dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-0f09a2bb51314285b6f991b9d512a73d
CC(C)(C)OC(=O)N1CCC(=O)CC1.CI>>CC(C)(C)OC(=O)N1CCC(=O)C(C)(C)C1
C(C)(C)(C)OC(=O)N1CCC(CC1)=O.O1CCCC1.[H-].[Na+].CI>>C(C)(C)(C)OC(=O)N1CC(C(CC1)=O)(C)C
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][C:11](=[O:12])[CH2:13][CH2:16]1.I[CH3:15]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][C:11](=[O:12])[C:13]([CH3:14])([CH3:15])[CH2:16]1
CC(C)(C)OC(=O)N1CCC(=O)CC1.CI
CC(C)(C)OC(=O)N1CCC(=O)C(C)(C)C1
null
null
null
C-C Coupling
OtherReaction
adac5963216d307b6de224f49f25d68455d025ace9329a773c47c2937f141090
6c72a64362b644ff7380f8d0c7bdda962edffb1f22535d7f0916fcd367b6b992
O=C1CCNCC1
I-[CH3;D1;+0:1].[C;D1;H3:2]-[C:3](-[C;D1;H3:4])(-[C;D1;H3:5])-[#8:6]-[C:7](=[O;D1;H0:8])-[#7:9]1-[C:10]-[CH2;D2;+0:11]-[C:12](=[O;D1;H0:13])-[C:14]-[C:15]-1>>[C;D1;H3:16]-[C;H0;D4;+0:11]1(-[CH3;D1;+0:1])-[C:10]-[#7:9](-[C:7](=[O;D1;H0:8])-[#8:6]-[C:3](-[C;D1;H3:2])(-[C;D1;H3:4])-[C;D1;H3:5])-[C:15]-[C:14]-[C:12]-1=[O;D...
32
[{"value": 32.0, "product": "C(C)(C)(C)OC(=O)N1CC(C(CC1)=O)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
10
MINUTE
4-Oxo-piperidine-1-carboxylic acid tert-butyl ester (5 g, 25 mmol) was dissolved in tetrahydrofuran (100 mL) and the resulting solution was cooled to 0° C. Sodium hydride (60% in mineral oil, 2.10 g, 53 mmol) was added to the cooled solution in a single portion, and the resulting cloudy mixture was allowed to stir 10 m...
10.6084/m9.figshare.5104873.v1
null
Ketone
Ketone
C1CC[NH]CC1
C1CC[NH]CC1
C1CC[NH]CC1
null
null
0
0.166667
CC(C)(C)OC(=O)N1CCC(=O)CC1.CI>>CC(C)(C)OC(=O)N1CCC(=O)C(C)(C)C1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-56dffb8badf046c4b6812a170c7583af
CC(C)(C)OC(=O)N1CCC(=O)C(C)(C)C1>>CC1(C)CNCCC1=O
C(C)(C)(C)OC(=O)N1CC(C(CC1)=O)(C)C.FC(C(=O)O)(F)F.FC(C(=O)O)(F)F>>CC1(CNCCC1=O)C
CC(C)(C)OC(=O)[N:5]1[CH2:4][C:2]([CH3:1])([CH3:3])[C:8](=[O:9])[CH2:7][CH2:6]1>>[CH3:1][C:2]1([CH3:3])[CH2:4][NH:5][CH2:6][CH2:7][C:8]1=[O:9]
CC(C)(C)OC(=O)N1CCC(=O)C(C)(C)C1
CC1(C)CNCCC1=O
null
null
C(Cl)Cl
Reduction
Boc amine deprotection
bf3cd5dc3e17e694d8665c89f5d7e08e8763b18436a633eb66e9bf530b8b0316
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=C1CCNCC1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[C:4](=[O;D1;H0:5])-[C:6]-[C:7]-1>>[O;D1;H0:5]=[C:4]1-[C:3]-[C:2]-[NH;D2;+0:1]-[C:7]-[C:6]-1
null
[]
null
null
2
HOUR
The 3,3-dimethyl-4-oxo-piperidine-1-carboxylic acid tert-butyl ester thus prepared (450 mg, 1.97 mmol) was dissolved in methylene chloride (10 mL). Trifluoroacetic acid was added (305 uL) and the resulting solution stirred at room temperature 2 h. Additional trifluoroacetic acid was added (300 uL) and the reaction stir...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1CC[NH]CC1
C1CCNCC1
C1CCNCC1
HO-
C(Cl)Cl
null
2
CC(C)(C)OC(=O)N1CCC(=O)C(C)(C)C1>C(Cl)Cl>CC1(C)CNCCC1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-8f1b7bacbef04f158bc05613acb1e601
COC(=O)c1c(N)c([N+](=O)[O-])cc(B2OC(C)(C)C(C)(C)O2)c1F.Cn1ccc(OS(=O)(=O)C(F)(F)F)cc1=O>>COC(=O)c1c(N)c([N+](=O)[O-])cc(-c2ccn(C)c(=O)c2)c1F
CN1C(C=C(C=C1)OS(=O)(=O)C(F)(F)F)=O.[Cl-].[Li+].C([O-])([O-])=O.[Na+].[Na+].COC(C1=C(C(=CC(=C1F)B1OC(C(O1)(C)C)(C)C)[N+](=O)[O-])N)=O>>COC(C1=C(C(=CC(=C1F)C1=CC(N(C=C1)C)=O)[N+](=O)[O-])N)=O
CC1(C)OB([c:13]2[cH:12][c:8]([N+:9](=[O:10])[O-:11])[c:6]([NH2:7])[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:22]2[F:23])OC1(C)C.O=S(=O)(O[c:14]1[cH:15][cH:16][n:17]([CH3:18])[c:19](=[O:20])[cH:21]1)C(F)(F)F>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH2:7])[c:8]([N+:9](=[O:10])[O-:11])[cH:12][c:13](-[c:14]2[cH:15][cH:16][n:17]([CH...
COC(=O)c1c(N)c([N+](=O)[O-])cc(B2OC(C)(C)C(C)(C)O2)c1F.Cn1ccc(OS(=O)(=O)C(F)(F)F)cc1=O
COC(=O)c1c(N)c([N+](=O)[O-])cc(-c2ccn(C)c(=O)c2)c1F
null
null
COCCOC
C-C Coupling
Suzuki coupling with boronic esters OTf
a3d570e4e0fd76e9f22489a70a6350782719cf47be069d1c7a3ebdc884544e3b
c376e10fbe6bc6c372c1e0d96cbf0a9d9ea35ea77075840731f29cc7280d2ecc
O=c1cc(-c2ccccc2)cc[nH]1
C-C1(-C)-O-B(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[F;D1;H0:5]):[c:6]-[C:7](-[#8:8])=[O;D1;H0:9])-O-C-1(-C)-C.F-C(-F)(-F)-S(=O)(=O)-O-[c;H0;D3;+0:10]1:[c:11]:[c:12]:[#7;a:13](-[C;D1;H3:14]):[c:15](=[O;D1;H0:16]):[c:17]:1>>[#8:8]-[C:7](=[O;D1;H0:9])-[c:6]:[c:4](-[F;D1;H0:5]):[c;H0;D3;+0:1](-[c;H0;D3;+0:10]1:[c:11]:[c:12]...
25
[{"value": 25.0, "product": "COC(C1=C(C(=CC(=C1F)C1=CC(N(C=C1)C)=O)[N+](=O)[O-])N)=O", "details": "PERCENTYIELD", "is_desired": false}]
90
CELSIUS
18
HOUR
To a solution of 2-amino-5-bromo-6-fluoro-3-nitro-benzoic acid methyl ester (1.0 g, 3.4 mmol) in dioxane (25 mL), under nitrogen atmosphere, was added bispinacoladaboron (1.3 g, 5.1 mmol), dichloro[1,1′-bis(diphenylphosphine)ferrocene]palladium (II) dichlormethane adduct (0.125 g, 0.17 mmol), and potassium acetate (1.0...
10.6084/m9.figshare.5104873.v1
null
Triflate.Boronic ester
null
B1OCCO1.c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
TfOH.HO-.B
COCCOC
90
18
COC(=O)c1c(N)c([N+](=O)[O-])cc(B2OC(C)(C)C(C)(C)O2)c1F.Cn1ccc(OS(=O)(=O)C(F)(F)F)cc1=O>COCCOC>COC(=O)c1c(N)c([N+](=O)[O-])cc(-c2ccn(C)c(=O)c2)c1F
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e16e26ba504e42cea01239161cdd285d
Nc1c(C(=O)C2CCCCC2)cc(Br)cc1[N+](=O)[O-].c1cncc(B2OCCCO2)c1>>Nc1c(C(=O)C2CCCCC2)cc(-c2cccnc2)cc1[N+](=O)[O-]
C(=O)(O)[O-].[Na+].B1(OCCCO1)C2=CN=CC=C2.NC1=C(C=C(C=C1[N+](=O)[O-])Br)C(=O)C1CCCCC1>>NC1=C(C=C(C=C1[N+](=O)[O-])C=1C=NC=CC1)C(=O)C1CCCCC1
Br[c:13]1[cH:12][c:3]([C:4](=[O:5])[CH:6]2[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11]2)[c:2]([NH2:1])[c:21]([N+:22](=[O:23])[O-:24])[cH:20]1.C1COB([c:14]2[cH:15][cH:16][cH:17][n:18][cH:19]2)OC1>>[NH2:1][c:2]1[c:3]([C:4](=[O:5])[CH:6]2[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11]2)[cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][n:18][cH:...
Nc1c(C(=O)C2CCCCC2)cc(Br)cc1[N+](=O)[O-].c1cncc(B2OCCCO2)c1
Nc1c(C(=O)C2CCCCC2)cc(-c2cccnc2)cc1[N+](=O)[O-]
null
null
CCOC(=O)C.COCCOC
C-C Coupling
Suzuki coupling with boronic esters
24090aed37a48c66cce36a374df588b856a5a96d58744799fd5f32d2bb560bf0
48892094855745f5c51f8910c27ce7c101e08ad3f9da2a58d5512e3d9c1b432f
O=C(c1cccc(-c2cccnc2)c1)C1CCCCC1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]-[C:4]=[O;D1;H0:5]):[c:6]:[c:7].C1-C-O-B(-[c;H0;D3;+0:8]2:[c:9]:[c:10]:[c:11]:[#7;a:12]:[c:13]:2)-O-C-1>>[O;D1;H0:5]=[C:4]-[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8]1:[c:9]:[c:10]:[c:11]:[#7;a:12]:[c:13]:1):[c:6]:[c:7]
89
[{"value": 89.0, "product": "NC1=C(C=C(C=C1[N+](=O)[O-])C=1C=NC=CC1)C(=O)C1CCCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.5, "product": "NC1=C(C=C(C=C1[N+](=O)[O-])C=1C=NC=CC1)C(=O)C1CCCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
90
MINUTE
To a solution of (2-amino-5-bromo-3-nitro-phenyl)-cyclohexyl-methanone (600 mg, 1.83 mmol) in DME (25 mL) was added, successively, pyridine-3-boronic acid 1,3-propanediol cyclic ester (388 mg, 2.38 mmol), (tetrakistriphenylphosphine) palladium(0) (212 mg, 0.18 mmol), and 1N NaHCO3 (3.7 mL, 3.7 mmol). The resulting mixt...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccccc1.B1OCCCO1.c1ccncc1
c1ccccc1.c1ccncc1
c1ccccc1.C1CCCCC1.c1ccncc1
HBr.B
CCOC(=O)C.COCCOC
null
1.5
Nc1c(C(=O)C2CCCCC2)cc(Br)cc1[N+](=O)[O-].c1cncc(B2OCCCO2)c1>CCOC(=O)C.COCCOC>Nc1c(C(=O)C2CCCCC2)cc(-c2cccnc2)cc1[N+](=O)[O-]
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-becf597f931c48eab6d0ab9385f0ebff
BrBr.COC(=O)c1cccc([N+](=O)[O-])c1N>>COC(=O)c1cc(Br)cc([N+](=O)[O-])c1N
COC(C1=C(C(=CC=C1)[N+](=O)[O-])N)=O.BrBr>>COC(C1=C(C(=CC(=C1)Br)[N+](=O)[O-])N)=O
Br[Br:8].[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:9][c:10]([N+:11](=[O:12])[O-:13])[c:14]1[NH2:15]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([Br:8])[cH:9][c:10]([N+:11](=[O:12])[O-:13])[c:14]1[NH2:15]
BrBr.COC(=O)c1cccc([N+](=O)[O-])c1N
COC(=O)c1cc(Br)cc([N+](=O)[O-])c1N
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
f6effe61353895b318215d8bd9b6bb1105cafbf7be8c217d748df587260b32c3
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccccc1
Br-[Br;H0;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]:[c:6]:[cH;D2;+0:7]:[c:8]:[c:9]>>[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]:[c:6]:[c;H0;D3;+0:7](-[Br;H0;D1;+0:1]):[c:8]:[c:9]
87.4
[{"value": 82.0, "product": "COC(C1=C(C(=CC(=C1)Br)[N+](=O)[O-])N)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.4, "product": "COC(C1=C(C(=CC(=C1)Br)[N+](=O)[O-])N)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of 2.23 g (10.4 mmol) of 2-amino-3-nitro-benzoic acid methyl ester in 12 mL of acetic acid was added dropwise over 5 minutes a solution of 0.53 mL (10.4 mmol, 1 eq) of bromine in 2 mL of acetic acid. The mixture was stirred at room temperature for 30 minutes and poured into 100 grams of ice. The precipita...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1
HBr
C(C)(=O)O
null
0.5
BrBr.COC(=O)c1cccc([N+](=O)[O-])c1N>C(C)(=O)O>COC(=O)c1cc(Br)cc([N+](=O)[O-])c1N
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a1eedacf1b8549838884bd4e41b128f0
COC(=O)c1cc(B2OC(C)(C)C(C)(C)O2)cc([N+](=O)[O-])c1N.Cc1cccnc1-n1c(C)cc(OS(=O)(=O)C(F)(F)F)cc1=O>>COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc([N+](=O)[O-])c1N
COC(C1=C(C(=CC(=C1)B1OC(C(O1)(C)C)(C)C)[N+](=O)[O-])N)=O.CC=1C(=NC=CC1)N1C(C=C(C=C1C)OS(=O)(=O)C(F)(F)F)=O.C([O-])([O-])=O.[Na+].[Na+]>>COC(C1=C(C(=CC(=C1)C1=CC(C(C(=C1)C)CC1=NC=CC=C1)=O)[N+](=O)[O-])N)=O
CC1(C)OB([c:7]2[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:28]([NH2:29])[c:24]([N+:25](=[O:26])[O-:27])[cH:23]2)O[C:12]1(C)C.O=S(=O)(O[c:8]1[cH:9][c:10](=[O:11])n(-[c:14]2[c:15]([CH3:13])[cH:16][cH:17][cH:18][n:19]2)[c:20]([CH3:21])[cH:22]1)C(F)(F)F>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([C:8]2=[CH:9][C:10](=[O:11])[...
COC(=O)c1cc(B2OC(C)(C)C(C)(C)O2)cc([N+](=O)[O-])c1N.Cc1cccnc1-n1c(C)cc(OS(=O)(=O)C(F)(F)F)cc1=O
COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc([N+](=O)[O-])c1N
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
COCCOC
C-C Coupling
OtherReaction
ff374bc0f966ac2c660c8c98edfc5f1bde6d27ce574152e42066dfdfcefbf961
edd4560b8a1be426237062e9a97abe24adb8300f6c980bf4d4d1bfac5151ff0f
O=C1C=C(c2ccccc2)C=CC1Cc1ccccn1
C-C1(-C)-O-B(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]-[C:6](-[#8:7])=[O;D1;H0:8])-O-[C;H0;D4;+0:9]-1(-C)-C.F-C(-F)(-F)-S(=O)(=O)-O-[c;H0;D3;+0:10]1:[cH;D2;+0:11]:[c;H0;D3;+0:12](-[C;D1;H3:13]):n(-[c;H0;D3;+0:14]2:[#7;a:15]:[c:16]:[c:17]:[c:18]:[c;H0;D3;+0:19]:2-[CH3;D1;+0:20]):[c;H0;D3;+0:21](=[O;D1;H0:22]):[cH;D2;+0:...
175.4
[{"value": 89.0, "product": "COC(C1=C(C(=CC(=C1)C1=CC(C(C(=C1)C)CC1=NC=CC=C1)=O)[N+](=O)[O-])N)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 175.4, "product": "COC(C1=C(C(=CC(=C1)C1=CC(C(C(=C1)C)CC1=NC=CC=C1)=O)[N+](=O)[O-])N)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 2-amino-3-nitro-5-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-benzoic acid methyl ester (0.163 g, 0.51 mmol) in ethylene glycol dimethylether (5 mL) was added N-(methyl-2-pyridinyl)-6-methyl-4-trifluoromethylsulfonyloxy-2-pyridone (0.136 g, 0.41 mmol), bis(triphenylphoshine)palladium (II) dichloride...
10.6084/m9.figshare.5104873.v1
null
Triflate.Boronic ester
Ketone
B1OCCO1.c1ccccc1.c1ccncc1.c1ccncc1
c1ccccc1.C1=CCCC=C1.c1ccncc1
c1ccccc1.C1=CCCC=C1.c1ccncc1
TfOH.HO-.B
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.COCCOC
null
null
COC(=O)c1cc(B2OC(C)(C)C(C)(C)O2)cc([N+](=O)[O-])c1N.Cc1cccnc1-n1c(C)cc(OS(=O)(=O)C(F)(F)F)cc1=O>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.COCCOC>COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc([N+](=O)[O-])c1N
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-7f08f46a32ed4e2799df6df233f19d76
COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc([N+](=O)[O-])c1N>>COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc(N)c1N
COC(C1=C(C(=CC(=C1)C1=CC(C(C(=C1)C)CC1=NC=CC=C1)=O)[N+](=O)[O-])N)=O>>COC(C1=C(C(=CC(=C1)C1=CC(C(C(=C1)C)CC1=NC=CC=C1)=O)N)N)=O
O=[N+:25]([O-])[c:24]1[cH:23][c:7]([C:8]2=[CH:9][C:10](=[O:11])[CH:12]([CH2:13][c:14]3[cH:15][cH:16][cH:17][cH:18][n:19]3)[C:20]([CH3:21])=[CH:22]2)[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:26]1[NH2:27]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([C:8]2=[CH:9][C:10](=[O:11])[CH:12]([CH2:13][c:14]3[cH:15][cH:16][cH:17][c...
COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc([N+](=O)[O-])c1N
COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc(N)c1N
null
[Pd]
C(C)(=O)OCC
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
O=C1C=C(c2ccccc2)C=CC1Cc1ccccn1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
24
HOUR
To a slurry of 10% palladium on carbon (0.045 g) in ethyl acetate (20 mL) was added 2-amino-5-(5-methyl-3-oxo-4-pyridin-2-ylmethyl-cyclohexa-1,5-dienyl)-3-nitro-benzoic acid methyl ester (0.176 g, 0.44 mmol). The resulting mixture was hydrogenated at 30 psi for 24 hours. The reaction was filtered, concentrated in vacuo...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.C1=CCCC=C1.c1ccncc1
Other
[Pd].C(C)(=O)OCC
null
24
COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc([N+](=O)[O-])c1N>[Pd].C(C)(=O)OCC>COC(=O)c1cc(C2=CC(=O)C(Cc3ccccn3)C(C)=C2)cc(N)c1N
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-81533076c8b148cfa53adb9113171694
Cc1cc(O)cc(=O)o1.NCc1ccccn1>>Cc1cc(O)cc(=O)n1Cc1ccccn1
OC1=CC(OC(=C1)C)=O.NCC1=NC=CC=C1>>OC1=CC(N(C(=C1)C)CC1=NC=CC=C1)=O
o1[c:2]([CH3:1])[cH:3][c:4]([OH:5])[cH:6][c:7]1=[O:8].[NH2:9][CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][n:16]1>>[CH3:1][c:2]1[cH:3][c:4]([OH:5])[cH:6][c:7](=[O:8])[n:9]1[CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][n:16]1
Cc1cc(O)cc(=O)o1.NCc1ccccn1
Cc1cc(O)cc(=O)n1Cc1ccccn1
null
null
O
Miscellaneous
OtherReaction
820fdf5c7d90563efa4f0fcdced261f60cc5772161039256cfa8cd4dfa87d9f6
74f861e099b6420f2f6d4f3094b402eaca1d0baec018283dff42a39bacc23c31
O=c1ccccn1Cc1ccccn1
[#7;a:1]:[c:2]-[C:3]-[NH2;D1;+0:4].[C;D1;H3:5]-[c;H0;D3;+0:6]1:[c:7]:[c:8]:[c:9]:[c;H0;D3;+0:10](=[O;D1;H0:11]):o:1>>[#7;a:1]:[c:2]-[C:3]-[n;H0;D3;+0:4]1:[c;H0;D3;+0:6](-[C;D1;H3:5]):[c:7]:[c:8]:[c:9]:[c;H0;D3;+0:10]:1=[O;D1;H0:11]
92
[{"value": 92.0, "product": "OC1=CC(N(C(=C1)C)CC1=NC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.8, "product": "OC1=CC(N(C(=C1)C)CC1=NC=CC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 12.6 g (0.1 mol) of 4-hydroxy-6-methyl-2-pyrone in 50 ml water was added 2-(aminomethyl)pyridine (10.3 ml, 0.1 mol) and the mixture heated to reflux for 2.5 hours. The resulting light yellow compound was filtered from the cooled mixture. Concentration of the filtrate and trituration of the resulting ...
10.6084/m9.figshare.5104873.v1
null
Primary amine
null
c1ccocc1
c1ccncc1
c1ccncc1.c1ccncc1
HO-
O
null
null
Cc1cc(O)cc(=O)o1.NCc1ccccn1>O>Cc1cc(O)cc(=O)n1Cc1ccccn1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-7c5490cbc6894f5eace522a61c214842
CCC(=O)c1cc(-c2cccnc2)cc(N)c1N.CCOC(=O)Cl.CSC(=N)N>>CCOC(=O)Nc1nc2cc(-c3cccnc3)cc(C(=O)CC)c2[nH]1
[OH-].[Na+].CSC(N)=N.ClC(=O)OCC.NC1=C(C=C(C=C1N)C=1C=NC=CC1)C(CC)=O>>C(C)OC(NC1=NC2=C(N1)C(=CC(=C2)C=2C=NC=CC2)C(CC)=O)=O
N[c:9]1[cH:10][c:11](-[c:12]2[cH:13][cH:14][cH:15][n:16][cH:17]2)[cH:18][c:19]([C:20](=[O:21])[CH2:22][CH3:23])[c:24]1[NH2:25].Cl[C:4]([O:3][CH2:2][CH3:1])=[O:5].CS[C:7](=[NH:6])[NH2:8]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[NH:6][c:7]1[n:8][c:9]2[cH:10][c:11](-[c:12]3[cH:13][cH:14][cH:15][n:16][cH:17]3)[cH:18][c:19]([C:20]...
CCC(=O)c1cc(-c2cccnc2)cc(N)c1N.CCOC(=O)Cl.CSC(=N)N
CCOC(=O)Nc1nc2cc(-c3cccnc3)cc(C(=O)CC)c2[nH]1
null
null
CCOC(=O)C.O.CC(=O)O
Aromatic Heterocycle Formation
OtherReaction
4f29f3a8af52fec42d5fedbc355b03722bbdaeb3b09af1107ebe5468967a34c5
805e227b2c6755047f43a4a1a2e9d66e7cbb3ddfe7dff9346d36caf7629b7b5a
c1cncc(-c2ccc3[nH]cnc3c2)c1
C-S-[C;H0;D3;+0:1](-[NH2;D1;+0:2])=[NH;D1;+0:3].Cl-[C;H0;D3;+0:4](=[O;D1;H0:5])-[#8:6]-[C:7].N-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11](-[NH2;D1;+0:12]):[c:13]-[C:14]=[O;D1;H0:15]>>[C:7]-[#8:6]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[NH;D2;+0:3]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:2]:[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11](:[c:13]-[C:14]=[O;D1...
null
[]
90
CELSIUS
null
null
To a mixture of 2-methyl-2-thiopseudourea (109 mg, 0.39 mmol) and ethyl chloroformate (75 μL, 0.78 mmol) in water (2 mL) at 5° C. was added over 40 minutes a 6N aqueous NaOH solution until pH stabilized to 8. The pH was then adjusted to 5 with glacial AcOH. A suspension of 1-(2,3-diamino-5-pyridin-3-yl-phenyl)-propan-1...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine.Primary amine.Primary amine.Monosulfide
Carbamic ester.Ether
c1ccccc1
c1ccc2[nH]cnc2c1
c1ccc2[nH]cnc2c1.c1ccncc1
HCl
CCOC(=O)C.O.CC(=O)O
90
null
CCC(=O)c1cc(-c2cccnc2)cc(N)c1N.CCOC(=O)Cl.CSC(=N)N>CCOC(=O)C.O.CC(=O)O>CCOC(=O)Nc1nc2cc(-c3cccnc3)cc(C(=O)CC)c2[nH]1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2a5afcdb095849ddb861073e42e5abbe
CN(CCCN)CCCNC(=O)OC(C)(C)C.O=C1OC(=O)c2cccc3cccc1c23>>CN(CCCNC(=O)OC(C)(C)C)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32
C=1C=C2C=CC=C3C2=C(C1)C(=O)OC3=O.C(C)(C)(C)OC(NCCCN(C)CCCN)=O>>C(C)(C)(C)OC(NCCCN(C)CCCN1C(C2=CC=CC=3C2C(C1=O)C=CC3)=O)=O
[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])[CH2:14][CH2:15][CH2:16][NH2:17].O1[C:18](=[O:19])[c:20]2[cH:21][cH:22][cH:23][c:24]3[cH:25][cH:26][cH:27][c:28]([c:31]23)[C:29]1=[O:30]>>[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:...
CN(CCCN)CCCNC(=O)OC(C)(C)C.O=C1OC(=O)c2cccc3cccc1c23
CN(CCCNC(=O)OC(C)(C)C)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32
null
null
C(C)O
Acylation
OtherReaction
22f1b70036b326cbdeda8645a1baab3f0ee3c30ace9b39f67ef3491a99d192d0
bb5fdd7481898ce385823b84bf0948a8494704a7a4bb697222c9736fb995b96a
O=C1NC(=O)C2C=CC=C3C=CC=C1C32
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c;H0;D3;+0:8]2:[cH;D2;+0:9]:[cH;D2;+0:10]:[cH;D2;+0:11]:[c;H0;D3;+0:12]3:[cH;D2;+0:13]:[cH;D2;+0:14]:[cH;D2;+0:15]:[c;H0;D3;+0:16]-1:[c;H0;D3;+0:17]:3:2>>[C:1]-[C:2]-[N;H0;D3;+0:3]1-[C;H0;D3;+0:5](=[O;D1;H0:4])-[C;H0;D3;+0:16]2=[CH;D2...
90
[{"value": 90.0, "product": "C(C)(C)(C)OC(NCCCN(C)CCCN1C(C2=CC=CC=3C2C(C1=O)C=CC3)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
1,8-naphthalic anhydride (0.18 g, 0.9 mmol) was added to a solution of [3-[(3-aminopropyl)methylamino]propyl]carbamic acid tert-butyl ester previously prepared (Spicer at el., Bioorg. Med. Chem. 2002, vol. 10, p. 19) (0.2 g, 0.8 mmol) in absolute ethanol (20 ml). The reaction mixture was heated at reflux overnight. Rem...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Primary amine
Substituted dicarboximide.Conjugated diene.Conjugated diene
c1cc2c3c(cccc3c1)COC2
C1=CC2=CC=CC3C[NH]CC(=C1)C23
C1=CC2=CC=CC3C[NH]CC(=C1)C23
Other
C(C)O
null
null
CN(CCCN)CCCNC(=O)OC(C)(C)C.O=C1OC(=O)c2cccc3cccc1c23>C(C)O>CN(CCCNC(=O)OC(C)(C)C)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-146cb0dd04144bee85c6a1e7e2520d6e
CN(CCCNC(=O)OC(C)(C)C)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32>>CN(CCCN)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32
C(C)(C)(C)OC(NCCCN(C)CCCN1C(C2=CC=CC=3C2C(C1=O)C=CC3)=O)=O.FC(C(=O)O)(F)F>>NCCCN(CCCN1C(C2=CC=CC=3C2C(C1=O)C=CC3)=O)C
CC(C)(C)OC(=O)[NH:6][CH2:5][CH2:4][CH2:3][N:2]([CH3:1])[CH2:7][CH2:8][CH2:9][N:10]1[C:11](=[O:12])[C:13]2=[CH:14][CH:15]=[CH:16][C:17]3=[CH:18][CH:19]=[CH:20][CH:21]([C:22]1=[O:23])[CH:24]23>>[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][NH2:6])[CH2:7][CH2:8][CH2:9][N:10]1[C:11](=[O:12])[C:13]2=[CH:14][CH:15]=[CH:16][C:17]3=[CH:1...
CN(CCCNC(=O)OC(C)(C)C)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32
CN(CCCN)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32
null
null
C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=C1NC(=O)C2C=CC=C3C=CC=C1C32
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]-[C:3]>>[C:3]-[C:2]-[NH2;D1;+0:1]
92
[{"value": 92.0, "product": "NCCCN(CCCN1C(C2=CC=CC=3C2C(C1=O)C=CC3)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.5, "product": "NCCCN(CCCN1C(C2=CC=CC=3C2C(C1=O)C=CC3)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
To a solution of [3-[[3-(1,3-dioxo-3a,9b-dihydro-1H,3H-benzo[de]isoquinolin-2-yl)propyl]methylamino]propyl]carbamic acid tert-butyl ester (0.34 g, 0.81 mmol) in CH2Cl2 (24 ml) was added trifluoroacetic acid (6 ml). The reaction mixture was stirred at room temperature for 16 h at which point the reaction was completed b...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
C1=CC2=CC=CC3C[NH]CC(=C1)C23
HO-
C(Cl)Cl
null
16
CN(CCCNC(=O)OC(C)(C)C)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32>C(Cl)Cl>CN(CCCN)CCCN1C(=O)C2=CC=CC3=CC=CC(C1=O)C32
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2f3f5155806b4c4baa1dd17e76b333bc
CN(CCCN)CCCNC(=O)OC(C)(C)C.Cn1c2c3ccccc3nc-2c(Cl)c2ccccc21>>CN(CCCNC(=O)OC(C)(C)C)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12
ClC1=C2C(N(C3=CC=CC=C13)C)=C1C=CC=CC1=N2.C(C)(C)(C)OC(NCCCN(C)CCCN)=O>>C(C)(C)(C)OC(NCCCN(CCCNC1=C2C(N(C3=CC=CC=C13)C)=C1C=CC=CC1=N2)C)=O
[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])[CH2:14][CH2:15][CH2:16][NH2:17].Cl[c:18]1[c:19]2[n:20][c:21]3[cH:22][cH:23][cH:24][cH:25][c:26]3[c:27]-2[n:28]([CH3:29])[c:30]2[cH:31][cH:32][cH:33][cH:34][c:35]12>>[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][NH:6][C:7](=[O:8])[O:9][C:...
CN(CCCN)CCCNC(=O)OC(C)(C)C.Cn1c2c3ccccc3nc-2c(Cl)c2ccccc21
CN(CCCNC(=O)OC(C)(C)C)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12
null
null
C(C)OCCO
Heteroatom Alkylation and Arylation
Buchwald-Hartwig/Ullmann-Goldberg/N-arylation primary amine
69609c4e4cf9899b9e03307454546bc48609f2b76dae99c49aa2731f943f6380
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc2[nH]c3c4ccccc4nc-3cc2c1
Cl-[c;H0;D3;+0:1]1:[c:2](:[#7;a:3]:[c:4])-[c:5]:[#7;a:6](-[C;D1;H3:7]):[c:8](:[c:9]):[c:10]:1:[c:11].[C:12]-[C:13]-[NH2;D1;+0:14]>>[C:12]-[C:13]-[NH;D2;+0:14]-[c;H0;D3;+0:1]1:[c:2](:[#7;a:3]:[c:4])-[c:5]:[#7;a:6](-[C;D1;H3:7]):[c:8](:[c:9]):[c:10]:1:[c:11]
490
[{"value": 490.0, "product": "C(C)(C)(C)OC(NCCCN(CCCNC1=C2C(N(C3=CC=CC=C13)C)=C1C=CC=CC1=N2)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
A solution of 11-chloro-5-methyl-5H-indolo[3,2-b]quinoline (cf. Bierer et al., J. Med. Chem. 1998, vol. 41, pp. 2754) (61 mg, 0.23 mmol) and [[3-[(3-amino-propyl)methylamino]propyl]carbamic acid tert-butyl ester previously prepared (Spicer at el., Bioorg. Med. Chem. 2002, vol. 10, p. 19) (84_l, 0.34 mmol) in 2-ethoxyet...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1c2ccccc2nc2c1[nH]c1ccccc12
c1c2ccccc2nc2c1[nH]c1ccccc12
c1c2ccccc2nc2c1[nH]c1ccccc12
HCl
C(C)OCCO
120
null
CN(CCCN)CCCNC(=O)OC(C)(C)C.Cn1c2c3ccccc3nc-2c(Cl)c2ccccc21>C(C)OCCO>CN(CCCNC(=O)OC(C)(C)C)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f3e9c5fcd68140c49a2971d0f6558957
CN(CCCNC(=O)OC(C)(C)C)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12>>CN(CCCN)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12
C(C)(C)(C)OC(NCCCN(CCCNC1=C2C(N(C3=CC=CC=C13)C)=C1C=CC=CC1=N2)C)=O.FC(C(=O)O)(F)F>>CN(CCCN)CCCNC1=C2C(N(C3=CC=CC=C13)C)=C1C=CC=CC1=N2
CC(C)(C)OC(=O)[NH:6][CH2:5][CH2:4][CH2:3][N:2]([CH3:1])[CH2:7][CH2:8][CH2:9][NH:10][c:11]1[c:12]2[n:13][c:14]3[cH:15][cH:16][cH:17][cH:18][c:19]3[c:20]-2[n:21]([CH3:22])[c:23]2[cH:24][cH:25][cH:26][cH:27][c:28]12>>[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][NH2:6])[CH2:7][CH2:8][CH2:9][NH:10][c:11]1[c:12]2[n:13][c:14]3[cH:15][c...
CN(CCCNC(=O)OC(C)(C)C)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12
CN(CCCN)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12
null
null
C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
c1ccc2[nH]c3c4ccccc4nc-3cc2c1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]-[C:3]>>[C:3]-[C:2]-[NH2;D1;+0:1]
101.2
[{"value": 92.0, "product": "CN(CCCN)CCCNC1=C2C(N(C3=CC=CC=C13)C)=C1C=CC=CC1=N2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 101.2, "product": "CN(CCCN)CCCNC1=C2C(N(C3=CC=CC=C13)C)=C1C=CC=CC1=N2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
To a solution of [3-[methyl-[3-(5-methyl-5H-indolo[3,2-b]quinolin-11-ylamino)-propyl]amino]propyl)-carbamic acid tert-butyl ester (49 mg, 0.1 mmol) in CH2Cl2 (10 ml), was added trifluoroacetic acid (12_l). This mixture was stirred at room temperature for 16 h, at which point the reaction was completed by TLC. All solve...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1c2ccccc2nc2c1[nH]c1ccccc12
HO-
C(Cl)Cl
null
16
CN(CCCNC(=O)OC(C)(C)C)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12>C(Cl)Cl>CN(CCCN)CCCNc1c2nc3ccccc3c-2n(C)c2ccccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-5ef6c1c4b096459d8233747f623d138d
CN(C)CCN.O=C(O)c1c2ccccc2nc2c1[nH]c1ccccc12>>CN(C)CCNC(=O)c1c2ccccc2nc2c1[nH]c1ccccc12
CN(CCN)C.C(C)N(CC)CC.C1=C2C(=C3C(=NC2=CC=C1)C1=CC=CC=C1N3)C(=O)O>>CN(CCNC(=O)C1=C2C(=NC3=CC=CC=C13)C1=CC=CC=C1N2)C
[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH2:6].O[C:7](=[O:8])[c:9]1[c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[n:16][c:17]2[c:18]1[nH:19][c:20]1[cH:21][cH:22][cH:23][cH:24][c:25]21>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH:6][C:7](=[O:8])[c:9]1[c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[n:16][c:17]2[c:18]1[nH:19][c:20]1[cH:21]...
CN(C)CCN.O=C(O)c1c2ccccc2nc2c1[nH]c1ccccc12
CN(C)CCNC(=O)c1c2ccccc2nc2c1[nH]c1ccccc12
null
null
O=S(Cl)Cl.C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
c1ccc2nc3c(cc2c1)[nH]c1ccccc13
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1:[#7;a:9]:[c:10].[C:11]-[C:12]-[NH2;D1;+0:13]>>[C:11]-[C:12]-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1:[#7;a:9]:[c:10]
61
[{"value": 61.0, "product": "CN(CCNC(=O)C1=C2C(=NC3=CC=CC=C13)C1=CC=CC=C1N2)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.2, "product": "CN(CCNC(=O)C1=C2C(=NC3=CC=CC=C13)C1=CC=CC=C1N2)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
10H-indolo[3,2-b]quinoline-11-carboxylic acid (0.5 g, 1.9 mmol) was dissolved in 20 ml of refluxing SOCl2, After 6 hours a clear solution was obtained, and all volatiles were removed in vacuo. The crude acid chloride was suspended in 10 ml of CH2Cl2. A solution of N,N-dimethylethylendiamine (0.2 mL, 2.26 mmol) and trie...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2nc3c(cc2c1)[nH]c1ccccc13
HO-
O=S(Cl)Cl.C(Cl)Cl
null
14
CN(C)CCN.O=C(O)c1c2ccccc2nc2c1[nH]c1ccccc12>O=S(Cl)Cl.C(Cl)Cl>CN(C)CCNC(=O)c1c2ccccc2nc2c1[nH]c1ccccc12
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-35de871dc825411f82857dabd9c55ffb
CC(N)CN(C)C.O=C(O)c1c2ccccc2nc2c1[nH]c1ccccc12>>CC(CNC(=O)c1c2ccccc2nc2c1[nH]c1ccccc12)N(C)C
CN(CC(C)N)C.C(C)N(CC)CC.C1=C2C(=C3C(=NC2=CC=C1)C1=CC=CC=C1N3)C(=O)O>>CN(C(CNC(=O)C1=C2C(=NC3=CC=CC=C13)C1=CC=CC=C1N2)C)C
[CH3:1][CH:2]([CH2:3][N:24]([CH3:25])[CH3:26])[NH2:4].O[C:5](=[O:6])[c:7]1[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[n:14][c:15]2[c:16]1[nH:17][c:18]1[cH:19][cH:20][cH:21][cH:22][c:23]21>>[CH3:1][CH:2]([CH2:3][NH:4][C:5](=[O:6])[c:7]1[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[n:14][c:15]2[c:16]1[nH:17][c:18]1[cH:19][cH:20]...
CC(N)CN(C)C.O=C(O)c1c2ccccc2nc2c1[nH]c1ccccc12
CC(CNC(=O)c1c2ccccc2nc2c1[nH]c1ccccc12)N(C)C
null
null
O=S(Cl)Cl.C(Cl)Cl
Acylation
OtherReaction
c996ad5dbf7289e706e061ab1b9f479c4034ccc7d44d3c472cdd0f07dfb90f02
bf57ff0584568f6455b9e238ebd2c49e1ed2227f45884308bd5a02d975532948
c1ccc2nc3c(cc2c1)[nH]c1ccccc13
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1:[#7;a:9]:[c:10].[C;D1;H3:11]-[CH;D3;+0:12](-[NH2;D1;+0:13])-[CH2;D2;+0:14]-[N;H0;D3;+0:15](-[C;D1;H3:16])-[C;D1;H3:17]>>[C;D1;H3:11]-[CH;D3;+0:12](-[CH2;D2;+0:14]-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1...
31
[{"value": 31.0, "product": "CN(C(CNC(=O)C1=C2C(=NC3=CC=CC=C13)C1=CC=CC=C1N2)C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
10H-Indolo[3,2-b]quinoline-11-carboxylic acid (0.2 g, 0.76 mmol) was dissolved in 8 ml of refluxing SOCl2. After 6 hours a clear solution was obtained, and all volatiles were removed in vacuo. The crude acid chloride was suspended in 10 ml of CH2Cl2. A solution of N,N-dimethylproylendiamine (0.1 mL, 0.97 mmol) and trie...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine.Tertiary amine
Secondary amide.Tertiary amine
null
null
c1ccc2nc3c(cc2c1)[nH]c1ccccc13
HO-
O=S(Cl)Cl.C(Cl)Cl
null
14
CC(N)CN(C)C.O=C(O)c1c2ccccc2nc2c1[nH]c1ccccc12>O=S(Cl)Cl.C(Cl)Cl>CC(CNC(=O)c1c2ccccc2nc2c1[nH]c1ccccc12)N(C)C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-50c8a89c96a84c2d904d41d6dcbe2b7b
COC(=O)c1ccc(N)c(NC(=O)c2cc(-c3ccncc3)n[nH]c2=O)c1>>COC(=O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
NC1=C(C=C(C(=O)OC)C=C1)NC(=O)C=1C(NN=C(C1)C1=CC=NC=C1)=O>>O=C1NN=C(C=C1C1=NC2=C(N1)C=CC(=C2)C(=O)OC)C2=CC=NC=C2
O=[C:10]([c:11]1[cH:12][c:13](-[c:14]2[cH:15][cH:16][n:17][cH:18][cH:19]2)[n:20][nH:21][c:22]1=[O:23])[NH:24][c:25]1[c:8]([NH2:9])[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:26]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[nH:9][c:10](-[c:11]3[cH:12][c:13](-[c:14]4[cH:15][cH:16][n:17][cH:18][cH:19]4)[n:20][n...
COC(=O)c1ccc(N)c(NC(=O)c2cc(-c3ccncc3)n[nH]c2=O)c1
COC(=O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
76e10ab81a93773d04ca0e55f8fb55bcd635323b5b4a9b9acd135658778da8ae
a079090652d9d6c0e17c70eeab94f6d7afea064f52cf5fa9036d5feedd14143a
O=c1[nH]nc(-c2ccncc2)cc1-c1nc2ccccc2[nH]1
O=[C;H0;D3;+0:1](-[NH;D2;+0:2]-[c:3](:[c:4]):[c:5](-[NH2;D1;+0:6]):[c:7])-[c;H0;D3;+0:8]1:[c:9]:[c:10](-[c:11]):[#7;a:12]:[#7;a:13]:[c:14]:1=[O;D1;H0:15]>>[O;D1;H0:15]=[c:14]1:[#7;a:13]:[#7;a:12]:[c:10](-[c:11]):[c:9]:[c;H0;D3;+0:8]:1-[c;H0;D3;+0:1]1:[n;H0;D2;+0:2]:[c:3](:[c:4]):[c:5](:[c:7]):[nH;D2;+0:6]:1
null
[]
100
CELSIUS
10
HOUR
A mixture of 1.3 g of methyl 4-amino-3-[(3-oxo-6-pyridin-4-yl-2,3-dihydro-pyridazine-4-carbonyl)amino]benzoate and 20 ml of glacial acetic acid is heated with stirring at 100° C. for 10 hours. The precipitate which has formed is filtered off with suction, washed with water and dried in vacuo at 50° C. Conditions: See r...
10.6084/m9.figshare.5104873.v1
null
Secondary amide.Primary amine
null
c1ccccc1
c1ccc2[nH]cnc2c1
c1ccc2[nH]cnc2c1.c1cnncc1.c1ccncc1
HO-
C(C)(=O)O
100
10
COC(=O)c1ccc(N)c(NC(=O)c2cc(-c3ccncc3)n[nH]c2=O)c1>C(C)(=O)O>COC(=O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c0220b86ef074eb9b947f35d3d72c66d
COC(=O)c1ccc(N)c(NC(=O)c2cc(-c3ccncc3)n[nH]c2=O)c1>>O=C(O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
Cl.NC1=C(C=C(C(=O)OC)C=C1)NC(=O)C=1C(NN=C(C1)C1=CC=NC=C1)=O.O1CCCC1.[OH-].[Li+]>>O=C1NN=C(C=C1C1=NC2=C(N1)C=CC(=C2)C(=O)O)C2=CC=NC=C2
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][c:7]([NH2:8])[c:24]([NH:23][C:9](=O)[c:10]2[cH:11][c:12](-[c:13]3[cH:14][cH:15][n:16][cH:17][cH:18]3)[n:19][nH:20][c:21]2=[O:22])[cH:25]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]2[nH:8][c:9](-[c:10]3[cH:11][c:12](-[c:13]4[cH:14][cH:15][n:16][cH:17][cH:18]4)[n:19][nH:20][c:21]3=[...
COC(=O)c1ccc(N)c(NC(=O)c2cc(-c3ccncc3)n[nH]c2=O)c1
O=C(O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
null
null
CO.O
Aromatic Heterocycle Formation
OtherReaction
48aa9b5dad0229f6283247a10f81eecd28630344f9188cdec5da8e2b5d867970
58ce411da13c66f484c8e30f72657c28f494944e68bff64e897497550b25cb23
O=c1[nH]nc(-c2ccncc2)cc1-c1nc2ccccc2[nH]1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[c:6](-[NH;D2;+0:7]-[C;H0;D3;+0:8](=O)-[c;H0;D3;+0:9]1:[c:10]:[c:11](-[c:12]):[#7;a:13]:[#7;a:14]:[c:15]:1=[O;D1;H0:16]):[c:17](-[NH2;D1;+0:18]):[c:19]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]:[c:5]:[c:6]1:[n;H0;D2;+0:7]:[c;H0;D3;+0:8](-[c;H0;D3;+0:9]2:[c:10]:[c:11](-[c:1...
null
[]
50
CELSIUS
5
HOUR
A mixture consisting of 500 mg of methyl 4-amino-3-[(3-oxo-6-pyridin-4-yl-2,3-dihydropyridazine-4-carbonyl)amino]benzoate, 6 ml of tetrahydrofuran (THF), 6 ml of methanol, 6 ml of water and 173 mg of lithium hydroxide is stirred at 50° C. for 5 hours. After cooling to room temperature, the pH is adjusted to 4-5 with 1N...
10.6084/m9.figshare.5104873.v1
null
Ester.Secondary amide.Primary amine
Carboxylic acid
c1ccccc1
c1ccc2[nH]cnc2c1
c1ccc2[nH]cnc2c1.c1cnncc1.c1ccncc1
HO-
CO.O
50
5
COC(=O)c1ccc(N)c(NC(=O)c2cc(-c3ccncc3)n[nH]c2=O)c1>CO.O>O=C(O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e1a5216f3afb44469e559d9e36406dd2
CCN(CC)CCN.O=C(O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1>>CCN(CC)CCNC(=O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
C(C)N(CC)CCN.O=C1NN=C(C=C1C1=NC2=C(N1)C=CC(=C2)C(=O)O)C2=CC=NC=C2.C(C)N(CC)CC.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1N=CC=C2)OC(=[N+](C)C)N(C)C>>C(C)N(CCNC(=O)C1=CC2=C(NC(=N2)C=2C(NN=C(C2)C2=CC=NC=C2)=O)C=C1)CC
[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[CH2:6][CH2:7][NH2:8].O[C:9](=[O:10])[c:11]1[cH:12][cH:13][c:14]2[nH:15][c:16](-[c:17]3[cH:18][c:19](-[c:20]4[cH:21][cH:22][n:23][cH:24][cH:25]4)[n:26][nH:27][c:28]3=[O:29])[n:30][c:31]2[cH:32]1>>[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[CH2:6][CH2:7][NH:8][C:9](=[O:10])[c:11]1[cH:12][cH:13...
CCN(CC)CCN.O=C(O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
CCN(CC)CCNC(=O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
null
null
O.CN(C=O)C
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=c1[nH]nc(-c2ccncc2)cc1-c1nc2ccccc2[nH]1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[c:6]:[#7;a:7].[C:8]-[C:9]-[NH2;D1;+0:10]>>[#7;a:7]:[c:6]:[c:5]:[c:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:10]-[C:9]-[C:8]):[c:4]
null
[]
null
null
10
MINUTE
A mixture consisting of 50 mg of 2-(3-oxo-6-pyridin-4-yl-2,3-dihydropyridazin-4-yl)-1H-benzoimidazole-5-carboxylic acid, 0.065 ml of triethylamine and 1.5 ml of dimethylformamide (DMF) is stirred at room temperature for 10 minutes, mixed with 68.4 mg of O-(7-azabenzotriazol-1-yl)-N,N,N′,N′-tetramethyluronium hexafluoro...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2[nH]cnc2c1.c1cnncc1.c1ccncc1
HO-
O.CN(C=O)C
null
0.166667
CCN(CC)CCN.O=C(O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1>O.CN(C=O)C>CCN(CC)CCNC(=O)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)nc2c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-51cce0ef0913412cbbe7e442c680ab1a
CCNC(=N)N.COC(C)(OC)C(=O)C=CN(C)C>>CCNc1nccc(C(C)=O)n1
CN(C=CC(C(C)(OC)OC)=O)C.Cl.C(C)NC(=N)N.[O-]CC.[Na+]>>C(C)NC1=NC=CC(=N1)C(C)=O
[CH3:1][CH2:2][NH:3][C:4](=[NH:5])[NH2:12].CO[C:9]([C:8](=O)[CH:7]=[CH:6]N(C)C)([CH3:10])[O:11]C>>[CH3:1][CH2:2][NH:3][c:4]1[n:5][cH:6][cH:7][c:8]([C:9]([CH3:10])=[O:11])[n:12]1
CCNC(=N)N.COC(C)(OC)C(=O)C=CN(C)C
CCNc1nccc(C(C)=O)n1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
1afa3d3b2993e219b919f6c309f76cb12069a08b72248b10b8c5223892bde6ae
cd3e3aec4550e62a12c260fe4030270c82d1dfd512053f92544190b939fd4229
c1cncnc1
C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-[O;H0;D2;+0:3]-C)-[C;H0;D3;+0:4](=O)-[CH;D2;+0:5]=[CH;D2;+0:6]-N(-C)-C.[C:7]-[#7:8]-[C;H0;D3;+0:9](-[NH2;D1;+0:10])=[NH;D1;+0:11]>>[C:7]-[#7:8]-[c;H0;D3;+0:9]1:[n;H0;D2;+0:10]:[c;H0;D3;+0:4](-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;H0;D1;+0:3]):[cH;D2;+0:5]:[cH;D2;+0:6]:[n;H0;D2;+0:11]:1
null
[]
null
null
8
HOUR
A mixture of 6 g of 1-dimethylamino-4,4-dimethoxypent-1-en-3-one, 3.96 g of N-ethylguanidine hydrochloride and 26 ml of 20% strength ethanolic sodium ethoxide solution is heated under reflux for 2 hours. After cooling, the solid is filtered off with suction, and the filtrate is concentrated in vacuo and mixed with 20 m...
10.6084/m9.figshare.5104873.v1
null
Enamine.Ketone.Ether.Ether.Primary amine
Ketone
null
c1cncnc1
c1cncnc1
HO-
null
null
8
CCNC(=N)N.COC(C)(OC)C(=O)C=CN(C)C>>CCNc1nccc(C(C)=O)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-0d9dbd0ceb884aa9952e31fab8bb9478
CCNc1nccc(C(C)=O)n1.CCOC(=O)C(=O)C(=O)OCC>>CCNc1nccc(C(=O)CC(O)(C(=O)OCC)C(=O)OCC)n1
C(C)NC1=NC=CC(=N1)C(C)=O.O=C(C(=O)OCC)C(=O)OCC>>C(C)NC1=NC=CC(=N1)C(CC(C(=O)OCC)(C(=O)OCC)O)=O
[CH3:1][CH2:2][NH:3][c:4]1[n:5][cH:6][cH:7][c:8]([C:9](=[O:10])[CH3:11])[n:24]1.[C:12](=[O:13])([C:14](=[O:15])[O:16][CH2:17][CH3:18])[C:19](=[O:20])[O:21][CH2:22][CH3:23]>>[CH3:1][CH2:2][NH:3][c:4]1[n:5][cH:6][cH:7][c:8]([C:9](=[O:10])[CH2:11][C:12]([OH:13])([C:14](=[O:15])[O:16][CH2:17][CH3:18])[C:19](=[O:20])[O:21][...
CCNc1nccc(C(C)=O)n1.CCOC(=O)C(=O)C(=O)OCC
CCNc1nccc(C(=O)CC(O)(C(=O)OCC)C(=O)OCC)n1
null
null
null
C-C Coupling
OtherReaction
e88a4a7d8d6b5dee5ec6739bba985b00a792654307585b505d721a6c4424a1e7
622d9e177646f51219fadf1ea3ee007cb7d9c42cff173da68f5fdf3c13916e74
c1cncnc1
[#7;a:1]:[c:2]-[C:3](-[CH3;D1;+0:4])=[O;D1;H0:5].[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[C:12](=[O;D1;H0:13])-[#8:14]-[C:15]>>[#7;a:1]:[c:2]-[C:3](=[O;D1;H0:5])-[CH2;D2;+0:4]-[C;H0;D4;+0:10](-[OH;D1;+0:11])(-[C:8](=[O;D1;H0:9])-[#8:7]-[C:6])-[C:12](=[O;D1;H0:13])-[#8:14]-[C:15]
null
[]
110
CELSIUS
null
null
A mixture consisting of 1.9 g of 1-(2-ethylaminopyrimidin-4-yl)ethanone and 1.86 ml of diethyl ketomalonate is heated at 110° C. for 18 hours. The mixture is purified by column chromatography (silica gel, mobile phase:methylene chloride:methanol=98:2). Conditions: See reaction.notes.procedure_details. Workup: The mixtu...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone
Ketone.Ester.Ester.Tertiary alcohol
null
null
c1cncnc1
null
null
110
null
CCNc1nccc(C(C)=O)n1.CCOC(=O)C(=O)C(=O)OCC>>CCNc1nccc(C(=O)CC(O)(C(=O)OCC)C(=O)OCC)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-d8366a1b2fef4b479476f79a57cde650
CCNc1nccc(C(=O)CC(O)(C(=O)OCC)C(=O)OCC)n1.NN>>CCNc1nccc(-c2cc(C(=O)OCC)c(=O)[nH]n2)n1
C(C)NC1=NC=CC(=N1)C(CC(C(=O)OCC)(C(=O)OCC)O)=O.Cl.NN>>C(C)NC1=NC=CC(=N1)C=1C=C(C(NN1)=O)C(=O)OCC
CCO[C:17]([C:11](O)([CH2:10][C:9](=O)[c:8]1[cH:7][cH:6][n:5][c:4]([NH:3][CH2:2][CH3:1])[n:21]1)[C:12](=[O:13])[O:14][CH2:15][CH3:16])=[O:18].[NH2:19][NH2:20]>>[CH3:1][CH2:2][NH:3][c:4]1[n:5][cH:6][cH:7][c:8](-[c:9]2[cH:10][c:11]([C:12](=[O:13])[O:14][CH2:15][CH3:16])[c:17](=[O:18])[nH:19][n:20]2)[n:21]1
CCNc1nccc(C(=O)CC(O)(C(=O)OCC)C(=O)OCC)n1.NN
CCNc1nccc(-c2cc(C(=O)OCC)c(=O)[nH]n2)n1
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
54634d418c8596de45ab35c5695b00785263669907ca8fff6518a837f0632bdf
aa93ed92552ed79af2c3e55f1caa04b7f5a7360562e21df7516ddca07861385e
O=c1ccc(-c2ccncn2)n[nH]1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D4;+0:3](-O)(-[CH2;D2;+0:4]-[C;H0;D3;+0:5](=O)-[c;H0;D3;+0:6]1:[#7;a:7]:[c:8](-[#7:9]):[#7;a:10]:[c:11]:[c:12]:1)-[C:13](=[O;D1;H0:14])-[#8:15]-[C:16].[NH2;D1;+0:17]-[NH2;D1;+0:18]>>[#7:9]-[c:8]1:[#7;a:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:5]2:[cH;D2;+0:4]:[c;H0;D3;+0:3](-[C:13](=[O;D1...
null
[]
130
CELSIUS
null
null
A mixture of 2 g of diethyl 2-[2-(2-ethylaminopyrimidin-4-yl)-2-oxo-ethyl]-2-hydroxy-malonate, 485 mg of hydrazine hydrochloride and 20 ml of ethanol is stirred under reflux for 24 hours. After cooling while stirring, the precipitate is filtered off with suction, heated in 4 ml of N-methylpyrrolidinone (NMP) at 130° C....
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Ketone.Ester.Ester.Tertiary alcohol
Ester
null
c1cnncc1
c1cncnc1.c1cnncc1
HO-
C(C)O
130
null
CCNc1nccc(C(=O)CC(O)(C(=O)OCC)C(=O)OCC)n1.NN>C(C)O>CCNc1nccc(-c2cc(C(=O)OCC)c(=O)[nH]n2)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-01b279a3c593478bb244d5db8ca3aad0
CCNc1nccc(-c2cc(C(=O)OCC)c(=O)[nH]n2)n1>>CCNc1nccc(-c2cc(C(=O)O)c(=O)[nH]n2)n1
C(C)NC1=NC=CC(=N1)C=1C=C(C(NN1)=O)C(=O)OCC.C1CCOC1.O.[OH-].[Li+]>>C(C)NC1=NC=CC(=N1)C=1C=C(C(NN1)=O)C(=O)O
CC[O:14][C:12]([c:11]1[cH:10][c:9](-[c:8]2[cH:7][cH:6][n:5][c:4]([NH:3][CH2:2][CH3:1])[n:19]2)[n:18][nH:17][c:15]1=[O:16])=[O:13]>>[CH3:1][CH2:2][NH:3][c:4]1[n:5][cH:6][cH:7][c:8](-[c:9]2[cH:10][c:11]([C:12](=[O:13])[OH:14])[c:15](=[O:16])[nH:17][n:18]2)[n:19]1
CCNc1nccc(-c2cc(C(=O)OCC)c(=O)[nH]n2)n1
CCNc1nccc(-c2cc(C(=O)O)c(=O)[nH]n2)n1
null
null
CO
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=c1ccc(-c2ccncn2)n[nH]1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
1
HOUR
A mixture of 400 mg of ethyl 6-(2-ethylaminopyrimidin-4-yl)-3-oxo-2,3-dihydro-pyridazine-4-carboxylate, 2 ml of THF, 2 ml of water, 2 ml of methanol and 100 mg of lithium hydroxide is stirred at room temperature for 1 hour, and the volatile constituents are removed in vacuo. A pH of 4 is adjusted by dropwise addition o...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cncnc1.c1cnncc1
Other
CO
null
1
CCNc1nccc(-c2cc(C(=O)OCC)c(=O)[nH]n2)n1>CO>CCNc1nccc(-c2cc(C(=O)O)c(=O)[nH]n2)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c6db62493a0541ae9904ac2a0c41fb10
CCNc1nccc(-c2cc(C(=O)O)c(=O)[nH]n2)n1.Nc1ccc(Cl)cc1N>>CCNc1nccc(-c2cc(C(=O)Nc3ccc(Cl)cc3N)c(=O)[nH]n2)n1
ClC1=CC(=C(C=C1)N)N.C(C)NC1=NC=CC(=N1)C=1C=C(C(NN1)=O)C(=O)O.CN(C)C=O.C(C)N(CC)CC>>NC1=C(C=CC(=C1)Cl)NC(=O)C=1C(NN=C(C1)C1=NC(=NC=C1)NCC)=O
O[C:12]([c:11]1[cH:10][c:9](-[c:8]2[cH:7][cH:6][n:5][c:4]([NH:3][CH2:2][CH3:1])[n:27]2)[n:26][nH:25][c:23]1=[O:24])=[O:13].[NH2:14][c:15]1[cH:16][cH:17][c:18]([Cl:19])[cH:20][c:21]1[NH2:22]>>[CH3:1][CH2:2][NH:3][c:4]1[n:5][cH:6][cH:7][c:8](-[c:9]2[cH:10][c:11]([C:12](=[O:13])[NH:14][c:15]3[cH:16][cH:17][c:18]([Cl:19])[...
CCNc1nccc(-c2cc(C(=O)O)c(=O)[nH]n2)n1.Nc1ccc(Cl)cc1N
CCNc1nccc(-c2cc(C(=O)Nc3ccc(Cl)cc3N)c(=O)[nH]n2)n1
null
null
O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccc1)c1cc(-c2ccncn2)n[nH]c1=O
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1=[O;D1;H0:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1=[O;D1;H0:9]
null
[]
null
null
30
MINUTE
A solution of 110 mg of 6-(2-ethylaminopyrimidin-4-yl)-3-oxo-2,3-dihydropyridazine-4-carboxylic acid, 2 ml of DMF and 0.17 ml of triethylamine is mixed with 192 mg of Hatu and stirred at room temperature for 30 minutes. Then 66 mg of 4-chloro-phenylenediamine are added, and the mixture is stirred at room temperature ov...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1cncnc1.c1cnncc1.c1ccccc1
HO-
O
null
0.5
CCNc1nccc(-c2cc(C(=O)O)c(=O)[nH]n2)n1.Nc1ccc(Cl)cc1N>O>CCNc1nccc(-c2cc(C(=O)Nc3ccc(Cl)cc3N)c(=O)[nH]n2)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-72c1b37601314bc3b8dc57e3b5fa4dc1
CCNc1nccc(-c2cc(C(=O)Nc3ccc(Cl)cc3N)c(=O)[nH]n2)n1>>CCNc1nccc(-c2cc(-c3nc4cc(Cl)ccc4[nH]3)c(=O)[nH]n2)n1
NC1=C(C=CC(=C1)Cl)NC(=O)C=1C(NN=C(C1)C1=NC(=NC=C1)NCC)=O>>ClC1=CC2=C(NC(=N2)C=2C(NN=C(C2)C2=NC(=NC=C2)NCC)=O)C=C1
O=[C:12]([c:11]1[cH:10][c:9](-[c:8]2[cH:7][cH:6][n:5][c:4]([NH:3][CH2:2][CH3:1])[n:26]2)[n:25][nH:24][c:22]1=[O:23])[NH:21][c:20]1[c:14]([NH2:13])[cH:15][c:16]([Cl:17])[cH:18][cH:19]1>>[CH3:1][CH2:2][NH:3][c:4]1[n:5][cH:6][cH:7][c:8](-[c:9]2[cH:10][c:11](-[c:12]3[n:13][c:14]4[cH:15][c:16]([Cl:17])[cH:18][cH:19][c:20]4[...
CCNc1nccc(-c2cc(C(=O)Nc3ccc(Cl)cc3N)c(=O)[nH]n2)n1
CCNc1nccc(-c2cc(-c3nc4cc(Cl)ccc4[nH]3)c(=O)[nH]n2)n1
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
76e10ab81a93773d04ca0e55f8fb55bcd635323b5b4a9b9acd135658778da8ae
a079090652d9d6c0e17c70eeab94f6d7afea064f52cf5fa9036d5feedd14143a
O=c1[nH]nc(-c2ccncn2)cc1-c1nc2ccccc2[nH]1
O=[C;H0;D3;+0:1](-[NH;D2;+0:2]-[c:3](:[c:4]):[c:5](-[NH2;D1;+0:6]):[c:7])-[c;H0;D3;+0:8]1:[c:9]:[c:10](-[c:11]:[#7;a:12]):[#7;a:13]:[#7;a:14]:[c:15]:1=[O;D1;H0:16]>>[#7;a:12]:[c:11]-[c:10]1:[#7;a:13]:[#7;a:14]:[c:15](=[O;D1;H0:16]):[c;H0;D3;+0:8](-[c;H0;D3;+0:1]2:[n;H0;D2;+0:6]:[c:5](:[c:7]):[c:3](:[c:4]):[nH;D2;+0:2]:...
null
[]
null
null
null
null
6-(2-Ethylaminopyrimidin-4-yl)-3-oxo-2,3-dihydropyridazine-4-carboxylic acid (2-amino-4-chlorophenyl)amide (50 mg) are stirred in 1 ml of glacial acetic acid at 100° C. for 3 hours. After cooling, the precipitate is filtered off with suction, stirred with aqueous sodium bicarbonate solution and again filtered off with ...
10.6084/m9.figshare.5104873.v1
null
Secondary amide.Primary amine
null
c1ccccc1
c1ccc2[nH]cnc2c1
c1cncnc1.c1cnncc1.c1ccc2[nH]cnc2c1
HO-
C(C)(=O)O
null
null
CCNc1nccc(-c2cc(C(=O)Nc3ccc(Cl)cc3N)c(=O)[nH]n2)n1>C(C)(=O)O>CCNc1nccc(-c2cc(-c3nc4cc(Cl)ccc4[nH]3)c(=O)[nH]n2)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-669cdacc1e58420e9b6082d0b7ac8879
Nc1ccc(Cl)cc1NC(=O)c1cc(Cl)n[nH]c1=O>>O=c1[nH]nc(Cl)cc1-c1nc2ccc(Cl)cc2[nH]1
NC1=C(C=C(C=C1)Cl)NC(=O)C=1C(NN=C(C1)Cl)=O.NC1=C(C=CC(=C1)Cl)NC(=O)C=1C(NN=C(C1)Cl)=O>>ClC=1C=C(C(NN1)=O)C1=NC2=C(N1)C=C(C=C2)Cl
O=[C:9]([c:8]1[c:2](=[O:1])[nH:3][n:4][c:5]([Cl:6])[cH:7]1)[NH:10][c:11]1[cH:12][c:13]([Cl:15])[cH:14][cH:16][c:17]1[NH2:18]>>[O:1]=[c:2]1[nH:3][n:4][c:5]([Cl:6])[cH:7][c:8]1-[c:9]1[n:10][c:11]2[cH:12][cH:13][c:14]([Cl:15])[cH:16][c:17]2[nH:18]1
Nc1ccc(Cl)cc1NC(=O)c1cc(Cl)n[nH]c1=O
O=c1[nH]nc(Cl)cc1-c1nc2ccc(Cl)cc2[nH]1
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
b8a14eed92d407c7877eafdd1aae168755826fc260dd09432d2786866f0a8b75
13a243a4a3d01197eb229b4226a0ab42e57cf7cc6968477100676d27a1f5f0f3
O=c1[nH]nccc1-c1nc2ccccc2[nH]1
O=[C;H0;D3;+0:1](-[NH;D2;+0:2]-[c:3]1:[c:4]:[c;H0;D3;+0:5](-[Cl;H0;D1;+0:6]):[cH;D2;+0:7]:[c:8]:[c:9]:1-[NH2;D1;+0:10])-[c;H0;D3;+0:11]1:[c:12]:[c:13](-[Cl;D1;H0:14]):[#7;a:15]:[#7;a:16]:[c:17]:1=[O;D1;H0:18]>>[Cl;D1;H0:14]-[c:13]1:[#7;a:15]:[#7;a:16]:[c:17](=[O;D1;H0:18]):[c;H0;D3;+0:11](-[c;H0;D3;+0:1]2:[n;H0;D2;+0:2...
null
[]
120
CELSIUS
null
null
A mixture of 6-chloro-3-oxo-2,3-dihydropyridazine-4-carboxylic acid (2-amino-5-chlorophenyl)amide and 6-chloro-3-oxo-2,3-dihydropyridazine-4-carboxylic acid (2-amino-4-chlorophenyl)amide (1.0 g; 1.67 mmol) is dissolved in 100 ml of glacial acetic acid and heated at 120° C. for 90 min. A precipitate separates out on coo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amide.Primary amine
Aromatic halide
c1ccccc1
c1ccc2[nH]cnc2c1
c1cnncc1.c1ccc2[nH]cnc2c1
HO-
C(C)(=O)O
120
null
Nc1ccc(Cl)cc1NC(=O)c1cc(Cl)n[nH]c1=O>C(C)(=O)O>O=c1[nH]nc(Cl)cc1-c1nc2ccc(Cl)cc2[nH]1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2239869004564afb8a547ed16cac6743
C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(Cl)cc3n2COCC[Si](C)(C)C)c1=O.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O>>Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(C)c1O
CC1=C(C(=CC(=C1)B1OC(C(O1)(C)C)(C)C)C)O.C([O-])([O-])=O.[Na+].[Na+].ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)Cl>>ClC=1C=CC2=C(N(C(=N2)C=2C(N(N=C(C2)C2=CC(=C(C(=C2)C)O)C)COCC[Si](C)(C)C)=O)COCC[Si](C)(C)C)C1
Cl[c:5]1[cH:6][c:7](-[c:8]2[n:9][c:10]3[cH:11][cH:12][c:13]([Cl:14])[cH:15][c:16]3[n:17]2[CH2:18][O:19][CH2:20][CH2:21][Si:22]([CH3:23])([CH3:24])[CH3:25])[c:26](=[O:27])[n:28]([CH2:29][O:30][CH2:31][CH2:32][Si:33]([CH3:34])([CH3:35])[CH3:36])[n:37]1.CC1(C)OB([c:4]2[cH:3][c:2]([CH3:1])[c:41]([OH:42])[c:39]([CH3:40])[cH...
C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(Cl)cc3n2COCC[Si](C)(C)C)c1=O.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O
Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(C)c1O
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
COCCOC
C-C Coupling
Suzuki coupling with boronic esters
7d3abbda54e933df9ff9dc39c70f4c4ada1c268870f29590395c2cc6bed1dda1
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
O=c1[nH]nc(-c2ccccc2)cc1-c1nc2ccccc2[nH]1
C-C1(-C)-O-B(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-O-C-1(-C)-C.Cl-[c;H0;D3;+0:6]1:[#7;a:7]:[#7;a:8](-[C:9]):[c:10]:[c:11]:[c:12]:1>>[C:9]-[#7;a:8]1:[#7;a:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:12]:[c:11]:[c:10]:1
null
[]
95
CELSIUS
null
null
6-Chloro-4-[6-chloro-1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2-(2-trimethylsilanylethoxymethyl)-2H-pyridazin-3-one (100 mg; 0.185 mmol) and tetrakis(triphenylphosphine) palladium(0) (0.15 equivalents) are dissolved in DME, and argon is passed in for 10 min. 2,6-Dimethyl-4-(4,4,5,5-tetramethyl-1,3,2-dio...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1ccnnc1.B1OCCO1.c1ccccc1
c1ccccc1.c1ccnnc1
c1ccccc1.c1ccnnc1.c1ccc2[nH]cnc2c1
HCl.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.COCCOC
95
null
C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(Cl)cc3n2COCC[Si](C)(C)C)c1=O.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.COCCOC>Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4n3COCC[Si](C)(C)C)c(=O)n...
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-515db933f0c14a0293ea111721cec9cc
Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(C)c1O>>Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4[nH]3)c(=O)[nH]n2)cc(C)c1O
Cl.FC(C(=O)O)(F)F.ClC=1C=CC2=C(N(C(=N2)C=2C(N(N=C(C2)C2=CC(=C(C(=C2)C)O)C)COCC[Si](C)(C)C)=O)COCC[Si](C)(C)C)C1.[OH-].[Na+]>>ClC=1C=CC2=C(NC(=N2)C=2C(NN=C(C2)C2=CC(=C(C(=C2)C)O)C)=O)C1
C[Si](C)(C)CCOC[n:17]1[c:8](-[c:7]2[cH:6][c:5](-[c:4]3[cH:3][c:2]([CH3:1])[c:25]([OH:26])[c:23]([CH3:24])[cH:22]3)[n:21][n:20](COCC[Si](C)(C)C)[c:18]2=[O:19])[n:9][c:10]2[cH:11][cH:12][c:13]([Cl:14])[cH:15][c:16]21>>[CH3:1][c:2]1[cH:3][c:4](-[c:5]2[cH:6][c:7](-[c:8]3[n:9][c:10]4[cH:11][cH:12][c:13]([Cl:14])[cH:15][c:16...
Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(C)c1O
Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4[nH]3)c(=O)[nH]n2)cc(C)c1O
null
null
ClCCl.CO.O
Reduction
OtherReaction
c1f0b959e3270c73ea431d54a86cf99be394391b1aeed84bffc9169fd737a4fd
4c2ed0f567254ea4c771872583c9a3c5a0aabe43ba2b8e508678a1ced83aca48
O=c1[nH]nc(-c2ccccc2)cc1-c1nc2ccccc2[nH]1
C-[Si](-C)(-C)-C-C-O-C-[n;H0;D3;+0:1]1:[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]:1-[c:8]:[c:9](=[O;D1;H0:10]):[n;H0;D3;+0:11](-C-O-C-C-[Si](-C)(-C)-C):[#7;a:12]:[c:13]>>[O;D1;H0:10]=[c:9](:[c:8]-[c:7]1:[#7;a:6]:[c:4](:[c:5]):[c:2](:[c:3]):[nH;D2;+0:1]:1):[nH;D2;+0:11]:[#7;a:12]:[c:13]
null
[]
null
null
30
MINUTE
4-[6-Chloro-1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-6-(4-hydroxy-3,5-dimethylphenyl)-2-(2-trimethylsilanylethoxymethyl)-2H-pyridazin-3-one is stirred in dichloromethane:trifluoroacetic acid/1:1 at RT for 30 min. The solvent is stripped off in vacuo, and the residue is dissolved in methanol, and 2M sodi...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Silyl protective group.Silyl protective group
null
c1ccnnc1.c1ccc2nc[nH]c2c1
c1cnncc1.c1ccc2[nH]cnc2c1
c1ccccc1.c1cnncc1.c1ccc2[nH]cnc2c1
HO-
ClCCl.CO.O
null
0.5
Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(C)c1O>ClCCl.CO.O>Cc1cc(-c2cc(-c3nc4ccc(Cl)cc4[nH]3)c(=O)[nH]n2)cc(C)c1O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-bb9f641574f3407fbcc52c5df3b9224e
CC1(C)OB(B2OC(C)(C)C(C)(C)O2)OC1(C)C.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O>>C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O
ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)C(F)(F)F.B1(OC(C(O1)(C)C)(C)C)B2OC(C(O2)(C)C)(C)C.C(C)(=O)[O-].[K+]>>O=C1C(=CC(=NN1COCC[Si](C)(C)C)B(O)O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)C(F)(F)F
CC1(C)OB([B:12]2[O:13]C(C)(C)C(C)(C)[O:14]2)OC1(C)C.Cl[c:11]1[n:10][n:9]([CH2:8][O:7][CH2:6][CH2:5][Si:2]([CH3:1])([CH3:3])[CH3:4])[c:38](=[O:39])[c:16](-[c:17]2[n:18][c:19]3[cH:20][cH:21][c:22]([C:23]([F:24])([F:25])[F:26])[cH:27][c:28]3[n:29]2[CH2:30][O:31][CH2:32][CH2:33][Si:34]([CH3:35])([CH3:36])[CH3:37])[cH:15]1>...
CC1(C)OB(B2OC(C)(C)C(C)(C)O2)OC1(C)C.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O
null
null
CS(=O)C
Miscellaneous
OtherReaction
0f862682a552a117cbdb4251701683c41ea8d7c93834f0609621794a8532f1bb
dafd25fbe01879c365f8c874026e570f49824f4bb82016b29d0c5d21aeb58ca3
O=c1[nH]nccc1-c1nc2ccccc2[nH]1
C-C1(-C)-O-B(-[B;H0;D3;+0:1]2-[O;H0;D2;+0:2]-C(-C)(-C)-C(-C)(-C)-[O;H0;D2;+0:3]-2)-O-C-1(-C)-C.Cl-[c;H0;D3;+0:4]1:[#7;a:5]:[#7;a:6](-[C:7]):[c:8]:[c:9]:[c:10]:1>>[C:7]-[#7;a:6]1:[#7;a:5]:[c;H0;D3;+0:4](-[B;H0;D3;+0:1](-[OH;D1;+0:2])-[OH;D1;+0:3]):[c:10]:[c:9]:[c:8]:1
null
[]
95
CELSIUS
null
null
6-Chloro-4-[6-trifluormethyl-1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2-(2-trimethylsilanylethoxymethyl)-2H-pyridazin-3-one (prepared in analogy to example 15b), bis(pinacolato)diboron, (1,1′-bis(diphenylphosphine)ferrocene)-palladium(II) chloride-dichloromethane complex and potassium acetate are dissol...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Boronic acid
B1OCCO1.[B]1OCCO1.c1ccnnc1
c1ccnnc1
c1ccnnc1.c1ccc2[nH]cnc2c1
HCl.B
CS(=O)C
95
null
CC1(C)OB(B2OC(C)(C)C(C)(C)O2)OC1(C)C.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O>CS(=O)C>C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-de6193c7d6a84e4199662d280a686708
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O.Clc1ccnc(Cl)n1>>C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O
O=C1C(=CC(=NN1COCC[Si](C)(C)C)B(O)O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)C(F)(F)F.ClC1=NC=CC(=N1)Cl.[F-].[K+]>>ClC1=NC=CC(=N1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)C(F)(F)F
OB(O)[c:11]1[n:10][n:9]([CH2:8][O:7][CH2:6][CH2:5][Si:2]([CH3:1])([CH3:3])[CH3:4])[c:42](=[O:43])[c:20](-[c:21]2[n:22][c:23]3[cH:24][cH:25][c:26]([C:27]([F:28])([F:29])[F:30])[cH:31][c:32]3[n:33]2[CH2:34][O:35][CH2:36][CH2:37][Si:38]([CH3:39])([CH3:40])[CH3:41])[cH:19]1.Cl[c:12]1[cH:13][cH:14][n:15][c:16]([Cl:17])[n:18...
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O.Clc1ccnc(Cl)n1
C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd]
C1CCOC1
C-C Coupling
Suzuki coupling with boronic acids
f8f5c061fa0766cf8bf2b56a909373cb6775dd68fbe7d26541aa38df8e9d5b4c
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=c1[nH]nc(-c2ccncn2)cc1-c1nc2ccccc2[nH]1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[Cl;D1;H0:4]):[#7;a:5]:[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8]1:[#7;a:9]:[#7;a:10](-[C:11]):[c:12]:[c:13]:[c:14]:1>>[C:11]-[#7;a:10]1:[#7;a:9]:[c;H0;D3;+0:8](-[c;H0;D3;+0:1]2:[#7;a:2]:[c:3](-[Cl;D1;H0:4]):[#7;a:5]:[c:6]:[c:7]:2):[c:14]:[c:13]:[c:12]:1
null
[]
null
null
16
HOUR
6-Oxo-5-[6-tri-fluoromethyl-1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-1-(2-trimethylsilanylethoxymethyl)-1,6-dihydropyridazine-3-boronic acid, 2,4-di-chloropyrimidine, potassium fluoride and tris(dibenzylideneacetone)dipalladium(0) are dissolved in dry THF and degassed with argon for 10 minutes. Tri-tert...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccnnc1.c1cncnc1
c1ccnnc1.c1cncnc1
c1ccnnc1.c1cncnc1.c1ccc2[nH]cnc2c1
HCl.B
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C1CCOC1
null
16
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O.Clc1ccnc(Cl)n1>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C1CCOC1>C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccc(C(F)(F)F)cc3n2COCC[Si](C)(C)C)c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-54dfd9217eb84573b049cba999822dc4
COc1ccc(Cl)nn1>>COc1nnc(Cl)cc1C=O
C(CCC)[Li].CC1(NC(CCC1)(C)C)C.ClC=1N=NC(=CC1)OC.Cl.C(=O)(O)[O-].[Na+]>>ClC1=CC(=C(N=N1)OC)C=O
[CH3:1][O:2][c:3]1[n:4][n:5][c:6]([Cl:7])[cH:8][cH:9]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6]([Cl:7])[cH:8][c:9]1[CH:10]=[O:11]
COc1ccc(Cl)nn1
COc1nnc(Cl)cc1C=O
null
null
C1CCOC1.CN(C)C=O.C(C)O
Miscellaneous
OtherReaction
be7ff8b1310c070d854f9ef41f58f5c15ed6d3196fad23a27fa694b91ad9ce8f
3cccf922e74135722ee21a46ad7578302a8603e1f71d6f2113cd42de4ba0cf73
c1ccnnc1
[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](-[Cl;D1;H0:6]):[c:7]:[cH;D2;+0:8]:1>>[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](-[Cl;D1;H0:6]):[c:7]:[c;H0;D3;+0:8]:1-[C:9]=[O;D1;H0:10]
null
[]
0
CELSIUS
30
MINUTE
n-Butyllithium is added dropwise at −75° C. to a solution of 2,2,6,6-tetramethyl-piperidine in THF. The solution is stirred at 0° C. for 30 minutes. After cooling to −75° C., a solution, precooled to −75° C., of 3-chloro-6-methoxypyridazine in THF is added dropwise. The reaction is stirred at −75° C. for 30 minutes. Su...
10.6084/m9.figshare.5104873.v1
null
null
Aldehyde
c1ccnnc1
c1ccnnc1
c1ccnnc1
Other
C1CCOC1.CN(C)C=O.C(C)O
0
0.5
COc1ccc(Cl)nn1>C1CCOC1.CN(C)C=O.C(C)O>COc1nnc(Cl)cc1C=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e986e39eba024f0d9b164fdcba6d54bc
COc1nnc(Cl)cc1C=O.Cc1cccc(N)c1N>>COc1nnc(Cl)cc1-c1nc2cccc(C)c2[nH]1
ClC1=CC(=C(N=N1)OC)C=O.NC1=C(C=CC=C1N)C>>ClC1=CC(=C(N=N1)OC)C1=NC2=C(N1)C(=CC=C2)C
O=[CH:10][c:9]1[c:3]([O:2][CH3:1])[n:4][n:5][c:6]([Cl:7])[cH:8]1.[NH2:11][c:12]1[cH:13][cH:14][cH:15][c:16]([CH3:17])[c:18]1[NH2:19]>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6]([Cl:7])[cH:8][c:9]1-[c:10]1[n:11][c:12]2[cH:13][cH:14][cH:15][c:16]([CH3:17])[c:18]2[nH:19]1
COc1nnc(Cl)cc1C=O.Cc1cccc(N)c1N
COc1nnc(Cl)cc1-c1nc2cccc(C)c2[nH]1
null
null
CN(C)C=O
Aromatic Heterocycle Formation
Benzimidazole aldehyde
357211f0cea48f6066cc617c063d8f639b186739754abf69a9bef955d42b7d06
947e8e758a50553bad3d8f39fd1540e5051c4c73055f7a5a9da00894523e8ba0
c1ccc2[nH]c(-c3ccnnc3)nc2c1
O=[CH;D2;+0:1]-[c;H0;D3;+0:2]1:[c:3]:[c:4](-[Cl;D1;H0:5]):[#7;a:6]:[#7;a:7]:[c:8]:1-[#8:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13](-[NH2;D1;+0:14]):[c:15]>>[#8:9]-[c:8]1:[#7;a:7]:[#7;a:6]:[c:4](-[Cl;D1;H0:5]):[c:3]:[c;H0;D3;+0:2]:1-[c;H0;D3;+0:1]1:[n;H0;D2;+0:10]:[c:11](:[c:12]):[c:13](:[c:15]):[nH;D2;+0:14]:1
null
[]
120
CELSIUS
null
null
6-Chloro-3-methoxypyridazine-4-carbaldehyde is dissolved in DMF, und 2,3-diaminotoluene is added. The reaction solution is heated at 120° C. in a microwave for 30 minutes. The crude product is purified on silica gel (eluent ethyl acetate in heptane). MS (ES+) m/z 275 (M+H). Conditions: See reaction.notes.procedure_deta...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine.Primary amine
null
c1ccccc1
c1ccc2[nH]cnc2c1
c1ccnnc1.c1ccc2[nH]cnc2c1
HO-
CN(C)C=O
120
null
COc1nnc(Cl)cc1C=O.Cc1cccc(N)c1N>CN(C)C=O>COc1nnc(Cl)cc1-c1nc2cccc(C)c2[nH]1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2bb6dd6c1f964b519f78e8c155863158
COC(=O)c1ccc2nc(-c3cc(Cl)nn(COCC[Si](C)(C)C)c3=O)n(COCC[Si](C)(C)C)c2c1>>C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C=O)cc3n2COCC[Si](C)(C)C)c1=O
ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)C(=O)OC>>ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)C=O
CO[C:21]([c:20]1[cH:19][cH:18][c:17]2[n:16][c:15](-[c:14]3[cH:13][c:11]([Cl:12])[n:10][n:9]([CH2:8][O:7][CH2:6][CH2:5][Si:2]([CH3:1])([CH3:3])[CH3:4])[c:34]3=[O:35])[n:25]([CH2:26][O:27][CH2:28][CH2:29][Si:30]([CH3:31])([CH3:32])[CH3:33])[c:24]2[cH:23]1)=[O:22]>>[CH3:1][Si:2]([CH3:3])([CH3:4])[CH2:5][CH2:6][O:7][CH2:8]...
COC(=O)c1ccc2nc(-c3cc(Cl)nn(COCC[Si](C)(C)C)c3=O)n(COCC[Si](C)(C)C)c2c1
C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C=O)cc3n2COCC[Si](C)(C)C)c1=O
null
[O-2].[Mn+2].[O-2].[Mn+4].[O-2]
ClCCl.C1(=CC=CC=C1)C
Reduction
OtherReaction
ec1c6c64dd9be73981e5a6c952ab740869d298b20e87e097e88e1179cc5bc6dc
33ddc7b9457742ba0a376f08a972e4f33779267f6f1fe15e3be786427ae9f4ec
O=c1[nH]nccc1-c1nc2ccccc2[nH]1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[c:6]:[#7;a:7]>>[#7;a:7]:[c:6]:[c:5]:[c:3](-[CH;D2;+0:1]=[O;D1;H0:2]):[c:4]
null
[]
0
CELSIUS
1
HOUR
6-Chloro-4-(6-methoxycarbonyl-1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2-(2-trimethylsilanylethoxymethyl)-2H-pyridazin-3-one (3.0 g, 5.3 mmol) is dissolved in dichloromethane, and the solution is cooled to 0° C. 15% DIBA1H in toluene is added dropwise, and the reaction mixture is stirred at room tempera...
10.6084/m9.figshare.5104873.v1
null
Ester
Aldehyde
null
null
c1ccnnc1.c1ccc2[nH]cnc2c1
HO-
[O-2].[Mn+2].[O-2].[Mn+4].[O-2].ClCCl.C1(=CC=CC=C1)C
0
1
COC(=O)c1ccc2nc(-c3cc(Cl)nn(COCC[Si](C)(C)C)c3=O)n(COCC[Si](C)(C)C)c2c1>[O-2].[Mn+2].[O-2].[Mn+4].[O-2].ClCCl.C1(=CC=CC=C1)C>C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C=O)cc3n2COCC[Si](C)(C)C)c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-e36806988f24499e97201003b5c7807a
CN1CCNCC1.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C=O)cc3n2COCC[Si](C)(C)C)c1=O>>CN1CCN(Cc2ccc3nc(-c4cc(Cl)nn(COCC[Si](C)(C)C)c4=O)n(COCC[Si](C)(C)C)c3c2)CC1
C(=O)(O)[O-].[Na+].ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)C=O.CN1CCNCC1.C(=O)=O.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+]>>ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=C(C=C2)CN2CCN(CC2)C
[CH3:1][N:2]1[CH2:3][CH2:4][NH:5][CH2:40][CH2:41]1.O=[CH:6][c:7]1[cH:8][cH:9][c:10]2[n:11][c:12](-[c:13]3[cH:14][c:15]([Cl:16])[n:17][n:18]([CH2:19][O:20][CH2:21][CH2:22][Si:23]([CH3:24])([CH3:25])[CH3:26])[c:27]3=[O:28])[n:29]([CH2:30][O:31][CH2:32][CH2:33][Si:34]([CH3:35])([CH3:36])[CH3:37])[c:38]2[cH:39]1>>[CH3:1][N...
CN1CCNCC1.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C=O)cc3n2COCC[Si](C)(C)C)c1=O
CN1CCN(Cc2ccc3nc(-c4cc(Cl)nn(COCC[Si](C)(C)C)c4=O)n(COCC[Si](C)(C)C)c3c2)CC1
null
null
ClCCl.C(C)(=O)O
Heteroatom Alkylation and Arylation
reductive amination
66e6667395903ee1c54d8aecc784ece1bccbdcbc9661ebcae0e6a980f9380640
2d03f38884b1fbb0c0d6e6f2de31afb25102fec87f347c3a123e064c1bfef0ad
O=c1[nH]nccc1-c1nc2ccc(CN3CCNCC3)cc2[nH]1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6].[#7:7]1-[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]-1>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[CH2;D2;+0:1]-[N;H0;D3;+0:10]1-[C:11]-[C:12]-[#7:7]-[C:8]-[C:9]-1):[c:3]
null
[]
null
null
15
MINUTE
6-Chloro-4-(6-formyl-1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2-(2-trimethylsilanylethoxymethyl)-2H-pyridazin-3-one is dissolved in dichloro-methane. 4-Methylpiperazine and acetic acid are added. After 15 minutes, sodium triacetoxyborohydride is added in several portions over the course of 3 hours. Afte...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary amine
Tertiary amine
C1C[NH]CCN1
C1C[NH]CC[NH]1
C1C[NH]CC[NH]1.c1ccc2[nH]cnc2c1.c1ccnnc1
Other
ClCCl.C(C)(=O)O
null
0.25
CN1CCNCC1.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccc(C=O)cc3n2COCC[Si](C)(C)C)c1=O>ClCCl.C(C)(=O)O>CN1CCN(Cc2ccc3nc(-c4cc(Cl)nn(COCC[Si](C)(C)C)c4=O)n(COCC[Si](C)(C)C)c3c2)CC1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-9feb74f319eb4940b9784589c395aa8d
Nc1ccccc1N.O=C(O)c1cc(Cl)n[nH]c1=O>>Nc1ccccc1NC(=O)c1cc(Cl)n[nH]c1=O
ClC=1C=C(C(NN1)=O)C(=O)O.C1(=C(C=CC=C1)N)N.Cl.C(C)N=C=NCCCN(C)C>>NC1=C(C=CC=C1)NC(=O)C=1C(NN=C(C1)Cl)=O
[NH2:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[NH2:8].O[C:9](=[O:10])[c:11]1[cH:12][c:13]([Cl:14])[n:15][nH:16][c:17]1=[O:18]>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[NH:8][C:9](=[O:10])[c:11]1[cH:12][c:13]([Cl:14])[n:15][nH:16][c:17]1=[O:18]
Nc1ccccc1N.O=C(O)c1cc(Cl)n[nH]c1=O
Nc1ccccc1NC(=O)c1cc(Cl)n[nH]c1=O
null
CN(C)C=1C=CN=CC1
CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccc1)c1ccn[nH]c1=O
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1=[O;D1;H0:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1=[O;D1;H0:9]
null
[]
null
null
4
HOUR
30.5 g of 6-chloro-3-oxo-2,3-dihydropyridazine-4-carboxylic acid, 18 g of ortho-phenylenediamine and 2 g of DMAP are dissolved in 800 ml of DMF, at room temperature 32.2 g of 1-ethyl-3-(3-dimethylaminopropyl)carbodiimide hydrochloride are added, and the resulting solution is stirred at room temperature for 4 hours. For...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1cnncc1
HO-
CN(C)C=1C=CN=CC1.CN(C)C=O
null
4
Nc1ccccc1N.O=C(O)c1cc(Cl)n[nH]c1=O>CN(C)C=1C=CN=CC1.CN(C)C=O>Nc1ccccc1NC(=O)c1cc(Cl)n[nH]c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-0a5a35357a4242119c12cf0fec91f87f
Nc1ccccc1NC(=O)c1cc(Cl)n[nH]c1=O>>O=c1[nH]nc(Cl)cc1-c1nc2ccccc2[nH]1
NC1=C(C=CC=C1)NC(=O)C=1C(NN=C(C1)Cl)=O>>N1C(=NC2=C1C=CC=C2)C=2C(NN=C(C2)Cl)=O
O=[C:9]([c:8]1[c:2](=[O:1])[nH:3][n:4][c:5]([Cl:6])[cH:7]1)[NH:17][c:16]1[c:11]([NH2:10])[cH:12][cH:13][cH:14][cH:15]1>>[O:1]=[c:2]1[nH:3][n:4][c:5]([Cl:6])[cH:7][c:8]1-[c:9]1[n:10][c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]2[nH:17]1
Nc1ccccc1NC(=O)c1cc(Cl)n[nH]c1=O
O=c1[nH]nc(Cl)cc1-c1nc2ccccc2[nH]1
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
76e10ab81a93773d04ca0e55f8fb55bcd635323b5b4a9b9acd135658778da8ae
a079090652d9d6c0e17c70eeab94f6d7afea064f52cf5fa9036d5feedd14143a
O=c1[nH]nccc1-c1nc2ccccc2[nH]1
O=[C;H0;D3;+0:1](-[NH;D2;+0:2]-[c:3](:[c:4]):[c:5](-[NH2;D1;+0:6]):[c:7])-[c;H0;D3;+0:8]1:[c:9]:[c:10](-[Cl;D1;H0:11]):[#7;a:12]:[#7;a:13]:[c:14]:1=[O;D1;H0:15]>>[Cl;D1;H0:11]-[c:10]1:[#7;a:12]:[#7;a:13]:[c:14](=[O;D1;H0:15]):[c;H0;D3;+0:8](-[c;H0;D3;+0:1]2:[n;H0;D2;+0:6]:[c:5](:[c:7]):[c:3](:[c:4]):[nH;D2;+0:2]:2):[c:...
null
[]
null
null
null
null
A solution of 26.4 g of 6-chloro-3-oxo-2,3-dihydropyridazine-4-carboxylic acid (2-aminophenyl)amide in 500 ml of acetic acid is stirred at 110° C. for 2.5 hours and then the solvent is distilled off. The crude product obtained in this way is employed without further purification. Conditions: See reaction.notes.procedur...
10.6084/m9.figshare.5104873.v1
null
Secondary amide.Primary amine
null
c1ccccc1
c1ccc2[nH]cnc2c1
c1cnncc1.c1ccc2[nH]cnc2c1
HO-
C(C)(=O)O
null
null
Nc1ccccc1NC(=O)c1cc(Cl)n[nH]c1=O>C(C)(=O)O>O=c1[nH]nc(Cl)cc1-c1nc2ccccc2[nH]1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-89db74143efc4aeca5ac7a1cab291567
C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.OB(O)c1ccsc1>>C[Si](C)(C)CCOCn1nc(-c2ccsc2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2.S1C=C(C=C1)B(O)O.C([O-])([O-])=O.[K+].[K+].O>>S1C=C(C=C1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2
Cl[c:11]1[n:10][n:9]([CH2:8][O:7][CH2:6][CH2:5][Si:2]([CH3:1])([CH3:3])[CH3:4])[c:36](=[O:37])[c:18](-[c:19]2[n:20][c:21]3[cH:22][cH:23][cH:24][cH:25][c:26]3[n:27]2[CH2:28][O:29][CH2:30][CH2:31][Si:32]([CH3:33])([CH3:34])[CH3:35])[cH:17]1.OB(O)[c:12]1[cH:13][cH:14][s:15][cH:16]1>>[CH3:1][Si:2]([CH3:3])([CH3:4])[CH2:5][...
C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.OB(O)c1ccsc1
C[Si](C)(C)CCOCn1nc(-c2ccsc2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
null
null
C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
8a8f836bc650bf77052c587b6c83ef7234124a1e9a8c8578cf10835ba68ae5f7
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=c1[nH]nc(-c2ccsc2)cc1-c1nc2ccccc2[nH]1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[#7;a:3](-[C:4]):[c:5]:[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8]1:[c:9]:[c:10]:[#16;a:11]:[c:12]:1>>[C:4]-[#7;a:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8]2:[c:9]:[c:10]:[#16;a:11]:[c:12]:2):[c:7]:[c:6]:[c:5]:1
null
[]
85
CELSIUS
4
HOUR
44 mg of 6-chloro-2-(2-trimethylsilanylethoxymethyl)-4-[1-(2-trimethylsilanyl-ethoxymethyl)-1H-benzimidazol-2-yl]-2H-pyridazin-3-one, 14 mg of thiophene-3-boronic acid and 36 mg of potassium carbonate are dissolved 1.5 ml of a 1:2 mixture of water and dimethoxyethane, and argon is passed through the solution for degass...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccnnc1.c1ccsc1
c1ccnnc1.c1ccsc1
c1ccnnc1.c1ccsc1.c1nc2ccccc2[nH]1
HCl.B
C(OC)COC
85
4
C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.OB(O)c1ccsc1>C(OC)COC>C[Si](C)(C)CCOCn1nc(-c2ccsc2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-a0bb0e36af1c4605afc2d9a01c94eb29
C[Si](C)(C)CCOCn1nc(-c2ccsc2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>>O=c1[nH]nc(-c2ccsc2)cc1-c1nc2ccccc2[nH]1
S1C=C(C=C1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2>>N1C(=NC2=C1C=CC=C2)C=2C(NN=C(C2)C2=CSC=C2)=O
C[Si](C)(C)CCOC[n:3]1[c:2](=[O:1])[c:12](-[c:13]2[n:14][c:15]3[cH:16][cH:17][cH:18][cH:19][c:20]3[n:21]2COCC[Si](C)(C)C)[cH:11][c:5](-[c:6]2[cH:7][cH:8][s:9][cH:10]2)[n:4]1>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][s:9][cH:10]2)[cH:11][c:12]1-[c:13]1[n:14][c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[nH:21]1
C[Si](C)(C)CCOCn1nc(-c2ccsc2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
O=c1[nH]nc(-c2ccsc2)cc1-c1nc2ccccc2[nH]1
null
null
ClCCl.FC(C(=O)O)(F)F.C(C)(S)S
Reduction
OtherReaction
7d1cf985bab34d788925de517a3955cc09e2a5635cb594c2eed22bd60af4aaef
4c2ed0f567254ea4c771872583c9a3c5a0aabe43ba2b8e508678a1ced83aca48
O=c1[nH]nc(-c2ccsc2)cc1-c1nc2ccccc2[nH]1
C-[Si](-C)(-C)-C-C-O-C-[n;H0;D3;+0:1]1:[c:2](-[c:3]:[c:4](=[O;D1;H0:5]):[n;H0;D3;+0:6](-C-O-C-C-[Si](-C)(-C)-C):[#7;a:7]:[c:8]):[#7;a:9]:[c:10](:[c:11]):[c:12]:1:[c:13]>>[O;D1;H0:5]=[c:4](:[c:3]-[c:2]1:[#7;a:9]:[c:10](:[c:11]):[c:12](:[c:13]):[nH;D2;+0:1]:1):[nH;D2;+0:6]:[#7;a:7]:[c:8]
null
[]
null
null
18
HOUR
30 mg of 6-thiophen-3-yl-2-(2-trimethylsilanylethoxymethyl)-4-[1-(2-trimethylsilanyl -ethoxymethyl)-1H-benzimidazol-2-yl]-2H-pyridazin-3-one is dissolved in a mixture of dichloromethane (1 ml) and trifluoroacetic acid (1 ml), 18 μl of ethanedithiol are added, and the resulting solution is stirred at room temperature fo...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Silyl protective group.Silyl protective group
null
c1ccnnc1.c1nc2ccccc2[nH]1
c1cnncc1.c1ccc2[nH]cnc2c1
c1cnncc1.c1ccsc1.c1ccc2[nH]cnc2c1
HO-
ClCCl.FC(C(=O)O)(F)F.C(C)(S)S
null
18
C[Si](C)(C)CCOCn1nc(-c2ccsc2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>ClCCl.FC(C(=O)O)(F)F.C(C)(S)S>O=c1[nH]nc(-c2ccsc2)cc1-c1nc2ccccc2[nH]1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-ae34da666d0c49ec9f96cd03cabe9afb
CC1(C)OB(B2OC(C)(C)C(C)(C)O2)OC1(C)C.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>>C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2.B1(OC(C(O1)(C)C)(C)C)B2OC(C(O2)(C)C)(C)C.C(C)(=O)[O-].[K+]>>O=C1C(=CC(=NN1COCC[Si](C)(C)C)B(O)O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2
CC1(C)OB([B:12]2[O:13]C(C)(C)C(C)(C)[O:14]2)OC1(C)C.Cl[c:11]1[n:10][n:9]([CH2:8][O:7][CH2:6][CH2:5][Si:2]([CH3:1])([CH3:3])[CH3:4])[c:34](=[O:35])[c:16](-[c:17]2[n:18][c:19]3[cH:20][cH:21][cH:22][cH:23][c:24]3[n:25]2[CH2:26][O:27][CH2:28][CH2:29][Si:30]([CH3:31])([CH3:32])[CH3:33])[cH:15]1>>[CH3:1][Si:2]([CH3:3])([CH3:...
CC1(C)OB(B2OC(C)(C)C(C)(C)O2)OC1(C)C.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
null
null
CS(=O)C
Miscellaneous
OtherReaction
0f862682a552a117cbdb4251701683c41ea8d7c93834f0609621794a8532f1bb
dafd25fbe01879c365f8c874026e570f49824f4bb82016b29d0c5d21aeb58ca3
O=c1[nH]nccc1-c1nc2ccccc2[nH]1
C-C1(-C)-O-B(-[B;H0;D3;+0:1]2-[O;H0;D2;+0:2]-C(-C)(-C)-C(-C)(-C)-[O;H0;D2;+0:3]-2)-O-C-1(-C)-C.Cl-[c;H0;D3;+0:4]1:[#7;a:5]:[#7;a:6](-[C:7]):[c:8]:[c:9]:[c:10]:1>>[C:7]-[#7;a:6]1:[#7;a:5]:[c;H0;D3;+0:4](-[B;H0;D3;+0:1](-[OH;D1;+0:2])-[OH;D1;+0:3]):[c:10]:[c:9]:[c:8]:1
null
[]
95
CELSIUS
null
null
4 g of 6-chloro-2-(2-trimethylsilanylethoxymethyl)-4-[1-(2-trimethylsilanylethoxy-methyl) -1H-benzimidazol-2-yl]-2H-pyridazin-3-one (example 46), 4.1 g of bis(pinacolato)diboron, 0.19 g of (1,1 ′-bis(diphenylphosphine)-ferrocene)palladium(II) chloride-dichloromethane complex and 2.3 g of potassium acetate are dissolved...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Boronic acid
B1OCCO1.[B]1OCCO1.c1ccnnc1
c1ccnnc1
c1ccnnc1.c1nc2ccccc2[nH]1
HCl.B
CS(=O)C
95
null
CC1(C)OB(B2OC(C)(C)C(C)(C)O2)OC1(C)C.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>CS(=O)C>C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-4020a0a57845445b83289a2bc3d60e68
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.Clc1ccnc(Cl)n1>>C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
O=C1C(=CC(=NN1COCC[Si](C)(C)C)B(O)O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2.ClC1=NC=CC(=N1)Cl.C([O-])([O-])=O.[Cs+].[Cs+]>>ClC1=NC=CC(=N1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2
OB(O)[c:11]1[n:10][n:9]([CH2:8][O:7][CH2:6][CH2:5][Si:2]([CH3:1])([CH3:3])[CH3:4])[c:38](=[O:39])[c:20](-[c:21]2[n:22][c:23]3[cH:24][cH:25][cH:26][cH:27][c:28]3[n:29]2[CH2:30][O:31][CH2:32][CH2:33][Si:34]([CH3:35])([CH3:36])[CH3:37])[cH:19]1.Cl[c:12]1[cH:13][cH:14][n:15][c:16]([Cl:17])[n:18]1>>[CH3:1][Si:2]([CH3:3])([C...
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.Clc1ccnc(Cl)n1
C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
null
null
O.O1CCOCC1
C-C Coupling
Suzuki coupling with boronic acids
f8f5c061fa0766cf8bf2b56a909373cb6775dd68fbe7d26541aa38df8e9d5b4c
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=c1[nH]nc(-c2ccncn2)cc1-c1nc2ccccc2[nH]1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[Cl;D1;H0:4]):[#7;a:5]:[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8]1:[#7;a:9]:[#7;a:10](-[C:11]):[c:12]:[c:13]:[c:14]:1>>[C:11]-[#7;a:10]1:[#7;a:9]:[c;H0;D3;+0:8](-[c;H0;D3;+0:1]2:[#7;a:2]:[c:3](-[Cl;D1;H0:4]):[#7;a:5]:[c:6]:[c:7]:2):[c:14]:[c:13]:[c:12]:1
null
[]
97
CELSIUS
3
HOUR
1.32 g of 6-oxo-1-(2-trimethylsilanylethoxymethyl)-5-[1-(2-trimethylsilanylethoxy-methyl)-1H-benzimidazol-2-yl]-1,6-dihydropyridazine-3-boronic acid, 583 mg of 2,4-dichlorpyrimidine and 3,3 g of cesium carbonate are dissolved in 17 ml of a 1:4 mixture of water and dioxane, and argon is passed through the solution for d...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccnnc1.c1cncnc1
c1ccnnc1.c1cncnc1
c1ccnnc1.c1cncnc1.c1nc2ccccc2[nH]1
HCl.B
O.O1CCOCC1
97
3
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.Clc1ccnc(Cl)n1>O.O1CCOCC1>C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-da03c4138f9d41ce88d2d0a3dba761c6
C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.NCCN1CCOCC1>>C[Si](C)(C)CCOCn1nc(-c2ccnc(NCCN3CCOCC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ClC1=NC=CC(=N1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2.NCCN1CCOCC1>>N1(CCOCC1)CCNC1=NC=CC(=N1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2
Cl[c:16]1[n:15][cH:14][cH:13][c:12](-[c:11]2[n:10][n:9]([CH2:8][O:7][CH2:6][CH2:5][Si:2]([CH3:1])([CH3:3])[CH3:4])[c:46](=[O:47])[c:28](-[c:29]3[n:30][c:31]4[cH:32][cH:33][cH:34][cH:35][c:36]4[n:37]3[CH2:38][O:39][CH2:40][CH2:41][Si:42]([CH3:43])([CH3:44])[CH3:45])[cH:27]2)[n:26]1.[NH2:17][CH2:18][CH2:19][N:20]1[CH2:21...
C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.NCCN1CCOCC1
C[Si](C)(C)CCOCn1nc(-c2ccnc(NCCN3CCOCC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
null
null
null
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
c38b7155556ff28144ae37859ff6668b20d59da60c705d26b158542b6d8385da
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
O=c1[nH]nc(-c2ccnc(NCCN3CCOCC3)n2)cc1-c1nc2ccccc2[nH]1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5]
null
[]
100
CELSIUS
null
null
100 mg of 6-(2-chloropyrimidin-4-yl)-2-(2-trimethylsilanylethoxymethyl)-4-[1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2H-pyridazin-3-one are suspended in 0.5 ml of N-(2-aminoethyl)morpholine, and the reaction mixture is heated at 100° C. in a microwave for 20 minutes. The product is purified by preparativ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cncnc1
c1cncnc1
c1ccnnc1.c1cncnc1.C1COCC[NH]1.c1nc2ccccc2[nH]1
HCl
null
100
null
C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.NCCN1CCOCC1>>C[Si](C)(C)CCOCn1nc(-c2ccnc(NCCN3CCOCC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-1ed32532581c41498e6c601434eb109f
C[Si](C)(C)CCOCn1nc(-c2ccnc(NCCN3CCOCC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>>O=c1[nH]nc(-c2ccnc(NCCN3CCOCC3)n2)cc1-c1nc2ccccc2[nH]1
N1(CCOCC1)CCNC1=NC=CC(=N1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2>>N1C(=NC2=C1C=CC=C2)C=2C(NN=C(C2)C2=NC(=NC=C2)NCCN2CCOCC2)=O
C[Si](C)(C)CCOC[n:3]1[c:2](=[O:1])[c:22](-[c:23]2[n:24][c:25]3[cH:26][cH:27][cH:28][cH:29][c:30]3[n:31]2COCC[Si](C)(C)C)[cH:21][c:5](-[c:6]2[cH:7][cH:8][n:9][c:10]([NH:11][CH2:12][CH2:13][N:14]3[CH2:15][CH2:16][O:17][CH2:18][CH2:19]3)[n:20]2)[n:4]1>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][c:10]([NH:11][CH...
C[Si](C)(C)CCOCn1nc(-c2ccnc(NCCN3CCOCC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
O=c1[nH]nc(-c2ccnc(NCCN3CCOCC3)n2)cc1-c1nc2ccccc2[nH]1
null
null
ClCCl.FC(C(=O)O)(F)F
Reduction
OtherReaction
7d1cf985bab34d788925de517a3955cc09e2a5635cb594c2eed22bd60af4aaef
4c2ed0f567254ea4c771872583c9a3c5a0aabe43ba2b8e508678a1ced83aca48
O=c1[nH]nc(-c2ccnc(NCCN3CCOCC3)n2)cc1-c1nc2ccccc2[nH]1
C-[Si](-C)(-C)-C-C-O-C-[n;H0;D3;+0:1]1:[c:2](-[c:3]:[c:4](=[O;D1;H0:5]):[n;H0;D3;+0:6](-C-O-C-C-[Si](-C)(-C)-C):[#7;a:7]:[c:8]):[#7;a:9]:[c:10](:[c:11]):[c:12]:1:[c:13]>>[O;D1;H0:5]=[c:4](:[c:3]-[c:2]1:[#7;a:9]:[c:10](:[c:11]):[c:12](:[c:13]):[nH;D2;+0:1]:1):[nH;D2;+0:6]:[#7;a:7]:[c:8]
null
[]
null
null
2
HOUR
88 mg of 6-[2-(2-morpholin-4-ylethylamino)pyrimidin-4-yl]-2-(2-trimethylsilanyl-ethoxymethyl)-4-[1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2H-pyridazin-3-one are dissolved in 2 ml of a 1:1 mixture of dichloromethane and trifluoroacetic acid, and the mixture is stirred at room temperature for 2 hours. The...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Silyl protective group.Silyl protective group
null
c1ccnnc1.c1nc2ccccc2[nH]1
c1cnncc1.c1ccc2[nH]cnc2c1
c1cnncc1.c1cncnc1.C1COCC[NH]1.c1ccc2[nH]cnc2c1
HO-
ClCCl.FC(C(=O)O)(F)F
null
2
C[Si](C)(C)CCOCn1nc(-c2ccnc(NCCN3CCOCC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>ClCCl.FC(C(=O)O)(F)F>O=c1[nH]nc(-c2ccnc(NCCN3CCOCC3)n2)cc1-c1nc2ccccc2[nH]1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2c8b3ade3271450f9aea1bf3410a9b3b
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1ccnc(SC)n1.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>>CSc1nccc(-c2cc(-c3nc4ccccc4[nH]3)c(=O)[nH]n2)n1
ClC=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2.CSC1=NC=CC(=N1)[Sn](CCCC)(CCCC)CCCC.[F-].[K+]>>N1C(=NC2=C1C=CC=C2)C=2C(NN=C(C2)C2=NC(=NC=C2)SC)=O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c:7]1[cH:6][cH:5][n:4][c:3]([S:2][CH3:1])[n:24]1.C[Si](C)(C)CCOC[n:19]1[c:11](-[c:10]2[cH:9][c:8](Cl)[n:23][n:22](COCC[Si](C)(C)C)[c:20]2=[O:21])[n:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]21>>[CH3:1][S:2][c:3]1[n:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][c:10](-[c:11]3[n:12][c:13]4[cH:14][c...
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1ccnc(SC)n1.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
CSc1nccc(-c2cc(-c3nc4ccccc4[nH]3)c(=O)[nH]n2)n1
null
[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
CN(C)C=O
C-C Coupling
OtherReaction
a8e5eb9fcb21c11b951297cb6cb6786be2ba17b443b370247ca2ac2ddeceecab
ac334791059cb918059e3bc1de4d0b64599a26cda3fbc8254e9a0dd486c2ef69
O=c1[nH]nc(-c2ccncn2)cc1-c1nc2ccccc2[nH]1
C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[#16:4]):[#7;a:5]:[c:6]:[c:7]:1.C-[Si](-C)(-C)-C-C-O-C-[n;H0;D3;+0:8]1:[c:9](-[c:10]2:[c:11]:[c;H0;D3;+0:12](-Cl):[#7;a:13]:[n;H0;D3;+0:14](-C-O-C-C-[Si](-C)(-C)-C):[c:15]:2=[O;D1;H0:16]):[#7;a:17]:[c:18](:[c:19]):[c:20]:1:[c:21]>>[#16:4]-[c:3...
null
[]
80
CELSIUS
30
MINUTE
The compound is prepared in analogy to example 15. A Stille coupling is carried out instead of the Suzuki coupling. This entails dissolving 6-chloro-4-[1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2-(2-trimethylsilanylethoxy-methyl)-2H-pyridazin-3-one, 2-methylsulfanyl-4-tributylstannylpyrimidine, tetra-eth...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Ether.Silyl protective group.Silyl protective group.Tin
null
c1cncnc1.c1ccnnc1.c1nc2ccccc2[nH]1
c1cncnc1.c1cnncc1.c1ccc2[nH]cnc2c1
c1cncnc1.c1cnncc1.c1ccc2[nH]cnc2c1
HCl.Sn
[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O
80
0.5
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1ccnc(SC)n1.C[Si](C)(C)CCOCn1nc(Cl)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O>CSc1nccc(-c2cc(-c3nc4ccccc4[nH]3)c(=O)[nH]n2)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-0b1e3bb90b464aa88133a65f8742aa21
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.c1c[nH]cn1>>C[SiH](C)CCOCn1c(-c2cc(-n3ccnc3)nn(COCC[Si](C)(C)C)c2=O)nc2ccccc21
O=C1C(=CC(=NN1COCC[Si](C)(C)C)B(O)O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2.N1C=NC=C1>>C[SiH](CCOCN1C(=NC2=C1C=CC=C2)C=2C(N(N=C(C2)N2C=NC=C2)COCC[Si](C)(C)C)=O)C
C[Si:2]([CH3:1])([CH3:3])[CH2:4][CH2:5][O:6][CH2:7][n:8]1[c:9](-[c:10]2[cH:11][c:12](B(O)O)[n:18][n:19]([CH2:20][O:21][CH2:22][CH2:23][Si:24]([CH3:25])([CH3:26])[CH3:27])[c:28]2=[O:29])[n:30][c:31]2[cH:32][cH:33][cH:34][cH:35][c:36]12.[nH:13]1[cH:14][cH:15][n:16][cH:17]1>>[CH3:1][SiH:2]([CH3:3])[CH2:4][CH2:5][O:6][CH2:...
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.c1c[nH]cn1
C[SiH](C)CCOCn1c(-c2cc(-n3ccnc3)nn(COCC[Si](C)(C)C)c2=O)nc2ccccc21
null
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-]
O.N1=CC=CC=C1
Heteroatom Alkylation and Arylation
OtherReaction
6467f9b8cfd58f6a53283597ffd368b9d3ea804dc7d6a518754aab70540629a5
fa6d8644f910d21bb1c1692e112b1c812d7af5afcda733004f9d45091a0873f3
O=c1[nH]nc(-n2ccnc2)cc1-c1nc2ccccc2[nH]1
C-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4]-[C:5].O-B(-O)-[c;H0;D3;+0:6]1:[#7;a:7]:[#7;a:8](-[C:9]):[c:10]:[c:11]:[c:12]:1.[#7;a:13]1:[c:14]:[c:15]:[nH;D2;+0:16]:[c:17]:1>>[C:9]-[#7;a:8]1:[#7;a:7]:[c;H0;D3;+0:6](-[n;H0;D3;+0:16]2:[c:15]:[c:14]:[#7;a:13]:[c:17]:2):[c:12]:[c:11]:[c:10]:1.[C:5]-[C:4]-[SiH;D3;+0:1]...
null
[]
80
CELSIUS
3
HOUR
100 mg of 6-oxo-1-(2-trimethylsilanylethoxymethyl)-5-[1-(2-trimethylsilanyl-ethoxymethyl)-1H-benzimidazol-2-yl]-1,6-dihydropyridazine-3-boronic acid (example 55), 35.5 mg of copper(II) acetate and 20 mg of imidazole are dissolved in dry pyridine, and the solution is stirred at 80° C. for 3 hours. For workup, it is dilu...
10.6084/m9.figshare.5104873.v1
null
Boronic acid.Silyl protective group
null
c1ccnnc1.c1c[nH]cn1
c1ccnnc1.c1c[nH]cn1
c1ccnnc1.c1c[nH]cn1.c1nc2ccccc2[nH]1
HO-.B
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].O.N1=CC=CC=C1
80
3
C[Si](C)(C)CCOCn1nc(B(O)O)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.c1c[nH]cn1>C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].O.N1=CC=CC=C1>C[SiH](C)CCOCn1c(-c2cc(-n3ccnc3)nn(COCC[Si](C)(C)C)c2=O)nc2ccccc21
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-afba9e13ab974bc092140c0feb185cb3
C[SiH](C)CCOCn1c(-c2cc(-n3ccnc3)nn(COCC[Si](C)(C)C)c2=O)nc2ccccc21>>O=c1[nH]nc(-n2ccnc2)cc1-c1nc2ccccc2[nH]1
C[SiH](CCOCN1C(=NC2=C1C=CC=C2)C=2C(N(N=C(C2)N2C=NC=C2)COCC[Si](C)(C)C)=O)C>>N1C(=NC2=C1C=CC=C2)C=2C(NN=C(C2)N2C=NC=C2)=O
C[SiH](C)CCOC[n:21]1[c:13](-[c:12]2[c:2](=[O:1])[n:3](COCC[Si](C)(C)C)[n:4][c:5](-[n:6]3[cH:7][cH:8][n:9][cH:10]3)[cH:11]2)[n:14][c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]21>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[n:6]2[cH:7][cH:8][n:9][cH:10]2)[cH:11][c:12]1-[c:13]1[n:14][c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[nH:21]1
C[SiH](C)CCOCn1c(-c2cc(-n3ccnc3)nn(COCC[Si](C)(C)C)c2=O)nc2ccccc21
O=c1[nH]nc(-n2ccnc2)cc1-c1nc2ccccc2[nH]1
null
null
ClCCl.FC(C(=O)O)(F)F
Reduction
OtherReaction
69c0abd1a33ee5635ff31db131553721d00e2fdb697abe991abc87f32e437d8e
0ba73238bad7c29e9afad223c6a4c9bb32fde37408eb7a5e7c67288f0e8d8816
O=c1[nH]nc(-n2ccnc2)cc1-c1nc2ccccc2[nH]1
C-[SiH](-C)-C-C-O-C-[n;H0;D3;+0:1]1:[c:2](-[c:3]:[c:4](=[O;D1;H0:5]):[n;H0;D3;+0:6](-C-O-C-C-[Si](-C)(-C)-C):[#7;a:7]:[c:8]):[#7;a:9]:[c:10](:[c:11]):[c:12]:1:[c:13]>>[O;D1;H0:5]=[c:4](:[c:3]-[c:2]1:[#7;a:9]:[c:10](:[c:11]):[c:12](:[c:13]):[nH;D2;+0:1]:1):[nH;D2;+0:6]:[#7;a:7]:[c:8]
null
[]
null
null
2
HOUR
40 mg of 4-[1-(2-dimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-6-imidazol-1-yl-2-(2-trimethylsilanylethoxymethyl)-2H-pyridazin-3-one are dissolved in 2 ml of a 1:1 mixture of dichloromethane and trifluoroacetic acid, and the mixture is stirred at room temperature for 2 hours. The volatile components are then disti...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Silyl protective group
null
c1ccnnc1.c1nc2ccccc2[nH]1
c1cnncc1.c1ccc2[nH]cnc2c1
c1cnncc1.c1c[nH]cn1.c1ccc2[nH]cnc2c1
HO-
ClCCl.FC(C(=O)O)(F)F
null
2
C[SiH](C)CCOCn1c(-c2cc(-n3ccnc3)nn(COCC[Si](C)(C)C)c2=O)nc2ccccc21>ClCCl.FC(C(=O)O)(F)F>O=c1[nH]nc(-n2ccnc2)cc1-c1nc2ccccc2[nH]1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-ec95a085efed4ea4bd8fe4a25e73c26c
COc1cc(Br)cc(C=O)c1O.C[Si](C)(C)CCOCCl>>COc1cc(Br)cc(C=O)c1OCOCC[Si](C)(C)C
BrC=1C=C(C(=C(C=O)C1)O)OC.C([O-])([O-])=O.[K+].[K+].ClCOCC[Si](C)(C)C>>BrC=1C=C(C(=C(C=O)C1)OCOCC[Si](C)(C)C)OC
[CH3:1][O:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8]([CH:9]=[O:10])[c:11]1[OH:12].Cl[CH2:13][O:14][CH2:15][CH2:16][Si:17]([CH3:18])([CH3:19])[CH3:20]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8]([CH:9]=[O:10])[c:11]1[O:12][CH2:13][O:14][CH2:15][CH2:16][Si:17]([CH3:18])([CH3:19])[CH3:20]
COc1cc(Br)cc(C=O)c1O.C[Si](C)(C)CCOCCl
COc1cc(Br)cc(C=O)c1OCOCC[Si](C)(C)C
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
6e90ffbf0683e1a3ee55c5e3ea453aefc5ddd369c0150ed0150f9546d7e47f4f
efd670663709b79afcad1306da9f69b33a0147cfa3639ca4c0b54b35ef4b1852
c1ccccc1
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3].[O;D1;H0:4]=[C:5]-[c:6]:[c:7](-[OH;D1;+0:8]):[c:9]>>[C:3]-[#8:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:8]-[c:7](:[c:9]):[c:6]-[C:5]=[O;D1;H0:4]
null
[]
null
null
48
HOUR
10 g of 5-bromo-2-hydroxy-3-methoxybenzaldehyde, 23.9 g of potassium carbonate and 12.2 g of (2-chloromethoxyethyl)trimethylsilane is suspended in 500 ml of DMF and stirred at room temperature for 48 hours. The DMF is distilled off in vacuo, the residue is dissolved in ethyl acetate, and the resulting solution is extra...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ether.Aromatic alcohol
Ether.Ether
null
null
c1ccccc1
HCl
CN(C)C=O
null
48
COc1cc(Br)cc(C=O)c1O.C[Si](C)(C)CCOCCl>CN(C)C=O>COc1cc(Br)cc(C=O)c1OCOCC[Si](C)(C)C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-3838062fb5794b499372a71d6efce843
CN.COc1cc(-c2cc(-c3nc4ccccc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(C=O)c1OCOCC[Si](C)(C)C>>CNCc1cc(-c2cc(-c3nc4ccccc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(OC)c1OCOCC[Si](C)(C)C
COC=1C(=C(C=O)C=C(C1)C1=NN(C(C(=C1)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2)=O)COCC[Si](C)(C)C)OCOCC[Si](C)(C)C.CN.C1CCOC1.C(#N)[BH3-].[Na+]>>COC=1C=C(C=C(C1OCOCC[Si](C)(C)C)CNC)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2
[CH3:1][NH2:2].O=[CH:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][c:9](-[c:10]3[n:11][c:12]4[cH:13][cH:14][cH:15][cH:16][c:17]4[n:18]3[CH2:19][O:20][CH2:21][CH2:22][Si:23]([CH3:24])([CH3:25])[CH3:26])[c:27](=[O:28])[n:29]([CH2:30][O:31][CH2:32][CH2:33][Si:34]([CH3:35])([CH3:36])[CH3:37])[n:38]2)[cH:39][c:40]([O:41][CH3:42])[c:43]...
CN.COc1cc(-c2cc(-c3nc4ccccc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(C=O)c1OCOCC[Si](C)(C)C
CNCc1cc(-c2cc(-c3nc4ccccc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(OC)c1OCOCC[Si](C)(C)C
null
null
CO.C(C)(=O)O
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
O=c1[nH]nc(-c2ccccc2)cc1-c1nc2ccccc2[nH]1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[NH2;D1;+0:6]>>[C;D1;H3:5]-[NH;D2;+0:6]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
16
HOUR
200 mg of methoxy-5-{6-oxo-1-(2-trimethylsilanylethoxymethyl)-5-[1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-1,6-dihydropyridazin-3-yl}-2-(2-trimethylsilanylethoxymethoxy)benzaldehyde are dissolved in 4.5 ml of methanol and methylamine (0.146 ml of a THF solution), and 18.4 mg of sodium cyanoborohydride ar...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccnnc1.c1nc2ccccc2[nH]1
Other
CO.C(C)(=O)O
null
16
CN.COc1cc(-c2cc(-c3nc4ccccc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(C=O)c1OCOCC[Si](C)(C)C>CO.C(C)(=O)O>CNCc1cc(-c2cc(-c3nc4ccccc4n3COCC[Si](C)(C)C)c(=O)n(COCC[Si](C)(C)C)n2)cc(OC)c1OCOCC[Si](C)(C)C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-552dac4e3cd44625bf490bacd309abfc
COc1cc(Br)cc(C=O)c1OCOCC[Si](C)(C)C.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1>>COc1cc(Br)cc(-c2cnco2)c1OCOCC[Si](C)(C)C
BrC=1C=C(C(=C(C=O)C1)OCOCC[Si](C)(C)C)OC.C1(=CC=C(C=C1)S(=O)(=O)C[N+]#[C-])C>>BrC=1C=C(C(=C(C1)C1=CN=CO1)OCOCC[Si](C)(C)C)OC
[CH3:1][O:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8]([CH:9]=[O:13])[c:14]1[O:15][CH2:16][O:17][CH2:18][CH2:19][Si:20]([CH3:21])([CH3:22])[CH3:23].Cc1ccc(S(=O)(=O)[CH2:10][N+:11]#[C-:12])cc1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8](-[c:9]2[cH:10][n:11][cH:12][o:13]2)[c:14]1[O:15][CH2:16][O:17][CH2:18][CH2:19][Si:20...
COc1cc(Br)cc(C=O)c1OCOCC[Si](C)(C)C.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1
COc1cc(Br)cc(-c2cnco2)c1OCOCC[Si](C)(C)C
null
null
CO
Functional Group Interconversion
OtherReaction
350ec210554942a1358fcbd88dfbddb6e2b23a43f1c83725aa708598a14ee7ab
c716b04888bf3cb683ec79e24be07b585e1dc289053b42331c058bc5f98fd4eb
c1ccc(-c2cnco2)cc1
C-c1:c:c:c(-S(=O)(=O)-[CH2;D2;+0:1]-[N+;H0;D2:2]#[C-;H0;D1:3]):c:c:1.[#8:4]-[c:5](:[c:6]):[c;H0;D3;+0:7](-[CH;D2;+0:8]=[O;H0;D1;+0:9]):[c:10]:[c:11]>>[#8:4]-[c:5](:[c:6]):[c;H0;D3;+0:7](-[c;H0;D3;+0:8]1:[cH;D2;+0:1]:[n;H0;D2;+0:2]:[cH;D2;+0:3]:[o;H0;D2;+0:9]:1):[c:10]:[c:11]
null
[]
null
null
null
null
1 g of 5-bromo-3-methoxy-2-(2-trimethylsilanylethoxymethoxy)benzaldehyde and 0.54 g of p-toluenesulfonylmethyl isocyanide are dissolved in 40 ml of methanol, 0.38 g of o-potassiumcarbonate is added in portions, and the reaction mixture is heated to reflux for 18 h. The solvent is then distilled off, and the crude produ...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Aldehyde.Isocyanide
null
c1ccccc1
c1cocn1
c1ccccc1.c1cocn1
TsOH.HO-
CO
null
null
COc1cc(Br)cc(C=O)c1OCOCC[Si](C)(C)C.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1>CO>COc1cc(Br)cc(-c2cnco2)c1OCOCC[Si](C)(C)C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-75bad0bdb18843a0926daf2d162608bf
C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.OB(O)C1CC1>>C[Si](C)(C)CCOCn1nc(-c2ccnc(C3CC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ClC1=NC=CC(=N1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2.C1(CC1)B(O)O.P(=O)([O-])([O-])[O-].[K+].[K+].[K+]>>C1(CC1)C1=NC=CC(=N1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2
Cl[c:16]1[n:15][cH:14][cH:13][c:12](-[c:11]2[n:10][n:9]([CH2:8][O:7][CH2:6][CH2:5][Si:2]([CH3:1])([CH3:3])[CH3:4])[c:40](=[O:41])[c:22](-[c:23]3[n:24][c:25]4[cH:26][cH:27][cH:28][cH:29][c:30]4[n:31]3[CH2:32][O:33][CH2:34][CH2:35][Si:36]([CH3:37])([CH3:38])[CH3:39])[cH:21]2)[n:20]1.OB(O)[CH:17]1[CH2:18][CH2:19]1>>[CH3:1...
C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.OB(O)C1CC1
C[Si](C)(C)CCOCn1nc(-c2ccnc(C3CC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
null
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2]
O.C1(=CC=CC=C1)C
C-C Coupling
OtherReaction
412d14d936f2fe74271076c2d85cda822694d627c10e4da821198f343e0c85d8
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=c1[nH]nc(-c2ccnc(C3CC3)n2)cc1-c1nc2ccccc2[nH]1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].O-B(-O)-[CH;D3;+0:6]1-[C:7]-[C:8]-1>>[c:5]:[#7;a:4]:[c;H0;D3;+0:1](-[CH;D3;+0:6]1-[C:7]-[C:8]-1):[#7;a:2]:[c:3]
null
[]
100
CELSIUS
9
HOUR
100 mg of 6-(2-chloropyrimidin-4-yl)-2-(2-trimethylsilanylethoxymethyl)-4-[1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2H-pyridazin-3-one, 29.2 mg of cyclopropylboronic acid and 138 mg of potassium phosphate are dissolved in 1 ml of toluene and 0.05 ml of water and, under an argon atmosphere, 17 mg of 1,1′...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cncnc1.C1CC1
c1cncnc1.C1CC1
c1ccnnc1.c1cncnc1.C1CC1.c1nc2ccccc2[nH]1
HCl.B
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].O.C1(=CC=CC=C1)C
100
9
C[Si](C)(C)CCOCn1nc(-c2ccnc(Cl)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O.OB(O)C1CC1>C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].O.C1(=CC=CC=C1)C>C[Si](C)(C)CCOCn1nc(-c2ccnc(C3CC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-836e08e052fe43058a58ca664df681f1
C[Si](C)(C)CCOCn1nc(-c2ccnc(C3CC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>>O=c1[nH]nc(-c2ccnc(C3CC3)n2)cc1-c1nc2ccccc2[nH]1
C1(CC1)C1=NC=CC(=N1)C=1C=C(C(N(N1)COCC[Si](C)(C)C)=O)C1=NC2=C(N1COCC[Si](C)(C)C)C=CC=C2.C(C)O>>N1C(=NC2=C1C=CC=C2)C=2C(NN=C(C2)C2=NC(=NC=C2)C2CC2)=O
C[Si](C)(C)CCOC[n:3]1[c:2](=[O:1])[c:16](-[c:17]2[n:18][c:19]3[cH:20][cH:21][cH:22][cH:23][c:24]3[n:25]2COCC[Si](C)(C)C)[cH:15][c:5](-[c:6]2[cH:7][cH:8][n:9][c:10]([CH:11]3[CH2:12][CH2:13]3)[n:14]2)[n:4]1>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][c:10]([CH:11]3[CH2:12][CH2:13]3)[n:14]2)[cH:15][c:16]1-[c:17...
C[Si](C)(C)CCOCn1nc(-c2ccnc(C3CC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O
O=c1[nH]nc(-c2ccnc(C3CC3)n2)cc1-c1nc2ccccc2[nH]1
null
null
O1CCOCC1.Cl
Reduction
OtherReaction
7d1cf985bab34d788925de517a3955cc09e2a5635cb594c2eed22bd60af4aaef
4c2ed0f567254ea4c771872583c9a3c5a0aabe43ba2b8e508678a1ced83aca48
O=c1[nH]nc(-c2ccnc(C3CC3)n2)cc1-c1nc2ccccc2[nH]1
C-[Si](-C)(-C)-C-C-O-C-[n;H0;D3;+0:1]1:[c:2](-[c:3]:[c:4](=[O;D1;H0:5]):[n;H0;D3;+0:6](-C-O-C-C-[Si](-C)(-C)-C):[#7;a:7]:[c:8]):[#7;a:9]:[c:10](:[c:11]):[c:12]:1:[c:13]>>[O;D1;H0:5]=[c:4](:[c:3]-[c:2]1:[#7;a:9]:[c:10](:[c:11]):[c:12](:[c:13]):[nH;D2;+0:1]:1):[nH;D2;+0:6]:[#7;a:7]:[c:8]
null
[]
null
null
3
HOUR
27 mg of 6-(2-cyclopropylpyrimidin-4-yl)-2-(2-trimethylsilanylethoxymethyl)-4-[1-(2-trimethylsilanylethoxymethyl)-1H-benzimidazol-2-yl]-2H-pyridazin-3-one are dissolved in 2.5 ml of 4M hydrochloric acid solution in dioxane and 1 ml of ethanol and stirred at room temperature for 2 days. The solvent is then distilled off...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Silyl protective group.Silyl protective group
null
c1ccnnc1.c1nc2ccccc2[nH]1
c1cnncc1.c1ccc2[nH]cnc2c1
c1cnncc1.c1cncnc1.C1CC1.c1ccc2[nH]cnc2c1
HO-
O1CCOCC1.Cl
null
3
C[Si](C)(C)CCOCn1nc(-c2ccnc(C3CC3)n2)cc(-c2nc3ccccc3n2COCC[Si](C)(C)C)c1=O>O1CCOCC1.Cl>O=c1[nH]nc(-c2ccnc(C3CC3)n2)cc1-c1nc2ccccc2[nH]1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-0989b2748d704d2894e860d20aea4ea4
CO.O=C(O)Cc1ccc(Cl)cc1>>COC(=O)Cc1ccc(Cl)cc1
ClC1=CC=C(C=C1)CC(=O)O.Cl.CO>>ClC1=CC=C(C=C1)CC(=O)OC
[CH3:1][OH:2].O[C:3](=[O:4])[CH2:5][c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1
CO.O=C(O)Cc1ccc(Cl)cc1
COC(=O)Cc1ccc(Cl)cc1
null
null
null
Protection
Esterification of Carboxylic Acids
9cecdbd189c6f9c3648521d17154d013842a5498de4e76e65efb1d842973340b
af0b8064f2e82ebe66c4c29d2391785ac1b993104265ccdc4d67ca79e36fa3c8
c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4].[C;D1;H3:5]-[OH;D1;+0:6]>>[C;D1;H3:5]-[O;H0;D2;+0:6]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4]
null
[]
null
null
null
null
4-Chlorophenylacetic acid (5.0 g) was dissolved in 10% hydrogen chloride-methanol solution (50 ml) and heated under reflex for 14 hours. The solvent then was removed under reduced pressure and saturated sodium hydrogencarbonate solution was added to the residue, followed by extraction with ethyl acetate. The organic la...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Methanol
Ester
null
null
c1ccccc1
HO-
null
null
null
CO.O=C(O)Cc1ccc(Cl)cc1>>COC(=O)Cc1ccc(Cl)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-605b849843804862a90b8e36f41a45f4
CI.COC(=O)C(c1ccc(Cl)cc1)C1CCCC1>>COC(=O)C(C)(c1ccc(Cl)cc1)C1CCCC1
C(C)(C)NC(C)C.ClC1=CC=C(C=C1)C(C(=O)OC)C1CCCC1.CI>>ClC1=CC=C(C=C1)C(C(=O)OC)(C)C1CCCC1
I[CH3:6].[CH3:1][O:2][C:3](=[O:4])[CH:5]([c:7]1[cH:8][cH:9][c:10]([Cl:11])[cH:12][cH:13]1)[CH:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1>>[CH3:1][O:2][C:3](=[O:4])[C:5]([CH3:6])([c:7]1[cH:8][cH:9][c:10]([Cl:11])[cH:12][cH:13]1)[CH:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1
CI.COC(=O)C(c1ccc(Cl)cc1)C1CCCC1
COC(=O)C(C)(c1ccc(Cl)cc1)C1CCCC1
null
null
C1CCOC1.C(CCC)[Li].[Cl-].[NH4+]
C-C Coupling
Methylation with MeI_tertiary
4a52ebe9ffae5bdd307b0b4ac6a7069bc533ab8d42293ed2712c32b846010273
49d6f28766066d07dffbcc6f4da77792f6ba67b4de619800bad651525d6fe2e7
c1ccc(CC2CCCC2)cc1
I-[CH3;D1;+0:1].[C:2]-[C:3](-[CH;D3;+0:4](-[C:5](=[O;D1;H0:6])-[#8:7]-[C;D1;H3:8])-[c:9](:[c:10]):[c:11])-[C:12]>>[C:2]-[C:3](-[C;H0;D4;+0:4](-[CH3;D1;+0:1])(-[C:5](=[O;D1;H0:6])-[#8:7]-[C;D1;H3:8])-[c:9](:[c:10]):[c:11])-[C:12]
null
[]
-35
CELSIUS
10
MINUTE
To a solution of diisopropylamine (0.15 ml) in THF (2 ml), n-butyl lithium (1.5 M hexane solution, 0.6 ml) was added at −78° C., stirred for 10 minutes and another solution of methyl 2-(4-chlorophenyl)-2-cyclopentylacetate (200 mg) in THF (1.5 ml) was added dropwise. After 15 minutes' stirring, the system temperature w...
10.6084/m9.figshare.5104873.v1
null
Ester
Ester
null
null
c1ccccc1.C1CCCC1
HI
C1CCOC1.C(CCC)[Li].[Cl-].[NH4+]
-35
0.166667
CI.COC(=O)C(c1ccc(Cl)cc1)C1CCCC1>C1CCOC1.C(CCC)[Li].[Cl-].[NH4+]>COC(=O)C(C)(c1ccc(Cl)cc1)C1CCCC1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-b6e31047605947038cdd2e34c6fc6eb3
Brc1cccnc1.CCOC(=O)C(=O)c1ccc(Cl)cc1>>CCOC(=O)C(O)(c1ccc(Cl)cc1)c1cccnc1
BrC=1C=NC=CC1.ClC1=CC=C(C=C1)C(C(=O)OCC)=O.[Cl-].[NH4+]>>ClC1=CC=C(C=C1)C(C(=O)OCC)(C=1C=NC=CC1)O
Br[c:15]1[cH:16][cH:17][cH:18][n:19][cH:20]1.[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[O:7])[c:8]1[cH:9][cH:10][c:11]([Cl:12])[cH:13][cH:14]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6]([OH:7])([c:8]1[cH:9][cH:10][c:11]([Cl:12])[cH:13][cH:14]1)[c:15]1[cH:16][cH:17][cH:18][n:19][cH:20]1
Brc1cccnc1.CCOC(=O)C(=O)c1ccc(Cl)cc1
CCOC(=O)C(O)(c1ccc(Cl)cc1)c1cccnc1
null
null
C(CCC)[Li].C(C)OCC
C-C Coupling
Grignard_alcohol
72d307076f6defa0943f87bbc847fe67f35fbaa78203fa718ec66467f1588bf4
9ad4a4524e70e857006264b5570f9463fa55d41dbe0be303433eb1b99baa979d
c1ccc(Cc2cccnc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1.[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[C;H0;D3;+0:11](=[O;H0;D1;+0:12])-[c:13](:[c:14]):[c:15]>>[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[C;H0;D4;+0:11](-[OH;D1;+0:12])(-[c:13](:[c:14]):[c:15])-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1
48.3
[{"value": 48.3, "product": "ClC1=CC=C(C=C1)C(C(=O)OCC)(C=1C=NC=CC1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
To a solution of 3-bromopyridine (640 mg) in diethyl ether (10 ml), n-butyl lithium (2.5M-hexane solution, 1.80 ml) was added at −74° C. After 15 minutes' stirring at the same temperature, a solution of ethyl 2-(4-chlorophenyl)-2-oxoacetate (960 mg) in diethyl ether (100 ml) was added. The temperature of the system was...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ketone
Ester.Tertiary alcohol
c1ccncc1
c1ccncc1
c1ccccc1.c1ccncc1
Br-
C(CCC)[Li].C(C)OCC
null
0.25
Brc1cccnc1.CCOC(=O)C(=O)c1ccc(Cl)cc1>C(CCC)[Li].C(C)OCC>CCOC(=O)C(O)(c1ccc(Cl)cc1)c1cccnc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c5bb6ebc07cd49ad9ab13e25aeb3b07a
COC(=O)C(Br)c1ccc(Cl)cc1.c1c[nH]cn1>>COC(=O)C(c1ccc(Cl)cc1)n1ccnc1
O.N1C=NC=C1.C(C)N(CC)CC.BrC(C(=O)OC)C1=CC=C(C=C1)Cl>>ClC1=CC=C(C=C1)C(C(=O)OC)N1C=NC=C1
Br[CH:5]([C:3]([O:2][CH3:1])=[O:4])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1.[nH:13]1[cH:14][cH:15][n:16][cH:17]1>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1)[n:13]1[cH:14][cH:15][n:16][cH:17]1
COC(=O)C(Br)c1ccc(Cl)cc1.c1c[nH]cn1
COC(=O)C(c1ccc(Cl)cc1)n1ccnc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
6e796d385604f3d786cae1d46df3d343d7680e137c2fb51f458a62eeb83d5c95
88c92d2671864e93a5b5578ca874d1de41e4f02ddd75a3966019ee10f35d4923
c1ccc(Cn2ccnc2)cc1
Br-[CH;D3;+0:1](-[C:2](=[O;D1;H0:3])-[#8:4]-[C;D1;H3:5])-[c:6](:[c:7]):[c:8].[#7;a:9]1:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:1>>[C;D1;H3:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[CH;D3;+0:1](-[c:6](:[c:7]):[c:8])-[n;H0;D3;+0:12]1:[c:11]:[c:10]:[#7;a:9]:[c:13]:1
64
[{"value": 64.0, "product": "ClC1=CC=C(C=C1)C(C(=O)OC)N1C=NC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of imidazole (170 mg) and triethylamine (350 ml) in DMF (1 ml), a solution of methyl 2-bromo-2-(4-chlorophenyl)-acetate (657 mg) in DMF (3 ml) was added. After stirring for an overnight, water was added to the reaction liquid, followed by extraction with ethyl acetate, washing with saturated brine and dry...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ester
Ester
c1c[nH]cn1
c1c[nH]cn1
c1ccccc1.c1c[nH]cn1
HBr
CN(C)C=O
null
8
COC(=O)C(Br)c1ccc(Cl)cc1.c1c[nH]cn1>CN(C)C=O>COC(=O)C(c1ccc(Cl)cc1)n1ccnc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-d993797223ee4d3ca68c621030b8b789
CC(C)(C)OC(=O)N1CCC(=O)CC1.Fc1ccc(Br)cn1>>Fc1ccc(C2CCNCC2)cn1
O.C(CCC)[Li].FC1=NC=C(C=C1)Br.O=C1CCN(CC1)C(=O)OC(C)(C)C>>FC1=CC=C(C=N1)C1CCNCC1
CC(C)(C)OC(=O)[N:9]1[CH2:8][CH2:7][C:6](=O)[CH2:11][CH2:10]1.Br[c:5]1[cH:4][cH:3][c:2]([F:1])[n:13][cH:12]1>>[F:1][c:2]1[cH:3][cH:4][c:5]([CH:6]2[CH2:7][CH2:8][NH:9][CH2:10][CH2:11]2)[cH:12][n:13]1
CC(C)(C)OC(=O)N1CCC(=O)CC1.Fc1ccc(Br)cn1
Fc1ccc(C2CCNCC2)cn1
null
null
C(C)OCC
C-C Coupling
OtherReaction
17baea866cb419c2d98bbfc24c0f6d4c3b0290618dd26f428f7bc9c349f7a7a8
f252626502c0f696a1ffbbbaa2d43e4011a92af8563197ce7c691972462c5955
c1cncc(C2CCNCC2)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1.C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:7]1-[C:8]-[C:9]-[C;H0;D3;+0:10](=O)-[C:11]-[C:12]-1>>[#7;a:3]1:[c:2]:[c;H0;D3;+0:1](-[CH;D3;+0:10]2-[C:9]-[C:8]-[NH;D2;+0:7]-[C:12]-[C:11]-2):[c:6]:[c:5]:[c:4]:1
52.7
[{"value": 52.7, "product": "FC1=CC=C(C=N1)C1CCNCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-35
CELSIUS
15
MINUTE
A solution of 2-fluoro-5-bromopyridine (7.69 g) in diethyl ether (160 ml) was cooled to −78° C., and into which n-butyl lithium (1,56M-hexane solution, 30 ml) was added dropwise at a temperature not higher than −70° C. After 15 minutes' stirring, tert-butyl 4-oxo-1-piperidinecarboxylate (8.7 g) was added. Temperature o...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carbamic ester.Ketone.Ether.Boc
Secondary amine
C1CC[NH]CC1.c1ccncc1
c1ccncc1.C1CCNCC1
c1ccncc1.C1CCNCC1
HBr
C(C)OCC
-35
0.25
CC(C)(C)OC(=O)N1CCC(=O)CC1.Fc1ccc(Br)cn1>C(C)OCC>Fc1ccc(C2CCNCC2)cn1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2c44211d2794451a9309e1c184ab987a
CN(CCCO)C(=O)OC(C)(C)C.CS(=O)(=O)Cl>>CN(CCCOS(C)(=O)=O)C(=O)OC(C)(C)C
OCCCN(C(OC(C)(C)C)=O)C.C(C)N(CC)CC.CS(=O)(=O)Cl.C(O)([O-])=O.[Na+]>>CS(=O)(=O)OCCCN(C)C(=O)OC(C)(C)C
[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][OH:6])[C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17].Cl[S:7]([CH3:8])(=[O:9])=[O:10]>>[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][O:6][S:7]([CH3:8])(=[O:9])=[O:10])[C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17]
CN(CCCO)C(=O)OC(C)(C)C.CS(=O)(=O)Cl
CN(CCCOS(C)(=O)=O)C(=O)OC(C)(C)C
null
null
C(C)(=O)OCC
Acylation
Formation of Sulfonic Esters
2fa969eb2c954bb96793348a1b2335ec63fbd290dadec6e3e02295e1768e64cf
cb77b899e4adf980b1def97230ef2861660fd7f9602260ec64747d9afd3a795a
null
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].[C:5]-[C:6]-[OH;D1;+0:7]>>[C:5]-[C:6]-[O;H0;D2;+0:7]-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4]
null
[]
null
null
2
HOUR
To a solution of tert-butyl N-(3-hydroxypropyl)-N-methylcarbamate (12.0 g) and triethylamine (11.5 ml) in ethyl acetate (300 ml), methanesulfonyl chloride (5.4 ml) was added under cooling with ice. After 2 hours' stirring, saturated aqueous sodium hydrogencarbonate solution was added to the reaction liquid and extracte...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Sulfonyl halide
Mesylate
null
null
null
HCl
C(C)(=O)OCC
null
2
CN(CCCO)C(=O)OC(C)(C)C.CS(=O)(=O)Cl>C(C)(=O)OCC>CN(CCCOS(C)(=O)=O)C(=O)OC(C)(C)C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2755bc43f82549f695ad2387daaac869
Fc1ccc(C2CCNCC2)cn1.O=C(O)C(c1ccc(F)c(F)c1)N1CCCC1=O.O=C(O)C(c1ccc(F)cc1)c1ccc(F)cc1>>CN(CCCN1CCC(c2ccc(F)nc2)CC1)C(=O)C(c1ccc(F)cc1)c1ccc(F)cc1
FC1=CC=C(C=C1)C(C(=O)O)C1=CC=C(C=C1)F.Cl.N1CCC2(CC1)OCC1=CC=CC=C12.FC1=CC=C(C=N1)C1CCNCC1.FC=1C=C(C=CC1F)C(C(=O)O)N1C(CCC1)=O>>FC1=CC=C(C=C1)C(C(=O)N(CCCN1CCC(CC1)C=1C=NC(=CC1)F)C)C1=CC=C(C=C1)F
[NH:6]1[CH2:7][CH2:8][CH:9]([c:10]2[cH:11][cH:12][c:13]([F:14])[n:15][cH:16]2)[CH2:17][CH2:18]1.O=C(O)C(c1ccc(F)c(F)c1)[N:2]1[C:1](=O)[CH2:5][CH2:4][CH2:3]1.O[C:19](=[O:20])[CH:21]([c:22]1[cH:23][cH:24][c:25]([F:26])[cH:27][cH:28]1)[c:29]1[cH:30][cH:31][c:32]([F:33])[cH:34][cH:35]1>>[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][N...
Fc1ccc(C2CCNCC2)cn1.O=C(O)C(c1ccc(F)c(F)c1)N1CCCC1=O.O=C(O)C(c1ccc(F)cc1)c1ccc(F)cc1
CN(CCCN1CCC(c2ccc(F)nc2)CC1)C(=O)C(c1ccc(F)cc1)c1ccc(F)cc1
null
null
null
Acylation
OtherReaction
6dc8ce944f8ef99676c344b9de2ea6b6a36d7d67e160d1bf4cc9aa1906ebb522
da1c8aee4e3057b85d770db5d4db0174050a94cbaf55234256b22869faf4b463
O=C(NCCCN1CCC(c2cccnc2)CC1)C(c1ccccc1)c1ccccc1
F-c1:c:c:c(-C(-C(-O)=O)-[N;H0;D3;+0:1]2-[C:2]-[C:3]-[CH2;D2;+0:4]-[C;H0;D3;+0:5]-2=O):c:c:1-F.O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[C:8](-[c:9])-[c:10].[C:11]-[C:12]-[NH;D2;+0:13]-[C:14]-[C:15]>>[C:11]-[C:12]-[N;H0;D3;+0:13](-[CH2;D2;+0:4]-[C:3]-[C:2]-[N;H0;D3;+0:1](-[CH3;D1;+0:5])-[C;H0;D3;+0:6](=[O;D1;H0:7])-[C:8](-[c:9])-...
null
[]
null
null
null
null
Example 9 was repeated except that spiro[isobenzofuran-1(3H), 4′-piperidine] hydrochloride which was used in Example 9-(2) was replaced with 4-(6-fluoro-3-pyridinyl)piperidine, and 2-(3,4-difluorophenyl)-2-(2-oxo-1-pyrrolidinyl)acetic acid which was used in Example 9-(4), with 2,2-bis(4-fluorophenyl)acetic acid, to pro...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Carboxylic acid.Carboxylic acid.Tertiary amide.Secondary amine
Tertiary amide.Tertiary amine
C1CCNCC1.c1ccccc1.C1CC[NH]C1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccncc1.c1ccccc1.c1ccccc1
HF
null
null
null
Fc1ccc(C2CCNCC2)cn1.O=C(O)C(c1ccc(F)c(F)c1)N1CCCC1=O.O=C(O)C(c1ccc(F)cc1)c1ccc(F)cc1>>CN(CCCN1CCC(c2ccc(F)nc2)CC1)C(=O)C(c1ccc(F)cc1)c1ccc(F)cc1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c64554637d384b8ca3dde17f86b2075e
Nc1ccc(Cl)nc1>>Nc1ccc(Cl)nc1I
C([O-])([O-])=O.[Ca+2].I(=O)(=O)Cl.I(=O)(=O)Cl.C(C1=CC=CC=C1)[N+](C)(C)C.NC=1C=CC(=NC1)Cl>>NC=1C(=NC(=CC1)Cl)I
[NH2:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[n:7][cH:8]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[n:7][c:8]1[I:9]
Nc1ccc(Cl)nc1
Nc1ccc(Cl)nc1I
null
null
ClCCl.CO
Functional Group Addition
Aromatic iodination
7c108e53aa6849672ac0ea1998cfd24df7835b0d1bc5738d16f4d561a472c88e
0a2f22058f27970cef4a98a778644dbe9c44e91f66c74cd24db321993177608a
c1ccncc1
[N;D1;H2:1]-[c:2](:[c:3]):[cH;D2;+0:4]:[#7;a:5]:[c:6]>>[I;D1;H0:7]-[c;H0;D3;+0:4](:[#7;a:5]:[c:6]):[c:2](-[N;D1;H2:1]):[c:3]
39.1
[{"value": 39.1, "product": "NC=1C(=NC(=CC1)Cl)I", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}, {"value": 30.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
23.2 g (180.5 mM) of 5-amino-2-chloropyridine are mixed in 70 ml of dichloro-methane (DCM) and 180 ml of methanol, and 21.6 g (216 mM) of calcium carbonate and 75.3 g (226 mM) of benzyltrimethylammonium dichloroiodate are added. The reaction mixture is stirred at room temperature for 16 hours, and then filtered to remo...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccncc1
c1ccncc1
c1ccncc1
Other
ClCCl.CO
null
16
Nc1ccc(Cl)nc1>ClCCl.CO>Nc1ccc(Cl)nc1I
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-d8ab2f2da6704ce983b0aa772fa77a07
II.Nc1ccc(C(F)(F)F)nc1>>Nc1ccc(C(F)(F)F)nc1I
NC=1C=CC(=NC1)C(F)(F)F.II>>NC=1C(=NC(=CC1)C(F)(F)F)I
I[I:12].[NH2:1][c:2]1[cH:3][cH:4][c:5]([C:6]([F:7])([F:8])[F:9])[n:10][cH:11]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([C:6]([F:7])([F:8])[F:9])[n:10][c:11]1[I:12]
II.Nc1ccc(C(F)(F)F)nc1
Nc1ccc(C(F)(F)F)nc1I
null
S(=O)(=O)([O-])[O-].[Ag+2]
C(C)O
Functional Group Interconversion
OtherReaction
66a492ff31bfcbb52d9a760416ba269a4cf5a439a6c2ca9c2c3a3ed0a750b974
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccncc1
I-[I;H0;D1;+0:1].[N;D1;H2:2]-[c:3](:[c:4]):[cH;D2;+0:5]:[#7;a:6]:[c:7]>>[I;H0;D1;+0:1]-[c;H0;D3;+0:5](:[#7;a:6]:[c:7]):[c:3](-[N;D1;H2:2]):[c:4]
96
[{"value": 96.0, "product": "NC=1C(=NC(=CC1)C(F)(F)F)I", "details": "PERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
3.85 g (12.3 mM) of silver sulfate are added, with stirring and at room temperature, to a solution of 2 g (12.3 mM) of 5-amino-2-(trifluoromethyl)pyridine in 100 ml of ethanol. 3.13 g of iodine are then added and the reaction mixture is stirred at room temperature for 24 hours. The solid in suspension in the medium is ...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccncc1
c1ccncc1
c1ccncc1
HI
S(=O)(=O)([O-])[O-].[Ag+2].C(C)O
null
24
II.Nc1ccc(C(F)(F)F)nc1>S(=O)(=O)([O-])[O-].[Ag+2].C(C)O>Nc1ccc(C(F)(F)F)nc1I
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-27352282c0af4dfbb16addeee00b36b0
BrBr.COc1ccc(N)cn1>>COc1ccc(N)c(Br)n1
BrBr.NC=1C=CC(=NC1)OC.C(C)(=O)[O-].[Na+].S(=S)(=O)([O-])[O-].[Na+].[Na+]>>NC=1C(=NC(=CC1)OC)Br
Br[Br:9].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH2:7])[cH:8][n:10]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH2:7])[c:8]([Br:9])[n:10]1
BrBr.COc1ccc(N)cn1
COc1ccc(N)c(Br)n1
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
66a492ff31bfcbb52d9a760416ba269a4cf5a439a6c2ca9c2c3a3ed0a750b974
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccncc1
Br-[Br;H0;D1;+0:1].[N;D1;H2:2]-[c:3](:[c:4]):[cH;D2;+0:5]:[#7;a:6]:[c:7]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:5](:[#7;a:6]:[c:7]):[c:3](-[N;D1;H2:2]):[c:4]
null
[]
null
null
null
null
A mixture of 1.83 g (14.7 mM) of 5-amino-2-methoxypyridine and 1.21 g (14.7 mM) of sodium acetate in 12 ml of acetic acid is prepared and 0.75 ml (14.7 mM) of bromine is added gently, with stirring and while maintaining at room temperature. The reaction mixture is kept stirring for 30 minutes, at room temperature, and ...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccncc1
c1ccncc1
c1ccncc1
HBr
C(C)(=O)O
null
null
BrBr.COc1ccc(N)cn1>C(C)(=O)O>COc1ccc(N)c(Br)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-547db05fcb5b4d15ad1859b271b0aa20
Cc1ccc(N)c(Br)n1.O=S(=O)(Cl)c1ccc2ncsc2c1>>Cc1ccc(NS(=O)(=O)c2ccc3ncsc3c2)c(Br)n1
NC=1C(=NC(=CC1)C)Br.S1C=NC2=C1C=C(C=C2)S(=O)(=O)Cl>>BrC1=NC(=CC=C1NS(=O)(=O)C1=CC2=C(N=CS2)C=C1)C
[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH2:6])[c:19]([Br:20])[n:21]1.Cl[S:7](=[O:8])(=[O:9])[c:10]1[cH:11][cH:12][c:13]2[n:14][cH:15][s:16][c:17]2[cH:18]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH:6][S:7](=[O:8])(=[O:9])[c:10]2[cH:11][cH:12][c:13]3[n:14][cH:15][s:16][c:17]3[cH:18]2)[c:19]([Br:20])[n:21]1
Cc1ccc(N)c(Br)n1.O=S(=O)(Cl)c1ccc2ncsc2c1
Cc1ccc(NS(=O)(=O)c2ccc3ncsc3c2)c(Br)n1
null
null
null
Miscellaneous
Sulfonamide synthesis (Schotten-Baumann) primary amine
a86b0632821e188c0a5dc5a5a2aac298ab3eccaee8a52ba46078c3d5975a290d
50f8fbf3d327483c3eeff8f6cbd4065e4c7600bb501fbe08958a5c79a0926428
O=S(=O)(Nc1cccnc1)c1ccc2ncsc2c1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[c:7]:[#16;a:8].[Br;D1;H0:9]-[c:10](:[#7;a:11]:[c:12]):[c:13](-[NH2;D1;+0:14]):[c:15]>>[#16;a:8]:[c:7]:[c:6]:[c:4](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[NH;D2;+0:14]-[c:13](:[c:15]):[c:10](-[Br;D1;H0:9]):[#7;a:11]:[c:12]):[c:5]
35
[{"value": 35.0, "product": "BrC1=NC(=CC=C1NS(=O)(=O)C1=CC2=C(N=CS2)C=C1)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By working in a manner similar to that of Preparation VII, starting with 3-amino-2-bromo-6-methylpyridine and 6-benzothiazolesulfonyl chloride, the expected product is obtained in the form of a beige-colored paste (yield=35%). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccncc1.c1ccc2scnc2c1
HCl
null
null
null
Cc1ccc(N)c(Br)n1.O=S(=O)(Cl)c1ccc2ncsc2c1>>Cc1ccc(NS(=O)(=O)c2ccc3ncsc3c2)c(Br)n1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-45295142de3d4273a02e51470b6ed47e
Nc1ccc(Cl)nc1I.O=S(=O)(Cl)c1ccc2ncsc2c1>>O=S(=O)(Nc1ccc(Cl)nc1I)c1ccc2ncsc2c1
NC=1C(=NC(=CC1)Cl)I.S1C=NC2=C1C=C(C=C2)S(=O)(=O)Cl>>IC1=NC(=CC=C1NS(=O)(=O)C1=CC2=C(N=CS2)C=C1)Cl
[NH2:4][c:5]1[cH:6][cH:7][c:8]([Cl:9])[n:10][c:11]1[I:12].Cl[S:2](=[O:1])(=[O:3])[c:13]1[cH:14][cH:15][c:16]2[n:17][cH:18][s:19][c:20]2[cH:21]1>>[O:1]=[S:2](=[O:3])([NH:4][c:5]1[cH:6][cH:7][c:8]([Cl:9])[n:10][c:11]1[I:12])[c:13]1[cH:14][cH:15][c:16]2[n:17][cH:18][s:19][c:20]2[cH:21]1
Nc1ccc(Cl)nc1I.O=S(=O)(Cl)c1ccc2ncsc2c1
O=S(=O)(Nc1ccc(Cl)nc1I)c1ccc2ncsc2c1
null
null
null
Miscellaneous
Sulfonamide synthesis (Schotten-Baumann) primary amine
a86b0632821e188c0a5dc5a5a2aac298ab3eccaee8a52ba46078c3d5975a290d
50f8fbf3d327483c3eeff8f6cbd4065e4c7600bb501fbe08958a5c79a0926428
O=S(=O)(Nc1cccnc1)c1ccc2ncsc2c1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[c:7]:[#16;a:8].[I;D1;H0:9]-[c:10](:[#7;a:11]:[c:12]):[c:13](-[NH2;D1;+0:14]):[c:15]>>[#16;a:8]:[c:7]:[c:6]:[c:4](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[NH;D2;+0:14]-[c:13](:[c:15]):[c:10](-[I;D1;H0:9]):[#7;a:11]:[c:12]):[c:5]
33
[{"value": 33.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By working in a manner similar to that of Example 50, starting with 3-amino-2-iodo-6-chloropyridine and 6-benzothiazolesulfonyl chloride, the expected product is obtained in the form of an orange-colored solid (yield=33%). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccncc1.c1ccc2scnc2c1
HCl
null
null
null
Nc1ccc(Cl)nc1I.O=S(=O)(Cl)c1ccc2ncsc2c1>>O=S(=O)(Nc1ccc(Cl)nc1I)c1ccc2ncsc2c1
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-cdfec3e05fd34f118eb29ce450fe758e
CC1(C)NCc2ccccc2O1>>CC(C)Nc1ccccc1CO
CC1(OC2=C(CN1)C=CC=C2)C.C1CCOC1.[H-].[H-].[H-].[H-].[Li+].[Al+3].C1CCOC1>>C(C)(C)NC1=C(C=CC=C1)CO
[CH3:1][C:2]1([CH3:3])[NH:4][CH2:11][c:10]2[c:5]([cH:6][cH:7][cH:8][cH:9]2)[O:12]1>>[CH3:1][CH:2]([CH3:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[CH2:11][OH:12]
CC1(C)NCc2ccccc2O1
CC(C)Nc1ccccc1CO
null
null
null
Miscellaneous
OtherReaction
bf0fd08faea41f249ad245c627ae5eaa44305b733aa8f021166c9982d83d6e4c
6731e713966699a550554bf52935dfe7a2b2eb2cafc83e524d2ff6fcc59af15d
c1ccccc1
[C;D1;H3:1]-[C;H0;D4;+0:2]1(-[C;D1;H3:3])-[NH;D2;+0:4]-[CH2;D2;+0:5]-[c:6](:[c:7]):[c;H0;D3;+0:8](:[c:9]:[c:10])-[O;H0;D2;+0:11]-1>>[C;D1;H3:1]-[CH;D3;+0:2](-[C;D1;H3:3])-[NH;D2;+0:4]-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:6](-[CH2;D2;+0:5]-[OH;D1;+0:11]):[c:7]
95
[{"value": 95.0, "product": "C(C)(C)NC1=C(C=CC=C1)CO", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of 2,2-dimethyl-1,4-dihydro-2H-benzo[1,3]oxazine (125 g, 0.77 mol) in THF (1 L) was filtered through a scintillation funnel and then added dropwise via an addition funnel, over a period of 2.5 h, to a stirred solution of 1.0 M LiAlH4 in THF (800 mL) at 0° C. The reaction was quenched by slow portionwise addi...
10.6084/m9.figshare.5104873.v1
null
Ether.Secondary amine
Primary alcohol.Secondary amine
c1ccc2c(c1)CNCO2
c1ccccc1
c1ccccc1
null
null
null
8
CC1(C)NCc2ccccc2O1>>CC(C)Nc1ccccc1CO
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-cf4a38b7d8274eeea2920ed5a8e9106a
CC(C)Nc1ccccc1CO>>CC(C)Nc1ccccc1C=O
C(C)(C)NC1=C(C=CC=C1)CO>>C(C)(C)NC1=C(C=O)C=CC=C1
[CH3:1][CH:2]([CH3:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[CH2:11][OH:12]>>[CH3:1][CH:2]([CH3:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[CH:11]=[O:12]
CC(C)Nc1ccccc1CO
CC(C)Nc1ccccc1C=O
null
[O-2].[O-2].[Mn+4]
C1(=CC=CC=C1)C
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccccc1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]
90.6
[{"value": 90.0, "product": "C(C)(C)NC1=C(C=O)C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.6, "product": "C(C)(C)NC1=C(C=O)C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
117
CELSIUS
null
null
Manganese dioxide (85% 182.6 g, 1.79 mol) was added to a stirred solution of 2-isopropylaminophenylmethanol (118 g, 0.71 mol) in toluene (800 mL) and the reaction mixture was heated to 117° C. for 4 h. The reaction mixture was allowed to cool to room temperature overnight and then filtered through a pad of Celite which...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccccc1
null
[O-2].[O-2].[Mn+4].C1(=CC=CC=C1)C
117
null
CC(C)Nc1ccccc1CO>[O-2].[O-2].[Mn+4].C1(=CC=CC=C1)C>CC(C)Nc1ccccc1C=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-9b73b2020f5846258bd4e50f40a5b179
CC(C)Nc1ccccc1C=O.CC1(C)OC(=O)CC(=O)O1>>CC(C)n1c(=O)c(C(=O)O)cc2ccccc21
CC1(OC(CC(O1)=O)=O)C.CC1(OC(=O)CC(=O)O1)C.C(C)(C)NC1=C(C=O)C=CC=C1.C(C)(=O)O.C(CN)N>>C(C)(C)N1C(C(=CC2=CC=CC=C12)C(=O)O)=O
O=[CH:11][c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[NH:4][CH:2]([CH3:1])[CH3:3].CC1(C)O[C:5](=[O:6])[CH2:7][C:8](=[O:9])[O:10]1>>[CH3:1][CH:2]([CH3:3])[n:4]1[c:5](=[O:6])[c:7]([C:8](=[O:9])[OH:10])[cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]12
CC(C)Nc1ccccc1C=O.CC1(C)OC(=O)CC(=O)O1
CC(C)n1c(=O)c(C(=O)O)cc2ccccc21
null
null
CO
Miscellaneous
OtherReaction
7da7c8932064b44b257d05fda8b8362a79f28b679166e64d691318db6946232e
ddbf93ce274a07b125aec0b5e9bfc602f13d41e2bbc449e0d8b2eac033b184d0
O=c1ccc2ccccc2[nH]1
C-C1(-C)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH2;D2;+0:3]-[C:4](=[O;D1;H0:5])-[O;H0;D2;+0:6]-1.O=[CH;D2;+0:7]-[c:8](:[c:9]):[c:10](-[NH;D2;+0:11]-[C:12](-[C;D1;H3:13])-[C;D1;H3:14]):[c:15]>>[C;D1;H3:13]-[C:12](-[C;D1;H3:14])-[n;H0;D3;+0:11]1:[c:10](:[c:15]):[c:8](:[c:9]):[cH;D2;+0:7]:[c;H0;D3;+0:3](-[C:4](=[O;D1;H0:5])-[OH...
98
[{"value": 98.0, "product": "C(C)(C)N1C(C(=CC2=CC=CC=C12)C(=O)O)=O", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
2,2-Dimethyl-[1,3]dioxane-4,6-dione, commonly Meldrum's acid, (166.9 g, 1.16 mol) was added to a stirred solution of 2-isopropylaminobenzaldehyde (105 g, 0.64 mol), acetic acid (73.6 mL, 1.29 mol) and ethylenediamine (43.0 mL, 0.64 mol) in methanol (1 L) at 0° C. The reaction mixture was stirred for 1 h at 0° C. and th...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Ester.Ester.Secondary amine
Carboxylic acid
c1ccccc1.C1COCOC1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HO-
CO
0
1
CC(C)Nc1ccccc1C=O.CC1(C)OC(=O)CC(=O)O1>CO>CC(C)n1c(=O)c(C(=O)O)cc2ccccc21
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-520e1e20a5b74d83883664866993db0e
COC(=O)[C@@H]1C[C@H](OC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C>>COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
CC(=O)O[C@H]1C[C@H]([C@@]2(CC[C@H]3C(=O)O[C@@H](C[C@@]3([C@H]2C1=O)C)C=4C=COC4)C)C(=O)OC.C(=O)([O-])[O-].[Na+].[Na+]>>COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C
CC(=O)[O:8][C@H:7]1[CH2:6][C@@H:5]([C:3]([O:2][CH3:1])=[O:4])[C@@:27]2([CH3:28])[C@H:11]([C:9]1=[O:10])[C@@:12]1([CH3:13])[CH2:14][C@@H:15]([c:16]3[cH:17][cH:18][o:19][cH:20]3)[O:21][C:22](=[O:23])[C@@H:24]1[CH2:25][CH2:26]2>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:9](=[O:10])[C@@H:11]2[C@@:12]3([CH3...
COC(=O)[C@@H]1C[C@H](OC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
null
null
CO
Reduction
Hydrolysis or Hydrogenolysis of Carboxylic Esters or Thioesters
d7acfb2397f2b5b2a83b3bebf3698d6d984dd716982297f62a944222c79ce234
19dd58e0f83625e74b4b1375d88cb4c813ee60f593d812516d14eafc4ab68dc7
O=C1CCCC2CC[C@@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
C-C(=O)-[O;H0;D2;+0:1]-[C:2](-[C:3])-[C:4](=[O;D1;H0:5])-[C:6]>>[C:6]-[C:4](=[O;D1;H0:5])-[C:2](-[OH;D1;+0:1])-[C:3]
77
[{"value": 77.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.8, "product": "COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C", "details": "CALCULATEDPERCENTYIELD", "...
null
null
null
null
A mixture of 1 (3.5 g, 8.0 mmol) and Na2CO3 (3.4 g, 32.2 mmol) in absolute MeOH (150 mL) was stirred at room temperature for 4 b. The solvent was removed under reduced pressure and CH2Cl2 (500 mL) was added to the crude residue. The organic extract was washed successively with 2N HCl (50 mL) and saturated NaCl (50 mL) ...
10.6084/m9.figshare.5104873.v1
null
Ester
Secondary alcohol
null
null
c1ccoc1.C1CC[C@H]2[C@H](C1)CC[C@@H]1COCC[C@@H]12
HO-
CO
null
null
COC(=O)[C@@H]1C[C@H](OC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C>CO>COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-8cf51e6dc1724239bb5526d1cc06716b
CC(C)C(=O)Cl.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C>>COC(=O)[C@@H]1C[C@H](OC(=O)C(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
C(C(C)C)(=O)Cl.C(CC)(=O)OC(CC)=O.COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C(C)C)=O)=O)C)C1=COC=C1)=O)C
Cl[C:9](=[O:10])[CH:11]([CH3:12])[CH3:13].[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:14](=[O:15])[C@H:16]2[C@@:17]1([CH3:18])[CH2:19][CH2:20][C@@H:21]1[C:22](=[O:23])[O:24][C@H:25]([c:26]3[cH:27][cH:28][o:29][cH:30]3)[CH2:31][C@:32]21[CH3:33]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([O:8][C:9](...
CC(C)C(=O)Cl.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
COC(=O)[C@@H]1C[C@H](OC(=O)C(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
null
null
Protection
Schotten-Baumann to ester
0ff6f452f545c5714d297592668645b2f1aab4c7ba249a3331b014e41dc6881c
96f6d8bed38830913bc384a75a5a9e04ad1b99b6be7c7e9d85b6ecc9049f5127
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[C;D1;H3:5].[C:6]-[C:7](=[O;D1;H0:8])-[C:9](-[OH;D1;+0:10])-[C:11]>>[C:6]-[C:7](=[O;D1;H0:8])-[C:9](-[O;H0;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[C;D1;H3:5])-[C:11]
62
[{"value": 62.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C(C)C)=O)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure similar to that described in Example 4 except replacing the propionic anhydride used therein with the requisite anhydride, the title compound 10 (0.04 g, 62%) was prepared as a white solid, mp 209-211° C.; 10 was synthesized as described for 9 from 8a using isobutyryl chloride to afford 0.04 g (62%) o...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HCl
null
null
null
CC(C)C(=O)Cl.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C>>COC(=O)[C@@H]1C[C@H](OC(=O)C(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-9700a765425b427197d058b4d8da3fd1
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C(Cl)c1ccccc1>>COC(=O)[C@@H]1C[C@H](OC(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C.C(C1=CC=CC=C1)(=O)Cl.CO>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C1=CC=CC=C1)=O)=O)C)C1=COC=C1)=O)C
[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:17](=[O:18])[C@H:19]2[C@@:20]1([CH3:21])[CH2:22][CH2:23][C@@H:24]1[C:25](=[O:26])[O:27][C@H:28]([c:29]3[cH:30][cH:31][o:32][cH:33]3)[CH2:34][C@:35]21[CH3:36].Cl[C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][...
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C(Cl)c1ccccc1
COC(=O)[C@@H]1C[C@H](OC(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
O=C(O[C@H]1CCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@H]2C1=O)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7](=[O;D1;H0:8])-[C:9](-[OH;D1;+0:10])-[C:11]>>[C:6]-[C:7](=[O;D1;H0:8])-[C:9](-[O;H0;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:11]
98
[{"value": 98.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C1=CC=CC=C1)=O)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.3, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C1=CC=CC=C1)=O)=O)C)C1=COC=C1)=O)C", "details...
null
null
null
null
A solution of 8a (0.05 g, 0.13 mmol), benzoyl chloride (0.09 g, 0.92 mmol) and a catalytic amount of DMAP in CH2Cl2 (20 mL) was stirred at room temperature for 2 h. Absolute MeOH (15 mL) was added and the solvent was removed under reduced pressure. CH2Cl2 (25 mL) was added to the residue and the solution was washed wit...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
c1ccccc1.C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HCl
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
null
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C(Cl)c1ccccc1>CN(C)C=1C=CN=CC1.C(Cl)Cl>COC(=O)[C@@H]1C[C@H](OC(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-d9a5df717c8f4c4e9915b036f94d0c9a
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.CS(=O)(=O)Cl>>COC(=O)[C@@H]1C[C@H](OS(C)(=O)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C.CS(=O)(=O)Cl.CCN(CC)CC>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OS(=O)(=O)C)=O)C)C1=COC=C1)=O)C
[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:13](=[O:14])[C@H:15]2[C@@:16]1([CH3:17])[CH2:18][CH2:19][C@@H:20]1[C:21](=[O:22])[O:23][C@H:24]([c:25]3[cH:26][cH:27][o:28][cH:29]3)[CH2:30][C@:31]21[CH3:32].Cl[S:9]([CH3:10])(=[O:11])=[O:12]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([O:8][S:9]([CH3:10]...
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.CS(=O)(=O)Cl
COC(=O)[C@@H]1C[C@H](OS(C)(=O)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
null
C(Cl)Cl
Acylation
Formation of Sulfonic Esters
641955d0081c80f158ce2aacd31873a3f3301c87ca0800cf263e288ba8390217
4f9373df8a11470603daf885a5777cebf95940370e32739263d35df0f171a0dd
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].[C:5]-[C:6](=[O;D1;H0:7])-[C:8](-[OH;D1;+0:9])-[C:10]>>[C:5]-[C:6](=[O;D1;H0:7])-[C:8](-[O;H0;D2;+0:9]-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4])-[C:10]
32
[{"value": 32.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OS(=O)(=O)C)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 8a (0.05 g, 0.13 mmol), methanesulfonyl chloride (1 mL) and NEt3 (2 mL) in CH2Cl2 (30 mL) was stirred at room temperature overnight and then the mixture was washed with saturated NaHCO3 (20 mL) and saturated NaCl (2×15 mL) and dried (Na2SO4). The solvent was removed under reduced pressure. The resulting c...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol.Sulfonyl halide
Mesylate
null
null
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HCl
C(Cl)Cl
null
null
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.CS(=O)(=O)Cl>C(Cl)Cl>COC(=O)[C@@H]1C[C@H](OS(C)(=O)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-7caa50fd5b074b9d813eca73504ee6f7
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.C[Si](C)(C)Cl>>COC(=O)[C@@H]1C[C@H](O[Si](C)(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C.CCN(CC)CC.Cl[Si](C)(C)C>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O[Si](C)(C)C)=O)C)C1=COC=C1)=O)C
[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:13](=[O:14])[C@H:15]2[C@@:16]1([CH3:17])[CH2:18][CH2:19][C@@H:20]1[C:21](=[O:22])[O:23][C@H:24]([c:25]3[cH:26][cH:27][o:28][cH:29]3)[CH2:30][C@:31]21[CH3:32].Cl[Si:9]([CH3:10])([CH3:11])[CH3:12]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([O:8][Si:9]([CH3...
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.C[Si](C)(C)Cl
COC(=O)[C@@H]1C[C@H](O[Si](C)(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
null
C(Cl)Cl
Protection
Alcohol protection with silyl ethers
ea139b3cb6171a748fbc881d815cc598a14c6b8245b87168b4a15a10e325f24c
1e2a25dd539d267852f3b05b92dd4080ece1d4c7abb9db1b6fd2b64d2b33a864
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C;D1;H3:4].[C:5]-[C:6](=[O;D1;H0:7])-[C:8](-[OH;D1;+0:9])-[C:10]>>[C:5]-[C:6](=[O;D1;H0:7])-[C:8](-[O;H0;D2;+0:9]-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C;D1;H3:4])-[C:10]
68
[{"value": 68.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O[Si](C)(C)C)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 64.8, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O[Si](C)(C)C)=O)C)C1=COC=C1)=O)C", "details": "CALCUL...
null
null
null
null
A solution of 8a (0.08 g, 0.20 mmol), NEt3 (0.1 mL, 0.72 mmol) and chlorotrimethylsilane (0.1 mL, 0.79 mmol) in CH2Cl2 (30 mL) was stirred at room temperature overnight. The mixture was washed with saturated NaHCO3 (2×10 mL) and H20 (50 mL), dried (Na2SO4), and the solvent was removed under reduced pressure. The result...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol.Silyl protective group
Silyl protective group
null
null
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HCl
C(Cl)Cl
null
null
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.C[Si](C)(C)Cl>C(Cl)Cl>COC(=O)[C@@H]1C[C@H](O[Si](C)(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-aa8df4840fe94da7921b80707f1ba252
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.N#CC(Cl)(Cl)Cl>>COC(=O)[C@@H]1C[C@H](OC(=N)C(Cl)(Cl)Cl)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C.ClC(C#N)(Cl)Cl>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C(Cl)(Cl)Cl)=N)=O)C)C1=COC=C1)=O)C
[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:15](=[O:16])[C@H:17]2[C@@:18]1([CH3:19])[CH2:20][CH2:21][C@@H:22]1[C:23](=[O:24])[O:25][C@H:26]([c:27]3[cH:28][cH:29][o:30][cH:31]3)[CH2:32][C@:33]21[CH3:34].[C:9](#[N:10])[C:11]([Cl:12])([Cl:13])[Cl:14]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([O:8][C...
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.N#CC(Cl)(Cl)Cl
COC(=O)[C@@H]1C[C@H](OC(=N)C(Cl)(Cl)Cl)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
null
ClC(C)Cl
Acylation
OtherReaction
8045d30783d505e653fcb6064f74ac59e775d4240e5a26759512143eefde6598
2554d984b82cd13e50d59270df17cf414095f213aef52eb5729ce2a3821b08e4
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
[C:1]-[C:2](=[O;D1;H0:3])-[C:4](-[OH;D1;+0:5])-[C:6].[Cl;D1;H0:7]-[C:8](-[Cl;D1;H0:9])(-[Cl;D1;H0:10])-[C;H0;D2;+0:11]#[N;H0;D1;+0:12]>>[C:1]-[C:2](=[O;D1;H0:3])-[C:4](-[O;H0;D2;+0:5]-[C;H0;D3;+0:11](=[NH;D1;+0:12])-[C:8](-[Cl;D1;H0:7])(-[Cl;D1;H0:9])-[Cl;D1;H0:10])-[C:6]
37
[{"value": 37.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C(Cl)(Cl)Cl)=N)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 28.8, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C(Cl)(Cl)Cl)=N)=O)C)C1=COC=C1)=O)C", "details...
null
null
null
null
A solution of 8a (0.05 g, 0.13 mmol), trichloroacetonitrile (0.1 mL, 1.0 mmol), 1,8-Diazobicylo[5.4.0]undec-7-ene (0.05 mL, 0.3 mmol) in dichloroethane (20 mL) was stirred at 0° C. for 24 h. The reaction mixture was then washed with saturated NaHCO3 (10 mL) and H2O (10 mL) and dried (Na2SO4). The solvent was removed un...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Secondary alcohol
Ether
null
null
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
null
ClC(C)Cl
null
null
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.N#CC(Cl)(Cl)Cl>ClC(C)Cl>COC(=O)[C@@H]1C[C@H](OC(=N)C(Cl)(Cl)Cl)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-9edfd93c7b884bb8a336fb912c356863
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C=Nc1ccccc1>>COC(=O)[C@@H]1C[C@H](OC(=O)Nc2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C.C[Si](C)(C)Cl.C1(=CC=CC=C1)N=C=O>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(NC1=CC=CC=C1)=O)=O)C)C1=COC=C1)=O)C
[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:18](=[O:19])[C@H:20]2[C@@:21]1([CH3:22])[CH2:23][CH2:24][C@@H:25]1[C:26](=[O:27])[O:28][C@H:29]([c:30]3[cH:31][cH:32][o:33][cH:34]3)[CH2:35][C@:36]21[CH3:37].[C:9](=[O:10])=[N:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH...
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C=Nc1ccccc1
COC(=O)[C@@H]1C[C@H](OC(=O)Nc2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
null
C(Cl)Cl
Protection
OtherReaction
c9b35f80646c04bc8fccaa97f413140cb97715d748dadcda1fae2c6d3c1b477c
cbb53c7ae1c600f566fbe6a1a5d75bfb802798fe2863db2e91856277c64ee7ca
O=C(Nc1ccccc1)O[C@H]1CCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@H]2C1=O
[C:1]-[C:2](=[O;D1;H0:3])-[C:4](-[OH;D1;+0:5])-[C:6].[O;D1;H0:7]=[C;H0;D2;+0:8]=[N;H0;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[C:1]-[C:2](=[O;D1;H0:3])-[C:4](-[O;H0;D2;+0:5]-[C;H0;D3;+0:8](=[O;D1;H0:7])-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[C:6]
14
[{"value": 14.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(NC1=CC=CC=C1)=O)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 14.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(NC1=CC=CC=C1)=O)=O)C)C1=COC=C1)=O)C", "detai...
null
null
null
null
A solution of 8a (0.06 g, 0.14 mmol), trimethylsilyl chloride (0.01 mL, 0.08 mmol) and phenylisocyanate (0.1 mL, 0.92 mmol) in CH2Cl2 was stirred at room temperature for 5 days. The reaction mixture was then washed with saturated NaHCO3 (10 mL) and H2O (10 mL) and dried (Na2SO4). The solvent was removed under reduced p...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Secondary alcohol
Carbamic ester
null
null
c1ccccc1.C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
null
C(Cl)Cl
null
null
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C=Nc1ccccc1>C(Cl)Cl>COC(=O)[C@@H]1C[C@H](OC(=O)Nc2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f9598e26fdd74eaabb3e1d58e0618d41
CC(=O)O.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C>>COC(=O)[C@@H]1C[C@H](OC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
CC(C)(C)OC(=O)/N=N/C(=O)OC(C)(C)C.COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C.C1(=CC=CC=C1)P(C1=NC=CC=C1)C1=CC=CC=C1.C(C)(=O)O>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C)=O)=O)C)C1=COC=C1)=O)C
O[C:9]([CH3:10])=[O:11].[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:12](=[O:13])[C@H:14]2[C@@:15]1([CH3:16])[CH2:17][CH2:18][C@@H:19]1[C:20](=[O:21])[O:22][C@H:23]([c:24]3[cH:25][cH:26][o:27][cH:28]3)[CH2:29][C@:30]21[CH3:31]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([O:8][C:9]([CH3:10])=[O:11])[...
CC(=O)O.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
COC(=O)[C@@H]1C[C@H](OC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
null
ClCCl.C1CCOC1
Acylation
Esterification of Carboxylic Acids
e916c5b009194e30c618975b40d7a233bfcf81339e65494c4e365f67cc5e011d
12ba7405a548c6b1674f05065819c74f53f1b6165cd54e84e1f2f208042fe660
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](=[O;D1;H0:6])-[C:7](-[OH;D1;+0:8])-[C:9]>>[C:4]-[C:5](=[O;D1;H0:6])-[C:7](-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[C:9]
81.6
[{"value": 80.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C)=O)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.6, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C)=O)=O)C)C1=COC=C1)=O)C", "details": "CALCULATEDPERCEN...
60
CELSIUS
18
HOUR
A mixture of 8a (0.20 g, 0.51 mmol), diphenyl-2-pyridylphosphine (0.20 g, 0.77 mmol) and acetic acid (0.12 mL, 2.05 mmol) was dissolved in anhydrous THF (15 mL) under an argon atmosphere. To this solution was added di-tert-butylazodicarboxylate (DBAD) (0.18 g, 0.77 mmol) in one portion and the mixture was stirred for 1...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary alcohol
Ester
null
null
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HO-
ClCCl.C1CCOC1
60
18
CC(=O)O.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C>ClCCl.C1CCOC1>COC(=O)[C@@H]1C[C@H](OC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-7c61a93160c64737938cc31ec6c2a77d
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C(O)c1ccccc1>>COC(=O)[C@@H]1C[C@H](OC(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C.C(C1=CC=CC=C1)(=O)O>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C1=CC=CC=C1)=O)=O)C)C1=COC=C1)=O)C
[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([OH:8])[C:17](=[O:18])[C@H:19]2[C@@:20]1([CH3:21])[CH2:22][CH2:23][C@@H:24]1[C:25](=[O:26])[O:27][C@H:28]([c:29]3[cH:30][cH:31][o:32][cH:33]3)[CH2:34][C@:35]21[CH3:36].O[C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C...
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C(O)c1ccccc1
COC(=O)[C@@H]1C[C@H](OC(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
null
null
Acylation
Esterification of Carboxylic Acids
e916c5b009194e30c618975b40d7a233bfcf81339e65494c4e365f67cc5e011d
12ba7405a548c6b1674f05065819c74f53f1b6165cd54e84e1f2f208042fe660
O=C(O[C@H]1CCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@H]2C1=O)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7](=[O;D1;H0:8])-[C:9](-[OH;D1;+0:10])-[C:11]>>[C:6]-[C:7](=[O;D1;H0:8])-[C:9](-[O;H0;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:11]
75
[{"value": 75.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C1=CC=CC=C1)=O)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Compound 35 was synthesized using a procedure similar to that described in Example 29 from 8a using benzoic acid to afford 0.19 g (75%) of 35 as a white crystalline solid, mp 223-225° C.; 1H NMR (CDCl3): δ 1.13 (3H, s); 1.40 (1H, dd, J=11.6, 13.1); 1.50 (3H, s); 1.64 (2H, m); 1.84 (1H, dd, J=2.9, 11.3); 2.10 (2H, m); 2...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary alcohol
Ester
null
null
c1ccccc1.C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HO-
null
null
null
COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.O=C(O)c1ccccc1>>COC(=O)[C@@H]1C[C@H](OC(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f9487c4143a64edc9e1870c4f003f434
BrC(Br)Br.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C>>COC(=O)[C@@H]1C[C@@H](Br)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)O)=O)C)C1=COC=C1)=O)C.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(Br)(Br)Br.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(Br)(Br)Br>>COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@@H](C1)Br)=O)C)C1=COC=C1)=O)C
BrC(Br)[Br:8].O[C@H:7]1[CH2:6][C@@H:5]([C:3]([O:2][CH3:1])=[O:4])[C@@:27]2([CH3:28])[C@H:11]([C:9]1=[O:10])[C@@:12]1([CH3:13])[CH2:14][C@@H:15]([c:16]3[cH:17][cH:18][o:19][cH:20]3)[O:21][C:22](=[O:23])[C@H:24]1[CH2:25][CH2:26]2>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@@H:7]([Br:8])[C:9](=[O:10])[C@@H:11]2[C@@:12]3(...
BrC(Br)Br.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
COC(=O)[C@@H]1C[C@@H](Br)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
null
null
C(Cl)Cl
Functional Group Interconversion
OtherReaction
faceb3c80d4ce343366ddb6496c95727c0909c094053a92f52456100c2b3c591
565bfd67b81973146f8f155d2d66b870454c4c44b79e27e96b8183d7d581cec0
O=C1CCCC2CC[C@@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
Br-C(-Br)-[Br;H0;D1;+0:1].O-[C@@H;D3;+0:2](-[C:3]-[C:4]-[C:5](-[#8:6])=[O;D1;H0:7])-[C:8](=[O;D1;H0:9])-[C:10]>>[#8:6]-[C:5](=[O;D1;H0:7])-[C:4]-[C:3]-[C@@H;D3;+0:2](-[Br;H0;D1;+0:1])-[C:8](=[O;D1;H0:9])-[C:10]
59
[{"value": 59.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@@H](C1)Br)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 58.1, "product": "COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@@H](C1)Br)=O)C)C1=COC=C1)=O)C", "details": "CALCULATEDPERCENTYIELD...
null
null
8
HOUR
A mixture of salvinorin B (8a) (0.15 g, 0.38 mmol), triphenylphosphine (0.21 g, 0.80 mmol), and bromoform (0.15 g, 0.45 mmol) in CH2Cl2 (30 mL) was stirred at room temperature overnight. TLC indicated that starting material was still present after 16 h, thus additional triphenylphosphine (0.11 g, 0.42 mmol) and bromofo...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Secondary halide.Secondary halide.Ketone.Secondary alcohol
Secondary halide
C1CC[C@H]2[C@H](C1)CC[C@@H]1COCC[C@@H]12
C1CC[C@H]2[C@H](C1)CC[C@@H]1COCC[C@@H]12
c1ccoc1.C1CC[C@H]2[C@H](C1)CC[C@@H]1COCC[C@@H]12
HBr
C(Cl)Cl
null
8
BrC(Br)Br.COC(=O)[C@@H]1C[C@H](O)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C>C(Cl)Cl>COC(=O)[C@@H]1C[C@@H](Br)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-1fe8c4491a6241759a422c3930951f7d
COC(=O)[C@@H]1C[C@@H](Br)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.[N-]=[N+]=[N-]>>COC(=O)[C@@H]1C[C@H](N=[N+]=[N-])C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
O.COC(=O)[C@H]1[C@@]2(CC[C@@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@@H](C1)Br)=O)C)C1=COC=C1)=O)C.[N-]=[N+]=[N-].[Na+].C(C)(=O)O>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N=[N+]=[N-])=O)C)C1=COC=C1)=O)C
Br[C@@H:7]1[CH2:6][C@@H:5]([C:3]([O:2][CH3:1])=[O:4])[C@@:14]2([CH3:15])[C@H:13]([C:11]1=[O:12])[C@:29]1([CH3:30])[C@H:18]([CH2:17][CH2:16]2)[C:19](=[O:20])[O:21][C@H:22]([c:23]2[cH:24][cH:25][o:26][cH:27]2)[CH2:28]1.[N-:8]=[N+:9]=[N-:10]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([N:8]=[N+:9]=[N-:10])[C:11](=[O...
COC(=O)[C@@H]1C[C@@H](Br)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.[N-]=[N+]=[N-]
COC(=O)[C@@H]1C[C@H](N=[N+]=[N-])C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
5c7109810c945939d2c8c3302f0b4dcb4495586c0a1c6b415a157c3d514ead82
06e32b8fc344f03e708f534c933054eeeb8596bf07b6161997913435e8cd3859
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
Br-[C@H;D3;+0:1](-[C:2]-[C:3]-[C:4](-[#8:5])=[O;D1;H0:6])-[C:7](=[O;D1;H0:8])-[C:9].[N-;H0;D1:10]=[#7;+:11]=[N;-;D1;H0:12]>>[#8:5]-[C:4](=[O;D1;H0:6])-[C:3]-[C:2]-[C@H;D3;+0:1](-[N;H0;D2;+0:10]=[#7;+:11]=[N;-;D1;H0:12])-[C:7](=[O;D1;H0:8])-[C:9]
87.5
[{"value": 86.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N=[N+]=[N-])=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.5, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N=[N+]=[N-])=O)C)C1=COC=C1)=O)C", "details": "CALCULAT...
null
null
null
null
A solution of 36 (0.10 g, 0.22 mmol), sodium azide (0.05 g, 0.77 mmol) and glacial acetic acid in DMF (3 mL) was stirred at room temperature for 4 h. H2O (30 mL) was added and the mixture was extracted with EtOAc (20 mL). The EtOAc solution was washed with H2O (2×20 mL) and saturated NaCl (20 mL) and dried (Na2SO4). Re...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ketone
Ketone.Azide
C1CC[C@H]2[C@H](C1)CC[C@@H]1COCC[C@@H]12
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
Br-
CN(C)C=O
null
null
COC(=O)[C@@H]1C[C@@H](Br)C(=O)[C@@H]2[C@@]3(C)C[C@@H](c4ccoc4)OC(=O)[C@H]3CC[C@]21C.[N-]=[N+]=[N-]>CN(C)C=O>COC(=O)[C@@H]1C[C@H](N=[N+]=[N-])C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c717980336e8416f8ee2af5881c025b5
COC(=O)[C@@H]1C[C@H](N=[N+]=[N-])C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C>>COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N=[N+]=[N-])=O)C)C1=COC=C1)=O)C.[NH4+].[Cl-]>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N)=O)C)C1=COC=C1)=O)C
[N-]=[N+]=[N:8][C@H:7]1[CH2:6][C@@H:5]([C:3]([O:2][CH3:1])=[O:4])[C@@:12]2([CH3:13])[C@H:11]([C:9]1=[O:10])[C@:27]1([CH3:28])[C@@H:16]([CH2:15][CH2:14]2)[C:17](=[O:18])[O:19][C@H:20]([c:21]2[cH:22][cH:23][o:24][cH:25]2)[CH2:26]1>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([NH2:8])[C:9](=[O:10])[C@H:11]2[C@@:12]1(...
COC(=O)[C@@H]1C[C@H](N=[N+]=[N-])C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
[Zn]
C(Cl)Cl.CO
Reduction
Azide to amine reduction (Staudinger)
4c9e4990dae2bb965dec06bd45e318560989ee3681b61e443f7aa363b7cfa222
cd009d687d606bf351eac9390a176d16be38f2c8216a599b398641009c215027
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
[C:1]-[C:2](=[O;D1;H0:3])-[C:4](-[N;H0;D2;+0:5]=[N+]=[N-])-[C:6]>>[C:1]-[C:2](=[O;D1;H0:3])-[C:4](-[NH2;D1;+0:5])-[C:6]
84
[{"value": 84.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.1, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N)=O)C)C1=COC=C1)=O)C", "details": "CALCULATEDPERCENTYIELD", "is...
null
null
3
HOUR
A mixture of 38 (0.08 g, 0.19 mmol), Zn dust (0.16 g, 2.45 mmol) and NH4Cl (g, mmol) in a mixture of CH2Cl2/MeOH (1:4, 20 mL) was stirred at room temperature for 3 h. The mixture was filtered and the filtrate was concentrated to dryness under reduced pressure. 2N NaOH (30 mL) was added to the residue and the mixture wa...
10.6084/m9.figshare.5104873.v1
null
Azide
Primary amine
null
null
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
Other
[Zn].C(Cl)Cl.CO
null
3
COC(=O)[C@@H]1C[C@H](N=[N+]=[N-])C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C>[Zn].C(Cl)Cl.CO>COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-0a37b151aa0046209d46305b4b391f88
CC(=O)OC(C)=O.COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C>>COC(=O)[C@@H]1C[C@H](NC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N)=O)C)C1=COC=C1)=O)C.C(C)(=O)OC(C)=O>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NC(C)=O)=O)C)C1=COC=C1)=O)C
CC(=O)O[C:9]([CH3:10])=[O:11].[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([NH2:8])[C:12](=[O:13])[C@H:14]2[C@@:15]1([CH3:16])[CH2:17][CH2:18][C@H:19]1[C:20](=[O:21])[O:22][C@H:23]([c:24]3[cH:25][cH:26][o:27][cH:28]3)[CH2:29][C@:30]21[CH3:31]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([NH:8][C:9]([CH3:10])=[...
CC(=O)OC(C)=O.COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@@H]1C[C@H](NC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Acylation
Aminolysis of esters
87d35e51b477fc9a658a6f307eb56d84c8879182772c9dd3a42ec0d584fd2684
627cbc0550c9f51ad0105d9fcf46677e8c93bed87ee95bfe69292a82550c95b7
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](=[O;D1;H0:6])-[C:7](-[NH2;D1;+0:8])-[C:9]>>[C:4]-[C:5](=[O;D1;H0:6])-[C:7](-[NH;D2;+0:8]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[C:9]
58
[{"value": 58.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NC(C)=O)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.9, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NC(C)=O)=O)C)C1=COC=C1)=O)C", "details": "CALCULATEDPERCEN...
null
null
null
null
A solution of 39 (0.06 g, 0.16 mmol), acetic anhydride (0.4 mL, 4.23 mmol) and a catalytic amount of DMAP in CH2Cl2 (30 mL) was stirred at room temperature for 2 h. The mixture was washed with 2N HCl (30 mL), 2N NaOH (30 mL), and H2O (30 mL) and dried (Na2SO4). Removal of the solvent under reduced pressure afforded a c...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary amine
Secondary amide
null
null
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HO-
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
null
CC(=O)OC(C)=O.COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C>CN(C)C=1C=CN=CC1.C(Cl)Cl>COC(=O)[C@@H]1C[C@H](NC(C)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c3231ec3b7b04f169d839bf51b685ede
CO.COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.O=C(Cl)c1ccccc1>>COC(=O)[C@@H]1C[C@H](OC(=O)C(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N)=O)C)C1=COC=C1)=O)C.C(C1=CC=CC=C1)(=O)Cl.CO>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C(C)C)=O)=O)C)C1=COC=C1)=O)C
C[OH:8].N[C@H:7]1[CH2:6][C@@H:5]([C:3]([O:2][CH3:1])=[O:4])[C@@:17]2([CH3:18])[C@H:16]([C:14]1=[O:15])[C@:32]1([CH3:33])[C@@H:21]([CH2:20][CH2:19]2)[C:22](=[O:23])[O:24][C@H:25]([c:26]2[cH:27][cH:28][o:29][cH:30]2)[CH2:31]1.Cl[C:9](=[O:10])[c:11]1[cH:12]ccc[cH:13]1>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([O:8...
CO.COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.O=C(Cl)c1ccccc1
COC(=O)[C@@H]1C[C@H](OC(=O)C(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Protection
OtherReaction
862476cb7bfa0b299b6bda8446b35088b6733227f3ff9b95ad63933419707f60
5528e9c46f2221c5ba9db86fcdf8258cf91882ed3b43678d1e0ae747a17c947b
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
C-[OH;D1;+0:1].Cl-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c;H0;D3;+0:4]1:[cH;D2;+0:5]:c:c:c:[cH;D2;+0:6]:1.N-[C@@H;D3;+0:7](-[C:8]-[C:9]-[C:10](-[#8:11])=[O;D1;H0:12])-[C:13](=[O;D1;H0:14])-[C:15]>>[#8:11]-[C:10](=[O;D1;H0:12])-[C:9]-[C:8]-[C@H;D3;+0:7](-[O;H0;D2;+0:1]-[C;H0;D3;+0:2](=[O;D1;H0:3])-[CH;D3;+0:4](-[CH3;D1;+0:5])-[C...
67
[{"value": 67.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)OC(C(C)C)=O)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 39 (0.10 g, 0.26 mmol), benzoyl chloride (0.11 g, 0.78 mmol) and DMAP (0.08 g, 0.78 mmol) in CH2Cl2 (20 mL) was stirred at room temperature for 2 h. Absolute MeOH (15 mL) was added and the solvent was removed under reduced pressure. CH2Cl2 (25 mL) was added to the residue and the solution was washed with ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ketone.Primary amine.Methanol
Ketone.Ester
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccccc1
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HCl
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
null
CO.COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.O=C(Cl)c1ccccc1>CN(C)C=1C=CN=CC1.C(Cl)Cl>COC(=O)[C@@H]1C[C@H](OC(=O)C(C)C)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c8cbe8556e3840b9b3958908f0a60857
COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.CS(=O)(=O)Cl>>COC(=O)[C@@H]1C[C@H](NS(C)(=O)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N)=O)C)C1=COC=C1)=O)C.CS(=O)(=O)Cl.CCN(CC)CC>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NS(=O)(=O)C)=O)C)C1=COC=C1)=O)C
[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([NH2:8])[C:13](=[O:14])[C@H:15]2[C@@:16]1([CH3:17])[CH2:18][CH2:19][C@H:20]1[C:21](=[O:22])[O:23][C@H:24]([c:25]3[cH:26][cH:27][o:28][cH:29]3)[CH2:30][C@:31]21[CH3:32].Cl[S:9]([CH3:10])(=[O:11])=[O:12]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([NH:8][S:9]([CH3:10...
COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.CS(=O)(=O)Cl
COC(=O)[C@@H]1C[C@H](NS(C)(=O)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1CCCC2CC[C@H]3C(=O)O[C@H](c4ccoc4)CC3[C@@H]12
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].[C:5]-[C:6](=[O;D1;H0:7])-[C:8](-[NH2;D1;+0:9])-[C:10]>>[C:5]-[C:6](=[O;D1;H0:7])-[C:8](-[NH;D2;+0:9]-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4])-[C:10]
575.9
[{"value": 56.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NS(=O)(=O)C)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 575.9, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NS(=O)(=O)C)=O)C)C1=COC=C1)=O)C", "details": "CALCULA...
null
null
null
null
A solution of 39 (0.10 g, 0.26 mmol), methanesulfonyl chloride (0.08 mL, 1.03 mmol), NEt3 (0.04 mL, 0.28 mmol) and a catalytic amount of DMAP in CH2Cl2 (50 mL) was stirred at room temperature for 2 h. The mixture was washed with 2N HCl (30 mL), 2N NaOH (30 mL), and H2O (30 mL) and dried (Na2SO4). Removal of the solvent...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HCl
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
null
COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.CS(=O)(=O)Cl>CN(C)C=1C=CN=CC1.C(Cl)Cl>COC(=O)[C@@H]1C[C@H](NS(C)(=O)=O)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f09243616f4044a5a3266a405d02034e
COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.O=S(=O)(Cl)c1ccccc1>>COC(=O)[C@@H]1C[C@H](NS(=O)(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)N)=O)C)C1=COC=C1)=O)C.C1(=CC=CC=C1)S(=O)(=O)Cl.C(C)N(CC)CC.CO>>COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NS(=O)(=O)C1=CC=CC=C1)=O)C)C1=COC=C1)=O)C
[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][C@H:7]([NH2:8])[C:18](=[O:19])[C@H:20]2[C@@:21]1([CH3:22])[CH2:23][CH2:24][C@H:25]1[C:26](=[O:27])[O:28][C@H:29]([c:30]3[cH:31][cH:32][o:33][cH:34]3)[CH2:35][C@:36]21[CH3:37].Cl[S:9](=[O:10])(=[O:11])[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]...
COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.O=S(=O)(Cl)c1ccccc1
COC(=O)[C@@H]1C[C@H](NS(=O)(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1[C@H]2C(CC[C@@H]1NS(=O)(=O)c1ccccc1)CC[C@H]1C(=O)O[C@H](c3ccoc3)CC21
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8](=[O;D1;H0:9])-[C:10](-[NH2;D1;+0:11])-[C:12]>>[C:7]-[C:8](=[O;D1;H0:9])-[C:10](-[NH;D2;+0:11]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[C:12]
98.9
[{"value": 97.0, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NS(=O)(=O)C1=CC=CC=C1)=O)C)C1=COC=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.9, "product": "COC(=O)[C@H]1[C@@]2(CC[C@H]3C(O[C@@H](C[C@@]3([C@H]2C([C@H](C1)NS(=O)(=O)C1=CC=CC=C1)=O)C)C1=COC=C1)=O)C", ...
null
null
null
null
A solution of 39 (0.08 g, 0.21 mmol), benzenesulfonyl chloride (0.07 g, 0.42 mmol), triethylamine (0.06 g, 0.63 mmol), and a catalytic amount of DMAP in CH2Cl2 (40 mL) was stirred at room temperature for 18 h. Absolute MeOH was then added and the solution was washed with 10% HCl (3×25 mL) and saturated NaCl (2×25 mL), ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.C1CC[C@H]2[C@H](C1)CC[C@H]1COCC[C@@H]12.c1ccoc1
HCl
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
null
COC(=O)[C@@H]1C[C@H](N)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C.O=S(=O)(Cl)c1ccccc1>CN(C)C=1C=CN=CC1.C(Cl)Cl>COC(=O)[C@@H]1C[C@H](NS(=O)(=O)c2ccccc2)C(=O)[C@H]2[C@@]1(C)CC[C@H]1C(=O)O[C@H](c3ccoc3)C[C@]21C
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-48ec6b01a3864024ac16587c981afead
CCOC(=O)CCCl.Nc1ccc2c(c1)CCC2>>CCOC(=O)CCNc1ccc2c(c1)CCC2
NC=1C=C2CCCC2=CC1.ClCCC(=O)OCC.C([O-])([O-])=O.[K+].[K+]>>C(C)OC(CCNC=1C=C2CCCC2=CC1)=O
Cl[CH2:7][CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].[NH2:8][c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[CH2:15][CH2:16][CH2:17]2>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][NH:8][c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[CH2:15][CH2:16][CH2:17]2
CCOC(=O)CCCl.Nc1ccc2c(c1)CCC2
CCOC(=O)CCNc1ccc2c(c1)CCC2
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
null
Heteroatom Alkylation and Arylation
N-alkylation of primary amines with alkyl halides
fc19a1445ff204e66e51735d0191465bda3c6691fd233624a54742c9d4828411
0b1d32f56ad00f1e5bdae9390f9227bbea012fa2f8203aac34726b8a6761cc7c
c1ccc2c(c1)CCC2
Cl-[CH2;D2;+0:1]-[C:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[C:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[C:2]-[CH2;D2;+0:1]-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]
71
[{"value": 71.0, "product": "C(C)OC(CCNC=1C=C2CCCC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 70.7, "product": "C(C)OC(CCNC=1C=C2CCCC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
16
HOUR
To a mixture of 5-aminoindane (5 g, 37.6 mmol), ethyl 3-chloropropionate (4.7 mL, 37.6 mmol) and potassium carbonate (5.2 g, 37.6 mmol) was added tetrabutylammonium bromide (200 mg). The mixture was stirred at 100° C. for 16 hours. After cooling to room temperature (rt), the mixture was extracted into ethyl acetate (Et...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary amine
Secondary amine
null
null
c1ccc2c(c1)CCC2
HCl
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
100
16
CCOC(=O)CCCl.Nc1ccc2c(c1)CCC2>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC>CCOC(=O)CCNc1ccc2c(c1)CCC2
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-388c20312aad4c688e3949a8286aa8af
CCOC(=O)CCNc1ccc2c(c1)CCC2.CCOC(=O)c1cnc(SC)nc1Cl>>CCOC(=O)CCN(c1ccc2c(c1)CCC2)c1nc(SC)ncc1C(=O)OCC
C(C)OC(CCNC=1C=C2CCCC2=CC1)=O.ClC1=NC(=NC=C1C(=O)OCC)SC.C(C)N(CC)CC>>C(C)OC(=O)C=1C(=NC(=NC1)SC)N(C=1C=C2CCCC2=CC1)CCC(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][NH:8][c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[CH2:15][CH2:16][CH2:17]2.Cl[c:18]1[n:19][c:20]([S:21][CH3:22])[n:23][cH:24][c:25]1[C:26](=[O:27])[O:28][CH2:29][CH3:30]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][N:8]([c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[CH2:15]...
CCOC(=O)CCNc1ccc2c(c1)CCC2.CCOC(=O)c1cnc(SC)nc1Cl
CCOC(=O)CCN(c1ccc2c(c1)CCC2)c1nc(SC)ncc1C(=O)OCC
null
null
C(CCC)O
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution amine
8a13b42f4b06102b68f4963e65202071bf1d0630fbad1b11bbd8e99b9f9c8f34
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1cc(Nc2ccc3c(c2)CCC3)ncn1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]:[c:6]:1-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10].[#8:11]-[C:12](=[O;D1;H0:13])-[C:14]-[C:15]-[NH;D2;+0:16]-[c:17](:[c:18]):[c:19]>>[#8:11]-[C:12](=[O;D1;H0:13])-[C:14]-[C:15]-[N;H0;D3;+0:16](-[c:17](:[c:18]):[c:19])-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]:[c:6]:1-[C:7](=[...
90
[{"value": 90.0, "product": "C(C)OC(=O)C=1C(=NC(=NC1)SC)N(C=1C=C2CCCC2=CC1)CCC(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.2, "product": "C(C)OC(=O)C=1C(=NC(=NC1)SC)N(C=1C=C2CCCC2=CC1)CCC(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
DAY
To a solution of 3-(indan-5-ylamino)-propionic acid ethyl ester (5 g, 21.4 mmol) and ethyl 4-chloro-2-methylthio-5-pyrimidinecarboxylate (5 g, 21.4 mmol) in 40 mL of n-butanol was added triethylamine (3 mL, 21.4 mmol). The solution was stirred at rt for 2 days. The solvent was removed under vacuum. The residue was extr...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1cncnc1
c1cncnc1
c1ccc2c(c1)CCC2.c1cncnc1
HCl
C(CCC)O
null
48
CCOC(=O)CCNc1ccc2c(c1)CCC2.CCOC(=O)c1cnc(SC)nc1Cl>C(CCC)O>CCOC(=O)CCN(c1ccc2c(c1)CCC2)c1nc(SC)ncc1C(=O)OCC
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-97b2d45e987f4f5581a86c3d7fc3bcd7
CCOC(=O)CCN(c1ccc2c(c1)CCC2)c1nc(SC)ncc1C(=O)OCC>>CCOC(=O)C1CN(c2ccc3c(c2)CCC3)c2nc(SC)ncc2C1=O
C(C)OC(=O)C=1C(=NC(=NC1)SC)N(C=1C=C2CCCC2=CC1)CCC(=O)OCC.CC(C)([O-])C.[Na+].N#N.Cl.[Na]>>C(C)OC(=O)C1C(C2=C(N=C(N=C2)SC)N(C1)C=1C=C2CCCC2=CC1)=O
CCO[C:26]([c:25]1[c:18]([N:8]([CH2:7][CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[CH2:15][CH2:16][CH2:17]3)[n:19][c:20]([S:21][CH3:22])[n:23][cH:24]1)=[O:27]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][N:8]([c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[CH2:15][CH2:16][CH2:17]3)[...
CCOC(=O)CCN(c1ccc2c(c1)CCC2)c1nc(SC)ncc1C(=O)OCC
CCOC(=O)C1CN(c2ccc3c(c2)CCC3)c2nc(SC)ncc2C1=O
null
null
C(C)(C)(C)O.C1(=CC=CC=C1)C
Functional Group Interconversion
OtherReaction
30bc859f342e7454d65786ffc9dd9e1f370c7689a335282691882093ec0ad590
6f130a746a78d10ca37f94948711de2b0c76f45052ca887b0e681c66276a7764
O=C1CCN(c2ccc3c(c2)CCC3)c2ncncc21
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:1-[#7:9]-[C:10]-[CH2;D2;+0:11]-[C:12](=[O;D1;H0:13])-[#8:14]-[C:15]>>[C:15]-[#8:14]-[C:12](=[O;D1;H0:13])-[CH;D3;+0:11]1-[C:10]-[#7:9]-[c:8]2:[#7;a:7]:[c:6]:[#7;a:5]:[c:4]:[c:3]:2-[C;H0;D3;+0:1]-1=[O;D1;H0:2]
null
[]
90
CELSIUS
10
MINUTE
To sodium (25 wt % dispersion in paraffin wax, 1.6 g, 16.9 mmol) was added t-butanol (30 mL) under stirring and N2. After 10 minutes, a solution of 4-[(2-ethoxycarbonyl-ethyl)-indan-5-yl-amino]-2-methylsulfanyl-pyrimidine-5-carboxylic acid ethyl ester (6.6 g, 15.4 mmol) in 40 mL of toluene was added to the sodium t-but...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Ketone
null
c1ncc2c(n1)[NH]CCC2
c1ccc2c(c1)CCC2.c1ncc2c(n1)[NH]CCC2
HO-
C(C)(C)(C)O.C1(=CC=CC=C1)C
90
0.166667
CCOC(=O)CCN(c1ccc2c(c1)CCC2)c1nc(SC)ncc1C(=O)OCC>C(C)(C)(C)O.C1(=CC=CC=C1)C>CCOC(=O)C1CN(c2ccc3c(c2)CCC3)c2nc(SC)ncc2C1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2321ae9f98384267a85d98e9a630843a
CCOC(=O)C1CN(c2ccc3c(c2)CCC3)c2nc(SC)ncc2C1=O>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(SC)ncc2c1=O
C(C)N(CC)CC.C(C)OC(=O)C1C(C2=C(N=C(N=C2)SC)N(C1)C=1C=C2CCCC2=CC1)=O.BrBr.N#N>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)SC)N(C1)C=1C=C2CCCC2=CC1)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][N:8]([c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[CH2:15][CH2:16][CH2:17]3)[c:18]2[n:19][c:20]([S:21][CH3:22])[n:23][cH:24][c:25]2[C:26]1=[O:27]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[CH2:15][CH2:16][CH2:17]3)[c:18]2[...
CCOC(=O)C1CN(c2ccc3c(c2)CCC3)c2nc(SC)ncc2C1=O
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(SC)ncc2c1=O
null
null
C(Cl)Cl
Oxidation
OtherReaction
e6fdfa5ad0e8b814bf3d3d5cf077356d203a162eff2c4a4b9336450468009711
90d664ba841914112433e4101d37ffefd1e45e7dce983b85577c7f1d5a635093
O=c1ccn(-c2ccc3c(c2)CCC3)c2ncncc12
[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH;D3;+0:5]1-[CH2;D2;+0:6]-[N;H0;D3;+0:7](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12])-[c:13]2:[#7;a:14]:[c:15]:[#7;a:16]:[c:17]:[c:18]:2-[C;H0;D3;+0:19]-1=[O;D1;H0:20]>>[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[c;H0;D3;+0:5]1:[cH;D2;+0:6]:[n;H0;D3;+0:7](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:...
94
[{"value": 94.0, "product": "C(C)OC(=O)C=1C(C2=C(N=C(N=C2)SC)N(C1)C=1C=C2CCCC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.6, "product": "C(C)OC(=O)C=1C(C2=C(N=C(N=C2)SC)N(C1)C=1C=C2CCCC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 8-indan-5-yl-2-methylsulfanyl-5-oxo-5,6,7,8-tetrahydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (0.32 g, 0.84 mmol) in 5 mL of methylene chloride (CH2Cl2) was added bromine (43 μL, 0.84 mmol) slowly under N2. The solution was stirred at room temperature for 2 hours (or to completion). The ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Tertiary amine
Ester
c1ncc2c(n1)[NH]CCC2
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1
null
C(Cl)Cl
null
2
CCOC(=O)C1CN(c2ccc3c(c2)CCC3)c2nc(SC)ncc2C1=O>C(Cl)Cl>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(SC)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-5e2c409cf06f4d6b8bfbb2bddbc35dab
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(SC)ncc2c1=O>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O
C([O-])(O)=O.[Na+].S(=S)(=O)([O-])[O-].[Na+].[Na+].C(C)OC(=O)C=1C(C2=C(N=C(N=C2)SC)N(C1)C=1C=C2CCCC2=CC1)=O.ClC=1C=C(C(=O)OO)C=CC1>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[CH2:15][CH2:16][CH2:17]3)[c:18]2[n:19][c:20]([S:21][CH3:22])[n:25][cH:26][c:27]2[c:28]1=[O:29]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[CH2:15][CH2:16][CH2:17]3)[c:18]2[n...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(SC)ncc2c1=O
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O
null
null
C(Cl)Cl
Oxidation
OtherReaction
20dd6d48007b4fe7cd760226f21413eb5e71e6468db112596c2e7ea4858c8ac1
5cedc1bf0f43f21d78a249521ecfcec19fc5ac4895c41eed0e84f0c2618149fa
O=c1ccn(-c2ccc3c(c2)CCC3)c2ncncc12
[#7;a:1]:[c:2]:[#7;a:3]:[c:4](-[S;H0;D2;+0:5]-[C;D1;H3:6]):[#7;a:7]:[c:8]>>[#7;a:1]:[c:2]:[#7;a:3]:[c:4](-[S;H0;D4;+0:5](-[C;D1;H3:6])(=[O;D1;H0:9])=[O;D1;H0:10]):[#7;a:7]:[c:8]
67
[{"value": 67.0, "product": "C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a solution of 8-indan-5-yl-2-methylsulfanyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (0.3 g, 0.79 mmol) in 5 mL of CH2Cl2, was added 3-chloroperoxybenzoic acid (m-CPBA, 69.5%, 431 mg, 1.73 mmol) portionwise. The solution was stirred at room temperature for 3 hours. An aqueous solution ...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfone
null
null
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1
null
C(Cl)Cl
null
3
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(SC)ncc2c1=O>C(Cl)Cl>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2e80798a5f184cd09efdc0cbdbcb7c58
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCN1CCCCC1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCCCC3)ncc2c1=O
N1(CCCCC1)CCN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCN2CCCCC2)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:33](=[O:34])[c:32]2[cH:31][n:30]1.[NH2:21][CH2:22][CH2:23][N:24]1[CH2:25][CH2:26][CH2:27][CH2:28][CH2:29]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCN1CCCCC1
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCCCC3)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCCCC3)ncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1(Step F) the title compound was prepared from 2-piperidin-1-yl-ethylamine (5.2 μL, 0.036 mmol) and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1(Step E), 15 mg, 0.036 mmol). 6.6 mg of 8-indan-5-yl-5-oxo-2-(...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.C1CC[NH]CC1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCN1CCCCC1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCCCC3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-09ed7dd69e214258a42cde07500db0dc
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCn1ccnc1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O
N1(C=NC=C1)CCCN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCCN2C=NC=C2)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:33](=[O:34])[c:32]2[cH:31][n:30]1.[NH2:21][CH2:22][CH2:23][CH2:24][n:25]1[cH:26][cH:27][n:28][cH:29]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCn1ccnc1
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1(Step F) the title compound was prepared from 3-imidazol-1-yl-propylamine (4.4 μL, 0.036 mmol) and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1(Step E), 15 mg, 0.036 mmol). 19.2 mg of 2-(3-imidazol-1-yl-pr...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.c1c[nH]cn1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCn1ccnc1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c631ee24ba914cb3bfcfa098644fb64f
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCN1CCOCC1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCOCC3)ncc2c1=O
N1(CCOCC1)CCN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCN2CCOCC2)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:33](=[O:34])[c:32]2[cH:31][n:30]1.[NH2:21][CH2:22][CH2:23][N:24]1[CH2:25][CH2:26][O:27][CH2:28][CH2:29]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCN1CCOCC1
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCOCC3)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCOCC3)ncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1(Step F) the title compound was prepared from 2-morpholin-4-yl-ethylamine (4.8 μL, 0.036 mmol) and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1(Step E), 15 mg, 0.036 mmol). 15.5 mg of 8-indan-5-yl-2-(2-mor...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.C1COCC[NH]1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCN1CCOCC1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCOCC3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-221d7370a8be4b47a16e7531e653c480
CC(CN)N1CCOCC1.CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCC(C)N3CCOCC3)ncc2c1=O
N1(CCOCC1)C(CN)C.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCC(C)N2CCOCC2)N(C1)C=1C=C2CCCC2=CC1)=O
[NH2:21][CH2:22][CH:23]([CH3:24])[N:25]1[CH2:26][CH2:27][O:28][CH2:29][CH2:30]1.CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:34](=[O:35])[c:33]2[cH:32][n:31]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-...
CC(CN)N1CCOCC1.CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCC(C)N3CCOCC3)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCCN3CCOCC3)ncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1(Step F) the title compound was prepared from 2-morpholin-4-yl-propylamine (5.3 μL, 0.036 mmol) and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1(Step E), 15 mg, 0.036 mmol). 17.2 mg of 8-indan-5-yl-2-(2-mo...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.C1COCC[NH]1
HO-
null
null
null
CC(CN)N1CCOCC1.CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCC(C)N3CCOCC3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-c76918262cac4fbda4c8bbbb28c023b4
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.CN(C)CCCN>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O
CN(CCCN)C.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCCN(C)C)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:31](=[O:32])[c:30]2[cH:29][n:28]1.[NH2:21][CH2:22][CH2:23][CH2:24][N:25]([CH3:26])[CH3:27]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][c:...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.CN(C)CCCN
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2ncncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1(Step F) the title compound was prepared from N1,N1-dimethyl-propane-1,3-diamine (4.6 μL, 0.036 mmol) and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1(Step E), 15 mg, 0.036 mmol). 9.7 mg of 2-(3-dimethylam...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.CN(C)CCCN>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-5416bb0874aa4c6b90233d86501eee42
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COCCCN>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCOC)ncc2c1=O
COCCCN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCCOC)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:30](=[O:31])[c:29]2[cH:28][n:27]1.[NH2:21][CH2:22][CH2:23][CH2:24][O:25][CH3:26]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COCCCN
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCOC)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2ncncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1 Step F, the title compound was prepared from 3-methoxy-propylamine and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1(Step E), 20 mg, 0.040 mmol). 11 mg of 8-Indan-5-yl-2-(3-methoxy-propylamino)-5-oxo-5,8-d...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COCCCN>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCOC)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-7103322ccabc4c2ba5b9486553491181
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCN1CCCC1=O>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN3CCCC3=O)ncc2c1=O
NCCCN1C(CCC1)=O.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCCN2C(CCC2)=O)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:34](=[O:35])[c:33]2[cH:32][n:31]1.[NH2:21][CH2:22][CH2:23][CH2:24][N:25]1[CH2:26][CH2:27][CH2:28][C:29]1=[O:30]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCN1CCCC1=O
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN3CCCC3=O)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=C1CCCN1CCCNc1ncc2c(=O)ccn(-c3ccc4c(c3)CCC4)c2n1
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1 Step F, the title compound was prepared from 1-(3-amino-propyl)-pyrrolidin-2-one and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1(Step E) 25 mg, 0.052 mmol). 17 mg of 8-Indan-5-yl-5-oxo-2-[3-(2-oxo-pyrrol...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.C1CC[NH]C1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCN1CCCC1=O>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN3CCCC3=O)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-1919b9c11bfd4ee3b0e8b1354be000fd
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCN1CCCC1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN3CCCC3)ncc2c1=O
N1(CCCC1)CCCN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCCN2CCCC2)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:33](=[O:34])[c:32]2[cH:31][n:30]1.[NH2:21][CH2:22][CH2:23][CH2:24][N:25]1[CH2:26][CH2:27][CH2:28][CH2:29]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCN1CCCC1
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN3CCCC3)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCCCN3CCCC3)ncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure described in Example 1 Step F, the title compound was prepared from 3-pyrrolidin-1-yl-propylamine and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1(Step E), 10 mg, 0.022 mmol). 7 mg of 8-Indan-5-yl-5-oxo-2-(3-pyrrolidin-1-yl-pr...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.C1CC[NH]C1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.NCCCN1CCCC1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN3CCCC3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-b7ba26de978f4a50af0d8f824c40513a
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COCCN>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCOC)ncc2c1=O
COCCN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCOC)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:29](=[O:30])[c:28]2[cH:27][n:26]1.[NH2:21][CH2:22][CH2:23][O:24][CH3:25]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COCCN
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCOC)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2ncncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1 Step F, the title compound was prepared from 2-methoxy-ethylamine and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (Example 1, Step E, 10 mg, 0.022 mmol). 7 mg of 8-indan-5-yl-2-(2-methoxy-ethylamino)-5-oxo-5,8-dihydro-p...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COCCN>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCOC)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-2c8622961eb94f9ca0d59f465c4d5070
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1cc(CN)cc(OC)c1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCc3cc(OC)cc(OC)c3)ncc2c1=O
COC=1C=C(CN)C=C(C1)OC.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCC2=CC(=CC(=C2)OC)OC)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:36](=[O:37])[c:35]2[cH:34][n:33]1.[NH2:21][CH2:22][c:23]1[cH:24][c:25]([O:26][CH3:27])[cH:28][c:29]([O:30][CH3:31])[cH:32]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1cc(CN)cc(OC)c1
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCc3cc(OC)cc(OC)c3)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCc3ccccc3)ncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[NH2;D1;+0:7]-[C:8]-[c:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:7]-[C:8]-[c:9]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1 Step F, the title compound was prepared from 3,5-dimethoxybenzylamine and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (10 mg, 0.02 mmol). 10 mg of 2-(3,5-Dimethoxy-benzylamino)-8-indan-5-yl-5-oxo-5,8-dihydro-pyrido[2,3-...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.c1ccccc1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1cc(CN)cc(OC)c1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCc3cc(OC)cc(OC)c3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-f01a3334192e489f87d7b57eca61d2a1
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O.CN>>CNC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O
CN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCCN(C)C)N(C1)C=1C=C2CCCC2=CC1)=O>>CNC(=O)C=1C(C2=C(N=C(N=C2)NCCCN(C)C)N(C1)C=1C=C2CCCC2=CC1)=O
CCO[C:3](=[O:4])[c:5]1[cH:6][n:7](-[c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13]2)[CH2:14][CH2:15][CH2:16]3)[c:17]2[n:18][c:19]([NH:20][CH2:21][CH2:22][CH2:23][N:24]([CH3:25])[CH3:26])[n:27][cH:28][c:29]2[c:30]1=[O:31].[CH3:1][NH2:2]>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][n:7](-[c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13]2)[CH...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O.CN
CNC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O
null
null
null
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
O=c1ccn(-c2ccc3c(c2)CCC3)c2ncncc12
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6](-[c:7]):[c:8]:[#7;a:9].[C;D1;H3:10]-[NH2;D1;+0:11]>>[#7;a:9]:[c:8]:[#7;a:6](-[c:7]):[c:5]:[c:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:11]-[C;D1;H3:10]):[c:4]
77
[{"value": 77.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
DAY
A solution of methylamine (1N, 1 mL in methanol) was added to 2-(3-dimethylamino-propylamino)-8-indan-5-yl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (Example 6 Step A, 6 mg, 0.015 mmol). The mixture was kept in a sealed tube at 110° C. with stirring for 2 days. The solution, after cooling ...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1
HO-
null
null
48
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O.CN>>CNC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCN(C)C)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-1b855d8e9b0c46178a8fa3663c80ab40
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1ccc(CCN)cc1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCc3ccc(OC)cc3)ncc2c1=O
COC1=CC=C(C=C1)CCN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCC2=CC=C(C=C2)OC)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:35](=[O:36])[c:34]2[cH:33][n:32]1.[NH2:21][CH2:22][CH2:23][c:24]1[cH:25][cH:26][c:27]([O:28][CH3:29])[cH:30][cH:31]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1ccc(CCN)cc1
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCc3ccc(OC)cc3)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCCc3ccccc3)ncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1 Step F, the title compound was prepared 2-(4-methoxyphenyl)-ethylamine and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (from Example 1 Step E, 20 mg, 0.04 mmol). 19 mg of 8-Indan-5-yl-2-[2-(4-methoxy-phenyl)-ethylamino]...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.c1ccccc1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1ccc(CCN)cc1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCc3ccc(OC)cc3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-586bc51c127c4e3c8344b2f9a0952509
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O.CON>>CONC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O
C(C)N(CC)CC.Cl.CON.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCCN2C=NC=C2)N(C1)C=1C=C2CCCC2=CC1)=O>>CONC(=O)C=1C(C2=C(N=C(N=C2)NCCCN2C=NC=C2)N(C1)C=1C=C2CCCC2=CC1)=O
CCO[C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[CH2:15][CH2:16][CH2:17]3)[c:18]2[n:19][c:20]([NH:21][CH2:22][CH2:23][CH2:24][n:25]3[cH:26][cH:27][n:28][cH:29]3)[n:30][cH:31][c:32]2[c:33]1=[O:34].[CH3:1][O:2][NH2:3]>>[CH3:1][O:2][NH:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][c:...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O.CON
CONC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O
null
null
CO.O
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc12
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6](-[c:7]):[c:8]:[#7;a:9].[C;D1;H3:10]-[#8:11]-[NH2;D1;+0:12]>>[#7;a:9]:[c:8]:[#7;a:6](-[c:7]):[c:5]:[c:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:12]-[#8:11]-[C;D1;H3:10]):[c:4]
65
[{"value": 65.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
DAY
Triethylamine (0.5 mL) was added to a mixture of O-methylhydroxylamine hydrochloride (220 mg) and 2-(3-imidazol-1-yl-propylamino)-8-indan-5-yl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (Example 3 Step A, 3.0 mg, 0.006 mmol) in 0.5 mL of methanol. The reaction mixture was kept in a sealed t...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.c1c[nH]cn1
HO-
CO.O
null
48
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O.CON>CO.O>CONC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCCn3ccnc3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-919543a4f7864fcdaad14c824ac2a07e
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1ccc(CCN)cc1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCc3ccc(OC)cc3)ncc2c1=O
COC1=CC=C(C=C1)CCN.C(C)OC(=O)C=1C(C2=C(N=C(N=C2)S(=O)(=O)C)N(C1)C=1C=C2CCCC2=CC1)=O>>C(C)OC(=O)C=1C(C2=C(N=C(N=C2)NCCC2=CC=C(C=C2)OC)N(C1)C=1C=C2CCCC2=CC1)=O
CS(=O)(=O)[c:20]1[n:19][c:18]2[n:8](-[c:9]3[cH:10][cH:11][c:12]4[c:13]([cH:14]3)[CH2:15][CH2:16][CH2:17]4)[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:35](=[O:36])[c:34]2[cH:33][n:32]1.[NH2:21][CH2:22][CH2:23][c:24]1[cH:25][cH:26][c:27]([O:28][CH3:29])[cH:30][cH:31]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8...
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1ccc(CCN)cc1
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCc3ccc(OC)cc3)ncc2c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1ccn(-c2ccc3c(c2)CCC3)c2nc(NCCc3ccccc3)ncc12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]:[#7;a:4]):[#7;a:5]:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[C:8]-[C:7]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Using the procedure outlined in Example 1 Step F, the title compound was prepared from 2-(4-methoxy-phenyl)-ethylamine and 8-indan-5-yl-2-methanesulfonyl-5-oxo-5,8-dihydro-pyrido[2,3-d]pyrimidine-6-carboxylic acid ethyl ester (Example 1 Step E, 20 mg, 0.040 mmol). 16 mg of 8-Indan-5-yl-2-(2-(4-methoxy-phenyl)-ethylamin...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccc2c(c1)CCC2.c1cnc2ncncc2c1.c1ccccc1
HO-
null
null
null
CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(S(C)(=O)=O)ncc2c1=O.COc1ccc(CCN)cc1>>CCOC(=O)c1cn(-c2ccc3c(c2)CCC3)c2nc(NCCc3ccc(OC)cc3)ncc2c1=O
ord_dataset-03ba810b7f464a06b5d8787af2e8b64e
ord-66ca2717a0e24c2293f8cef297ade30e
CCOC(=O)CCCl.NC1CCCCC1>>CCOC(=O)CCNC1CCCCC1
C1(CCCCC1)N.C(C)OC(CCCl)=O.C(=O)([O-])[O-].[K+].[K+]>>C(C)OC(CCNC1CCCCC1)=O
Cl[CH2:7][CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].[NH2:8][CH:9]1[CH2:10][CH2:11][CH2:12][CH2:13][CH2:14]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][NH:8][CH:9]1[CH2:10][CH2:11][CH2:12][CH2:13][CH2:14]1
CCOC(=O)CCCl.NC1CCCCC1
CCOC(=O)CCNC1CCCCC1
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC
null
Heteroatom Alkylation and Arylation
N-alkylation of primary amines with alkyl halides
fc19a1445ff204e66e51735d0191465bda3c6691fd233624a54742c9d4828411
0b1d32f56ad00f1e5bdae9390f9227bbea012fa2f8203aac34726b8a6761cc7c
C1CCCCC1
Cl-[CH2;D2;+0:1]-[C:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6].[C:7]-[C:8](-[NH2;D1;+0:9])-[C:10]>>[C:7]-[C:8](-[NH;D2;+0:9]-[CH2;D2;+0:1]-[C:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6])-[C:10]
72.3
[{"value": 72.0, "product": "C(C)OC(CCNC1CCCCC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.3, "product": "C(C)OC(CCNC1CCCCC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
Cyclohexylamine (0.86 g, 8.7 mmol) and 3-chloro-propionic acid ethyl ester (1.18 g, 8.67 mmol) were combined neat and K2CO3 (1.2 g, 8.7 mmol) and a catalytic amount of tetrabutylammonium iodide (ca. 5 mg) was added. The mixture was heated at 80° C. overnight. The resulting mixture was then partitioned between water and...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary amine
Secondary amine
null
null
C1CCCCC1
HCl
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC
80
null
CCOC(=O)CCCl.NC1CCCCC1>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC>CCOC(=O)CCNC1CCCCC1