dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-aff4bb6560f44a6c9e3a0009d8d22301
Nc1ccc(Br)cn1.O=C(Cl)c1ccccc1[N+](=O)[O-]>>O=C(Nc1ccc(Br)cn1)c1ccccc1[N+](=O)[O-]
[N+](=O)([O-])C1=C(C(=O)Cl)C=CC=C1.NC1=NC=C(C=C1)Br.N1=CC=CC=C1>>BrC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)[N+](=O)[O-]
[NH2:3][c:4]1[cH:5][cH:6][c:7]([Br:8])[cH:9][n:10]1.Cl[C:2](=[O:1])[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[N+:17](=[O:18])[O-:19]>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][c:7]([Br:8])[cH:9][n:10]1)[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[N+:17](=[O:18])[O-:19]
Nc1ccc(Br)cn1.O=C(Cl)c1ccccc1[N+](=O)[O-]
O=C(Nc1ccc(Br)cn1)c1ccccc1[N+](=O)[O-]
null
null
C(Cl)Cl
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(Nc1ccccn1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:3](:[c:4]):[c:5]
77.9
[{"value": 77.0, "product": "BrC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.9, "product": "BrC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 2-nitrobenzoyl chloride (3.70 g, 20 mmol, 1.0 equiv), 2-amino-5-bromopyridine (3.50 g, 1.0 equiv), pyridine (10 mL) in 25 mL of methylene chloride was stirred overnight. The volatile was evaporated, flash chromatography on silica gel gave N-(5-bromo-2-pyridinyl)-(2-nitro)phenylcarboxamide (5.02 g, 77%). M...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccncc1.c1ccccc1
HCl
C(Cl)Cl
null
null
Nc1ccc(Br)cn1.O=C(Cl)c1ccccc1[N+](=O)[O-]>C(Cl)Cl>O=C(Nc1ccc(Br)cn1)c1ccccc1[N+](=O)[O-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-d06354339c1c4248aa2e70c96f4c2652
CC1=CC(=O)OC1=O.Nc1ccc(Br)cn1>>CC1=CC(=O)N(c2ccc(Br)cn2)C1=O
C1(\C(\C)=C/C(=O)O1)=O.NC1=NC=C(C=C1)Br>>BrC=1C=CC(=NC1)N1C(C(=CC1=O)C)=O
O1[C:4](=[O:5])[CH:3]=[C:2]([CH3:1])[C:14]1=[O:15].[NH2:6][c:7]1[cH:8][cH:9][c:10]([Br:11])[cH:12][n:13]1>>[CH3:1][C:2]1=[CH:3][C:4](=[O:5])[N:6]([c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][n:13]2)[C:14]1=[O:15]
CC1=CC(=O)OC1=O.Nc1ccc(Br)cn1
CC1=CC(=O)N(c2ccc(Br)cn2)C1=O
null
null
C1(=CC=CC=C1)C
Acylation
OtherReaction
cab1acd179957d4f5c27ba23f314ee257f7d508deff2838c7964b1019063e651
2a4a20e639c386292668b0b265a8e1b50d707d5f0576437dc5ade3e7fd444d29
O=C1C=CC(=O)N1c1ccccn1
[C;D1;H3:1]-[C:2]1=[C:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-O-[C;H0;D3;+0:6]-1=[O;D1;H0:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[#7;a:11]:[c:12]>>[C;D1;H3:1]-[C:2]1=[C:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[N;H0;D3;+0:8](-[c:9](:[c:10]):[#7;a:11]:[c:12])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
71
[{"value": 71.0, "product": "BrC=1C=CC(=NC1)N1C(C(=CC1=O)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 70.8, "product": "BrC=1C=CC(=NC1)N1C(C(=CC1=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of citraconic anhydride (1.00 mL, 11.1 mmol) and 2-amino-5-bromopyridine (1.93 g, 11.2 mmol) in toluene (60 mL) was heated to reflux overnight. The solution was cooled down, filtered. The filtrate was concentrated in vacuo to give a solid (2.10 g, yield: 71%). MS 267 and 269 (M+H). Conditions: See reaction.no...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary amine
Substituted dicarboximide
C1=CCOC1
C1=CC[NH]C1
C1=CC[NH]C1.c1ccncc1
HO-
C1(=CC=CC=C1)C
null
null
CC1=CC(=O)OC1=O.Nc1ccc(Br)cn1>C1(=CC=CC=C1)C>CC1=CC(=O)N(c2ccc(Br)cn2)C1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a9b6035cb27d4c51a725621d2aa97cec
Nc1ccc(Cl)cn1.O=c1[nH]c2ccc(Cl)cc2c(=O)o1>>Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1
ClC1=CC=C2C(C(=O)OC(N2)=O)=C1.NC1=NC=C(C=C1)Cl.C[Si](C)(C)[N-][Si](C)(C)C.[K+].C1(=CC=CC=C1)C>>NC1=C(C=C(C=C1)Cl)C(=O)NC1=NC=C(C=C1)Cl
[NH2:11][c:12]1[cH:13][cH:14][c:15]([Cl:16])[cH:17][n:18]1.O=c1o[c:9](=[O:10])[c:8]2[c:2]([nH:1]1)[cH:3][cH:4][c:5]([Cl:6])[cH:7]2>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[cH:7][c:8]1[C:9](=[O:10])[NH:11][c:12]1[cH:13][cH:14][c:15]([Cl:16])[cH:17][n:18]1
Nc1ccc(Cl)cn1.O=c1[nH]c2ccc(Cl)cc2c(=O)o1
Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1
null
null
O1CCCC1
Acylation
OtherReaction
b4c245015e48b9b60756b62e3f8985928af86452315d98417a25faace320d9ae
b609a70ccab739990a9ccc4ea2adcc77011bcd0c07154489a12420f7c0e7382e
O=C(Nc1ccccn1)c1ccccc1
O=c1:[nH;D2;+0:1]:[c:2](:[c:3]):[c:4](:[c:5]):[c;H0;D3;+0:6](=[O;D1;H0:7]):o:1.[NH2;D1;+0:8]-[c:9](:[c:10]):[#7;a:11]:[c:12]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4](-[C;H0;D3;+0:6](=[O;D1;H0:7])-[NH;D2;+0:8]-[c:9](:[c:10]):[#7;a:11]:[c:12]):[c:5]
100
[{"value": 100.0, "product": "NC1=C(C=C(C=C1)Cl)C(=O)NC1=NC=C(C=C1)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.7, "product": "NC1=C(C=C(C=C1)Cl)C(=O)NC1=NC=C(C=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
0.5
HOUR
To a solution of 2-amino-5-chloropyridine (328 mg, 2.55 mmol) in tetrahydrofuran (5 ml) was 0.5M potassium bis(trimethylsilyl)amide in toluene (10 ml, 5.05 mmol) dropwise at −78° C. After stirred for additional 0.5 hr at −78° C., the mixture was added 5-chloroisatoic anhydride (0.5 g, 2.55 mmol) at −78° C. The mixture ...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Secondary amide.Primary amine
c1ccc2ncocc2c1
c1ccccc1
c1ccccc1.c1ccncc1
Other
O1CCCC1
-78
0.5
Nc1ccc(Cl)cn1.O=c1[nH]c2ccc(Cl)cc2c(=O)o1>O1CCCC1>Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-521deda5768143b9ba3ef322a90cc5ba
CNCCN.N#Cc1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1>>CN1CCN=C1c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
CNCCN.ClC1=CC(=C(C=C1)NC(=O)C1=CC=C(C=C1)C#N)C(NC1=NC=C(C=C1)Cl)=O.S.IC>>ClC1=CC(=C(C=C1)NC(=O)C1=CC=C(C=C1)C=1N(CCN1)C)C(NC1=NC=C(C=C1)Cl)=O
N[CH2:4][CH2:3][NH:2][CH3:1].[N:5]#[C:6][c:7]1[cH:8][cH:9][c:10]([C:11](=[O:12])[NH:13][c:14]2[cH:15][cH:16][c:17]([Cl:18])[cH:19][c:20]2[C:21](=[O:22])[NH:23][c:24]2[cH:25][cH:26][c:27]([Cl:28])[cH:29][n:30]2)[cH:31][cH:32]1>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]=[C:6]1[c:7]1[cH:8][cH:9][c:10]([C:11](=[O:12])[NH:13][c:14]2...
CNCCN.N#Cc1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
CN1CCN=C1c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
null
null
N1=CC=CC=C1.CO.C(C)(=O)O.C(C)N(CC)CC
Heteroatom Alkylation and Arylation
OtherReaction
c60ad675bbef0aae4bc6f7e7229a0d6b3b6a784179e30b9e067ffd6151067a5c
4290e5b2bf07838a6d478b39c42778e9467fef0b3ea75c8d873e295925a35d9e
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(C2=NCCN2)cc1
N-[CH2;D2;+0:1]-[C:2]-[NH;D2;+0:3]-[C;D1;H3:4].[N;H0;D1;+0:5]#[C;H0;D2;+0:6]-[c:7](:[c:8]):[c:9]>>[C;D1;H3:4]-[N;H0;D3;+0:3]1-[C:2]-[CH2;D2;+0:1]-[N;H0;D2;+0:5]=[C;H0;D3;+0:6]-1-[c:7](:[c:8]):[c:9]
null
[]
null
null
8
HOUR
To a solution of the compound of N-{4-chloro-2-[N-(5-chloro(2-pyridyl))carbamoyl]phenyl}(4-cyanophenyl)carboxamide (683 mg, 1.66 mmol) in anhydrous pyridine (10 ml) and triethyl amine (1 ml) was saturated with hydrogen sulfide gas at 0° C. The mixture was stirred at r.t. overnight. After the evaporated the solvent, the...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine.Secondary amine
Tertiary amine
null
C1=NCC[NH]1
C1=NCC[NH]1.c1ccccc1.c1ccccc1.c1ccncc1
Other
N1=CC=CC=C1.CO.C(C)(=O)O.C(C)N(CC)CC
null
8
CNCCN.N#Cc1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1>N1=CC=CC=C1.CO.C(C)(=O)O.C(C)N(CC)CC>CN1CCN=C1c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-bd09f05c6fa3401a81f8a51176430386
Cc1ccc([N+](=O)[O-])c(C(=O)O)c1.Nc1ccc(Cl)cn1>>Cc1ccc([N+](=O)[O-])c(C(=O)Nc2ccc(Cl)cn2)c1
CC=1C=CC(=C(C(=O)O)C1)[N+](=O)[O-].C(C(=O)Cl)(=O)Cl.NC1=NC=C(C=C1)Cl.N1=CC=CC=C1>>ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)C)[N+](=O)[O-]
O[C:10]([c:9]1[c:5]([N+:6](=[O:7])[O-:8])[cH:4][cH:3][c:2]([CH3:1])[cH:20]1)=[O:11].[NH2:12][c:13]1[cH:14][cH:15][c:16]([Cl:17])[cH:18][n:19]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[c:9]([C:10](=[O:11])[NH:12][c:13]2[cH:14][cH:15][c:16]([Cl:17])[cH:18][n:19]2)[cH:20]1
Cc1ccc([N+](=O)[O-])c(C(=O)O)c1.Nc1ccc(Cl)cn1
Cc1ccc([N+](=O)[O-])c(C(=O)Nc2ccc(Cl)cn2)c1
null
CN(C=O)C
ClCCl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccn1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:3](:[c:4]):[c:5]
92
[{"value": 92.0, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)C)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.9, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)C)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 5-methyl-2-nitrobenzoic acid (1 g, 5.52 mmol) in dichloromethane (5 ml) was added oxalyl chloride (0.964 ml, 11.04 mmol) and a few drops of dimethylformamide. The mixture was stirred at r.t. for 2 hrs. After the evaporation of the solvent, the residue was dissolved in dichloromethane (5 ml). 2-amino-5-...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccncc1
HO-
CN(C=O)C.ClCCl
null
2
Cc1ccc([N+](=O)[O-])c(C(=O)O)c1.Nc1ccc(Cl)cn1>CN(C=O)C.ClCCl>Cc1ccc([N+](=O)[O-])c(C(=O)Nc2ccc(Cl)cn2)c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-24b595b9283a44c19b23094563f6a21c
Cc1ccc([N+](=O)[O-])c(C(=O)Nc2ccc(Cl)cn2)c1>>Nc1ccccc1C(=O)Nc1ccccn1.[Cl-]
ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)C)[N+](=O)[O-].[H][H]>>NC1=C(C=CC=C1)C(=O)NC1=NC=CC=C1.[Cl-]
C[c:5]1[cH:4][cH:3][c:2]([N+:1](=O)[O-])[c:7]([C:8](=[O:9])[NH:10][c:11]2[cH:12][cH:13][c:14]([Cl:17])[cH:15][n:16]2)[cH:6]1>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[C:8](=[O:9])[NH:10][c:11]1[cH:12][cH:13][cH:14][cH:15][n:16]1.[Cl-:17]
Cc1ccc([N+](=O)[O-])c(C(=O)Nc2ccc(Cl)cn2)c1
Nc1ccccc1C(=O)Nc1ccccn1.[Cl-]
null
[Pt]
CO
Functional Group Interconversion
OtherReaction
7335ad64e689ca4e08d92da67da5a4ba3d7b1ae27a9bb5d9a29f9de23a6b4f9a
f3a5ba2ad2c4d7897d16c1f6f55c603d6dd39035ce4ed56632c5b924cbe6ba83
O=C(Nc1ccccn1)c1ccccc1
C-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[N+;H0;D3:5](=O)-[O-]):[c:6](-[C:7](=[O;D1;H0:8])-[#7:9]-[c:10]2:[#7;a:11]:[c:12]:[c;H0;D3;+0:13](-[Cl;H0;D1;+0:14]):[c:15]:[c:16]:2):[c:17]:1>>[Cl-;H0;D0:14].[NH2;D1;+0:5]-[c:4]1:[c:3]:[c:2]:[cH;D2;+0:1]:[c:17]:[c:6]:1-[C:7](=[O;D1;H0:8])-[#7:9]-[c:10]1:[#7;a:11]:[c:12]:[cH;D2;+0:1...
null
[]
null
null
null
null
To a solution of the compound of N-(5-chloro(2-pyridyl))(5-methyl-2-nitrophenyl)carboxamide (1.48 g, 5.1 mmol) in methanol (10 ml) was added 5% Pt/C (1.48 g, 0.19 mmol). The mixture was applied hydrogen balloon at r.t. for 2 hrs. After the filtration by Celite, the filtrate was concentrated to give (2-aminophenyl)-N-(2...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Nitro group
Primary amine
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
Other
[Pt].CO
null
null
Cc1ccc([N+](=O)[O-])c(C(=O)Nc2ccc(Cl)cn2)c1>[Pt].CO>Nc1ccccc1C(=O)Nc1ccccn1.[Cl-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-fc958fa311974f6596f2ee991a7694ea
CNCCN.Cc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1>>Cc1ccc(NC(=O)c2ccc(C3=NCCN3C)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1
ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)C)NC(=O)C1=CC=C(C=C1)C#N.Cl.CNCCN>>ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)C)NC(=O)C1=CC=C(C=C1)C=1N(CCN1)C
[NH2:14][CH2:15][CH2:16][NH:17][CH3:18].N#[C:13][c:12]1[cH:11][cH:10][c:9]([C:7]([NH:6][c:5]2[cH:4][cH:3][c:2]([CH3:1])[cH:32][c:21]2[C:22](=[O:23])[NH:24][c:25]2[cH:26][cH:27][c:28]([Cl:29])[cH:30][n:31]2)=[O:8])[cH:20][cH:19]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH:6][C:7](=[O:8])[c:9]2[cH:10][cH:11][c:12]([C:13]3=[N:14...
CNCCN.Cc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1
Cc1ccc(NC(=O)c2ccc(C3=NCCN3C)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1
null
null
CO.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
c60ad675bbef0aae4bc6f7e7229a0d6b3b6a784179e30b9e067ffd6151067a5c
4290e5b2bf07838a6d478b39c42778e9467fef0b3ea75c8d873e295925a35d9e
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(C2=NCCN2)cc1
N#[C;H0;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[NH;D2;+0:6]-[C:7]-[C:8]-[NH2;D1;+0:9]>>[C;D1;H3:5]-[N;H0;D3;+0:6]1-[C:7]-[C:8]-[N;H0;D2;+0:9]=[C;H0;D3;+0:1]-1-[c:2](:[c:3]):[c:4]
null
[]
null
null
8
HOUR
To a lotion of the compound of N-{2-[N-(5-chloro(2-pyridyl))carbamoyl]-4-methylphenyl}(4-cyanophenyl)carboxamide (830 mg, 2.1 mmol) in anhydrous methanol (5 ml) and ethyl acetate (10 ml) was saturated with hydrogen chloride gas at 0° C. The mixture was stirred at r.t. overnight. After the evaporated the solvent, the re...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine.Secondary amine
Tertiary amine
null
C1=NCC[NH]1
c1ccccc1.c1ccccc1.C1=NCC[NH]1.c1ccncc1
Other
CO.C(C)(=O)OCC
null
8
CNCCN.Cc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1>CO.C(C)(=O)OCC>Cc1ccc(NC(=O)c2ccc(C3=NCCN3C)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a210a4371d564766a8f0071baf727a04
COc1cc(C(=O)O)c([N+](=O)[O-])c(OC)c1OC.Nc1ccc(Br)cn1>>COc1cc(C(=O)Nc2ccc(Br)cn2)c([N+](=O)[O-])c(OC)c1OC
COC=1C(=C(C(=O)O)C=C(C1OC)OC)[N+](=O)[O-].C(C(=O)Cl)(=O)Cl.NC1=NC=C(C=C1)Br.N1=CC=CC=C1>>BrC=1C=CC(=NC1)NC(=O)C1=C(C(=C(C(=C1)OC)OC)OC)[N+](=O)[O-]
O[C:6]([c:5]1[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH3:25])[c:20]([O:21][CH3:22])[c:16]1[N+:17](=[O:18])[O-:19])=[O:7].[NH2:8][c:9]1[cH:10][cH:11][c:12]([Br:13])[cH:14][n:15]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][n:15]2)[c:16]([N+:17](=[O:18])[O-:19])[c:20]([O:21...
COc1cc(C(=O)O)c([N+](=O)[O-])c(OC)c1OC.Nc1ccc(Br)cn1
COc1cc(C(=O)Nc2ccc(Br)cn2)c([N+](=O)[O-])c(OC)c1OC
null
CN(C=O)C
ClCCl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccn1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:3](:[c:4]):[c:5]
null
[]
null
null
2
HOUR
To a solution of 3,4,5-trimethoxy-2-nitrobenzoic acid (0.5 g, 1.95 mmol) in dichloromethane (5 ml) was added oxalyl chloride (0.34 ml, 3.9 mmol) and a few drops of dimethylformamide. The mixture was stirred at r.t. for 2 hrs. After the evaporation of the solvent, the residue was dissolved in dichloromethane (5 ml). 2-a...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccncc1
HO-
CN(C=O)C.ClCCl
null
2
COc1cc(C(=O)O)c([N+](=O)[O-])c(OC)c1OC.Nc1ccc(Br)cn1>CN(C=O)C.ClCCl>COc1cc(C(=O)Nc2ccc(Br)cn2)c([N+](=O)[O-])c(OC)c1OC
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f6ff2f43c9804f5a977194ab3f2eb2d2
COc1cc(C(=O)Nc2ccc(Br)cn2)c([N+](=O)[O-])c(OC)c1OC>>COc1cc(C(=O)Nc2ccc(Br)cn2)c(N)c(OC)c1OC
BrC=1C=CC(=NC1)NC(=O)C1=C(C(=C(C(=C1)OC)OC)OC)[N+](=O)[O-]>>NC1=C(C=C(C(=C1OC)OC)OC)C(=O)NC1=NC=C(C=C1)Br
O=[N+:17]([O-])[c:16]1[c:5]([C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][n:15]2)[cH:4][c:3]([O:2][CH3:1])[c:21]([O:22][CH3:23])[c:18]1[O:19][CH3:20]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][n:15]2)[c:16]([NH2:17])[c:18]([O:19][CH3:20])[c:21]1[O:22][CH...
COc1cc(C(=O)Nc2ccc(Br)cn2)c([N+](=O)[O-])c(OC)c1OC
COc1cc(C(=O)Nc2ccc(Br)cn2)c(N)c(OC)c1OC
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
C(C)(=O)OCC
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
O=C(Nc1ccccn1)c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]-[C:5](-[#7:6])=[O;D1;H0:7]>>[#7:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
77.7
[{"value": 77.0, "product": "NC1=C(C=C(C(=C1OC)OC)OC)C(=O)NC1=NC=C(C=C1)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.7, "product": "NC1=C(C=C(C(=C1OC)OC)OC)C(=O)NC1=NC=C(C=C1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of the compound of N-(5-bromo(2-pyridyl))(3,4,5-trimethoxy-2-nitrophenyl)carboxamide (790 mg, 1.92 mmol) in ethyl acetate (5 ml) was added tin chloride (II) hydrate (1.73 g, 7.67 mmol). The mixture was stirred under reflux condition for 2 hrs. After filtered by Celite, the filtrate was added 1N sodium hyd...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccncc1
Other
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.C(C)(=O)OCC
null
null
COc1cc(C(=O)Nc2ccc(Br)cn2)c([N+](=O)[O-])c(OC)c1OC>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.C(C)(=O)OCC>COc1cc(C(=O)Nc2ccc(Br)cn2)c(N)c(OC)c1OC
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-958271ca3f154d7696885840af850fec
CNCCN.COc1cc(C(=O)Nc2ccc(Br)cn2)c(NC(=O)c2ccc(C#N)cc2)c(OC)c1OC>>COc1cc(C(=O)Nc2ccc(Br)cn2)c(NC(=O)c2ccc(C3=NCCN3C)cc2)c(OC)c1OC
BrC=1C=CC(=NC1)NC(=O)C1=CC(=C(C(=C1NC(=O)C1=CC=C(C=C1)C#N)OC)OC)OC.Cl.CNCCN>>BrC=1C=CC(=NC1)NC(=O)C1=CC(=C(C(=C1NC(=O)C1=CC=C(C=C1)C=1N(CCN1)C)OC)OC)OC
[NH2:25][CH2:26][CH2:27][NH:28][CH3:29].N#[C:24][c:23]1[cH:22][cH:21][c:20]([C:18]([NH:17][c:16]2[c:5]([C:6](=[O:7])[NH:8][c:9]3[cH:10][cH:11][c:12]([Br:13])[cH:14][n:15]3)[cH:4][c:3]([O:2][CH3:1])[c:35]([O:36][CH3:37])[c:32]2[O:33][CH3:34])=[O:19])[cH:31][cH:30]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[NH:8][c:9]...
CNCCN.COc1cc(C(=O)Nc2ccc(Br)cn2)c(NC(=O)c2ccc(C#N)cc2)c(OC)c1OC
COc1cc(C(=O)Nc2ccc(Br)cn2)c(NC(=O)c2ccc(C3=NCCN3C)cc2)c(OC)c1OC
null
null
CO.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
c60ad675bbef0aae4bc6f7e7229a0d6b3b6a784179e30b9e067ffd6151067a5c
4290e5b2bf07838a6d478b39c42778e9467fef0b3ea75c8d873e295925a35d9e
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(C2=NCCN2)cc1
N#[C;H0;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[NH;D2;+0:6]-[C:7]-[C:8]-[NH2;D1;+0:9]>>[C;D1;H3:5]-[N;H0;D3;+0:6]1-[C:7]-[C:8]-[N;H0;D2;+0:9]=[C;H0;D3;+0:1]-1-[c:2](:[c:3]):[c:4]
32
[{"value": 32.0, "product": "BrC=1C=CC(=NC1)NC(=O)C1=CC(=C(C(=C1NC(=O)C1=CC=C(C=C1)C=1N(CCN1)C)OC)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 31.7, "product": "BrC=1C=CC(=NC1)NC(=O)C1=CC(=C(C(=C1NC(=O)C1=CC=C(C=C1)C=1N(CCN1)C)OC)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of the compound of N-{6-[N-(5-bromo(2-pyridyl))carbamoyl]-2,3,4-trimethoxyphenyl}(4-cyanophenyl)carboxamide (680 mg, 1.33 mmol) in anhydrous methanol (5 ml) and ethyl acetate (10 ml) was saturated with hydrogen chloride gas at 0° C. The mixture was stirred at r.t. overnight. After the evaporated the solve...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine.Secondary amine
Tertiary amine
null
C1=NCC[NH]1
c1ccccc1.c1ccncc1.c1ccccc1.C1=NCC[NH]1
Other
CO.C(C)(=O)OCC
null
8
CNCCN.COc1cc(C(=O)Nc2ccc(Br)cn2)c(NC(=O)c2ccc(C#N)cc2)c(OC)c1OC>CO.C(C)(=O)OCC>COc1cc(C(=O)Nc2ccc(Br)cn2)c(NC(=O)c2ccc(C3=NCCN3C)cc2)c(OC)c1OC
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-432e5e98f72e4755bd8a27be74a5a6c8
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)O)cc1.Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1>>CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
C(C)(C)(C)NS(=O)(=O)C1=C(C=CC=C1)C1=CC=C(C(=O)O)C=C1.C(C(=O)Cl)(=O)Cl.NC1=C(C=C(C=C1)Cl)C(=O)NC1=NC=C(C=C1)Cl.N1=CC=CC=C1>>C(C)(C)(C)NS(=O)(=O)C1=C(C=CC=C1)C1=CC=C(C=C1)C(=O)NC1=C(C=C(C=C1)Cl)C(=O)NC1=NC=C(C=C1)Cl
O[C:19]([c:18]1[cH:17][cH:16][c:15](-[c:14]2[c:9]([S:6]([NH:5][C:2]([CH3:1])([CH3:3])[CH3:4])(=[O:7])=[O:8])[cH:10][cH:11][cH:12][cH:13]2)[cH:40][cH:39]1)=[O:20].[NH2:21][c:22]1[cH:23][cH:24][c:25]([Cl:26])[cH:27][c:28]1[C:29](=[O:30])[NH:31][c:32]1[cH:33][cH:34][c:35]([Cl:36])[cH:37][n:38]1>>[CH3:1][C:2]([CH3:3])([CH3...
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)O)cc1.Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
null
CN(C=O)C
ClCCl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#7:6]-[C:7](=[O;D1;H0:8])-[c:9]:[c:10](-[NH2;D1;+0:11]):[c:12]>>[#7:6]-[C:7](=[O;D1;H0:8])-[c:9]:[c:10](-[NH;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]):[c:12]
null
[]
null
null
2
HOUR
To a solution of 4-{2-{[(tert-butyl)amino}sulfonyl}phenyl}benzoic acid (167 mg, 0.5 mmol) in dichloromethane (5 ml) was added oxalyl chloride (0.09 ml, 1 mmol) and a few drops of dimethylformamide. The mixture was stirred at r.t. for 2 hrs. After the evaporation of the solvent, the residue was dissolved in dichlorometh...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccncc1
HO-
CN(C=O)C.ClCCl
null
2
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)O)cc1.Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1>CN(C=O)C.ClCCl>CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-51b3463d197f4d3383bc60335e37cfca
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1>>NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
C(C)(C)(C)NS(=O)(=O)C1=C(C=CC=C1)C1=CC=C(C=C1)C(=O)NC1=C(C=C(C=C1)Cl)C(=O)NC1=NC=C(C=C1)Cl>>ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)Cl)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)S(N)(=O)=O
CC(C)(C)[NH:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1-[c:11]1[cH:12][cH:13][c:14]([C:15](=[O:16])[NH:17][c:18]2[cH:19][cH:20][c:21]([Cl:22])[cH:23][c:24]2[C:25](=[O:26])[NH:27][c:28]2[cH:29][cH:30][c:31]([Cl:32])[cH:33][n:34]2)[cH:35][cH:36]1>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][cH:8][cH:9...
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
null
null
FC(C(=O)O)(F)F
Deprotection
Tert-butyl deprotection of amine
f7e1da1b4c254f1e6d5afbf8cb56733a4fabd145b80e971e3b7e31007de9e7d6
278d0fb11b582c058ac903379d7fbe11ab8c395937a204965031cf0c344845a9
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(-c2ccccc2)cc1
C-C(-C)(-C)-[NH;D2;+0:1]-[#16:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5]>>[NH2;D1;+0:1]-[#16:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5]
25
[{"value": 25.0, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)Cl)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)S(N)(=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
The mixture of the compound of (2-{[4-(2-{[(tert-butyl)amino]sulfonyl}phenyl)phenyl]carbonylamino}-5-chlorophenyl)-N-(5-chloro(2-pyridyl))carboxamide example 12 (0.5 mmol) in trifluoroacetic acid (5 ml) was stirred at r.t. for 5 hrs. After the evaporation of solvent, the crude residue was purified by RP-HPLC to give N-...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide
Sulfonamide
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccncc1
Other
FC(C(=O)O)(F)F
null
5
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1>FC(C(=O)O)(F)F>NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-99c3ae0889fe4420b0409a609b3092ec
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>>N=C(N)c1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
S.ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)C#N.N1=CC=CC=C1.CI>>ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)C(=N)N
[N:1]#[C:2][c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1-[c:10]1[cH:11][cH:12][c:13]([C:14](=[O:15])[NH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]2[C:23](=[O:24])[NH:25][c:26]2[cH:27][cH:28][c:29]([Cl:30])[cH:31][n:32]2)[cH:33][cH:34]1>>[NH:1]=[C:2]([NH2:3])[c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1-[c:10]1[cH:11][cH:12][c:13]([C:1...
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
N=C(N)c1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
null
null
C(C)(=O)O.CO.CC(=O)C.CCN(CC)CC
Functional Group Addition
OtherReaction
b3aaef1538bea73aa85740ccbb089c1b6ca4b164a10fd32235acb6c78d1de6d9
d1a81d2cc57b1a744f94f80261b8629cf532e8b73012860cc8db4db5903fee1a
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(-c2ccccc2)cc1
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[N;D1;H2:6]-[C;H0;D3;+0:2](=[NH;D1;+0:1])-[c:3](:[c:4]):[c:5]
15
[{"value": 15.0, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)C(=N)N", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
DAY
A stream of H2S (g) was bubbled through a 0° C. solution of N-{2-[N-(5-chloro(2-pyridyl))carbamoyl]phenyl}[4-(2-cyanophenyl)phenyl]carboxamide (100 mg, 0.22 mmol, 1.0 equiv.) in 9 mL pyridine and 1 mL NEt3 until saturation. The mixture was stirred at rt for 1 day and evaporated. The resulting residue was treated with M...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccncc1
Other
C(C)(=O)O.CO.CC(=O)C.CCN(CC)CC
null
24
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>C(C)(=O)O.CO.CC(=O)C.CCN(CC)CC>N=C(N)c1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e9e8ade37fa045e6b205871fa78eff47
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1.NO>>O=C(Nc1ccccc1C(=O)Nc1ccc(Cl)cn1)c1ccc(-c2ccccc2C=NNO)cc1
ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)C#N.Cl.ON.C(C)N(CC)CC>>ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)C=NNO
[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1[C:10](=[O:11])[NH:12][c:13]1[cH:14][cH:15][c:16]([Cl:17])[cH:18][n:19]1)[c:20]1[cH:21][cH:22][c:23](-[c:24]2[cH:25][cH:26][cH:27][cH:28][c:29]2[C:30]#[N:31])[cH:34][cH:35]1.[NH2:32][OH:33]>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1[C:10](=[O:11])[NH:12...
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1.NO
O=C(Nc1ccccc1C(=O)Nc1ccc(Cl)cn1)c1ccc(-c2ccccc2C=NNO)cc1
null
null
C(C)O
Miscellaneous
OtherReaction
5ebc8ae9c43671ddb0100b0cbc1ec0c40d1e187e38be7171f745b68f0dc6a2a1
58f66636c1d89ede1b1e759542791677a2888499f20f253f7f8ee20c2e377b3e
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(-c2ccccc2)cc1
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[O;D1;H1:7]>>[O;D1;H1:7]-[NH;D2;+0:6]-[N;H0;D2;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]
27.5
[{"value": 27.5, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)C=NNO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 27.4, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)C=NNO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
6
DAY
A mixture of N-{2-[N-(5-chloro(2-pyridyl))carbamoyl]phenyl}[4-(2-cyanophenyl)phenyl]carboxamide (14 mg, 0.03 mmol, 1.0 equiv.), hydroxyamine hydrochloride (6.25 mg, 0.09 mmol, 3.0 equiv.) and triethyl amine (0.03 mL, 0.3 mmol, 10.0 equiv.) in ethanol (3 mL) was stirred at rt for 6 days, concentrated and HPLC (C18 rever...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine
Hydrazone
null
null
c1ccccc1.c1ccncc1.c1ccccc1.c1ccccc1
null
C(C)O
null
144
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1.NO>C(C)O>O=C(Nc1ccccc1C(=O)Nc1ccc(Cl)cn1)c1ccc(-c2ccccc2C=NNO)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e07f07c233194fffb8fe4e88631f016a
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>>NCc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)C#N.[BH4-].[Na+]>>NCC1=C(C=CC=C1)C1=CC=C(C=C1)C(=O)NC1=C(C=CC=C1)C(NC1=NC=C(C=C1)Cl)=O
[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[c:9]1[cH:10][cH:11][c:12]([C:13](=[O:14])[NH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[C:22](=[O:23])[NH:24][c:25]2[cH:26][cH:27][c:28]([Cl:29])[cH:30][n:31]2)[cH:32][cH:33]1>>[NH2:1][CH2:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[c:9]1[cH:10][cH:11][c:12]([C:13](=[O:14...
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
NCc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
null
[Co](Cl)Cl
CN(C)C=O
Reduction
Reduction of nitrile to amine
65bec2d9f430701d30dc9fcbe1c5418f3dfa174d67be035c50edfc71895dc9c7
e8d1bc928b94bd4f5bf4b23363ce8f88b1ce7d146ba93829e7b8ad8dbe0007a7
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(-c2ccccc2)cc1
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[NH2;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
43.1
[{"value": 43.0, "product": "NCC1=C(C=CC=C1)C1=CC=C(C=C1)C(=O)NC1=C(C=CC=C1)C(NC1=NC=C(C=C1)Cl)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 43.1, "product": "NCC1=C(C=CC=C1)C1=CC=C(C=C1)C(=O)NC1=C(C=CC=C1)C(NC1=NC=C(C=C1)Cl)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
DAY
A mixture of N-{2-[N-(5-chloro(2-pyridyl))carbamoyl]phenyl}[4-(2-cyanophenyl)phenyl]carboxamide (200 mg, 0.442 mmol, 1.0 equiv.), cobalt chloride (86 mg, 0.664 mmol, 1.5 equiv.) and sodium borohydride (50 mg, 1.33 mmol, 3.0 equiv.) in DMF (15 mL) was stirred at 0° C. to rt for 3 days. The reaction was quenched with ice...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccncc1
null
[Co](Cl)Cl.CN(C)C=O
null
72
N#Cc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>[Co](Cl)Cl.CN(C)C=O>NCc1ccccc1-c1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a33abca967ae4d04826e526108b5ff3e
N#Cc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>>NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)C#N.[BH4-].[Na+]>>NCC1=CC=C(C=C1)C(=O)NC1=C(C=CC=C1)C(NC1=NC=C(C=C1)Cl)=O
[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[NH:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[C:16](=[O:17])[NH:18][c:19]2[cH:20][cH:21][c:22]([Cl:23])[cH:24][n:25]2)[cH:26][cH:27]1>>[NH2:1][CH2:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[NH:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[C:16](=[O:17])[NH:18][c:19]2[cH:20...
N#Cc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
null
[Co](Cl)Cl
CN(C)C=O
Reduction
Reduction of nitrile to amine
65bec2d9f430701d30dc9fcbe1c5418f3dfa174d67be035c50edfc71895dc9c7
e8d1bc928b94bd4f5bf4b23363ce8f88b1ce7d146ba93829e7b8ad8dbe0007a7
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccccc1
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[NH2;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
32.3
[{"value": 30.0, "product": "NCC1=CC=C(C=C1)C(=O)NC1=C(C=CC=C1)C(NC1=NC=C(C=C1)Cl)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 32.3, "product": "NCC1=CC=C(C=C1)C(=O)NC1=C(C=CC=C1)C(NC1=NC=C(C=C1)Cl)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2.5
HOUR
A mixture of N-{2-[N-(5-chloro(2-pyridyl))carbamoyl]phenyl}(4-cyanophenyl)carboxamide (1 g, 2.6 mmol, 1.0 equiv.), cobalt chloride (0.5 g, 3.85 mmol, 1.5 equiv.) and sodium borohydride (0.295 g, 7.8 mmol, 3.0 equiv.) in DMF (20 mL) was stirred at 0° C. to rt for 2.5 hr. The reaction was quenched with ice cubes, diluted...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccncc1
null
[Co](Cl)Cl.CN(C)C=O
null
2.5
N#Cc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>[Co](Cl)Cl.CN(C)C=O>NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-1546da5dfd1f4983ae13230c459a50de
CSC1=NCCN1.NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>>O=C(Nc1ccccc1C(=O)Nc1ccc(Cl)cn1)c1ccc(CNC2=NCCN2)cc1
NCC1=CC=C(C=C1)C(=O)NC1=C(C=CC=C1)C(NC1=NC=C(C=C1)Cl)=O.I.CSC=1NCCN1.C(C)N(CC)CC>>ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)CNC=1NCCN1
CS[C:26]1=[N:27][CH2:28][CH2:29][NH:30]1.[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1[C:10](=[O:11])[NH:12][c:13]1[cH:14][cH:15][c:16]([Cl:17])[cH:18][n:19]1)[c:20]1[cH:21][cH:22][c:23]([CH2:24][NH2:25])[cH:31][cH:32]1>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1[C:10](=[O:11])[NH:12][c:13]1[cH:14]...
CSC1=NCCN1.NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
O=C(Nc1ccccc1C(=O)Nc1ccc(Cl)cn1)c1ccc(CNC2=NCCN2)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
b8b2c7cb02682d6c06684e6c7b2dfb49c6d9023dd6b43e4d41769a82c503b02f
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(CNC2=NCCN2)cc1
C-S-[C;H0;D3;+0:1]1=[#7:2]-[C:3]-[C:4]-[#7:5]-1.[NH2;D1;+0:6]-[C:7]-[c:8]>>[c:8]-[C:7]-[NH;D2;+0:6]-[C;H0;D3;+0:1]1=[#7:2]-[C:3]-[C:4]-[#7:5]-1
15
[{"value": 15.0, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)CNC=1NCCN1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 14.3, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)CNC=1NCCN1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A mixture of [4-(aminomethyl)phenyl]-N-{2-[N-(5-chloro(2-pyridyl))carbamoyl]phenyl}carboxamide (80 mg, 0.21 mmol), 2-methylthio-2-imidazoline hydriodide (77 mg, 0.315 mmol, 1.5 equiv.) and triethyl amine (0.5 mL) in 1 mL DMF was stirred at room temperature overnight, concentrated to dryness and HPLC (C18 reversed phase...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
C1=NCCN1
C1=NCCN1
c1ccccc1.c1ccncc1.c1ccccc1.C1=NCCN1
Other
CN(C)C=O
null
8
CSC1=NCCN1.NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>CN(C)C=O>O=C(Nc1ccccc1C(=O)Nc1ccc(Cl)cn1)c1ccc(CNC2=NCCN2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-30a4b1acec744fe7ac7ca91be30e3f4f
CSC1=NCCN1C.NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>>CN1CCN=C1NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
NCC1=CC=C(C=C1)C(=O)NC1=C(C=CC=C1)C(NC1=NC=C(C=C1)Cl)=O.CN1C(=NCC1)SC.CCN(CC)CC>>ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)CNC=1N(CCN1)C
CS[C:6]1=[N:5][CH2:4][CH2:3][N:2]1[CH3:1].[NH2:7][CH2:8][c:9]1[cH:10][cH:11][c:12]([C:13](=[O:14])[NH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[C:22](=[O:23])[NH:24][c:25]2[cH:26][cH:27][c:28]([Cl:29])[cH:30][n:31]2)[cH:32][cH:33]1>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]=[C:6]1[NH:7][CH2:8][c:9]1[cH:10][cH:11][c:12]([C:1...
CSC1=NCCN1C.NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
CN1CCN=C1NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
null
null
N1=CC=CC=C1
Heteroatom Alkylation and Arylation
OtherReaction
3d9229dd690869c9ac61e6b6820af19abd0e765828a31068efa43748fe7d0ebd
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccc(CNC2=NCCN2)cc1
C-S-[C;H0;D3;+0:1]1=[#7:2]-[C:3]-[C:4]-[#7:5]-1-[C;D1;H3:6].[NH2;D1;+0:7]-[C:8]-[c:9]>>[C;D1;H3:6]-[#7:5]1-[C:4]-[C:3]-[#7:2]=[C;H0;D3;+0:1]-1-[NH;D2;+0:7]-[C:8]-[c:9]
65
[{"value": 65.0, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)CNC=1N(CCN1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.6, "product": "ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC=C1)NC(=O)C1=CC=C(C=C1)CNC=1N(CCN1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
8
HOUR
A mixture of [4-(aminomethyl)phenyl]-N-{2-[N-(5-chloro(2-pyridyl))carbamoyl]phenyl}carboxamide (74 mg, 0.195 mmol), 1-methyl-2-methylthio-2-imidazoline (25 mg, 0.195 mmol), NEt3 (2 mL) and pyridine (5 mL) was stirred at 80° C. overnight, concentrated and HPLC (C18 reversed phase) eluting with 0.1% TFA in H2O/CH3CN gave...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
C1=NCC[NH]1
C1=NCC[NH]1
C1=NCC[NH]1.c1ccccc1.c1ccccc1.c1ccncc1
Other
N1=CC=CC=C1
80
8
CSC1=NCCN1C.NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1>N1=CC=CC=C1>CN1CCN=C1NCc1ccc(C(=O)Nc2ccccc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f5114e14d5ad490499ca327d32a64c19
Nc1ccc(Br)cn1.O=C(O)c1cc(F)ccc1[N+](=O)[O-]>>O=C(Nc1ccc(Br)cn1)c1cc(F)ccc1[N+](=O)[O-]
FC=1C=CC(=C(C(=O)O)C1)[N+](=O)[O-].NC1=NC=C(C=C1)Br.P(=O)(Cl)(Cl)Cl>>BrC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)F)[N+](=O)[O-]
[NH2:3][c:4]1[cH:5][cH:6][c:7]([Br:8])[cH:9][n:10]1.O[C:2](=[O:1])[c:11]1[cH:12][c:13]([F:14])[cH:15][cH:16][c:17]1[N+:18](=[O:19])[O-:20]>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][c:7]([Br:8])[cH:9][n:10]1)[c:11]1[cH:12][c:13]([F:14])[cH:15][cH:16][c:17]1[N+:18](=[O:19])[O-:20]
Nc1ccc(Br)cn1.O=C(O)c1cc(F)ccc1[N+](=O)[O-]
O=C(Nc1ccc(Br)cn1)c1cc(F)ccc1[N+](=O)[O-]
null
null
N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccn1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:3](:[c:4]):[c:5]
68.1
[{"value": 68.0, "product": "BrC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)F)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.1, "product": "BrC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)F)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-fluoro-2-nitrobenzoic acid (10.0 g, 54 mmol, 1.0 equiv), 2-amino-5-bromopyridine (12.2 g, 1.3 equiv), in 80 mL of pyridine was treated with phosphorous oxychloride (25.3 g, 3.0 equiv) for 30 min. The volatile was evaporated and the residue was redissolved into EtOAc., washed with 1N HCl, saturated aqueo...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccncc1.c1ccccc1
HO-
N1=CC=CC=C1
null
null
Nc1ccc(Br)cn1.O=C(O)c1cc(F)ccc1[N+](=O)[O-]>N1=CC=CC=C1>O=C(Nc1ccc(Br)cn1)c1cc(F)ccc1[N+](=O)[O-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-82bf9b1954454b0fb3915cb4422c3e72
COc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1.NO>>COc1ccc(NC(=O)c2ccc(C(N)=NO)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1
ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)OC)NC(=O)C1=CC=C(C=C1)C#N.Cl.ON.CCN(CC)CC>>NC(C1=CC=C(C=C1)C(=O)NC1=C(C=C(C=C1)OC)C(=O)NC1=NC=C(C=C1)Cl)=NO
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH:7][C:8](=[O:9])[c:10]2[cH:11][cH:12][c:13]([C:14]#[N:15])[cH:18][cH:19]2)[c:20]([C:21](=[O:22])[NH:23][c:24]2[cH:25][cH:26][c:27]([Cl:28])[cH:29][n:30]2)[cH:31]1.[NH2:16][OH:17]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH:7][C:8](=[O:9])[c:10]2[cH:11][cH:12][c:13]([C:14]([NH2:15])=[...
COc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1.NO
COc1ccc(NC(=O)c2ccc(C(N)=NO)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1
null
null
CCO
Heteroatom Alkylation and Arylation
Amidoxime from nitrile and hydroxylamine
5f2123b5002b6939ec57e4f55921371a47c78c3ff253c724d87881638fedcd4f
ad3f1127a4d99506976df608684863fb1e08b35faede2d4e31cf4ca96393cd2e
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccccc1
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[O;D1;H1:7]>>[NH2;D1;+0:1]-[C;H0;D3;+0:2](=[N;H0;D2;+0:6]-[O;D1;H1:7])-[c:3](:[c:4]):[c:5]
null
[]
60
CELSIUS
8
HOUR
To a suspension of compound N-(5-chloro(2-pyridyl)) {2-[(4-cyanophenyl)carbonylamino]-5-methoxyphenyl}carboxamide (150 mg) in EtOH (10 mL) was added hydroxyamine hydrochloride (80 mg) and Et3N (200 μL). The mixture was stirred at 60° C. overnight and the reaction was complete. The solvent was evaporated and the crude m...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine
Primary amine.Oxime
null
null
c1ccccc1.c1ccccc1.c1ccncc1
null
CCO
60
8
COc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1.NO>CCO>COc1ccc(NC(=O)c2ccc(C(N)=NO)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-972574041085479993d5ed752d7b11c2
COc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1>>N#Cc1ccc(C(=O)Nc2ccc(O)cc2C(=O)Nc2ccc(Cl)cn2)cc1
ClC=1C=CC(=NC1)NC(=O)C1=C(C=CC(=C1)OC)NC(=O)C1=CC=C(C=C1)C#N.B(Br)(Br)Br>>ClC=1C=CC(=NC1)NC(=O)C1=CC(=CC=C1NC(=O)C1=CC=C(C=C1)C#N)O
C[O:14][c:13]1[cH:12][cH:11][c:10]([NH:9][C:7]([c:6]2[cH:5][cH:4][c:3]([C:2]#[N:1])[cH:28][cH:27]2)=[O:8])[c:16]([C:17](=[O:18])[NH:19][c:20]2[cH:21][cH:22][c:23]([Cl:24])[cH:25][n:26]2)[cH:15]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[NH:9][c:10]2[cH:11][cH:12][c:13]([OH:14])[cH:15][c:16]2[C:17](=[O:18])[NH:1...
COc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1
N#Cc1ccc(C(=O)Nc2ccc(O)cc2C(=O)Nc2ccc(Cl)cn2)cc1
null
null
C(Cl)Cl
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
90
[{"value": 90.0, "product": "ClC=1C=CC(=NC1)NC(=O)C1=CC(=CC=C1NC(=O)C1=CC=C(C=C1)C#N)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
72
HOUR
To a suspension of compound N-(5-chloro(2-pyridyl)){2-[(4-cyanophenyl)-carbonylamino]-5-methoxyphenyl}carboxamide (500 mg, 1.2 mmol) in DCM (100 mL) at −78° C. was added BBr3 (2 mL). The mixture was stirred at ambient temperatures for 72 hours. The solid was collected by filtration and was washed by DCM and water, drie...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccccc1.c1ccccc1.c1ccncc1
Other
C(Cl)Cl
null
72
COc1ccc(NC(=O)c2ccc(C#N)cc2)c(C(=O)Nc2ccc(Cl)cn2)c1>C(Cl)Cl>N#Cc1ccc(C(=O)Nc2ccc(O)cc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-94770809738c4b598943bd373eeaa201
Nc1ccc(Cl)cn1.O=c1[nH]c2ccc(Cl)cc2c(=O)o1>>Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1
ClC1=CC=C2C(C(=O)OC(N2)=O)=C1.NC1=NC=C(C=C1)Cl.C[Si](C)(C)[N-][Si](C)(C)C.[K+].C1(=CC=CC=C1)C>>NC1=C(C=C(C=C1)Cl)C(=O)NC1=NC=C(C=C1)Cl
[NH2:11][c:12]1[cH:13][cH:14][c:15]([Cl:16])[cH:17][n:18]1.O=c1o[c:9](=[O:10])[c:8]2[c:2]([nH:1]1)[cH:3][cH:4][c:5]([Cl:6])[cH:7]2>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[cH:7][c:8]1[C:9](=[O:10])[NH:11][c:12]1[cH:13][cH:14][c:15]([Cl:16])[cH:17][n:18]1
Nc1ccc(Cl)cn1.O=c1[nH]c2ccc(Cl)cc2c(=O)o1
Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1
null
null
O1CCCC1
Acylation
OtherReaction
b4c245015e48b9b60756b62e3f8985928af86452315d98417a25faace320d9ae
b609a70ccab739990a9ccc4ea2adcc77011bcd0c07154489a12420f7c0e7382e
O=C(Nc1ccccn1)c1ccccc1
O=c1:[nH;D2;+0:1]:[c:2](:[c:3]):[c:4](:[c:5]):[c;H0;D3;+0:6](=[O;D1;H0:7]):o:1.[NH2;D1;+0:8]-[c:9](:[c:10]):[#7;a:11]:[c:12]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4](-[C;H0;D3;+0:6](=[O;D1;H0:7])-[NH;D2;+0:8]-[c:9](:[c:10]):[#7;a:11]:[c:12]):[c:5]
null
[]
-78
CELSIUS
0.5
HOUR
To a solution of 2-amino-5-chloropyridine (787 mg, 6.1 mmol) in tetrahydrofuran (5 ml) was added 0.5M potassium bis(trimethylsilyl)amide in toluene (20 ml, 10.1 mmol) dropwise at −78° C. After stirred for additional 0.5 hr at −78° C., the mixture was added 5-chloroisatoic anhydride (1 g, 5.1 mmol) at −78° C. The mixtur...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Secondary amide.Primary amine
c1ccc2ncocc2c1
c1ccccc1
c1ccccc1.c1ccncc1
Other
O1CCCC1
-78
0.5
Nc1ccc(Cl)cn1.O=c1[nH]c2ccc(Cl)cc2c(=O)o1>O1CCCC1>Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-48fd1d68fa0249118488f86d53172bd6
N#Cc1ccc(C(=O)O)c(F)c1.Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1>>N#Cc1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)c(F)c1
FC1=C(C(=O)O)C=CC(=C1)C#N.NC1=C(C=C(C=C1)Cl)C(=O)NC1=NC=C(C=C1)Cl.N1=CC=CC=C1>>ClC1=CC(=C(C=C1)NC(=O)C1=C(C=C(C=C1)C#N)F)C(NC1=NC=C(C=C1)Cl)=O
O[C:7]([c:6]1[cH:5][cH:4][c:3]([C:2]#[N:1])[cH:29][c:27]1[F:28])=[O:8].[NH2:9][c:10]1[cH:11][cH:12][c:13]([Cl:14])[cH:15][c:16]1[C:17](=[O:18])[NH:19][c:20]1[cH:21][cH:22][c:23]([Cl:24])[cH:25][n:26]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[NH:9][c:10]2[cH:11][cH:12][c:13]([Cl:14])[cH:15][c:16]2[C:17](=[O:18]...
N#Cc1ccc(C(=O)O)c(F)c1.Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1
N#Cc1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)c(F)c1
null
null
ClCCl.S(=O)(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccc1C(=O)Nc1ccccn1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#7:6]-[C:7](=[O;D1;H0:8])-[c:9]:[c:10](-[NH2;D1;+0:11]):[c:12]>>[#7:6]-[C:7](=[O;D1;H0:8])-[c:9]:[c:10](-[NH;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]):[c:12]
111.3
[{"value": 78.0, "product": "ClC1=CC(=C(C=C1)NC(=O)C1=C(C=C(C=C1)C#N)F)C(NC1=NC=C(C=C1)Cl)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 111.3, "product": "ClC1=CC(=C(C=C1)NC(=O)C1=C(C=C(C=C1)C#N)F)C(NC1=NC=C(C=C1)Cl)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of 2-fluoro-4-cyanobenzoic acid (1 g, 6.06 mmol) in thionyl chloride (5 ml) was refluxed for 2 hr. After concentration, the residue was dissolved in dichloromethane (5 ml). And a solution of the compound of (2-amino-5-chlorophenyl)-N-(5-chloro(2-pyridyl))carboxamide (1.2 g, 4.25 mmol) in dichloromethane (10 ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccncc1
HO-
ClCCl.S(=O)(Cl)Cl
null
8
N#Cc1ccc(C(=O)O)c(F)c1.Nc1ccc(Cl)cc1C(=O)Nc1ccc(Cl)cn1>ClCCl.S(=O)(Cl)Cl>N#Cc1ccc(C(=O)Nc2ccc(Cl)cc2C(=O)Nc2ccc(Cl)cn2)c(F)c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a52a3fbcacdd46b986124493621699a2
COC(=O)c1sccc1N.N#Cc1ccc(C(=O)Cl)cc1>>COC(=O)c1sccc1NC(=O)c1ccc(C#N)cc1
C(#N)C1=CC=C(C(=O)Cl)C=C1.NC1=C(SC=C1)C(=O)OC.C(C)N(CC)CC>>C(#N)C1=CC=C(C=C1)C(=O)NC1=C(SC=C1)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[c:5]1[s:6][cH:7][cH:8][c:9]1[NH2:10].Cl[C:11](=[O:12])[c:13]1[cH:14][cH:15][c:16]([C:17]#[N:18])[cH:19][cH:20]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[s:6][cH:7][cH:8][c:9]1[NH:10][C:11](=[O:12])[c:13]1[cH:14][cH:15][c:16]([C:17]#[N:18])[cH:19][cH:20]1
COC(=O)c1sccc1N.N#Cc1ccc(C(=O)Cl)cc1
COC(=O)c1sccc1NC(=O)c1ccc(C#N)cc1
null
null
ClCCl
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(Nc1ccsc1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[#16;a:10]:[c:11]:[c:12]:[c:13]:1-[NH2;D1;+0:14]>>[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[#16;a:10]:[c:11]:[c:12]:[c:13]:1-[NH;D2;+0:14]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
91
[{"value": 91.0, "product": "C(#N)C1=CC=C(C=C1)C(=O)NC1=C(SC=C1)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.5, "product": "C(#N)C1=CC=C(C=C1)C(=O)NC1=C(SC=C1)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
A mixture of 4-cyanobenzoyl chloride (1.0500 g, 6.4 mmol), methyl 3-aminothiophenecarboxylate (1.0000 g, 6.4 mmol), and triethylamine (1 mL, 7.0 mmol) in dichloromethane was stirred at room temperature for 18 hours. The mixture was poured into a separatory funnel and washed by 1 N HCl. The organic layers were combined,...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccsc1.c1ccccc1
HCl
ClCCl
null
18
COC(=O)c1sccc1N.N#Cc1ccc(C(=O)Cl)cc1>ClCCl>COC(=O)c1sccc1NC(=O)c1ccc(C#N)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-9aa9d5290cb44ccb99afcc55ad44795e
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Cl)cc1.Nc1ccsc1C(=O)Nc1cc(Cl)ccn1>>NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccsc2C(=O)Nc2ccc(Cl)cn2)cc1
C(C)(C)(C)NS(=O)(=O)C1=C(C=CC=C1)C1=CC=C(C(=O)Cl)C=C1.NC1=C(SC=C1)C(=O)NC1=NC=CC(=C1)Cl.N1=CC=CC=C1.ClCCl.ClCCl>>ClC=1C=CC(=NC1)NC(=O)C=1SC=CC1NC(=O)C1=CC=C(C=C1)C1=C(C=CC=C1)S(N)(=O)=O
CC(C)(C)[NH:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1-[c:11]1[cH:12][cH:13][c:14]([C:15](Cl)=[O:16])[cH:33][cH:34]1.[NH2:17][c:18]1[cH:19][cH:20][s:21][c:22]1[C:23](=[O:24])[NH:25][c:26]1[cH:27][c:29]([Cl:30])[cH:28][cH:31][n:32]1>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1-[c:...
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Cl)cc1.Nc1ccsc1C(=O)Nc1cc(Cl)ccn1
NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccsc2C(=O)Nc2ccc(Cl)cn2)cc1
null
null
null
Acylation
OtherReaction
62b79e27f73e217708be777171a101fdbc2ae1e8bb0a9b0fa120e1de8f226bfb
5bed3f68e2efbf0da9a9b01be7a80f098581b44c7deee6d8009e459217c3f840
O=C(Nc1ccsc1C(=O)Nc1ccccn1)c1ccc(-c2ccccc2)cc1
C-C(-C)(-C)-[NH;D2;+0:1]-[#16:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5].Cl-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10].[Cl;D1;H0:11]-[c;H0;D3;+0:12]1:[cH;D2;+0:13]:[c:14](-[#7:15]-[C:16](=[O;D1;H0:17])-[c:18]2:[#16;a:19]:[c:20]:[c:21]:[c:22]:2-[NH2;D1;+0:23]):[#7;a:24]:[cH;D2;+0:25]:[cH;D2;+0:26]:1>>[Cl;D1;H0:11]-[c;H...
null
[]
null
null
null
null
A solution of 4-(2-{[(tert-butyl)amino]sulfonyl}phenyl)benzoyl chloride (1 equiv), 3-amino-2-(4-chloro-2-pyridinyl)aminocarbonyl thiophene (1 equiv), pyridine (5 equiv) in dichloromethane was stirred at rt overnight. The mixture was diluted with dichloromethane, washed with water, dried over Na2SO4, filtered and evapor...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Sulfonamide.Aromatic halide.Primary amine
Sulfonamide.Aromatic halide.Secondary amide
c1ccncc1
c1ccncc1
c1ccccc1.c1ccccc1.c1ccsc1.c1ccncc1
HCl
null
null
null
CC(C)(C)NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Cl)cc1.Nc1ccsc1C(=O)Nc1cc(Cl)ccn1>>NS(=O)(=O)c1ccccc1-c1ccc(C(=O)Nc2ccsc2C(=O)Nc2ccc(Cl)cn2)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e3397632786e4f3d840b2b82c219eed2
CC1=CC(=O)OC1=O.Nc1ccc(Br)cn1>>CC1=CC(=O)N(c2ccc(Br)cn2)C1=O
C1(\C(\C)=C/C(=O)O1)=O.NC1=NC=C(C=C1)Br>>BrC=1C=CC(=NC1)N1C(C(=CC1=O)C)=O
O1[C:4](=[O:5])[CH:3]=[C:2]([CH3:1])[C:14]1=[O:15].[NH2:6][c:7]1[cH:8][cH:9][c:10]([Br:11])[cH:12][n:13]1>>[CH3:1][C:2]1=[CH:3][C:4](=[O:5])[N:6]([c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][n:13]2)[C:14]1=[O:15]
CC1=CC(=O)OC1=O.Nc1ccc(Br)cn1
CC1=CC(=O)N(c2ccc(Br)cn2)C1=O
null
null
C1(=CC=CC=C1)C
Acylation
OtherReaction
cab1acd179957d4f5c27ba23f314ee257f7d508deff2838c7964b1019063e651
2a4a20e639c386292668b0b265a8e1b50d707d5f0576437dc5ade3e7fd444d29
O=C1C=CC(=O)N1c1ccccn1
[C;D1;H3:1]-[C:2]1=[C:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-O-[C;H0;D3;+0:6]-1=[O;D1;H0:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[#7;a:11]:[c:12]>>[C;D1;H3:1]-[C:2]1=[C:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[N;H0;D3;+0:8](-[c:9](:[c:10]):[#7;a:11]:[c:12])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
71
[{"value": 71.0, "product": "BrC=1C=CC(=NC1)N1C(C(=CC1=O)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 70.8, "product": "BrC=1C=CC(=NC1)N1C(C(=CC1=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of citraconic anhydride (1.00 mL, 11.1 mmol) and 2-amino-5-bromopyridine (1.93 g, 11.2 mmol) in toluene (60 mL) was heated to reflux overnight. The solution was cooled down, filtered. The filtrate was concentrated in vacuo to give a solid (2.10 g, yield: 71%). MS 267 and 269 (M+H). Conditions: See reaction.no...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary amine
Substituted dicarboximide
C1=CCOC1
C1=CC[NH]C1
C1=CC[NH]C1.c1ccncc1
HO-
C1(=CC=CC=C1)C
null
null
CC1=CC(=O)OC1=O.Nc1ccc(Br)cn1>C1(=CC=CC=C1)C>CC1=CC(=O)N(c2ccc(Br)cn2)C1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-0cd93d207e004979a92ba2c0b525333b
N#Cc1cccc(O)c1.O=[N+]([O-])c1ccccc1F>>N#Cc1cccc(Oc2ccccc2[N+](=O)[O-])c1
FC1=C(C=CC=C1)[N+](=O)[O-].OC=1C=C(C#N)C=CC1.C(=O)([O-])[O-].[K+].[K+]>>[N+](=O)([O-])C1=C(OC=2C=C(C#N)C=CC2)C=CC=C1
[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([OH:8])[cH:18]1.F[c:9]1[cH:10][cH:11][cH:12][cH:13][c:14]1[N+:15](=[O:16])[O-:17]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[N+:15](=[O:16])[O-:17])[cH:18]1
N#Cc1cccc(O)c1.O=[N+]([O-])c1ccccc1F
N#Cc1cccc(Oc2ccccc2[N+](=O)[O-])c1
null
null
CCOC(=O)C.CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
e4ea1e38252bc3b9c5ec04486386725e6570ab3860d45e337a1d131319bbf0fc
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccccc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[#7;+:5]):[c:6].[OH;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[#7;+:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[O;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]):[c:2]:[c:3]
99.2
[{"value": 99.0, "product": "[N+](=O)([O-])C1=C(OC=2C=C(C#N)C=CC2)C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.2, "product": "[N+](=O)([O-])C1=C(OC=2C=C(C#N)C=CC2)C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
3
HOUR
To a solution of 2-fluoro nitrobenzene (1.41 g, 10 mmol, 1.0 equiv) and 3-hydroxybenzonitrile (1.19 g, 1.0 equiv) in 10 mL of DMF was added K2CO3 (2.76 g, 2 equiv). After stirring at 60° C. for 3 h, the mixture was diluted with EtOAc and washed with H2O. The organic layer was dried over MgSO4, filtered and evaporated t...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HF
CCOC(=O)C.CN(C)C=O
60
3
N#Cc1cccc(O)c1.O=[N+]([O-])c1ccccc1F>CCOC(=O)C.CN(C)C=O>N#Cc1cccc(Oc2ccccc2[N+](=O)[O-])c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a8a6e596c40a42de81190832f7c60776
N#Cc1cccc(Oc2ccccc2[N+](=O)[O-])c1>>N#Cc1cccc(Oc2ccccc2N)c1
[N+](=O)([O-])C1=C(OC=2C=C(C#N)C=CC2)C=CC=C1.O.O.Cl[Sn]Cl>>NC1=C(OC=2C=C(C#N)C=CC2)C=CC=C1
O=[N+:15]([O-])[c:14]1[c:9]([O:8][c:7]2[cH:6][cH:5][cH:4][c:3]([C:2]#[N:1])[cH:16]2)[cH:10][cH:11][cH:12][cH:13]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[NH2:15])[cH:16]1
N#Cc1cccc(Oc2ccccc2[N+](=O)[O-])c1
N#Cc1cccc(Oc2ccccc2N)c1
null
null
CCO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Oc2ccccc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
99
[{"value": 99.0, "product": "NC1=C(OC=2C=C(C#N)C=CC2)C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.9, "product": "NC1=C(OC=2C=C(C#N)C=CC2)C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-(2-nitrophenoxy)benzonitrile (1.21 g, 5 mmol, 1.0 equiv) in 30 mL of EtOH was treated with SnCl2.2H2O (3-38 g, 3 equiv) at reflux for 4 h. The volatile was evaporated and the residue was redissolved in EtOAc, washed with saturated aqueous NaHCO3 and 1N NaOH. The organic layer was dried over MgSO4, filte...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccccc1
Other
CCO
null
null
N#Cc1cccc(Oc2ccccc2[N+](=O)[O-])c1>CCO>N#Cc1cccc(Oc2ccccc2N)c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-95c8195467304d848c25fbc20d6485d1
Fc1ccc2c3c([nH]c2c1)CNCC3>>Fc1ccc2c(c1)[nH]c1cnccc12
FC1=CC=C2C=3CCNCC3NC2=C1>>FC1=CC=C2C=3C=CN=CC3NC2=C1
[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[nH:8][c:9]1[c:14]2[CH2:13][CH2:12][NH:11][CH2:10]1>>[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[nH:8][c:9]1[cH:10][n:11][cH:12][cH:13][c:14]21
Fc1ccc2c3c([nH]c2c1)CNCC3
Fc1ccc2c(c1)[nH]c1cnccc12
null
[Pd]
null
Oxidation
OtherReaction
49cd6b747906212b33e37895c90915d6d06eae54435fd41a9563191b791d0a0e
45f806b8e00071c3429c43b3544e10767c5f82b269d7c53bc7fada9a5eb3b8c6
c1ccc2c(c1)[nH]c1cnccc12
[#7;a:1]1:[c:2]:[c:3]:[c:4]2:[c:5]:1-[CH2;D2;+0:6]-[NH;D2;+0:7]-[CH2;D2;+0:8]-[CH2;D2;+0:9]-2>>[#7;a:1]1:[c:2]:[c:3]:[c:4]2:[cH;D2;+0:9]:[cH;D2;+0:8]:[n;H0;D2;+0:7]:[cH;D2;+0:6]:[c:5]:1:2
88
[{"value": 88.0, "product": "FC1=CC=C2C=3C=CN=CC3NC2=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.5, "product": "FC1=CC=C2C=3C=CN=CC3NC2=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
7-fluoro-2,3,4,9-tetrahydro-1H-β-carboline (3.5 g, 18.42 mmol) was suspended in xylenes (60 ml) in a 250 ml round-bottom flask equipped with a condenser that was open to the atmosphere, and heated. To this hot reaction mixture was added Pd/C (10 wt %, 0.2 eq, 700 mg) and the mixture refluxed in xylenes overnight (12-14...
10.6084/m9.figshare.5104873.v1
null
Secondary amine
null
c1ccc2c3c([nH]c2c1)CNCC3
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
null
[Pd]
null
null
Fc1ccc2c3c([nH]c2c1)CNCC3>[Pd]>Fc1ccc2c(c1)[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-b635247e1c454b27ad6122238f839d06
CO.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>>COc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
O.CO.[H-].[Na+].ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)[N+](=O)[O-]
[CH3:1][OH:2].F[c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[N+:17](=[O:18])[O-:19]>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[N+:17](=[O:18])[O-:19]
CO.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12
COc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
fb66b9ea00ae64d918ad46a3013245b82db1faee7bd623c477afa2b63f708680
23dafde907f7a74dc1d4cc65967b00a9b318897fe61a3d3c4a9fddf320485f17
c1ccc2c(c1)[nH]c1cnccc12
F-[c;H0;D3;+0:1]1:[c:2](-[#7;+:3]):[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11]:1-[Cl;D1;H0:12].[C;D1;H3:13]-[OH;D1;+0:14]>>[#7;+:3]-[c:2]1:[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11](-[Cl;D1;H0:12]):[c;H0;D3;+0:1]:1-[O;H0;D2;+0:14]-[C;D1;H3:13]
97
[{"value": 97.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.7, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
Methanol (0.462 ml, 11.4 mmol) was added to a stirring suspension of NaH (684 mg, 17.1 mmol) in DMF (10 ml) under an argon atmosphere. The resulting solution was allowed to stir at RT for 20 min. 6-chloro-7-fluoro-8-nitro-9H-β-carboline (500 mg, 1.9 mmol) was added to the stirring solution and the resulting mixture was...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Methanol
Ether
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
HF
CN(C)C=O
null
0.333333
CO.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>CN(C)C=O>COc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-becf4864ac49431f98c4bd814a232da9
COc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]>>COc1c(Cl)cc2c([nH]c3cnccc32)c1N
ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)[N+](=O)[O-].[H][H].C(=O)(O)[O-].[Na+]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)N
O=[N+:17]([O-])[c:16]1[c:3]([O:2][CH3:1])[c:4]([Cl:5])[cH:6][c:7]2[c:8]1[nH:9][c:10]1[cH:11][n:12][cH:13][cH:14][c:15]21>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[NH2:17]
COc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
COc1c(Cl)cc2c([nH]c3cnccc32)c1N
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)[nH]c1cnccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
112.3
[{"value": 112.3, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
6-chloro-7-methoxy-8-nitro-9H-β-carboline (510 mg, 1.84 mmol) was suspended in 50 ml of methanol and 100 mg of Pd/C (10%) was added. The flask was fitted with a balloon of hydrogen and the reaction mixture was stirred overnight at RT. Upon filtration through a pad of celite and evaporation of the methanol, a dark brown...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)[nH]c1cnccc12
Other
[Pd].CO
null
8
COc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]>[Pd].CO>COc1c(Cl)cc2c([nH]c3cnccc32)c1N
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-dbeb848e8fc94ab2bca7c131609a2899
COc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O>>COc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)N.CCN=C=NCCCN(C)C.CC1=C(C(=O)O)C=CC=N1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)NC(C1=C(N=CC=C1)C)=O
[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[NH2:17].O[C:18](=[O:19])[c:20]1[cH:21][cH:22][cH:23][n:24][c:25]1[CH3:26]>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[NH:17][C:18](=[O:19])[c:20]1[cH:2...
COc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O
COc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
null
null
N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]):[c:17]
50
[{"value": 50.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)NC(C1=C(N=CC=C1)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
6-chloro-7-methoxy-9H-β-carbolin-8-ylamine (100 mg, 0.4 mmol), EDCI (125 mg, 0.64 mmol) and 2-methyl nicotinic acid (66 mg, 0.48 mmol) were taken in a round-bottom flask and suspended in pyridine (2 ml). The resulting mixture was heated at 80° C. overnight. The pyridine was then removed by rotary evaporation and 5% Na2...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2c(c1)[nH]c1cnccc12.c1ccncc1
HO-
N1=CC=CC=C1
80
null
COc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O>N1=CC=CC=C1>COc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-64f20c9068f249069d4f82b9cd087d27
COc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncncc1C(=O)O>>COc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cncnc1C
ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)N.CC1=NC=NC=C1C(=O)O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)NC(=O)C=1C(=NC=NC1)C
[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[NH2:17].O[C:18](=[O:19])[c:20]1[cH:21][n:22][cH:23][n:24][c:25]1[CH3:26]>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[NH:17][C:18](=[O:19])[c:20]1[cH:21...
COc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncncc1C(=O)O
COc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cncnc1C
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cncnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:1-[C;D1;H3:9].[#7;a:10]:[c:11]:[c:12]:[#7;a:13]:[c:14](:[c:15]):[c:16](-[NH2;D1;+0:17]):[c:18]>>[#7;a:10]:[c:11]:[c:12]:[#7;a:13]:[c:14](:[c:15]):[c:16](-[NH;D2;+0:17]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:1-[C;D...
80
[{"value": 80.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OC)NC(=O)C=1C(=NC=NC1)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method A from 6-chloro-7-methoxy-9H-beta-carbolin-8-ylamine and 4-methyl-5-pyrimidine carboxylic acid in 80% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2c(c1)[nH]c1cnccc12.c1cncnc1
HO-
null
null
null
COc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncncc1C(=O)O>>COc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cncnc1C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-43669270af0443af8dcc4c27264a3edb
CC[O-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>>CCOc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
[O-]CC.[Na+].ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-].Cl>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC)[N+](=O)[O-]
[CH3:1][CH2:2][O-:3].F[c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[N+:18](=[O:19])[O-:20]>>[CH3:1][CH2:2][O:3][c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[N+:18](=[O:19])[O-:20]
CC[O-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12
CCOc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
null
null
CS(=O)C.O
Heteroatom Alkylation and Arylation
OtherReaction
1f0182aba60bda71c1cacefb53d4629b0f8909ff869c59859818a59c4bf2c769
51fd03eb6a688046e417b9ed09ea0e72062396d005af1318b9b5f376a97da959
c1ccc2c(c1)[nH]c1cnccc12
F-[c;H0;D3;+0:1]1:[c:2](-[#7;+:3]):[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11]:1-[Cl;D1;H0:12].[C;D1;H3:13]-[C:14]-[O-;H0;D1:15]>>[#7;+:3]-[c:2]1:[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11](-[Cl;D1;H0:12]):[c;H0;D3;+0:1]:1-[O;H0;D2;+0:15]-[C:14]-[C;D1;H3:13]
40
[{"value": 40.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Sodium ethoxide (232 mg, 3.4 mmol) was added to a solution of 6-chloro-7-fluoro-8-nitro-9H-β-carboline (200 mg, 0.76 mmol) in DMSO (4 ml) and the reaction mixture allowed to stir overnight. The reaction mixture was diluted with water and the pH of the solution was adjusted to about 4 by adding 1N HCl. The aqueous solut...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Ether
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
Other
CS(=O)C.O
null
8
CC[O-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>CS(=O)C.O>CCOc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a246859ab003474d815d88040d024039
CCOc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O>>CCOc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC)N.CC1=C(C(=O)O)C=CC=N1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC)NC(C1=C(N=CC=C1)C)=O
[CH3:1][CH2:2][O:3][c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[NH2:18].O[C:19](=[O:20])[c:21]1[cH:22][cH:23][cH:24][n:25][c:26]1[CH3:27]>>[CH3:1][CH2:2][O:3][c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[NH:18][C:19](=[O:...
CCOc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O
CCOc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]):[c:17]
40
[{"value": 40.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC)NC(C1=C(N=CC=C1)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method A from 6-chloro-7-ethoxy-9H-β-carbolin-8-ylamine and 2-methylnicotinic acid in 40% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2c(c1)[nH]c1cnccc12.c1ccncc1
HO-
null
null
null
CCOc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O>>CCOc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-88fe38c5b72d4d6db3a391486d78fc65
CN1CCNCC1.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>>CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2[N+](=O)[O-])CC1
CS(=O)C.ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-].CN1CCNCC1.CCN(C(C)C)C(C)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1N1CCN(CC1)C)[N+](=O)[O-]
[CH3:1][N:2]1[CH2:3][CH2:4][NH:5][CH2:23][CH2:24]1.F[c:6]1[c:7]([Cl:8])[cH:9][c:10]2[c:11]([nH:12][c:13]3[cH:14][n:15][cH:16][cH:17][c:18]23)[c:19]1[N+:20](=[O:21])[O-:22]>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([c:6]2[c:7]([Cl:8])[cH:9][c:10]3[c:11]([nH:12][c:13]4[cH:14][n:15][cH:16][cH:17][c:18]34)[c:19]2[N+:20](=[O:21])[O...
CN1CCNCC1.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2[N+](=O)[O-])CC1
null
null
O
Heteroatom Alkylation and Arylation
Buchwald-Hartwig/Ullmann-Goldberg/N-arylation secondary amine
77d260fc2f8702014dbc060ee1f8e9930a9aeacb102b3b42c4765e2337dbc842
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1cc2c(cn1)[nH]c1cc(N3CCNCC3)ccc12
F-[c;H0;D3;+0:1]1:[c:2](-[#7;+:3]):[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11]:1-[Cl;D1;H0:12].[#7:13]1-[C:14]-[C:15]-[NH;D2;+0:16]-[C:17]-[C:18]-1>>[#7;+:3]-[c:2]1:[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11](-[Cl;D1;H0:12]):[c;H0;D3;+0:1]:1-[N;H0;D3;+0:16]1-[C:15]-[C:14]-[#7:13]-[C:18]-[C:1...
91
[{"value": 91.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1N1CCN(CC1)C)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.4, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1N1CCN(CC1)C)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a DMSO solution (4 ml) of 200 mg (0.755 mmol) of 6-chloro-7-fluoro-8-nitro-9H-β-carboline was added 1-methylpiperazine (226 mg, 2.26 mmol) and DIEA (400 mg, 3.09 mmol) via a syringe. The reaction was allowed to stir at RT overnight. Upon addition of water, an orange solid precipitated out. The solid was filtered, wa...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
C1C[NH]CCN1.c1ccc2c(c1)[nH]c1cnccc12
C1C[NH]CC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
C1C[NH]CC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HF
O
null
8
CN1CCNCC1.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>O>CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2[N+](=O)[O-])CC1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-999c390fd09a4602b272acf153fb1264
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2[N+](=O)[O-])CC1>>CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2N)CC1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1N1CCN(CC1)C)[N+](=O)[O-]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1N1CCN(CC1)C)N
O=[N+:20]([O-])[c:19]1[c:6]([N:5]2[CH2:4][CH2:3][N:2]([CH3:1])[CH2:22][CH2:21]2)[c:7]([Cl:8])[cH:9][c:10]2[c:11]1[nH:12][c:13]1[cH:14][n:15][cH:16][cH:17][c:18]21>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([c:6]2[c:7]([Cl:8])[cH:9][c:10]3[c:11]([nH:12][c:13]4[cH:14][n:15][cH:16][cH:17][c:18]34)[c:19]2[NH2:20])[CH2:21][CH2:22]1
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2[N+](=O)[O-])CC1
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2N)CC1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1cc2c(cn1)[nH]c1cc(N3CCNCC3)ccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
55.2
[{"value": 55.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1N1CCN(CC1)C)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 55.2, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1N1CCN(CC1)C)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Suspended 236 mg of 6-chloro-7-(4-methyl-piperazin-1-yl)-8-nitro-9H-β-carboline in 100 ml of methanol and added 10% Pd/C(48 mg) under argon. The flask was flushed with hydrogen (3×) and the reaction mixture was stirred under a hydrogen atmosphere at RT overnight. The reaction mixture was filtered and Pd/C was removed u...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
C1C[NH]CC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
Other
[Pd].CO
null
8
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2[N+](=O)[O-])CC1>[Pd].CO>CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2N)CC1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e81169359fb94455a9946173265fc171
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2N)CC1.O=C(O)c1cccnc1Cl>>CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2NC(=O)c2cccnc2Cl)CC1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1N1CCN(CC1)C)N.ClC1=C(C(=O)O)C=CC=N1>>ClC1=C(C(=O)NC=2C(=C(C=C3C=4C=CN=CC4NC23)Cl)N2CCN(CC2)C)C=CC=N1
[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([c:6]2[c:7]([Cl:8])[cH:9][c:10]3[c:11]([nH:12][c:13]4[cH:14][n:15][cH:16][cH:17][c:18]34)[c:19]2[NH2:20])[CH2:30][CH2:31]1.O[C:21](=[O:22])[c:23]1[cH:24][cH:25][cH:26][n:27][c:28]1[Cl:29]>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([c:6]2[c:7]([Cl:8])[cH:9][c:10]3[c:11]([nH:12][c:13]4[cH:14][n:15...
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2N)CC1.O=C(O)c1cccnc1Cl
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2NC(=O)c2cccnc2Cl)CC1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1c(N2CCNCC2)ccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[Cl;D1;H0:6]):[#7;a:7]:[c:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[Cl;D1;H0:6]):[#7;a:7]:[c:8]):[c:17]
25
[{"value": 25.0, "product": "ClC1=C(C(=O)NC=2C(=C(C=C3C=4C=CN=CC4NC23)Cl)N2CCN(CC2)C)C=CC=N1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method A from 6-chloro-7-(4-methyl-piperazin-1-yl)-8-amino-9H-β-carboline and 2-chloro-nicotinic acid in 25% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1C[NH]CC[NH]1.c1ccc2c(c1)[nH]c1cnccc12.c1ccncc1
HO-
null
null
null
CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2N)CC1.O=C(O)c1cccnc1Cl>>CN1CCN(c2c(Cl)cc3c([nH]c4cnccc43)c2NC(=O)c2cccnc2Cl)CC1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-893383a6f6244cf79604ae38fdab3519
CN1C(=O)CC(C(=O)O)C1(C)C.Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CN1C(=O)CC(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)C1(C)C
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)N.CN1C(C(CC1=O)C(=O)O)(C)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1C(N(C(C1)=O)C)(C)C
O[C:7]([CH:6]1[CH2:5][C:3](=[O:4])[N:2]([CH3:1])[C:24]1([CH3:25])[CH3:26])=[O:8].[NH2:9][c:10]1[cH:11][c:12]([Cl:13])[cH:14][c:15]2[c:16]1[nH:17][c:18]1[cH:19][n:20][cH:21][cH:22][c:23]21>>[CH3:1][N:2]1[C:3](=[O:4])[CH2:5][CH:6]([C:7](=[O:8])[NH:9][c:10]2[cH:11][c:12]([Cl:13])[cH:14][c:15]3[c:16]2[nH:17][c:18]2[cH:19][...
CN1C(=O)CC(C(=O)O)C1(C)C.Nc1cc(Cl)cc2c1[nH]c1cnccc12
CN1C(=O)CC(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)C1(C)C
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C1CC(C(=O)Nc2cccc3c2[nH]c2cnccc23)CN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[C:8]-1.[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[C:8]-1):[c:17]
68
[{"value": 68.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1C(N(C(C1)=O)C)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method B from 6-chloro-9H-β-carboline-8-ylamine and 1,2,2-trimethyl-5-oxo-pyrrolidine-3-carboxylic acid in 68% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CC[NH]C1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CN1C(=O)CC(C(=O)O)C1(C)C.Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CN1C(=O)CC(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)C1(C)C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-d46c8f0fc93a42c984faa43c8c9ef0d6
N[C@@H](CO)C(=O)OCc1ccccc1.O=Cc1ccccc1>>O=C(OCc1ccccc1)[C@H](CO)NCc1ccccc1
C(#N)[BH3-].[Na+].Cl.C(C1=CC=CC=C1)OC([C@@H](N)CO)=O.C(C1=CC=CC=C1)=O.C(C)(=O)[O-].[Na+]>>C(C1=CC=CC=C1)OC([C@@H](NCC1=CC=CC=C1)CO)=O
[O:1]=[C:2]([O:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[C@H:11]([CH2:12][OH:13])[NH2:14].O=[CH:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1>>[O:1]=[C:2]([O:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[C@H:11]([CH2:12][OH:13])[NH:14][CH2:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1
N[C@@H](CO)C(=O)OCc1ccccc1.O=Cc1ccccc1
O=C(OCc1ccccc1)[C@H](CO)NCc1ccccc1
null
null
CO
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
O=C(CNCc1ccccc1)OCc1ccccc1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11]>>[C:5]-[C:6](-[NH;D2;+0:7]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11]
81
[{"value": 81.0, "product": "C(C1=CC=CC=C1)OC([C@@H](NCC1=CC=CC=C1)CO)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
15
HOUR
To a mixture of L-serine-benzyl ester-HCl (2.3 g), benzaldehyde(1.05 eq.) and sodium acetate (1 eq.) in methanol was added sodium cyanoborohydride (1.0 eq.). The resulting mixture was stirred at ambient temperature for 15 hrs, then partitioned into ether and aqueous saturated sodium bicarbonate. The separated organic p...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccccc1
Other
CO
null
15
N[C@@H](CO)C(=O)OCc1ccccc1.O=Cc1ccccc1>CO>O=C(OCc1ccccc1)[C@H](CO)NCc1ccccc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-77e443df8e2d403b81623c641b5e9394
C=C(C)CBr.II.O=C(OCc1ccccc1)[C@H](CO)NCc1ccccc1>>CC1(CI)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1
C(C1=CC=CC=C1)OC([C@@H](NCC1=CC=CC=C1)CO)=O.C(C1=CC=CC=C1)OC([C@@H](NCC1=CC=CC=C1)CO)=O.BrCC(=C)C.C(=O)([O-])[O-].[K+].[K+].II.BrCC(=C)C>>C(C1=CC=CC=C1)OC(=O)C1N(CC(OC1)(C)CI)CC1=CC=CC=C1
Br[CH2:3][C:2]([CH3:1])=[CH2:5].I[I:4].[NH:6]([CH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)[C@H:14]([C:15](=[O:16])[O:17][CH2:18][c:19]1[cH:20][cH:21][cH:22][cH:23][cH:24]1)[CH2:25][OH:26]>>[CH3:1][C:2]1([CH2:3][I:4])[CH2:5][N:6]([CH2:7][c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[CH:14]([C:15](=[O:16])[O:17][CH2:18]...
C=C(C)CBr.II.O=C(OCc1ccccc1)[C@H](CO)NCc1ccccc1
CC1(CI)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1
null
null
CC#N.CCOC(=O)C.CCCCCC
Heteroatom Alkylation and Arylation
OtherReaction
7fdda7499cb691fc9e08dbb17c4964c805059d7ec826a851e5e7c3a7d1683064
2b3f9402e95e7d2bbee1f40b67bc1facac10e2ef69e32213d57db76c382e04d4
O=C(OCc1ccccc1)C1COCCN1Cc1ccccc1
Br-[CH2;D2;+0:1]-[C;H0;D3;+0:2](-[C;D1;H3:3])=[CH2;D1;+0:4].I-[I;H0;D1;+0:5].[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C@H;D3;+0:10](-[C:11]-[OH;D1;+0:12])-[NH;D2;+0:13]-[C:14]-[c:15]>>[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[CH;D3;+0:10]1-[C:11]-[O;H0;D2;+0:12]-[C;H0;D4;+0:2](-[C;D1;H3:3])(-[CH2;D2;+0:1]-[I;H0;D1;+0:5])-[CH2;D2;+0:4...
64
[{"value": 64.0, "product": "C(C1=CC=CC=C1)OC(=O)C1N(CC(OC1)(C)CI)CC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
72
HOUR
To a solution of N-benzyl-serine benzyl ester (Intermediate 16, 6.35 g) in 90 ml of MeCN at ambient temperature was added 3-bromo-2-methyl-propene (5.6 ml), KI (740 mg) and K2CO3 (7.7 g). The reaction mixture was stirred at ambient temperature for 72 hrs. 1 ml of 3-bromo-2-methyl-propene was added and the reaction mixt...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary alcohol.Secondary amine.Vinyl
Primary halide.Ether.Tertiary amine
null
C1COCC[NH]1
C1COCC[NH]1.c1ccccc1.c1ccccc1
HBr.I-
CC#N.CCOC(=O)C.CCCCCC
null
72
C=C(C)CBr.II.O=C(OCc1ccccc1)[C@H](CO)NCc1ccccc1>CC#N.CCOC(=O)C.CCCCCC>CC1(CI)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-de82173cc7804e4cae31af4e4fc9d489
CC1(CI)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1>>CC1(C)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1
C(C1=CC=CC=C1)OC(=O)C1N(CC(OC1)(C)CI)CC1=CC=CC=C1.C(C1=CC=CC=C1)OC(=O)C1N(CC(OC1)(C)CI)CC1=CC=CC=C1.C(CCC)[SnH](CCCC)CCCC.CC(C)(C#N)N=NC(C)(C)C#N>>C(C1=CC=CC=C1)OC(=O)C1N(CC(OC1)(C)C)CC1=CC=CC=C1
I[CH2:3][C:2]1([CH3:1])[CH2:4][N:5]([CH2:6][c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[CH:13]([C:14](=[O:15])[O:16][CH2:17][c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[CH2:24][O:25]1>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[CH:13]([C:14](=[O:15])[O:16][CH2:17][c:18]2[cH:19][cH:...
CC1(CI)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1
CC1(C)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1
null
null
C1(=CC=CC=C1)C
Functional Group Interconversion
Dehalogenation
72a5231b07f184f0ef4a0648badd4176f521b95f1ba3340a0f90d8894af47260
47a659f5704a5b7ca1b92ff731f18f109c6bde1d45152a3a393eefbd10265508
O=C(OCc1ccccc1)C1COCCN1Cc1ccccc1
I-[CH2;D2;+0:1]-[C:2](-[C;D1;H3:3])(-[#8:4]-[C:5])-[C:6]-[#7:7]>>[#7:7]-[C:6]-[C:2](-[C;D1;H3:3])(-[CH3;D1;+0:1])-[#8:4]-[C:5]
85
[{"value": 85.0, "product": "C(C1=CC=CC=C1)OC(=O)C1N(CC(OC1)(C)C)CC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 4-benzyl-6-iodomethyl-6-methyl-morpholine-3-carboxylic acid benzyl ester (Intermediate 17, 1.23 g) and tributyltin hydride (1.8 ml, 2.5 eq.) in 11 ml of toluene under gentle reflux was added over 1.5 hr a solution of AIBN in toluene (25 mg/1 ml). The mixture was allowed to cool down and was concentrate...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
null
null
C1COCC[NH]1.c1ccccc1.c1ccccc1
I-
C1(=CC=CC=C1)C
null
null
CC1(CI)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1>C1(=CC=CC=C1)C>CC1(C)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-d6731d9b8e144b0e9b60dee94349263b
CC1(C)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1>>CC1(C)CNC(C(=O)O)CO1
C(C1=CC=CC=C1)OC(=O)C1N(CC(OC1)(C)C)CC1=CC=CC=C1.C(C1=CC=CC=C1)OC(=O)C1N(CC(OC1)(C)C)CC1=CC=CC=C1>>CC1(OCC(NC1)C(=O)O)C
c1ccc(C[N:5]2[CH2:4][C:2]([CH3:1])([CH3:3])[O:11][CH2:10][CH:6]2[C:7](=[O:8])[O:9]Cc2ccccc2)cc1>>[CH3:1][C:2]1([CH3:3])[CH2:4][NH:5][CH:6]([C:7](=[O:8])[OH:9])[CH2:10][O:11]1
CC1(C)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1
CC1(C)CNC(C(=O)O)CO1
null
[OH-].[OH-].[Pd+2]
CC(=O)O.CO
Deprotection
OtherReaction
fd133f20ece8af39de6ac98d2595c0684237870ac067b15eea0f5f441e9a4923
3d8e4bece6e5ac07ee91a76d9cf0561ba741378ef06008fae89f75f1d764c0c9
C1COCCN1
[O;D1;H0:1]=[C:2](-[O;H0;D2;+0:3]-C-c1:c:c:c:c:c:1)-[C:4]1-[C:5]-[#8:6]-[C:7]-[C:8]-[N;H0;D3;+0:9]-1-C-c1:c:c:c:c:c:1>>[O;D1;H0:1]=[C:2](-[OH;D1;+0:3])-[C:4]1-[C:5]-[#8:6]-[C:7]-[C:8]-[NH;D2;+0:9]-1
95.4
[{"value": 95.0, "product": "CC1(OCC(NC1)C(=O)O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.4, "product": "CC1(OCC(NC1)C(=O)O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
72
HOUR
To a solution of 4-benzyl-6,6-dimethyl-morpholine-3-carboxylic acid benzyl ester (Intermediate 18, 1.25 g) in 40 ml of 10% AcOH/MeOH (under nitrogen) was added 250 mg of 20% Pd(OH)2 on charcoal. The reaction mixture was purged with hydrogen (balloon) and was stirred at ambient temperature for 72 hrs. To the resulting g...
10.6084/m9.figshare.5104873.v1
null
Ester.Tertiary amine
Carboxylic acid.Secondary amine
c1ccccc1.C1COCC[NH]1.c1ccccc1
C1COCCN1
C1COCCN1
Other
[OH-].[OH-].[Pd+2].CC(=O)O.CO
null
72
CC1(C)CN(Cc2ccccc2)C(C(=O)OCc2ccccc2)CO1>[OH-].[OH-].[Pd+2].CC(=O)O.CO>CC1(C)CNC(C(=O)O)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-922f4d1b3fc74bca99bd38351a87de4c
C=O.CC1(C)CNC(C(=O)O)CO1>>CN1CC(C)(C)OCC1C(=O)O
C=O.CC1(OCC(NC1)C(=O)O)C.CC1(OCC(NC1)C(=O)O)C>>CN1C(COC(C1)(C)C)C(=O)O
O=[CH2:1].[NH:2]1[CH2:3][C:4]([CH3:5])([CH3:6])[O:7][CH2:8][CH:9]1[C:10](=[O:11])[OH:12]>>[CH3:1][N:2]1[CH2:3][C:4]([CH3:5])([CH3:6])[O:7][CH2:8][CH:9]1[C:10](=[O:11])[OH:12]
C=O.CC1(C)CNC(C(=O)O)CO1
CN1CC(C)(C)OCC1C(=O)O
null
[Pd]
C(C)O
Heteroatom Alkylation and Arylation
Eschweiler-Clarke Secondary Amine Methylation
fdddc65917853749f4468b50c6d27df95b134f4ca23d77fbc7927a814b9768f6
e1fdef8fde1c506d7c9deb8fd5e6f322eceea2abce3167abcf412a1fa4fd5443
C1COCCN1
O=[CH2;D1;+0:1].[O;D1;H0:2]=[C:3](-[O;D1;H1:4])-[C:5]1-[C:6]-[#8:7]-[C:8]-[C:9]-[NH;D2;+0:10]-1>>[CH3;D1;+0:1]-[N;H0;D3;+0:10]1-[C:9]-[C:8]-[#8:7]-[C:6]-[C:5]-1-[C:3](=[O;D1;H0:2])-[O;D1;H1:4]
97
[{"value": 97.0, "product": "CN1C(COC(C1)(C)C)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
To a suspension of 6,6-dimethyl-morpholine-3-carboxylic acid (Intermediate 19, 540 mg) in 17 ml of ethanol (under nitrogen) was added 100 mg of 10% Pd on charcoal and 830 ul (˜3 eq.) of 37% aqueous formaldehyde. The mixture was purged with hydrogen (balloon) and stirred at ambient temperature for 5 hrs. To the resultin...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Secondary amine
Tertiary amine
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1
Other
[Pd].C(C)O
null
5
C=O.CC1(C)CNC(C(=O)O)CO1>[Pd].C(C)O>CN1CC(C)(C)OCC1C(=O)O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-7af62963344d437cb6f1e896ba44c546
CN1CC(C)(C)OCC1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)N.CN1C(COC(C1)(C)C)C(=O)O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)C
O[C:10]([CH:9]1[N:2]([CH3:1])[CH2:3][C:4]([CH3:5])([CH3:6])[O:7][CH2:8]1)=[O:11].[NH2:12][c:13]1[cH:14][c:15]([Cl:16])[cH:17][c:18]2[c:19]1[nH:20][c:21]1[cH:22][n:23][cH:24][cH:25][c:26]21>>[CH3:1][N:2]1[CH2:3][C:4]([CH3:5])([CH3:6])[O:7][CH2:8][CH:9]1[C:10](=[O:11])[NH:12][c:13]1[cH:14][c:15]([Cl:16])[cH:17][c:18]2[c:...
CN1CC(C)(C)OCC1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12
CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)C1COCCN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4]-[#8:5])-[#7:6](-[C;D1;H3:7])-[C:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4]-[#8:5])-[#7:6](-[C;D1;H3:7])-[C:8]):[c:17]
61
[{"value": 61.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method B from 6-chloro-9H-β-carboline-8-ylamine and 4,6,6-trimethyl-morpholine-3-carboxylic acid in 61% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CN1CC(C)(C)OCC1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-652727651c6a4c0ca4ce9fbe27907fd7
O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12.OCC1CC1>>O=[N+]([O-])c1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
O.C1(CC1)CO.[H-].[Na+].ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)[N+](=O)[O-]
F[c:5]1[c:4]([N+:2](=[O:1])[O-:3])[c:15]2[c:14]([cH:13][c:11]1[Cl:12])[c:22]1[c:17]([nH:16]2)[cH:18][n:19][cH:20][cH:21]1.[OH:6][CH2:7][CH:8]1[CH2:9][CH2:10]1>>[O:1]=[N+:2]([O-:3])[c:4]1[c:5]([O:6][CH2:7][CH:8]2[CH2:9][CH2:10]2)[c:11]([Cl:12])[cH:13][c:14]2[c:15]1[nH:16][c:17]1[cH:18][n:19][cH:20][cH:21][c:22]21
O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12.OCC1CC1
O=[N+]([O-])c1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
eb9f6ceb14d04281e24cbf4d6354ca29ee2394b373406b20c365e94506dd7cee
a4cafa7bcd156e21cca6eaac1b32e28ec8540642a31181122e6957f3d7559631
c1cc2c(cn1)[nH]c1cc(OCC3CC3)ccc12
F-[c;H0;D3;+0:1]1:[c:2](-[Cl;D1;H0:3]):[c:4]:[c:5]:[c:6](:[#7;a:7]:[c:8]:[c:9]:[#7;a:10]):[c:11]:1-[#7;+:12].[C:13]-[C:14]-[OH;D1;+0:15]>>[#7;+:12]-[c:11]1:[c:6](:[#7;a:7]:[c:8]:[c:9]:[#7;a:10]):[c:5]:[c:4]:[c:2](-[Cl;D1;H0:3]):[c;H0;D3;+0:1]:1-[O;H0;D2;+0:15]-[C:14]-[C:13]
85
[{"value": 85.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.5, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
Cyclopropylmethyl alcohol (0.921 ml, 11.4 mmol) was added to a stirring suspension of NaH (455 mg, 11.4 mmol) in DMF (20 ml) under an argon atmosphere. The resulting solution was allowed to stir at RT for 20 min. 6-chloro-7-fluoro-8-nitro-9H-β-carboline (500 mg, 1.9 mmol) was added to the stirring solution and the resu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary alcohol
Ether
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
C1CC1.c1ccc2c(c1)[nH]c1cnccc12
HF
CN(C)C=O
null
0.333333
O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12.OCC1CC1>CN(C)C=O>O=[N+]([O-])c1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f36f8b53201943fe85c6b7396fde7d0e
O=[N+]([O-])c1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12>>Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)[N+](=O)[O-].[H][H].C(=O)(O)[O-].[Na+]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)N
O=[N+:1]([O-])[c:2]1[c:3]([O:4][CH2:5][CH:6]2[CH2:7][CH2:8]2)[c:9]([Cl:10])[cH:11][c:12]2[c:13]1[nH:14][c:15]1[cH:16][n:17][cH:18][cH:19][c:20]21>>[NH2:1][c:2]1[c:3]([O:4][CH2:5][CH:6]2[CH2:7][CH2:8]2)[c:9]([Cl:10])[cH:11][c:12]2[c:13]1[nH:14][c:15]1[cH:16][n:17][cH:18][cH:19][c:20]21
O=[N+]([O-])c1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1cc2c(cn1)[nH]c1cc(OCC3CC3)ccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
80.1
[{"value": 80.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.1, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
6-chloro-7-cyclopropylmethoxy-8-nitro-9H-β-carboline (510 mg, 1.61 mmol) was suspended in 12 ml of methanol and 100 mg of Pd/C(10%) was added. The flask was fitted with a balloon of hydrogen and the reaction mixture was stirred overnight at RT. Upon filtration through a pad of celite and evaporation of the methanol, a ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
C1CC1.c1ccc2c(c1)[nH]c1cnccc12
Other
[Pd].CO
null
8
O=[N+]([O-])c1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12>[Pd].CO>Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-970f2d8f6a31410c9eb7931d5d8ac635
Cc1ncccc1C(=O)O.Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12>>Cc1ncccc1C(=O)Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)N.CC1=C(C(=O)O)C=CC=N1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)NC(C1=C(N=CC=C1)C)=O
O[C:8]([c:7]1[c:2]([CH3:1])[n:3][cH:4][cH:5][cH:6]1)=[O:9].[NH2:10][c:11]1[c:12]([O:13][CH2:14][CH:15]2[CH2:16][CH2:17]2)[c:18]([Cl:19])[cH:20][c:21]2[c:22]1[nH:23][c:24]1[cH:25][n:26][cH:27][cH:28][c:29]21>>[CH3:1][c:2]1[n:3][cH:4][cH:5][cH:6][c:7]1[C:8](=[O:9])[NH:10][c:11]1[c:12]([O:13][CH2:14][CH:15]2[CH2:16][CH2:1...
Cc1ncccc1C(=O)O.Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
Cc1ncccc1C(=O)Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1c(OCC2CC2)ccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]):[c:17]
40
[{"value": 40.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1OCC1CC1)NC(C1=C(N=CC=C1)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method A from 6-chloro-7-cyclopropylmethoxy-9H-β-carbolin-8-ylamine and 2-methylnicotinic acid in a 40-60% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccncc1.C1CC1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
Cc1ncccc1C(=O)O.Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12>>Cc1ncccc1C(=O)Nc1c(OCC2CC2)c(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-4fd2ab0b382a4a5fafaa30220b5f686c
O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>>Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)N
O=[N+:1]([O-])[c:2]1[c:3]([F:4])[c:5]([Cl:6])[cH:7][c:8]2[c:9]1[nH:10][c:11]1[cH:12][n:13][cH:14][cH:15][c:16]21>>[NH2:1][c:2]1[c:3]([F:4])[c:5]([Cl:6])[cH:7][c:8]2[c:9]1[nH:10][c:11]1[cH:12][n:13][cH:14][cH:15][c:16]21
O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12
Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)[nH]c1cnccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
90.3
[{"value": 90.3, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
6
HOUR
A slurry of 6-chloro-7-fluoro-8-nitro-9H-β-carboline (500 mg, 1.88 mmol) in MeOH (25 ml) was degassed with argon. Palladium on charcoal (20% w/w on C, 50 mg) was added and the reaction vessel was flushed with hydrogen. The slurry was stirred under a balloon of hydrogen for 6 hr, then filtered through celite and concent...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)[nH]c1cnccc12
Other
[Pd].CO
null
6
O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>[Pd].CO>Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-212676db6bac4ade867f66bfad747cd6
Cc1ncccc1C(=O)O.Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12>>Cc1ncccc1C(=O)Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12
C1=CC(=NN=C1NN)N(CCO)CCO.Cl.Cl.CC1=C(C(=O)O)C=CC=N1.ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)N.CCN=C=NCCCN(C)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)NC(C1=C(N=CC=C1)C)=O
O[C:8]([c:7]1[c:2]([CH3:1])[n:3][cH:4][cH:5][cH:6]1)=[O:9].[NH2:10][c:11]1[c:12]([F:13])[c:14]([Cl:15])[cH:16][c:17]2[c:18]1[nH:19][c:20]1[cH:21][n:22][cH:23][cH:24][c:25]21>>[CH3:1][c:2]1[n:3][cH:4][cH:5][cH:6][c:7]1[C:8](=[O:9])[NH:10][c:11]1[c:12]([F:13])[c:14]([Cl:15])[cH:16][c:17]2[c:18]1[nH:19][c:20]1[cH:21][n:22...
Cc1ncccc1C(=O)O.Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12
Cc1ncccc1C(=O)Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12
null
null
N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]):[c:17]
null
[]
100
CELSIUS
null
null
A solution of 6-chloro-7-fluoro-9H-β-carbolin-8-ylamine (100 mg, 0.424 mmol) in pyridine (2.5 ml) was stirred at RT. 2-methyl nicotinic acid (70 mg, 0.509 mmol) was added, followed by EDCI (130 mg, 0.678 mmol). The suspension was stirred at 100° C. for a day. The pyridine was removed under reduced pressure and the resu...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccncc1.c1ccc2c(c1)[nH]c1cnccc12
HO-
N1=CC=CC=C1
100
null
Cc1ncccc1C(=O)O.Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12>N1=CC=CC=C1>Cc1ncccc1C(=O)Nc1c(F)c(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-831366161355451eb87675e81341adfa
C[S-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>>CSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-].ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-].CN(C)C=O.C[S-].[Na+]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1SC)[N+](=O)[O-]
[CH3:1][S-:2].F[c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[N+:17](=[O:18])[O-:19]>>[CH3:1][S:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[N+:17](=[O:18])[O-:19]
C[S-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12
CSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
278a1f60937c998ec02609c16c07f994a421fa5a3ed90fcfbeacdee2ebaa3bd2
1813ae14fbd9cacead4dcfaf9efbd2467a19b3e216836766b78aa6647dcfb48a
c1ccc2c(c1)[nH]c1cnccc12
F-[c;H0;D3;+0:1]1:[c:2](-[#7;+:3]):[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11]:1-[Cl;D1;H0:12].[C;D1;H3:13]-[S-;H0;D1:14]>>[#7;+:3]-[c:2]1:[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11](-[Cl;D1;H0:12]):[c;H0;D3;+0:1]:1-[S;H0;D2;+0:14]-[C;D1;H3:13]
91.8
[{"value": 91.8, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SC)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
A 250 ml round-bottom flask with magnetic stirrer was charged with 6-chloro-7-fluoro-8-nitro-β-carboline (Intermediate 5, 3.959 g, 14.9 mmol) and 100 ml anhydrous DMF. The resulting orange mixture was cooled to 0° C. (ice and water bath) and sodium thiomethoxide (1.809 g, 25.8 mmol) in powder form was added slowly ther...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Monosulfide
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
Other
O
0
1
C[S-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>O>CSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-fe7796a45668470a88b977caac4dbba7
CSc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O>>CSc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
Cl.CN(CCCN=C=NCC)C.ClC=1C=C2C=3C=CN=CC3NC2=C(C1SC)N.ClC=1C=C2C=3C=CN=CC3NC2=C(C1SC)N.CC1=C(C(=O)O)C=CC=N1.O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1SC)NC(C1=C(N=CC=C1)C)=O
[CH3:1][S:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[NH2:17].O[C:18](=[O:19])[c:20]1[cH:21][cH:22][cH:23][n:24][c:25]1[CH3:26]>>[CH3:1][S:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]2[c:8]([nH:9][c:10]3[cH:11][n:12][cH:13][cH:14][c:15]23)[c:16]1[NH:17][C:18](=[O:19])[c:20]1[cH:2...
CSc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O
CSc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
null
null
CO.N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]):[c:17]
89.5
[{"value": 89.5, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SC)NC(C1=C(N=CC=C1)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
18
HOUR
A 250 ml round-bottom flask with magnetic stirrer was charged with 6-chloro-7-methylsulfanyl-9H-β-carbolin-8-ylamine (Intermediate 28, 2.336 g, 8.86 mmol) and 2-methylnicotinic acid (3.219 g, 23.4 mmol) in 80 ml anhydrous pyridine. To the resulting reaction mixture at RT was added solid 1-(3-dimethylaminopropyl)-3-ethy...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2c(c1)[nH]c1cnccc12.c1ccncc1
HO-
CO.N1=CC=CC=C1
100
18
CSc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O>CO.N1=CC=CC=C1>CSc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e3ed8d18dc2b4a6db03c647fd794b654
CC[S-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>>CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-].[S-]CC.[Na+].O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)[N+](=O)[O-]
[CH3:1][CH2:2][S-:3].F[c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[N+:18](=[O:19])[O-:20]>>[CH3:1][CH2:2][S:3][c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[N+:18](=[O:19])[O-:20]
CC[S-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
278a1f60937c998ec02609c16c07f994a421fa5a3ed90fcfbeacdee2ebaa3bd2
1813ae14fbd9cacead4dcfaf9efbd2467a19b3e216836766b78aa6647dcfb48a
c1ccc2c(c1)[nH]c1cnccc12
F-[c;H0;D3;+0:1]1:[c:2](-[#7;+:3]):[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11]:1-[Cl;D1;H0:12].[C;D1;H3:13]-[C:14]-[S-;H0;D1:15]>>[#7;+:3]-[c:2]1:[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11](-[Cl;D1;H0:12]):[c;H0;D3;+0:1]:1-[S;H0;D2;+0:15]-[C:14]-[C;D1;H3:13]
81.2
[{"value": 79.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.2, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
45
MINUTE
A 25 ml round-bottom flask with a magnetic stirrer was charged with 6-chloro-7-fluoro-8-nitro-9H-β-carboline (102 mg, 0.38 mmol) in 5 ml of anhydrous DMF. To the resulting orange mixture at RT was slowly added sodium thioethoxide (80% pure, 69.7 mg, 0.66 mmol) in powder form. The reaction mixture was stirred at RT for ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Monosulfide
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
Other
CN(C)C=O
null
0.75
CC[S-].O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>CN(C)C=O>CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-99de42632e8e4623a5dd2ee602d10fb0
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]>>CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N
C.ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)[N+](=O)[O-].[Cl-].[NH4+]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)N
O=[N+:18]([O-])[c:17]1[c:4]([S:3][CH2:2][CH3:1])[c:5]([Cl:6])[cH:7][c:8]2[c:9]1[nH:10][c:11]1[cH:12][n:13][cH:14][cH:15][c:16]21>>[CH3:1][CH2:2][S:3][c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[NH2:18]
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N
null
[Fe]
C(C)(=O)OCC.C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)[nH]c1cnccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
100
[{"value": 99.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
20
HOUR
A 50 ml round-bottom flask with magnetic stirrer was charged with 6-chloro-7-ethylsulfanyl-8-nitro-9H-β-carboline (85.0 mg, 0.28 mmol) in 10 ml anhydrous ethanol. To the resulting orange mixture at RT was added 0.33 M aqueous ammonium chloride (2.0 ml, 0.66 mmol) and iron powder (680 mg, 12.2 mmol). The reaction mixtur...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)[nH]c1cnccc12
Other
[Fe].C(C)(=O)OCC.C(C)O
60
20
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]>[Fe].C(C)(=O)OCC.C(C)O>CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-44615147f6f746779af7e52873f60a22
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O>>CCSc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
O.ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)N.CC1=C(C(=O)O)C=CC=N1.Cl.CN(CCCN=C=NCC)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)NC(C1=C(N=CC=C1)C)=O
[CH3:1][CH2:2][S:3][c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[NH2:18].O[C:19](=[O:20])[c:21]1[cH:22][cH:23][cH:24][n:25][c:26]1[CH3:27]>>[CH3:1][CH2:2][S:3][c:4]1[c:5]([Cl:6])[cH:7][c:8]2[c:9]([nH:10][c:11]3[cH:12][n:13][cH:14][cH:15][c:16]23)[c:17]1[NH:18][C:19](=[O:...
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
null
null
CO.N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]):[c:17]
40.7
[{"value": 38.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)NC(C1=C(N=CC=C1)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 40.7, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCC)NC(C1=C(N=CC=C1)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
2.5
HOUR
A 25 ml round-bottom flask with magnetic stirrer was charged with 6-chloro-7-ethylsulfanyl-9H-β-carbolin-8-ylamine (37.2 mg, 0.13 mmol) and 2-methylnicotinic acid (36.2 mg, 0.26 mmol) in 3 ml anhydrous pyridine. To the resulting light-orange mixture at RT was added solid 1-(3-dimethylaminopropyl)-3-ethylcarbodiimide hy...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2c(c1)[nH]c1cnccc12.c1ccncc1
HO-
CO.N1=CC=CC=C1
80
2.5
CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N.Cc1ncccc1C(=O)O>CO.N1=CC=CC=C1>CCSc1c(Cl)cc2c([nH]c3cnccc32)c1NC(=O)c1cccnc1C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-bc514ad0e3e84d83be2220180f062766
CN(C)CCS.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>>CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
C(CCC)[Li].O.Cl.CN(CCS)C.ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-].ClC=1C=C2C=3C=CN=CC3NC2=C(C1F)[N+](=O)[O-]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCCN(C)C)[N+](=O)[O-]
[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][SH:6].F[c:7]1[c:8]([Cl:9])[cH:10][c:11]2[c:12]([nH:13][c:14]3[cH:15][n:16][cH:17][cH:18][c:19]23)[c:20]1[N+:21](=[O:22])[O-:23]>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][S:6][c:7]1[c:8]([Cl:9])[cH:10][c:11]2[c:12]([nH:13][c:14]3[cH:15][n:16][cH:17][cH:18][c:19]23)[c:20]1[N+:21](=[O:22])[O...
CN(C)CCS.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12
CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
thioether_nucl_sub
3da7ce1aea3b8504c3ad35910fac5c4b5425645a60840f47f11ee73ab00296e4
b7fe376f7aad2517725eef26ab981e4baa6c31c5f38fdf89e7c52a4a2c6cc1d2
c1ccc2c(c1)[nH]c1cnccc12
F-[c;H0;D3;+0:1]1:[c:2](-[#7;+:3]):[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11]:1-[Cl;D1;H0:12].[C:13]-[C:14]-[SH;D1;+0:15]>>[#7;+:3]-[c:2]1:[c:4](:[#7;a:5]:[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:[c:11](-[Cl;D1;H0:12]):[c;H0;D3;+0:1]:1-[S;H0;D2;+0:15]-[C:14]-[C:13]
84
[{"value": 83.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCCN(C)C)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCCN(C)C)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
A 25 ml round-bottom flask with magnetic stirrer was charged with 6-chloro-7-fluoro-8-nitro-9H-β-carboline (98 mg, 0.37 mmol) in 2 ml of anhydrous DMF. A second 10 ml round-bottom flask with magnetic stirrer was charged with 2-dimethylamino-ethanethiol hydrochloride (100 mg, 0.70 mmol) in 2 ml anhydrous DMF. To the res...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aliphatic thiol
Monosulfide
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
HF
CN(C)C=O
null
0.083333
CN(C)CCS.O=[N+]([O-])c1c(F)c(Cl)cc2c1[nH]c1cnccc12>CN(C)C=O>CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-6cee690533f34e0b838930aeaf183eee
CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]>>CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N
C.ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCCN(C)C)[N+](=O)[O-].[Cl-].[NH4+]>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCCN(C)C)N
O=[N+:21]([O-])[c:20]1[c:7]([S:6][CH2:5][CH2:4][N:2]([CH3:1])[CH3:3])[c:8]([Cl:9])[cH:10][c:11]2[c:12]1[nH:13][c:14]1[cH:15][n:16][cH:17][cH:18][c:19]21>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][S:6][c:7]1[c:8]([Cl:9])[cH:10][c:11]2[c:12]([nH:13][c:14]3[cH:15][n:16][cH:17][cH:18][c:19]23)[c:20]1[NH2:21]
CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]
CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N
null
[Fe]
C(C)(=O)OCC.C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)[nH]c1cnccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
107
[{"value": 107.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1SCCN(C)C)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
20
HOUR
A 50 ml round-bottom flask with a magnetic stirrer was charged with [2-(6-chloro-8-nitro-9H-β-carbolin-7-ylsulfanyl)-ethyl]-dimethyl-amine (106 mg, 0.30 mmol) in 8 ml of anhydrous ethanol. To the resulting orange mixture at RT was added 0.33 M aqueous ammonium chloride (1.95 ml, 0.64 mmol) and iron powder (540 mg, 9.67...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)[nH]c1cnccc12
Other
[Fe].C(C)(=O)OCC.C(C)O
60
20
CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1[N+](=O)[O-]>[Fe].C(C)(=O)OCC.C(C)O>CN(C)CCSc1c(Cl)cc2c([nH]c3cnccc32)c1N
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-3ffd78dd4f844473bdb2ea6319713d8b
C=O.Nc1cc(Cl)cc2c1[nH]c1cnccc12.O=C(O)[C@@H]1COCCN1>>CN1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)N.[H][H].[H][H].CCN=C=NCCCN(C)C.C=O.N1[C@@H](COCC1)C(=O)O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CCOC1)C
O=[CH2:1].[NH2:10][c:11]1[cH:12][c:13]([Cl:14])[cH:15][c:16]2[c:17]1[nH:18][c:19]1[cH:20][n:21][cH:22][cH:23][c:24]21.O[C:8]([C@H:7]1[NH:2][CH2:3][CH2:4][O:5][CH2:6]1)=[O:9]>>[CH3:1][N:2]1[CH2:3][CH2:4][O:5][CH2:6][C@H:7]1[C:8](=[O:9])[NH:10][c:11]1[cH:12][c:13]([Cl:14])[cH:15][c:16]2[c:17]1[nH:18][c:19]1[cH:20][n:21][...
C=O.Nc1cc(Cl)cc2c1[nH]c1cnccc12.O=C(O)[C@@H]1COCCN1
CN1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
[OH-].[OH-].[Pd+2]
CCOC(=O)C.O.CCO.N1=CC=CC=C1
Acylation
OtherReaction
1140aa8e8a72239787370cdb74da1e146344133144d5b62cd65b1ad8eb815c35
a78fd64159b1fe951d321c8198aec02a42ac5f4d2ec5f5a84b6bc592c4e1891e
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[#8:5]-[C:6]-[C:7]-[NH;D2;+0:8]-1.O=[CH2;D1;+0:9].[#7;a:10]:[c:11]:[c:12]:[#7;a:13]:[c:14](:[c:15]):[c:16](-[NH2;D1;+0:17]):[c:18]>>[#7;a:10]:[c:11]:[c:12]:[#7;a:13]:[c:14](:[c:15]):[c:16](-[NH;D2;+0:17]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[#8:5]-[C:6]-[C:7]-[N;H0;D3;+0...
54.5
[{"value": 54.5, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CCOC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
A slurry of morpholine-3(S)-carboxylic acid (3.00 g, 22.9 mmol) in EtOH (115 ml) was stirred at RT. A solution of aqueous CH2O (3.42 ml, 45.8 mmol, 37% w/w in H2O) was added, followed by Pd(OH)2 (600 mg, 20% w/w on charcoal). The flask was charged with hydrogen (1 atm) and the grey slurry was stirred for 24 hr at RT un...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Carboxylic acid.Primary amine.Secondary amine
Secondary amide.Tertiary amine
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
[OH-].[OH-].[Pd+2].CCOC(=O)C.O.CCO.N1=CC=CC=C1
null
24
C=O.Nc1cc(Cl)cc2c1[nH]c1cnccc12.O=C(O)[C@@H]1COCCN1>[OH-].[OH-].[Pd+2].CCOC(=O)C.O.CCO.N1=CC=CC=C1>CN1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2b280253fe694eeb9c97b4f613f7983b
CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
CCN=C=NCCCN(C)C.CCOC(=O)C.C(C)(C)(C)OC(=O)N1[C@@H](COCC1)C(=O)O.ClC=1C=C2C=3C=CN=CC3NC2=C(C1)N>>C(C)(C)(C)OC(=O)N1[C@@H](COCC1)C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O
O[C:14]([C@H:13]1[N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:9][CH2:10][O:11][CH2:12]1)=[O:15].[NH2:16][c:17]1[cH:18][c:19]([Cl:20])[cH:21][c:22]2[c:23]1[nH:24][c:25]1[cH:26][n:27][cH:28][cH:29][c:30]21>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][O:11][CH2:12][C@H:13]1[C:14](=...
CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12
CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
O.[Cl-].[Na+].O.N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4]-[#8:5])-[#7:6](-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13])-[C:14].[#7;a:15]:[c:16]:[c:17]:[#7;a:18]:[c:19](:[c:20]):[c:21](-[NH2;D1;+0:22]):[c:23]>>[#7;a:15]:[c:16]:[c:17]:[#7;a:18]:[c:19](:[c:20]):[c:21](-[NH;D2;+0:22]-[C;H0;D3;+0:1](=[O;D1...
null
[]
null
null
14
HOUR
A solution of morpholine-3(S),4-dicarboxylic acid 4-tert-butyl ester (2.83 g, 12.7 mmol) in pyridine (106 ml) was stirred at RT. 6-chloro-9H-β-carbolin-8-ylamine (2.30 g, 10.6 mmol) was added, followed by EDCI (4.06 g, 21.2 mmol). The clear orange-to-brown solution was stirred at RT for 14 hr. The solution was diluted ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
O.[Cl-].[Na+].O.N1=CC=CC=C1
null
14
CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12>O.[Cl-].[Na+].O.N1=CC=CC=C1>CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-50d4c2e26ecd476e9c7e1be4b22dd7e7
CC(C)(C)OC(=O)N1CCC[C@@H]1C=O.CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CC(C)(C)OC(=O)N1CCC[C@@H]1CN1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+].FC(C(=O)O)(F)F.C(C)(C)(C)OC(=O)N1[C@@H](COCC1)C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O.C(C)(C)(C)OC(=O)N1[C@@H](C=O)CCC1>>C(C)(C)(C)OC(=O)N1[C@H](CCC1)CN1[C@@H](COCC1)C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O
O=[CH:13][C@@H:12]1[N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:9][CH2:10][CH2:11]1.CC(C)(C)OC(=O)[N:14]1[CH2:15][CH2:16][O:17][CH2:18][C@H:19]1[C:20](=[O:21])[NH:22][c:23]1[cH:24][c:25]([Cl:26])[cH:27][c:28]2[c:29]1[nH:30][c:31]1[cH:32][n:33][cH:34][cH:35][c:36]21>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:...
CC(C)(C)OC(=O)N1CCC[C@@H]1C=O.CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
CC(C)(C)OC(=O)N1CCC[C@@H]1CN1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
C1CCOC1.CO.C(Cl)Cl.C(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
07a8dd0a63a2f032256383ed14d5b2300f3182a12f0d3bca1f1edfc26fa061f9
cf54569061a197ba9f3cab07727ad571966e8f550ff4245a3fd82ef36fe97477
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1C[C@H]1CCCN1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1-[C:7](=[O;D1;H0:8])-[#7:9]-[c:10]:[c:11]:[#7;a:12].O=[CH;D2;+0:13]-[C:14](-[C:15])-[#7:16](-[C:17](=[O;D1;H0:18])-[#8:19]-[C:20](-[C;D1;H3:21])(-[C;D1;H3:22])-[C;D1;H3:23])-[C:24]>>[#7;a:12]:[c:11]:[c:10]-[#7:9]-[C:7](=[O;D1;H0:8])-[C:6]1-[C:5]-[#8:4]...
76.7
[{"value": 76.7, "product": "C(C)(C)(C)OC(=O)N1[C@H](CCC1)CN1[C@@H](COCC1)C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
45
MINUTE
A solution of 3(S)-(6-chloro-9H-β-carbolin-8-ylcarbamoyl)-morpholine-4-carboxylic acid tert-butyl ester (1.00 g, 2.32 mmol) in CH2Cl2 (6 ml) was stirred at RT. Trifluoroacetic acid (6 ml) was added and the solution was stirred at RT for 45 min, then concentrated to a residue. The residue was concentrated once more from...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Carbamic ester.Ether.Boc
Tertiary amine
C1COCC[NH]1
C1COCC[NH]1
C1CC[NH]C1.C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
C1CCOC1.CO.C(Cl)Cl.C(Cl)Cl
null
0.75
CC(C)(C)OC(=O)N1CCC[C@@H]1C=O.CC(C)(C)OC(=O)N1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>C1CCOC1.CO.C(Cl)Cl.C(Cl)Cl>CC(C)(C)OC(=O)N1CCC[C@@H]1CN1CCOC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-d432fcaf3af3447bbf3a4599b44cc9a3
CC(C)(C)OC(=O)NC1CCCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>>N[C@H]1CCC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1C(CCC1)NC(=O)OC(C)(C)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1[C@H](CCC1)N
CC(C)(C)OC(=O)[NH:1][CH:2]1[CH2:3][CH2:4][CH2:5][CH:6]1[C:7](=[O:8])[NH:9][c:10]1[cH:11][c:12]([Cl:13])[cH:14][c:15]2[c:16]1[nH:17][c:18]1[cH:19][n:20][cH:21][cH:22][c:23]21>>[NH2:1][C@H:2]1[CH2:3][CH2:4][CH2:5][C@H:6]1[C:7](=[O:8])[NH:9][c:10]1[cH:11][c:12]([Cl:13])[cH:14][c:15]2[c:16]1[nH:17][c:18]1[cH:19][n:20][cH:2...
CC(C)(C)OC(=O)NC1CCCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
N[C@H]1CCC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
FC(C(=O)O)(F)F
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=C(Nc1cccc2c1[nH]c1cnccc12)C1CCCC1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[CH;D3;+0:2]1-[C:3]-[C:4]-[C:5]-[CH;D3;+0:6]-1-[C:7](=[O;D1;H0:8])-[#7:9]-[c:10]:[c:11]:[#7;a:12]>>[#7;a:12]:[c:11]:[c:10]-[#7:9]-[C:7](=[O;D1;H0:8])-[C@@H;D3;+0:6]1-[C:5]-[C:4]-[C:3]-[C@@H;D3;+0:2]-1-[NH2;D1;+0:1]
106.1
[{"value": 106.1, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1[C@H](CCC1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A solution of 2-(tert-butoxycarbonylamino)-cyclopentanecarboxylic acid (6-chloro-9H-β-carbolin-8-yl) amide (736 mg, 1.72 mmol) in trifluoroacetic acid (5 ml) was stirred at RT for 20 min, then concentrated to an orange oil. The oil was dissolved in MeOH (5 ml) and neutralized with a saturated aqueous sodium bicarbonate...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
C1CCCC1.c1ccc2c(c1)[nH]c1cnccc12
HO-
FC(C(=O)O)(F)F
null
0.5
CC(C)(C)OC(=O)NC1CCCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>FC(C(=O)O)(F)F>N[C@H]1CCC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-89d195654d274ffc9909fd1658d0890f
CC(C)(C)OC(=O)N[C@H]1CCCC[C@H]1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12.[Na+]>>NC1CCCCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.[Na+]
FC(C(=O)O)(F)F.ClC=1C=C2C=3C=CN=CC3NC2=C(C1)N.CCN=C=NCCCN(C)C.C(C)(C)(C)OC(=O)N[C@@H]1[C@@H](CCCC1)C(=O)O.C(=O)([O-])[O-].[Na+].[Na+]>>C(=O)([O-])[O-].[Na+].[Na+].ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1C(CCCC1)N
CC(C)(C)OC(=O)[NH:1][C@H:2]1[CH2:3][CH2:4][CH2:5][CH2:6][C@H:7]1[C:8](O)=[O:9].[NH2:10][c:11]1[cH:12][c:13]([Cl:14])[cH:15][c:16]2[c:17]1[nH:18][c:19]1[cH:20][n:21][cH:22][cH:23][c:24]21.[Na+:29]>>[NH2:1][CH:2]1[CH2:3][CH2:4][CH2:5][CH2:6][CH:7]1[C:8](=[O:9])[NH:10][c:11]1[cH:12][c:13]([Cl:14])[cH:15][c:16]2[c:17]1[nH:...
CC(C)(C)OC(=O)N[C@H]1CCCC[C@H]1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12.[Na+]
NC1CCCCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.[Na+]
null
null
CCOC(=O)C.O.CO.C(Cl)Cl.N1=CC=CC=C1
Acylation
OtherReaction
b4c20342f55b434660078663f02be082076e2ff9b9068db91acc0b381022a32e
e525bb030a9f5f4a2fc47bce923bf921a3769ce3300b3fa2600575194671a3f3
O=C(Nc1cccc2c1[nH]c1cnccc12)C1CCCCC1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C@H;D3;+0:2]1-[C:3]-[C:4]-[C:5]-[C:6]-[C@H;D3;+0:7]-1-[C;H0;D3;+0:8](-O)=[O;D1;H0:9].[#7;a:10]:[c:11]:[c:12]:[#7;a:13]:[c:14](:[c:15]):[c:16](-[NH2;D1;+0:17]):[c:18]>>[#7;a:10]:[c:11]:[c:12]:[#7;a:13]:[c:14](:[c:15]):[c:16](-[NH;D2;+0:17]-[C;H0;D3;+0:8](=[O;D1;H0:9])-[CH;D3;+0:7]1-[C:6...
null
[]
null
null
16
HOUR
A solution of cis-2-(tert-butoxycarbonylamino)-cyclohexane carboxylic acid (255 mg, 1.05 mmol) in pyridine (10 ml) was stirred at RT. 6-chloro-9H-β-carbolin-8-ylamine (218 mg, 1.00 mmol) was added, followed by EDCI (315 mg, 1.64 mmol) and the slightly turbid pale orange solution was stirred at RT for 16 hr. The solutio...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Carboxylic acid.Ether.Primary amine.Boc
Secondary amide.Primary amine
null
null
C1CCCCC1.c1ccc2c(c1)[nH]c1cnccc12
HO-
CCOC(=O)C.O.CO.C(Cl)Cl.N1=CC=CC=C1
null
16
CC(C)(C)OC(=O)N[C@H]1CCCC[C@H]1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12.[Na+]>CCOC(=O)C.O.CO.C(Cl)Cl.N1=CC=CC=C1>NC1CCCCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.[Na+]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a9c8b2ef391f41859897bec5f3ce5352
O.O=C(c1ccccc1)N1CCc2c([nH]c3ccc(Cl)cc23)C1>>O=C1CN(C(=O)c2ccccc2)Cc2[nH]c3ccc(Cl)cc3c21
ClC=1C=C2C=3CCN(CC3NC2=CC1)C(=O)C1=CC=CC=C1.C(#N)C1=C(C(=O)C(=C(C1=O)Cl)Cl)C#N.C1CCOC1.O>>C(C1=CC=CC=C1)(=O)N1CC=2NC3=CC=C(C=C3C2C(C1)=O)Cl
[OH2:1].[CH2:2]1[CH2:3][N:4]([C:5](=[O:6])[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[CH2:13][c:14]2[nH:15][c:16]3[cH:17][cH:18][c:19]([Cl:20])[cH:21][c:22]3[c:23]21>>[O:1]=[C:2]1[CH2:3][N:4]([C:5](=[O:6])[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[CH2:13][c:14]2[nH:15][c:16]3[cH:17][cH:18][c:19]([Cl:20])[cH:21][c:22]3[c:2...
O.O=C(c1ccccc1)N1CCc2c([nH]c3ccc(Cl)cc23)C1
O=C1CN(C(=O)c2ccccc2)Cc2[nH]c3ccc(Cl)cc3c21
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
94fb5a061868702b7ba4b162fda0d481a656d3f8461c89d8da115f78d870c628
a196f7191876ee39420290ab9d6c2b9eeb3251b37ae345fc435efba1949a85d9
O=C1CN(C(=O)c2ccccc2)Cc2[nH]c3ccccc3c21
[O;D1;H0:1]=[C:2]-[#7:3]1-[C:4]-[c:5]2:[#7;a:6]:[c:7]:[c:8]:[c:9]:2-[CH2;D2;+0:10]-[C:11]-1.[OH2;D0;+0:12]>>[O;D1;H0:1]=[C:2]-[#7:3]1-[C:4]-[c:5]2:[#7;a:6]:[c:7]:[c:8]:[c:9]:2-[C;H0;D3;+0:10](=[O;H0;D1;+0:12])-[C:11]-1
75.1
[{"value": 75.0, "product": "C(C1=CC=CC=C1)(=O)N1CC=2NC3=CC=C(C=C3C2C(C1)=O)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 75.1, "product": "C(C1=CC=CC=C1)(=O)N1CC=2NC3=CC=C(C=C3C2C(C1)=O)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
2
HOUR
(6-chloro-1,3,4,9-tetrahydro-β-carbolin-2-yl)-phenyl-methanone (1.76 g, 5.66 mmol, 1 equiv.) and DDQ (2.31 g, 10.2 mmol, 1.8 equiv.) were mixed as solids and cooled to −78° C. 15 ml of a 9:1 THF/H2O solution was cooled to −78° C. and the resulting slurry was added to the cooled solids followed by an additional 15 ml of...
10.6084/m9.figshare.5104873.v1
null
null
Ketone
c1ccc2c3c(nc2c1)C[N]CC3
c1ccc2c3c(nc2c1)C[N]CC3
c1ccccc1.c1ccc2c3c(nc2c1)C[N]CC3
null
C1CCOC1
-78
2
O.O=C(c1ccccc1)N1CCc2c([nH]c3ccc(Cl)cc23)C1>C1CCOC1>O=C1CN(C(=O)c2ccccc2)Cc2[nH]c3ccc(Cl)cc3c21
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-7898338d32e44508a9b26d36d2f6cd9f
NN.O=C1CN(C(=O)c2ccccc2)Cc2[nH]c3ccc(Cl)cc3c21>>Nc1cncc2[nH]c3ccc(Cl)cc3c12
C(C1=CC=CC=C1)(=O)N1CC=2NC3=CC=C(C=C3C2C(C1)=O)Cl.NN>>NC1=CN=CC=2NC3=CC=C(C=C3C12)Cl
N[NH2:1].O=C(c1ccccc1)[N:4]1[CH2:3][C:2](=O)[c:15]2[c:6]([nH:7][c:8]3[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]32)[CH2:5]1>>[NH2:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]3[c:15]12
NN.O=C1CN(C(=O)c2ccccc2)Cc2[nH]c3ccc(Cl)cc3c21
Nc1cncc2[nH]c3ccc(Cl)cc3c12
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
74c41a61e84a9469a525e15f8dfef263462c61ba637c9c616d03a23850e3333b
2a646b944ed492fc0f255d8794451efd5267945a96cfe9177952895f86f62143
c1ccc2c(c1)[nH]c1cnccc12
N-[NH2;D1;+0:1].O=C(-[N;H0;D3;+0:2]1-[CH2;D2;+0:3]-[C;H0;D3;+0:4](=O)-[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2-[CH2;D2;+0:10]-1)-c1:c:c:c:c:c:1>>[NH2;D1;+0:1]-[c;H0;D3;+0:4]1:[cH;D2;+0:3]:[n;H0;D2;+0:2]:[cH;D2;+0:10]:[c:9]2:[#7;a:8]:[c:7]:[c:6]:[c:5]:2:1
30
[{"value": 30.0, "product": "NC1=CN=CC=2NC3=CC=C(C=C3C12)Cl", "details": "PERCENTYIELD", "is_desired": false}]
130
CELSIUS
8
HOUR
Crude 2-benzoyl-6-chloro-1,2,3,9-tetrahydro-β-carbolin-4-one (4 g) was dissolved in 30 ml of anhydrous hydrazine and stirred at reflux (130° C. oil bath) under N2 for 6 hours, after which the reaction mixture was allowed to cool to room temperature and sit overnight. The precipitated yellow solids were removed by filtr...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Ketone.Tertiary amide
Primary amine
c1ccccc1.c1ccc2c3c(nc2c1)C[N]CC3
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
HO-
null
130
8
NN.O=C1CN(C(=O)c2ccccc2)Cc2[nH]c3ccc(Cl)cc3c21>>Nc1cncc2[nH]c3ccc(Cl)cc3c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f4a8badd434f420299d63634ba616cce
O=C(Nc1cncc2[nH]c3ccc(Cl)cc3c12)C(F)(F)F.O=N[O-]>>O=C(Nc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12)C(F)(F)F
ClC=1C=C2C=3C(=CN=CC3NC2=CC1)NC(C(F)(F)F)=O.N(=O)[O-].[Na+]>>ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)[N+](=O)[O-])NC(C(F)(F)F)=O
[O:1]=[C:2]([NH:3][c:4]1[cH:5][n:6][cH:7][c:8]2[nH:9][c:10]3[cH:11][cH:15][c:16]([Cl:17])[cH:18][c:19]3[c:20]12)[C:21]([F:22])([F:23])[F:24].[N:12](=[O:13])[O-:14]>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][n:6][cH:7][c:8]2[nH:9][c:10]3[c:11]([N+:12](=[O:13])[O-:14])[cH:15][c:16]([Cl:17])[cH:18][c:19]3[c:20]12)[C:21]([F:22])([F:2...
O=C(Nc1cncc2[nH]c3ccc(Cl)cc3c12)C(F)(F)F.O=N[O-]
O=C(Nc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12)C(F)(F)F
null
null
C(=O)(C(F)(F)F)O
Heteroatom Alkylation and Arylation
Aromatic nitration with NO2 salt
27d40c1a20be8489ca12a83b18d23e1c4bd9993bff3d46a4c37aaa2b269b5ab4
1afb031e90b32de55305394c30af064cce0ffa4f7a6ceb037d1648f24219cbc1
c1ccc2c(c1)[nH]c1cnccc12
[#7;a:1]:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[cH;D2;+0:7]:[c:8]:[c:9].[O;-;D1;H0:10]-[N;H0;D2;+0:11]=[O;D1;H0:12]>>[#7;a:1]:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c;H0;D3;+0:7](-[N+;H0;D3:11](-[O;-;D1;H0:10])=[O;D1;H0:12]):[c:8]:[c:9]
92
[{"value": 92.0, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)[N+](=O)[O-])NC(C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.0, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)[N+](=O)[O-])NC(C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
N-(6-chloro-9H-β-carbolin-4-yl)-2,2,2-trifluoro-acetamide (125 mg, 0.4 mmol, 1 equiv.) was dissolved in 2 ml TFA and NaNO2 (541 mg, 7.84 mmol, 2 equiv.) was added in one portion. The solution was stirred at room temperature for 4 hr. Volatiles were removed by rotovap, and the resulting oily orange solids were suspended...
10.6084/m9.figshare.5104873.v1
null
Nitroso
Nitro group
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
null
C(=O)(C(F)(F)F)O
null
4
O=C(Nc1cncc2[nH]c3ccc(Cl)cc3c12)C(F)(F)F.O=N[O-]>C(=O)(C(F)(F)F)O>O=C(Nc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12)C(F)(F)F
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-43960de9c44a4b3286a26c07d143e575
O=C(Nc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12)C(F)(F)F>>Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12
ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)[N+](=O)[O-])NC(C(F)(F)F)=O>>NC=1C=C(C=C2C=3C(=CN=CC3NC12)NC(C(F)(F)F)=O)Cl
O=[N+:1]([O-])[c:2]1[cH:3][c:4]([Cl:5])[cH:6][c:7]2[c:8]1[nH:9][c:10]1[cH:11][n:12][cH:13][c:14]([NH:15][C:16](=[O:17])[C:18]([F:19])([F:20])[F:21])[c:22]21>>[NH2:1][c:2]1[cH:3][c:4]([Cl:5])[cH:6][c:7]2[c:8]1[nH:9][c:10]1[cH:11][n:12][cH:13][c:14]([NH:15][C:16](=[O:17])[C:18]([F:19])([F:20])[F:21])[c:22]21
O=C(Nc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12)C(F)(F)F
Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12
null
null
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)[nH]c1cnccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
95
[{"value": 95.0, "product": "NC=1C=C(C=C2C=3C(=CN=CC3NC12)NC(C(F)(F)F)=O)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.7, "product": "NC=1C=C(C=C2C=3C(=CN=CC3NC12)NC(C(F)(F)F)=O)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The crude N-(6-chloro-8-nitro-9H-β-carbolin-4-yl)-2,2,2-trifluoro-acetamide (130 mg, 0.36 mmol) was dissolved in 7 ml of MeOH and the reaction vessel was vacuum purged 3× with N2. Platinum (20 mg, 20% wt. on activated carbon) was added quickly, and the reaction vessel was again vacuum purged 3× with N2, followed by 3 a...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)[nH]c1cnccc12
Other
CO
null
8
O=C(Nc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12)C(F)(F)F>CO>Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-729d7e71038f4e0fbe7010d97014baa8
Cc1ncccc1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12>>Cc1ncccc1C(=O)Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12
NC=1C=C(C=C2C=3C(=CN=CC3NC12)NC(C(F)(F)F)=O)Cl.CC1=C(C(=O)O)C=CC=N1.CCN=C=NCCCN(C)C>>ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=C(N=CC=C1)C)=O)NC(C(F)(F)F)=O
O[C:8]([c:7]1[c:2]([CH3:1])[n:3][cH:4][cH:5][cH:6]1)=[O:9].[NH2:10][c:11]1[cH:12][c:13]([Cl:14])[cH:15][c:16]2[c:17]1[nH:18][c:19]1[cH:20][n:21][cH:22][c:23]([NH:24][C:25](=[O:26])[C:27]([F:28])([F:29])[F:30])[c:31]21>>[CH3:1][c:2]1[n:3][cH:4][cH:5][cH:6][c:7]1[C:8](=[O:9])[NH:10][c:11]1[cH:12][c:13]([Cl:14])[cH:15][c:...
Cc1ncccc1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12
Cc1ncccc1C(=O)Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12
null
null
N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]):[c:17]
33.4
[{"value": 3.0, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=C(N=CC=C1)C)=O)NC(C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 33.4, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=C(N=CC=C1)C)=O)NC(C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
N-(8-amino-6-chloro-9H-β-carbolin-4-yl)-2,2,2-trifluoro-acetamide (90 mg, 0.274 mmol, 1 equiv.) and 2-methylnicotinic acid (45 mg, 0.329 mmol, 1.2 equiv.) were dissolved in 1.5 ml of anhydrous pyridine under N2. EDCI (84 mg, 0.438 mmol, 1.6 equiv.) was added in one portion and the reaction mixture was stirred at room t...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccncc1.c1ccc2c(c1)[nH]c1cnccc12
HO-
N1=CC=CC=C1
null
2
Cc1ncccc1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12>N1=CC=CC=C1>Cc1ncccc1C(=O)Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-0ba7be200a0745fa8dcb6c2a37b8dd3a
Cc1ncccc1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12>>O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1
NC=1C=C(C=C2C=3C(=CN=CC3NC12)NC(C(F)(F)F)=O)Cl.CC1=C(C(=O)O)C=CC=N1.CCN=C=NCCCN(C)C>>ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=CN=CC=C1)=O)NC(C(F)(F)F)=O
C[c:30]1[c:25]([C:2](O)=[O:1])[cH:26][cH:27][cH:28][n:29]1.[NH2:3][c:4]1[cH:5][c:6]([Cl:7])[cH:8][c:9]2[c:10]1[nH:11][c:12]1[cH:13][n:14][cH:15][c:16]([NH:17][C:18](=[O:19])[C:20]([F:21])([F:22])[F:23])[c:24]21>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][c:6]([Cl:7])[cH:8][c:9]2[c:10]1[nH:11][c:12]1[cH:13][n:14][cH:15][c:16]([NH:1...
Cc1ncccc1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12
O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1
null
null
N1=CC=CC=C1
Acylation
OtherReaction
b405a961806bf7c0480e9ba70bff09e2357d2e443a48745daf408dff4513f433
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
C-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[C;H0;D3;+0:5](-O)=[O;D1;H0:6]):[c:7].[#7;a:8]:[c:9]:[c:10]:[#7;a:11]:[c:12](:[c:13]):[c:14](-[NH2;D1;+0:15]):[c:16]>>[#7;a:8]:[c:9]:[c:10]:[#7;a:11]:[c:12](:[c:13]):[c:14](-[NH;D2;+0:15]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[c:4](:[c:7]):[cH;D2;+0:1]:[#7;a:2]:[c:3]):[c:16]
32
[{"value": 32.0, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=CN=CC=C1)=O)NC(C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 32.0, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=CN=CC=C1)=O)NC(C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
N-(8-amino-6-chloro-9H-β-carbolin-4-yl)-2,2,2-trifluoro-acetamide (90 mg, 0.274 mmol, 1 equiv.) and 2-methylnicotinic acid (40 mg, 0.329 mmol, 1.2 equiv.) were dissolved in 1.5 ml of anhydrous pyridine under N2. EDCI (84 mg, 0.438 mmol, 1.6 equiv.) was added in one portion and the reaction mixture was stirred at room t...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
c1ccncc1
c1ccncc1
c1ccc2c(c1)[nH]c1cnccc12.c1ccncc1
HO-
N1=CC=CC=C1
null
2
Cc1ncccc1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12>N1=CC=CC=C1>O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-49d4afb4172b4e4e82801fe1f568d711
O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1>>Cc1ncccc1C(=O)Nc1cc(Cl)cc2c1[nH]c1cncc(N)c12
O.ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=CN=CC=C1)=O)NC(C(F)(F)F)=O.C(=O)([O-])[O-].[K+].[K+]>>NC1=CN=CC=2NC3=C(C=C(C=C3C12)Cl)NC(C1=C(N=CC=C1)C)=O
O=C(C(F)(F)F)[NH:24][c:23]1[cH:22][n:21][cH:20][c:19]2[nH:18][c:17]3[c:11]([NH:10][C:8]([c:7]4[cH:2][n:3][cH:4][cH:5][cH:6]4)=[O:9])[cH:12][c:13]([Cl:14])[cH:15][c:16]3[c:25]21>>[CH3:1][c:2]1[n:3][cH:4][cH:5][cH:6][c:7]1[C:8](=[O:9])[NH:10][c:11]1[cH:12][c:13]([Cl:14])[cH:15][c:16]2[c:17]1[nH:18][c:19]1[cH:20][n:21][cH...
O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1
Cc1ncccc1C(=O)Nc1cc(Cl)cc2c1[nH]c1cncc(N)c12
null
null
CO
Functional Group Interconversion
OtherReaction
7bdade8e10f63ec35b6f5b02073a2818fdc259338138d32e1d3670d7016f6d6a
93e9ea1ae4bf2c4ff35caff092b0418f72119be3ac8ebfa7d8fb2a9b49b6c3cb
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
F-C(-F)(-F)-C(=O)-[NH;D2;+0:1]-[c:2]1:[c:3]:[#7;a:4]:[c:5]:[c:6](:[#7;a:7]:[c:8]:[c:9]-[#7:10]-[C:11](=[O;D1;H0:12])-[c:13](:[c:14]):[cH;D2;+0:15]:[#7;a:16]:[c:17]):[c:18]:1>>[C;D1;H3:19]-[c;H0;D3;+0:15](:[#7;a:16]:[c:17]):[c:13](-[C:11](=[O;D1;H0:12])-[#7:10]-[c:9]:[c:8]:[#7;a:7]:[c:6]1:[c:5]:[#7;a:4]:[c:3]:[c:2](-[NH...
56
[{"value": 56.0, "product": "NC1=CN=CC=2NC3=C(C=C(C=C3C12)Cl)NC(C1=C(N=CC=C1)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 55.6, "product": "NC1=CN=CC=2NC3=C(C=C(C=C3C12)Cl)NC(C1=C(N=CC=C1)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
N-[6-chloro-4-(2,2,2-trifluoro-acetylamino)-9H-β-carbolin-8-yl]-nicotinamide (41 mg, 0.092 mmol, 1 equiv.) was suspended in 5 ml of MeOH and a 2 ml aqueous solution of K2CO3 (127 mg, 0.92 mmol, 10 equiv.) was added thereto. The resulting clear solution was heated at 60° C. for 16 hr and then allowed to cool to RT. Addi...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Secondary amide
Primary amine
c1ccncc1
c1ccncc1
c1ccncc1.c1ccc2c(c1)[nH]c1cnccc12
Other
CO
60
null
O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1>CO>Cc1ncccc1C(=O)Nc1cc(Cl)cc2c1[nH]c1cncc(N)c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-fdd49f50cce6498b86f686e7514911b8
O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1>>Nc1cncc2[nH]c3c(NC(=O)c4cccnc4)cc(Cl)cc3c12
ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=CN=CC=C1)=O)NC(C(F)(F)F)=O.C(=O)([O-])[O-].[K+].[K+]>>NC1=CN=CC=2NC3=C(C=C(C=C3C12)Cl)NC(C1=CN=CC=C1)=O
O=C(C(F)(F)F)[NH:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[c:9]([NH:10][C:11](=[O:12])[c:13]4[cH:14][cH:15][cH:16][n:17][cH:18]4)[cH:19][c:20]([Cl:21])[cH:22][c:23]3[c:24]12>>[NH2:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[c:9]([NH:10][C:11](=[O:12])[c:13]4[cH:14][cH:15][cH:16][n:17][cH:18]4)[cH:19][c:20]([Cl:21])[c...
O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1
Nc1cncc2[nH]c3c(NC(=O)c4cccnc4)cc(Cl)cc3c12
null
null
CO
Reduction
Hydrogenolysis of amides/imides/carbamates
44b36597c7daf0608965c52c8db8a9220c21d9447ce54e0af375898475f3493f
caaeb83af2cb178156ae90fe7f610a106cd4bb5397d23f56d37a7fe11e2668ed
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
F-C(-F)(-F)-C(=O)-[NH;D2;+0:1]-[c:2]1:[c:3]:[c:4](:[#7;a:5]):[c:6]:[#7;a:7]:[c:8]:1>>[#7;a:5]:[c:4]1:[c:3]:[c:2](-[NH2;D1;+0:1]):[c:8]:[#7;a:7]:[c:6]:1
10
[{"value": 10.0, "product": "NC1=CN=CC=2NC3=C(C=C(C=C3C12)Cl)NC(C1=CN=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 9.4, "product": "NC1=CN=CC=2NC3=C(C=C(C=C3C12)Cl)NC(C1=CN=CC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
N-[6-chloro-4-(2,2,2-trifluoro-acetylamino)-9H-β-carbolin-8-yl]-nicotinamide (38 mg, 0.088 mmol, 1 equiv.) was suspended in 5 ml of MeOH and a 2 ml aqueous solution of K2CO3 (121 mg, 0.92 mmol, 10 equiv.) was added thereto. The resulting clear solution was heated at 60° C. for 11 hr. After cooling to RT, fine solids pr...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Secondary amide
Primary amine
null
null
c1ccncc1.c1ccc2c(c1)[nH]c1cnccc12
Other
CO
60
null
O=C(Nc1cc(Cl)cc2c1[nH]c1cncc(NC(=O)C(F)(F)F)c12)c1cccnc1>CO>Nc1cncc2[nH]c3c(NC(=O)c4cccnc4)cc(Cl)cc3c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-1a045f84366a4f88ac017f6c5af9c4fc
CC(C)(C)OC(=O)n1cc(CC#N)c2ccccc21.CI>>CC(C#N)c1cn(C(=O)OC(C)(C)C)c2ccccc12
O.C[Si](C)(C)[N-][Si](C)(C)C.[Na+].C(C)(C)(C)OC(=O)N1C=C(C2=CC=CC=C12)CC#N.IC>>C(C)(C)(C)OC(=O)N1C=C(C2=CC=CC=C12)C(C)C#N
[CH2:2]([C:3]#[N:4])[c:5]1[cH:6][n:7]([C:8](=[O:9])[O:10][C:11]([CH3:12])([CH3:13])[CH3:14])[c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]12.I[CH3:1]>>[CH3:1][CH:2]([C:3]#[N:4])[c:5]1[cH:6][n:7]([C:8](=[O:9])[O:10][C:11]([CH3:12])([CH3:13])[CH3:14])[c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]12
CC(C)(C)OC(=O)n1cc(CC#N)c2ccccc21.CI
CC(C#N)c1cn(C(=O)OC(C)(C)C)c2ccccc12
null
null
C1CCOC1.CCOC(=O)C
C-C Coupling
Methylation with MeI_secondary
0e09d968095a587418cca2841b1e4f096e8103de8fbb60e833faf1fb3df36a41
410ec9b1cc243569e4ff568c248f0b402403802e002b4018f576af3f6960507b
c1ccc2[nH]ccc2c1
I-[CH3;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[#7;a:5]1:[c:6]:[c:7]:[c:8](-[CH2;D2;+0:9]-[C:10]#[N;D1;H0:11]):[c:12]:1>>[#8:2]-[C:3](=[O;D1;H0:4])-[#7;a:5]1:[c:6]:[c:7]:[c:8](-[CH;D3;+0:9](-[CH3;D1;+0:1])-[C:10]#[N;D1;H0:11]):[c:12]:1
79.4
[{"value": 79.4, "product": "C(C)(C)(C)OC(=O)N1C=C(C2=CC=CC=C12)C(C)C#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
A stirred solution of 3-cyanomethyl-indole-1-carboxylic acid tert-butyl ester (2.15 g, 8.39 mmol) in THF (40 ml) was cooled to −78° C. under an argon atmosphere. Sodium bis(trimethylsilyl)amide (1 M in THF, 10 ml, 10 mmol) was added thereto and the cold solution was stirred for 30 minutes. Iodomethane (627 uL, 10 mmol)...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1c[nH]c2ccccc12
HI
C1CCOC1.CCOC(=O)C
0
0.5
CC(C)(C)OC(=O)n1cc(CC#N)c2ccccc21.CI>C1CCOC1.CCOC(=O)C>CC(C#N)c1cn(C(=O)OC(C)(C)C)c2ccccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-5a8b7785a1c44cd4a637d2c07fb8374d
CC1CNCc2[nH]c3ccccc3c21>>Cc1cncc2[nH]c3ccccc3c12
CC1CNCC=2NC3=CC=CC=C3C12>>CC1=CN=CC=2NC3=CC=CC=C3C12
[CH3:1][CH:2]1[CH2:3][NH:4][CH2:5][c:6]2[nH:7][c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3[c:14]21>>[CH3:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3[c:14]12
CC1CNCc2[nH]c3ccccc3c21
Cc1cncc2[nH]c3ccccc3c12
null
[Pd]
null
Oxidation
OtherReaction
523352700f59a97369e704a2d9a8c0a34702d7e100a14629f0bde803b65f20e2
45f806b8e00071c3429c43b3544e10767c5f82b269d7c53bc7fada9a5eb3b8c6
c1ccc2c(c1)[nH]c1cnccc12
[C;D1;H3:1]-[CH;D3;+0:2]1-[CH2;D2;+0:3]-[NH;D2;+0:4]-[CH2;D2;+0:5]-[c:6]2:[#7;a:7]:[c:8]:[c:9]:[c:10]:2-1>>[C;D1;H3:1]-[c;H0;D3;+0:2]1:[cH;D2;+0:3]:[n;H0;D2;+0:4]:[cH;D2;+0:5]:[c:6]2:[#7;a:7]:[c:8]:[c:9]:[c:10]:2:1
98.5
[{"value": 98.5, "product": "CC1=CN=CC=2NC3=CC=CC=C3C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
160
CELSIUS
24
HOUR
4-methyl-2,3,4,9-tetrahydro-1H-β-carboline (214 mg, 1.17 mmol) was suspended in xylenes (10 ml). Pd (10% wt. on carbon, 21 mg) catalyst was added thereto and the reaction mixture was stirred at 160° C. for 24 hours, then cooled to RT and filtered through celite. The filtrate was concentrated to dryness to give 4-methyl...
10.6084/m9.figshare.5104873.v1
null
Secondary amine
null
c1ccc2c3c(nc2c1)CNCC3
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
null
[Pd]
160
24
CC1CNCc2[nH]c3ccccc3c21>[Pd]>Cc1cncc2[nH]c3ccccc3c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-6c4fa2e590f5443b9ababf7aea0a81bf
Cc1cncc2[nH]c3ccccc3c12.O=C1CCC(=O)N1Cl>>Cc1cncc2[nH]c3ccc(Cl)cc3c12
CC1=CN=CC=2NC3=CC=CC=C3C12.C1CC(=O)N(C1=O)Cl.C([O-])(O)=O.[Na+]>>ClC=1C=C2C=3C(=CN=CC3NC2=CC1)C
[CH3:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[cH:9][cH:10][cH:11][cH:13][c:14]3[c:15]12.O=C1CCC(=O)N1[Cl:12]>>[CH3:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]3[c:15]12
Cc1cncc2[nH]c3ccccc3c12.O=C1CCC(=O)N1Cl
Cc1cncc2[nH]c3ccc(Cl)cc3c12
null
null
Cl
Functional Group Interconversion
Chlorination
0c7815949c87db4c10c2c62b5e92cc3444285641e2a838b0bc2e29f461599b8f
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1ccc2c(c1)[nH]c1cnccc12
O=C1-C-C-C(=O)-N-1-[Cl;H0;D1;+0:1].[#7;a:2]:[c:3]1:[c:4]:[c:5]:[cH;D2;+0:6]:[c:7]:[c:8]:1>>[#7;a:2]:[c:3]1:[c:4]:[c:5]:[c;H0;D3;+0:6](-[Cl;H0;D1;+0:1]):[c:7]:[c:8]:1
93.7
[{"value": 93.7, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
4-methyl-9H-β-carboline (97 mg, 0.532 mmol) was dissolved in HCl (1N, 4 ml) and stirred at RT. NCS (85 mg, 0.637 mmol) was added thereto and the reaction mixture was stirred for 5 hr. Saturated sodium bicarbonate solution (20 ml) was added thereto and the reaction mixture was extracted twice with EtOAc (100 ml). The co...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1ccc2c(c1)[nH]c1cnccc12.C1CCNC1
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
HO-
Cl
null
null
Cc1cncc2[nH]c3ccccc3c12.O=C1CCC(=O)N1Cl>Cl>Cc1cncc2[nH]c3ccc(Cl)cc3c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-9040f27fcadd491cafbf69bcb116f9b7
Cc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12>>Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12
ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)[N+](=O)[O-])C>>ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)N)C
O=[N+:10]([O-])[c:9]1[c:8]2[nH:7][c:6]3[cH:5][n:4][cH:3][c:2]([CH3:1])[c:16]3[c:15]2[cH:14][c:12]([Cl:13])[cH:11]1>>[CH3:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[c:9]([NH2:10])[cH:11][c:12]([Cl:13])[cH:14][c:15]3[c:16]12
Cc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12
Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12
null
[Pt]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)[nH]c1cnccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
93.3
[{"value": 93.3, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)N)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
A solution of 6-chloro-4-methyl-8-nitro-9H-β-carboline (80 mg, 0.31 mmol) in MeOH (10 ml) was stirred at RT. Platinum (10% wt. on carbon, 24 mg) catalyst was added thereto and the reaction vessel was capped and vacuum purged 3 times with argon, followed similarly by hydrogen. The reaction mixture was stirred 1.5 hr und...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)[nH]c1cnccc12
Other
[Pt].CO
null
1.5
Cc1cncc2[nH]c3c([N+](=O)[O-])cc(Cl)cc3c12>[Pt].CO>Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-6ae8c9d0d8654400b65d536d16c21f9b
Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12.O=C(Cl)c1cccnc1>>Cc1cncc2[nH]c3c(NC(=O)c4cccnc4)cc(Cl)cc3c12
CCOC(=O)C.ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)N)C.Cl.C(C1=CN=CC=C1)(=O)Cl>>ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=CN=CC=C1)=O)C
[CH3:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[c:9]([NH2:10])[cH:19][c:20]([Cl:21])[cH:22][c:23]3[c:24]12.Cl[C:11](=[O:12])[c:13]1[cH:14][cH:15][cH:16][n:17][cH:18]1>>[CH3:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[c:9]([NH:10][C:11](=[O:12])[c:13]4[cH:14][cH:15][cH:16][n:17][cH:18]4)[cH:19][c:20]([Cl:21])[cH:22][c:...
Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12.O=C(Cl)c1cccnc1
Cc1cncc2[nH]c3c(NC(=O)c4cccnc4)cc(Cl)cc3c12
null
null
O.N1=CC=CC=C1
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7].[#7;a:8]:[c:9]:[c:10]:[#7;a:11]:[c:12](:[c:13]):[c:14](-[NH2;D1;+0:15]):[c:16]>>[#7;a:8]:[c:9]:[c:10]:[#7;a:11]:[c:12](:[c:13]):[c:14](-[NH;D2;+0:15]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]):[c:16]
8.1
[{"value": 8.1, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)NC(C1=CN=CC=C1)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
A solution of 6-chloro-4-methyl-9H-β-carbolin-8-ylamine (43 mg, 0.19 mmol) in pyridine (4 ml) was stirred at RT under an argon atmosphere. Nicotinoyl chloride hydrochloride (40 mg, 0.22 mmol) was added thereto and the reaction mixture was stirred for 12 hr. The solution was diluted with H2O (5 ml) and poured into a sep...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccncc1.c1ccc2c(c1)[nH]c1cnccc12
HCl
O.N1=CC=CC=C1
null
12
Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12.O=C(Cl)c1cccnc1>O.N1=CC=CC=C1>Cc1cncc2[nH]c3c(NC(=O)c4cccnc4)cc(Cl)cc3c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a27e6a4f7bd746fdaef7e84f334dece2
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CC(C)(C)OC(=O)N1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)N.C(C)(C)(C)OC(=O)N1C(COC(C1)(C)C)C(=O)O>>C(C)(C)(C)OC(=O)N1CC(OC[C@H]1C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O)(C)C
O[C:16]([CH:15]1[N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:9][C:10]([CH3:11])([CH3:12])[O:13][CH2:14]1)=[O:17].[NH2:18][c:19]1[cH:20][c:21]([Cl:22])[cH:23][c:24]2[c:25]1[nH:26][c:27]1[cH:28][n:29][cH:30][cH:31][c:32]21>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][C:10]([CH3:11])([CH3:...
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12
CC(C)(C)OC(=O)N1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH;D3;+0:3]1-[C:4]-[#8:5]-[C:6]-[C:7]-[#7:8]-1-[C:9](=[O;D1;H0:10])-[#8:11]-[C:12](-[C;D1;H3:13])(-[C;D1;H3:14])-[C;D1;H3:15].[#7;a:16]:[c:17]:[c:18]:[#7;a:19]:[c:20](:[c:21]):[c:22](-[NH2;D1;+0:23]):[c:24]>>[#7;a:16]:[c:17]:[c:18]:[#7;a:19]:[c:20](:[c:21]):[c:22](-[NH;D2;+0:23]-[C;H0;D3...
87
[{"value": 87.0, "product": "C(C)(C)(C)OC(=O)N1CC(OC[C@H]1C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method C from 6-chloro-9H-β-carboline-8-ylamine and 6,6-dimethyl-morpholine-3,4-dicarboxylic acid 4-tert-butyl ester in 87% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)O.Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CC(C)(C)OC(=O)N1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-4a68d3ab7de74215a577f8527d987335
CC(=O)OC(C)=O.CC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CC(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(C)N.C(C)(=O)OC(C)=O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)C[C@H](C)NC(C)=O
CC(=O)O[C:2]([CH3:1])=[O:3].[NH2:4][CH:5]([CH3:6])[CH2:7][N:8]1[CH2:9][C:10]([CH3:11])([CH3:12])[O:13][CH2:14][CH:15]1[C:16](=[O:17])[NH:18][c:19]1[cH:20][c:21]([Cl:22])[cH:23][c:24]2[c:25]1[nH:26][c:27]1[cH:28][n:29][cH:30][cH:31][c:32]21>>[CH3:1][C:2](=[O:3])[NH:4][C@@H:5]([CH3:6])[CH2:7][N:8]1[CH2:9][C:10]([CH3:11])...
CC(=O)OC(C)=O.CC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
CC(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
null
Acylation
Aminolysis of esters
87d35e51b477fc9a658a6f307eb56d84c8879182772c9dd3a42ec0d584fd2684
627cbc0550c9f51ad0105d9fcf46677e8c93bed87ee95bfe69292a82550c95b7
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#7:4]-[C:5]-[CH;D3;+0:6](-[C;D1;H3:7])-[NH2;D1;+0:8]>>[#7:4]-[C:5]-[C@H;D3;+0:6](-[C;D1;H3:7])-[NH;D2;+0:8]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]
null
[]
null
null
null
null
The desired compound was prepared according to the previous example from 4-(2-Amino-propyl)-6,6-dimethyl-morpholine-3-carboxylic acid (6-chloro-9H-β-carbolin-8yl)-amide (3 CF3COOH salt) and acetic anhydride. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary amine
Secondary amide
null
null
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC(=O)OC(C)=O.CC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CC(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f0e5fa4ede3b47dca9055aebff913347
C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O>>Cc1ncccc1C(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
FC(C(=O)O)(F)F.ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)C[C@H](C)N.CC1=C(C(=O)O)C=CC=N1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)C[C@H](C)NC(=O)C=1C(=NC=CC1)C
[NH2:10][C@@H:11]([CH3:12])[CH2:13][N:14]1[CH2:15][C:16]([CH3:17])([CH3:18])[O:19][CH2:20][C@H:21]1[C:22](=[O:23])[NH:24][c:25]1[cH:26][c:27]([Cl:28])[cH:29][c:30]2[c:31]1[nH:32][c:33]1[cH:34][n:35][cH:36][cH:37][c:38]21.O[C:8]([c:7]1[c:2]([CH3:1])[n:3][cH:4][cH:5][cH:6]1)=[O:9]>>[CH3:1][c:2]1[n:3][cH:4][cH:5][cH:6][c:...
C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O
Cc1ncccc1C(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCCN1CCOC[C@H]1C(=O)Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[C:9]-[C:10](-[C;D1;H3:11])-[NH2;D1;+0:12]>>[C:9]-[C:10](-[C;D1;H3:11])-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]
75
[{"value": 75.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)C[C@H](C)NC(=O)C=1C(=NC=CC1)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method E from (S)-4-((S)-2-Amino-propyl)-6,6-dimethyl-morpholine-3-carboxylic acid (6-chloro-9H-beta-carbolin-8-yl)-amide trifluoroacetate salt and 2-methyl-nicotinic acid in 75% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccncc1.C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O>>Cc1ncccc1C(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-511991e8196149f8bbc6a6fd32b06b34
COC(=O)Cl.C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>>COC(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
O.C(Cl)Cl.Cl.ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)C[C@H](C)N.ClC(=O)OC>>COC(N[C@H](CN1CC(OC[C@H]1C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O)(C)C)C)=O
Cl[C:3]([O:2][CH3:1])=[O:4].[NH2:5][C@@H:6]([CH3:7])[CH2:8][N:9]1[CH2:10][C:11]([CH3:12])([CH3:13])[O:14][CH2:15][C@H:16]1[C:17](=[O:18])[NH:19][c:20]1[cH:21][c:22]([Cl:23])[cH:24][c:25]2[c:26]1[nH:27][c:28]1[cH:29][n:30][cH:31][cH:32][c:33]21>>[CH3:1][O:2][C:3](=[O:4])[NH:5][C@@H:6]([CH3:7])[CH2:8][N:9]1[CH2:10][C:11]...
COC(=O)Cl.C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
COC(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
N1=CC=CC=C1
Protection
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
038720aa61a7efa0f2a9ee6f2e0adf63a9ffdc2be4697c11a6215baef34f97b2
205f353513ce9506ab61831799da8fb73ec2ef5cfa927664496d3ce72c438860
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].[C:5]-[C:6](-[C;D1;H3:7])-[NH2;D1;+0:8]>>[C:5]-[C:6](-[C;D1;H3:7])-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4]
77
[{"value": 77.0, "product": "COC(N[C@H](CN1CC(OC[C@H]1C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O)(C)C)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of (S)-4-((S)-2-Amino-propyl)-6,6-dimethyl-morpholine-3 carboxylic acid (6-chloro-9H-beta-carbolin-8-yl)-amide hydrochloride salt (3.45 g, 6.59 mmole) in 68 ml of dry pyridine, was added in three portions over 1.5 hr, a 3M DCM solution of methyl chloroformate (9.2 ml, 27.6 mmole, 4.2 eq). After 2 h, 10 ml...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine
Carbamic ester
null
null
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HCl
N1=CC=CC=C1
null
2
COC(=O)Cl.C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>N1=CC=CC=C1>COC(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-1b856251211042118c2fe543f99e5df8
C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ccncc1C(=O)O>>Cc1ccncc1C(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
FC(C(=O)O)(F)F.ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)C[C@H](C)N.CC1=CC=NC=C1C(=O)O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)C[C@H](C)NC(=O)C=1C=NC=CC1C
[NH2:10][C@@H:11]([CH3:12])[CH2:13][N:14]1[CH2:15][C:16]([CH3:17])([CH3:18])[O:19][CH2:20][C@H:21]1[C:22](=[O:23])[NH:24][c:25]1[cH:26][c:27]([Cl:28])[cH:29][c:30]2[c:31]1[nH:32][c:33]1[cH:34][n:35][cH:36][cH:37][c:38]21.O[C:8]([c:7]1[c:2]([CH3:1])[cH:3][cH:4][n:5][cH:6]1)=[O:9]>>[CH3:1][c:2]1[cH:3][cH:4][n:5][cH:6][c:...
C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ccncc1C(=O)O
Cc1ccncc1C(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCCN1CCOC[C@H]1C(=O)Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7].[C:8]-[C:9](-[C;D1;H3:10])-[NH2;D1;+0:11]>>[C:8]-[C:9](-[C;D1;H3:10])-[NH;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]
79
[{"value": 79.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)C[C@H](C)NC(=O)C=1C=NC=CC1C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method E from (S)-4-((S)-2-Amino-propyl)-6,6-dimethyl-morpholine-3-carboxylic acid (6-chloro-9H-beta-carbolin-8-yl)-amide trifluoroacetate salt and 4-methyl-nicotinic acid in 79% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccncc1.C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
C[C@H](N)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ccncc1C(=O)O>>Cc1ccncc1C(=O)N[C@@H](C)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-dc48c1aa823841a2aefa898d79268900
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>>CC1(C)CNC(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
C(C)(C)(C)OC(=O)N1CC(OCC1C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O)(C)C.Cl.CCOCC>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1NCC(OC1)(C)C
CC(C)(C)OC(=O)[N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[O:25][CH2:24][CH:6]1[C:7](=[O:8])[NH:9][c:10]1[cH:11][c:12]([Cl:13])[cH:14][c:15]2[c:16]1[nH:17][c:18]1[cH:19][n:20][cH:21][cH:22][c:23]21>>[CH3:1][C:2]1([CH3:3])[CH2:4][NH:5][CH:6]([C:7](=[O:8])[NH:9][c:10]2[cH:11][c:12]([Cl:13])[cH:14][c:15]3[c:16]2[nH:17][c:18]2[cH:...
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
CC1(C)CNC(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
CO.O1CCOCC1
Reduction
Boc amine deprotection
711003132a3fa45641804f0f1112f2c6083a93e7723a03dc1bfa10a86d322b68
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=C(Nc1cccc2c1[nH]c1cnccc12)C1COCCN1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1-[C:7](=[O;D1;H0:8])-[#7:9]-[c:10]:[c:11]:[#7;a:12]>>[#7;a:12]:[c:11]:[c:10]-[#7:9]-[C:7](=[O;D1;H0:8])-[C:6]1-[C:5]-[#8:4]-[C:3]-[C:2]-[NH;D2;+0:1]-1
119.2
[{"value": 99.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1NCC(OC1)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 119.2, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1NCC(OC1)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a clear brown solution of 5-(6-chloro-9H-β-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholine-4-carboxylic acid tert-butyl ester (10.4 g, 22.7 mmol) in methanol (41 mL) was added HCl in dioxane (4M, 91 mL). The reaction was stirred for 30 minutes at room temperature, during which time a pale brown precipitate began to ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1COCC[NH]1
C1COCCN1
C1COCCN1.c1ccc2c(c1)[nH]c1cnccc12
HO-
CO.O1CCOCC1
null
0.5
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12>CO.O1CCOCC1>CC1(C)CNC(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-ff9c6f32cd5a4c24819f000ea55e2c8b
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.CCC(C=O)NC(=O)OC(C)(C)C>>CCC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
C(C)(C)(C)OC(=O)N1CC(OCC1C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O)(C)C.C(C)(C)(C)OC(NC(CC)C=O)=O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(CC)N
CC(C)(C)OC(=O)[N:6]1[CH2:7][C:8]([CH3:9])([CH3:10])[O:11][CH2:12][CH:13]1[C:14](=[O:15])[NH:16][c:17]1[cH:18][c:19]([Cl:20])[cH:21][c:22]2[c:23]1[nH:24][c:25]1[cH:26][n:27][cH:28][cH:29][c:30]21.CC(C)(C)OC(=O)[NH:4][CH:3]([CH2:2][CH3:1])[CH:5]=O>>[CH3:1][CH2:2][CH:3]([NH2:4])[CH2:5][N:6]1[CH2:7][C:8]([CH3:9])([CH3:10])...
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.CCC(C=O)NC(=O)OC(C)(C)C
CCC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
c22af3bcded745a2ef0ab806662eb69a5ce6d90965df4d21f23275b1defe0c0c
60a50d1b1b66a3cdcbad6664ebf06a1f4154a3f50ef2ff881074ba8a50b0b949
O=C(Nc1cccc2c1[nH]c1cnccc12)C1COCCN1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1-[C:7](=[O;D1;H0:8])-[#7:9]-[c:10]:[c:11]:[#7;a:12].C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:13]-[C:14](-[C:15])-[CH;D2;+0:16]=O>>[#7;a:12]:[c:11]:[c:10]-[#7:9]-[C:7](=[O;D1;H0:8])-[C:6]1-[C:5]-[#8:4]-[C:3]-[C:2]-[N;H0;D3;+0:1]-1-[CH2;D2;+0:16]-[C:14](-[C:15])-[N...
null
[]
null
null
null
null
Method C was followed, using 5-(6-chloro-9H-β-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholine-4-carboxylic acid tert-butyl ester and the appropriate aldehyde, (1-formyl-propyl)-carbamic acid tert-butyl ester. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Carbamic ester.Carbamic ester.Ether.Ether.Boc.Boc
Primary amine.Tertiary amine
C1COCC[NH]1
C1COCC[NH]1
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.CCC(C=O)NC(=O)OC(C)(C)C>>CCC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-86d07ec1acad4deaa6bd9c111eed8bdd
CCC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O>>CCC(CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12)NC(=O)c1cccnc1C
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(CC)N.CC1=C(C(=O)O)C=CC=N1.CCN=C=NCCCN(C)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(CC)NC(=O)C=1C(=NC=CC1)C
[CH3:1][CH2:2][CH:3]([CH2:4][N:5]1[CH2:6][C:7]([CH3:8])([CH3:9])[O:10][CH2:11][CH:12]1[C:13](=[O:14])[NH:15][c:16]1[cH:17][c:18]([Cl:19])[cH:20][c:21]2[c:22]1[nH:23][c:24]1[cH:25][n:26][cH:27][cH:28][c:29]21)[NH2:30].O[C:31](=[O:32])[c:33]1[cH:34][cH:35][cH:36][n:37][c:38]1[CH3:39]>>[CH3:1][CH2:2][CH:3]([CH2:4][N:5]1[C...
CCC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O
CCC(CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12)NC(=O)c1cccnc1C
null
null
O.N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCCN1CCOCC1C(=O)Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[C:9]-[C:10](-[C:11])-[NH2;D1;+0:12]>>[C:9]-[C:10](-[C:11])-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]
80.5
[{"value": 71.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(CC)NC(=O)C=1C(=NC=CC1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.5, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(CC)NC(=O)C=1C(=NC=CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": fal...
null
null
8
HOUR
To a solution of 4-(2-amino-butyl)-6,6-dimethyl-morpholine-3-carboxylic acid (6-chloro-9H-β-carbolin-8-yl)-amide (100 mg, 0.233 mmol) in pyridine (4 mL) was added 2-methyl-nicotinic acid (38.4 mg, 0.280 mmol) and EDCI (71.5 mg, 0.373 mmol). The solution was stirred overnight at room temperature, then diluted with water...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12.c1ccncc1
HO-
O.N1=CC=CC=C1
null
8
CCC(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O>O.N1=CC=CC=C1>CCC(CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12)NC(=O)c1cccnc1C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2cf74021c1fb4b08a135f3920f25b9d6
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.CC(C)C(C=O)NC(=O)OC(C)(C)C>>CC(C)C(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
C(C)(C)(C)OC(=O)N1CC(OCC1C(NC=1C=C(C=C2C=3C=CN=CC3NC12)Cl)=O)(C)C.C(C)(C)(C)OC(NC(C(C)C)C=O)=O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(C(C)C)N
CC(C)(C)OC(=O)[N:7]1[CH2:8][C:9]([CH3:10])([CH3:11])[O:12][CH2:13][CH:14]1[C:15](=[O:16])[NH:17][c:18]1[cH:19][c:20]([Cl:21])[cH:22][c:23]2[c:24]1[nH:25][c:26]1[cH:27][n:28][cH:29][cH:30][c:31]21.CC(C)(C)OC(=O)[NH:5][CH:4]([CH:2]([CH3:1])[CH3:3])[CH:6]=O>>[CH3:1][CH:2]([CH3:3])[CH:4]([NH2:5])[CH2:6][N:7]1[CH2:8][C:9]([...
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.CC(C)C(C=O)NC(=O)OC(C)(C)C
CC(C)C(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
c22af3bcded745a2ef0ab806662eb69a5ce6d90965df4d21f23275b1defe0c0c
60a50d1b1b66a3cdcbad6664ebf06a1f4154a3f50ef2ff881074ba8a50b0b949
O=C(Nc1cccc2c1[nH]c1cnccc12)C1COCCN1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1-[C:7](=[O;D1;H0:8])-[#7:9]-[c:10]:[c:11]:[#7;a:12].C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:13]-[C:14](-[C:15])-[CH;D2;+0:16]=O>>[#7;a:12]:[c:11]:[c:10]-[#7:9]-[C:7](=[O;D1;H0:8])-[C:6]1-[C:5]-[#8:4]-[C:3]-[C:2]-[N;H0;D3;+0:1]-1-[CH2;D2;+0:16]-[C:14](-[C:15])-[N...
null
[]
null
null
null
null
Method C was followed, using 5-(6-chloro-9H-β-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholine-4-carboxylic acid tert-butyl ester and the appropriate aldehyde, (1-formyl-2-methyl-propyl)-carbamic acid tert-butyl ester. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Carbamic ester.Carbamic ester.Ether.Ether.Boc.Boc
Primary amine.Tertiary amine
C1COCC[NH]1
C1COCC[NH]1
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC(C)(C)OC(=O)N1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.CC(C)C(C=O)NC(=O)OC(C)(C)C>>CC(C)C(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-8c05c8b7442241ab9e8f8efb8e990e3f
CC(C)C(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O>>Cc1ncccc1C(=O)NC(CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12)C(C)C
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(C(C)C)N.CC1=C(C(=O)O)C=CC=N1.CCN=C=NCCCN(C)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(C(C)C)NC(=O)C=1C(=NC=CC1)C
[NH2:10][CH:11]([CH2:12][N:13]1[CH2:14][C:15]([CH3:16])([CH3:17])[O:18][CH2:19][CH:20]1[C:21](=[O:22])[NH:23][c:24]1[cH:25][c:26]([Cl:27])[cH:28][c:29]2[c:30]1[nH:31][c:32]1[cH:33][n:34][cH:35][cH:36][c:37]21)[CH:38]([CH3:39])[CH3:40].O[C:8]([c:7]1[c:2]([CH3:1])[n:3][cH:4][cH:5][cH:6]1)=[O:9]>>[CH3:1][c:2]1[n:3][cH:4][...
CC(C)C(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O
Cc1ncccc1C(=O)NC(CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12)C(C)C
null
null
CCOC(=O)C.O.N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCCN1CCOCC1C(=O)Nc1cccc2c1[nH]c1cnccc12)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8].[C:9]-[C:10](-[C:11])-[NH2;D1;+0:12]>>[C:9]-[C:10](-[C:11])-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]
77
[{"value": 77.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(C(C)C)NC(=O)C=1C(=NC=CC1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.7, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(C(C)C)NC(=O)C=1C(=NC=CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired...
null
null
6.5
HOUR
To a solution of 4-(2-amino-3-methyl-butyl)-6,6-dimethyl-morpholine-3-carboxylic acid (6-chloro-9H-β-carbolin-8-yl)-amide (1.47 g, 3.31 mmol) in pyridine (35 mL) was added 2-methyl-nicotinic acid (544 mg, 3.97 mmol) and EDCI (1.02 g, 5.30 mmol). The solution was stirred 6.5 hours at room temperature, then diluted with ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccncc1.C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
CCOC(=O)C.O.N1=CC=CC=C1
null
6.5
CC(C)C(N)CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12.Cc1ncccc1C(=O)O>CCOC(=O)C.O.N1=CC=CC=C1>Cc1ncccc1C(=O)NC(CN1CC(C)(C)OCC1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12)C(C)C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-de19231c6bd74670afea944e8f43a29e
C[C@@H](CN1CC(C)(C)OC[C@H]1C(=O)O)NC(=O)OC(C)(C)C.Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12>>Cc1cncc2[nH]c3c(NC(=O)[C@@H]4COC(C)(C)CN4C[C@H](C)NC(=O)OC(C)(C)C)cc(Cl)cc3c12
CCN=C=NCCCN(C)C.C(C)(C)(C)OC(=O)N[C@H](CN1[C@@H](COC(C1)(C)C)C(=O)O)C.CC1(OC[C@H](NC1)C(=O)O)C.ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)N)C>>C(C)(C)(C)OC(N[C@H](CN1CC(OC[C@H]1C(NC=1C=C(C=C2C=3C(=CN=CC3NC12)C)Cl)=O)(C)C)C)=O
O[C:11](=[O:12])[C@@H:13]1[CH2:14][O:15][C:16]([CH3:17])([CH3:18])[CH2:19][N:20]1[CH2:21][C@H:22]([CH3:23])[NH:24][C:25](=[O:26])[O:27][C:28]([CH3:29])([CH3:30])[CH3:31].[CH3:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7][c:8]3[c:9]([NH2:10])[cH:32][c:33]([Cl:34])[cH:35][c:36]3[c:37]12>>[CH3:1][c:2]1[cH:3][n:4][cH:5][c:6]2[nH:7...
C[C@@H](CN1CC(C)(C)OC[C@H]1C(=O)O)NC(=O)OC(C)(C)C.Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12
Cc1cncc2[nH]c3c(NC(=O)[C@@H]4COC(C)(C)CN4C[C@H](C)NC(=O)OC(C)(C)C)cc(Cl)cc3c12
null
null
CO.C(Cl)Cl.N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4]-[#8:5])-[#7:6](-[C:7])-[C:8].[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:[c:13](:[c:14]):[c:15](-[NH;D2;+0:16]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4]-[#8:5])-[#7:6](-[C:7])-[C:8]):[c:17]
62.7
[{"value": 62.7, "product": "C(C)(C)(C)OC(N[C@H](CN1CC(OC[C@H]1C(NC=1C=C(C=C2C=3C(=CN=CC3NC12)C)Cl)=O)(C)C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of (S)-4-((S)-2-tert-butoxycarbonylamino-propyl)-6,6-dimethyl-morpholine-3-carboxylic acid (3.316 g, 10.5 mmol) (prepared by reductively alkylating (S)-6,6-dimethyl-morpholine-3-carboxylic acid with N-(tert-butoxycarbonyl)-L-alanal) in anhydrous pyridine (75 mL) was stirred at room temperature. 6-chloro-4-me...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
CO.C(Cl)Cl.N1=CC=CC=C1
null
null
C[C@@H](CN1CC(C)(C)OC[C@H]1C(=O)O)NC(=O)OC(C)(C)C.Cc1cncc2[nH]c3c(N)cc(Cl)cc3c12>CO.C(Cl)Cl.N1=CC=CC=C1>Cc1cncc2[nH]c3c(NC(=O)[C@@H]4COC(C)(C)CN4C[C@H](C)NC(=O)OC(C)(C)C)cc(Cl)cc3c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-89abf249a0f54f24b8c894f543473385
CCC[CH2][Sn]([Cl])([CH2]CCC)[CH2]CCC.Fc1cncc(F)c1>>CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1c(F)cncc1F
C(CCC)[Sn](CCCC)(CCCC)Cl.C(CCC)[Li].C(C)(C)NC(C)C.FC=1C=NC=C(C1)F>>FC=1C=NC=C(C1[Sn](CCCC)(CCCC)CCCC)F
[Cl][Sn:5]([CH2:4][CH2:3][CH2:2][CH3:1])([CH2:6][CH2:7][CH2:8][CH3:9])[CH2:10][CH2:11][CH2:12][CH3:13].[cH:14]1[c:15]([F:16])[cH:17][n:18][cH:19][c:20]1[F:21]>>[CH3:1][CH2:2][CH2:3][CH2:4][Sn:5]([CH2:6][CH2:7][CH2:8][CH3:9])([CH2:10][CH2:11][CH2:12][CH3:13])[c:14]1[c:15]([F:16])[cH:17][n:18][cH:19][c:20]1[F:21]
CCC[CH2][Sn]([Cl])([CH2]CCC)[CH2]CCC.Fc1cncc(F)c1
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1c(F)cncc1F
null
null
C1CCOC1.O
Functional Group Interconversion
OtherReaction
157ed86a47fdc4e2a8a8cbaf40c9e8c836526372fc356d6404550bda901a11a9
8ed099106fd03cd2d2d78800a2ee5fc34a9ebd85fa643ab7cdafec1855cc2f69
c1ccncc1
[C:1]-[C:2]-[Sn;H0;D4;+0:3](-[Cl])(-[C:4]-[C:5])-[C:6]-[C:7].[F;D1;H0:8]-[c:9]1:[c:10]:[#7;a:11]:[c:12]:[c:13](-[F;D1;H0:14]):[cH;D2;+0:15]:1>>[C:1]-[C:2]-[Sn;H0;D4;+0:3](-[C:4]-[C:5])(-[C:6]-[C:7])-[c;H0;D3;+0:15]1:[c:9](-[F;D1;H0:8]):[c:10]:[#7;a:11]:[c:12]:[c:13]:1-[F;D1;H0:14]
89.5
[{"value": 88.0, "product": "FC=1C=NC=C(C1[Sn](CCCC)(CCCC)CCCC)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.5, "product": "FC=1C=NC=C(C1[Sn](CCCC)(CCCC)CCCC)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
30
MINUTE
n-Butyl lithium (1.0 eq, 76 mmol, 47.6 mL, 1.6 M in hexanes) was added via dropping funnel to a solution of diisopropylamine (1.05 eq, 80 mmol, 11.2 mL) in THF (300 mL) at −78° C. under nitrogen (N2). The solution was stirred for 30 min at −78° C., then a solution of 3,5-difluoropyridine (1.05 eq, 80 mmol, 9.2 g) in TH...
10.6084/m9.figshare.5104873.v1
null
Tin
Tin
c1ccncc1
c1ccncc1
c1ccncc1
HCl
C1CCOC1.O
-78
0.5
CCC[CH2][Sn]([Cl])([CH2]CCC)[CH2]CCC.Fc1cncc(F)c1>C1CCOC1.O>CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1c(F)cncc1F
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-981b4dc1e0c84bf89a142b850617dd70
Fc1cncc2[nH]c3ccc(Cl)cc3c12>>O=[N+]([O-])c1cc(Cl)cc2c1[nH]c1cncc(F)c12
C([O-])(O)=O.[Na+].[N+](=O)([O-])[O-].[Na+].ClC=1C=C2C=3C(=CN=CC3NC2=CC1)F.CO>>ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)[N+](=O)[O-])F
[cH:4]1[cH:5][c:6]([Cl:7])[cH:8][c:9]2[c:10]1[nH:11][c:12]1[cH:13][n:14][cH:15][c:16]([F:17])[c:18]21>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][c:6]([Cl:7])[cH:8][c:9]2[c:10]1[nH:11][c:12]1[cH:13][n:14][cH:15][c:16]([F:17])[c:18]21
Fc1cncc2[nH]c3ccc(Cl)cc3c12
O=[N+]([O-])c1cc(Cl)cc2c1[nH]c1cncc(F)c12
null
null
FC(C(=O)O)(F)F
Functional Group Addition
OtherReaction
3933ccedcb89087e8369e8b96a6fdb15b3900ebc2ce7ca0a1f7fac4c3c421e4c
22f3183026a2d99c91ec0c53f0059a15c8421016bd62c8ab45281362b96dc686
c1ccc2c(c1)[nH]c1cnccc12
[#7;a:1]:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[cH;D2;+0:7]:[c:8]:[c:9]>>[#7;a:1]:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c;H0;D3;+0:7](-[#7;+:10](-[O;-;D1;H0:11])=[O;D1;H0:12]):[c:8]:[c:9]
102.2
[{"value": 102.2, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)[N+](=O)[O-])F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
15
MINUTE
Sodium nitrate (1.5 eq, 53 mmol, 4.5 g) was added portionwise to a solution of Intermediate 65 (1.0 eq, 35 mmol, 7.8 g) in trifluoroacetic acid (200 mL) and the resulting mixture heated at 70° C. for 3 h. After cooling to RT the trifluoroacetic acid was removed on a rotary evaporator to afford a crude solid which was s...
10.6084/m9.figshare.5104873.v1
null
null
Nitro group
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
c1ccc2c(c1)[nH]c1cnccc12
Other
FC(C(=O)O)(F)F
70
0.25
Fc1cncc2[nH]c3ccc(Cl)cc3c12>FC(C(=O)O)(F)F>O=[N+]([O-])c1cc(Cl)cc2c1[nH]c1cncc(F)c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-534f3688ab12471ab15900e5214ec6b6
O=[N+]([O-])c1cc(Cl)cc2c1[nH]c1cncc(F)c12>>Nc1cc(Cl)cc2c1[nH]c1cncc(F)c12
ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)[N+](=O)[O-])F.C(=O)[O-].[NH4+].C([O-])(O)=O.[Na+].[Cl-].[Na+]>>ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)N)F
O=[N+:1]([O-])[c:2]1[cH:3][c:4]([Cl:5])[cH:6][c:7]2[c:8]1[nH:9][c:10]1[cH:11][n:12][cH:13][c:14]([F:15])[c:16]21>>[NH2:1][c:2]1[cH:3][c:4]([Cl:5])[cH:6][c:7]2[c:8]1[nH:9][c:10]1[cH:11][n:12][cH:13][c:14]([F:15])[c:16]21
O=[N+]([O-])c1cc(Cl)cc2c1[nH]c1cncc(F)c12
Nc1cc(Cl)cc2c1[nH]c1cncc(F)c12
null
null
CO.C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)[nH]c1cnccc12
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]:[c:7]:[#7;a:6]:[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3]
70.3
[{"value": 70.0, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)N)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 70.3, "product": "ClC=1C=C2C=3C(=CN=CC3NC2=C(C1)N)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
75
CELSIUS
15
MINUTE
Sulfated platinum (˜0.1 eq, 1 g) was added to a suspension of 6-chloro-4-fluoro-8-nitro-9H-β-carboline (1.0 eq, 35 mmol, 9.3 g) and ammonium formate (3.0 eq, 105 mmol, 6.6 g) in ethanol (175 mL) and the resulting mixture heated at 75° C. for 4 h. After cooling to RT the mixture was filtered through a short plug of Celi...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)[nH]c1cnccc12
Other
CO.C(C)O
75
0.25
O=[N+]([O-])c1cc(Cl)cc2c1[nH]c1cncc(F)c12>CO.C(C)O>Nc1cc(Cl)cc2c1[nH]c1cncc(F)c12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-5063a34e8e444b9699047499e466ff58
CC1(C)CN[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.O=CC(=O)O>>CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1NCC(OC1)(C)C.C(C)N(CC)CC.C(#N)[BH3-].[Na+].C(C=O)(=O)O>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C
[CH3:1][C:2]1([CH3:3])[CH2:4][NH:5][C@H:10]([C:11](=[O:12])[NH:13][c:14]2[cH:15][c:16]([Cl:17])[cH:18][c:19]3[c:20]2[nH:21][c:22]2[cH:23][n:24][cH:25][cH:26][c:27]32)[CH2:28][O:29]1.O=[CH:6][C:7](=[O:8])[OH:9]>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][C:7](=[O:8])[OH:9])[C@H:10]([C:11](=[O:12])[NH:13][c:14]2[cH:15][c...
CC1(C)CN[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.O=CC(=O)O
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
CO.O
Heteroatom Alkylation and Arylation
reductive amination
073d98e7dcd77aafeef71a76da7e61b2751c934600f6fff04db700a08f3e4453
2d03f38884b1fbb0c0d6e6f2de31afb25102fec87f347c3a123e064c1bfef0ad
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1
O=[CH;D2;+0:1]-[C:2](=[O;D1;H0:3])-[O;D1;H1:4].[#7;a:5]:[c:6]:[c:7]-[#7:8]-[C:9](=[O;D1;H0:10])-[C:11]1-[C:12]-[#8:13]-[C:14]-[C:15]-[NH;D2;+0:16]-1>>[#7;a:5]:[c:6]:[c:7]-[#7:8]-[C:9](=[O;D1;H0:10])-[C:11]1-[C:12]-[#8:13]-[C:14]-[C:15]-[N;H0;D3;+0:16]-1-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[O;D1;H1:4]
72
[{"value": 71.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
To a suspension of (S)-6,6-Dimethyl-morpholine-3-carboxylic acid (6-chloro-9H-beta-carbolin-8-yl)-amide (2.6 g, 6.0 mmoles) in 60 ml of methanol was added 1.7 ml of triethylamine (2.0 eq.), sodium cyanoborohydride (575 mg, 9.1 mmoles) and glyoxylic acid (780 mg, 8.5 mmoles). The reaction mixture was stirred at ambient ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary amine
Tertiary amine
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
Other
CO.O
null
1.5
CC1(C)CN[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.O=CC(=O)O>CO.O>CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-1192430b6c8e43849ca85c195b6c749f
C1CCNC1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1>>CC1(C)CN(CC(=O)N2CCCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C.N1CCCC1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(N1CCCC1)=O
[NH:9]1[CH2:10][CH2:11][CH2:12][CH2:13]1.O[C:7]([CH2:6][N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[O:33][CH2:32][C@H:14]1[C:15](=[O:16])[NH:17][c:18]1[cH:19][c:20]([Cl:21])[cH:22][c:23]2[c:24]1[nH:25][c:26]1[cH:27][n:28][cH:29][cH:30][c:31]21)=[O:8]>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][C:7](=[O:8])[N:9]2[CH2:10][CH2:11...
C1CCNC1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
CC1(C)CN(CC(=O)N2CCCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
a590d96426a2fbaed42913d9daf8a16471a16de4978200f1d35a30a10009ebe7
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1CC(=O)N1CCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[C:5]1-[C:6]-[C:7]-[C:8]-[NH;D2;+0:9]-1>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:9]1-[C:5]-[C:6]-[C:7]-[C:8]-1
82
[{"value": 82.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(N1CCCC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method F from [(S)-5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid and pyrrolidine in 82% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNC1
C1CC[NH]C1
C1COCC[NH]1.C1CC[NH]C1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
C1CCNC1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1>>CC1(C)CN(CC(=O)N2CCCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-86725e0e521e4e15b28a05337dd003f8
C1CCNCC1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1>>CC1(C)CN(CC(=O)N2CCCCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C.N1CCCCC1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(N1CCCCC1)=O
[NH:9]1[CH2:10][CH2:11][CH2:12][CH2:13][CH2:14]1.O[C:7]([CH2:6][N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[O:34][CH2:33][C@H:15]1[C:16](=[O:17])[NH:18][c:19]1[cH:20][c:21]([Cl:22])[cH:23][c:24]2[c:25]1[nH:26][c:27]1[cH:28][n:29][cH:30][cH:31][c:32]21)=[O:8]>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][C:7](=[O:8])[N:9]2[CH2:10...
C1CCNCC1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
CC1(C)CN(CC(=O)N2CCCCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1CC(=O)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[C:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:7](-[C:6]-[C:5])-[C:8]-[C:9]
90
[{"value": 90.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(N1CCCCC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method F from [(S)-5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid and piperidine in 90% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1COCC[NH]1.C1CC[NH]CC1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
C1CCNCC1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1>>CC1(C)CN(CC(=O)N2CCCCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-bfedcd2a84d44b00a677751687926cb9
C1COCCN1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1>>CC1(C)CN(CC(=O)N2CCOCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C.N1CCOCC1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(=O)N1CCOCC1
[NH:9]1[CH2:10][CH2:11][O:12][CH2:13][CH2:14]1.O[C:7]([CH2:6][N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[O:34][CH2:33][C@H:15]1[C:16](=[O:17])[NH:18][c:19]1[cH:20][c:21]([Cl:22])[cH:23][c:24]2[c:25]1[nH:26][c:27]1[cH:28][n:29][cH:30][cH:31][c:32]21)=[O:8]>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][C:7](=[O:8])[N:9]2[CH2:10][...
C1COCCN1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
CC1(C)CN(CC(=O)N2CCOCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
2ef483949e7ba3e5f888cf14cdce25fa611f75be09fdf1854a473be519821b59
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1CC(=O)N1CCOCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[#8:5]1-[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]-1>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:8]1-[C:7]-[C:6]-[#8:5]-[C:10]-[C:9]-1
86
[{"value": 86.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(=O)N1CCOCC1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method F from [(S)-5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid and morpholine in 86% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1.C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
C1COCCN1.CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1>>CC1(C)CN(CC(=O)N2CCOCC2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-fdc31d4a04884c65be3b0a14626b16d8
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CNCCO>>CN(CCO)C(=O)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C.CNCCO>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(N(C)CCO)=O
O[C:6](=[O:7])[CH2:8][N:9]1[CH2:10][C:11]([CH3:12])([CH3:13])[O:14][CH2:15][C@H:16]1[C:17](=[O:18])[NH:19][c:20]1[cH:21][c:22]([Cl:23])[cH:24][c:25]2[c:26]1[nH:27][c:28]1[cH:29][n:30][cH:31][cH:32][c:33]21.[CH3:1][NH:2][CH2:3][CH2:4][OH:5]>>[CH3:1][N:2]([CH2:3][CH2:4][OH:5])[C:6](=[O:7])[CH2:8][N:9]1[CH2:10][C:11]([CH3...
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CNCCO
CN(CCO)C(=O)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
ac72df6259d5d7baee7abdbd4706ef4b4627f86ead9dc94f0cefcfcb37c21def
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(Nc1cccc2c1[nH]c1cnccc12)[C@@H]1COCCN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[C:5]-[C:6]-[NH;D2;+0:7]-[C;D1;H3:8]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:7](-[C;D1;H3:8])-[C:6]-[C:5]
55
[{"value": 55.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(N(C)CCO)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method F from [(S)-5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid and 2-methylamino-ethanol in 55% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
null
null
C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CNCCO>>CN(CCO)C(=O)CN1CC(C)(C)OC[C@H]1C(=O)Nc1cc(Cl)cc2c1[nH]c1cnccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-44c3725d926f4530a664ee1f3c677576
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.Nc1cccnc1>>CC1(C)CN(CC(=O)Nc2cccnc2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C.NC=1C=NC=CC1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(NC=1C=NC=CC1)=O
O[C:7]([CH2:6][N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[O:35][CH2:34][C@H:16]1[C:17](=[O:18])[NH:19][c:20]1[cH:21][c:22]([Cl:23])[cH:24][c:25]2[c:26]1[nH:27][c:28]1[cH:29][n:30][cH:31][cH:32][c:33]21)=[O:8].[NH2:9][c:10]1[cH:11][cH:12][cH:13][n:14][cH:15]1>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][C:7](=[O:8])[NH:9][c:10]...
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.Nc1cccnc1
CC1(C)CN(CC(=O)Nc2cccnc2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(CN1CCOC[C@H]1C(=O)Nc1cccc2c1[nH]c1cnccc12)Nc1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8]:[#7;a:9]:[c:10]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]:[#7;a:9]:[c:10]
55
[{"value": 55.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(NC=1C=NC=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method F from [(S)-5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid and 3-aminopyridine. The product was isolated as hydrochloride salt in 55% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1COCC[NH]1.c1ccncc1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.Nc1cccnc1>>CC1(C)CN(CC(=O)Nc2cccnc2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-5ff6e38a931646ee87264518ffe95579
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.NCc1ccncc1>>CC1(C)CN(CC(=O)NCc2ccncc2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@@H]1COC(CN1CC(=O)O)(C)C.NCC1=CC=NC=C1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(NCC1=CC=NC=C1)=O
O[C:7]([CH2:6][N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[O:36][CH2:35][C@H:17]1[C:18](=[O:19])[NH:20][c:21]1[cH:22][c:23]([Cl:24])[cH:25][c:26]2[c:27]1[nH:28][c:29]1[cH:30][n:31][cH:32][cH:33][c:34]21)=[O:8].[NH2:9][CH2:10][c:11]1[cH:12][cH:13][n:14][cH:15][cH:16]1>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][C:7](=[O:8])[NH:...
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.NCc1ccncc1
CC1(C)CN(CC(=O)NCc2ccncc2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(CN1CCOC[C@H]1C(=O)Nc1cccc2c1[nH]c1cnccc12)NCc1ccncc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[NH2;D1;+0:5]-[C:6]-[c:7]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:5]-[C:6]-[c:7]
53
[{"value": 53.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)[C@H]1N(CC(OC1)(C)C)CC(NCC1=CC=NC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared according to Method F from [(S)-5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid and 4-(aminomethyl)pyridine. The product was isolated as hydrochloride salt in 53% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1COCC[NH]1.c1ccncc1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC1(C)CN(CC(=O)O)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.NCc1ccncc1>>CC1(C)CN(CC(=O)NCc2ccncc2)[C@H](C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-33dc103cec324a1ca3caf890d6d35bbd
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.OCC1CCNCC1>>CC1(C)CN(CC(=O)N2CCC(CO)CC2)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
O.ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1COC(CN1CC(=O)O)(C)C.N1CCC(CC1)CO.C(CCl)Cl>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(=O)N1CCC(CC1)CO
O[C:7]([CH2:6][N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[O:36][CH2:35][CH:17]1[C:18](=[O:19])[NH:20][c:21]1[cH:22][c:23]([Cl:24])[cH:25][c:26]2[c:27]1[nH:28][c:29]1[cH:30][n:31][cH:32][cH:33][c:34]21)=[O:8].[NH:9]1[CH2:10][CH2:11][CH:12]([CH2:13][OH:14])[CH2:15][CH2:16]1>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][C:7](=[O:8...
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.OCC1CCNCC1
CC1(C)CN(CC(=O)N2CCC(CO)CC2)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
N1=CC=CC=C1
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(Nc1cccc2c1[nH]c1cnccc12)C1COCCN1CC(=O)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[C:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:7](-[C:6]-[C:5])-[C:8]-[C:9]
62
[{"value": 62.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(=O)N1CCC(CC1)CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 61.6, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(=O)N1CCC(CC1)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
10
MINUTE
[5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid (200 mg, 0.48 mmol) and piperidin-4-yl-methanol (111 mg, 0.96 mmol) were dissolved in pyridine (4 mL). The resulting yellow solution was stirred at room temperature for 10 min and then EDC (184 mg, 0.96 mmol) was added in a single por...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
C1COCC[NH]1.C1CC[NH]CC1.c1ccc2c(c1)[nH]c1cnccc12
HO-
N1=CC=CC=C1
null
0.166667
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.OCC1CCNCC1>N1=CC=CC=C1>CC1(C)CN(CC(=O)N2CCC(CO)CC2)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f451cb243ac244ca9c1117bdd2491195
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CN1CCNCC1>>CN1CCN(C(=O)CN2CC(C)(C)OCC2C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CC1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1COC(CN1CC(=O)O)(C)C.CN1CCNCC1>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(=O)N1CCN(CC1)C
O[C:6](=[O:7])[CH2:8][N:9]1[CH2:10][C:11]([CH3:12])([CH3:13])[O:14][CH2:15][CH:16]1[C:17](=[O:18])[NH:19][c:20]1[cH:21][c:22]([Cl:23])[cH:24][c:25]2[c:26]1[nH:27][c:28]1[cH:29][n:30][cH:31][cH:32][c:33]21.[CH3:1][N:2]1[CH2:3][CH2:4][NH:5][CH2:34][CH2:35]1>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([C:6](=[O:7])[CH2:8][N:9]2[CH2...
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CN1CCNCC1
CN1CCN(C(=O)CN2CC(C)(C)OCC2C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CC1
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
be4b86020a065d99e289e528d425e25dd0737bea0f2fd81bb05a4d03f92a7d75
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(Nc1cccc2c1[nH]c1cnccc12)C1COCCN1CC(=O)N1CCNCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[#7:5]1-[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]-1>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:8]1-[C:7]-[C:6]-[#7:5]-[C:10]-[C:9]-1
12
[{"value": 12.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(=O)N1CCN(CC1)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The desired compound was prepared using [5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid and 1-methyl piperazine following Method F in 12% yield. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1C[NH]CCN1
C1C[NH]CC[NH]1
C1C[NH]CC[NH]1.C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CN1CCNCC1>>CN1CCN(C(=O)CN2CC(C)(C)OCC2C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CC1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-497f81d843fd40b38b68639b9989b285
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CC1CNCC(C)O1>>CC1CN(C(=O)CN2CC(C)(C)OCC2C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CC(C)O1
ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1COC(CN1CC(=O)O)(C)C.CC1CNCC(O1)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(=O)N1CC(OC(C1)C)C
O[C:5](=[O:6])[CH2:7][N:8]1[CH2:9][C:10]([CH3:11])([CH3:12])[O:13][CH2:14][CH:15]1[C:16](=[O:17])[NH:18][c:19]1[cH:20][c:21]([Cl:22])[cH:23][c:24]2[c:25]1[nH:26][c:27]1[cH:28][n:29][cH:30][cH:31][c:32]21.[CH3:1][CH:2]1[CH2:3][NH:4][CH2:33][CH:34]([CH3:35])[O:36]1>>[CH3:1][CH:2]1[CH2:3][N:4]([C:5](=[O:6])[CH2:7][N:8]2[C...
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CC1CNCC(C)O1
CC1CN(C(=O)CN2CC(C)(C)OCC2C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CC(C)O1
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
2ef483949e7ba3e5f888cf14cdce25fa611f75be09fdf1854a473be519821b59
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(Nc1cccc2c1[nH]c1cnccc12)C1COCCN1CC(=O)N1CCOCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[#8:5]1-[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]-1>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:8]1-[C:9]-[C:10]-[#8:5]-[C:6]-[C:7]-1
null
[]
null
null
null
null
The desired compound was prepared using [5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid and 2,6-dimethyl morpholine following Method F. Chromatographic purification gave the desired product in 70-80% yield. Conditions: See reaction.notes.procedure_details. Workup: The desired compo...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1.C1COCC[NH]1.c1ccc2c(c1)[nH]c1cnccc12
HO-
null
null
null
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.CC1CNCC(C)O1>>CC1CN(C(=O)CN2CC(C)(C)OCC2C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CC(C)O1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-8b72ff95936842d0a95d831f3c3c8d3b
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.N[C@H]1CC[C@H](O)CC1>>CC1(C)CN(CC(=O)N[C@@H]2CC[C@@H](O)CC2)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
C(CCl)Cl.ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1COC(CN1CC(=O)O)(C)C.Cl.N[C@@H]1CC[C@H](CC1)O.C(C)(C)N(CC)C(C)C>>ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(N[C@@H]1CC[C@H](CC1)O)=O
O[C:7]([CH2:6][N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[O:36][CH2:35][CH:17]1[C:18](=[O:19])[NH:20][c:21]1[cH:22][c:23]([Cl:24])[cH:25][c:26]2[c:27]1[nH:28][c:29]1[cH:30][n:31][cH:32][cH:33][c:34]21)=[O:8].[NH2:9][C@H:10]1[CH2:11][CH2:12][C@H:13]([OH:14])[CH2:15][CH2:16]1>>[CH3:1][C:2]1([CH3:3])[CH2:4][N:5]([CH2:6][C:7](=[O...
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.N[C@H]1CC[C@H](O)CC1
CC1(C)CN(CC(=O)N[C@@H]2CC[C@@H](O)CC2)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1
null
null
O.N1=CC=CC=C1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(CN1CCOCC1C(=O)Nc1cccc2c1[nH]c1cnccc12)NC1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[C:6](-[C:5])-[C:8]
60
[{"value": 59.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(N[C@@H]1CC[C@H](CC1)O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.0, "product": "ClC=1C=C2C=3C=CN=CC3NC2=C(C1)NC(=O)C1N(CC(OC1)(C)C)CC(N[C@@H]1CC[C@H](CC1)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": f...
null
null
null
null
[5-(6-Chloro-9H-beta-carbolin-8-ylcarbamoyl)-2,2-dimethyl-morpholin-4-yl]-acetic acid (200 mg, 0.48 mmol), trans-4-aminocyclohexanol hydrochloride (145 mg, 0.96 mmol) and diisopropylethylamine (124 mg, 167 uL, 0.96 mmol) were dissolved in pyridine (4 mL) and stirred at room temperature10 min. EDC (184 mg) was added and...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1COCC[NH]1.C1CCCCC1.c1ccc2c(c1)[nH]c1cnccc12
HO-
O.N1=CC=CC=C1
null
null
CC1(C)CN(CC(=O)O)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1.N[C@H]1CC[C@H](O)CC1>O.N1=CC=CC=C1>CC1(C)CN(CC(=O)N[C@@H]2CC[C@@H](O)CC2)C(C(=O)Nc2cc(Cl)cc3c2[nH]c2cnccc23)CO1