expect that this processes can be distinguished from the analysis of the equivalent width of the iron line and time variations of the width can be predicted. The line intensity from the clouds depends on their distance from Sgr A$^\ast$ and the coefficient of spacial diffusion near the Galactic center. We expect that in a few years the line intensity for the cloud G\,0.11$-$0.11 which is relatively close to Sgr A$^\ast$ will decreases to the level $\lesssim$ 10% from its present value. For the cloud Sagittarius B2 (Sgr B2) the situation is more intricate. If the diffusion coefficient $D\gtrsim 10^{27}$ cm$^2$ s$^{-1}$ then the expected stationary flux should be about 10% of its level in 2000. In the opposite case the line intensity from Sgr B2 should drop down to zero because the protons do not reach the cloud.
1104.4484v1
2011-07-05
A giant planet in the triple system HD132563
As part of our radial velocity planet-search survey performed with SARG at TNG, we monitored the components of HD 132563 for ten years. It is a binary system formed by two rather similar solar type stars with a projected separation of 4.1 arcsec, which corresponds to 400 AU at the distance of 96 pc. The two components are moderately metal-poor and the age of the system is about 5 Gyr. We detected RV variations of HD 132563B with period of 1544 days and semi-amplitude of 26 m/s. From the star characteristics and line profile measurements, we infer their Keplerian origin. Therefore HD 132563B turns out to host a planet with a projected mass msini=1.49 MJup at 2.6 AU with a moderately eccentric orbit (e=0.22). The planet around HD 132563B is one of the few that are known in triple stellar systems, as we found that the primary HD 132563A is itself a spectroscopic binary with a period longer than 15 years and an eccentricity higher than 0.65. The spectroscopic component was not detected in adaptive-optics images taken with AdOpt@TNG, since it expected at a projected separation that was smaller than 0.2 arcsec at the time of our observations. A small excess in K band difference between the components with respect to the difference in V band is compatible with a companion of about 0.55 Msun. A preliminary statistical analysis of the occurrence of planets in triple systems indicate a similar frequency of planets around the isolated component in a triple system, components of wide binaries and single stars. There is no significant iron abundance difference between the components. The lack of stars in binary systems and open clusters showing strong enhancements of iron abundance, comparable to the typical metallicity difference between stars with and without giant planets, agrees with the idea that accretion of planetary material producing iron abundance anomalies larger than 0.1 dex is rare.
1107.0918v1
2011-11-21
Iron and alpha-element Production in the First One Billion Years after the Big Bang
We present measurements of carbon, oxygen, silicon, and iron in quasar absorption systems existing when the universe was roughly one billion years old. We measure column densities in nine low-ionization systems at 4.7 < z < 6.3 using Keck, Magellan, and VLT optical and near-infrared spectra with moderate to high resolution. The column density ratios among C II, O I, Si II, and Fe II are nearly identical to sub-DLAs and metal-poor ([M/H] < -1) DLAs at lower redshifts, with no significant evolution over 2 < z < 6. The estimated intrinsic scatter in the ratio of any two elements is also small, with a typical r.m.s. deviation of <0.1 dex. These facts suggest that dust depletion and ionization effects are minimal in our z > 4.7 systems, as in the lower-redshift DLAs, and that the column density ratios are close to the intrinsic relative element abundances. The abundances in our z > 4.7 systems are therefore likely to represent the typical integrated yields from stellar populations within the first gigayear of cosmic history. Due to the time limit imposed by the age of the universe at these redshifts, our measurements thus place direct constraints on the metal production of massive stars, including iron yields of prompt supernovae. The lack of redshift evolution further suggests that the metal inventories of most metal-poor absorption systems at z > 2 are also dominated by massive stars, with minimal contributions from delayed Type Ia supernovae or AGB winds. The relative abundances in our systems broadly agree with those in very metal-poor, non-carbon-enhanced Galactic halo stars. This is consistent with the picture in which present-day metal-poor stars were potentially formed as early as one billion years after the Big Bang.
1111.4843v1
2012-01-04
Synthesis and physical properties of the new potassium iron selenide superconductor K0.80Fe1.76Se2
In this article we review our studies of the K0.80Fe1.76Se2 superconductor, with an attempt to elucidate the crystal growth details and basic physical properties over a wide range of temperatures and applied magnetic field, including anisotropic magnetic and electrical transport properties, thermodynamic, London penetration depth, magneto-optical imaging and Mossbauer measurements. We find that: (i) Single crystals of similar stoichiometry can be grown both by furnace-cooled and decanted methods; (ii) Single crystalline K0.80Fe1.76Se2 shows moderate anisotropy in both magnetic susceptibility and electrical resistivity and a small modulation of stoichiometry of the crystal, which gives rise to broadened transitions; (iii) The upper critical field, Hc2(T) is ~ 55 T at 2 K for H||c, manifesting a temperature dependent anisotropy that peaks near 3.6 at 27 K and drops to 2.5 by 18 K; (iv) Mossbauer measurements reveal that the iron sublattice in K0.80Fe1.76Se2 clearly exhibits magnetic order, probably of the first order, from well below Tc to its Neel temperature of Tn = 532 +/- 2 K. It is very important to note that, although, at first glance there is an apparent dilemma posed by these data: high Tc superconductivity in a near insulating, large ordered moment material, analysis indicates that the sample may well consist of two phases with the minority superconducting phase (that does not exhibit magnetic order) being finely distributed, but connected with in an antiferromagnetic, poorly conducting, matrix, essentially making a superconducting aerogel.
1201.0953v2
2012-02-13
A Variable Partial Covering Model for the Seyfert 1 Galaxy MCG-6-30-15
We propose a simple spectral model for the Seyfert 1 Galaxy MCG-6-30-15 that can explain most of the 1 - 40 keV spectral variation by change of the partial covering fraction, similar to the one proposed by Miller et al. (2008). Our spectral model is composed of three continuum components; (1) a direct power-law component, (2) a heavily absorbed power-law component by mildly ionized intervening matter, and (3) a cold disk reflection component far from the black hole with moderate solid-angle ({\Omega}/2{\pi} \approx 0.3) accompanying a narrow fluorescent iron line. The first two components are affected by the surrounding highly ionized thin absorber with N_H \approx 10^{23.4}cm-2 and log {\xi} \approx 3.4. The heavy absorber in the second component is fragmented into many clouds, each of which is composed of radial zones with different ionization states and column densities, the main body (N_H \approx 10^24.2cm-2, log {\xi} \approx 1.6), the envelope (N_H \approx 10^22.1cm-2, log {\xi} \approx 1.9) and presumably a completely opaque core. These parameters of the ionized absorbers, as well as the intrinsic spectral shape of the X-ray source, are unchanged at all. The central X-ray source is moderately extended, and its luminosity is not significantly variable. The observed flux and spectral variations are mostly explained by variation of the geometrical partial covering fraction of the central source from 0 (uncovered) to \sim0.63 by the intervening ionized clouds in the line of sight. The ionized iron K-edge of the heavily absorbed component explains most of the seemingly broad line-like feature, a well-known spectral characteristic of MCG-6-30-15. The direct component and the absorbed component anti-correlate, cancelling their variations each other, so that the fractional spectral variation becomes the minimum at the iron energy band; another observational characteristic of MCG-6-30-15 is thus explained.
1202.2797v3
2012-02-23
The Similarity of Broad Iron Lines in X-ray Binaries and Active Galactic Nuclei
We have compared the 2001 XMM-Newton spectra of the stellar mass black hole binary XTE J1650-500 and the active galaxy MGC-6-30-15, focusing on the broad, excess emission features at ~4--7 keV displayed by both sources. Such features are frequently observed in both low mass X-ray binaries and active galactic nuclei. For the former case it is generally accepted that the excess arises due to iron emission, but there is some controversy over whether their width is partially enhanced by instrumental processes, and hence also over the intrinsic broadening mechanism. Meanwhile, in the latter case, the origin of this feature is still subject to debate; physically motivated reflection and absorption interpretations are both able to reproduce the observed spectra. In this work we make use of the contemporaneous BeppoSAX data to demonstrate that the breadth of the excess observed in XTE J1650-500 is astrophysical rather than instrumental, and proceed to highlight the similarity of the excesses present in this source and MGC-6-30-15. Both optically thick accretion discs and optically thin coronae, which in combination naturally give rise to relativistically-broadened iron lines when the disc extends close to the black hole, are commonly observed in both class of object. The simplest solution is that the broad emission features present arise from a common process, which we argue must be reflection from the inner regions of an accretion disc around a rapidly rotating black hole; for XTE J1650-500 we find spin constraints of 0.84 < a* < 0.98 at the 90 per cent confidence level. Other interpretations proposed for AGN add potentially unnecessary complexities to the theoretical framework of accretion in strong gravity.
1202.5193v1
2012-03-02
Testing the effects of opacity and the chemical mixture on the excitation of pulsations in B stars of the Magellanic Clouds
The B-type pulsators known as \beta Cephei and Slowly Pulsating B (SPB) stars present pulsations driven by the \kappa mechanism, which operates thanks to an opacity bump due to the iron group elements. In low-metallicity environments such as the Magellanic Clouds, \beta Cep and SPB pulsations are not expected. Nevertheless, recent observations show evidence for the presence of B-type pulsator candidates in both galaxies. We seek an explanation for the excitation of \beta Cep and SPB modes in those galaxies by examining basic input physics in stellar modelling: i) the specific metal mixture of B-type stars in the Magellanic Clouds; ii) the role of a potential underestimation of stellar opacities. We first derive the present-day chemical mixtures of B-type stars in the Magellanic Clouds. Then, we compute stellar models for that metal mixture and perform a non-adiabatic analysis of these models. In a second approach, we simulate parametric enhancements of stellar opacities due to different iron group elements. We then study their effects in models of B stars and their stability. We find that adopting a representative chemical mixture of B stars in the Small Magellanic Cloud cannot explain the presence of B-type pulsators there. An increase of the opacity in the region of the iron-group bump could drive B-type pulsations, but only if this increase occurs at the temperature corresponding to the maximum contribution of Ni to this opacity bump. We recommend an accurate computation of Ni opacity to understand B-type pulsators in the Small Magellanic Cloud, as well as the frequency domain observed in some Galactic hybrid \beta Cep-SPB stars.
1203.0527v1
2012-03-19
Hot Gas in Galaxy Groups: Recent Observations
Galaxy groups are the least massive systems where the bulk of baryons begin to be accounted for. Not simply the scaled-down versions of rich clusters following self-similar relations, galaxy groups are ideal systems to study baryon physics, which is important for both cluster cosmology and galaxy formation. We review the recent observational results on the hot gas in galaxy groups. The first part of the paper is on the scaling relations, including X-ray luminosity, entropy, gas fraction, baryon fraction and metal abundance. Compared to clusters, groups have a lower fraction of hot gas around the center (e.g., r < r_2500), but may have a comparable gas fraction at large radii (e.g., r_2500 < r < r_500). Better constraints on the group gas and baryon fractions require sample studies with different selection functions and deep observations at r > r_500 regions. The hot gas in groups is also iron poor at large radii (0.3 r_500 - 0.7 r_500). The iron content of the hot gas within the central regions (r < 0.3 r_500) correlates with the group mass, in contrast to the trend of the stellar mass fraction. It remains to be seen where the missing iron in low-mass groups is. In the second part, we discuss several aspects of X-ray cool cores in galaxy groups, including their difference from cluster cool cores, radio AGN heating in groups and the cold gas in group cool cores. Because of the vulnerability of the group cool cores to radio AGN heating and the weak heat conduction in groups, group cool cores are important systems to test the AGN feedback models and the multiphase cool core models. At the end of the paper, some outstanding questions are listed.
1203.4228v1
2012-03-28
Dependence of the structural and physical properties of Tl1-yFe2-z(Se1-xSx)2 with isovalent substitution of Se by S: decrease of TNeel with S content
The effect of selenium substitution by sulfur or tellurium in the Tl1-yFe2-zSe2 antiferromagnet was studied by x-ray and electron diffraction, magnetization and transport measurements. Tl0.8Fe1.5(Se1-xXx)2 (nominal composition) solid solutions were synthesized in the full x range (0<x<1) for X=S and up to x=0.5 for X=Te, using the sealed tube technique. No superconductivity was found down to 4.2K in the case of sulfur despite the fact that the optimal crystallographic parameters, determined by Rietveld refinements, are reached in the series (i.e. the Fe-(Se,S) interplane height and (Se,S)-Fe-(Se,S) angle for which the critical superconducting transition T$_{c}$ is usually maximal in pnictides). Quasi full Tl site (y=0.05) compared to significant alkaline deficiency (y=0.2-0.3) in analogous A1-yFe2-zSe2 (A = K, Rb, Cs), and the resulting differences in iron valency, density of states and doping, are suggested to explain this absence of superconductivity. Compounds substituted with tellurium, at least up to x=0.25, show superconducting transitions but probably due to tetragonal Fe(Se,Te) impurity phase. Transmission electron microscopy confirmed the existence of ordered iron vacancies network in the samples from the Tl$_{0.8}$Fe$_{1.5}$(Se$_{1-x}$S$_{x}$)$_{2}$ series in the form of the tetragonal $\sqrt{5}$ a $\times \sqrt{5}$ a $\times$ c superstructure (\textit{I4/m}) (mixed with the orthorhombic $\sqrt{2}$ a $\times 2\sqrt{2}$ a $\times$ c form (\textit{Ibam}) if the iron vacancies level is increased). The N\'{e}el temperature (T$_{N}$) indicating the onset of antiferromagnetism order in the $\sqrt{5}$ a $\times \sqrt{5}$ a $\times$ c supercell decreases from 450K in the selenide (x=0) to 330K in the sulfide (x=1). We finally demonstrate a direct linear relationship between $T_{N\acute{e}el}$ and the Fe-(Se,S) bond length (or Fe-(Se,S) height).
1203.6181v2
2012-05-21
Very High Resolution Solar X-ray Imaging Using Diffractive Optics
This paper describes the development of X-ray diffractive optics for imaging solar flares with better than 0.1 arcsec angular resolution. X-ray images with this resolution of the \geq10 MK plasma in solar active regions and solar flares would allow the cross-sectional area of magnetic loops to be resolved and the coronal flare energy release region itself to be probed. The objective of this work is to obtain X-ray images in the iron-line complex at 6.7 keV observed during solar flares with an angular resolution as fine as 0.1 arcsec - over an order of magnitude finer than is now possible. This line emission is from highly ionized iron atoms, primarily Fe xxv, in the hottest flare plasma at temperatures in excess of \approx10 MK. It provides information on the flare morphology, the iron abundance, and the distribution of the hot plasma. Studying how this plasma is heated to such high temperatures in such short times during solar flares is of critical importance in understanding these powerful transient events, one of the major objectives of solar physics. We describe the design, fabrication, and testing of phase zone plate X-ray lenses with focal lengths of \approx100 m at these energies that would be capable of achieving these objectives. We show how such lenses could be included on a two-spacecraft formation-flying mission with the lenses on the spacecraft closest to the Sun and an X-ray imaging array on the second spacecraft in the focal plane \approx100 m away. High resolution X-ray images could be obtained when the two spacecraft are aligned with the region of interest on the Sun. Requirements and constraints for the control of the two spacecraft are discussed together with the overall feasibility of such a formation-flying mission.
1205.4762v1
2012-07-04
Nematic and meta-nematic transitions in the iron pnictides
Strongly interacting electrons can exhibit novel collective phases, among which the electronic nematic phases are perhaps the most surprising as they spontaneously break rotational symmetry of the underlying crystal lattice. The electron nematicity has been recently observed in the iron-pnictide and cuprate high-temperature superconductors. Whether such a tendency of electrons to self-organise unidirectionally has a common feature in these superconductors is, however, a highly controversial issue. In the cuprates, the nematicity has been suggested as a possible source of the pseudogap phase, whilst in the iron-pnictides, it has been commonly associated with the tetragonal-to-orthorhombic structural phase transition at $T_s$. Here, we provide the first thermodynamic evidence in BaFe2(As1-xPx)2 that the nematicity develops well above the structural transition and persists to the nonmagnetic superconducting regime, resulting in a new phase diagram strikingly similar to the pseudogap phase diagram in the cuprates. Our highly sensitive magnetic anisotropy measurements using microcantilever torque-magnetometry under in-plane field rotation reveal pronounced two-fold oscillations, which break the tetragonal symmetry. Combined with complementary high-resolution synchrotron X-ray and resistivity measurements, our results consistently identify two distinct temperatures - one at $T^{\ast}$, signifying a true nematic transition, and the other at $T_s (< T^{\ast})$, which we show to be not a true phase transition, but rather what we refer to as a "meta-nematic transition", in analogy to the well-known metamagnetic transition in the theory of magnetism. Our observation of the extended nematic phase above the superconducting dome establishes that the nematicity has primarily an electronic origin, inherent in the normal state of high-temperature superconductors.
1207.1045v1
2012-08-24
Failed-Detonation Supernovae: Sub-Luminous Low-Velocity Ia Supernovae and Their Kicked Remnant White Dwarfs with Iron-Rich Cores
Type Ia supernovae (SNe Ia) originate from the thermonuclear explosions of carbon-oxygen (C-O) white dwarfs (WDs). The single-degenerate scenario is a well-explored model of SNe Ia where unstable thermonuclear burning initiates in an accreting, Chandrasekhar-mass WD and forms an advancing flame. By several proposed physical processes the rising, burning material triggers a detonation, which subsequently consumes and unbinds the WD. However, if a detonation is not triggered and the deflagration is too weak to unbind the star, a completely different scenario unfolds. We explore the failure of the Gravitationally-Confined Detonation (GCD) mechanism of SNe Ia, and demonstrate through 2D and 3D simulations the properties of failed-detonation SNe. We show that failed-detonation SNe expel a few 0.1 solar masses of burned and partially-burned material and that a fraction of the material falls back onto the WD, polluting the remnant WD with intermediate-mass and iron-group elements, that likely segregate to the core forming an WD whose core is iron rich. The remaining material is asymmetrically ejected at velocities comparable to the escape velocity from the WD, and in response, the WD is kicked to velocities of a few hundred km/s. These kicks may unbind the binary and eject a runaway/hyper-velocity WD. Although the energy and ejected mass of the failed-detonation SN are a fraction of typical thermonuclear SNe, they are likely to appear as sub-luminous low-velocity SNe Ia. Such failed detonations might therefore explain or are related to the observed branch of peculiar SNe Ia, such as the family of low-velocity sub-luminous SNe (SN 2002cx/SN 2008ha-like SNe).
1208.5069v2
2012-11-26
Local Structure and Hyperfine Interactions of 57Fe in NaFeAs Studied by Mossbauer Spectroscopy
Detailed 57Fe Mossbauer spectroscopy measurements on superconducting NaFeAs powder samples have been performed in the temperature range 13 K < T < 300 K. The 57Fe spectra recorded in the paramagnetic range (T > TN ~ 46 K) were discussed supposing that most of the Fe2+ ions are located in distorted (FeAs4) tetrahedral of NaFeAs phase, while additional minor (< 10%) component of the spectra corresponds to impurity or intergrowth NaFe2As2 phase with a nominal composition near "NaFe2As2". Our results reveal that the structural transition (TS ~ 55K) has a weak effect on the electronic structure of iron ions, while at T < TN the spectra show a continuous distribution of hyperfine fields HFe . Shape of these spectra was analyzed in term of two models: (i) an incommensurate spin density wave modulation of iron magnetic structure, (ii) a formation of a microdomain structure or phase separation. It was shown that the hyperfine parameters obtained using these two methods have very similar values over the whole temperature range. The analysis of the temperature dependence HFe(T) with the Bean-Rodbell model leads to ksi = 1.16 +/- 0.05, suggesting that the magnetic phase transition is first-order in nature. A sharp evolution of the VZZ(T) and etha(T) parameters of the full Hamiltonian of hyperfine interactions near T ~ (TN, TS), were interpreted as a manifestation of the anisotropic electron redistribution between the dxz, dyz- and dxy-orbitals of the iron ions.
1211.5967v3
2012-12-02
Tunable interplay between 3d and 4f electrons in Co-doped iron pnictides
We study the interplay of 3d and 4f electrons in the iron pnictides CeFe$_{1-x}$Co$_x$AsO and GdFe$_{1-y}$Co$_y$AsO, which correspond to two very different cases of $4f$-magnetic moment. Both CeFeAsO and GdFeAsO undergo a spin-density-wave (SDW) transition associated with Fe 3d electrons at high temperatures, which is rapidly suppressed by Fe/Co substitution. Superconductivity appears in a narrow doping range: $0.05 < x < 0.2$ for CeFe$_{1-x}$Co$_x$AsO and $0.05 < y < 0.25$ for GdFe$_{1-y}$Co$_y$AsO, showing a maximum transition temperature $T_\textup{sc}$ of about 13.5 K for Ce and 19 K for Gd. In both compounds, the $4f$-electrons form an antiferromagnetic (AFM) order at low temperatures over the entire doping range and Co 3d electrons are ferromagnetically ordered on the Co-rich side; the Curie temperature reaches $T_\textup{C}^\textup{Co} \approx$ 75 K at $x = 1$ and $y = 1$. In the Ce-compounds, the N\'{e}el temperature $T_\textup{N}^\textup{Ce}$ increases upon suppressing the SDW transition of Fe and then remains nearly unchanged with further increasing Co concentration up to $x \simeq 0.8$ ($T_\textup{N}^\textup{Ce}\approx$ 4 K). Furthermore, evidence of Co-induced polarization on Ce-moments is observed on the Co-rich side. In the Gd-compounds, the two magnetic species of Gd and Co are coupled antiferromagnetically to give rise to ferrimagnetic behavior in the magnetic susceptibility on the Co-rich side. For $0.7 \leq y < 1.0$, the system undergoes a possible magnetic reorientation below the N\'{e}el temperature of Gd ($T_\textup{N}^\textup{Gd}$). Our results suggest that the effects of both electron hybridizations and magnetic exchange coupling between the 3d-4f electrons give rise to a rich phase diagram in the rare-earth iron pnictides.
1212.0221v2
2013-01-15
Pulse phase and precession phase resolved spectroscopy of Her X-1: studying a representative Main-On with RXTE
We performed a detailed pulse phase resolved spectroscopy of the accreting binary X-ray pulsar Her X-1 in the energy range 3.5-75 keV and have established pulse phase profiles for all spectral parameters. For the centroid of the cyclotron line, the photon index and the flux of the 6.4 keV iron line, we have studied the variation as a function of 35 d phase. We analyzed RXTE observations of the Main-On of November 2002. Four different time intervals of about 1 d duration were selected to provide a good coverage of a complete Main-On. The intervals are centered at 35 d phase 0.03, 0.10, 0.15, and 0.20, respectively. All spectral parameters show a strong modulation with pulse phase. While the centroid energy of the cyclotron line follows roughly the shape of the pulse profile, both the photon index and the iron line intensity exhibit distinct minima around the peak of the X-ray pulse. With respect to variations of the observed profiles with 35 d phase, we find that there is a clear evolution of the shape of the pulse profiles (flux versus pulse phase), a moderate increase of the maximum cyclotron line energy (found around pulse phase 0.7), but no significant evolution of the shape of the pulse phase profiles of the cyclotron line energy, the spectral power law index or the iron line intensity. The variation of spectral parameters as a function of the pulse phase provides important information about the system: 1. the disappearance of the Fe line flux near the highest continuum flux may be an indication of a hollow cone geometry of the accretion structure; ii. the apparent non-dependence of the cyclotron line energy profiles on 35 d phase provides a new possibility to test the model of free precession of the neutron star, proposed to be responsible for the systematic variations in the pulse profiles.
1301.3378v1
2013-01-24
The wind of the M-type AGB star RT Virginis probed by VLTI/MIDI
We study the circumstellar environment of the M-type AGB star RT Vir using mid-infrared high spatial resolution observations from the ESO-VLTI focal instrument MIDI. The aim of this study is to provide observational constraints on theoretical prediction that the winds of M-type AGB objects can be driven by photon scattering on iron-free silicate grains located in the close environment (about 2 to 3 stellar radii) of the star. We interpreted spectro-interferometric data, first using wavelength-dependent geometric models. We then used a self-consistent dynamic model atmosphere containing a time-dependent description of grain growth for pure forsterite dust particles to reproduce the photometric, spectrometric, and interferometric measurements of RT Vir. Since the hydrodynamic computation needs stellar parameters as input, a considerable effort was first made to determine these parameters. MIDI differential phases reveal the presence of an asymmetry in the stellar vicinity. Results from the geometrical modeling give us clues to the presence of aluminum and silicate dust in the close circumstellar environment (< ~5 stellar radii). Comparison between spectro-interferometric data and a self-consistent dust-driven wind model reveals that silicate dust has to be present in the region between 2 to 3 stellar radii to reproduce the 59 and 63 m baseline visibility measurements around 9.8 micron. This gives additional observational evidence in favor of winds driven by photon scattering on iron-free silicate grains located in the close vicinity of an M-type star. However, other sources of opacity are clearly missing to reproduce the 10-13 micron visibility measurements for all baselines. This study is a first attempt to understand the wind mechanism of M-type AGB stars by comparing photometric, spectrometric, and interferometric measurements with state-of-the-art, self-consistent dust-driven wind models. The agreement of the dynamic model atmosphere with interferometric measurements in the 8-10 micron spectral region gives additional observational evidence that the winds of M-type stars can be driven by photon scattering on iron-free silicate grains. Finally, a larger statistical study and progress in advanced self-consistent 3D modeling are still required to solve the remaining problems.
1301.5872v1
2013-03-15
The 69 micron forsterite band in spectra of protoplanetary disks - Results from the Herschel DIGIT programme
Context: We have analysed Herschel-PACS spectra of 32 circumstellar disks around Herbig Ae/Be and T-Tauri stars obtained within the Herschel key programme DIGIT. In this paper we focus on the 69mu emission band of the crystalline silicate forsterite. Aims: This work provides an overview of the 69mu forsterite bands in the DIGIT sample. We aim to derive the temperature and composition of the forsterite grains. With this information, constraints can be placed on the spatial distribution of the forsterite in the disk and its formation history. Methods: Position and shape of the 69mu band are used to derive the temperature and composition of the dust by comparison to laboratory spectra of that band. We combine our data with existing Spitzer IRS spectra to compare the presence and strength of the 69mu band to the forsterite bands at shorter wavelengths. Results: A total of 32 sources have been observed, 8 of them show a 69mu emission band that can be attributed to forsterite. With the exception of the T-Tauri star AS205, all of the detections are for disks associated with Herbig Ae/Be stars. Most of the forsterite grains that give rise to the 69mu bands are warm (~100-200 K) and iron-poor (less than ~2% iron). Only AB-Aur requires approximately 3-4% of iron. Conclusions: Our findings support the hypothesis that the forsterite grains form through an equilibrium condensation process at high temperatures. The connection between the strength of the 69 and 33mu bands shows that at least part of the emission in these bands originates from the same dust grains. Further, any model that explains the PACS and the Spitzer IRS observations must take the effects of a wavelength dependent optical depth into account. We find indications of a correlation of the detection rate of the 69mu band with the spectral type of the host stars. However, our sample is too small to obtain a definitive result.
1303.3744v1
2013-04-30
Superconductivity induced by hydrogen anion substitution in 1111-type iron arsenides
Hydrogen is the simplest bipolar element and its valence state can be controlled from +1 to -1. We synthesized the 1111-type CaFeAsH and LnFeAsO1-xHx (Ln = lanthanide) with the ZrCuSiAs type structure by a high-pressure synthesis method. The position and valence state of the substituted H were determined by neutron diffraction and density functional theory calculations. The close similarity in the structural and electrical properties of CaFeAsH and CaFeAsF indicated the formation of the hydride ion (H-), which is isovalent with the fluoride ion (F-), in the 1111-type iron arsenides. When some of the O2- ions in LnFeAsO are replaced by H-, superconductivity is induced by electron doping to the FeAs-layer to maintain charge neutrality. Since the substitution limit of hydrogen in LnFeAsO (x~0.5) is much higher than that of fluorine (x~0.2), the hydrogen substitution technique provides an effective pathway for high-density electron-doping, making it possible to draw the complete electronic phase diagram of LnFeAsO. The x-T diagrams of LnFeAsO1-xHx (Ln = La, Ce, Sm, Gd) have a wide superconducting (SC) region spanning the range x = 0.04 to 0.4, which is far from the parent antiferromagnetic region near x = 0.0. For Ln=La, another SC dome region was found in the range x = ~ 0.2 to ~0.5 with a maximum Tc = 36 K, in addition to a conventional SC dome located at x ~0.08 with maximum Tc = 29 K. Density functional theory calculations performed for LaFeAsO1-xHx indicated that the newly observed Tc is correlated with the appearance of degeneration of the Fe 3d bands (dxy, dyz and dzx), which is caused not only by regularization of the tetrahedral shape of FeAs4 due to chemical pressure effects but also by selective band occupation with doped electrons. In this article, we review the recent progress of superconductivity in iron (oxy)arsenides and related compounds induced by hydrogen substitution.
1304.7900v1
2013-05-23
On magnetic inhibition of photospheric macro-turbulence generated in the iron-bump opacity zone of O-stars
Massive, hot OB-stars show clear evidence of strong macroscopic broadening (in addition to rotation) in their photospheric spectral lines. This paper examines the occurrence of such "macro-turbulence" in slowly rotating O-stars with strong, organised surface magnetic fields. Focusing on the CIV 5811A line, we find evidence for significant macro-turbulent broadening in all stars except NGC1624-2, which also has (by far) the strongest magnetic field. Instead, the very sharp CIV lines in NGC1624-2 are dominated by magnetic Zeeman broadening, from which we estimate a dipolar field of approximately 20 kG. By contrast, magnetic broadening is negligible in the other stars (due to their weaker field strengths, on order 1 kG), and their CIV profiles are typically very broad and similar to corresponding lines observed in non-magnetic O-stars. Quantifying this by an isotropic, Gaussian macro-turbulence, we derive vmac = 2.2 (+- 0.9/2.2) km/s for NGC1624-2, and vmac = 20-65 km/s for the rest of the magnetic sample. We use these observational results to test the hypothesis that the field can stabilise the atmosphere and suppress the generation of macro-turbulence down to stellar layers where the magnetic pressure PB and the gas pressure Pg are comparable. Using a simple grey atmosphere to estimate the temperature T0 at which PB = Pg, we find that T0 > Teff for all investigated magnetic stars, but that T0 reaches the ~160000 K layers associated with the iron opacity-bump in hot stars only for NGC1624-2. This is consistent with the view that the responsible physical mechanism for photospheric O-star macro-turbulence may be stellar gravity-mode oscillations excited by sub-surface convection zones, and suggests that a sufficiently strong magnetic field can suppress such iron-bump generated convection and associated pulsational excitation.
1305.5549v1
2013-06-14
Dynamic Transcript Profiling of Candida Albicans Infection in Zebrafish: a Pathogen-Host Interaction Study
Candida albicans is responsible for a number of life-threatening infections and causes considerable morbidity and mortality in immunocompromised patients. Previous studies of C. albicans pathogenesis have suggested several steps must occur before virulent infection, including early adhesion, invasion, and late tissue damage. However, the mechanism that triggers C. albicans transformation from yeast to hyphae form during infection has yet to be fully elucidated. This study used a systems biology approach to investigate C. albicans infection in zebrafish. The surviving fish were sampled at different post-infection time points to obtain time-lapsed, genome-wide transcriptomic data from both organisms, which were accompanied with in sync histological analyses. Principal component analysis (PCA) was used to analyze the dynamic gene expression profiles of significant variations in both C. albicans and zebrafish. The results categorized C. albicans infection into three progressing phases: adhesion, invasion, and damage. Such findings were highly supported by the corresponding histological analysis. Furthermore, the dynamic interspecies transcript profiling revealed that C. albicans activated its filamentous formation during invasion and the iron scavenging functions during the damage phases, whereas zebrafish ceased its iron homeostasis function following massive hemorrhage during the later stages of infection. This was followed by massive hemorrhaging toward the end stage of infection. Most of the immune related genes were expressed as the infection progressed from invasion to the damage phase. Such global, inter-species evidence of virulence-immune and iron competition dynamics during C. albicans infection could be crucial in understanding control fungal pathogenesis.
1306.3312v1
2013-10-09
Electron doping evolution of the magnetic excitations in BaFe2-xNixAs2
We use inelastic neutron scattering (INS) spectroscopy to study the magnetic excitations spectra throughout the Brioullion zone in electron-doped iron pnictide superconductors BaFe$_{2-x}$Ni$_{x}$As$_{2}$ with $x=0.096,0.15,0.18$. While the $x=0.096$ sample is near optimal superconductivity with $T_c=20$ K and has coexisting static incommensurate magnetic order, the $x=0.15,0.18$ samples are electron-overdoped with reduced $T_c$ of 14 K and 8 K, respectively, and have no static antiferromagnetic (AF) order. In previous INS work on undoped ($x=0$) and electron optimally doped ($x=0.1$) samples, the effect of electron-doping was found to modify spin waves in the parent compound BaFe$_2$As$_2$ below $\sim$100 meV and induce a neutron spin resonance at the commensurate AF ordering wave vector that couples with superconductivity. While the new data collected on the $x=0.096$ sample confirms the overall features of the earlier work, our careful temperature dependent study of the resonance reveals that the resonance suddenly changes its $Q$-width below $T_c$ similar to that of the optimally hole-doped iron pnictides Ba$_{0.67}$K$_{0.33}$Fe$_2$As$_2$. In addition, we establish the dispersion of the resonance and find it to change from commensurate to transversely incommensurate with increasing energy. Upon further electron-doping to overdoped iron pnictides with $x=0.15$ and 0.18, the resonance becomes weaker and transversely incommensurate at all energies, while spin excitations above $\sim$100 meV are still not much affected. Our absolute spin excitation intensity measurements throughout the Brillouin zone for $x=0.096,0.15,0.18$ confirm the notion that the low-energy spin excitation coupling with itinerant electron is important for superconductivity in these materials, even though the high-energy spin excitations are weakly doping dependent.
1310.2333v1
2013-10-11
The return to the hard state of GX 339-4 as seen by Suzaku
The microquasar GX 339-4 was observed by Suzaku five times, spaced by a few days, during its transition back to the hard state at the end of its 2010-2011 outburst. The 2-10 keV source flux decreases by a factor ~10 between the beginning and the end of the monitoring. Simultaneous radio and OIR observations highlighted the re-ignition of the radio emission just before the beginning of the campaign, the maximum radio emission being reached between the two first Suzaku pointings, while the IR peaked a few weeks latter. A fluorescent iron line is always significantly detected. Fits with a gaussian or Laor profiles give statistically equivalent results. In the case of a Laor profile, fits of the five data sets simultaneously agree with a disk inclination angle of ~20 degrees. The disk inner radius is <10-30 R_g in the first two observations but almost unconstrained in the last three. A soft X-ray excess is also present in these two first observations. Fits with a multicolor disk component give disk inner radii in agreement with those obtained with the iron line fits. The use of a physically more realistic model, including a blurred reflection component and a comptonization continuum, give some hints of the increase of the disk inner radius but the significances are always weak. Interestingly, the addition of warm absorption significantly improves the fit of OBS1 while it is not needed in the other observations. The radio-jet re-ignition occurring between OBS1 and OBS2, these absorption features may indicate the natural evolution from a disk wind and a jet. The comparison with a long 2008 Suzaku observation of GX 339-4 in a persistent faint hard state where a narrow iron line clearly indicates a disk recession, is discussed.
1310.3039v2
2013-10-30
On the Origin of the 6.4 keV Line in the Galactic Center Region
We analyse the 6.4 keV iron line component produced in the Galactic Center (GC) region by cosmic rays in dense molecular clouds (MCs) and in the diffuse molecular gas. We showed that this component, in principle, can be seen in several years in the direction of the cloud Srg B2. If this emission is produced by low energy CRs which ionize the interstellar molecular gas the intensity of the line is quite small, < 1%. However, we cannot exclude that local sources of CRs or X-ray photons nearby the cloud may provide much higher intensity of the line from there. Production of the line emission from molecular clouds depends strongly on processes of CR penetration into them. We show that turbulent motions of neutral gas may generate strong magnetic fluctuations in the clouds which prevent free penetration of CRs into the clouds from outside. We provide a special analysis of the line production by high energy electrons. We concluded that these electrons hardly provide the diffuse 6.4 keV line emission from the GC because their density is depleted by ionization losses. We do not exclude that local sources of electrons may provide an excesses of the 6.4 keV line emission in some molecular clouds and even reproduce a relatively short time variations of the iron line emission. However, we doubt whether a single electron source provides the simultaneous short time variability of the iron line emission from clouds which are distant from each other on hundred pc as observed for the GC clouds. An alternative speculation is that local electron sources could also provide the necessary effect of the line variations in different clouds that are seen simultaneously by chance that seems, however, very unlikely.
1310.8177v1
2013-11-04
On the role of AGN feedback on the thermal and chemodynamical properties of the hot intra-cluster medium
We present an analysis of the properties of the ICM in an extended set of cosmological hydrodynamical simulations of galaxy clusters and groups performed with the TreePM+SPH GADGET-3 code. Besides a set of non-radiative simulations, we carried out two sets of simulations including radiative cooling, star formation, metal enrichment and feedback from supernovae, one of which also accounts for the effect of feedback from AGN resulting from gas accretion onto super-massive black holes. These simulations are analysed with the aim of studying the relative role played by SN and AGN feedback on the general properties of the diffuse hot baryons in galaxy clusters and groups: scaling relations, temperature, entropy and pressure radial profiles, and ICM chemical enrichment. We find that simulations including AGN feedback produce scaling relations that are in good agreement with X-ray observations at all mass scales. However, our simulations are not able to account for the observed diversity between CC and NCC clusters: unlike for observations, we find that temperature and entropy profiles of relaxed and unrelaxed clusters are quite similar and resemble more the observed behaviour of NCC clusters. As for the pattern of metal enrichment, we find that an enhanced level of iron abundance is produced by AGN feedback with respect to the case of purely SN feedback. As a result, while simulations including AGN produce values of iron abundance in groups in agreement with observations, they over-enrich the ICM in massive clusters. The efficiency of AGN feedback in displacing enriched gas from halos into the inter-galactic medium at high redshift also creates a widespread enrichment in the outskirts of clusters and produces profiles of iron abundance whose slope is in better agreement with observations.
1311.0818v1
2013-11-07
GIANO-TNG spectroscopy of red supergiants in the young star cluster RSGC2
The inner disk of the Galaxy has a number of young star clusters dominated by red supergiants that are heavily obscured by dust extinction and observable only at infrared wavelengths. These clusters are important tracers of the recent star formation and chemical enrichment history in the inner Galaxy. During the technical commissioning and as a first science verification of the GIANO spectrograph at the Telescopio Nazionale Galileo, we secured high-resolution (R~50,000) near-infrared spectra of three red supergiants in the young Scutum cluster RSGC2. Taking advantage of the full YJHK spectral coverage of GIANO in a single exposure, we were able to identify several tens of atomic and molecular lines suitable for chemical abundance determinations. By means of spectral synthesis and line equivalent width measurements, we obtained abundances of Fe and other iron-peak elements such as V, Cr, Ni, of alpha (O, Mg, Si, Ca and Ti) and other light elements (C, N, Na, Al, K, Sc), and of some s-process elements (Y, Sr). We found iron abundances between half and one third solar and solar-scaled [X/Fe] abundance patterns of iron-peak, alpha and most of the light elements, consistent with a thin-disk chemistry. We found a depletion of [C/Fe] and enhancement of [N/Fe], consistent with CN burning, and low 12C/13C abundance ratios (between 9 and 11), requiring extra-mixing processes in the stellar interiors during the post-main sequence evolution. Finally, we found a slight [Sr/Fe] enhancement and a slight [Y/Fe] depletion (by a factor of <=2), with respect to solar.
1311.1639v1
2013-12-20
Nematic order in iron superconductors - who is in the driver's seat?
Although the existence of nematic order in iron-based superconductors is now a well-established experimental fact, its origin remains controversial. Nematic order breaks the discrete lattice rotational symmetry by making the $x$ and $y$ directions in the Fe plane non-equivalent. This can happen because of (i) a tetragonal to orthorhombic structural transition, (ii) a spontaneous breaking of an orbital symmetry, or (iii) a spontaneous development of an Ising-type spin-nematic order - a magnetic state that breaks rotational symmetry but preserves time-reversal symmetry. The Landau theory of phase transitions dictates that the development of one of these orders should immediately induce the other two, making the origin of nematicity a physics realization of a "chicken and egg problem". The three scenarios are, however, quite different from a microscopic perspective. While in the structural scenario lattice vibrations (phonons) play the dominant role, in the other two scenarios electronic correlations are responsible for the nematic order. In this review, we argue that experimental and theoretical evidence strongly points to the electronic rather than phononic mechanism, placing the nematic order in the class of correlation-driven electronic instabilities, like superconductivity and density-wave transitions. We discuss different microscopic models for nematicity in the iron pnictides, and link nematicity to other ordered states of the global phase diagram of these materials -- magnetism and superconductivity. In the magnetic model nematic order pre-empts stripe-type magnetic order, and the same interaction which favors nematicity also gives rise to an unconventional $s^{+-}$ superconductivity. In the charge/orbital model magnetism appears as a secondary effect of ferro-orbital order, and the interaction which favors nematicity gives rise to a conventional $s^{++}$ superconductivity.
1312.6085v1
2014-03-24
On the fine structure of the Cepheid metallicity gradient in the Galactic thin disk
We present homogeneous and accurate iron abundances for 42 Galactic Cepheids based on high-spectral resolution (R~38,000) high signal-to-noise ratio (SNR>100) optical spectra collected with UVES at VLT (128 spectra). The above abundances were complemented with high-quality iron abundances provided either by our group (86) or available in the literature. We paid attention in deriving a common metallicity scale and ended up with a sample of 450 Cepheids. We also estimated for the entire sample accurate individual distances by using homogeneous near-infrared photometry and the reddening free Period-Wesenheit relations. The new metallicity gradient is linear over a broad range of Galactocentric distances (Rg~5-19 kpc) and agrees quite well with similar estimates available in the literature (-0.060+/-0.002 dex/kpc). We also uncover evidence which suggests that the residuals of the metallicity gradient are tightly correlated with candidate Cepheid Groups (CGs). The candidate CGs have been identified as spatial overdensities of Cepheids located across the thin disk. They account for a significant fraction of the residual fluctuations, and in turn for the large intrinsic dispersion of the metallicity gradient. We performed a detailed comparison with metallicity gradients based on different tracers: OB stars and open clusters. We found very similar metallicity gradients for ages younger than 3 Gyrs, while for older ages we found a shallower slope and an increase in the intrinsic spread. The above findings rely on homogeneous age, metallicity and distance scales. Finally we found, by using a large sample of Galactic and Magellanic Cepheids for which are available accurate iron abundances, that the dependence of the luminosity amplitude on metallicity is vanishing.
1403.6128v1
2014-07-03
The Detection of Earth-mass Planets around Active Stars: The Mass of Kepler-78b
Kepler-78b is a transiting Earth-mass planet in an 8.5 hr orbit discovered by the Kepler Space Mission. We performed an analysis of the published radial velocity measurements for Kepler-78 in order to derive a refined measurement for the planet mass. Kepler-78 is an active star and radial velocity variations due to activity were removed using a Floating Chunk Offset (FCO) method where an orbital solution was made to the data by allowing the velocity offsets of individual nights to vary. We show that if we had no a priori knowledge of the transit period the FCO method used as a periodogram would still have detected Kepler-78b in the radial velocity data. It can thus be effective at finding unknown short-period signals in the presence of significant activity noise. Using the FCO method while keeping the ephemeris and orbital phase fixed to the photometric values and using only data from nights where 6-10 measurements were taken results in a K-amplitude of 1.34 +/- 0.25 m/s. a planet mass of 1.31 +/- 0.24 M_Earth, and a planet density of rho = 4.5 (-2.0/+2.2) g/cm^3. Allowing the orbital phase to be a free parameter reproduces the transit phase to within the uncertainty. The corresponding density implies that Kepler-78b may have a structure that is deficient in iron and is thus more like the Moon. Although the various approaches that were used to filter out the activity of Kepler 78 produce consistent radial velocity amplitudes to within the errors, these are still too large to constrain the structure of this planet. The uncertainty in the mass for Kepler-78b is large enough to encompass models with structures ranging from Mercury-like (iron enriched) to Moon-like (iron deficient). A more accurate K-amplitude as well as a better determination of the planet radius are needed to distinguish between these models.
1407.0853v1
2014-08-06
Theory of the evolution of magnetic order in Fe$_{1+y}$Te compounds with increasing interstitial iron
We examine the influence of the excess of interstitial Fe on the magnetic properties of Fe$_{1+y}$Te compounds. Because in iron chalcogenides the correlations are stronger than in the iron arsenides, we assume in our model that some of the Fe orbitals give rise to localized magnetic moments. These moments interact with each other via exchange interactions as well as phonon-mediated biquadratic interactions that favor a collinear double-stripe state, corresponding to the ordering vectors $\left(\pm\pi/2,\pm\pi/2\right)$. The remaining Fe orbitals are assumed to be itinerant, giving rise to the first-principle derived Fermi surface displaying nesting features at momenta $\left(\pi,0\right)/\left(0,\pi\right)$. Increasing the amount of itinerant electrons due to excess Fe, $y$, leads to changes in the Fermi surface and to the suppression of its nesting properties. As a result, due to the Hund's coupling between the itinerant and localized moments, increasing $y$ leads to modifications in the local moments' exchange interactions via the multi-orbital generalization of the long-range Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. By numerically computing the RKKY corrections and minimizing the resulting effective exchange Hamiltonian, we find, in general, that the excess electrons introduced in the system change the classical magnetic ground state from a double-stripe state to an incommensurate spiral, consistent with the experimental observations. We show that these results can be understood as a result of the suppression of magnetic spectral weight of the itinerant electrons at momenta $\left(\pi,0\right)/\left(0,\pi\right)$, combined with the transfer of broad magnetic spectral weight from large to small momenta, promoted by the introduction of excess Fe.
1408.1418v2
2014-11-28
Superconducting properties and pseudogap from preformed Cooper pairs in the triclinic (CaFe$_{1-x}$Pt$_x$As)$_{10}$Pt$_3$As$_8$
Using a combination of muon-spin relaxation ($\mu$SR), inelastic neutron scattering (INS) and nuclear magnetic resonance (NMR), we investigated the novel iron-based superconductor with a triclinic crystal structure (CaFe$_{1-x}$Pt$_x$As)$_{10}$Pt$_3$As$_8$ (T$_{\rm c}$ = 13 K), containing platinum-arsenide intermediary layers. The temperature dependence of the superfluid density obtained from the $\mu$SR relaxation-rate measurements indicates the presence of two superconducting gaps, $\Delta_\text{1}\gg\Delta_\text{2}$. According to our INS measurements, commensurate spin fluctuations are centered at the ($\pi$, 0) wave vector, like in most other iron arsenides. Their intensity remains unchanged across T$_\text{c}$, indicating the absence of a spin resonance typical for many Fe-based superconductors. Instead, we observed a peak in the spin-excitation spectrum around $\hslash\omega_0=\,$7 meV at the same wave vector, which persists above T$_{\rm c}$ and is characterized by the ratio $\hslash\omega_0/k_\text{B}T_\text{c}\approx\,$6.2, which is significantly higher than typical values for the magnetic resonant modes in iron pnictides (~4.3). The temperature dependence of magnetic intensity at 7 meV revealed an anomaly around T* = 45 K related to the disappearance of this new mode. A suppression of the spin-lattice relaxation rate, $1/T_1T$, observed by NMR immediately below T* without any notable subsequent anomaly at T$_{\rm c}$, indicates that T* could mark the onset of a pseudogap in (CaFe$_{1-x}$Pt$_x$As)$_{10}$Pt$_3$As$_8$, which is likely associated with the emergence of preformed Cooper pairs.
1411.7858v1
2014-12-30
An XSPEC model to explore spectral features from black-hole sources - II. The relativistic iron line in the lamp-post geometry
In X-ray spectra of several active galactic nuclei and Galactic black hole binaries a broad relativistically smeared iron line is observed. This feature arises by fluorescence when the accretion disc is illuminated by hot corona above it. Due to central location of the corona the illumination and thus also the line emission decrease with radius. It was reported in the literature that this decrease is very steep in some of the sources, suggesting a highly compact corona. We revisit the lamp-post setup in which the corona is positioned on the axis above the rotating black hole and investigate to what extent the steep emissivity can be explained by this scenario. We show the contributions of the relativistic effects to the disc illumination by the primary source - energy shift, light bending and aberration. The lamp-post radial illumination pattern is compared to the widely used radial broken power-law emissivity profile. We find that very steep emissivities require the primary illuminating source to be positioned very near the black hole horizon and/or the spectral power-law index of the primary emission to be very high. The broken power-law approximation of the illumination can be safely used when the primary source is located at larger heights. However, for low heights the lamp-post illumination considerably differs from this approximation. We also show the variations of the iron line local flux over the disc due to the flux dependence on incident and emission angles. The former depends mainly on the height of the primary source while the latter depends on the inclination angle of the observer. Thus the strength of the line varies substantially across the disc. This effect may contribute to the observed steeper emissivity.
1412.8627v1
2015-03-14
Deep SDSS optical spectroscopy of distant halo stars II. Iron, calcium, and magnesium abundances
We analyze a sample of 3,944 low-resolution (R ~ 2000) optical spectra from the Sloan Digital Sky Survey (SDSS), focusing on stars with effective temperatures 5800 < Teff < 6300 K, and distances from the Milky Way plane in excess of 5 kpc, and determine their abundances of Fe, Ca, and Mg. We followed the same methodology as in the previous paper in this series, deriving atmospheric parameters by chi2 minimization, but this time we obtained the abundances of individual elements by fitting their associated spectral lines. Distances were calculated from absolute magnitudes obtained by a statistical comparison of our stellar parameters with stellar-evolution models. The observations reveal a decrease in the abundances of iron, calcium, and magnesium at large distances from the Galactic center. The median abundances for the halo stars analyzed are fairly constant up to a Galactocentric distance r ~ 20 kpc, rapidly decrease between r ~ 20 and r ~ 40 kpc, and flatten out to significantly lower values at larger distances, consistent with previous studies. In addition, we examine the [Ca/Fe] and [Mg/Fe] as a function of Fe/H and Galactocentric distance. Our results show that the most distant parts of the halo show a steeper variation of the [Ca/Fe] and [Mg/Fe] with iron. We found that at the range -1.6 < [Fe/H] < -0.4 [Ca/Fe] decreases with distance, in agreement with earlier results based on local stars. However, the opposite trend is apparent for [Mg/Fe]. Our conclusion that the outer regions of the halo are more metal-poor than the inner regions, based on in situ observations of distant stars, agrees with recent results based on inferences from the kinematics of more local stars, and with predictions of recent galaxy formation simulations for galaxies similar to the Milky Way.
1503.04362v1
2015-05-29
NuSTAR and Suzaku observations of the hard state in Cygnus X-1: locating the inner accretion disk
We present simultaneous Nuclear Spectroscopic Telescope Array (NuSTAR ) and Suzaku observations of the X-ray binary Cygnus X-1 in the hard state. This is the first time this state has been observed in Cyg X-1 with NuSTAR, which enables us to study the reflection and broad-band spectra in unprecedented detail. We confirm that the iron line cannot be fit with a combination of narrow lines and absorption features, and instead requires a relativistically blurred profile in combination with a narrow line and absorption from the companion wind. We use the reflection models of Garcia et al. (2014) to simultaneously measure the black hole spin, disk inner radius, and coronal height in a self-consistent manner. Detailed fits to the iron line profile indicate a high level of relativistic blurring, indicative of reflection from the inner accretion disk. We find a high spin, a small inner disk radius, and a low source height, and rule out truncation to greater than three gravitational radii at the 3{\sigma} confidence level. In addition, we find that the line profile has not changed greatly in the switch from soft to hard states, and that the differences are consistent with changes in the underlying reflection spectrum rather than the relativistic blurring. We find that the blurring parameters are consistent when fitting either just the iron line or the entire broad-band spectrum, which is well modelled with a Comptonized continuum plus reflection model.
1506.00007v1
2015-06-03
The complex accretion geometry of GX 339-4 as seen by NuSTAR and Swift
We present spectral analysis of five NuSTAR and Swift observations of GX 339-4 taken during a failed outburst in summer 2013. These observations cover Eddington luminosity fractions in the range ~0.9-6%. Throughout this outburst, GX 339-4 stayed in the hard state, and all five observations show similar X-ray spectra with a hard power-law with a photon index near 1.6 and significant contribution from reflection. Using simple reflection models we find unrealistically high iron abundances. Allowing for different photon indices for the continuum incident on the reflector relative to the underlying observed continuum results in a statistically better fit and reduced iron abundances. With a photon index around 1.3, the input power-law on the reflector is significantly harder than that which is directly observed. We study the influence of different emissivity profiles and geometries and consistently find an improvement when using separate photon indices. The inferred inner accretion disk radius is strongly model dependent, but we do not find evidence for a truncation radius larger than 100 r_g in any model. The data do not allow independent spin constraints but the results are consistent with the literature (i.e., a>0). Our best-fit models indicate an inclination angle in the range 40-60 degrees, consistent with limits on the orbital inclination but higher than reported in the literature using standard reflection models. The iron line around 6.4 keV is clearly broadened, and we detect a superimposed narrow core as well. This core originates from a fluorescence region outside the influence of the strong gravity of the black hole and we discuss possible geometries.
1506.01381v1
2015-06-05
NuSTAR and Swift observations of the black hole candidate XTE J1908+094 during its 2013 outburst
The black hole candidate XTE J1908+094 went into outburst for the first time since 2003 in October 2013. We report on an observation with the Nuclear Spectroscopic Telescope Array (NuSTAR) and monitoring observations with Swift during the outburst. NuSTAR caught the source in the soft state: the spectra show a broad relativistic iron line, and the light curves reveal a ~40 ks flare with the count rate peaking about 40% above the non-flare level and with significant spectral variation. A model combining a multi-temperature thermal component, a power-law, and a reflection component with an iron line provides a good description of the NuSTAR spectrum. Although relativistic broadening of the iron line is observed, it is not possible to constrain the black hole spin with these data. The variability of the power-law component, which can also be modeled as a Comptonization component, is responsible for the flux and spectral change during the flare, suggesting that changes in the corona (or possibly continued jet activity) are the likely cause of the flare.
1506.02001v2
2015-07-28
Probing M subdwarf metallicity with an esdK5+esdM5.5 binary
We present a spectral analysis of the binary G 224-58 AB that consists of the coolest M extreme subdwarf (esdM5.5) and a brighter primary (esdK5). This binary may serve as a benchmark for metallicity measurement calibrations and as a test-bed for atmospheric and evolutionary models for esdM objects. We determine abundances primarily using high resolution optical spectra of the primary. Other parameters were determined from the fits of synthetic spectra computed with these abundances to the observed spectra from 0.4 to 2.5 microns for both components. We determine \Tef =4625 $\pm$ 100 K, \logg = 4.5 $\pm$ 0.5 for the A component and \Tef = 3200 $\pm$ 100 K, \logg = 5.0 $\pm$ 0.5, for the B component. We obtained abundances of [Mg/H]=$-$1.51$\pm$0.08, [Ca/H]=$-$1.39$\pm$0.03, [Ti/H]=$-$1.37$\pm$0.03 for alpha group elements and [CrH]=$-$1.88$\pm$0.07, [Mn/H]=$-$1.96$\pm$0.06, [Fe/H]=$-$1.92$\pm$0.02, [Ni/H]=$-$1.81$\pm$0.05 and [Ba/H]W=$-$1.87$\pm$0.11 for iron group elements from fits to the spectral lines observed in the optical and infrared spectral regions of the primary. We find consistent abundances with fits to the secondary albeit at lower signal-to-noise. Abundances of elements in \ga and \gb atmospheres cannot be described by one metallicity parameter. The offset of $\sim$ 0.4 dex between the abundances derived from alpha element and iron group elements corresponds with our expectation for metal-deficient stars. We thus clarify that some indices used to date to measure metallicities for establishing esdM stars based on CaH, MgH and TiO band system strength ratios in the optical and H$_2$O in the infrared relate to abundances of alpha-element group rather than to iron peak elements. For metal deficient M dwarfs with [Fe/H] < -1.0, this provides a ready explanation for apparently inconsistent "metallicities" derived using different methods.
1507.07740v1
2015-10-16
The Transient Accereting X-Ray Pulsar XTE J1946+274: Stability of the X-Ray Properties at Low Flux and Updated Orbital Solution
We present a timing and spectral analysis of the X-ray pulsar XTE J1946+274 observed with Suzaku during an outburst decline in 2010 October and compare with previous results. XTE J1946+274 is a transient X-ray binary consisting of a Be-type star and a neutron star with a 15.75 s pulse period in a 172 d orbit with 2-3 outbursts per orbit during phases of activity. We improve the orbital solution using data from multiple instruments. The X-ray spectrum can be described by an absorbed Fermi-Dirac cutoff power law model along with a narrow Fe K line at 6.4 keV and a weak Cyclotron Resonance Scattering Feature (CRSF) at ~35 keV. The Suzaku data are consistent with the previously observed continuum flux versus iron line flux correlation expected from fluorescence emission along the line of sight. However, the observed iron line flux is slightly higher, indicating the possibility of a higher iron abundance or the presence of non-uniform material. We argue that the source most likely has only been observed in the subcritical (non-radiation dominated) state since its pulse profile is stable over all observed luminosities and the energy of the CRSF is approximately the same at the highest (~$5 \times 10^{37} $erg s$^{-1}$) and lowest (~$5 \times 10^{36} $erg s$^{-1}$) observed 3-60 keV luminosities.
1510.05032v1
2015-11-02
Electron correlation effects and scattering rates in Fe$_{1+y}$Te$_{1-x}$Se$_x$ superconductor
Using angle-resolved photoemission spectroscopy we have studied the low-energy electronic structure and the Fermi surface topology of Fe$_{1+y}$Te$_{1-x}$Se$_x$ superconductors. Similar to the known iron pnictides we observe hole pockets at the center and electron pockets at the corner of the Brillouin zone (BZ). However, on a finer level, the electronic structure around the $\Gamma$- and $Z$-points in $k$-space is substantially different from other iron pnictides, in that we observe two hole pockets at the $\Gamma$-point, and more interestingly only one hole pocket is seen at the $Z$-point, whereas in $1111$-, $111$-, and $122$-type compounds, three hole pockets could be readily found at the zone center. Another major difference noted in the Fe$_{1+y}$Te$_{1-x}$Se$_x$ superconductors is that the top of innermost hole-like band moves away from the Fermi level to higher binding energy on going from $\Gamma$ to $Z$, quite opposite to the iron pnictides. The polarization dependence of the observed features was used to aid the attribution of the orbital character of the observed bands. Photon energy dependent measurements suggest a weak $k_z$ dispersion for the outer hole pocket and a moderate $k_z$ dispersion for the inner hole pocket. By evaluating the momentum and energy dependent spectral widths, the single-particle self-energy was extracted and interestingly this shows a pronounced non-Fermi liquid behaviour for these compounds. The experimental observations are discussed in context of electronic band structure calculations and models for the self-energy such as the spin-fermion model and the marginal-Fermi liquid.
1511.00424v1
2015-12-03
Strong anisotropy in nearly ideal-tetrahedral superconducting FeS single crystals
We report the novel preparation of single crystals of tetragonal iron sulfide, FeS, which exhibits a nearly ideal tetrahedral geometry with S--Fe--S bond angles of 110.2(2) $^\circ$ and 108.1(2) $^\circ$. Grown via hydrothermal de-intercalation of K${_x}$Fe${_{2-y}}$S${_2}$ crystals under basic and reducing conditions, the silver, plate-like crystals of FeS remain stable up to 200 $^\circ$C under air and 250 $^\circ$C under inert conditions, even though the mineral "mackinawite" (FeS) is known to be metastable. FeS single crystals exhibit a superconducting state below $T_c=4$ K as determined by electrical resistivity, magnetic susceptibility, and heat capacity measurements, confirming the presence of a bulk superconducting state. Normal state measurements yield an electronic specific heat of 5~mJ/mol-K$^2$, and paramagnetic, metallic behavior with a low residual resistivity of 250~$\mu\Omega\cdot$cm. Magnetoresistance measurements performed as a function of magnetic field angle tilted toward both transverse and longitudinal orientations with respect to the applied current reveal remarkable two-dimensional behavior. This is paralleled in the superconducting state, which exhibits the largest known upper critical field $H_{c2}$ anisotropy of all iron-based superconductors, with $H_{c2}^{||ab}(0) / H_{c2}^{||c}(0)=$(2.75~T)/(0.275~T)=10. Comparisons to theoretical models for 2D and anisotropic-3D superconductors, however, suggest that FeS is the latter case with a large effective mass anisotropy. We place FeS in context to other closely related iron-based superconductors and discuss the role of structural parameters such as anion height on superconductivity.
1512.01245v3
2016-01-26
Low-energy Population III supernovae and the origin of extremely metal-poor stars
Some ancient, dim, metal-poor stars may have formed in the ashes of the first supernovae (SNe). If their chemical abundances can be reconciled with the elemental yields of specific Population III (Pop III) explosions, they could reveal the properties of primordial stars. But multidimensional simulations of such explosions are required to predict their yields because dynamical instabilities can dredge material up from deep in the ejecta that would otherwise be predicted to fall back on to the central remnant and be lost in one-dimensional (1D) models. We have performed two-dimensional (2D) numerical simulations of two low-energy Pop III SNe, a 12.4 Msun explosion and a 60 Msun explosion, and find that they produce elemental yields that are a good fit to those measured in the most iron-poor star discovered to date, SMSS J031300.36-670839.3 (J031300). Fallback on to the compact remnant in these weak explosions accounts for the lack of measurable iron in J031300 and its low iron-group abundances in general. Our 2D explosions produce higher abundances of heavy elements (atomic number Z > 20) than their 1D counterparts due to dredge-up by fluid instabilities. Since almost no Ni is ejected by these weak SNe, their low luminosities will prevent their detection in the near-infrared with the James Webb Space Telescope and future 30-m telescopes on the ground. The only evidence that they ever occurred will be in the fossil abundance record.
1601.06896v3
2016-02-29
Andreev spectroscopy of iron-based superconductors: temperature dependence of the order parameters and scaling of the $Δ_{L,S}$ with $T_C$
We studied iron-based superconductors of various families with critical temperatures covering almost all range $T_C = 9 - 53$ K. In natural arrays of contacts formed in these materials we observed intrinsic multiple Andreev reflections effect (IMARE). By using IMARE spectroscopy, we detected the two-gap superconductivity, determined the value of the large and the small superconducting gaps, and the corresponding BCS-ratios. The temperature dependencies of the large and the small gaps $\Delta_{L,S}(T)$ are similar for various families of the Fe-based superconductors and could be well-fitted in the framework of the two-band model by Moskalenko and Suhl. We concluded on the extended s-wave symmetry of the $\Delta_L$ order parameter (20-30 % anisotropy in k-space) and on the absence of nodes for $\Delta_S$. The BCS-ratio $2\Delta_L/k_BT_C \approx 5.2$ is nearly constant within the whole range of $T_C$ (this means that coupling rate is unchanged), reflecting the 20 % reduction of the $T_C^{local}$ in relation to the eigen $T_C^L$, and the large gap roughly corresponds to the energy of magnetic resonance $2\Delta_L \approx E_{res}$. This result requires a special theoretical consideration. Our estimation of the relative coupling constants and eigen parameters of each condensate (in a hypothetical case of a zero interband interaction) $2\Delta_L/k_BT_C^L = 4.2 - 4.8$ and $2\Delta_S/k_BT_C^S = 3.5 - 4.5$ leads to indirect conclusion that namely a strong electron-phonon interaction in each condensate described in the framework of the Eliashberg theory plays the key role in the superconductivity of iron-based oxypnictides. With it, the two condensates interact weakly with each other. The observed scaling of $\Delta_{L,S}$ with $T_C$, as was discussed above, is caused mainly by changing of the density of states $N_{L,S}$ in the bands, whereas Ln-O spacers act as charge reservoirs.
1602.09114v2
2016-03-01
X-ray-binary spectra in the lamp post model
[Abridged] Context. The high-energy radiation from black-hole binaries may be due to the reprocessing of a lamp located on the black hole axis, emitting X-rays. The observed spectrum is made of 3 components: the direct spectrum; the thermal bump; and the reflected spectrum made of the Compton hump and the iron-line complex. Aims. We aim at computing accurately the complete reprocessed spectrum (thermal bump + reflected) of black-hole binaries over the entire X-ray band. We also determine the strength of the direct component. Our choice of parameters is adapted to a source showing an important thermal component. Methods. We compute in full GR the illumination of a thin disk by a lamp along the rotation axis. We use the ATM21 radiative transfer code to compute the spectrum emitted along the disk. We ray trace this local spectrum to determine the reprocessed spectrum as observed at infinity. We discuss the dependence of the local and ray-traced spectra on the emission angle and spin. Results. We show the importance of the angle dependence of the total disk specific intensity spectrum emitted by the illuminated atmosphere when the thermal disk emission if fully taken into account. High spin implies high temperature in the inner regions, so the emitted thermal disk spectrum covers the iron-line complex. As a result we locally observe absorption lines produced in the hot disk atmosphere. Absorption lines are narrow and disappear after ray tracing the local spectrum. Conclusions. Our results mainly highlight the importance of considering the angle dependence of the local spectrum when computing reprocessed spectra, as was already found in a recent study. The main new result of our work is to show the importance of computing the thermal bump of the spectrum, as this feature can change considerably the observed iron-line complex.
1603.00185v2
2016-09-15
Self-consistent mapping: Effect of local environment on formation of magnetic moment in alpha-FeSi2
We suggest here the method of the mapping of DFT calculations on the multiorbital model in a following way: the parameters of the formulated multiorbital model should be determined from the requirement that the self-consistent charge and spin densities found from the ab initio and model calculations have to be as close to each other as possible. The analysis of the model allows for detailed understanding of the role played by different parameters of the model in the physics of interest. As an example of the approach we present the study of the effect of silicon atoms substitution by the iron atoms and vice versa on the magnetic properties in the iron silicide alpha-FeSi2. The DFT+GGA calculations are mapped to the model with intraatomic Coulomb and exchange interactions, hoppings to nearest and next nearest atoms and exchange of the delocalized electrons between iron atoms; the magnetic moments on atoms and charge densities of the material are found self-consistently within the Hartree-Fock approximation. We find that while the stoichiometric alpha-FeSi2 is nonmagnetic, the substitutions generate different magnetic structures. For example, the substitution of three Si atoms by the Fe atoms results in the ferrimagnetic structure whereas the substitution of four Si atoms by Fe atoms gives rise to either the nonmagnetic or the ferromagnetic state depending on the type of local enviroment of the substitutional Fe atoms. Besides, contrary to the commonly accepted statement that the destruction of the magnetic moment is controlled only by the number of Fe-Si nearest neighbors, we find that actually it is controlled by the Fe-Fe next-nearest-neighbors. This finding led us to the counterintuitive conclusion: an increase of Si concentration in Fe1-xSi2+x ordered alloys may lead to a ferromagnetism. This conclusion is confirmed by the calculation within GGA-to-DFT.
1609.04624v1
2016-09-26
Phase Transition of Iron-based Single Crystals at Extreme Strain Rates under Dynamic Loadings
Phase transition of iron, as a prototype of martensite phase transition under dynamic loadings, exhibits huge diverges in its TP among experiments with different pressure medium and loading rates, even in the same initial samples. Great achievements are made in understanding strain or stress dependence of the TP under dynamic loadings. However, present understandings on the strain rate dependence of the TP are far from clear, even a virgin for extreme high strain rates. In this work, large scale NEMD simulations are conducted to study the effects of strain rates on the phase transition of iron-based single crystals. Our results show that the phase transition is preceded by lattice instabilities under ramp compressions, but present theory, represented by modified Born criteria, cannot correctly predict observed onsets of the instability. Through considering both strain and strain gradient disturbances, new instability criteria are proposed, which could be generally applied for studying instabilities under either static or dynamic loadings. For the ramp with a strain rate smaller than about 1010s-1, the observed onset of instabilities is indeed equal to the one predicted by the new instability criteria under small gradient disturbances. The observed onsets deviates from the predicted one at lager strain rates because of finite strain gradient effect. Interestingly, the strain rate dependence of the TP also exhibits an obvious change at the same strain rate, i.e., 1010 s-1. When 1010 s-1, a certain power law is obeyed, but it is not applicable at larger strain rates. This strain rate effect on the TP is well interpreted with nucleation time and the finite strain gradient effect. According to these basic understandings, the roles of strain rates on nucleation and growth of the phase transition are studied.
1609.07829v2
2017-01-24
Nucleosynthesis in the Innermost Ejecta of Neutrino-Drive Supernova Explosions in Two Dimensions
We examine the nucleosynthesis in the innermost, neutrino-processed ejecta (a few $10^{-3}\,M_\odot$) of self-consistent, two-dimensional explosion models of core-collapse supernovae for six progenitor stars with different initial masses. Three models have initial masses near the low-mass end of the supernova range, $8.8\,M_\odot$ (e8.8; electron-capture supernova), $9.6\,M_\odot$ (z9.6), and $8.1\,M_\odot$ (u8.1), with initial metallicities of 1, 0, and $10^{-4}$ times the solar metallicity, respectively. The other three are solar-metallicity models with initial masses of $11.2\,M_\odot$ (s11), $15\,M_\odot$ (s15), and $27\,M_\odot$ (s27). The low-mass models e8.8, z9.6, and u8.1 exhibit high production factors (nucleosynthetic abundances relative to the solar ones) of 100--200 for light trans-iron elements from Zn to Zr. This is associated with appreciable ejection of neutron-rich matter in these models. Remarkably, the nucleosynthetic outcomes for progenitors e8.8 and z9.6 are almost identical, including interesting productions of $^{48}$Ca and $^{60}$Fe, irrespective of their quite different (O-Ne-Mg and Fe) cores prior to collapse. In the more massive models s11, s15, and s27, several proton-rich isotopes of light trans-iron elements, including the $p$-isotope $^{92}$Mo (for s27) are made, up to production factors of $\sim$30. Both electron-capture and core-collapse supernovae near the low-mass end can therefore be dominant contributors to the Galactic inventory of light trans-iron elements from Zn to Zr and probably $^{48}$Ca and live $^{60}$Fe. The innermost ejecta of more massive supernovae may have only sub-dominant contributions to the chemical enrichment of the Galaxy except for $^{92}$Mo.
1701.06786v2
2017-04-04
Competing spin density wave, collinear, and helical magnetism in Fe1+xTe
The Fe1+xTe phase diagram consists of two distinct magnetic structures with collinear order present at low interstitial iron concentrations and a helical phase at large values of x with these phases separated by a Lifshitz point. We use unpolarized single crystal diffraction to confirm the helical phase for large interstitial iron concentrations and polarized single crystal diffraction to demonstrate the collinear order for the iron deficient side of the Fe1+xTe phase diagram. Polarized neutron inelastic scattering show that the fluctuations associated with this collinear order are predominately transverse at low energy transfers, consistent with a localized magnetic moment picture. We then apply neutron inelastic scattering and polarization analysis to investigate the dynamics and structure near the boundary between collinear and helical order in the Fe1+xTe phase diagram. We first show that the phase separating collinear and helical order is characterized by a spin-density wave with a single propagation wave vector of (~ 0.45, 0, 0.5). We do not observe harmonics or the presence of a charge density wave. The magnetic fluctuations associated with this wavevector are different from the collinear phase being strongly longitudinal in nature and correlated anisotropically in the (H,K) plane. The excitations preserve the C4 symmetry of the lattice, but display different widths in momentum along the two tetragonal directions at low energy transfers. While the low energy excitations and minimal magnetic phase diagram can be understood in terms of localized interactions, we suggest that the presence of density wave phase implies the importance of electronic and orbital properties.
1704.01111v1
2017-05-07
The peculiar Na-O anticorrelation of the bulge globular cluster NGC 6440
Context. Galactic Globular Clusters (GCs) are essential tools to understand the earliest epoch of the Milky Way, since they are among the oldest objects in the Universe and can be used to trace its formation and evolution. Current studies using high resolution spectroscopy for many stars in each of a large sample of GCs allow us to develop a detailed observational picture about their formation and their relation with the Galaxy. However, it is necessary to complete this picture by including GCs that belong to all major Galactic components, including the Bulge. Aims. Our aim is to perform a detailed chemical analyses of the bulge GC NGC 6440 in order to determine if this object has Multiple Populations (MPs) and investigate its relation with the Bulge of the Milky Way and with the other Galactic GCs, especially those associated with the Bulge, which are largely poorly studied. Methods. We determined the stellar parameters and the chemical abundances of light elements (Na, Al), iron-peak elements (Fe, Sc, Mn, Co, Ni), $\alpha$-elements (O, Mg, Si, Ca, Ti) and heavy elements (Ba, Eu) in seven red giant members of NGC 6440 using high resolution spectroscopy from FLAMES@UVES. Results. We found a mean iron content of [Fe/H]=-0.50$\pm$0.03 dex in agreement with other studies. We found no internal iron spread. On the other hand, Na and Al show a significant intrinsic spread, but the cluster has no significant O-Na anticorrelation nor exhibits a Mg-Al anticorrelation. The $\alpha$-elements show good agreement with the Bulge field star trend, although they are at the high alpha end and are also higher than those of other GCs of comparable metallicity. The heavy elements are dominated by the r-process, indicating a strong contribution by SNeII. The chemical analysis suggests an origin similar to that of the Bulge field stars.
1705.02684v1
2017-05-10
Direct Measurement of Nuclear Dependence of Charged Current Quasielastic-like Neutrino Interactions using MINERvA
Charged-current $\nu_{\mu}$ interactions on carbon, iron, and lead with a final state hadronic system of one or more protons with zero mesons are used to investigate the influence of the nuclear environment on quasielastic-like interactions. The transfered four-momentum squared to the target nucleus, $Q^2$, is reconstructed based on the kinematics of the leading proton, and differential cross sections versus $Q^2$ and the cross-section ratios of iron, lead and carbon to scintillator are measured for the first time in a single experiment. The measurements show a dependence on atomic number. While the quasielastic-like scattering on carbon is compatible with predictions, the trends exhibited by scattering on iron and lead favor a prediction with intranuclear rescattering of hadrons accounted for by a conventional particle cascade treatment. These measurements help discriminate between different models of both initial state nucleons and final state interactions used in the neutrino oscillation experiments.
1705.03791v1
2017-05-30
Chemical Complexity in the Eu-enhanced Monometallic Globular Cluster NGC 5986
NGC 5986 is a poorly studied but relatively massive Galactic globular cluster that shares several physical and morphological characteristics with "iron-complex" clusters known to exhibit significant metallicity and heavy element dispersions. In order to determine if NGC 5986 joins the iron-complex cluster class, we investigated the chemical composition of 25 red giant branch and asymptotic giant branch cluster stars using high resolution spectra obtained with the Magellan-M2FS instrument. Cluster membership was verified using a combination of radial velocity and [Fe/H] measurements, and we found the cluster to have a mean heliocentric radial velocity of +99.76 km s^-1 (sigma = 7.44 km s^-1). We derived a mean metallicity of [Fe/H] = -1.54 dex (sigma = 0.08 dex), but the cluster's small dispersion in [Fe/H] and low [La/Eu] abundance preclude it from being an iron-complex cluster. NGC 5986 has <[Eu/Fe]> = +0.76 dex (sigma = 0.08 dex), which is among the highest ratios detected in a Galactic cluster. NGC 5986 exhibits classical globular cluster characteristics, such as uniformly enhanced [alpha/Fe] ratios, a small dispersion in Fe-peak abundances, and (anti-)correlated light element variations. Similar to NGC 2808, we find evidence that NGC 5986 may host at least 4-5 populations with distinct light element compositions, and the presence of a clear Mg-Al anti-correlation along with an Al-Si correlation suggests that the cluster gas experienced processing at temperatures >65-70 MK. However, the current data do not support burning temperatures exceeding ~100 MK. We find some evidence that the first and second generation stars in NGC 5986 may be fully spatially mixed, which could indicate that the cluster has lost a significant fraction of its original mass. [abridged]
1705.10840v1
2017-07-11
First results from the IllustrisTNG simulations: A tale of two elements -- chemical evolution of magnesium and europium
The distribution of elements in galaxies provides a wealth of information about their production sites and their subsequent mixing into the interstellar medium. Here we investigate the distribution of elements within stars in the IllustrisTNG simulations. In particular, we analyze the abundance ratios of magnesium and europium in Milky Way-like galaxies from the TNG100 simulation (stellar masses ${\log} (M_\star / {\rm M}_\odot) \sim 9.7 - 11.2$). As abundances of magnesium and europium for individual stars in the Milky Way are observed across a variety of spatial locations and metallicities, comparison with the stellar abundances in our more than $850$ Milky Way-like galaxies provides stringent constraints on our chemical evolutionary methods. To this end we use the magnesium to iron ratio as a proxy for the effects of our SNII and SNIa metal return prescription, and a means to compare our simulated abundances to a wide variety of galactic observations. The europium to iron ratio tracks the rare ejecta from neutron star -- neutron star mergers, the assumed primary site of europium production in our models, which in turn is a sensitive probe of the effects of metal diffusion within the gas in our simulations. We find that europium abundances in Milky Way-like galaxies show no correlation with assembly history, present day galactic properties, and average galactic stellar population age. In general, we reproduce the europium to iron spread at low metallicities observed in the Milky Way, with the level of enhancement being sensitive to gas properties during redshifts $z \approx 2-4$. We show that while the overall normalization of [Eu/Fe] is susceptible to resolution and post-processing assumptions, the relatively large spread of [Eu/Fe] at low [Fe/H] when compared to that at high [Fe/H] is very robust.
1707.03401v2
2017-08-20
Large anomalous Nernst and spin Nernst effects in noncollinear antiferromagnets Mn$_3X$ ($X$ = Sn, Ge, Ga)
Noncollinear antiferromagnets have recently been attracting considerable interest partly due to recent surprising discoveries of the anomalous Hall effect (AHE) in them and partly because they have promising applications in antiferromagnetic spintronics. Here we study the anomalous Nernst effect (ANE), a phenomenon having the same origin as the AHE, and also the spin Nernst effect (SNE) as well as AHE and the spin Hall effect (SHE) in noncollinear antiferromagnetic Mn$_3X$ ($X$ = Sn, Ge, Ga) within the Berry phase formalism based on {\it ab initio} relativistic band structure calculations. For comparison, we also calculate the anomalous Nernst conductivity (ANC) and anomalous Hall conductivity (AHC) of ferromagnetic iron as well as the spin Nernst conductivity (SNC) of platinum metal. Remarkably, the calculated ANC at room temperature (300 K) for all three alloys is huge, being up to 5 times larger than that of iron. Moreover, the calculated SNC for Mn$_3$Sn and Mn$_3$Ga is also large, being as large as that of platinum. This suggests that these anitferromagnets would be useful materials for thermoelectronic devices and spin caloritronic devices. The calculated ANC of Mn$_3$Sn and iron are in reasonably good agreement with the very recent experiments. The calculated SNC of platinum also agrees with the very recent experiments in both sign and magnitude. The calculated thermoelectric and thermomagnetic properties are analyzed in terms of the band structures as well as the energy-dependent AHC, ANC, SNC and spin Hall conductivity via the Mott relations.
1708.05933v3
2017-09-15
Investigating the interstellar dust through the Fe K-edge
The chemical and physical properties of interstellar dust in the densest regions of the Galaxy are still not well understood. X-rays provide a powerful probe since they can penetrate gas and dust over a wide range of column densities (up to $10^{24}\ \rm{cm}^{-2}$). The interaction (scattering and absorption) with the medium imprints spectral signatures that reflect the individual atoms which constitute the gas, molecule, or solid. In this work we investigate the ability of high resolution X-ray spectroscopy to probe the properties of cosmic grains containing iron. Although iron is heavily depleted into interstellar dust, the nature of the Fe-bearing grains is still largely uncertain. In our analysis we use iron K-edge synchrotron data of minerals likely present in the ISM dust taken at the European Synchrotron Radiation Facility. We explore the prospects of determining the chemical composition and the size of astrophysical dust in the Galactic centre and in molecular clouds with future X-ray missions. The energy resolution and the effective area of the present X-ray telescopes are not sufficient to detect and study the Fe K-edge, even for bright X-ray sources. From the analysis of the extinction cross sections of our dust models implemented in the spectral fitting program SPEX, the Fe K-edge is promising for investigating both the chemistry and the size distribution of the interstellar dust. We find that the chemical composition regulates the X-ray absorption fine structures in the post edge region, whereas the scattering feature in the pre-edge is sensitive to the mean grain size. Finally, we note that the Fe K-edge is insensitive to other dust properties, such as the porosity and the geometry of the dust.
1709.05359v1
2017-10-11
Fermi surface with Dirac fermions in CaFeAsF determined via quantum oscillation measurements
Despite the fact that 1111-type iron arsenides hold the record transition temperature of iron-based superconductors, their electronic structures have not been studied much because of the lack of high-quality single crystals. In this study, we completely determine the Fermi surface in the antiferromagnetic state of CaFeAsF, a 1111 iron-arsenide parent compound, by performing quantum oscillation measurements and band-structure calculations. The determined Fermi surface consists of a symmetry-related pair of Dirac electron cylinders and a normal hole cylinder. From analyses of quantum-oscillation phases, we demonstrate that the electron cylinders carry a nontrivial Berry phase $\pi$. The carrier density is of the order of 10$^{-3}$ per Fe. This unusual metallic state with the extremely small carrier density is a consequence of the previously discussed topological feature of the band structure which prevents the antiferromagnetic gap from being a full gap. We also report a nearly linear-in-$B$ magnetoresistance and an anomalous resistivity increase above about 30 T for $B \parallel c$, the latter of which is likely related to the quantum limit of the electron orbit. Intriguingly, the electrical resistivity exhibits a nonmetallic temperature dependence in the paramagnetic tetragonal phase ($T >$ 118 K), which may suggest an incoherent state. Our study provides a detailed knowledge of the Fermi surface in the antiferromagnetic state of 1111 parent compounds and moreover opens up a new possibility to explore Dirac-fermion physics in those compounds.
1710.03938v3
2017-10-26
X-ray reflection from cold white dwarfs in magnetic cataclysmic variables
We model X-ray reflection from white dwarfs (WD) in magnetic cataclysmic variables (mCVs) with a Monte Carlo simulation. A point source with a power-law spectrum or a realistic post-shock accretion column (PSAC) source irradiates a cool and spherical WD. The PSAC source emits thermal spectra of various temperatures stratified along the column according to the PSAC model. In the point source simulation, we confirm (1) a source harder and nearer to the WD enhances the reflection, (2) higher iron abundance enhances the equivalent widths (EWs) of fluorescent iron K${\alpha}_{1,2}$ lines and their Compton shoulder, and increases cut-off energy of a Compton hump, and (3) significant reflection appears from an area that is more than 90 deg apart from the position right under the point X-ray source because of the WD curvature. The PSAC simulation reveals that (1) a more massive WD basically enhances the intensities of the fluorescent iron K${\alpha}_{1,2}$ lines and the Compton hump, except for some specific accretion rate, because the more massive WD makes the hotter PSAC from which higher energy X-rays are preferentially emitted, (2) a larger specific accretion rate monotonically enhances the reflection because it makes the hotter and shorter PSAC, and (3) the intrinsic thermal component hardens by occultation of the cool base of the PSAC by the WD. We quantitatively evaluate influences of the parameters on the EWs and the Compton hump with both types of sources. We also calculate X-ray modulation profiles brought about by the WD spin. They depend on angles of the spin axis from the line of sight and from the PSAC, and whether the two PSACs can be seen. The reflection spectral model and the modulation model involve the fluorescent lines and the Compton hump and can directly be compared to the data which allow us to evaluate these geometrical parameters with unprecedented accuracy.
1710.09931v1
2017-12-19
Magnetic phase diagram of the iron pnictides in the presence of spin-orbit coupling: Frustration between $C_2$ and $C_4$ magnetic phases
We investigate the impact of spin anisotropic interactions, promoted by spin-orbit coupling, on the magnetic phase diagram of the iron-based superconductors. Three distinct magnetic phases with Bragg peaks at $(\pi,0)$ and $(0,\pi)$ are possible in these systems: one $C_2$ (i.e. orthorhombic) symmetric stripe magnetic phase and two $C_4$ (i.e. tetragonal) symmetric magnetic phases. While the spin anisotropic interactions allow the magnetic moments to point in any direction in the $C_2$ phase, they restrict the possible moment orientations in the $C_4$ phases. As a result, an interesting scenario arises in which the spin anisotropic interactions favor a $C_2$ phase, but the other spin isotropic interactions favor a $C_4$ phase. We study this frustration via both mean-field and renormalization-group approaches. We find that, to lift this frustration, a rich magnetic landscape emerges well below the magnetic transition temperature, with novel $C_2$, $C_4$, and mixed $C_2$-$C_4$ phases. Near the putative magnetic quantum critical point, spin anisotropies promote a stable Gaussian fixed point in the renormalization-group flow, which is absent in the spin isotropic case, and is associated with a near-degeneracy between $C_2$ and $C_4$ phases. We argue that this frustration is the reason why most $C_4$ phases in the iron pnictides only appear inside the $C_2$ phase, and discuss additional manifestations of this frustration in the phase diagrams of these materials.
1712.07192v4
2018-01-03
Sequential structural and antiferromagnetic transitions in BaFe$_2$Se$_3$ under pressure
The discovery of superconductivity in the two-leg ladder compound BaFe$_2$S$_3$ has established the 123-type iron chalcogenides as a novel and interesting subgroup of the iron-based superconductors family. However, in this 123 series, BaFe$_2$Se$_3$ is an exceptional member, with a magnetic order and crystalline structure different from all others. Recently, an exciting experiment reported the emergence of superconductivity in BaFe$_2$Se$_3$ at high pressure [J.-J. Ying, et al., Phys. Rev. B 95, 241109 (R) (2017)]. In this publication, we report a first principles study of BaFe$_2$Se$_3$. Our analysis unveils a variety of qualitative differences between BaFe$_2$S$_3$ and BaFe$_2$Se$_3$, including in the latter an unexpected chain of transitions with increasing pressure. First, by gradually reducing the tilting angle of iron ladders, the crystalline structure smoothly transforms from Pnma to Cmcm at ~6 GPa. Second, the system becomes metallic at 10.4 GPa. Third, its unique ambient pressure Block antiferromagnetic ground state is replaced by the more common CX antiferromagnetic order at ~12 GPa, the same magnetic state of the 123-S ladder. This transition is found at a pressure very similar to the experimental superconducting transition. Finally, all magnetic moments vanish at 30 GPa. This reported theoretical diagram of the complete phase evolution is important because of the technical challenges to capture many physical properties in high-pressure experiments. The information obtained in our calculations suggest different characteristics for superconductivity in BaFe$_2$Se$_3$ and BaFe$_2$S$_3$: in 123-S pairing occurs when magnetic moments vanish, while in 123-Se the transition region from Block- to CX-type magnetism appears to catalyze superconductivity. Finally, an additional superconducting dome above ~30 GPa is expected to occur.
1801.00877v1
2018-02-12
Superconducting transition temperatures in the electronic and magnetic phase diagrams of Sr2VFeAsO3-delta, a superconductor
We elucidate the magnetic phases and superconducting transition temperatures (Tc) in Sr2VFeAsO3-delta (21113V), an iron-based superconductor with a thick-blocking layer fabricated from a perovskite-related transition metal oxide. At low temperatures (T < 37.1 K), 21113V exhibited a superconducting phase in the range 0.031 =< delta =< 0.145 and an antiferromagnetic (AFM) iron sublattice in the range 0.267 =< delta =< 0.664. Mixed-valent vanadium exhibited a dominant AFM phase in 0.031 =< delta =< 0.088, and a partial ferrimagnetic (Ferri.) phase in the range 0.124 =< delta =< 0.664. The Ferri. phase was the most dominant at a delta value of 0.267, showing an AFM phase of Fe at T < 20 K. Increasing the spontaneous magnetic moments reduced the magnetic shielding volume fraction due to the superconducting phase. This result was attributed to the magnetic phase of vanadium, which dominates the superconductivity of Fe in 21113V. The Tc-delta curve showed two maxima. The smaller and larger of Tc maxima occurred at delta = 0.073 and delta = 0.145, respectively; the latter resides on the phase boundary between AFM and the partial Ferri. phases of vanadium. 21113V is a useful platform for verifing new mechanisms of Tc enhancement in iron-based superconductors.
1802.03907v2
2018-07-20
Measurement of the Iron Spectrum in Cosmic Rays by VERITAS
We present a new measurement of the energy spectrum of iron nuclei in cosmic rays from 20 to 500 TeV. The measurement makes use of a template-based analysis method, which, for the first time, is applied to the energy reconstruction of iron-induced air showers recorded by the VERITAS array of imaging atmospheric Cherenkov telescopes. The event selection makes use of the direct Cherenkov light which is emitted by charged particles before the first interaction, as well as other parameters related to the shape of the recorded air shower images. The measured spectrum is well described by a power law $\frac{\mathrm{d} F}{\mathrm{d} E}=f_0\cdot \left(\frac{E}{E_0}\right)^{-\gamma}$ over the full energy range, with $\gamma = 2.82 \pm 0.30 \mathrm{(stat.)} ^{+0.24}_{-0.27} \mathrm{(syst.)}$ and $f_0 = \left( 4.82 \pm 0.98 \mathrm{(stat.)}^{+2.12}_{-2.70} \mathrm{(syst.)} \right)\cdot 10^{-7}$m$^{-2}$s$^{-1}$sr$^{-1}$TeV$^{-1}$ at $E_0=50$TeV, with no indication of a cutoff or spectral break. The measured differential flux is compatible with previous results, with improved statistical uncertainty at the highest energies.
1807.08010v1
2018-07-23
The Quantum Field Of A Magnet Shown By A Nanomagnetic Ferrolens
It has been more than two hundred years since the first iron filings experiment, showing us the 2D macroscopic magnetic imprint of the field of a permanent magnet. However, latest developments in modern nanomagnetic passive direct observation devices reveal in real-time and color a more intriguing 3D dynamic and detailed image of the field of a magnet, with surprising new findings, that can change our perspective for dipole magnetism forever and lead to new research. This research is a continuation of our previous work (DOI: 10.1016/j.jmmm.2017.12.023). The magnetostatic fields were under our scope and examined with the aid of the ferrolens. We are presenting experimental and photographical evidence, demonstrating the true complex 3D Euclidian geometry of the quantum field of permanent magnets that have never been seen before and the classic iron filings experiment, apart of its 2D limitations, fails to depict. An analysis of why and what these iron filings inherent limitations are, giving us an incomplete and also in some degree misguiding image of the magnetic field of a magnet is carried out, whereas, as we prove the ferrolens is free of these limitations and its far more advanced visualization capabilities is allowing it to show the quantum image with depth of field information, of the dipole field of a permanent magnet. For the first time the domain wall (i.e. Bloch or Neel wall) region of the field of a magnet is clearly made visible by the ferrolens along with what phenomenon is actually taking place there, leading to the inescapable conclusion, novel observation and experimental evidence that the field of any dipole magnet actually consists of two distinct and separate toroidal shaped 3D magnetic bubbles, each located at either side of the dipole around the exact spatial regions where the two poles of the magnet reside.
1807.08751v1
2018-10-05
(16) Psyche: A mesosiderite-like asteroid?
Asteroid (16) Psyche is the target of the NASA Psyche mission. It is considered one of the few main-belt bodies that could be an exposed proto-planetary metallic core and that would thus be related to iron meteorites. Such an association is however challenged by both its near- and mid-infrared spectral properties and the reported estimates of its density. Here, we aim to refine the density of (16) Psyche to set further constraints on its bulk composition and determine its potential meteoritic analog. We observed (16) Psyche with ESO VLT/SPHERE/ZIMPOL as part of our large program (ID 199.C-0074). We used the high angular resolution of these observations to refine Psyche's three-dimensional (3D) shape model and subsequently its density when combined with the most recent mass estimates. In addition, we searched for potential companions around the asteroid. We derived a bulk density of 3.99\,$\pm$\,0.26\,g$\cdot$cm$^{-3}$ for Psyche. While such density is incompatible at the 3-sigma level with any iron meteorites ($\sim$7.8\,g$\cdot$cm$^{-3}$), it appears fully consistent with that of stony-iron meteorites such as mesosiderites (density $\sim$4.25\,$\cdot$cm$^{-3}$). In addition, we found no satellite in our images and set an upper limit on the diameter of any non-detected satellite of 1460\,$\pm$\,200}\,m at 150\,km from Psyche (0.2\%\,$\times$\,R$_{Hill}$, the Hill radius) and 800\,$\pm$\,200\,m at 2,000\,km (3\%\,$\times$\,$R_{Hill}$). Considering that the visible and near-infrared spectral properties of mesosiderites are similar to those of Psyche, there is merit to a long-published initial hypothesis that Psyche could be a plausible candidate parent body for mesosiderites.
1810.02771v1
2018-11-26
Confirming the presence of second population stars and the iron discrepancy along the AGB of the globular cluster NGC 6752
Asymptotic giant branch (AGB) stars in the globular cluster NGC6752 have been found to exhibit some chemical peculiarities with respect to the red giant branch (RGB) stars. A discrepancy between [FeI/H] and [FeII/H] (not observed in RGB stars) has been detected adopting spectroscopic temperatures. Moreover, a possible lack of second-population stars along the AGB was claimed. The use of photometric temperatures based on (V-K) colors was proposed to erase this iron discrepancy. Also, ad hoc scenarios have been proposed to explain the absence of second-population AGB stars. Here we analyzed a sample of 19 AGB and 14 RGB stars of NGC6752 observed with the spectrographs UVES. The two temperature scales agree very well for the RGB stars while for the AGB stars there is a systematic offset of ~100 K. We found that even if the photometric temperatures alleviate the iron discrepancy with respect to the spectroscopic ones, a systematic difference between [FeI/H] and [FeII/H] is still found among the AGB stars. An unexpected result is that the photometric temperatures do not satisfy the excitation equilibrium in the AGB stars. This suggests that standard 1D-LTE model atmospheres are unable to properly describe the thermal structure of AGB stars, at variance with the RGB stars. The use of photometric temperatures confirms the previous detection of second-population AGB stars in this cluster, with the presence of clear correlations/anticorrelations among the light element abundances. This firmly demonstrates that both first and second-population stars evolve along the AGB of NGC6752.
1811.10626v1
2019-03-06
Lattice Disorder Effect on Magnetic Ordering of Iron Arsenides
This study investigates the changes of magnetic ordering temperature via nano- and mesoscale structural features in an iron arsenide. Although magnetic ground states in quantum materials can be theoretically predicted from known crystal structures and chemical compositions, the ordering temperature is harder to pinpoint due to such local lattice variations. In this work we find surprisingly that a locally disordered material can exhibit a significantly larger Neel temperature (TN) than an ordered material of precisely the same chemical stoichiometry. Here, a EuFe2As2 crystal, which is a 122 parent of iron arsenide superconductors, is found through synthesis to have ordering below TN = 195 K (for the disordered crystal) or TN = 175 K (for the ordered crystal). In the higher TN crystals, there are shorter planar Fe-Fe bonds [2.7692(2) A vs. 2.7745(3) A], a randomized in-plane defect structure, and diffuse scattering along the [00L] crystallographic direction that manifests as a rather broad specific heat peak. For the lower TN crystals, the a-lattice parameter is larger and the in-plane microscopic structure shows defect ordering along the antiphase boundaries, giving a larger TN and a higher superconducting temperature (Tc) upon the application of pressure. First principles calculations find a strong interaction between c-axis strain and interlayer magnetic coupling, but little impact of planar strain on the magnetic order. Neutron single-crystal diffraction shows that the low-temperature magnetic phase transition due to localized Eu moments is not lattice or disorder sensitive, unlike the higher-temperature Fe sublattice ordering. This study demonstrates a higher magnetic ordering point arising from local disorder in 122.
1903.02545v2
2019-05-24
How much of the Solar System should we leave as Wilderness?
"How much of the Solar System should we reserve as wilderness, off-limits to human development?" We argue that, as a matter of policy, development should be limited to one eighth, with the remainder set aside. We argue that adopting a "1/8 principle" is far less restrictive, overall, than it might seem. One eighth of the iron in the asteroid belt is more than a million times greater than all of the Earth's estimated iron reserves and may suffice for centuries. A limit of some sort is needed because of the problems associated with exponential growth. Humans are poor at estimating the pace of such growth, so the limitations of a resource are hard to recognize before the final three doubling times which take utilization successively from 1/8 to 1/4 to 1/2, and then to the point of exhaustion. Population growth and climate change are instances of unchecked exponential growth. Each places strains upon ouru available resources. Each is a problem we would like to control but attempts to do so at this comparatively late stage have not been encouraging. Our limited ability to see ahead suggests that we should set ourselves a 'tripwire' that gives us at least 3 doubling times as leeway, i.e. when 1/8 of Solar System resources are close to being exploited. At a 3.5 percent growth rate for the space economy, comparable to that of the iron use from the beginning of the Industrial Revolution until now, the 1/8 point would be reached after 400 years. At that point the 20 year doubling time of a 3.5 percent growth rate means that only 60 years would remain to transition the economic system to new "steady state" conditions. The rationale for adopting the 1/8 principle now is that it may be far easier to implement in principle restrictions at an early stage, rather than later, when vested and competing interests have come into existence.
1905.13681v1
2019-07-26
Stabilization of $\varepsilon$-Fe$_2$O$_3$ epitaxial layer on MgO(111)/GaN via an intermediate $γ$-Fe$_2$O$_3$-phase
In the present study we have demonstrated epitaxial stabilization of the metastable magnetically-hard $\varepsilon$-Fe$_2$O$_3$ phase on top of a thin MgO(111) buffer layer grown onto the GaN (0001) surface. The primary purpose to introduce a 4\,nm-thick buffer layer of MgO in between Fe$_2$O$_3$ and GaN was to stop thermal migration of Ga into the iron oxide layer. Though such migration and successive formation of the orthorhombic GaFeO$_3$ was supposed earlier to be a potential trigger of the nucleation of the isostructural $\varepsilon$-Fe$_2$O$_3$, the present work demonstrates that the growth of single crystalline uniform films of epsilon ferrite by pulsed laser deposition is possible even on the MgO capped GaN. The structural properties of the 60\,nm thick Fe$_2$O$_3$ layer on MgO / GaN were probed by electron and x-ray diffraction, both suggesting that the growth of $\varepsilon$-Fe$_2$O$_3$ is preceded by formation of a thin layer of $\gamma$-Fe$_2$O$_3$. The presence of the magnetically hard epsilon ferrite was independently confirmed by temperature dependent magnetometry measurements. The depth-resolved x-ray and polarized neutron reflectometry reveal that the 10\,nm iron oxide layer at the interface has a lower density and a higher magnetization than the main volume of the $\varepsilon$-Fe$_2$O$_3$ film. The density and magnetic moment depth profiles derived from fitting the reflectometry data are in a good agreement with the presence of the magnetically degraded $\gamma$-Fe$_2$O$_3$ transition layer between MgO and $\varepsilon$-Fe$_2$O$_3$. The natural occurrence of the interface between magnetoelectric $\varepsilon$- and spin caloritronic $\gamma$- iron oxide phases can enable further opportunities to design novel all-oxide-on-semiconductor devices.
1907.11611v2
2019-08-06
On the use of field RR Lyrae as Galactic probes: I. The Oosterhoff dichotomy based on fundamental variables
We collected a large data set of field RR Lyrae stars (RRLs) by using catalogues already available in the literature and Gaia DR2. We estimated the iron abundances for a sub-sample of 2,382 fundamental RRLs ($\Delta$S method: CaIIK, H$\beta$, H$\gamma$ and H$\delta$ lines) for which are publicly available medium-resolution SDSS-SEGUE spectra. We also included similar estimates available in the literature ending up with the largest and most homogeneous spectroscopic data set ever collected for RRLs (2,903). The metallicity scale was validated by using iron abundances based on high resolution spectra for a fundamental field RRL (V~Ind), for which we collected X-shooter spectra covering the entire pulsation cycle. The peak ([Fe/H]=-1.59$\pm$0.01) and the standard deviation ($\sigma$=0.43 dex) of the metallicity distribution agree quite well with similar estimates available in the literature. The current measurements disclose a well defined metal-rich tail approaching Solar iron abundance. The spectroscopic sample plotted in the Bailey diagram (period vs luminosity amplitude) shows a steady variation when moving from the metal-poor ([Fe/H]=-3.0/-2.5) to the metal-rich ([Fe/H]=-0.5/0.0) regime. The smooth transition in the peak of the period distribution as a function of the metallicity strongly indicates that the long-standing problem of the Oosterhoff dichotomy among Galactic globulars is the consequence of the lack of metal-intermediate clusters hosting RRLs. We also found that the luminosity amplitude, in contrast with period, does not show a solid correlation with metallicity. This suggests that period-amplitude-metallicity relations should be cautiously treated.
1908.02064v2
2019-08-27
Carbon, oxygen, and iron abundances in disk and halo stars. Implications of 3D non-LTE spectral line formation
The abundances of carbon, oxygen, and iron in late-type stars are important parameters in exoplanetary and stellar physics, as well as key tracers of stellar populations and Galactic chemical evolution. We carried out three-dimensional (3D) non-LTE radiative transfer calculations for CI and OI, and 3D LTE radiative transfer calculations for FeII, across the STAGGER-grid of 3D hydrodynamic model atmospheres. The absolute 3D non-LTE versus 1D LTE abundance corrections can be as severe as $-0.3$ dex for CI lines in low-metallicity F dwarfs, and $-0.6$ dex for OI lines in high-metallicity F dwarfs. The 3D LTE versus 1D LTE abundance corrections for FeII lines are less severe, typically less than $+0.15$ dex. We used the corrections in a re-analysis of carbon, oxygen, and iron in $187$ F and G dwarfs in the Galactic disk and halo. Applying the differential 3D non-LTE corrections to 1D LTE abundances visibly reduces the scatter in the abundance plots. The thick disk and high-$\alpha$ halo population rise in carbon and oxygen with decreasing metallicity, and reach a maximum of [C/Fe]$\approx0.2$ and a plateau of [O/Fe]$\approx0.6$ at [Fe/H]$\approx-1.0$. The low-$\alpha$ halo population is qualitatively similar, albeit offset towards lower metallicities and with larger scatter. Nevertheless, these populations overlap in the [C/O] versus [O/H] plane, decreasing to a plateau of [C/O]$\approx-0.6$ below [O/H]$\approx-1.0$. In the thin-disk, stars having confirmed planet detections tend to have higher values of C/O at given [O/H]; this potential signature of planet formation is only apparent after applying the abundance corrections to the 1D LTE results. Our grids of line-by-line abundance corrections are publicly available and can be readily used to improve the accuracy of spectroscopic analyses of late-type stars.
1908.10319v2
2020-01-03
The chemical composition of the accretion disk and donor star in Ultra Compact X-ray Binaries: A comprehensive X-ray analysis
We have analyzed the X-ray spectra of all known Ultra Compact X-ray Binaries (UCXBs), with the purpose of constraining the chemical composition of their accretion disk and donor star. Our investigation was focused on the presence (or absence) of the Fe K${\alpha}$ emission line, which was used as the probe of chemical composition of the disk, based on previously established theoretical predictions for the reflection of X-ray radiation off the surface of C/O-rich or He-rich accretion disks in UCXBs. We have contrasted the results of our spectral analysis to the history of type I X-ray bursts from these systems, which can also indicate donor star composition. We found that UCXBs with prominent and persistent iron K${\alpha}$ emission also featured repeat bursting activity. On the other hand, the UCXBs for which no iron line was detected, appear to have few or no type I X-ray bursts detected over more than a decade of monitoring. Based on Monte Carlo simulations, demonstrating a strong correlation between the Fe K${\alpha}$ line strength and the abundance of C and O in the accretion disk material and given the expected correlation between the H/He abundance and the recurrence rate of type I X-ray bursts, we propose that there is a considerable likelihood that UCXBs with persistent iron emission have He-rich donors, while those that do not, likely have C/O or O/Ne/Mg-rich donors. Our results strongly advocate for the development of more sophisticated simulations of X-ray reflection from hydrogen-poor accretion disks.
2001.00716v2
2020-01-20
The extreme CNO-enhanced composition of the primitive iron-poor dwarf star J0815+4729
We present an analysis of high-resolution Keck/HIRES spectroscopic observations of J0815+4729, an extremely carbon-enhanced, iron-poor dwarf star. These high-quality data allow us to derive a metallicity of [Fe/H]$=-5.49{\pm}0.14$ from the three strongest \ion{Fe}{1} lines and to measure a high [Ca/Fe]~$=0.75{\pm}0.14$. The large carbon abundance of A(C)~$=7.43{\pm}0.17$ (or [C/Fe]~$\sim 4.49{\pm}0.11$) places this star in the upper boundary of the low-carbon band in the A(C)-[Fe/H] diagram, suggesting no contamination from a binary AGB companion. We detect the oxygen triplet at 777nm for the first time in an ultra-metal poor star, indicating a large oxygen-to-iron abundance ratio of [O/Fe]~$=4.03{\pm}0.12$ (A(O)~$=7.23{\pm}0.14$), significantly higher than the previously most metal-poor dwarf J2209-0028 with an oxygen triplet detection with [O/Fe]~$\sim2.2$~dex at [Fe/H]~$\sim -3.9$. Nitrogen is also dramatically enhanced with (A(N)~$=6.75{\pm}0.08$) and an abundance ratio [N/Fe]~$\sim 4.41{\pm}0.08$. We also detect Ca, Na and Mg, while provide upper limits for eight other elements. The abundance pattern of J0815+4729 resembles that of HE~1327-2326, indicating that both are second-generation stars contaminated by a $\sim 21-27$~\msun~single, zero-metallicity low-energy supernova with very little mixing and substantial fallback. The absence of lithium implies an upper-limit abundance A(Li)~$<1.3$~dex, about 0.7~dex below the detected Li abundance in J0023+0307 which has a similar metallicity, exacerbating the cosmological lithium problem.
2001.07257v2
2020-01-21
Observation of magnetic adatom-induced Majorana vortex and its hybridization with field-induced Majorana vortex in an iron-based superconductor
Braiding Majorana zero modes is essential for fault-tolerant topological quantum computing. Iron-based superconductors with nontrivial band topology have recently emerged as a surprisingly promising platform for creating distinct Majorana zero modes in magnetic vortices in a single material and at relatively high temperatures. The magnetic field-induced Abrikosov vortex lattice makes it difficult to braid a set of Majorana zero modes or to study the coupling of a Majorana doublet due to overlapping wave functions. Here we report the observation of the proposed quantum anomalous vortex with integer quantized vortex core states and the Majorana zero mode induced by magnetic Fe adatoms deposited on the surface. We observe its hybridization with a nearby field-induced Majorana vortex in iron-based superconductor FeTe0.55Se0.45. We also observe vortex-free Yu-Shiba-Rusinov bound states at the Fe adatoms with a weaker coupling to the substrate, and discover a reversible transition between Yu-Shiba-Rusinov states and Majorana zero mode by manipulating the exchange coupling strength. The dual origin of the Majorana zero modes, from magnetic adatoms and external magnetic field, provides a new single-material platform for studying their interactions and braiding in superconductors bearing topological band structures.
2001.07376v2
2020-06-05
Chandra View of the LINER-type Nucleus in the Radio-Loud Galaxy CGCG 292-057: Ionized Iron Line and Jet-ISM Interactions
We present an analysis of the new, deep (94\,ksec) {\it Chandra} ACIS-S observation of radio-loud active galaxy CGCG\,292$-$057, characterized by a LINER-type nucleus and a complex radio structure that indicates intermittent jet activity. On the scale of the host galaxy bulge, we detected excess X-ray emission with a spectrum best fit by a thermal plasma model with a temperature of $\sim 0.8$\,keV. We argue that this excess emission results from compression and heating of the hot diffuse fraction of the interstellar medium displaced by the expanding inner, $\sim 20$\, kpc-scale lobes observed in this restarted radio galaxy. The nuclear X-ray spectrum of the target clearly displays an ionized iron line at $\sim 6.7$\,keV, and is best fitted with a phenomenological model consisting of a power-law (photon index $\simeq 1.8$) continuum absorbed by a relatively large amount of cold matter (hydrogen column density $\simeq 0.7 \times 10^{23}$\,cm$^{-2}$), and partly scattered (fraction $\sim 3\%$) by ionized gas, giving rise to a soft excess component and K$\alpha$ line from iron ions. We demonstrate that the observed X-ray spectrum, particularly the equivalent width of Fe\,\texttt{XXV} K$\alpha$ (of order $0.3$\,keV) can in principle, be explained in a scenario involving a Compton-thin gas located at the scale of the broad-lined region in this source and photoionized by nuclear illumination. We compare the general spectral properties of the CGCG\,292$-$057 nucleus, with those of other nearby LINERs studied in X-rays.
2006.03717v2
2020-06-29
No Redshift Evolution in the Broad Line Region Metallicity up to z=7.54: Deep NIR Spectroscopy of ULAS J1342+0928
We present deep (9 hours) Gemini-N/GNIRS near-infrared spectroscopic observations of ULAS J1342+0928, a luminous quasar at z=7.54. Various broad emission lines were detected, as well as the underlying continuum and iron forests over the rest-frame wavelength 970-2930A. There is a clear trend that higher-ionization emission lines show larger blueshifts with CIV1549 exhibiting 5510^{+240}_{-110} km s-1 blueshift with respect to the systematic redshift from the far-infrared [CII] 158um emission line. Those high ionization lines have wide profiles with FWHM more than 10000 km s-1. A modest blueshift of 340^{+110}_{-80} km s-1 is also seen in MgII, the lowest ionization line identified in the spectrum. The updated MgII-based black hole mass of M_BH=9.1_{-1.3}^{+1.4} x 10^8 M_sun and the Eddington ratio of L_bol/L_Edd=1.1_{-0.2}^{+0.2} confirm that ULAS J1342+0928 is powered by a massive and actively accreting black hole. There is no significant difference in the emission line ratios such as SiIV/CIV and AlIII/CIV when compared to lower-redshift quasars in a similar luminosity range, which suggests early metal pollution of the broad-line-region clouds. This trend also holds for the FeII/MgII line ratio, known as a cosmic clock that traces the iron enrichment in the early universe. Different iron templates and continuum fitting ranges were used to explore how the FeII/MgII measurement changes as a function of spectral modeling. Quasars at even higher redshift or at fainter luminosity range (L_bol<10^46 erg s-1) are needed to probe the sites of early metal enrichment and a corresponding change in the FeII/MgII ratio.
2006.16268v1
2020-08-05
Orbital-selective spin waves in detwinned NaFeAs
The existence of orbital-dependent electronic correlations has been recognized as an essential ingredient to describe the physics of iron-based superconductors. NaFeAs, a parent compound of iron based superconductors, exhibits a tetragonal-to-orthorhombic lattice distortion below $T_s\approx 60$ K, forming an electronic nematic phase with two 90$^\circ$ rotated (twinned) domains, and orders antiferromagnetically below $T_N\approx 42$ K. We use inelastic neutron scattering to study spin waves in uniaxial pressure-detwinned NaFeAs. By comparing the data with combined density functional theory and dynamical mean-field theory calculations, we conclude that spin waves up to an energy scale of $E_\text{crossover} \approx 100$ meV are dominated by $d_{yz}$-$d_{yz}$ intra-orbital scattering processes, which have the two-fold ($C_2$) rotational symmetry of the underlying lattice. On the other hand, the spin wave excitations above $E_\text{crossover}$, which have approximately fourfold ($C_4$) rotational symmetry, arise from the $d_{xy}$-$d_{xy}$ intra-orbital scattering that controls the overall magnetic bandwidth in this material. In addition, we find that the low-energy ($E\approx 6$ meV) spin excitations change from approximate $C_4$ to $C_2$ rotational symmetry below a temperature $T^\ast$ ($>T_s$), while spin excitations at energies above $E_\text{crossover}$ have approximate $C_4$ rotational symmetry and are weakly temperature dependent. These results are consistent with angle resolved photoemission spectroscopy measurements, where the presence of an uniaxial strain necessary to detwin NaFeAs also raises the onset temperature $T^\ast$ of observable orbital-dependent band splitting to above $T_s$, thus supporting the notion of orbital selective spin waves in the nematic phase of iron-based superconductors.
2008.02314v1
2020-10-26
Simulation of hydrogen permeation through pure iron for trapping and surface phenomena characterisation
There is a need for numerical models capable of predicting local accumulation of hydrogen near stress concentrators and crack tips to prevent and mitigate hydrogen assisted fracture in steels. The experimental characterisation of trapping parameters in metals, which is required for an accurate simulation of hydrogen transport, is usually performed through the electropermeation test. In order to study grain size influence and grain boundary trapping during permeation, two modelling approaches are explored; a 1D Finite Element model including trap density and binding energy as input parameters and a polycrystalline model based on the assignment of a lower diffusivity and solubility to the grain boundaries. Samples of pure iron after two different heat treatments - 950C for 40 minutes and 1100C for 5 minutes - are tested applying three consecutive rising permeation steps and three decaying steps. Experimental results show that the finer grain microstructure promotes a diffusion delay due to grain boundary trapping. The usual methodology for the determination of trap densities and binding energies is revisited in which the limiting diluted and saturated cases are considered. To this purpose, apparent diffusivities are fitted including also the influence of boundary conditions and comparing results provided by the constant concentration with the constant flux assumption. Grain boundaries are characterised for pure iron with a binding energy between 37.8 and 39.9 kJ/mol and a low trap density but it is numerically demonstrated that saturated or diluted assumptions are not always verified, and a univocal determination of trapping parameters requires a broader range of charging conditions for permeation. The relationship between surface parameters, i.e. charging current, recombination current and surface concentrations, is also studied.
2010.13567v1
2020-11-11
Non-stoichiometric amorphous magnesium-iron silicates in circumstellar dust shells. Dust growth in outflows from supergiants
We investigate the dust growth in oxygen-rich stellar outflows for a set of nine well-observed massive supergiants with optically thin dust shells. Models of the infrared emission from their circumstellar dust shells are compared to their observed infrared spectra so as to derive the essential parameters that govern dust formation in the extended envelope of these stars. The results obtained from the comparative study are also compared with the predictions of a model for silicate dust condensation solely based on laboratory data and basic stellar properties. The infrared emission in the wavelength range between 6 and 25 mu can be reproduced rather well by a mixture of non-stoichiometric iron-bearing silicates, alumina, and metallic iron dust particles for all nine objects. The observed spectra obtained from three objects, mu Cep, RW Cyg, and RS Per, can be reproduced by a stationary and (essentially) spherically symmetric outflow which enables a direct comparison with predictions from a theoretical dust growth model. The temperature at the onset of massive silicate dust growth is of the order of 920 K and the corresponding outflow velocity of the order of the sound velocity for these objects. The condensation temperature suggests that the silicate dust grows on the corundum dust grains that are formed well in the interior of the silicate dust shell at a much higher temperature. Our results propose that regarding the two major problems of dust formation in stellar outflows: (i) formation of seed nuclei; (ii) their growth to macroscopic dust grains, we are gradually coming close to a quantitative understanding of the second item.
2011.05903v1
2020-11-17
On the Probability that a Rocky Planet's Composition Reflects its Host Star
The bulk density of a planet, as measured by mass and radius, is a result of planet structure and composition. Relative proportions of iron core, rocky mantle, and gaseous envelopes are degenerate for a given density. This degeneracy is reduced for rocky planets without significant gaseous envelopes when the structure is assumed to be a differentiated iron core and rocky mantle, in which the core mass fraction (CMF) is a first-order description of a planet's bulk composition. A rocky planet's CMF may be derived both from bulk density and by assuming the planet reflects the host star's major rock-building elemental abundances (Fe, Mg, and Si). Contrasting CMF measures, therefore, shed light on the outcome diversity of planet formation from processes including mantle stripping, out-gassing, and/or late-stage volatile delivery. We present a statistically rigorous analysis of the consistency of these two CMF measures accounting for observational uncertainties of planet mass and radius and host-star chemical abundances. We find that these two measures are unlikely to be resolvable as statistically different unless the bulk density CMF is at least 40% greater than or 50% less than the CMF as inferred from the host star. Applied to 11 probable rocky exoplanets, Kepler-107c has a CMF as inferred from bulk density that is significantly greater than the inferred CMF from its host star (2$\sigma$) and is therefore likely an iron-enriched super-Mercury. K2-229b, previously described as a super-Mercury, however, does not meet the threshold for a super-Mercury at a 1- or 2- $\sigma$ level.
2011.08893v4
2021-01-22
Spin dynamics in NaFeAs and NaFe$_{0.53}$Cu$_{0.47}$As probed by resonant inelastic X-ray scattering
The parent compounds of iron-based superconductors are magnetically-ordered bad metals, with superconductivity appearing near a putative magnetic quantum critical point. The presence of both Hubbard repulsion and Hund's coupling leads to rich physics in these multiorbital systems, and motivated descriptions of magnetism in terms of itinerant electrons or localized spins. The NaFe$_{1-x}$Cu$_x$As series consists of magnetically-ordered bad metal ($x=0$), superconducting ($x\approx0.02$) and magnetically-ordered semiconducing/insulating ($x\approx0.5$) phases, providing a platform to investigate the connection between superconductivity, magnetism and electronic correlations. Here we use X-ray absorption spectroscopy and resonant inelastic X-ray scattering to study the valence state of Fe and spin dynamics in two NaFe$_{1-x}$Cu$_x$As compounds ($x=0$ and 0.47). We find that magnetism in both compounds arises from Fe$^{2+}$ atoms, and exhibits underdamped dispersive spin waves in their respective ordered states. The dispersion of spin excitations in NaFe$_{0.53}$Cu$_{0.47}$As is consistent with being quasi-one-dimensional. Compared to NaFeAs, the band top of spin waves in NaFe$_{0.53}$Cu$_{0.47}$As is slightly softened with significantly more spectral weight of the spin excitations. Our results indicate the spin dynamics in NaFe$_{0.53}$Cu$_{0.47}$As arise from localized magnetic moments and suggest the iron-based superconductors are proximate to a correlated insulating state with localized iron moments.
2101.08948v1
2021-02-17
Single particle tunneling spectroscopy and superconducting gaps in layered iron based superconductor KCa$_{2}$Fe$_{4}$As$_{4}$F$_{2}$
We perform scanning tunneling microscopy/spectroscopy study on the layered iron based superconductor KCa$_2$Fe$_4$As$_4$F$_2$ with a critical temperature of about 33.5 K. Two types of terminated surfaces are generally observed after cleaving the samples in vacuum. On one commonly obtained surface, we observe a full gap feature with energy gap values close to 4.6 meV. This type of spectrum shows a clean and uniform full gap in space, which indicates the absence of gap nodes in this superconductor. Quasiparticle interference patterns have also been measured, which show no scattering patterns between the hole and tiny electron pockets, but rather an intra-band scattering pattern is observed possibly due to the hole-like $\alpha$ pocket. The Fermi energy of this band is only about $24\pm6$ meV as derived from the energy dispersion result. Meanwhile, impurity induced bound-state peaks can be observed at about $\pm2.2$ meV on some spectra, and the peak value seems to be independent to magnetic field. On the second type of surface which is rarely obtained, the fully gapped feature can still be observed on the tunneling spectra, although multiple gaps are obtained either from a single spectrum or separate ones, and the gap values determined from coherence peaks locate mainly in the range from 4 to 8 meV. Our results clearly indicate multiple and nodeless superconducting gap nature in this layered superconductor KCa$_2$Fe$_4$As$_4$F$_2$, and the superfluid is mainly contributed by the hole-like Fermi surfaces near $\Gamma$ point. This would inspire further consideration on the effect of the shallow and incipient bands near M point, and help to understand the pairing mechanism in this highly layered iron-based superconductor.
2102.08785v1
2021-03-11
Intertwined charge, spin, and pairing orders in doped iron ladders
Motivated by recent experimental progress on iron-based ladder compounds, we study the doped two-orbital Hubbard model for the two-leg ladder BaFe$_2$S$_3$. The model is constructed by using {\it ab initio} hopping parameters and the ground state properties are investigated using the density matrix renormalization group method. We show that the $(\pi,0)$ magnetic ordering at half-filling, with ferromagnetic rungs and antiferromagnetic legs, becomes incommensurate upon hole doping. Moreover, depending on the strength of the Hubbard $U$ coupling, other magnetic patterns, such as $(0,\pi)$, are also stabilized. We found that the binding energy for two holes becomes negative for intermediate Hubbard interaction strength, indicating hole pairing. Due to the crystal-field split among orbitals, the holes primarily reside in one orbital, with the other one remaining half-filled. This resembles orbital selective Mott states. The formation of tight hole pairs continues with increasing hole density, as long as the magnetic order remains antiferromagnetic in one direction. The study of pair-pair correlations indicates the dominance of the intra-orbital spin-singlet channel, as opposed to other pairing channels. Although in a range of hole doping pairing correlations decay slowly, our results can also be interpreted as corresponding to a charge-density-wave made of pairs, a precursor of eventual superconductivity after interladder couplings are included. Such scenario of intertwined orders has been extensively discussed before in the cuprates, and our results suggest a similar physics could exist in ladder iron-based superconductors. Finally, we also show that a robust Hund's coupling is needed for pairing to occur.
2103.06407v2
2021-03-11
Enhancement of Superconductivity Linked with Linear-in-Temperature/Field Resistivity in Ion-Gated FeSe Films
Iron selenide (FeSe) - the structurally simplest iron-based superconductor, has attracted tremendous interest in the past years. While the transition temperature (Tc) of bulk FeSe is $\sim$ 8 K, it can be significantly enhanced to 40 - 50 K by various ways of electron doping. However, the underlying physics for such great enhancement of Tc and so the Cooper pairing mechanism still remain puzzles. Here, we report a systematic study of the superconducting- and normal-state properties of FeSe films via ionic liquid gating. With fine tuning, Tc evolves continuously from below 10 K to above 40 K; in situ two-coil mutual inductance measurements unambiguously confirm the gating is a uniform bulk effect. Close to Tc, the normal-state resistivity shows a linear dependence on temperature and the linearity extends to lower temperatures with the superconductivity suppressed by high magnetic fields. At high fields, the normal-state magnetoresistance exhibits a linear-in-field dependence and obeys a simple scaling relation between applied field and temperature. Consistent behaviors are observed for different-Tc states throughout the gating process, suggesting the pairing mechanism very likely remains the same from low- to high-Tc state. Importantly, the coefficient of the linear-in-temperature resistivity is positively correlated with Tc, similarly to the observations in cuprates, Bechgaard salts and iron pnictide superconductors. Our study points to a short-range antiferromagnetic exchange interaction mediated pairing mechanism in FeSe.
2103.06512v2
2021-06-08
Atomic iron and nickel in the coma of C/1996 B2 (Hyakutake): production rates, emission mechanisms, and possible parents
Two papers recently reported the detection of gaseous nickel and iron in the comae of over 20 comets from observations collected over two decades, including interstellar comet 2I/Borisov. To evaluate the state of the laboratory data in support of these identifications, we re-analyzed archived spectra of comet C/1996 B2 (Hyakutake), one of the nearest and brightest comets of the last century, using a combined experimental and computational approach. We developed a new, many-level fluorescence model that indicates that the fluorescence emission of Fe I and Ni I vary greatly with heliocentric velocity. Combining this model with laboratory spectra of an Fe-Ni plasma, we identified 22 lines of Fe I and 14 lines of Ni I in the spectrum of Hyakutake. Using Haser models, we estimate the nickel and iron production rates as Q(Ni) = 2.6 - 4.1 x 10^22 s^-1 and Q(Fe) = 0.4 - 2.8 x 10^23 s^-1. From derived column densities, the Ni/Fe abundance ratio log10[Ni/Fe] = -0.15 +/- 0.07 deviates significantly from solar abundance ratios, and it is consistent with the ratios observed in solar system comets. Possible production and emission mechanisms are analyzed in context of existing laboratory measurements. Based on the observed spatial distributions, excellent fluorescence model agreement, and Ni/Fe ratio, our findings support an origin consisting of a short-lived unknown parent followed by fluorescence emission. Our models suggest that the strong heliocentric velocity dependence of the fluorescence efficiencies can provide a meaningful test of the physical process responsible for the Fe I and Ni I emission.
2106.04701v2
2021-09-01
No umbrella needed: Confronting the hypothesis of iron rain on WASP-76b with post-processed general circulation models
High-resolution spectra are unique indicators of three-dimensional processes in exoplanetary atmospheres. For instance, in 2020, Ehrenreich et al. reported transmission spectra from the ESPRESSO spectrograph yielding an anomalously large Doppler blueshift from the ultra-hot Jupiter WASP-76b. Interpretations of these observations invoke toy model depictions of gas-phase iron condensation in lower-temperature regions of the planet's atmosphere. In this work, we forward model the atmosphere of WASP-76b with double-gray general circulation models (GCMs) and ray-striking radiative transfer to diagnose the planet's high-resolution transmission spectrum. We confirm that a physical mechanism driving strong east-west asymmetries across the terminator must exist to reproduce large Doppler blueshifts in WASP-76b's transmission spectrum. We identify low atmospheric drag and a deep radiative-convective boundary as necessary components of our GCM to produce this asymmetry (the latter is consistent with existing Spitzer phase curves). However, we cannot reproduce either the magnitude or the time-dependence of the WASP-76b Doppler signature with gas-phase iron condensation alone. Instead, we find that high-altitude, optically thick clouds composed of $\rm Al_2O_3$, Fe, or $\rm Mg_2SiO_4$ provide reasonable fits to the Ehrenreich et al. observations -- with marginal contributions from condensation. This fit is further improved by allowing a small orbital eccentricity ($e \approx 0.017$), consistent with prior WASP-76b orbital constraints. We additionally validate our forward-modeled spectra by reproducing lines of nearly all species detected in WASP-76b by Tabernero et al. 2021. Our procedure's success in diagnosing phase-resolved Doppler shifts demonstrates the benefits of physical, self-consistent, three-dimensional simulations in modeling high-resolution spectra of exoplanet atmospheres.
2109.00163v2
2021-10-21
Heat Capacity of oxide scale in the range from 0 C to 1300 C: Generalized estimates with account for movability of phase transitions
The known data on the heat capacity of magnetite (Fe3O4), hematite (Fe2O3) and iron (Fe) at different temperatures are approximated by formulas containing phase transition temperatures as varying parameters. This allows to take into account the effect of phase transition shifts, for example, due to impurities, lattice defects, grain sizes or high cooling rates. For this purpose, the entire target temperature range from 0 C to 1300 C is divided by phase transition temperatures into separate intervals. The conjugation of the approximating functions between the intervals at the magnetic transition point is performed without a gap, and at the point of polymorphic transformation (alpha Fe - gamma Fe) with a finite gap of heat capacity values. For wustite Fe1-xO which does not experience phase transformations, the temperature dependence of the heat capacity is approximated by a single smooth function. In combination with previously obtained formulas for the density of iron oxides and iron the proposed approximations allow us to estimate the specific mass heat capacity of oxide scale depending of its structural composition and temperature. By model calculations it is shown that at temperatures of 200 C and 900 C specific mass heat capacity of oxide scale practically does not depend on the percentage of its individual components and is approximately 750 and 850 J/(kg K) respectively. At a temperature of about 575 C, on contrary, actually possible variations in the composition of oxide scale can lead to a change in its specific heat capacity from 850 to 1150 J/(kg K). The obtained dependencies are recommended for use in mathematical modeling of production and processing of steel products in the presence of oxide scale on their surface
2110.11101v1
2021-11-20
Gaia-ESO Survey: Detailed elemental abundances in red giants of the peculiar globular cluster NGC 1851
Context. NGC 1851 is one of several globular clusters for which multiple stellar populations of the subgiant branch have been clearly identified and a difference in metallicity detected. A crucial piece of information on the formation history of this cluster can be provided by the sum of A(C+N+O) abundances. However, these values have lacked a general consensus thus far. The separation of the subgiant branch can be based on age and/or A(C+N+O) abundance differences. Aims. Our main aim was to determine carbon, nitrogen, and oxygen abundances for evolved giants in the globular cluster NGC1851 in order to check whether or not the double populations of stars are coeval. Methods. High-resolution spectra, observed with the FLAMES-UVES spectrograph on the ESO VLT telescope, were analysed using a differential model atmosphere method. Results. We provide abundances of up to 29 chemical elements for a sample of 45 giants in NGC 1851. The investigated stars can be separated into two populations with a difference of 0.07 dex in the mean metallicity, 0.3 dex in the mean C/N, and 0.35 dex in the mean s-process dominated element-to-iron abundance ratios [s/Fe]. No significant difference was determined in the mean values of A(C+N+O) as well as in abundance to iron ratios of carbon, alpha- and iron-peak-elements, and of europium. Conclusions. As the averaged A(C+N+O) values between the two populations do not differ, additional evidence is given that NGC 1851 is composed of two clusters, the metal-rich cluster being by about 0.6 Gyr older than the metal-poor one. A global overview of NGC 1851 properties and the detailed abundances of chemical elements favour its formation in a dwarf spheroidal galaxy that was accreted by the Milky Way.
2111.10684v1
2021-12-12
Top-heavy stellar mass distribution in galactic nuclei inferred from the universally high abundance ratio of [Fe/Mg]
Recent observations of active galactic nuclei (AGNs) have shown a high Fe~II/Mg~II line-flux ratio in their broad-line regions, nearly independent of redshift up to $z \gtrsim 6$. The high flux ratio requires rapid production of iron in galactic nuclei to reach an abundance ratio of ${\rm [Fe/Mg]} \gtrsim 0.2$ as high as those observed in matured galaxies in the local universe. We propose a possible explanation of rapid iron enrichment in AGNs by massive star formation that follows a top-heavy initial mass function (IMF) with a power-law index of $\Gamma$ larger than the canonical value of $\Gamma=-2.35$ for a Salpeter IMF. Taking into account metal production channels from different types of SNe, we find that the high value of ${\rm [Fe/Mg]} \gtrsim 0.2$ requires the IMF to be characterized with $\Gamma \gtrsim -1$ ($\Gamma \gtrsim 0$) and a high-mass cutoff at $M_{\rm max} \simeq 100$--$150~{\rm M_\odot}$ $(M_{\rm max} \gtrsim 250~{\rm M_\odot})$. Given the conditions, core-collapse SNe with $M_\ast \gtrsim 70~{\rm M_\odot}$ and pair-instability SNe give a major contribution for iron enrichment. Such top-heavy stellar IMFs would be a natural consequence from mass growth of stars formed in dense AGN disks under Bondi-like gas accretion that is regulated by feedback at $M_\ast \gtrsim 10~{\rm M_\odot}$. The massive stellar population formed in AGN disks also leave stellar-mass black hole remnants, whose mergers associated with gravitational-wave emission account for at most 10 \% of the merger rate inferred from LIGO/Virgo observations to simultaneously explain the high ${\rm [Fe/Mg]}$ ratio with metal ejection.
2112.06151v1
2022-03-16
Measurements of protons and charged pions emitted from $ν_μ$ charged-current interactions on iron at a mean neutrino energy of 1.49$\,$GeV using a nuclear emulsion detector
This study conducted an analysis of muons, protons, and charged pions emitted from $\nu_{\mu}$ charged-current interactions on iron using a nuclear emulsion detector. The emulsion detector with a 65$\,$kg iron target was exposed to a neutrino beam corresponding to 4.0$\times$10$^{19}$ protons on target with a mean neutrino energy of 1.49$\,$GeV. The measurements were performed at a momentum threshold of 200 (50)$\,$MeV/$c$ for protons (pions), which are the lowest momentum thresholds attempted up to now. The measured quantities are the multiplicities, emission angles, and momenta of the muons, protons, and charged pions. In addition to these inclusive measurements, exclusive measurements such as the muon-proton emission-angle correlations of specific channels and the opening angle between the protons of CC0$\pi$2$p$ events were performed. The data were compared to Monte Carlo (MC) predictions and some significant differences were observed. The results of the study demonstrate the capability of detailed measurements of neutrino-nucleus interactions using a nuclear emulsion detector to improve neutrino interaction models.
2203.08367v3
2022-07-06
Atomic diffusion and turbulent mixing in solar-like stars: Impact on the fundamental properties of FG-type stars
Chemical composition is an important factor that affects stellar evolution. The element abundance on the stellar surface evolves along the lifetime of the star because of transport processes, including atomic diffusion. However, models of stars with masses higher than about 1.2Msun predict unrealistic variations at the stellar surface. This indicates the need for competing transport processes that are mostly computationally expensive for large grids of stellar models. The purpose of this study is to implement turbulent mixing in stellar models and assess the possibility of reproducing the effect of radiative accelerations with turbulent mixing for elements like iron in order to make the computation of large grids possible. We computed stellar models with MESA and assessed the effects of atomic diffusion (with radiative acceleration) in the presence of turbulent mixing. We parametrised the effect of radiative accelerations on iron with a turbulent diffusion coefficient. Finally, we tested this parametrisation by modelling two F-type stars of the Kepler Legacy sample. We found that, for iron, a parametrisation of turbulent mixing that simulates the effect of radiative acceleration is possible. This leads to an increase in the efficiency of the turbulent mixing to counteract the effect of gravitational settling. This approximation does not affect significantly the surface abundances of the other elements we studied, except for oxygen and calcium. We demonstrate that this parametrisation has a negligible impact on the accuracy of the seismic properties inferred with these models. Moreover, turbulent mixing makes the computation of realistic F-type star models including the effect atomic diffusion possible. This leads to differences of about 10% in the inferred ages compared to results obtained with models that neglect these processes.
2207.02779v1
2022-07-28
Symmetry protected 1D chains in mixed-valence iron oxides
During the last decade of high-pressure research a whole new series of iron oxides was discovered, like Fe$_4$O$_5$, Fe$_5$O$_6$, Fe$_7$O$_9$ etc., featuring closely related structures with arrays of one-dimensional (1D) chains of trigonal prisms embedded between slabs of octahedra. Here, we develop a unified approach to the series based on a specific crystallographic generation mechanism which predicts the structures of these oxides and naturally classifies them in terms of the slab cycle. When including magnetic interactions, we show that the 1D chains have a symmetry protection against magnetic perturbations from the iron ions in the slabs, and that the slab size determines the type of magnetic order, which is either ferromagnetic or antiferromagnetic. Dynamical mean-field theory calculations reveal the orbitally selective Mott state of the Fe ions and tendency of conductivity to low-dimensional behavior with particular enhancement along the 1D chains. Across the series, the decoupling of the chains increases, and so with the inherent charge ordering of the slabs, these structures have the potential to allow experimental realization of the model system of coupled 1D wires. We point out the possibility to stabilize these compounds in the thin-film form that, together with a wide range of possible ionic substitutions and fact that these compounds are recoverable at ambient pressure, makes them a very promising platform to engineer physical systems with interesting magnetotransport phenomena, as corroborated by the recent discovery of quantum Hall effect in ZrTe$_5$.
2207.14111v1
2022-08-01
Sustainable steel through hydrogen plasma reduction of iron ore: process, kinetics, microstructure, chemistry
Fe- and steelmaking is the largest single industrial CO2 emitter, accounting for 6.5% of all CO2 emissions on the planet. This fact challenges the current technologies to achieve carbon-lean steel production and to align with the requirement of a drastic reduction of 80% in all CO2 emissions by around 2050. Thus, alternative reduction technologies have to be implemented for extracting iron from its ores. The H-based direct reduction has been explored as a sustainable route to mitigate CO2 emissions, where the reduction kinetics of the intermediate oxide product FexO wustite into Fe is the rate-limiting step of the process. The total reaction has an endothermic net energy balance. Reduction based on a H plasma may offer an attractive alternative. Here, we present a study about the reduction of hematite using H plasma. The evolution of both, chemical composition and phase transformations was investigated in several intermediate states. We found that hematite reduction kinetics depends on the balance between the initial input mass and the arc power. For an optimized input mass-arc power ratio, complete reduction was obtained within 15 min of exposure to the H plasma. The wustite reduction is also the rate-limiting step towards complete reduction. Nonetheless, the reduction reaction is exothermic, and its rates are comparable with those found in H-based direct reduction. Chemical and microstructure analysis revealed that the gangue elements partition to the remaining oxide regions, probed by energy dispersive spectroscopy and atom probe tomography. Si-enrichment was observed in the interdendritic fayalite domains, at the wustite/Fe hetero-interfaces and in the primarily solidified oxide particles inside the Fe. With proceeding reduction, however, such elements are gradually removed from the samples so that the final iron product is nearly free of gangue-related impurities.
2208.00661v1
2022-09-27
3D non-LTE iron abundances in FG-type dwarfs
Spectroscopic measurements of iron abundances are prone to systematic modelling errors. We present 3D non-LTE calculations across 32 STAGGER-grid models with effective temperatures from 5000 K to 6500 K, surface gravities of 4.0 dex and 4.5 dex, and metallicities from $-$3 dex to 0 dex, and study the effects on 171 Fe I and 12 Fe II optical lines. In warm metal-poor stars, the 3D non-LTE abundances are up to 0.5 dex larger than 1D LTE abundances inferred from Fe I lines of intermediate excitation potential. In contrast, the 3D non-LTE abundances can be 0.2 dex smaller in cool metal-poor stars when using Fe I lines of low excitation potential. The corresponding abundance differences between 3D non-LTE and 1D non-LTE are generally less severe but can still reach $\pm$0.2 dex. For Fe II lines the 3D abundances range from up to 0.15 dex larger, to 0.10 dex smaller, than 1D abundances, with negligible departures from 3D LTE except for the warmest stars at the lowest metallicities. The results were used to correct 1D LTE abundances of the Sun and Procyon (HD 61421), and of the metal-poor stars HD 84937 and HD 140283, using an interpolation routine based on neural networks. The 3D non-LTE models achieve an improved ionisation balance in all four stars. In the two metal-poor stars, they remove excitation imbalances that amount to 250 K to 300 K errors in effective temperature. For Procyon, the 3D non-LTE models suggest [Fe/H] = 0.11 $\pm$ 0.03, which is significantly larger than literature values based on simpler models. We make the 3D non-LTE interpolation routine for FG-type dwarfs publicly available, in addition to 1D non-LTE departure coefficients for standard MARCS models of FGKM-type dwarfs and giants. These tools, together with an extended 3D LTE grid for Fe II from 2019, can help improve the accuracy of stellar parameter and iron abundance determinations for late-type stars.
2209.13449v3
2022-10-24
High-precision abundances of first population stars in NGC 2808: confirmation of a metallicity spread
Photometric investigations have revealed that Galactic globular clusters exhibit internal metallicity variations amongst the so-called first-population stars, until now considered to have a homogeneous initial chemical composition. This is not fully supported by the sparse spectroscopic evidence, which so far gives conflicting results. Here, we present a high-resolution re-analysis of five stars in the Galactic globular cluster NGC 2808 taken from the literature. Target stars are bright red giants with nearly identical atmospheric parameters belonging to the first population according to their identification in the chromosome map of the cluster, and we have measured precise differential abundances for Fe, Si, Ca, Ti, and Ni to the ~0.03 dex level. Thanks to the very small uncertainties associated to the differential atmospheric parameters and abundance measurements, we find that target stars span a range of iron abundance equal to 0.25 +/- 0.06 dex. The individual elemental abundances are highly correlated with the position of the star along the extended sequence described by first population objects in the cluster chromosome map: bluer stars have a lower iron content. This agrees with inferences from the photometric analysis. The differential abundances for all other elements also show statistically significant ranges that point to intrinsic abundance spreads. The Si, Ca, Ti, and Ni variations are highly correlated with iron variations and the total abundance spreads for all elements are consistent within the error bars. This suggests a scenario in which short-lived massive stars exploding as supernovae contributed to the self-enrichment of the gas in the natal cloud while star formation was still ongoing.
2210.13369v1
2023-01-07
Changes in the distribution of circum-binary material around the HMXB GX 301-2 during a rapid spin-up episode of the neutron star
Some accretion powered X-ray pulsars with supergiant companion stars undergo occasional rapid spin-up episodes that last for weeks to a few months. We explore the changes in the accretion environment of the pulsar GX 301-2 during its latest 80 days long spin-up episode in 2019 when the spin frequency of the pulsar increased by ~2% over two orbits of the binary. By performing time-resolved spectroscopy with the MAXI/GSC spectra of the source, we estimated the equivalent hydrogen column density and equivalent width of the iron fluorescence line during the spin-up episode, and compared them with the long-term average values estimated by orbital-phase resolved spectroscopy. The measured absorption column density during the spin-up episode is about twice that of an average orbit, while the equivalent width of the iron line is less than half of an average orbit. Though the spin-up episode started immediately after a pre-periastron flare and lasted for the two consecutive orbits of the binary, the associated enhancement in luminosity started a few days after the pre-periastron flare and lasted only during the first orbit, and some enhancement was seen again during the pre-periastron passage of the second orbit. The absorption column density and iron line equivalent width vary throughout the spin-up episode and are distinct from an average orbit. These observations indicate a significant change in the accretion and reprocessing environment in GX 301-2 during the spin-up episode and may hold important clues for the phenomenon in this source and several other sources with supergiant companions.
2301.02815v1
2023-03-09
Saline bolus for negative contrast perfusion imaging in magnetic particle imaging
Objective. Magnetic Particle Imaging (MPI) is capable of high temporal resolution measurements of the spatial distribution of magnetic nanoparticles and therefore well suited for perfusion imaging, which is an important tool in medical diagnosis. Perfusion imaging in MPI usually requires a fresh bolus of tracer material to capture the key signal dynamics. Here, we propose a method to decouple the imaging sequence from the injection of additional tracer material, without further increasing the administered iron dose in the body with each image. Approach. A bolus of physiological saline solution without any particles (negative contrast) diminishes the steady-state concentration of a long-circulating tracer during passage. This depression in the measured concentration contributes to the required contrast dynamics. The presence of a long-circulating tracer is therefore a prerequisite to obtain the negative contrast. As a quantitative tracer based imaging method, the signal is linear in the tracer concentration for any location that contains nanoparticles and zero in the surrounding tissue which does not provide any intrinsic signal. After tracer injection, the concentration over time (positive contrast) can be utilized to calculate dynamic diagnostic parameters like perfusion parameters in vessels and organs. Every acquired perfusion image thus requires a new bolus of tracer with a sufficiently large iron dose to be visible above the background. Main results. Perfusion parameters are calculated based on the time response of the proposed negative bolus and compared to a positive bolus. Results from phantom experiments show that normalized signals from positive and negative boli are concurrent and deviations of calculated perfusion maps are low. Significance. Our method opens up the possibility to increase the total monitoring time, while minimizing the iron dose per acquired image.
2303.05439v2
2023-03-19
In-situ visualization of local distortions in the high-$T_c$ molecule-intercalated $Li_x(C_5H_5N)_yFe_{2-z}Se_2$ superconductor
A time-resolved synchrotron X-ray total scattering study sheds light on the evolution of the different structural length scales involved during the intercalation of the layered iron-selenide host by organic molecular donors, aiming at the formation of the expanded lattice $Li_x(C_5H_5N)_yFe_{2-z}Se_2$ hybrid superconductor. The intercalates are found to crystallize in the tetragonal $ThCr_2Si_2$-type structure at the average level, however, with an enhanced interlayer iron-selenide spacing (d= 16.2 \r{A}) that accommodates the heterocyclic molecular spacers. Quantitative atomic pair distribution function (PDF) analysis at variable times, suggests distorted $FeSe_4$ tetrahedral local environments that appear swollen with respect to those in the parent $\beta$-FeSe. Simultaneously acquired, in-situ synchrotron X-ray powder diffraction data disclose that secondary phases ($\alpha$-Fe and $Li_2Se$), grow significantly when higher Li-concentration is used in the solvothermal reaction or when the solution is aged. These observations are in line with the strongly reducing character of the intercalation medium's solvated electrons that mediate the defect chemistry of the expanded lattice superconductor. In the latter, intralayer correlated local distortions indicate electron donating aspects that reflect in somewhat enlarged Fe-Se bonds. They also reveal a degree of relief of chemical pressure associated with a large distance between Fe and Se sheets ('taller' anion height) and a stretched Fe-Fe square planar topology. The elongation of the latter, derived from the in-situ PDF study, speaks for a plausible increase in the Fe-site vacancy concentration. The evolution of the local structural parameters suggests an optimum reaction window where kinetically stabilized phases resemble the distortions of the edge-sharing Fe-Se tetrahedra, required for high-$T_c$ in expanded lattice iron-chalcogenides.
2303.10698v1