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1999-03-15
Metal-insulator transition in CMR materials
We report on resistivity measurements in La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ and Nd$_{0.7}$Sr$_{0.3}$MnO$_{3}$ thin films in order to elucidate the underlying mechanism for the CMR behavior. The experimental results are analyzed in terms of quantum phase transition ideas to study the nature of the metal-insulator transition in manganese oxides. Resistivity curves as functions of magnetization for various temperatures show the absence of scaling behavior expected in a continuous quantum phase transition, which leads us to conclude that the observed metal-insulator transition is most likely a finite temperature crossover phenomenon.
9903238v2
2000-01-06
Time Dependent Effects and Transport Evidence for Phase Separation in La_{0.5}Ca_{0.5}MnO_{3}
The ground state of La_{1-x}Ca_{x}MnO_{3} changes from a ferromagnetic metallic to an antiferromagnetic charge-ordered state as a function of Ca concentration at x ~ 0.50. We present evidence from transport measurements on a sample with x = 0.50 that the two phases can coexist, in agreement with other observations of phase separation in these materials. We also observe that, by applying and then removing a magnetic field to the mainly charge-ordered state at some temperatures, we can "magnetically anneal" the charge order, resulting in a higher zero-field resistivity. We also observe logarithmic time dependence in both resistivity and magnetization after a field sweep at low temperatures.
0001064v1
2000-02-14
Transition Temperature and Magnetoresistance in Double-Exchange Compounds with Moderate Disorder
We develop a variational mean-field theory of the ferromagnetic transition in compounds like Lanthanum-Manganite within the framework of the Double-Exchange Model supplemented by modest disorder. We obtain analytical expressions for the transition temperature, its variation with the valence electron-density and its decrease with disorder. We derive an expression for the conductivity for both the paramagnetic and the ferromangetic metallic phases, and study its dependence on the temperature and magnetic field. A simple relation between the resistivity in the ferromagnetic phase and the spontaneous magnetization is found. Our results are in a good agreement with the experimental data on transition temperatures and resistivity in the manganite compounds with relatively small disorder. We comment on the effects of increased disorder.
0002191v1
2000-03-11
Effect of γ-irradiation on superconducting transition temperature and resistive transition in polycrystalline YBa_{2}Cu_{3}O_(7-δ)
A bulk polycrystalline sample of YBa_(2)Cu_(3)O_(7-\delta) (\delta \approx 0.1) has been irradiated by \gamma-rays with ^{60}Co source. Non-monotonic behavior of T_{c} with increasing irradiation dose \Phi (up to 220 MR) is observed: T_{c} decreases at low doses (\Phi < 50 MR) from initial value (\approx 93 K) by about 2 K and then rises, forming a minimum. At higher doses (\Phi > 120 MR) T_{c} goes down again. The temperature width of resistive transition increases rather sharply with dose below 75 MR and drops somewhat at higher dose. The results observed are discussed, taking into account the granular structure of sample studied and the influence of \gamma-rays on intergrain Josephson coupling.
0003192v1
2000-06-07
Step-wise Behavior of Vortex-Lattice Melting Transition in Tilted Magnetic Fields in Single Crystals Bi2Sr2CaCu2O8+d
The vortex lattice melting transition in single crystals Bi2Sr2CaCu2O8+d was studied by the in-plane resistivity measurements in magnetic fields tilted away from the c-axis to the ab-plane. In order to avoid the surface barrier effect which hinders the melting transition in the conventional transport measurements, we used the Corbino geometry of electric contacts. For the first time, the complete Hc-Hab phase diagram of the melting-transition in Bi2Sr2CaCu2O8+d is obtained. The c-axis melting field component Hc-melt exhibits the novel, step-wise dependence on the in-plane magnetic fields Hab which is discussed on the base of the crossing vortex lattice structure. The sharp change of resistance behavior observed near the ab-plane suggests transformation from first-order to second-order phase transition.
0006095v1
2000-08-07
Large two-level magnetoresistance effect in doped manganite grain boundary junctions
We performed a systematic analysis of the tunneling magnetoresistance (TMR) effect in single grain boundary junctions formed in epitaxial La(2/3)Ca(1/3)MnO(3) films deposited on SrTiO(3) bicrystals. For magnetic fields H applied parallel to the grain boundary barrier, an ideal two-level resistance switching behavior with sharp transitions is observed with a TMR effect of up to 300% at 4.2 K and still above 100% at 77 K. Varying the angle between H and the grain boundary results in differently shaped resistance vs H curves. The observed behavior is explained within a model of magnetic domain pinning at the grain boundary interface.
0008105v1
2000-10-20
Composite Spin Waves, Quasi-Particles and Low Temperature resistivity in Double Exchange Systems
We make a quantum description of the electron low temperature properties of double exchange materials. In these systems there is a strong coupling between the core spin and the carriers spin. This large coupling makes the low energy spin waves to be a combination of ion and electron density spin waves. We study the form and dispersion of these composite spin wave excitations. We also analyze the spin up and down spectral functions of the temperature dependent quasi-particles of this system. Finally we obtain that the thermally activated composite spin waves renormalize the carriers effective mass and this gives rise to a low temperature resistivity scaling as T ^{5/2}.
0010312v1
2000-12-13
Phase-coherence transition in granular superconductors with $π$ junctions
We study the three-dimensional XY-spin glass as a model for the resistive behavior of granular superconductors containing a random distribution of $\pi$ junctions, as in high-$T_c$ superconducting materials with d-wave symmetry. The $\pi$ junctions leads to quenched in circulating currents (chiralities) and to a chiral-glass state at low temperatures, even in the absence of an external magnetic field. Dynamical simulations in the phase representation are used to determine the nonlinear current-voltage characteristics as a function of temperature. Based on dynamic scaling analysis, we find a phase-coherence transition at finite temperature below which the linear resistivity should vanish and determine the corresponding critical exponents. The results suggest that the phase and chiralities may order simultaneously for decreasing temperatures into a superconducting chiral-glass state.
0012238v1
2000-12-19
Resistance Spikes at Transitions between Quantum Hall Ferromagnets
We report a new manifestation of first-order magnetic transitions in two-dimensional electron systems. This phenomenon occurs in aluminum arsenide quantum wells with sufficiently low carrier densities and appears as a set of hysteretic spikes in the resistance of a sample placed in crossed parallel and perpendicular magnetic fields, each spike occurring at the transition between states with different partial magnetizations. Our experiments thus indicate that the presence of magnetic domains at the transition starkly increases dissipation, an effect also suspected in other ferromagnetic materials. Analysis of the positions of the transition spikes allows us to deduce the change in exchange-correlation energy across the magnetic transition, which in turn will help improve our understanding of metallic ferromagnetism.
0012367v1
2001-01-30
Stress-induced metallic behavior under magnetic field in Pr$_{1-x}$Ca$_{x}$MnO$_{3}$ (x = 0.5 and 0.4) thin films
We have investigated the role of the stress-induced by the presence of the substrate in thin films of colossal magnetoresistive manganites on structural, resistive and magnetic properties. Because of the strong coupling between the small structural distortions related to the charge-ordering (CO) and the resistive properties, the presence of the substrate prevents the full developpement of the charge ordering in Pr$_{0.5}$Ca$_{0.5}$MnO$_{3}$, especially in the very thin films. For thicker films, the CO state exists, but is not fully developped. Correlatively, the magnetic field which is necessary to suppress the CO is decreased drastically from 25 Tesla to about 5 Tesla on SrTiO$_{3}$ substrates. We have also investigated the influence of the doping level by studying the case of Pr$_{0.6}$Ca$_{0.4}$MnO$_{3}$.
0101448v1
2001-04-18
Electron Transport in Diborides: Observation of Superconductivity in ZrB2
We report on syntheses and electron transport properties of polycrystalline samples of diborides (AB2) with different transition metals atoms (A=Zr,Nb,Ta). The temperature dependence of resistivity, \rho(T), and ac susceptibility of these samples reveal superconducting transition of ZrB2 with Tc=5.5 K, while NbB2 and TaB2 have been observed nonsuperconducting up to 0.37 K. Hc2(T) is linear in temperature below Tc, leading to a rather low Hc2(0)= 0.1 T. At T close to Tc, Hc2(T) demonstrates a downward curvature. We conclude that these diborides as well as MgB2 samples behaves like a simple metals in the normal state with usual Bloch-Gr\"uneisen temperature dependence of resistivity and with Debye temperatures: 280 K, 460 K and 440 K, for ZrB2, NbB2 and MgB2, respectively, rather than T^2 and T^3 as previously reported for MgB2.
0104323v1
2001-05-02
In-plane Hall effect in c-axis-oriented MgB2 thin films
We have measured the longitudinal resistivity and the Hall resistivity in the ab-plane of highly c-axis-oriented MgB2 thin films. In the normal state, the Hall coefficient (R_H) behaves as R_H ~ T with increasing temperature (T) up to 130 K and then deviates from that linear T-dependence at higher temperatures. The T^2 dependence of the cotangent of the Hall angle is only observed above 130 K. The mixed-state Hall effect reveals no sign anomaly over a wide range of current densities from 10^2 to 10^4 A/cm^2 and for magnetic fields up to 5 T.
0105024v2
2001-05-04
A New Method of Probing the Phonon Mechanism in Superconductors including MgB$_{2}$
Weak localization has a strong influence on both the normal and superconducting properties of metals. In particular, since weak localization leads to the decoupling of electrons and phonons, the temperature dependence of resistance (i.e., $\lambda_{tr}$) is decreasing with increasing disorder, as manifested by Mooij's empirical rule. In addition, Testardi's universal correlation of $T_{c}$ (i.e., $\lambda$) and the resistance ratio (i.e., $\lambda_{tr}$) follows. This understanding provides a new means to probe the phonon mechanism in superconductors including MgB$_{2}$. The merits of this method are its applicability to any superconductors and its reliability because the McMillan's electron-phonon coupling constant $\lambda$ and $\lambda_{tr}$ change in a broad range, from finite values to zero, due to weak localization. Karkin et al's preliminary data of irradiated MgB$_{2}$ show the Testardi correlation, indicating that the dominant pairing mechanism in MgB$_{2}$ is the phonon-mediated interaction.
0105091v1
2002-01-25
Degradation of LaMnO{3-y} surface layer in LaMnO{3-y}/ metal interface
We report electrical measurements showing the degradation processes of LaMnO$_{3-y}$ (LaMnO) in LaMnO/normal metal interface in both point contact and planar-type junctions. Immediately after the preparation of the interface, the degradation process was followed by measuring the evolution of the junction resistance versus time. This process is characterized by the appearance of a second maximum in the resistance vs. temperature (R-T) dependence at temperatures lower than the Curie temperature T$_c$, at which the metal-insulator transition occurs in the bulk. These effects are explained in terms of the formation of a depleted interface layer in LaMnO caused by an out-diffusion of oxygen from the manganite surface to the normal metal. This assumption is confirmed by XPS measurement. Similar results on LaSrMnO$_{3-y}$ interfaces are also obtained.
0201460v1
2002-02-06
Thermoelectric properties of the brownmillerite oxide Ca_{2-y}La_yCo_{2-x}Al_xO_5
We prepared the brownmillerite oxide Ca_{2-y}La_yCo_{2-x}Al_xO_5, and found that it was an n-type conductor. The thermopower and the resistivity of the single crystal are -90 microV/K and 68 mOhm cm along the ab direction at 440 K, which suggest relatively good thermoelectrical properties, compared with other transition-metal oxides. Their temperature dependences are of activation type, and the activation energies are 0.2 eV for the resistivity and 0.04 eV for the thermopower. These energies differ by one order in magnitude, which implies that a polaron dominates the charge transport. A sign of the thermopower of the polycrystals changes from negative to positive at 500 K, indicating that holes are excited thermally to decrease the magnitude of thermopower.
0202087v1
2002-04-29
Concentration of Charge Carriers and Anomalous Gap Parameter in the Normal State of High-$T_c$ Superconductors
Fermi-Dirac statistics has been utilized by introducing the average ionization energy ($E_I$) as an additional anomalous energy gap in order to derive the two-dimensional concentration of charge carriers and the phenomenological resistivity model for the superconducting polycrystalline materials. The best fitted values of $E_I$ and the charge carriers' concentration ranges in the vicinity of 4 to 9 meV and 10$^{16}$ m$^{-2}$ respectively for the superconducting single crystal samples and polycrystalline compounds synthesized with various compositions via solid-state reactions. The phenomenological resistivity model is further redefined here based on the gapless nature of charge-carriers' dynamics within the Cu-O$_2$ planes that corresponds to anomalous Fermi liquid behavior, which is in accordance with the nested Fermi liquid theory.
0204601v1
2002-08-09
Quasi-one-dimensional superconductivity above 300 K and quantum phase slips in individual carbon nanotubes
A great number of the existing data for electrical transport, the Altshuler Aronov Spivak and Aharonov Bohm effects, as well as the tunneling spectra of individual carbon nanotubes can be well explained by theories of the quantum phase slips in quasi-one-dimensional superconductors. The existing data consistently suggest that the mean-field superconducting transition temperature T_{c0} in both single-walled and multi-walled carbon nanotubes could be higher than 600 K. The quantum phase slip theories naturally explain why the on-tube resistances in the closely packed nanotube bundles or in the individual multi-walled nanotubes with large diameters approach zero at room temperature, while a single tube with a small diameter has a substantial resistance.
0208198v4
2002-08-13
Characterization of one-dimensional quantum channels in InAs/AlSb
We report the magnetoresistance characteristics of one-dimensional electrons confined in a single InAs quantum well sandwiched between AlSb barriers. As a result of a novel nanofabrication scheme that utilizes a 3nm-shallow wet chemical etching to define the electrostatic lateral confinement, the system is found to possess three important properties: specular boundary scattering, a strong lateral confinement potential, and a conducting channel width that is approximately the lithography width. Ballistic transport phenomena, including the quenching of the Hall resistance, the last Hall plateau, and a strong negative bend resistance, are observed at 4K in cross junctions with sharp corners. In a ring geometry, we have observed Aharonov-Bohm interference that exhibits characteristics different from those of the GaAs counterpart due to the ballistic nature of electron transport and the narrowness of the conducting channel width.
0208265v1
2002-08-27
Anomalous Hall Effect of Calcium-doped Lanthanum Cobaltite Films
The Hall resistivity, magnetoresistance, and magnetization of La_{1-x}Ca_{x}CoO_{3} epitaxial films with x between 0.25 and 0.4 grown on lanthanum aluminate were measured in fields up to 7 T. The x=1/3 film, shows a reentrant metal insulator transition. Below 100 K, the x=1/3 and 0.4 films have significant coercivity which increases with decreasing temperature. At low temperature the Hall resistivity remains large and essentially field independent in these films, except for a sign change at the coercive field that is more abrupt than the switching of the magnetization. A unique magnetoresistance behavior accompanies this effect. These results are discussed in terms of a percolation picture and the mixed spin state model for this system. We propose that the low-temperature Hall effect is caused by spin-polarized carriers scattering off of orbital disorder in the spin-ordered clusters.
0208530v1
2003-01-24
Semiconductive and Photoconductive Properties of the Single Molecule Magnets Mn$_{12}$-Acetate and Fe$_8$Br$_8$
Resistivity measurements are reported for single crystals of Mn$_{12}$-Acetate and Fe$_8$Br$_8$. Both materials exhibit a semiconductor-like, thermally activated behavior over the 200-300 K range. The activation energy, $E_a$, obtained for Mn$_{12}$-Acetate was 0.37 $\pm$ 0.05 eV, which is to be contrasted with the value of 0.55 eV deduced from the earlier reported absorption edge measurements and the range of 0.3-1 eV from intramolecular density of states calculations, assuming $2E_a$= $E_g$, the optical band gap. For Fe$_8$Br$_8$, $E_a$ was measured as 0.73 $\pm$ 0.1 eV, and is discussed in light of the available approximate band structure calculations. Some plausible pathways are indicated based on the crystal structures of both lattices. For Mn$_{12}$-Acetate, we also measured photoconductivity in the visible range; the conductivity increased by a factor of about eight on increasing the photon energy from 632.8 nm (red) to 488 nm (blue). X-ray irradiation increased the resistivity, but $E_a$ was insensitive to exposure.
0301497v1
2003-02-12
Avoided Antiferromagnetic Order and Quantum Critical Point in CeCoIn$_5$
We measured specific heat and resistivity of heavy fermion CeCoIn5 between the superconducting critical field $H_{c2} = 5 T$ and 9 T, with field in the [001] direction, and at temperatures down to 50mK. At 5T the data show Non Fermi Liquid behavior down to the lowest temperatures. At field above 8T the data exhibit crossover from the Fermi liquid to a Non Fermi Liquid behavior. We analyzed the scaling properties of the specific heat, and compared both resistivity and the specific heat with the predictions of a spin-fluctuation theory. Our analysis leads us to suggest that the NFL behavior is due to incipient antiferromagnetism (AF) in CeCoIn5, with the quantum critical point in the vicinity of the $H_{c2}$. Below $H_{c2}$ the AF phase which competes with the paramagnetic ground state is superseded by the superconducting transition.
0302226v1
2003-02-21
Anomalous Hall Effect and Magnetoresistance of SrFe1-xCoxO3-d
Transport and magnetic studies on polycrystalline samples of SrFe1-xCoxO3-d have been carried out to investigate the relationship between the magnetic structure and the anomalous Hall resistivity rH. The hysteretic behavior of the magnetization observed in the measurements with varying temperature T up and then down after zero field cooling indicates that the system has the reentrant spin-glass phase, which is supported by the increasing width of the magnetic reflections observed by neutron diffraction with decreasing T below the Curie temperature TC. Detailed analyses of the observed Hall resistivity rH indicate that the anomalous Hall coefficient exhibits unusual behavior in the reentrant spin-glass phase. The magnetic field (H)- and T-dependence of the magnetoresistance of the present system can be understood by a spin dependent tunneling model.
0302436v1
2003-02-24
Spin-wave scattering at low temperatures in manganite films
The temperature $T$ and magnetic field $H$ dependence of the resistivity $\rho$ has been measured for La$_{0.8-y}$Sr$_{0.2}$MnO$_{3}$ (y=0 and 0.128) films grown on (100) SrTiO$_{3}$ substrates. The low-temperature $\rho$ in the ferromagnetic metallic region follows well $\rho (H,T)=\rho _{0}(H)+A(H)\omega_{s}/\sinh (\hbar \omega_{s}/2k_{B}T)+B(H)T^{7/2}$ with $\rho _{0}$ being the residual resistivity. We attribute the second and third term to small-polaron and spin-wave scattering, respectively. Our analysis based on these scattering mechanisms also gives the observed difference between the metal-insulator transition temperatures of the films studied. Transport measurements in applied magnetic field further indicate that spin-wave scattering is a key transport mechanism at low temperatures.
0302486v1
2003-04-07
Thickness dependence of the properties of epitaxial MgB2 thin films grown by hybrid physical-chemical vapor deposition
We have studied the effect of deposition rate and layer thickness on the properties of epitaxial MgB2 thin films grown by hybrid physical-chemical vapor deposition on 4H-SiC substrates. The MgB2 film deposition rate depends linearly on the concentration of B2H6 in the inlet gas mixture. We found that the superconducting and normal-state properties of the MgB2 films are determined by the film thickness, not by the deposition rate. When the film thickness was increased, the transition temperature, Tc, increased and the residual resistivity, rho0, decreased. Above about 300 nm, a Tc of 41.8 K, a rho0 of 0.28 mikroOhm.cm, and a residual resistance ratio RRR of over 30 were obtained. These values represent the best MgB2 properties reported thus far.
0304164v1
2003-06-05
Variable-range-hopping conductivity of half-doped bilayer manganite LaSr$_{2}$Mn$_{2}$O$_{7}$
We report measurements of in-plane $\rho_{ab}$ and out-of-plane $\rho_{c}$ resistivities on a single crystal of the half-doped bilayer manganite LaSr$_{2}$Mn$_{2}$O$_{7}$. In the temperature $T$ range 220 to 300 K, the resistive anisotropy $\rho_{c}/\rho_{ab}=A+B/T$ ($A$ and $B$ constants), which provides evidence for the variable-range-hopping conduction in the presence of a Coulomb gap. This hopping mechanism also accounts for the quadratic magnetic field $H$ and $\sin^{2}\phi$ dependences of the negative magnetoresistivity $\ln [\rho_{i}(T,H,\phi)/\rho_{i}(T,H=0)]$ ($i=ab,c$), where $\phi$ is the in-plane angle between the magnetic field and the current.
0306133v1
2003-06-11
Enhanced electrical resistivity before Néel order in the metals, RCuAs$_2$ (R= Sm, Gd, Tb and Dy
We report an unusual temperature (T) dependent electrical resistivity($\rho$) behavior in a class of ternary intermetallic compounds of the type RCuAs$_2$ (R= Rare-earths). For some rare-earths (Sm, Gd, Tb and Dy) with negligible 4f-hybridization, there is a pronounced minimum in $\rho$(T) far above respective N\'eel temperatures (T$_N$). However, for the rare-earths which are more prone to exhibit such a $\rho$(T) minimum due to 4f-covalent mixing and the Kondo effect, this minimum is depressed. These findings, difficult to explain within the hither-to-known concepts, present an interesting scenario in magnetism.
0306266v1
2003-07-14
Interplay between disorder, quantum and thermal fluctuations in ferromagnetic alloys: The case of UCu2Si(2-x)Ge(x)
We consider, theoretically and experimentally, the effects of structural disorder, quantum and thermal fluctuations in the magnetic and transport properties of certain ferromagnetic alloys.We study the particular case of UCu2Si(2-x)Ge(x). The low temperature resistivity, rho(T,x), exhibits Fermi liquid (FL) behavior as a function of temperature T for all values of x, which can be interpreted as a result of the magnetic scattering of the conduction electrons from the localized U spins. The residual resistivity, rho(0,x), follows the behavior of a disordered binary alloy. The observed non-monotonic dependence of the Curie temperature, Tc(x), with x can be explained within a model of localized spins interacting with an electronic bath whose transport properties cross-over from ballistic to diffusive regimes. Our results clearly show that the Curie temperature of certain alloys can be enhanced due to the interplay between quantum and thermal fluctuations with disorder.
0307328v2
2003-10-20
Studies of Current-Driven Excitations in Co/Cu/Co Trilayer Nanopillars
We measure the dynamic resistance of a Co/Cu/Co trilayer nanopillar at varied magnetic field $H$ and current $I$. The resistance displays the usual behavior, almost symmetric in $H$, both when magnetization switching is hysteretic at small $I,H$, and reversible at larger $I,H$. We show differences in the $I,H$ magnetization stability diagram measured by holding $I$ fixed and varying $H$ and vice versa. We also show how the peak in $dV/dI$ associated with telegraph noise in the reversible switching regime, is calculated from the telegraph noise variations with $I$. Lastly, we show data for a similar sample that displays behavior asymmetric in $H$, and a negative reversible switching peak instead of a usual positive one.
0310472v1
2003-11-17
The Normal State Resistivity of Grain Boundaries in YBa2Cu3O7-delta
Using an optimized bridge geometry we have been able to make accurate measurements of the properties of YBa2Cu3O7-delta grain boundaries above Tc. The results show a strong dependence of the change of resistance with temperature on grain boundary angle. Analysis of our results in the context of band-bending allows us to estimate the height of the potential barrier present at the grain boundary interface.
0311386v1
2004-02-09
Molecular electronics exploiting sharp structure in the electrode density-of-states. Negative differential resistance and Resonant Tunneling in a poled molecular layer on Al/LiF electrodes
Density-functional calculations are used to clarify the role of an ultrathin LiF layer on Al electrodes used in molecular electronics. The LiF layer creates a sharp density of states (DOS), as in a scanning-tunneling microscope (STM) tip. The sharp DOS, coupled with the DOS of the molecule leads to negative differential resistance (NDR). Electron transfer between oriented molecules occurs via resonant tunneling. The I-V characteristic for a thin-film of tris (8-hydroxyquinoline)- aluminum (AlQ) molecules, oriented using electric-field poling, and sandwiched between two Al/LiF electrodes is in excellent agreement with theory. This molecular device presents a new paradigm for a convenient, robust, inexpensive alternative to STM or mechanical break-junction structures.
0402257v1
2004-05-06
The antiferromagnetic transition of UPd2Al3 break-junctions: A new realization of N-shaped current-voltage characteristics
We have investigated metallic break junctions of the heavy-fermion compound UPd2Al3 at low temperatures between 0.1K and 9K and in magnetic fields up to 8T. Both the current-voltage I(V) characteristics and the dV/dI (V) spectra clearly showed the superconducting ($T_{\rm c}\simeq$ 1.8K) as well as the antiferromagnetic ($T_{\rm N}\simeq$14K) transition at low temperatures when the bias voltage is raised. The junctions with lateral size of order 200nm had huge critical current densities around $5\times 10^{10} A/m^2 at the antiferromagnetic transition and hysteretic I(V) characteristics. Degrading the quality of the contacts by in situ increasing the local residual resistivity reduced the hysteresis. We show that those hysteretic I(V) curves can be reproduced theoretically by assuming the constriction to be in the thermal regime. It turns out that these point contacts represent non-linear devices with N-shaped I(V) characteristics that have a negative differential resistance like an Esaki tunnel diode.
0405118v1
2004-05-11
Weak links and phase slip centers in superconducting MgB2 wires
MgB2 superconducting wires were produced by the Mg diffusion method. Scanning electron microscopy (SEM), optical microscopy, dispersive x-ray analysis (EDS) and XRD diffraction were used to study the physical structure and content of the wires. Magnetic properties (Tcm, Hc1, Hc2, Jc by the Bean model) were obtained with a SQUID magnetometer, and transport properties (Tcr, Hc2, resistivity and residual resistivity ratio) were measured using a standard four-lead configuration. The V-I characteristics of the wires close to the critical temperature showed a staircase response, which was attributed to the presence of weak links, creating phase slip centers. The origin of those weak links is discussed in relation to their formation and structure.
0405219v1
2004-05-27
Magnetic, electrical resistivity, heat-capacity and thermopower anomalies in CeCuAs2
The results of magnetic susceptibility, electrical resistivity ($\rho$), heat-capacity (C) and thermopower (S) measurements on CeCuAs2, forming in ZrCuSi2-type tetragonal structure, are reported. Our investigations reveal that Ce is trivalent and there is no clear evidence for long range magnetic ordering down to 45 mK. The $\rho$ behavior is notable in the sense that (i) the temperature (T)-coefficient of $\rho$ is negative in the entire range of measurement (45 mK to 300 K) with large values of $\rho$, while S behavior is typical of metallic Kondo lattices, and (ii) $\rho$ is proportional to T-0.6 at low temperatures, without any influence on the exponent by the application of a magnetic field, which does not seem to classify this compound into hither-to-known non-Fermi liquid (NFL) systems. In contrast to the logarithmic increase known for NFL systems, C/T measured down to 0.5 K exhibits a fall below 2 K. The observed properties of this compound are unusual among Ce systems.
0405638v1
2004-06-24
On Electron Transport in ZrB12, ZrB2 and MgB2
We report on measurements of the temperature dependence of resistivity, $\rho(T)$, for single crystal samples of ZrB$_{12}$, ZrB$_{2}$ and polycrystalline samples of MgB$_{2}$. It is shown that cluster compound ZrB$_{12}$ behaves like a simple metal in the normal state, with a typical Bloch -- Gr\"uneisen $\rho(T)$ dependence. However, the resistive Debye temperature, $T_{R}=300 K$, is three times smaller than $T_{D}$ obtained from specific heat data. We observe the $T^{2}$ term in $\rho(T)$ of these borides, which could be interpreted as an indication of strong electron-electron interaction. Although the $\rho (T)$ dependence of ZrB$_{12}$ reveals a sharp superconductive transition at $T_{c}=6.0 K$, no superconductivity was observed for single crystal samples of ZrB$_{2}$ down to $1.3 K$.
0406615v1
2004-07-07
Kondo Behavior of U in CaB$_6$
Replacing U for Ca in semiconducting CaB$_6$ at the few at.% level induces metallic behaviour and Kondo-type phenomena at low temperatures, a rather unusual feature for U impurities in metallic hosts. For Ca$_{0.992}$U$_{0.008}$B$_6$, the resistance minimum occurs at $T$ = 17 K. The subsequent characteristic logarithmic increase of the resistivity with decreasing temperature merges into the expected $T^2$ dependence below 0.8 K. Data of the low-temperature specific heat and the magnetization are analyzed by employing a simple resonance-level model. Analogous measurements on LaB$_6$ with a small amount of U revealed no traces of Kondo behavior, above 0.4 K.
0407158v1
2004-08-11
Conductivity, weak ferromagnetism and charge instability in $α-MnS$ single crystal
The temperature dependence of resistivity, magnetization and electron-spin resonance of the $\alpha- MnS $ single crystal were measured in temperature range of $5 K < T < 550 K$. Magnetization hysteresis in applied magnetic field up to 0.7 T at $T=5 K, 77 K, 300 K$, irreversible temperature behavior of magnetization and resistivity were found . The obtained data were explained in terms of degenerate tight binding model using random phase approximation. The contribution of holes in $t_{2g}$ and $e_g$ bands of manganese ions to the conductivity, optical absorbtion spectra and charge instability in $\alpha -MnS $ were studied. Charge susceptibility maxima resulted from the competition of the on-site Coulomb interaction between the holes in different orbitals and small hybridization of sub-bands were calculated at $T=160 K, 250 K, 475 K$.
0408232v1
2004-08-26
Deviations from plastic barriers in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ thin films
Resistive transitions of an epitaxial Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ thin film were measured in various magnetic fields ($H\parallel c$), ranging from 0 to 22.0 T. Rounded curvatures of low resistivity tails are observed in Arrhenius plot and considered to relate to deviations from plastic barriers. In order to characterize these deviations, an empirical barrier form is developed, which is found to be in good agreement with experimental data and coincide with the plastic barrier form in a limited magnetic field range. Using the plastic barrier predictions and the empirical barrier form, we successfully explain the observed deviations.
0408555v2
2004-08-27
Examination of the c-axis resistivity of Bi_{2}Sr_{2-x}La_xCuO_{6+δ} in magnetic fields up to 58 T
We measure the magnetic-field dependence of the c-axis resistivity, \rho_c(H), in a series of Bi_{2}Sr_{2-x}La_xCuO_{6+\delta} (BSLCO) single crystals for a wide range of doping using pulsed magnetic fields up to 58 T. The behavior of \rho_c(H) is examined in light of the recent determination of the upper critical field H_{c2} for this material using Nernst effect measurements. We find that the peak in \rho_c(H) shows up at a field H_p that is much lower than H_{c2} and there is no discernable feature in \rho_c(H) at H_{c2}. Intriguingly, H_p shows a doping dependence similar to that of T_c, and there is an approximate relation k_{B}T_c \simeq {1/2}g\mu_{B}H_p. Moreover, we show that the data for the lowest-T_c sample can be used to estimate the pseudogap closing field H_{pg}, but the method to estimate H_{pg} proposed by Shibauchi {\it et al.} [Phys. Rev. Lett. {\bf 86}, 5763 (2001)] must be modified to apply to the BSLCO system.
0408603v1
2004-10-06
Ballistic resistivity in aluminum nanocontacts
One of the major industrial challenges is to profit from some fascinating physical features present at the nanoscale. The production of dissipationless nanoswitches (or nanocontacts) is one of such attractive applications. Nevertheless, the lack of knowledge of the real efficiency of electronic ballistic/non dissipative transport limits future innovations. For multi-valent metallic nanosystems -where several transport channels per atom are involved- the only experimental technique available for statistical transport characterization is the conductance histogram. Unfortunately its interpretation is difficult because transport and mechanical properties are intrinsically interlaced. We perform a representative series of semiclassical molecular dynamics simulations of aluminum nanocontact breakages, coupled to full quantum conductance calculations, and put in evidence a linear relationship between the conductance and the contact minimum cross-section for the geometrically favored aluminum nanocontact configurations. Valid in a broad range of conductance values, such relation allows the definition of a transport parameter for nanomaterials, that represents the novel concept of ballistic resistivity.
0410138v1
2004-12-01
Magnetoresistive Effects in Ferromagnet-Superconductor Multilayers
We consider a nanoscale system consisting of Manganite-ferromagnet and Cuprate-superconductor multilayers in a spin valve configuration. The magnetization of the bottom Manganite-ferromagnet is pinned by a Manganite-antiferromagnet. The magnetization of the top Manganite-ferromagnet is coupled to the bottom one via indirect exchange through the superconducting layers. We study the behavior of the critical temperature and the magnetoresistance as a function of an externally applied parallel magnetic field, when the number of Cuprate-superconductor layers are changed. There are two typical behaviors in the case of a few monolayers of the Cuprates: a) For small magnetic fields, the critical temperature and the magnetoresistance change abruptly when the flipping field of the top Manganite-ferromagnet is reached. b) For large magnetic fields, the multilayered system re-enters the zero-resistance (superconducting) state after having become resistive (normal).
0412005v1
2004-12-12
Effect of oxygen content on the transport properties and magnetoresistance in [Ca$_{2}$CoO$_{3-δ}$]$_{0.62}$[CoO$_{2}$] single crystals
Transport property is investigated in [Ca$_{2}$CoO$_{3-\delta}$]$_{0.62}$[CoO$_{2}$] single crystals obtained by varying annealing conditions. The $\rho_{ab}(T)$ exhibits a resistivity minimum, and the temperature corresponding to this minimum increases with the loss of oxygen content, indicative of the enhancement of spin density wave (SDW). Large negative magnetoresistance (MR) was observed in all single crystals [Ca$_{2}$CoO$_{3-\delta}$]$_{0.62}$[CoO$_{2}$], while a magnetic-field-driven insulator-to-metal (IM) transition in oxygen annealed samples. These results suggest a ferromagnetic correlation in system enhanced by oxygen content. In addition, a low temperature thermal activation resistivity induced by fields was observed in single crystals annealed in oxygen atmosphere.
0412298v1
2004-12-27
Ferromagnetism and possible heavy fermion behavior in single crystals of NdOs$_4$Sb$_{12}$
Single crystals of the filled-skutterudite compound NdOs$_4$Sb$_{12}$ have been investigated by means of electrical resistivity, magnetization, and specific heat measurements. The NdOs$_4$Sb$_{12}$ crystals have the LaFe$_4$P$_{12}$-type cubic structure with a lattice parameter of 9.3 \AA. Possible heavy-fermion behavior is inferred from specific heat measurements, which reveal a large electronic specific heat coefficient $\gamma \approx 520$ mJ/mol-K$^2$, corresponding to an effective mass $m^* \sim$ 98 $m_e$. Features related to a ferromagnetic transition at {$\sim$ 0.9 K} can be observed in electrical resistivity, magnetization and specific heat. Conventional Arrott-plot analysis indicates that NdOs$_4$Sb$_{12}$ conforms to mean-field ferromagnetism.
0412713v3
2005-02-03
Transverse "resistance overshoot" in a Si/SiGe two-dimensional electron gas in the quantum Hall effect regime
We investigate the peculiarities of the "overshoot" phenomena in the transverse Hall resistance R_{xy} in Si/SiGe. Near the low magnetic field end of the quantum Hall effect plateaus, when the filling factor \nu approaches an integer i, R_{xy} overshoots the normal plateau value h/ie^2. However, if magnetic field B increases further, R_{xy} decreases to its normal value. It is shown that in the investigated sample n-Si/Si_{0.7}Ge_{0.3}, overshoots exist for almost all \nu. Existence of overshoot in R_{xy} observed in different materials and for different \nu, where splitting of the adjacent Landau bands has different character, hints at the common origin of this effect. Comparison of the experimental curves R_{xy}(\nu) for \nu = 3 and \nu = 5 with and without overshoot showed that this effect exist in the whole interval between plateaus, not only in the region where R_{xy} exceeds the normal plateau value.
0502094v1
2005-03-03
Transport properties of diluted magnetic semiconductors: Dynamical mean field theory and Boltzmann theory
The transport properties of diluted magnetic semiconductors (DMS) are calculated using dynamical mean field theory (DMFT) and Boltzmann transport theory. Within DMFT we study the density of states and the dc-resistivity, which are strongly parameter dependent such as temperature, doping, density of the carriers, and the strength of the carrier-local impurity spin exchange coupling. Characteristic qualitative features are found distinguishing weak, intermediate, and strong carrier-spin coupling and allowing quantitative determination of important parameters defining the underlying ferromagnetic mechanism. We find that spin-disorder scattering, formation of bound state, and the population of the minority spin band are all operational in DMFT in different parameter range. We also develop a complementary Boltzmann transport theory for scattering by screened ionized impurities. The difference in the screening properties between paramagnetic ($T>T_c$) and ferromagnetic ($T<T_c$) states gives rise to the temperature dependence (increase or decrease) of resistivity, depending on the carrier density, as the system goes from the paramagnetic phase to the ferromagnetic phase. The metallic behavior below $T_c$ for optimally doped DMS samples can be explained in the Boltzmann theory by temperature dependent screening and thermal change of carrier spin polarization.
0503077v1
2005-04-22
Blue light-emitting diode based on ZnO
A near-band-edge bluish electroluminescence (EL) band centered at around 440 nm was observed from ZnO p-i-n homojunction diodes through a semi-transparent electrode deposited on the p-type ZnO top layer. The EL peak energy coincided with the photoluminescence peak energy of an equivalent p-type ZnO layer, indicating that the electron injection from the n-type layer to the p-type layer dominates the current, giving rise to the radiative recombination in the p-type layer. The imbalance in charge injection is considered to originate from the lower majority carrier concentration in the p-type layer, which is one or two orders of magnitude lower than that in the n-type one. The current-voltage characteristics showed the presence of series resistance of several hundreds ohms, corresponding to the current spread resistance within the bottom n-type ZnO. The employment of conducting ZnO substrates may solve the latter problem.
0504587v1
2005-05-17
Transport properties of moderately disordered UCu$_4$Pd
We present a detailed study on the (magneto)transport properties of as-cast and heat treated material UCu$_4$Pd. We find a pronounced sample dependence of the resistivity $\rho$ of as-cast samples, and reproduce the annealing dependence of $\rho$. In our study of the Hall effect we determine a metallic carrier density for all samples, and a temperature dependence of the Hall constant which is inconsistent with the Skew scattering prediction. The magnetoresistive response is very small and characteristic for spin disorder scattering, suggesting that overall the resistivity is controlled mostly by nonmagnetic scattering processes. We discuss possible sources for the temperature and field dependence of the transport properties, in particular with respect to quantum criticality and electronic localization effects.
0505418v1
2005-07-02
Drastic ground state changes induced by Ni substitution in NaxCoO2
We report on the effect of Ni substitution at the Co site on the physical properties of NaxCoO2 system by investigating the series NaxCo1-yNiyO2 (x=0.75, 0<y<0.15). An upturn in the resistivity is observed in all Ni substituted samples as the temperature is lowered, suggestive of the occurrence of a Metal-Insulator Transition (MIT). The temperature at which this transition occurs increases with Ni content. The temperature dependence of the resistivity in the metallic region in the Ni substituted samples shows a T2 dependence, which is qualitatively different from that observed in the pristine sample. The evolution of the Fano asymmetry parameter, extracted by analyzing the lineshape of the IR active in-plane Co-O mode, both as a function of Ni concentration and temperature corroborates the occurrence of the MIT. It is argued that the progressive substitution of the Co4+ ions with Ni increases the probability of double occupancy and therefore the on-site Coulomb interaction energy leading to a shift in the thermodynamically driven MIT to higher temperatures.
0507045v1
2005-08-19
Determination of the intrinsic anomalous Hall effect of SrRuO$_3$
The anomalous Hall effect (AHE) of epitaxial SrRuO$_3$ films with varying lattice parameters is investigated, and analyzed according to the Berry-phase scenario. SrRuO$_3$ thin films were deposited on SrTiO$_3$ substrates directly, or using intermediate buffer layers, in order to finely control the epitaxial strain. The AHE of the different films exhibits intrinsic features such as the sign change of the Hall resistivity with the temperature, even for small thicknesses of SrRuO$_3$. However, the anomalous Hall conductivity is greatly reduced from its intrinsic value as the carrier scattering is increased when the epitaxial strain is released. We argue that the AHE of fully strained SrRuO$_3$ film with low residual resistivity represents the intrinsic AHE of SrRuO$_3$.
0508443v1
2005-09-05
Magnetic and electronic transport percolation in epitaxial GeMn films
Electronic transport and magnetic properties of Ge1-xMnx/Ge(100) films are investigated as a function of Mn dilution. Depending on x, characteristic temperatures separate different regimes in both properties. Resistivity exhibits an insulator-like behavior in the whole temperature range and, below about 80 K, two distinct activation energies are observed. At a higher temperature value, TR, resistivity experiences a sudden reduction. Hall coefficient shows a strong contribution from the anomalous Hall effect and, at TR, a sign inversion, from positive to negative, is recorded. The magnetic properties, inferred from magneto-optical Kerr effect, evidence a progressive decrease of the ferromagnetic long range order as the temperature is raised, with a Curie temperature TC not far from TR. The transport and magnetic results are qualitatively consistent with a percolation mechanism due to bound magnetic polarons in a GeMn diluted magnetic semiconductor, with localized holes [A. Kaminski and S. Das Sarma, Phys. Rev. B 68, 235210 (2003)].
0509111v1
2005-10-07
Size Dependent Breakdown of Superconductivity in Ultranarrow Nanowires
Below a certain temperature Tc (typically cryogenic), some materials lose their electric resistance R entering a superconducting state. Folowing the general trend toward a large scale integration of a greater number of electronic components, it is desirable to use superconducting elements in order to minimize heat dissipation. It is expected that the basic property of a superconductor, i.e. dissipationless electric current, will be preserved at reduced scales required by modern nanoelectronics. Unfortunately, there are indications that for a certain critical size limit of the order of 10 nm, below which a "superconducting" wire is no longer a superconductor in a sense that it acquires a finite resistance even at temperatures close to absolute zero. In the present paper we report an experimental evidence for a superconductivity breakdown in ultranarrow quasi-1D aluminum nanowires.
0510181v1
2005-10-07
Evidence of ratchet effect in nanowires of a conducting polymer
Ratchet effect, observed in many systems starting from living organism to artificially designed device, is a manifestation of motion in asymmetric potential. Here we report results of a conductivity study of Polypyrrole nanowires, which have been prepared by a simple method to generate a variation of doping concentration along the length. This variation gives rise to an asymmetric potential profile that hinders the symmetry of the hopping process of charges and hence the value of measured resistance of these nanowires become sensitive to the direction of current flow. The asymmetry in resistance was found to increase with decreasing nanowire diameter and increasing temperature. The observed phenomena could be explained with the assumption that the spatial extension of localized state involved in hopping process reduces as the doping concentration reduces along the length of the nanowires.
0510188v1
2005-10-11
Highly oriented VO2 thin films prepared by sol-gel deposition method
Highly oriented VO2 thin films were grown on sapphire substrates by the sol-gel method that includes a low pressure annealing in an oxygen atmosphere. This reduction process effectively promotes the formation of the VO2 phase over a relatively wide range of pressures below 100 mTorr and temperatures above 400oC. X-ray diffraction analysis showed that as-deposited films crystallize directly to the VO2 phase without passing through intermediate phases. VO2 films have been found to be with [100]- and [010]-preferred orientations on Al2O3(1012) and Al2O3(1010) substrates, respectively. Both films undergo a metal-insulator transition with an abrupt change in resistance, with different transition behaviors observed for the differently oriented films. For the [010]-oriented VO2 films a larger change in resistance of 1.2x10^4 and a lower transition temperature are found compared to the values obtained for the [100]-oriented films.
0510267v2
2005-11-10
Thermoelectric properties of the layered Pd oxide R_2PdO_4 (R = La, Nd, Sm and Gd)
We prepared polycrystalline samples of R$_2$PdO$_4$ (R = La, Nd, Sm and Gd) using a NaCl-flux technique. The measured resistivity is of the order of 10$^3-10^4$ $\Omega$cm at room temperature, which is two orders of magnitude smaller than the values reported so far. We further studied the substitution effects of Ce for Nd in Nd$_{1.9}$Ce$_{0.1}$PdO$_4$, where the substituted Ce decreases the resistivity and the magnitude of the thermopower. The activation energy gap of 70-80 meV and the effective mass of 15 evaluated from the measured data are suitable for thermoelectric materials, but the mobility of 10$^{-6}$ cm$^2$/Vs is much lower than a typical value of 1-10 cm$^2$/Vs for other thermoelectric oxides.
0511245v1
2005-11-10
Anderson localization in carbon nanotubes: defect density and temperature effects
The role of irradiation induced defects and temperature in the conducting properties of single-walled (10,10) carbon nanotubes has been analyzed by means of a first-principles approach. We find that di-vacancies modify strongly the energy dependence of the differential conductance, reducing also the number of contributing channels from two (ideal) to one. A small number of di-vacancies (5-9) brings up strong Anderson localization effects and a seemly universal curve for the resistance as a function of the number of defects. It is also shown that low temperatures, around 15-65 K, are enough to smooth out the fluctuations of the conductance without destroying the exponential dependence of the resistivity as a function of the tube length.
0511265v1
2005-11-17
Electrical Switching in Metallic Carbon Nanotubes
We present first-principles calculations of quantum transport which show that the resistance of metallic carbon nanotubes can be changed dramatically with homogeneous transverse electric fields if the nanotubes have impurities or defects. The change of the resistance is predicted to range over more than two orders of magnitude with experimentally attainable electric fields. This novel property has its origin that backscattering of conduction electrons by impurities or defects in the nanotubes is strongly dependent on the strength and/or direction of the applied electric fields. We expect this property to open a path to new device applications of metallic carbon nanotubes.
0511447v1
2005-11-28
Laser microscopy of tunneling magnetoresistance in manganite grain-boundary junctions
Using low-temperature scanning laser microscopy we directly image electric transport in a magnetoresistive element, a manganite thin film intersected by a grain boundary (GB). Imaging at variable temperature allows reconstruction and comparison of the local resistance vs temperature for both, the manganite film and the GB. Imaging at low temperature also shows that the GB switches between different resistive states due to the formation and growth of magnetic domains along the GB. We observe different types of domain wall growth; in most cases a domain wall nucleates at one edge of the bridge and then proceeds towards the other edge.
0511662v1
2006-03-16
Coordinate transformation in the model of long Josephson junctions: geometrically equivalent Josephson junctions
The transition from the model of a long Josephson junction of variable width to the model of a junction with a coordinate-dependent Josephson current amplitude is effected through a coordinate transformation. This establishes the correspondence between the classes of Josephson junctions of variable width and quasi-one-dimensional junctions with a variable thickness of the barrier layer. It is shown that for a junction of exponentially varying width the barrier layer of the equivalent quasi-one-dimensional junction has a distributed resistive inhomogeneity that acts as an attractor for magnetic flux vortices. The curve of the critical current versus magnetic field for a Josephson junction with a resistive microinhomogeneity is constructed with the aid of a numerical simulation, and a comparison is made with the critical curve of a junction of exponentially varying width. The possibility of replacing a distributed inhomogeneity in a Josephson junction by a local inhomogeneity at the end of the junction is thereby demonstrated; this can have certain advantages from a technological point of view.
0603439v1
2006-03-28
Depolarizing-Field Effect in Strained Nanoscale Ferroelectric Capacitors and Tunnel Junctions
The influence of depolarizing field on the magnitude and stability of a uniform polarization in ferroelectric capacitors and tunnel junctions is studied using a nonlinear thermodynamic theory. It is predicted that, in heterostructures involving strained epitaxial films and metal electrodes, the homogeneous polarization state may remain stable against transformations into the paraelectric phase and into polydomain states down to the nanoscale. This result supports the possibility of depolarizing-field-related resistive switching in ferroelectric tunnel junctions with dissimilar electrodes. The resistance on/off ratio in such junctions is shown to be governed by the difference between the reciprocal capacitances of screening space charges in the electrodes.
0603762v2
2006-03-31
Mechanism and Scalability in Resistive Switching of Metal-Pr0.7Ca0.3MnO3 Interface
The polarity-dependent resistive-switching across metal-Pr0.7Ca0.3MnO3 interfaces is investigated. The data suggest that shallow defects in the interface dominate the switching. Their density and fluctuation, therefore, will ultimately limit the device size. While the defects generated/annihilated by the pulses and the associated carrier depletion seem to play the major role at lower defect density, the defect correlations and their associated hopping ranges appear to dominate at higher defect density. Therefore, the switching characteristics, especially the size-scalability, may be altered through interface treatments.
0603832v1
2006-04-12
Influence of Domain Wall on Magnetocaloric Effect in GdPt$_{2}$
The resistivity, magnetoresistance and in-field heat capacity measurements were performed on GdPt$_{2}$ intermetallic compound. The magnetocaloric parameters $\Delta T_{ad}$ and $-\Delta S$ were derived from the in-field heat capacity data. Comparison has been made between the magnetocaloric effect $-\Delta S$ and difference in resistivity $-\Delta \rho$ $(=\rho(H)-\rho(0))$ as a function of temperature. There is distinct difference in the temperature dependence of $-\Delta S$ and $-\Delta \rho$ below the ferromagnetic transition temperature. However after removing the domain wall contribution from $-\Delta \rho$, the nature of $-\Delta S$ and $-\Delta \rho$ dependence as a function of temperature are similar. Our observation indicates that the domain wall contribution in magnetocaloric effect is negligible in spite of the fact that it has significant contribution in magnetotransport.
0604297v1
2006-06-08
Weak localization correction to the anomalous Hall effect in polycrystalline Fe films
In situ transport measurements have been made on ultrathin ($<$100 {\AA} thick) polycrystalline Fe films as a function of temperature and magnetic field for a wide range of disorder strengths. For sheet resistances $R_{xx}$ less than $\sim 3k\Omega$, we find a logarithmic temperature dependence of the anomalous Hall conductivity $\sigma_{xy}$ which is shown for the first time to be due to a universal scale dependent weak localization correction within the skew scattering model. For higher sheet resistance, granularity becomes important and the break down of universal behavior becomes manifest as the prefactors to $\sigma_{xx}$ and $\sigma_{xy}$ decrease at different rates with increasing disorder.
0606215v2
2006-07-24
Magnetoresistance in Thin Permalloy Film (10nm-thick and 30-200nm-wide) Nanocontacts Fabricated by e-Beam Lithography
In this paper we show spin dependent transport experiments in nanoconstrictions ranging from 30 to 200nm. These nanoconstrictions were fabricated combining electron beam lithography and thin film deposition techniques. Two types of geometries have been fabricated and investigated. We compare the experimental results with the theoretical estimation of the electrical resistance. Finally we show that the magnetoresistance for the different geometries does not scale with the resistance of the structure and obtain drops in voltage of 20mV at 20Oe.
0607608v1
2006-07-28
Magnetic hysteresis in the microwave surface resistance of Nb samples in the critical state
We discuss the hysteretic behavior of the field-induced variations of the microwave surface resistance in superconductors in the critical state. Measurements have been performed in a bulk sample of Nb and a powdered one at different values of the temperature. We discuss a model, based on the Coffey and Clem theory, in which we take into account the flux distribution inside the sample, due to the critical state. The experimental results are justified quantitatively in the framework of our model. We show that by fitting the experimental data it is possible to determine the value of the critical current density and its field dependence.
0607754v1
2006-09-25
Doping Dependence of Polaron Hopping Energies in La(1-x)Ca(x)MnO(3) (0<= x<= 0.15)
Measurements of the low-frequency (f<= 100 kHz) permittivity at T<= 160 K and dc resistivity (T<= 430 K) are reported for La(1-x)Ca(x)MnO(3) (0<= x<= 0.15). Static dielectric constants are determined from the low-T limiting behavior of the permittivity. The estimated polarizability for bound holes ~ 10^{-22} cm^{-3} implies a radius comparable to the interatomic spacing, consistent with the small polaron picture established from prior transport studies near room temperature and above on nearby compositions. Relaxation peaks in the dielectric loss associated with charge-carrier hopping yield activation energies in good agreement with low-T hopping energies determined from variable-range hopping fits of the dc resistivity. The doping dependence of these energies suggests that the orthorhombic, canted antiferromagnetic ground state tends toward an insulator-metal transition that is not realized due to the formation of the ferromagnetic insulating state near Mn(4+) concentration ~ 0.13.
0609634v1
2006-10-10
Spin-polarized transport in ferromagnetic multilayered semiconductor nanostructures
The occurrence of inhomogeneous spin-density distribution in multilayered ferromagnetic diluted magnetic semiconductor nanostructures leads to strong dependence of the spin-polarized transport properties on these systems. The spin-dependent mobility, conductivity and resistivity in (Ga,Mn)As/GaAs,(Ga,Mn)N/GaN, and (Si,Mn)/Si multilayers are calculated as a function of temperature, scaled by the average magnetization of the diluted magnetic semiconductor layers. An increase of the resistivity near the transition temperature is obtained. We observed that the spin-polarized transport properties changes strongly among the three materials.
0610275v1
2006-10-12
Domain wall magnetoresistance in a nanopatterned La(2/3)Sr(1/3)MnO3 track
We have measured the contribution of magnetic domain walls (DWs) to the electric resistance in epitaxial manganite films patterned by electron-beam lithography into a track containing a set of notches. We find a DW resistance-area (RA) product of ~2.5 10^(-13) Ohm/m^2 at low temperature and bias, which is several orders of magnitude larger than the values reported for 3d ferromagnets. However, the current-voltage characteristics are highly linear which indicates that the DWs are not phase separated but metallic. The DWRA is found to increase upon increasing the injected current, presumably reflecting some deformation of the wall by spin-transfer. When increasing temperature, the DWRA vanishes at ~225K which is likely related to the temperature dependence of the film anisotropy.
0610338v1
2006-10-25
Origin of negative differential resistance in molecular junctions of Rose Bengal
Negative differential resistance (NDR) is tuned at junctions of electronically different dimer and trimer of Rose Bengal on an atomic flat gold (111) surface. Isolated molecule did not show any NDR. But it was induced to show double NDR with large peak to valley ratio (1.8~3.1) in room temperature via charging its neighbor reproducibly by an electrical pulse. In some sections of junction by applying pulse one could destroy the phenomenon or regenerate it by STM manipulation of molecules. NDR was also independent of polaronic nature. It was possible to write bits 1 and 0 for cationic NDR (in dimer) and 00, 01, 10, 11 for di-anionic NDR (trimer) which generated 2/4 bit memory in a atomic scale junction showing importance of junction electronics in future of moletronics.
0610683v1
2006-11-13
Weak antilocalization in epitaxial graphene: evidence for chiral electrons
Transport in ultrathin graphite grown on silicon carbide is dominated by the electron-doped epitaxial layer at the interface. Weak anti-localization in 2D samples manifests itself as a broad cusp-like depression in the longitudinal resistance for magnetic fields 10 mT$< B <$ 5 T. An extremely sharp weak-localization resistance peak at B=0 is also observed. These features quantitatively agree with graphene weak-(anti)localization theory implying the chiral electronic character of the samples. Scattering contributions from the trapped charges in the substrate and from trigonal warping due to the graphite layer on top are tentatively identified. The Shubnikov-de Haas oscillations are remarkably small and show an anomalous Berry's phase.
0611339v2
2006-12-19
Semiconductors between spin-polarized source and drain
Injecting spins into a semiconductor channel and transforming the spin information into a significant electrical output signal is a long standing problem in spintronics. Actually, this is the prerequisite of several concepts of spin transistor. In this tutorial article, we discuss the general problem of spin transport in a nonmagnetic channel between source and drain. Two problems must be mastered: i) In the diffusive regime, the injection of a spin polarized current from a magnetic metal beyond the ballistic transport zone requires the insertion of a spin dependent and large enough interface resistance. ii) In both the diffusive and ballistic regimes, and whatever the metallic or semiconducting character of the source/drain, a small enough interface resistance is the condition to keep the dwell time shorter than the spin lifetime and thus to conserve the spin accumulation-induced output signal at an optimum level. Practically, the main difficulties come from the second condition. In our presentation of experimental results, we show why the transformation of spin information into a large electrical signal has been more easily achieved with carbon nanotubes than with semiconductors and we discuss how the situation could be improved in the later case.
0612495v1
2007-01-17
Anomalous Hall effect in anatase Ti1-xCoxO2 at low temperature regime
Anomalous Hall effect (AHE) of a ferromagnetic semiconductor anatase \cotio thin film is studied from 10K to 300K. Magnetic field dependence of anomalous Hall resistance is coincident with that of magnetization, while the anomalous Hall resistance decreases at low temperature in spite of nearly temperature-independent magnetization. Anomalous Hall conductivity sigma_AHE is found to be proportional to the square of Hall mobility, suggesting that charge scattering strongly affects the AHE in this system. The anatase Ti1-xCoxO2 also follows a scaling relationship to conductivity sigma_xx as sigma_AHE ~ sigma_xx^1.6, which was observed for another polymorph rutile Ti1-xCoxO2, suggesting an identical mechanism of their AHE.
0701395v2
2007-02-17
Room-Temperature Quantum Hall Effect in Graphene
The quantum Hall effect (QHE), one example of a quantum phenomenon that occur on a truly macroscopic scale, has been attracting intense interest since its discovery in 1980 and has helped elucidate many important aspects of quantum physics. It has also led to the establishment of a new metrological standard, the resistance quantum. Disappointingly, however, the QHE could only have been observed at liquid-helium temperatures. Here, we show that in graphene - a single atomic layer of carbon - the QHE can reliably be measured even at room temperature, which is not only surprising and inspirational but also promises QHE resistance standards becoming available to a broader community, outside a few national institutions.
0702408v1
2007-02-20
Anomalous electric conductions in KSbO3-type metallic rhenium oxides
Single crystals of KSbO3-type rhenium oxides, La4Re6O$19, Pb6Re6O19, Sr2Re3O9 and Bi3Re3O11, were synthesized by a hydrothermal method. Their crystal structures can be regarded as a network of three-dimensional orthogonal-dimer lattice of edge-shared ReO6 octahedra. All of them exhibit small magnitude of Pauli paramagnetism, indicating metallic electronic states without strong electron correlations. The resistivity of these rhenates, except Bi3Re3O11, have a temperature dependence of $rho(T)=\rho_{0}+AT^{n}$ $(n \approx 1.6)$ in a wide temperature range between 5 K and 300 K, which is extraordinary for three-dimensional metals without strong electron correlations. The resistivity of Bi3Re3O11 shows an anomaly around at 50 K, where the magnetic susceptibility also detects a deviation from ordinary Pauli paramagnetism.
0702451v1
2007-03-14
Electrical transport and percolation in magnetoresistive manganite / insulating oxide composites: case of La0.7Ca0.3MnO3 / Mn3O4
We report the results of electrical resistivity measurements carried out on well-sintered La0.7Ca0.3MnO3 / Mn3O4 composite samples with almost constant composition of the magnetoresistive manganite phase (La0.7Ca0.3MnO3). A percolation threshold (fc) occurs when the La0.7Ca0.3MnO3 volume fraction is ~ 0.19. The dependence of the electrical resistivity as a function of La0.7Ca0.3MnO3 volume fraction (fLCMO) can be described by percolation-like phenomenological equations. Fitting the conducting regime (fLCMO > fc) by the percolation power law returns a critical exponent t value of 2.0 +/- 0.2 at room temperature and 2.6 +/-0.2 at 5 K. The increase of t is ascribed to the influence of the grain boundaries on the electrical conduction process at low temperature.
0703367v1
2007-03-25
Origin of superconductivity in nominally "undoped" T'-La$_{2-x}$Y$_{x}$CuO$_{4}$ films
We have systematically studied the transport properties of the La$_{2-x}$Y$_{x}$CuO$_{4}$(LYCO) films of T'-phase ($0.05\leq x \leq 0.30$). In this nominally "undoped" system, superconductivity was acquired in certain Y doping range ($0.10\leq x \leq 0.20$). Measurements of resistivity, Hall coefficients in normal states and resistive critical field ($H^\rho_{c2}$)in superconducting states of the T'-LYCO films show the similar behavior as the known Ce-doped n-type cuprate superconductors, indicating the intrinsic electron-doping nature. The charge carriers are induced by oxygen deficiency. Non-superconducting Y-doped Pr- or Nd-based T'-phase cuprate films were also investigated for comparison, suggesting the crucial role of the radii of A-site cations in the origin of superconductivity in the nominally "undoped" cuptates. Based on a reasonable scenario in the microscopic reduction process, we put forward a self-consistent interpretation of these experimental observations.
0703643v1
2005-11-13
Non-radiating and radiating configurations driven by left-handed metamaterials
It is shown that a pair of identical emitters (e.g. wire dipole antennas) in the focal points of a disc, made of left-handed metamaterial (a "perfect" lens), form a non-radiating electromagnetic configuration. The emitters are fed with voltages of equal magnitude and pi-out-of-phase. Detailed finite-difference time-domain (FDTD) modeling shows that there are non-propagating electromagnetic fields generated - fields that remain confined within the region between the emitters and the lens. The energy balance of the system shows that the radiation resistance of the system is very low. This means that the input power is converted to heat in the volume of the lens and only a small fraction of it is radiated. The system performance shows that disturbing the configuration of the non-propagating electromagnetic fields with the presence of an externally introduced object stimulates radiation. This suggests possible detector applications. In-phase feeding voltages are also studied with the consequence that the radiation resistance of the antennae is increased.
0511113v1
2007-04-16
Memory function formalism approach to electrical conductivity and optical response of dilute magnetic semiconductors
A combination of the memory function formalism and time-dependent density-functional theory is applied to transport in dilute magnetic semiconductors. The approach considers spin and charge disorder and electron-electron interaction on an equal footing. Within the weak disorder limit and using a simple parabolic approximation for the valence band we show that Coulomb and exchange scattering contributions to the resistivity in GaMnAs are of the same order of magnitude. The positional correlations of defects result in a significant increase of Coulomb scattering, while the suppression of localized spin fluctuations in the ferromagnetic phase contributes substantially to the experimentally observed drop of resistivity below T_c. A proper treatment of dynamical screening and collective excitations is essential for an accurate description of infrared absorption.
0704.2061v1
2007-05-15
Magnetic, magneto-thermal and magneto-transport properties in SmMn2Si2-xGex compounds
The effect of Ge substitution for Si in SmMMn2Si2-xGex compounds has been studied. The Sm ordering temperature is found to be much larger in the compound with x=2, as compared to the compounds with x=0 and 1. The increase in the intra layer Mn-Mn distance is found to be responsible for this increase. Among these three compounds, SmMn2Ge2 is found to show re-entrant ferromagnetism at low temperatures. The magnetic contribution to the heat capacity has been found in all the three compounds. The splitting of the ground state multiplet has been estimated by fitting the magnetic part of the heat capacity data using the Schottky formula. The isothermal magnetic entropy change is found to remain the same for x=0 and 1, but decrease in the compound with x=2, though the nature of magnetic transition changes from second order to first order, as x is increased from 0 to 2. The electrical resistivity increases with Ge concentration. The excess resistivity in the antiferromagnetic region has been calculated.
0705.2237v1
2007-06-01
Anomalous magnetoresistance of EuB$_{5.99}$C$_{0.01}$: Enhancement of magnetoresistance in systems with magnetic polarons
We present results of measurements of electrical, magnetic and thermal properties of EuB$_{5.99}$C$_{0.01}$. The observed anomalously large negative magnetoresistance as above, so below the Curie temperature of ferromagnetic ordering $T_C$ is attributed to fluctuations in carbon concentration. Below $T_C$ the carbon richer regions give rise to helimagnetic domains, which are responsible for an additional scattering term in the resistivity, which can be suppressed by a magnetic field. Above $T_C$ these regions prevent the process of percolation of magnetic polarons (MPs), acting as "spacers" between MPs. We propose that such "spacers", being in fact volumes incompatible with existence of MPs, may be responsible for the decrease of the percolation temperature and for the additional (magneto)resistivity increase in systems with MPs.
0706.0091v1
2007-07-03
Spatial correlation of linear and nonlinear electron transport in superconducting microwave resonator: laser scanning microscopy analysis
Spatially-resolved techniques of laser scanning microscopy (LSM) have been used to image simultaneously the spatial variations of (i) rf current flow, J$_RF$(x,y), of (ii) areas of resistive dissipation and (iii) the sources of microwave nonlinearity (NL) in an operating superconducting resonator. The RF power dependent spatial evolution of these linear and NL microwave properties in the meander strip YBCO/LAO superconducting resonator have been LSM probed at different temperatures below Tc. The influence of both topologies of the twin-domain YBCO structure and of J$_RF$(x,y) peaks at the edges of superconducting strip line on its NL properties was analyzed in detail with a micron-scale spatial resolution. Result shows the resistive origin of the dominant sources of microwave NLs
0707.0358v1
2007-07-04
Resistive Switching in Cr doped SrTiO3: An X-ray Absorption Spectroscopy study
X-ray absorption spectroscopy was used to study the microscopic origin of conductance and resistive switching in chromium doped strontium titanate (Cr:SrTiO3). Differences in the x-ray absorption near edge spectroscopy (XANES) at the Cr K-edge indicate that the valence of Cr changes from 3+ to 4+ underneath the anode of our sample device after the application of an electric field. Spatially resolved x-ray fluorescence microscopy ($\mu$-XRF) maps show that the Cr4+ region retracts from the anode-Cr:SrTiO3 interface after a conducting state has been achieved. This interface region is studied with extended x-ray absorption fine structure (EXAFS) and the results are compared with structural parameters obtained from density functional theory (DFT) calculations. They confirm that oxygen vacancies which are localized at the octahedron with a Cr at its center are introduced at the interface. It is proposed that the switching state is not due to a valence change of chromium but caused by changes of oxygen vacancies at the interface.
0707.0655v1
2007-08-21
Negative differential resistance of Styrene on an ideal Si[111] surface: dependence of the I-V characteristics on geometry, surface doping and shape of the STM-tip
We study the electron transport properties through a supported organic molecule styrene (C8H8) on an ideal silicon surface Si[111] and probed by a STM-tip. The I-V characteristics and the differential conductance of the molecule are calculated using a self consistent approach based on non equilibrium Green's functions. Two different adsorption configurations for the molecule on the surface were considered which corresponds to a global and a local minimum of the total energy. In both cases we find a negative differential resistance (NDR) in a given interval of bias voltages. This effect is controlled by the states available close to the Fermi level of the surface and can be manipulated by properly doping the substrate. We also analyze the influence of the tip-shape on the I-V characteristics.
0708.2834v1
2007-12-21
Vibronic polarons: comments on a model for the colossal field-resistance effects in manganites
In addition to mechanisms already proposed to account for the formation in manganites of a small-polaron superlattice above the Curie temperature Tc and to a metallic-like sea of large polarons below Tc, we now consider other observed colossal-resistance inducing fields, such as magnetic, electric, photon, or strain fields. We attribute the charge-ordered phase formation to the occurrence of strong dipolar binding of vibronic small polarons arising from the phonon coupling of highly polarizable two-level orbital systems. These species having associated inherent electric and magnetic off-center dipoles, they couple to the external fields leading to the observed colossal effects. The random phase appears due to polaron band widening in the external field.
0712.3803v1
2008-03-05
The behavior of magnetic ordering and the KOndo effect in the alloys, Ce2Rh(1-x)Co(x)Si3: Evidence from bulk studies for Fermi-surface change during magnetic ordering - QCP transformation and applicability of SDW pictur
The results of magnetic susceptibility, electrical resistivity (rho), and heat capacity measurements as a function of temperature are reported for the alloys, Ce2Rh(1-x)Co(x)Si3, crystallizing in an AlB2-derived hexagonal strcture. Ce2RhSi3 exhibits antiferromagnetic ordering at 7 K. The Neel temperature decreases gradually with the increase in Co concentration. For x greater than 0.6, no magnetic ordering is observed down to 0.5 K. Interestingly, the x= 0.6 alloy exhibits signatutes of non-Fermi liquid behavior, while the Co end member is a Fermi liquid. Thus, a transformation of magnetic ordering state to non-magnetism via non-Fermiliquid state by isoelectronic chemical doping is evident in this solid solution. The electrical resistivity data for x= 0.2 and 0.3 alloys show an upturn at respective Neel temperatures, establishing the formation of a magnetism-induced pseudo-gap for these intermediate compositions alone as though there is a gradual Fermi surface transformation as the quantum critical point is approached.
0803.0652v1
2008-03-09
Upper critical field, Hall effect and magnetoresistance in the iron-based layered superconductor LaFeAsO_{0.9}F_{0.1-δ}
By using a two-step method, we successfully synthesized the iron based new superconductor LaFeAsO_{0.9}F_{0.1-\delta}$. The resistive transition curves under different magnetic fields were measured, leading to the determination of the upper critical field Hc2(T) of this new superconductor. The value of Hc2 at zero temperature is estimated to be about 50 Tesla roughly. In addition, the Hall effect and magnetoresistance were measured in wide temperature region. A negative Hall coefficient R_H has been found, implying a dominant conduction mainly by electron-like charge carriers in this material. The charge carrier density determined at 100 K is about 9.8E20cm^{-3}, which is close to the cuprate superconductors. It is further found that the magnetoresistance does not follow Kohler's law. Meanwhile, the different temperature dependence behaviors of resistivity, Hall coefficient, and magnetoresistance have anomalous properties at about 230 K, which may be induced by some exotic scattering mechanism.
0803.1288v2
2008-03-12
Electron transport and thermoelectric properties of layered perovskite LaBaCo2O5.5
We have investigated the systematic transport properties of the layered 112-type cobaltite LaBaCo2O5.5 by means of electrical resistivity, magnetoresistance, electroresistance and thermoelectric measurements in various conditions. In order to understand the complex conduction mechanism of LaBaCo2O5.5, the transport data have been analyzed using different theoretical models. The system shows semiconductor-semiconductor like transition (TSC) around 326K, corresponding to ferromagnetic transition and in the low temperature region resistivity data follows the Motts variable range hopping model. Interestingly, near and below the room temperature this compound depicts significant change in electro- and magnetoresistance behavior, the latter one is noteworthy near the magnetic phase boundary. The temperature dependence of thermopower, S(T), exhibits p-type polaronic conductivity in the temperature range of 60-320K and reaches a maximum value of 303 uV/K (at 120K). In the low temperature AFM region, the unusual S(T) behavior, generally observed for the cobaltite series LnBaCo2O5.5 (Ln = Rare Earth), is explained by the electron magnon scattering mechanism as previously described for perovskite manganites.
0803.1806v1
2008-03-14
From Ohmic to Ballistic Transport in Oriented Graphite
In this work we show that for a quasi-2D system of size $\Omega$ and thickness $t$ the resistance goes as $(2\rho/\pi t)\ln(\Omega/W)$, diverging logarithmically with the size. Measurements in highly oriented pyrolytic graphite (HOPG) as well as numerical simulations confirm this relation. Furthermore, we present an experimental method that allows us to obtain the carriers mean free path $l(T)$, the Fermi wavelength $\lambda(T)$ and the mobility $\mu(T)$ directly from experiments without adjustable parameters. Measuring the electrical resistance through microfabricated constrictions in HOPG and observing the transition from ohmic to ballistic regime we obtain that $0.2 \mu$m $\lesssim l \lesssim 10 \mu$m, $0.1 \mu$m $\lesssim \lambda \lesssim 2 \mu$m and a mobility $5 \times 10^4$ cm$^2$/Vs $ \lesssim \mu \lesssim 4 \times 10^7$ cm$^2$/Vs when the temperature decreases from 270K to 3K. A comparison of these results with those from literature indicates that conventional, multiband Boltzmann-Drude approaches are inadequate for oriented graphite. The upper value obtained for the mobility is much larger than the mobility graphene samples of micrometer size can have.
0803.2203v2
2008-03-19
Theory of quantum metal to superconductor transitions in highly conducting systems
We derive the theory of the quantum (zero temperature) superconductor to metal transition in disordered materials when the resistance of the normal metal near criticality is small compared to the quantum of resistivity. This can occur most readily in situations in which ``Anderson's theorem'' does not apply. We explicitly study the transition in superconductor-metal composites, in an s-wave superconducting film in the presence of a magnetic field, and in a low temperature disordered d-wave superconductor. Near the point of the transition, the distribution of the superconducting order parameter is highly inhomogeneous. To describe this situation we employ a procedure which is similar to that introduced by Mott for description of the temperature dependence of the variable range hopping conduction. As the system approaches the point of the transition from the metal to the superconductor, the conductivity of the system diverges, and the Wiedemann-Franz law is violated. In the case of d-wave (or other exotic) superconductors we predict the existence of (at least) two sequential transitions as a function of increasing disorder: a d-wave to s-wave, and then an s-wave to metal transition.
0803.2902v2
2008-03-23
Origin of negative differential resistance in a strongly coupled single molecule-metal junction device
A new mechanism is proposed to explain the origin of negative differential resistance (NDR) in a strongly coupled single molecule-metal junction. A first-principles quantum transport calculation in a Fe-terpyridine linker molecule sandwiched between a pair of gold electrodes is presented. Upon increasing applied bias, it is found that a new phase in the broken symmetry wavefunction of the molecule emerges from the mixing of occupied and unoccupied molecular orbital. As a consequence, a non-linear change in the coupling between molecule and lead is evolved resulting to NDR. This model can be used to explain NDR in other class of metal-molecule junction device.
0803.3342v1
2008-04-13
Conductance of p-n-p graphene structures with 'air-bridge' top gates
We have fabricated graphene devices with a top gate separated from the graphene layer by an air gap--a design which does not decrease the mobility of charge carriers under the gate. This gate is used to realise p-n-p structures where the conducting properties of chiral carriers are studied. The band profile of the structures is calculated taking into account the specifics of the graphene density of states and is used to find the resistance of the p-n junctions expected for chiral carriers. We show that ballistic p-n junctions have larger resistance than diffusive ones. This is caused by suppressed transmission of chiral carriers at angles away from the normal to the junction.
0804.2081v3
2008-06-16
Metal-insulator transition and giant anisotropic magnetoresistance in ultra thin (Ga,Mn)As
MBE-grown, 5 nm-thick annealed Ga0.95Mn0.05As films with Tc~90K demonstrate transition from metallic to insulating state below To~10K, where sheet resistances Rsh~h/e2 and both longitudinal Rxx and transverse Rxy components become comparable. Below metal-insulator transition we found giant anisotropic magnetoresistance (GAMR), which depends on orientation of magnetization to crystallographic axes and manifests itself in positive magnetoresistance near 50% for Rxx at T=1.7K, H//[110] crystallographic direction and parallel to current in contrast to smaller and negative magnetoresistance for H// direction. We connect GAMR with anisotropic spin-orbit interaction resulting in formation of high- and low- resistance states with different localization along non-equivalent easy axes.
0806.2590v1
2008-06-28
Theory of spin magnetohydrodynamics
We develop a phenomenological hydrodynamic theory of coherent magnetic precession coupled to electric currents. Exchange interaction between electron spin and collective magnetic texture produces two reciprocal effects: spin-transfer torque on the magnetic order parameter and the Berry-phase gauge field experienced by the itinerant electrons. The dissipative processes are governed by three coefficients: the ohmic resistance, Gilbert damping of the magnetization, and the "beta coefficient" describing viscous coupling between magnetic dynamics and electric current, which stems from spin mistracking of the magnetic order. We develop general magnetohydrodynamic equations and discuss the net dissipation produced by the coupled dynamics. The latter in particular allows us to determine a lower bound on the magnetic-texture resistivity.
0806.4656v2
2008-07-28
Transport anomalies across the quantum limit in semimetallic Bi$_{0.96}$Sb$_{0.04}$
We report on a study of electronic transport in semi-metallic Bi$_{0.96}$Sb$_{0.04}$. At zero field, the system is a very dilute Fermi liquid displaying a T$^{2}$ resistivity with an enhanced prefactor. Quantum oscillations in resistivity as well as in Hall, Nernst and Seebeck responses of the system are detectable and their period quantifies the shrinking of the Fermi surface with antimony doping. For a field along the trigonal axis, the quantum limit was found to occur at a field as low as 3T. An ultraquantum anomaly at twice this field was detected in both charge transport and Nernst response. Its origin appears to lie beyond the one-particle picture and linked to unidentified many-body effects.
0807.4432v1
2008-07-30
Ultra-Thin Silver Films obtained by Sequential Quench-Anneal Processing
We have used the two-step growth technique, quench condensing followed by an anneal, to grow ultra thin films of silver on glass substrates. As has been seen with semiconductor substrates this process produces a metastable homogeneous covering of silver. By measuring the in situ resistance of the film during growth we are able to see that the low temperature growth onto substrates held at 100 Kelvin produces a precursor phase that is insulating until the film has been annealed. The transformation of the precursor phase into the final, metallic silver film occurs at a characteristic temperature near 150K where the sample reconstructs. This reconstruction is accompanied by a decrease in resistance of up to 10 orders of magnitude.
0807.4948v1
2008-08-09
Electronic transport and specific heat of 1T- VSe2
The results of low temperature thermoelectric power and the specific heat of 1T-VSe2 (Vanadium diselenide) have been reported along with the electrical resistivity, and Hall coefficient of the compound. The Charge Density Wave (CDW) transition is observed near 110K temperature in all these properties. The Thermoelectric power has been measured from 15K to 300K spanning the incommensurate and commensurate CDW regions. We observed a weak anomaly at the CDW transition for the first time in the specific heat of VSe2. The linear temperature dependence of resistivity and thermoelectric power at higher temperatures suggests a normal metallic behavior and electron-phonon scattering above the CDW transition. The positive thermoelectric power and negative Hall coefficient along with strongly temperature dependent behavior in the CDW phase suggest a mixed conduction related to the strongly hybridized s-p-d bands in this compound.
0808.1332v2
2008-08-11
Non-trivial length dependence of the conductance and negative differential resistance in atomic molecular wires
We study the electronic and transport properties of two novel molecular wires made of atomic chains of carbon atoms (polyynes) capped with either, benzene-thiols or pyridines. While both molecules are structurally similar, the electrical conductance of benzene-thiol-capped chains attached to gold electrodes is found to be much higher than that of pyridine-capped chains. We predict that the conductance is almost independent of molecular length, which suggests that these molecules could be ideal molecular wires for sub-10 nm circuitry. Both systems exhibit negative differential resistance (NDR) but its origin and characteristics depend on the type of molecule. We find a novel type of NDR mechanism produced by the movement of the LUMO resonance with bias. We also show that by gating the pyridine-capped molecules it is possible to make the NDR disappear and dramatically modify the $I$-$V$ characteristics and the length dependence.
0808.1494v2
2008-08-21
Electrons and holes in Si quantum well: a room-temperature transport and drag resistance study
We investigate carrier transport in a single 22 nm-thick double-gated Si quantum well device, which has independent contacts to electrons and holes. Conductance, Hall density and Hall mobility are mapped in a broad double-gate voltage window. When the gate voltage asymmetry is not too large only either electrons or holes occupy the Si well and the Hall mobility shows the fingerprints of volume inversion/accumulation. At strongly asymmetric double-gate voltage an electric field induced electron-hole (EH) bi-layer is formed inside the well. The EH drag resistance R_{he} is explored at balanced carrier densities: R_{he} decreases monotonically from 860 to 37 Ohms when the electron and hole density is varied between ~0.4-1.7x10^{16} m^{-2}.
0808.2914v1
2008-10-27
Abrupt Emergence of Pressure-Induced Superconductivity of 34 K in SrFe2As2: A Resistivity Study under Pressure
We report resistivity measurement under pressure in single crystals of SrFe_2As_2, which is one of the parent materials of Fe-based superconductors. The structural and antiferromagnetic (AFM) transition of T_0 = 198 K at ambient pressure is suppressed under pressure, and the ordered phase disappears above P_c ~ 3.6-3.7 GPa. Superconductivity with a sharp transition appears accompanied by the suppression of the AFM state. T_c exhibits a maximum of 34.1 K, which is realized close to the phase boundary at P_c. This T_c is the highest among those of the stoichiometric Fe-based superconductors.
0810.4856v2
2008-12-11
Difference of Oxide Hetero-Structure Junctions with Semiconductor Electronic Devices
Charge carrier injection performed in Pr0.7Ca0.3MnO3 (PCMO) hetero-structure junctions exhibits stable without electric fields and dramatic changes in both resistances and interface barriers, which are entirely different from behaviors of semiconductor devices. Disappearance and reversion of interface barriers suggest that the adjustable resistance switching of such hetero-structure oxide devices should associate with motion of charge carriers across interfaces. The results suggested that injected carriers should be still staying in devices and resulted in changes in properties, which guided to a carrier self-trapping and releasing picture in strongly correlated electronic framework. Observations in PCMO and oxygen deficient CeO2 devices show that oxides as functional materials could be used in microelectronics with some novel properties, in which interface is very important.
0812.2071v1
2008-12-11
Evidence for Coexistence of Superconductivity and Magnetism in Single Crystals of Co-doped SrFe$_2$As$_2$
In order to investigate whether magnetism and superconductivity coexist in Co-doped SrFe$_2$As$_2$, we have prepared single crystals of SrFe$_{2-x}$Co$_x$As$_2$, $x$ = 0 and 0.4, and characterized them via X-ray diffraction, electrical resistivity in zero and applied field up to 9 T as well as at ambient and applied pressure up to 1.6 GPa, and magnetic susceptibility. At $x$ = 0.4, there is both magnetic and resistive evidence for a spin density wave transition at 120 K, while $T_c$ = 19.5 K - indicating coexistent magnetism and superconductivity. A discussion of how these results compare with reported results, both in SrFe$_{2-x}$Co$_x$As$_2$ and in other doped 122 compounds, is given.
0812.2091v1
2009-01-10
Wafer-Scale, Sub-5 nm Junction Formation by Monolayer Doping and Conventional Spike Annealing
We report the formation of sub-5 nm ultrashallow junctions in 4 inch Si wafers enabled by the molecular monolayer doping of phosphorous and boron atoms and the use of conventional spike annealing. The junctions are characterized by secondary ion mass spectrometry and non-contact sheet resistance measurements. It is found that the majority (~70%) of the incorporated dopants are electrically active, therefore, enabling a low sheet resistance for a given dopant areal dose. The wafer-scale uniformity is investigated and found to be limited by the temperature homogeneity of the spike anneal tool used in the experiments. Notably, minimal junction leakage currents (<1 uA/cm2) are observed which highlights the quality of the junctions formed by this process. The results clearly demonstrate the versatility and potency of the monolayer doping approach for enabling controlled, molecular-scale ultrashallow junction formation without introducing defects in the semiconductor.
0901.1396v1