dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-199fcedcf8044722923baaa5b14e12bf
C#CC(=O)OC(C)(C)C.CCOC(=O)C(N)=NO>>CCOC(=O)c1nc(C(=O)OC(C)(C)C)c[nH]1
C(C#C)(=O)OC(C)(C)C.NC(C(=O)OCC)=NO.C=1(C(=CC=CC1)C)C>>C(C)OC(=O)C=1NC=C(N1)C(=O)OC(C)(C)C
[C:8]([C:9](=[O:10])[O:11][C:12]([CH3:13])([CH3:14])[CH3:15])#[CH:16].O[N:7]=[C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[NH2:17]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][c:8]([C:9](=[O:10])[O:11][C:12]([CH3:13])([CH3:14])[CH3:15])[cH:16][nH:17]1
C#CC(=O)OC(C)(C)C.CCOC(=O)C(N)=NO
CCOC(=O)c1nc(C(=O)OC(C)(C)C)c[nH]1
null
null
C(C)N(CC)CC
Aromatic Heterocycle Formation
OtherReaction
1a8eddfecd0917248b2f4bc96ba85ccddcb260b77275366dca5d8d7aae3edf0b
76dbfeda98b19c1e1248a8fac66bc22be17ead6952c98f11b2e36ab4bdbeafa6
c1c[nH]cn1
O-[N;H0;D2;+0:1]=[C;H0;D3;+0:2](-[NH2;D1;+0:3])-[C:4](=[O;D1;H0:5])-[#8:6]-[C:7].[C;D1;H3:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[#8:12]-[C:13](=[O;D1;H0:14])-[C;H0;D2;+0:15]#[CH;D1;+0:16]>>[C:7]-[#8:6]-[C:4](=[O;D1;H0:5])-[c;H0;D3;+0:2]1:[n;H0;D2;+0:1]:[c;H0;D3;+0:15](-[C:13](=[O;D1;H0:14])-[#8:12]-[C:9](-[C;D1;H3:8])...
null
[]
null
null
null
null
tert-Butyl 2-ethoxycarbonyl imidazole-4-carboxylate can be prepared as follows: the procedure is as in Example 1 but starting from 15 g of ethyl α-aminooximinoacetate, 500 ml of xylene, 19.1 of triethylamine and 14.3 ml of tert-butyl propiolate. The crude product (19 g) is chromatographed on a silica column, eluting wi...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Primary amine.Alkyne.Oxime
Ester.Ester
null
c1c[nH]cn1
c1c[nH]cn1
HO-
C(C)N(CC)CC
null
null
C#CC(=O)OC(C)(C)C.CCOC(=O)C(N)=NO>C(C)N(CC)CC>CCOC(=O)c1nc(C(=O)OC(C)(C)C)c[nH]1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-71deb639e501406b8994cac9a143516e
CC(C)CCON=O.CCOC(=O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3>>O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3=NO
O.[H-].[Na+].O=C1C=2N(C3=C(N1)C=1C=CC=CC1C3)C=C(N2)C(=O)OCC.N(=O)OCCC(C)C>>ON=C1C=2C=CC=CC2C=2NC(C=3N(C21)C=C(N3)C(=O)O)=O
CC(C)CCO[N:21]=[O:22].CC[O:3][C:2](=[O:1])[c:4]1[cH:5][n:6]2[c:7]3[c:8]([nH:9][c:10](=[O:11])[c:12]2[n:13]1)-[c:14]1[cH:15][cH:16][cH:17][cH:18][c:19]1[CH2:20]3>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][n:6]2[c:7]3[c:8]([nH:9][c:10](=[O:11])[c:12]2[n:13]1)-[c:14]1[cH:15][cH:16][cH:17][cH:18][c:19]1[C:20]3=[N:21][OH:22]
CC(C)CCON=O.CCOC(=O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3
O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3=NO
null
null
C(C)(=O)O.CS(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
58239249e615ec552798952b225c21cfaf0b2545ba18fba7dbc485e32ed12672
76a27e58b662a405c95e29e5fb6fdbef5dc765e93c458d81e56749745ac9d49d
N=C1c2ccccc2-c2[nH]c(=O)c3nccn3c21
C-C(-C)-C-C-O-[N;H0;D2;+0:1]=[O;H0;D1;+0:2].C-C-[O;H0;D2;+0:3]-[C:4](=[O;D1;H0:5])-[c:6]1:[#7;a:7]:[c:8]2:[c:9]:[#7;a:10]:[c:11]3:[c:12](:[#7;a:13]:2:[c:14]:1)-[CH2;D2;+0:15]-[c:16](:[c:17]):[c:18]-3>>[O;D1;H0:5]=[C:4](-[OH;D1;+0:3])-[c:6]1:[#7;a:7]:[c:8]2:[c:9]:[#7;a:10]:[c:11]3:[c:12](:[#7;a:13]:2:[c:14]:1)-[C;H0;D3;...
null
[]
null
null
18
HOUR
0.34 g of sodium hydride is added to 1 g of ethyl 4,5-dihydro-4-oxo-10H-imidazo[1,2-a]indeno[1,2-e]pyrazine-2-carboxylate in solution in 20 ml of anhydrous dimethyl sulphoxide, while the temperature of the reaction mixture is maintained below 20° C. 0.44 ml of isoamyl nitrite is then added and stirring is continued for...
10.6084/m9.figshare.5104873.v1
null
Ester.Nitroso
Carboxylic acid.Oxime
c1cn2c3c(ncc2n1)c1ccccc1C3
C1c2ccccc2c2ncc3nccn3c21
C1c2ccccc2c2ncc3nccn3c21
HO-
C(C)(=O)O.CS(=O)C
null
18
CC(C)CCON=O.CCOC(=O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3>C(C)(=O)O.CS(=O)C>O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3=NO
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2183c14e46bb4ed985660d3128597a1a
CCn1c2c(n3c(Cl)c(C(=O)[O-])nc3c1=O)Cc1ccccc1-2.Cl>>O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1cc(Cl)ccc1C3
C(C)N1C(C=2N(C3=C1C=1C=CC=CC1C3)C(=C(N2)C(=O)[O-])Cl)=O.Cl>>ClC=1C=CC=2CC3=C(NC(C=4N3C=C(N4)C(=O)O)=O)C2C1
CC[n:9]1[c:8]2[c:7]([n:6]3[c:5](Cl)[c:4]([C:2](=[O:1])[O-:3])[n:13][c:12]3[c:10]1=[O:11])[CH2:21][c:20]1[c:14]-2[cH:15][cH:16][cH:18][cH:19]1.[ClH:17]>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][n:6]2[c:7]3[c:8]([nH:9][c:10](=[O:11])[c:12]2[n:13]1)-[c:14]1[cH:15][c:16]([Cl:17])[cH:18][cH:19][c:20]1[CH2:21]3
CCn1c2c(n3c(Cl)c(C(=O)[O-])nc3c1=O)Cc1ccccc1-2.Cl
O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1cc(Cl)ccc1C3
null
null
null
Miscellaneous
OtherReaction
706a38f8d4c69a067eb32b6ad403e7ad392592acd7a7a81f0af6c1b942975906
955a001693f5f4b49fc4e2fdd67dfb091f2752f79e87ea36f0c95ba0e1c73fad
O=c1[nH]c2c(n3ccnc13)Cc1ccccc1-2
C-C-[n;H0;D3;+0:1]1:[c:2](=[O;D1;H0:3]):[c:4]2:[#7;a:5]:[c:6](-[C:7](-[O-;H0;D1:8])=[O;D1;H0:9]):[c;H0;D3;+0:10](-Cl):[#7;a:11]:2:[c:12](:[c:13]:1-[c:14]:[c:15]:[cH;D2;+0:16]:[c:17]:[c:18])-[C:19].[ClH;D0;+0:20]>>[C:19]-[c:12]1:[#7;a:11]2:[cH;D2;+0:10]:[c:6](-[C:7](=[O;D1;H0:9])-[OH;D1;+0:8]):[#7;a:5]:[c:4]:2:[c:2](=[O...
null
[]
null
null
null
null
0.58 g of ethyl-chloro-4,5-dihydro-4-oxo-10H-imidazo[1,2-a]indeno[1,2-e]pyrazine-2-carboxylate in suspension in 10 ml of 6N hydrochloric acid is heated to reflux for 24 hours. After cooling to a temperature close to 20° C., the insoluble matter is filtered off, washed with water and dried under reduced pressure (1 mm H...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Aromatic halide.Carboxylic acid
c1ccc2c(c1)Cc1c2ncc2nccn12
c1ccc2c(c1)c1ncc3nccn3c1C2
c1ccc2c(c1)c1ncc3nccn3c1C2
HCl
null
null
null
CCn1c2c(n3c(Cl)c(C(=O)[O-])nc3c1=O)Cc1ccccc1-2.Cl>>O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1cc(Cl)ccc1C3
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6c6c6d89b5d34913acc93848722ce98e
CCOC(=O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3.[OH-]>>O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3=O
[OH-].[Na+].O=C1C=2N(C3=C(N1)C=1C=CC=CC1C3)C=C(N2)C(=O)OCC>>O=C1C=2N(C3=C(N1)C=1C=CC=CC1C3=O)C=C(N2)C(=O)O
CC[O:3][C:2](=[O:1])[c:4]1[cH:5][n:6]2[c:7]3[c:8]([nH:9][c:10](=[O:11])[c:12]2[n:13]1)-[c:14]1[cH:15][cH:16][cH:17][cH:18][c:19]1[CH2:20]3.[OH-:21]>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][n:6]2[c:7]3[c:8]([nH:9][c:10](=[O:11])[c:12]2[n:13]1)-[c:14]1[cH:15][cH:16][cH:17][cH:18][c:19]1[C:20]3=[O:21]
CCOC(=O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3.[OH-]
O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3=O
null
null
O1CCOCC1
Heteroatom Alkylation and Arylation
OtherReaction
6d3703b8db8a90dadf0e806464da31576a6986d3b067935416ad073a4d22d574
89fece21d142fe5b25c7ee726efca0f4579a0f2dfb61f1727c636b2f861559cc
O=C1c2ccccc2-c2[nH]c(=O)c3nccn3c21
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#7;a:5]:[c:6]2:[c:7]:[#7;a:8]:[c:9]3:[c:10](:[#7;a:11]:2:[c:12]:1)-[CH2;D2;+0:13]-[c:14](:[c:15]):[c:16]-3.[OH-;D0:17]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]1:[#7;a:5]:[c:6]2:[c:7]:[#7;a:8]:[c:9]3:[c:10](:[#7;a:11]:2:[c:12]:1)-[C;H0;D3;+0:13](=[O;H0;D1;+0:17])-[c:14](:[c:...
null
[]
null
null
null
null
5 ml of 1N sodium hydroxide are added to a suspension of 0.2 g of ethyl 4,5-dihydro-4-oxo-10H-imidazo[1,2-a]indeno[1,2-e]pyrazine-2-carboxylate in 15 ml of dioxane, and the reaction mixture is stirred vigorously while compressed air is bubbled for 15 hours. After addition of 10 ml of distilled water the mixture is acid...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid.Ketone
c1cn2c3c(ncc2n1)c1ccccc1C3
C1c2ccccc2c2ncc3nccn3c21
C1c2ccccc2c2ncc3nccn3c21
Other
O1CCOCC1
null
null
CCOC(=O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3.[OH-]>O1CCOCC1>O=C(O)c1cn2c3c([nH]c(=O)c2n1)-c1ccccc1C3=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b57a278ca83a40158214026646782b72
O=C1CCCc2ccc(OCc3ccncc3)cc21>>OC1CCCc2ccc(OCc3ccncc3)cc21
N1=CC=C(C=C1)COC1=CC=C2CCCC(C2=C1)=O.[H-].C(C(C)C)[Al+]CC(C)C>>N1=CC=C(C=C1)COC1=CC=C2CCCC(C2=C1)O
[O:1]=[C:2]1[CH2:3][CH2:4][CH2:5][c:6]2[cH:7][cH:8][c:9]([O:10][CH2:11][c:12]3[cH:13][cH:14][n:15][cH:16][cH:17]3)[cH:18][c:19]21>>[OH:1][CH:2]1[CH2:3][CH2:4][CH2:5][c:6]2[cH:7][cH:8][c:9]([O:10][CH2:11][c:12]3[cH:13][cH:14][n:15][cH:16][cH:17]3)[cH:18][c:19]21
O=C1CCCc2ccc(OCc3ccncc3)cc21
OC1CCCc2ccc(OCc3ccncc3)cc21
null
null
C1(=CC=CC=C1)C.O1CCCC1
Reduction
Reduction of ketone to secondary alcohol
3712a1f2cb52729543ec421b1a5b2fd3f779bad4223604244414834ade516040
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1cc(COc2ccc3c(c2)CCCC3)ccn1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[c:5](:[c:6]):[c:7]>>[C:1]-[C:2]-[CH;D3;+0:3](-[OH;D1;+0:4])-[c:5](:[c:6]):[c:7]
78.2
[{"value": 78.2, "product": "N1=CC=C(C=C1)COC1=CC=C2CCCC(C2=C1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of Compound 1 (16.41 g, 64.9 mmol) in tetrahydrofuran (75 mL) at 0° C. was added dropwise a 1M solution of diisobutylaluminum hydride in toluene (97.3 mL). After 1 hr, the reaction was quenched with aqueous potassium sodium tartrate and diluted with ethyl acetate followed by warming to room temperature. A...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2.c1ccncc1
null
C1(=CC=CC=C1)C.O1CCCC1
null
1
O=C1CCCc2ccc(OCc3ccncc3)cc21>C1(=CC=CC=C1)C.O1CCCC1>OC1CCCc2ccc(OCc3ccncc3)cc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e88b3e62b23f461dad90710584c27c0b
NCc1ccccc1.O=C1CCCc2ccc(OCc3ccncc3)cc21>>c1ccc(CNC2CCCc3ccc(OCc4ccncc4)cc32)cc1
N1=CC=C(C=C1)COC1=CC=C2CCCC(C2=C1)=O.C(C1=CC=CC=C1)N>>C(C1=CC=CC=C1)NC1CCCC2=CC=C(C=C12)OCC1=CC=NC=C1
[cH:1]1[cH:2][cH:3][c:4]([CH2:5][NH2:6])[cH:25][cH:26]1.O=[C:7]1[CH2:8][CH2:9][CH2:10][c:11]2[cH:12][cH:13][c:14]([O:15][CH2:16][c:17]3[cH:18][cH:19][n:20][cH:21][cH:22]3)[cH:23][c:24]21>>[cH:1]1[cH:2][cH:3][c:4]([CH2:5][NH:6][CH:7]2[CH2:8][CH2:9][CH2:10][c:11]3[cH:12][cH:13][c:14]([O:15][CH2:16][c:17]4[cH:18][cH:19][n...
NCc1ccccc1.O=C1CCCc2ccc(OCc3ccncc3)cc21
c1ccc(CNC2CCCc3ccc(OCc4ccncc4)cc32)cc1
null
null
C1=CC=CC=C1
Heteroatom Alkylation and Arylation
Reductive amination with ketone
29755ba5f0cb4006bce04ebfcf05343f0b76e87f1bf151eb9789d383875ad425
07faf85ffe990e88a1de7fd04a339bf226f78d8bfae9712ea59eebd76bb54b9f
c1ccc(CNC2CCCc3ccc(OCc4ccncc4)cc32)cc1
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[C:8]-[c:9]>>[C:3]-[C:2]-[CH;D3;+0:1](-[NH;D2;+0:7]-[C:8]-[c:9])-[c:4](:[c:5]):[c:6]
97.7
[{"value": 97.7, "product": "C(C1=CC=CC=C1)NC1CCCC2=CC=C(C=C12)OCC1=CC=NC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
30
MINUTE
A solution of Compound 1 (820 mg, 3.24 mmol) and benzyl amine (354 μL, 3.24 mmol) in benzene (10 mL) was heated to reflux under azeotropic conditions. After the calculated amount of water was collected, the reaction was cooled and concentrated in vacuo. The residue was taken-up into ethanol (5 mL) and added to a slurry...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Secondary amine
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccccc1.c1ccc2c(c1)CCCC2.c1ccncc1
Other
C1=CC=CC=C1
80
0.5
NCc1ccccc1.O=C1CCCc2ccc(OCc3ccncc3)cc21>C1=CC=CC=C1>c1ccc(CNC2CCCc3ccc(OCc4ccncc4)cc32)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-10ff625fe5984e5b87fd676cfad5e889
CCCOc1cc2c(c(OCCC)c1C)CCC(=Cc1cccnc1)C2=O>>CCCOc1cc2c(c(OCCC)c1C)CCC(Cc1cccnc1)C2=O
CC=1C(=C2CCC(C(C2=CC1OCCC)=O)=CC=1C=NC=CC1)OCCC.[H][H]>>CC=1C(=C2CCC(C(C2=CC1OCCC)=O)CC=1C=NC=CC1)OCCC
[CH3:1][CH2:2][CH2:3][O:4][c:5]1[cH:6][c:7]2[c:8]([c:9]([O:10][CH2:11][CH2:12][CH3:13])[c:14]1[CH3:15])[CH2:16][CH2:17][C:18](=[CH:19][c:20]1[cH:21][cH:22][cH:23][n:24][cH:25]1)[C:26]2=[O:27]>>[CH3:1][CH2:2][CH2:3][O:4][c:5]1[cH:6][c:7]2[c:8]([c:9]([O:10][CH2:11][CH2:12][CH3:13])[c:14]1[CH3:15])[CH2:16][CH2:17][CH:18](...
CCCOc1cc2c(c(OCCC)c1C)CCC(=Cc1cccnc1)C2=O
CCCOc1cc2c(c(OCCC)c1C)CCC(Cc1cccnc1)C2=O
null
[Pd]
CO
Reduction
Hydrogenation (double to single)
ef5776194d0a56b0d0bcb4f3f44edabcb716b463d0f1a539f552dbead062784c
0e0db21233797ec1d2a9464a1f32cef94e53e6a41f96d680fa1307067bbf01f2
O=C1c2ccccc2CCC1Cc1cccnc1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[CH;D2;+0:4]-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9])-[C:10](=[O;D1;H0:11])-[c:12]>>[C:1]-[C:2]-[CH;D3;+0:3](-[CH2;D2;+0:4]-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9])-[C:10](=[O;D1;H0:11])-[c:12]
68.5
[{"value": 68.5, "product": "CC=1C(=C2CCC(C(C2=CC1OCCC)=O)CC=1C=NC=CC1)OCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of Compound 25 (3.96 g, 10.8 mmol) and 10% palladium on carbon (600 mg) in abs. methanol (100 mL) was hydrogenated at 1 atm for 12 hr. The hydrogen was replaced with nitrogen, the reaction was filtered and concentrated in vacuo. Chromatography of the residue on silica gel (elution with 20% ethyl acetate:hexan...
10.6084/m9.figshare.5104873.v1
null
Ketone
Ketone
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2.c1ccncc1
null
[Pd].CO
null
null
CCCOc1cc2c(c(OCCC)c1C)CCC(=Cc1cccnc1)C2=O>[Pd].CO>CCCOc1cc2c(c(OCCC)c1C)CCC(Cc1cccnc1)C2=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3e15f22347a94a73bb5a31fc83b5b69f
CCOC(=O)[C@@H]1CCCNC1.N>>NC(=O)[C@@H]1CCCNC1
N1C[C@H](C(=O)OCC)CCC1.N>>N1C[C@H](C(=O)N)CCC1
CCO[C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][NH:8][CH2:9]1.[NH3:1]>>[NH2:1][C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][NH:8][CH2:9]1
CCOC(=O)[C@@H]1CCCNC1.N
NC(=O)[C@@H]1CCCNC1
null
null
null
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
C1CCNCC1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5]-[#7:6].[NH3;D0;+0:7]>>[#7:6]-[C:5]-[C:3](-[C;H0;D3;+0:1](-[NH2;D1;+0:7])=[O;D1;H0:2])-[C:4]
null
[]
null
null
3
DAY
To 14.7 g (93.5 mmol) of (R)-ethyl nipecotate in a 300 ml round-bottomed flask were added 200 ml of concentrated aqueous ammonia at room temperature, and the mixture was allowed to stand for 3 days at room temperature. The reaction mixture was distilled off at a water bath temperature of lower than 40° C. to obtain (R)...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
C1CCNCC1
HO-
null
null
72
CCOC(=O)[C@@H]1CCCNC1.N>>NC(=O)[C@@H]1CCCNC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-44351331f59d49308273d55a1a4782d5
COCC(=O)Cl.N[C@@H]1CCCN(Cc2ccccc2)C1>>COCC(=O)N[C@@H]1CCCN(Cc2ccccc2)C1
O1CCCC1.COCC(=O)Cl.O1CCCC1.C1(=CC=CC=C1)CN1C[C@@H](CCC1)N.O1CCCC1.C(C)N(CC)CC>>COCC(=O)N[C@H]1CN(CCC1)CC1=CC=CC=C1
Cl[C:4]([CH2:3][O:2][CH3:1])=[O:5].[NH2:6][C@@H:7]1[CH2:8][CH2:9][CH2:10][N:11]([CH2:12][c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[CH2:19]1>>[CH3:1][O:2][CH2:3][C:4](=[O:5])[NH:6][C@@H:7]1[CH2:8][CH2:9][CH2:10][N:11]([CH2:12][c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[CH2:19]1
COCC(=O)Cl.N[C@@H]1CCCN(Cc2ccccc2)C1
COCC(=O)N[C@@H]1CCCN(Cc2ccccc2)C1
null
null
C(Cl)Cl.O
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccc(CN2CCCCC2)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#8:4].[#7:5]-[C:6]-[C:7](-[NH2;D1;+0:8])-[C:9]>>[#7:5]-[C:6]-[C:7](-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#8:4])-[C:9]
97
[{"value": 97.0, "product": "COCC(=O)N[C@H]1CN(CCC1)CC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.8, "product": "COCC(=O)N[C@H]1CN(CCC1)CC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a 50 ml anhydrous tetrahydrofuran solution of 5.00 g (26.3 mmol) of (R)-1-phenylmethyl-3-aminopiperidine (Referential example 7) in a 300 ml three-necked flask was added a 50 ml anhydrous tetrahydrofuran solution of 3.20 g (1.2 eg.) of triethylamine, and, to this reaction mixture was added dropwise a 50 ml anhydrous...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
C1CC[NH]CC1.c1ccccc1
HCl
C(Cl)Cl.O
null
null
COCC(=O)Cl.N[C@@H]1CCCN(Cc2ccccc2)C1>C(Cl)Cl.O>COCC(=O)N[C@@H]1CCCN(Cc2ccccc2)C1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e6ecab20c64a406a8e7634f4425b54c1
COCC(=O)N[C@@H]1CCCN(Cc2ccccc2)C1>>COCCN[C@@H]1CCCN(Cc2ccccc2)C1
[H-].[Al+3].[Li+].[H-].[H-].[H-].S(=O)(=O)([O-])[O-].[Mg+2].COCC(=O)N[C@H]1CN(CCC1)CC1=CC=CC=C1.[OH-].[Na+].[H-].[Al+3].[Li+].[H-].[H-].[H-]>>COCCN[C@H]1CN(CCC1)CC1=CC=CC=C1
O=[C:4]([CH2:3][O:2][CH3:1])[NH:5][C@@H:6]1[CH2:7][CH2:8][CH2:9][N:10]([CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[CH2:18]1>>[CH3:1][O:2][CH2:3][CH2:4][NH:5][C@@H:6]1[CH2:7][CH2:8][CH2:9][N:10]([CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[CH2:18]1
COCC(=O)N[C@@H]1CCCN(Cc2ccccc2)C1
COCCN[C@@H]1CCCN(Cc2ccccc2)C1
null
null
C(C)(=O)OCC.O1CCCC1
Reduction
Reduction of secondary amides to amines
85b757f1833edc9e5c6365ee6b904683f414e7b9a5f9bfcfd7addca401447058
ab40188eef2f825df7003af0ffae31d0ce53d126542122535627d3d354cbc9fe
c1ccc(CN2CCCCC2)cc1
O=[C;H0;D3;+0:1](-[#7:2]-[C:3])-[C:4]-[#8:5]>>[#8:5]-[C:4]-[CH2;D2;+0:1]-[#7:2]-[C:3]
72
[{"value": 72.0, "product": "COCCN[C@H]1CN(CCC1)CC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 71.7, "product": "COCCN[C@H]1CN(CCC1)CC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a 50 ml anhydrous tetrahydrofuran suspension of 0.87 g (2.0 eg.) of lithium aluminum hydride in a 300 ml round-bottomed flask was added dropwise a 20 ml anhydrous tetrahydrofuran solution of 3.00 g (11.4 mmol) of (R)-3-(2-methoxyacetylamino)-1-phenylmethylpiperidine. After stirred for 1 hour at room temperature, the...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
null
null
null
C1CC[NH]CC1.c1ccccc1
Other
C(C)(=O)OCC.O1CCCC1
null
1
COCC(=O)N[C@@H]1CCCN(Cc2ccccc2)C1>C(C)(=O)OCC.O1CCCC1>COCCN[C@@H]1CCCN(Cc2ccccc2)C1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-ebab14589329403cb0aad45984b1c528
CCCCN1CCC(CO)CC1.O=C(Cl)N1c2ccccc2C2CCCCC21>>CCCCN1CCC(CC2CCCC3c4ccccc4N(C(=O)O)C23)CC1
ClC(=O)N1C2=CC=CC=C2C2CCCCC12.C1CCOC1.C(CCC)N1CCC(CC1)CO.C1CCOC1.C[Li]>>C(=O)(O)N1C2=CC=CC=C2C2CCCC(C12)CC1CCN(CC1)CCCC
[CH3:1][CH2:2][CH2:3][CH2:4][N:5]1[CH2:6][CH2:7][CH:8]([CH2:9][OH:24])[CH2:26][CH2:27]1.Cl[C:22]([N:21]1[c:20]2[c:15]([cH:16][cH:17][cH:18][cH:19]2)[CH:14]2[CH2:13][CH2:12][CH2:11][CH2:10][CH:25]21)=[O:23]>>[CH3:1][CH2:2][CH2:3][CH2:4][N:5]1[CH2:6][CH2:7][CH:8]([CH2:9][CH:10]2[CH2:11][CH2:12][CH2:13][CH:14]3[c:15]4[cH:...
CCCCN1CCC(CO)CC1.O=C(Cl)N1c2ccccc2C2CCCCC21
CCCCN1CCC(CC2CCCC3c4ccccc4N(C(=O)O)C23)CC1
null
null
null
Acylation
OtherReaction
daaa169bbd82c6bb3bc9edab65c24b8665f67e454f89501db60b5753128f8c9c
89dc7006595d86d858314bba2f7057755c60bb7654986b0568cafe8764794404
c1ccc2c(c1)NC1C(CC3CCNCC3)CCCC21
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3](-[c:4])-[C:5](-[C:6])-[CH2;D2;+0:7]-[C:8]-[C:9].[C:10]-[C:11](-[CH2;D2;+0:12]-[OH;D1;+0:13])-[C:14]>>[C:9]-[C:8]-[CH;D3;+0:7](-[CH2;D2;+0:12]-[C:11](-[C:10])-[C:14])-[C:5](-[C:6])-[#7:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[OH;D1;+0:13])-[c:4]
null
[]
null
null
10
MINUTE
1-Butyl-4-piperidinylmethanol (0.500 g 2.12 mmol) was dissolved in dry THF (3 ml) and treated with methyllithium (1.5M solution in diethyl ether) 2.16 ml, 2.33 mmol) with stirring under nitrogen. After 10 minutes, N-chlorocarbonyl-1,2,3,4,4a,9a-hexahydrocarbazole (0.630 g, 2.68 mmol) (Ref: WO 89/09217) in dry THF (5 ml...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Tertiary amide.Primary alcohol
Carbamic acid
c1ccc2c(c1)[NH]C1CCCCC21
c1ccc2c(c1)[NH]C1CCCCC21
C1CC[NH]CC1.c1ccc2c(c1)[NH]C1CCCCC21
HCl
null
null
0.166667
CCCCN1CCC(CO)CC1.O=C(Cl)N1c2ccccc2C2CCCCC21>>CCCCN1CCC(CC2CCCC3c4ccccc4N(C(=O)O)C23)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4f6016db03934931aac4c3c4d6a66417
CCCCN1CCC(CC2CCCC3c4ccccc4N(C(=O)O)C23)CC1>>CCCCN1CCC(Cc2cccc3c4ccccc4n(C(=O)O)c23)CC1
C(=O)(O)N1C2=CC=CC=C2C2CCCC(C12)CC1CCN(CC1)CCCC.ClC=1C(C(=C(C(C1Cl)=O)C#N)C#N)=O.ClC=1C(C(=C(C(C1Cl)=O)C#N)C#N)=O>>C(=O)(O)N1C2=CC=CC=C2C=2C=CC=C(C12)CC1CCN(CC1)CCCC
[CH3:1][CH2:2][CH2:3][CH2:4][N:5]1[CH2:6][CH2:7][CH:8]([CH2:9][CH:10]2[CH2:11][CH2:12][CH2:13][CH:14]3[c:15]4[cH:16][cH:17][cH:18][cH:19][c:20]4[N:21]([C:22](=[O:23])[OH:24])[CH:25]23)[CH2:26][CH2:27]1>>[CH3:1][CH2:2][CH2:3][CH2:4][N:5]1[CH2:6][CH2:7][CH:8]([CH2:9][c:10]2[cH:11][cH:12][cH:13][c:14]3[c:15]4[cH:16][cH:17...
CCCCN1CCC(CC2CCCC3c4ccccc4N(C(=O)O)C23)CC1
CCCCN1CCC(Cc2cccc3c4ccccc4n(C(=O)O)c23)CC1
null
null
C(Cl)(Cl)Cl
Oxidation
OtherReaction
235d31f3703f6d5aee1f563a32a6c415cf3b9b7d36153d01cdc413c0a36d7f52
29b8c465c2ca0e8412ed7ba786d08f9c3cb9639c5d5e81f94fec4733fdb413e6
c1ccc2c(c1)[nH]c1c(CC3CCNCC3)cccc12
[C:1]-[C:2]-[CH;D3;+0:3]1-[CH2;D2;+0:4]-[CH2;D2;+0:5]-[CH2;D2;+0:6]-[CH;D3;+0:7]2-[CH;D3;+0:8]-1-[N;H0;D3;+0:9](-[C:10](=[O;D1;H0:11])-[O;D1;H1:12])-[c:13](:[c:14]):[c:15]-2:[c:16]>>[C:1]-[C:2]-[c;H0;D3;+0:3]1:[cH;D2;+0:4]:[cH;D2;+0:5]:[cH;D2;+0:6]:[c;H0;D3;+0:7]2:[c:15](:[c:16]):[c:13](:[c:14]):[n;H0;D3;+0:9](-[C:10](...
null
[]
null
null
null
null
N-Carboxy-[1-butylpiperidin-4-ylmethyl]-1,2,3,4,4a,9a-hexahydrocarbazole (0.530 g, 1.32 mmol) was dissolved in chloroform (25 ml) and treated with 2,3-dichloro-5,6-dicyano-1, 4-benzoquinone (0.329 g, 1.58 mmol) with stirring. The mixture was heated to reflux for 12 hours, cooled, and more 2,3-dichloro-5,6-dicyano-1,4-b...
10.6084/m9.figshare.5104873.v1
null
Carbamic acid
null
c1ccc2c(c1)[NH]C1CCCCC21
c1cccc2c1[nH]c1ccccc12
C1CC[NH]CC1.c1cccc2c1[nH]c1ccccc12
null
C(Cl)(Cl)Cl
null
null
CCCCN1CCC(CC2CCCC3c4ccccc4N(C(=O)O)C23)CC1>C(Cl)(Cl)Cl>CCCCN1CCC(Cc2cccc3c4ccccc4n(C(=O)O)c23)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-33fdd502bd9b4b6ab4abded4f14a5ab2
C#CCBr.COC(=O)c1cc2ccccc2cc1O>>C#CCOc1cc2ccccc2cc1C(=O)OC
COC(=O)C1=CC2=CC=CC=C2C=C1O.[H-].[Na+].C(C#C)Br>>COC(=O)C1=CC2=CC=CC=C2C=C1OCC#C
Br[CH2:3][C:2]#[CH:1].[OH:4][c:5]1[cH:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[cH:13][c:14]1[C:15](=[O:16])[O:17][CH3:18]>>[CH:1]#[C:2][CH2:3][O:4][c:5]1[cH:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[cH:13][c:14]1[C:15](=[O:16])[O:17][CH3:18]
C#CCBr.COC(=O)c1cc2ccccc2cc1O
C#CCOc1cc2ccccc2cc1C(=O)OC
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccc2ccccc2c1
Br-[CH2;D2;+0:1]-[C:2]#[C;D1;H1:3].[#8:4]-[C:5](=[O;D1;H0:6])-[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[#8:4]-[C:5](=[O;D1;H0:6])-[c:7]:[c:8](-[O;H0;D2;+0:9]-[CH2;D2;+0:1]-[C:2]#[C;D1;H1:3]):[c:10]
35
[{"value": 35.0, "product": "COC(=O)C1=CC2=CC=CC=C2C=C1OCC#C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
0.5
HOUR
Methyl-3-hydroxy-2-naphthoate (2.63 g, 0.013 mol) was dissolved in dry THF (80 ml) and treated with sodium hydride (80%) ((0.398 g, 0.013 mol), with stirring under N2. After 0.5 h, propargyl bromide (80% in toluene) (2.57 ml 0.017 mol) was added and the mixture heated to reflux. After 20 h, the reaction mixture was all...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccc2ccccc2c1
HBr
C1CCOC1
null
0.5
C#CCBr.COC(=O)c1cc2ccccc2cc1O>C1CCOC1>C#CCOc1cc2ccccc2cc1C(=O)OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6d542e3dbdd248a898a4ea74dbd0c2eb
CCCCN1CCC(CN)CC1.Cc1nc2cc(Cl)cc(C(=O)O)c2o1>>CCCCN1CCC(CNC(=O)c2cc(Cl)cc3nc(C)oc23)CC1
C(CCC)N1CCC(CC1)CN.ClC=1C=C(C2=C(N=C(O2)C)C1)C(=O)O.C(C(=O)Cl)(=O)Cl>>C(CCC)N1CCC(CC1)CNC(=O)C1=CC(=CC=2N=C(OC21)C)Cl
[CH3:1][CH2:2][CH2:3][CH2:4][N:5]1[CH2:6][CH2:7][CH:8]([CH2:9][NH2:10])[CH2:24][CH2:25]1.O[C:11](=[O:12])[c:13]1[cH:14][c:15]([Cl:16])[cH:17][c:18]2[n:19][c:20]([CH3:21])[o:22][c:23]12>>[CH3:1][CH2:2][CH2:3][CH2:4][N:5]1[CH2:6][CH2:7][CH:8]([CH2:9][NH:10][C:11](=[O:12])[c:13]2[cH:14][c:15]([Cl:16])[cH:17][c:18]3[n:19][...
CCCCN1CCC(CN)CC1.Cc1nc2cc(Cl)cc(C(=O)O)c2o1
CCCCN1CCC(CNC(=O)c2cc(Cl)cc3nc(C)oc23)CC1
null
null
C(C)N(CC)CC
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC1CCNCC1)c1cccc2ncoc12
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]1:[#8;a:6]:[c:7]:[#7;a:8]:[c:9]:1.[C:10]-[C:11]-[NH2;D1;+0:12]>>[C:10]-[C:11]-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]1:[#8;a:6]:[c:7]:[#7;a:8]:[c:9]:1
null
[]
null
null
null
null
5-Chloro-2-methylbenzoxazole-7-carboxylic acid (Ger. Offen. 2,225,544) is converted to its acid chloride by treatment with oxalyl chloride. The acid chloride is treated with N-(1-butyl-4-piperidinyl)methylamine in the presence of triethylamine to afford the title compound. Conditions: See reaction.notes.procedure_detai...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CC[NH]CC1.c1ccc2ocnc2c1
HO-
C(C)N(CC)CC
null
null
CCCCN1CCC(CN)CC1.Cc1nc2cc(Cl)cc(C(=O)O)c2o1>C(C)N(CC)CC>CCCCN1CCC(CNC(=O)c2cc(Cl)cc3nc(C)oc23)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6320ae92480446599727eaa48b88a8bc
O=[N+]([O-])c1cccc(S(=O)(=O)Nc2ccc3nsnc3c2)c1>>Nc1cccc(S(=O)(=O)Nc2ccc3nsnc3c2)c1
[N+](=O)([O-])C=1C=C(C=CC1)S(=O)(=O)NC1=CC=2C(=NSN2)C=C1>>NC=1C=C(C=CC1)S(=O)(=O)NC1=CC=2C(=NSN2)C=C1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][cH:5][c:6]([S:7](=[O:8])(=[O:9])[NH:10][c:11]2[cH:12][cH:13][c:14]3[n:15][s:16][n:17][c:18]3[cH:19]2)[cH:20]1>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][c:6]([S:7](=[O:8])(=[O:9])[NH:10][c:11]2[cH:12][cH:13][c:14]3[n:15][s:16][n:17][c:18]3[cH:19]2)[cH:20]1
O=[N+]([O-])c1cccc(S(=O)(=O)Nc2ccc3nsnc3c2)c1
Nc1cccc(S(=O)(=O)Nc2ccc3nsnc3c2)c1
null
[Ni]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
O=S(=O)(Nc1ccc2nsnc2c1)c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
A solution of 1 g of 3-nitro-N-(2,1,3-benzothiadiazol-5-yl)-1-benzenesulfonamide in 25 ml of methanol is hydrogenated to completion on 1 g of Raney Nickel at normal pressure and 20°. The solution is filtered, evaporated and 3-amino-N-(2,1,3-benzothiadiazol-5-yl)-1-benzenesulfonamide is obtained. Conditions: See reactio...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccc2nsnc2c1
Other
[Ni].CO
null
null
O=[N+]([O-])c1cccc(S(=O)(=O)Nc2ccc3nsnc3c2)c1>[Ni].CO>Nc1cccc(S(=O)(=O)Nc2ccc3nsnc3c2)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4f6afdd55a85475bb49ce92f2b6145ed
CCc1ccccc1S(=O)(=O)Cl.Nc1ccc2nonc2c1>>CCc1ccccc1S(=O)(=O)Nc1ccc2nonc2c1
NC1=CC=2C(=NON2)C=C1.C(C)C1=C(C=CC=C1)S(=O)(=O)Cl>>C(C)C1=C(C=CC=C1)S(=O)(=O)NC1=CC=2C(=NON2)C=C1
Cl[S:9]([c:8]1[c:3]([CH2:2][CH3:1])[cH:4][cH:5][cH:6][cH:7]1)(=[O:10])=[O:11].[NH2:12][c:13]1[cH:14][cH:15][c:16]2[n:17][o:18][n:19][c:20]2[cH:21]1>>[CH3:1][CH2:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1[S:9](=[O:10])(=[O:11])[NH:12][c:13]1[cH:14][cH:15][c:16]2[n:17][o:18][n:19][c:20]2[cH:21]1
CCc1ccccc1S(=O)(=O)Cl.Nc1ccc2nonc2c1
CCc1ccccc1S(=O)(=O)Nc1ccc2nonc2c1
null
null
null
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccc2nonc2c1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[#7;a:7]:[c:8]:[c:9]:[c:10](-[NH2;D1;+0:11]):[c:12]>>[#7;a:7]:[c:8]:[c:9]:[c:10](-[NH;D2;+0:11]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]):[c:12]
null
[]
null
null
null
null
Analogously to Example 1, by reaction of 5-amino-2,1,3-benzoxadiazole (obtainable by reduction of 5-nitro-2,1,3-benzoxadiazole-1- or 3-N-oxide with triethyl phosphite) with 2-ethylbenzenesulfonyl chloride, 2-ethyl-N-(2,1,3-benzoxadiazol-5-yl)-1-benzenesulfonamide is obtained. Conditions: See reaction.notes.procedure_de...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2nonc2c1
HCl
null
null
null
CCc1ccccc1S(=O)(=O)Cl.Nc1ccc2nonc2c1>>CCc1ccccc1S(=O)(=O)Nc1ccc2nonc2c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7917d2b512334ae09464c8fd110ae2ba
CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1Br>>CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C#N
CN(C1=C2C=CC=C(C2=CC=C1)S(=O)(=O)NC1=C(C(=CC2=NON=C21)CC)Br)C.[Cu](C#N)C#N.N>>CN(C1=C2C=CC=C(C2=CC=C1)S(=O)(=O)NC1=C(C(=CC2=NON=C21)CC)C#N)C
Br[c:28]1[c:3]([CH2:2][CH3:1])[cH:4][c:5]2[n:6][o:7][n:8][c:9]2[c:10]1[NH:11][S:12](=[O:13])(=[O:14])[c:15]1[cH:16][cH:17][cH:18][c:19]2[c:20]([N:21]([CH3:22])[CH3:23])[cH:24][cH:25][cH:26][c:27]12>>[CH3:1][CH2:2][c:3]1[cH:4][c:5]2[n:6][o:7][n:8][c:9]2[c:10]([NH:11][S:12](=[O:13])(=[O:14])[c:15]2[cH:16][cH:17][cH:18][c...
CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1Br
CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C#N
null
null
N1=CC=CC=C1
Miscellaneous
OtherReaction
b5ec4c140b1cbe117e9bb656507e270a1fb4a9a3ce34a67d4138d3e556f53979
73a96fe5e833259ca394a42f82d6cc2ee7231bcde92d95030d2893b90c3fef76
O=S(=O)(Nc1cccc2nonc12)c1cccc2ccccc12
Br-[c;H0;D3;+0:1]1:[c:2](-[#7:3]):[c:4]2:[#7;a:5]:[#8;a:6]:[#7;a:7]:[c:8]:2:[c:9]:[c:10]:1-[C:11]>>[#7:3]-[c:2]1:[c:4]2:[#7;a:5]:[#8;a:6]:[#7;a:7]:[c:8]:2:[c:9]:[c:10](-[C:11]):[c;H0;D3;+0:1]:1-[C:12]#[N;D1;H0:13]
null
[]
null
null
null
null
A mixture of 4.6 g of 5-dimethylamino-N-(5-bromo-6-ethyl-2,1,3-benzoxadiazol-4-yl)-1-naphthalenesulfonamide and 1.3 g of copper cyanide is heated for 8 hours at 120° in 30 ml of pyridine. The mixture is poured onto aqueous ammonia solution, worked up in the customary manner and 5-dimethylamino- N-(5-cyano-6-ethyl-2,1,3...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Nitrile
c1ccc2nonc2c1
c1ccc2nonc2c1
c1ccc2nonc2c1.c1ccc2ccccc2c1
Br-
N1=CC=CC=C1
null
null
CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1Br>N1=CC=CC=C1>CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C#N
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-f96c52e9536a47d1afa277c765192b43
CCO.CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C#N.[OH-]>>CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C(=O)O
CN(C1=C2C=CC=C(C2=CC=C1)S(=O)(=O)NC1=C(C(=CC2=NON=C21)CC)C#N)C.[OH-].[K+].C(C)O>>CN(C1=C2C=CC=C(C2=CC=C1)S(=O)(=O)NC1=C(C(=CC2=NON=C21)CC)C(=O)O)C
CC[OH:30].N#[C:29][c:28]1[c:3]([CH2:2][CH3:1])[cH:4][c:5]2[n:6][o:7][n:8][c:9]2[c:10]1[NH:11][S:12](=[O:13])(=[O:14])[c:15]1[cH:16][cH:17][cH:18][c:19]2[c:20]([N:21]([CH3:22])[CH3:23])[cH:24][cH:25][cH:26][c:27]12.[OH-:31]>>[CH3:1][CH2:2][c:3]1[cH:4][c:5]2[n:6][o:7][n:8][c:9]2[c:10]([NH:11][S:12](=[O:13])(=[O:14])[c:15...
CCO.CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C#N.[OH-]
CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C(=O)O
null
null
O
Acylation
OtherReaction
e41cdaf6ecb9257286a05c8e01433d124042c5939fb4d758964487a1f4637b56
e38d1b350c527156572f58ef95bb65354ed43ce776b83f166b6fd042d5d9aca9
O=S(=O)(Nc1cccc2nonc12)c1cccc2ccccc12
C-C-[OH;D1;+0:1].N#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]:[c:6]:[#7;a:7].[OH-;D0:8]>>[#7;a:7]:[c:6]:[c:5]:[c:3](-[C;H0;D3;+0:2](=[O;H0;D1;+0:1])-[OH;D1;+0:8]):[c:4]
null
[]
null
null
8
HOUR
A solution of 1 g of 5-dimethylamino-N-(5-cyano-6-ethyl-2,1,3-benzoxadiazol-4-yl)-1-naphthalenesulfonamide and 0.7 g of potassium hydroxide in 20 ml of ethanol and 5 ml of water is bailed with stirring for 8 hours. The solvents are removed, the residue is dissolved in water and treated with hydrochloric acid and 5-dime...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary alcohol
Carboxylic acid
null
null
c1ccc2nonc2c1.c1ccc2ccccc2c1
Other
O
null
8
CCO.CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C#N.[OH-]>O>CCc1cc2nonc2c(NS(=O)(=O)c2cccc3c(N(C)C)cccc23)c1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a7fa891adf0d455598641c30d6e12a91
CC=O.Nc1ccc(S(=O)(=O)Nc2ccc3nsnc3c2)cc1>>CCNc1ccc(S(=O)(=O)Nc2ccc3nsnc3c2)cc1
Cl.NC1=CC=C(C=C1)S(=O)(=O)NC1=CC=2C(=NSN2)C=C1.C(C)=O.C(#N)[BH3-].[Na+]>>C(C)NC1=CC=C(C=C1)S(=O)(=O)NC1=CC=2C(=NSN2)C=C1
O=[CH:2][CH3:1].[NH2:3][c:4]1[cH:5][cH:6][c:7]([S:8](=[O:9])(=[O:10])[NH:11][c:12]2[cH:13][cH:14][c:15]3[n:16][s:17][n:18][c:19]3[cH:20]2)[cH:21][cH:22]1>>[CH3:1][CH2:2][NH:3][c:4]1[cH:5][cH:6][c:7]([S:8](=[O:9])(=[O:10])[NH:11][c:12]2[cH:13][cH:14][c:15]3[n:16][s:17][n:18][c:19]3[cH:20]2)[cH:21][cH:22]1
CC=O.Nc1ccc(S(=O)(=O)Nc2ccc3nsnc3c2)cc1
CCNc1ccc(S(=O)(=O)Nc2ccc3nsnc3c2)cc1
null
[Ti](Cl)(Cl)(Cl)Cl
CO
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
O=S(=O)(Nc1ccc2nsnc2c1)c1ccccc1
O=[CH;D2;+0:1]-[C;D1;H3:2].[NH2;D1;+0:3]-[c:4](:[c:5]):[c:6]>>[C;D1;H3:2]-[CH2;D2;+0:1]-[NH;D2;+0:3]-[c:4](:[c:5]):[c:6]
null
[]
null
null
30
HOUR
A solution of 6 g of 4-amino-N-(2,1,3-benzothiadiazol-5-yl)-1-benzenesulfonamide and 0.5 g of titanium tetrachloride in 100 ml of methanol is treated with 1 ml of freshly distilled acetaldehyde. 4 g of sodium cyanoborohydride are then added thereto and the mixture is stirred for 30 hours. Cold half-concentrated hydroch...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccc2nsnc2c1
Other
[Ti](Cl)(Cl)(Cl)Cl.CO
null
30
CC=O.Nc1ccc(S(=O)(=O)Nc2ccc3nsnc3c2)cc1>[Ti](Cl)(Cl)(Cl)Cl.CO>CCNc1ccc(S(=O)(=O)Nc2ccc3nsnc3c2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-ffa107eae87c458391df6e58d5d78f6e
C[Si](C)(C)N=[N+]=[N-].N#Cc1ccc(Oc2ccccc2)cc1>>c1ccc(Oc2ccc(-c3nnn[nH]3)cc2)cc1
O(C1=CC=CC=C1)C1=CC=C(C#N)C=C1.C(CCC)[Sn](CCCC)=O.C[Si](C)(C)N=[N+]=[N-]>>O(C1=CC=CC=C1)C1=CC=C(C=C1)C1=NN=NN1
C[Si](C)(C)[N:14]=[N+:13]=[N-:12].[cH:1]1[cH:2][cH:3][c:4]([O:5][c:6]2[cH:7][cH:8][c:9]([C:10]#[N:11])[cH:15][cH:16]2)[cH:17][cH:18]1>>[cH:1]1[cH:2][cH:3][c:4]([O:5][c:6]2[cH:7][cH:8][c:9](-[c:10]3[n:11][n:12][n:13][nH:14]3)[cH:15][cH:16]2)[cH:17][cH:18]1
C[Si](C)(C)N=[N+]=[N-].N#Cc1ccc(Oc2ccccc2)cc1
c1ccc(Oc2ccc(-c3nnn[nH]3)cc2)cc1
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
22a456949a340700c38f1369557e2324d3627ca94291920d5593a13d13f086c0
b0b652611f3449be50404e3527083f5e03f8f4207de666d5db2f0953bd23d0a3
c1ccc(Oc2ccc(-c3nnn[nH]3)cc2)cc1
C-[Si](-C)(-C)-[N;H0;D2;+0:1]=[N+;H0;D2:2]=[N-;H0;D1:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:5]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:3]:[n;H0;D2;+0:2]:[nH;D2;+0:1]:1):[c:9]:[c:10]
null
[]
null
null
null
null
A solution of 4-phenoxybenzonitrile (9.87 g), dibutyltin oxide (3.88 g), and trimethylsilyl azide (33.5 ml) in anhydrous toluene (200 ml) was heated to reflux for 6 hours. The reaction mixture was washed with 1.6M sodium hydroxide (2×250 ml). The combined aqueous layer was washed with diethyl ether (4×120 ml) then acid...
10.6084/m9.figshare.5104873.v1
null
Azide.Nitrile.Silyl protective group
null
null
c1nnn[nH]1
c1ccccc1.c1ccccc1.c1nnn[nH]1
Other
C1(=CC=CC=C1)C
null
null
C[Si](C)(C)N=[N+]=[N-].N#Cc1ccc(Oc2ccccc2)cc1>C1(=CC=CC=C1)C>c1ccc(Oc2ccc(-c3nnn[nH]3)cc2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-fd2ce529eb5e4230a968d9b7a9207cfc
C#Cc1ccc(C#N)cc1.O=[N+]([O-])c1ccc(Br)o1>>N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])o2)cc1
BrC=1OC(=CC1)[N+](=O)[O-].C(C)N(CC)CC.C(#C)C1=CC=C(C#N)C=C1>>[N+](=O)([O-])C1=CC=C(O1)C#CC1=CC=C(C#N)C=C1
[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([C:7]#[CH:8])[cH:17][cH:18]1.Br[c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[o:16]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([C:7]#[C:8][c:9]2[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[o:16]2)[cH:17][cH:18]1
C#Cc1ccc(C#N)cc1.O=[N+]([O-])c1ccc(Br)o1
N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])o2)cc1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
C(C)#N
C-C Coupling
Sonogashira alkyne_aryl halide
85c427816ae28bd4dbb19650a00c34ca6489eaef6ce7658febdd08dde476e105
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
C(#Cc1ccco1)c1ccccc1
Br-[c;H0;D3;+0:1]1:[#8;a:2]:[c:3]:[c:4]:[c:5]:1.[CH;D1;+0:6]#[C:7]-[c:8]>>[c:8]-[C:7]#[C;H0;D2;+0:6]-[c;H0;D3;+0:1]1:[#8;a:2]:[c:3]:[c:4]:[c:5]:1
null
[]
null
null
8
HOUR
To a solution of 2-bromo-5-nitrofuran (1.65 g) and triethylamine (34 ml) in anhydrous acetonitrile (55 ml) under nitrogen was added bis(triphenylphosphine)palladium dichloride (130 mg) and cuprous iodide (35 mg). 4-Ethynylbenzonitrile (1.09 g) was added and the reaction mixture was stirred under nitrogen overnight. The...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1ccoc1
c1ccoc1
c1ccccc1.c1ccoc1
HBr
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.C(C)#N
null
8
C#Cc1ccc(C#N)cc1.O=[N+]([O-])c1ccc(Br)o1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.C(C)#N>N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])o2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-f537d62089cd4cba9bc833054c2f705b
C#Cc1ccc(C#N)cc1.O=[N+]([O-])c1ccc(Br)s1>>N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])s2)cc1
[Cl-].[Na+].C(#C)C1=CC=C(C#N)C=C1.BrC=1SC(=CC1)[N+](=O)[O-].C(C)N(CC)CC>>[N+](=O)([O-])C1=CC=C(S1)C#CC1=CC=C(C#N)C=C1
[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([C:7]#[CH:8])[cH:17][cH:18]1.Br[c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[s:16]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([C:7]#[C:8][c:9]2[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[s:16]2)[cH:17][cH:18]1
C#Cc1ccc(C#N)cc1.O=[N+]([O-])c1ccc(Br)s1
N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])s2)cc1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
CN(C=O)C.C(C)(=O)OCC
C-C Coupling
Sonogashira alkyne_aryl halide
80f1154e8228406a6c3574cdd1c2a206480f305ea213bae402b2ac8502ab2f9e
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
C(#Cc1cccs1)c1ccccc1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1.[CH;D1;+0:6]#[C:7]-[c:8]>>[c:8]-[C:7]#[C;H0;D2;+0:6]-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1
null
[]
null
null
3
DAY
To a solution of 4-ethynylbenzonitrile (0.5 g), 2-bromo-5-nitrothiophene (0.9 g) and bis(triphenylphosphine)palladium dichloride (83 mg) in anhydrous dimethylformamide (4 ml) was added triethylamine (2.2 ml). The reaction mixture was stirred at room temperature for 3 days then ethyl acetate (200 ml) and saturated sodiu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1ccsc1
c1ccsc1
c1ccccc1.c1ccsc1
HBr
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C=O)C.C(C)(=O)OCC
null
72
C#Cc1ccc(C#N)cc1.O=[N+]([O-])c1ccc(Br)s1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C=O)C.C(C)(=O)OCC>N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])s2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-ba45a428014e4c71895cdbed1fea1c2d
C[Si](C)(C)N=[N+]=[N-].N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])s2)cc1>>O=[N+]([O-])c1ccc(C#Cc2ccc(-c3nnn[nH]3)cc2)s1
[N+](=O)([O-])C1=CC=C(S1)C#CC1=CC=C(C#N)C=C1.C(CCC)[Sn](CCCC)=O.C[Si](C)(C)N=[N+]=[N-]>>[N+](=O)([O-])C1=CC=C(S1)C#CC1=CC=C(C=C1)C1=NN=NN1
C[Si](C)(C)[N:18]=[N+:16]=[N-:17].[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([C:8]#[C:9][c:10]2[cH:11][cH:12][c:13]([C:14]#[N:15])[cH:19][cH:20]2)[s:21]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([C:8]#[C:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[n:15][n:16][n:17][nH:18]3)[cH:19][cH:20]2)[s:21]1
C[Si](C)(C)N=[N+]=[N-].N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])s2)cc1
O=[N+]([O-])c1ccc(C#Cc2ccc(-c3nnn[nH]3)cc2)s1
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
22a456949a340700c38f1369557e2324d3627ca94291920d5593a13d13f086c0
b0b652611f3449be50404e3527083f5e03f8f4207de666d5db2f0953bd23d0a3
C(#Cc1cccs1)c1ccc(-c2nnn[nH]2)cc1
C-[Si](-C)(-C)-[N;H0;D2;+0:1]=[N+;H0;D2:2]=[N-;H0;D1:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:5]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:2]:[n;H0;D2;+0:3]:[nH;D2;+0:1]:1):[c:9]:[c:10]
null
[]
null
null
null
null
To a solution of 4-[(5-nitro-2-thienyl)ethynyl]benzonitrile (0.6 g) and dibutyltin oxide (59 mg) in anhydrous toluene (30 ml) was added trimethylsilyl azide (0.5 ml). The reaction mixture was heated to reflux in the dark for 12 hours, then allowed to cool to room temperature. The reaction mixture was washed with satura...
10.6084/m9.figshare.5104873.v1
null
Azide.Nitrile.Silyl protective group
null
null
c1nnn[nH]1
c1ccsc1.c1ccccc1.c1nnn[nH]1
Other
C1(=CC=CC=C1)C
null
null
C[Si](C)(C)N=[N+]=[N-].N#Cc1ccc(C#Cc2ccc([N+](=O)[O-])s2)cc1>C1(=CC=CC=C1)C>O=[N+]([O-])c1ccc(C#Cc2ccc(-c3nnn[nH]3)cc2)s1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-25fc14e42f424677aa73d3c6c5b9ae9d
C[Si](C)(C)N=[N+]=[N-].N#CCc1ccc(Oc2ccccc2)cc1>>c1ccc(Oc2ccc(Cc3nnn[nH]3)cc2)cc1
[OH-].[Na+].O(C1=CC=CC=C1)C1=CC=C(C=C1)CC#N.C[Si](C)(C)N=[N+]=[N-].C(CCC)[Sn](CCCC)=O>>O(C1=CC=CC=C1)C1=CC=C(C=C1)CC1=NN=NN1
C[Si](C)(C)[N:15]=[N+:13]=[N-:14].[cH:1]1[cH:2][cH:3][c:4]([O:5][c:6]2[cH:7][cH:8][c:9]([CH2:10][C:11]#[N:12])[cH:16][cH:17]2)[cH:18][cH:19]1>>[cH:1]1[cH:2][cH:3][c:4]([O:5][c:6]2[cH:7][cH:8][c:9]([CH2:10][c:11]3[n:12][n:13][n:14][nH:15]3)[cH:16][cH:17]2)[cH:18][cH:19]1
C[Si](C)(C)N=[N+]=[N-].N#CCc1ccc(Oc2ccccc2)cc1
c1ccc(Oc2ccc(Cc3nnn[nH]3)cc2)cc1
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
22a456949a340700c38f1369557e2324d3627ca94291920d5593a13d13f086c0
b0b652611f3449be50404e3527083f5e03f8f4207de666d5db2f0953bd23d0a3
c1ccc(Oc2ccc(Cc3nnn[nH]3)cc2)cc1
C-[Si](-C)(-C)-[N;H0;D2;+0:1]=[N+;H0;D2:2]=[N-;H0;D1:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[C:6]-[c:7]>>[c:7]-[C:6]-[c;H0;D3;+0:5]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:2]:[n;H0;D2;+0:3]:[nH;D2;+0:1]:1
null
[]
null
null
null
null
To a solution of 4-phenoxyphenylacetonitrile (1.16 g) in anhydrous toluene (30 ml) was added trimethylsilylazide (1.1 ml) and dibutyltin oxide (0.19 g). The mixture was heated to reflux for 19 hours then allowed to cool to room temperature. The reaction mixture was then added to 1M sodium hydroxide (100 ml) and washed ...
10.6084/m9.figshare.5104873.v1
null
Azide.Nitrile.Silyl protective group
null
null
c1nnn[nH]1
c1ccccc1.c1ccccc1.c1nnn[nH]1
Other
C1(=CC=CC=C1)C
null
null
C[Si](C)(C)N=[N+]=[N-].N#CCc1ccc(Oc2ccccc2)cc1>C1(=CC=CC=C1)C>c1ccc(Oc2ccc(Cc3nnn[nH]3)cc2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9c7cc9bbc71144c7ae9f1e2d0e680324
O=C1NC(=O)c2cc(Cl)ccc21>>Clc1cccc2c1CNC2
ClC=1C=C2C(C(=O)NC2=O)=CC1.Cl>>ClC1=C2CNCC2=CC=C1
O=[C:8]1[c:7]2[cH:2][c:3]([Cl:1])[cH:4][cH:5][c:6]2[C:10](=O)[NH:9]1>>[Cl:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[CH2:8][NH:9][CH2:10]2
O=C1NC(=O)c2cc(Cl)ccc21
Clc1cccc2c1CNC2
null
null
O1CCCC1
Functional Group Addition
OtherReaction
106327c249cf5b274d3cd701f19740fc83f3bb2c9dcfabcd3e04bdc802a8246e
c611a163eef2f0598d60d9d37ad9b17d64e4ef0dbf9dfba690515b4ad6bf1fa7
c1ccc2c(c1)CNC2
O=[C;H0;D3;+0:1]1-[#7:2]-[C;H0;D3;+0:3](=O)-[c:4]2:[cH;D2;+0:5]:[c;H0;D3;+0:6](-[Cl;H0;D1;+0:7]):[c:8]:[c:9]:[c:10]:2-1>>[Cl;H0;D1;+0:7]-[c;H0;D3;+0:5]1:[cH;D2;+0:6]:[c:8]:[c:9]:[c:10]2:[c:4]:1-[CH2;D2;+0:3]-[#7:2]-[CH2;D2;+0:1]-2
null
[]
null
null
null
null
To a solution of 4-chlorophthalimide (60 g) in 1 liter of tetrahydrofuran was added borane-methyl sulfide complex (100 ml of 10M), and the mixture was refluxed overnight. After cooling, 100 ml of 6N hydrochloric acid was added slowly, the mixture refluxed for 2 hours, and then filtered. The filtrate was concentrated un...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Unsubstituted dicarboximide
Aromatic halide
c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2
Other
O1CCCC1
null
null
O=C1NC(=O)c2cc(Cl)ccc21>O1CCCC1>Clc1cccc2c1CNC2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0591013fd92545f5bf5092992c26919f
CSC1=NCCS1.Clc1cccc2c1CNC2>>Clc1cccc2c1CN(C1=NCCS1)C2
ClC1=C2CNCC2=CC=C1.CSC=1SCCN1.C1=C(C=CC2=CC=CC=C12)S(=O)(=O)O>>ClC1=C2CN(CC2=CC=C1)C=1SCCN1
CS[C:10]1=[N:11][CH2:12][CH2:13][S:14]1.[Cl:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[CH2:8][NH:9][CH2:15]2>>[Cl:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[CH2:8][N:9]([C:10]1=[N:11][CH2:12][CH2:13][S:14]1)[CH2:15]2
CSC1=NCCS1.Clc1cccc2c1CNC2
Clc1cccc2c1CN(C1=NCCS1)C2
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
a668efb51512d8228bf8a4303df72f4ce701e31a18e7cebe5b171cd8ab0c703e
bfc582950bdf0b5fb9b3d55b1008f32b1f1c2ec643ca7f4d617bfc2865cc9bc5
c1ccc2c(c1)CN(C1=NCCS1)C2
C-S-[C;H0;D3;+0:1]1=[#7:2]-[C:3]-[C:4]-[#16:5]-1.[C:6]1-[NH;D2;+0:7]-[C:8]-[c:9]:[c:10]-1>>[#16:5]1-[C:4]-[C:3]-[#7:2]=[C;H0;D3;+0:1]-1-[N;H0;D3;+0:7]1-[C:6]-[c:10]:[c:9]-[C:8]-1
null
[]
150
CELSIUS
null
null
A mixture of 4-chloroisoindoline (700 mg), 2-methylthio-2-thiazoline (600 mg), and β-naphthylsulfonic acid (35 mg) was heated at 150° C. for 30 minutes. The product was cooled, dissolved in methylene chloride, washed with water, the organic layer dried over anhydrous potassium carbonate, filtered, and solvent removed f...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Monosulfide.Monosulfide
Tertiary amine.Monosulfide
C1=NCCS1.c1ccc2c(c1)CNC2
c1ccc2c(c1)C[NH]C2.C1=NCCS1
c1ccc2c(c1)C[NH]C2.C1=NCCS1
Other
C(Cl)Cl
150
null
CSC1=NCCS1.Clc1cccc2c1CNC2>C(Cl)Cl>Clc1cccc2c1CN(C1=NCCS1)C2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0aed4da618f94372b6ebcb5dce352131
CCOC1=NCCO1.Fc1cccc2c1CNC2>>Fc1cccc2c1CN(C1=NCCO1)C2
FC1=C2CNCC2=CC=C1.C(C)OC=1OCCN1.C1=C(C=CC2=CC=CC=C12)S(=O)(=O)O>>FC1=C2CN(CC2=CC=C1)C=1OCCN1
CCO[C:10]1=[N:11][CH2:12][CH2:13][O:14]1.[F:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[CH2:8][NH:9][CH2:15]2>>[F:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[CH2:8][N:9]([C:10]1=[N:11][CH2:12][CH2:13][O:14]1)[CH2:15]2
CCOC1=NCCO1.Fc1cccc2c1CNC2
Fc1cccc2c1CN(C1=NCCO1)C2
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
Displacement of ethoxy group by secondary amine
f6da5addeff690dff47c54c98a2b6a6446d1a91d82b399c0daec008e45bdf8b7
d8eb8c9b1e09b7f4b257948057ae13ffa7a454df2815ac36c03139e6598690c5
c1ccc2c(c1)CN(C1=NCCO1)C2
C-C-O-[C;H0;D3;+0:1]1=[#7:2]-[C:3]-[C:4]-[#8:5]-1.[C:6]1-[NH;D2;+0:7]-[C:8]-[c:9]:[c:10]-1>>[#7:2]1=[C;H0;D3;+0:1](-[N;H0;D3;+0:7]2-[C:6]-[c:10]:[c:9]-[C:8]-2)-[#8:5]-[C:4]-[C:3]-1
null
[]
100
CELSIUS
1
HOUR
A mixture of 4-fluoroisoindoline (400 mg), 2-ethoxy-2-oxazoline (400 mg), and β-naphthylsulfonic acid (30 mg) in 50 ml of toluene was stirred at 100° C. for 1 hour. The solvent as removed under reduced pressure, and the residue chromatographed on silica gel, eluting with 1-4% methanol in ethyl acetate, to give 4-fluoro...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary amine
Ether.Tertiary amine
C1=NCCO1.c1ccc2c(c1)CNC2
c1ccc2c(c1)C[NH]C2.C1=NCCO1
c1ccc2c(c1)C[NH]C2.C1=NCCO1
HO-
C1(=CC=CC=C1)C
100
1
CCOC1=NCCO1.Fc1cccc2c1CNC2>C1(=CC=CC=C1)C>Fc1cccc2c1CN(C1=NCCO1)C2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c4710f63ab8144a9acdfc1350b467c98
CCCCCCc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C.O=C(OCc1ccccc1)c1ccc(O)nc1>>CCCCCCc1cc2c(cc1C(=O)Oc1ccc(C(=O)OCc3ccccc3)cn1)C(C)(C)CCC2(C)C
C(CCCCC)C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C(=O)O.OC1=NC=C(C(=O)OCC2=CC=CC=C2)C=C1.C1(CCCCC1)N=C=NC1CCCCC1>>C(CCCCC)C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C(=O)OC1=NC=C(C(=O)OCC2=CC=CC=C2)C=C1
O[C:13]([c:12]1[c:7]([CH2:6][CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[cH:8][c:9]2[c:10]([cH:11]1)[C:32]([CH3:33])([CH3:34])[CH2:35][CH2:36][C:37]2([CH3:38])[CH3:39])=[O:14].[OH:15][c:16]1[cH:17][cH:18][c:19]([C:20](=[O:21])[O:22][CH2:23][c:24]2[cH:25][cH:26][cH:27][cH:28][cH:29]2)[cH:30][n:31]1>>[CH3:1][CH2:2][CH2:3][CH2:4]...
CCCCCCc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C.O=C(OCc1ccccc1)c1ccc(O)nc1
CCCCCCc1cc2c(cc1C(=O)Oc1ccc(C(=O)OCc3ccccc3)cn1)C(C)(C)CCC2(C)C
null
CN(C1=CC=NC=C1)C
C(Cl)Cl
Acylation
Mitsunobu esterification
f18451ac648b00cb7c6684a3e64bee855b0320c7eb0f62b757b29d5fb6745560
1489fe0065c6531b60fda87a3857d7da1cd21873868856f058c20706f927fa08
O=C(OCc1ccccc1)c1ccc(OC(=O)c2ccc3c(c2)CCCC3)nc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[O;H0;D2;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:3](:[c:4]):[c:5]
57
[{"value": 57.0, "product": "C(CCCCC)C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C(=O)OC1=NC=C(C(=O)OCC2=CC=CC=C2)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
2
HOUR
6 g of 3-hexyl-5,5,8,8-tetramethyl-5,6,7,8-tetrahydro-naphthalen-2-yl-carboxylic acid were dissolved in 180 ml of methylene chloride. After the addition of a solution of 4.8 g of benzyl 6-hydroxy-nicotinate in 160 ml of methylene chloride and of 2.3 g of 4-dimethylaminopyridine, the solution was cooled to 0° C. and tre...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Aromatic alcohol
Ester
null
null
c1ccncc1.c1ccccc1.c1ccc2c(c1)CCCC2
HO-
CN(C1=CC=NC=C1)C.C(Cl)Cl
0
2
CCCCCCc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C.O=C(OCc1ccccc1)c1ccc(O)nc1>CN(C1=CC=NC=C1)C.C(Cl)Cl>CCCCCCc1cc2c(cc1C(=O)Oc1ccc(C(=O)OCc3ccccc3)cn1)C(C)(C)CCC2(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4d21f97b1712426ea5d91e06fbf86981
CCCCCCc1cc2c(cc1Br)C(C)(C)CCC2(C)C.O=C=O>>CCCCCCc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C
C(=O)=O.C(C)(C)(C)[Li].BrC=1C=C2C(CCC(C2=CC1CCCCCC)(C)C)(C)C.Cl>>C(CCCCC)C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C(=O)O
Br[c:12]1[c:7]([CH2:6][CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[cH:8][c:9]2[c:10]([cH:11]1)[C:16]([CH3:17])([CH3:18])[CH2:19][CH2:20][C:21]2([CH3:22])[CH3:23].[C:13](=[O:14])=[O:15]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][c:7]1[cH:8][c:9]2[c:10]([cH:11][c:12]1[C:13](=[O:14])[OH:15])[C:16]([CH3:17])([CH3:18])[CH2:19][CH2...
CCCCCCc1cc2c(cc1Br)C(C)(C)CCC2(C)C.O=C=O
CCCCCCc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C
null
null
CCCCC.O1CCCC1
Acylation
OtherReaction
2c77db6aaec596a76b7a465634b3055972748ecc9b259d7fb098a14192761a6e
d0d963f3850574b1f0fda744314036458b2dd627cb0c4e2f893b9c52a88ad449
c1ccc2c(c1)CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C:5]):[c:6].[O;D1;H0:7]=[C;H0;D2;+0:8]=[O;H0;D1;+0:9]>>[C:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[C;H0;D3;+0:8](=[O;D1;H0:7])-[OH;D1;+0:9]):[c:2]:[c:3]
null
[]
-78
CELSIUS
1
HOUR
15 g of 6-bromo-7-hexyl-1,1,4,4-tetramethyl-1, 2,3,4-tetrahydro-naphthalene were dissolved in 180 ml of tetrahydrofuran and treated dropwise at -78° C. with 64.5 ml of a 1.5 molar solution of tert.butyl-lithium in pentane. After stirring at -78° C. for 1 hour, a carbon dioxide stream was conducted vigorously into the r...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carbon dioxide
Carboxylic acid
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
Br-
CCCCC.O1CCCC1
-78
1
CCCCCCc1cc2c(cc1Br)C(C)(C)CCC2(C)C.O=C=O>CCCCC.O1CCCC1>CCCCCCc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2e55407ae46c4beabc510d9038b027f8
O=C(O)c1ccc(O)nc1.OCc1ccccc1>>O=C(OCc1ccccc1)c1ccc(O)nc1
OC1=NC=C(C(=O)O)C=C1.S(O)(O)(=O)=O.C(C1=CC=CC=C1)O>>OC1=NC=C(C(=O)OCC2=CC=CC=C2)C=C1
O[C:2](=[O:1])[c:11]1[cH:12][cH:13][c:14]([OH:15])[n:16][cH:17]1.[OH:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1>>[O:1]=[C:2]([O:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][c:14]([OH:15])[n:16][cH:17]1
O=C(O)c1ccc(O)nc1.OCc1ccccc1
O=C(OCc1ccccc1)c1ccc(O)nc1
null
null
null
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
O=C(OCc1ccccc1)c1cccnc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7].[OH;D1;+0:8]-[C:9]-[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[O;H0;D2;+0:8]-[C:9]-[c:10])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]
null
[]
null
null
null
null
30 g of 6-hydroxynicotinic acid were treated with 500 ml of benzyl alcohol and 1 ml of concentrated sulfuric acid. After boiling at reflux for 3 days, the reaction mixture was poured on to ice-water, extracted several times with ethyl acetate, washed with water, dried over sodium sulfate and evaporated, firstly in a wa...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
c1ccccc1.c1ccncc1
HO-
null
null
null
O=C(O)c1ccc(O)nc1.OCc1ccccc1>>O=C(OCc1ccccc1)c1ccc(O)nc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-315e56646a1f498680f098449e45c81e
CCCCC#Cc1ccc2c(c1)C(C)(C)CCCC2>>CCCCCCc1ccc2c(c1)C(C)(C)CCCC2
C(#CCCCC)C=1C=CC2=C(C(CCCC2)(C)C)C1>>C(CCCCC)C=1C=CC2=C(C(CCCC2)(C)C)C1
[CH3:1][CH2:2][CH2:3][CH2:4][C:5]#[C:6][c:7]1[cH:8][cH:9][c:10]2[c:11]([cH:12]1)[C:13]([CH3:14])([CH3:15])[CH2:16][CH2:17][CH2:18][CH2:19]2>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][c:7]1[cH:8][cH:9][c:10]2[c:11]([cH:12]1)[C:13]([CH3:14])([CH3:15])[CH2:16][CH2:17][CH2:18][CH2:19]2
CCCCC#Cc1ccc2c(c1)C(C)(C)CCCC2
CCCCCCc1ccc2c(c1)C(C)(C)CCCC2
null
[Pd]
C(C)(=O)OCC
Reduction
OtherReaction
2bb8d5b532a2781e0a7c069a5cd3e8a7e8d44660c0ec1d9e17c04d8ba2cb383b
1990560e9c55934bde8ca0feaed9c61d80f37f94f0cf240a9929dc374d0a33aa
c1ccc2c(c1)CCCCC2
[C:1]-[C:2]-[C;H0;D2;+0:3]#[C;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]>>[C:1]-[C:2]-[CH2;D2;+0:3]-[CH2;D2;+0:4]-[c:5](:[c:6]):[c:7]
null
[]
null
null
null
null
This alkyne was dissolved in 30 ml of ethy acetate and hydrogenated over 2 g of Pd/C (10%) at room temperature and under 1 atm H2. Filtration over diatomaceous earth and removal of the solvent gave 3.08 g of 2-hexyl-9,9-dimethyl-6,7,8,9-tetrahydro-5H-benzocycloheptene as a colorless oil (GC purity: 98%). Conditions: Se...
10.6084/m9.figshare.5104873.v1
null
Alkyne
null
null
null
c1ccc2c(c1)CCCCC2
null
[Pd].C(C)(=O)OCC
null
null
CCCCC#Cc1ccc2c(c1)C(C)(C)CCCC2>[Pd].C(C)(=O)OCC>CCCCCCc1ccc2c(c1)C(C)(C)CCCC2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-f15578709608425ca7e804635f32e399
BrBr.CCCCCCc1ccc2c(c1)C(C)(C)CCCC2>>CCCCCCc1cc2c(cc1Br)CCCCC2(C)C
C(CCCCC)C=1C=CC2=C(C(CCCC2)(C)C)C1.BrBr>>BrC=1C(=CC2=C(CCCCC2(C)C)C1)CCCCCC
Br[Br:13].[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][c:7]1[cH:8][c:9]2[c:10]([cH:11][cH:12]1)[CH2:14][CH2:15][CH2:16][CH2:17][C:18]2([CH3:19])[CH3:20]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][c:7]1[cH:8][c:9]2[c:10]([cH:11][c:12]1[Br:13])[CH2:14][CH2:15][CH2:16][CH2:17][C:18]2([CH3:19])[CH3:20]
BrBr.CCCCCCc1ccc2c(c1)C(C)(C)CCCC2
CCCCCCc1cc2c(cc1Br)CCCCC2(C)C
null
[Fe]
C(Cl)Cl
Functional Group Interconversion
Bromination
4a6454c45deb843afe911cae2e4e04b415b9aa2380a0e17448996842b1f937f0
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc2c(c1)CCCCC2
Br-[Br;H0;D1;+0:1].[C:2]-[c:3](:[c:4]):[cH;D2;+0:5]:[c:6]:[c:7]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:5](:[c:6]:[c:7]):[c:3](-[C:2]):[c:4]
null
[]
null
null
30
MINUTE
This 3.08 g of 2-hexyl-9,9-dimethyl-6,7,8,9-tetrahydro-5H-benzocycloheptene were dissolved in 35 ml of CH2Cl2, treated at 0° with a spatula tip of Fe powder and then reacted with a solution of 0.67 ml of Br2 (1.1 eq.) in 5 ml of CH2Cl2. After 30 min., the mixture was poured on to ice, extracted with diethyl ether, wash...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)CCCCC2
c1ccc2c(c1)CCCCC2
c1ccc2c(c1)CCCCC2
HBr
[Fe].C(Cl)Cl
null
0.5
BrBr.CCCCCCc1ccc2c(c1)C(C)(C)CCCC2>[Fe].C(Cl)Cl>CCCCCCc1cc2c(cc1Br)CCCCC2(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-bec0b13badfd4aa9b7a9fafcead8a865
CCCCCCc1cc2c(cc1Br)CCCCC2(C)C.O=C=O>>CCCCCCc1cc2c(cc1C(=O)O)CCCCC2(C)C
C(=O)=O.[Li]CCCC.BrC=1C(=CC2=C(CCCCC2(C)C)C1)CCCCCC>>C(CCCCC)C1=CC2=C(CCCCC2(C)C)C=C1C(=O)O
Br[c:12]1[c:7]([CH2:6][CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[cH:8][c:9]2[c:10]([cH:11]1)[CH2:16][CH2:17][CH2:18][CH2:19][C:20]2([CH3:21])[CH3:22].[C:13](=[O:14])=[O:15]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][c:7]1[cH:8][c:9]2[c:10]([cH:11][c:12]1[C:13](=[O:14])[OH:15])[CH2:16][CH2:17][CH2:18][CH2:19][C:20]2([CH3:21]...
CCCCCCc1cc2c(cc1Br)CCCCC2(C)C.O=C=O
CCCCCCc1cc2c(cc1C(=O)O)CCCCC2(C)C
null
null
O1CCCC1
Acylation
OtherReaction
ba320636bb74c150bbda303a1bba98ca25ba6cb1c2e144aaf6ffcd505d4cde2b
d0d963f3850574b1f0fda744314036458b2dd627cb0c4e2f893b9c52a88ad449
c1ccc2c(c1)CCCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C:5]):[c:6].[O;D1;H0:7]=[C;H0;D2;+0:8]=[O;H0;D1;+0:9]>>[C:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[C;H0;D3;+0:8](=[O;D1;H0:7])-[OH;D1;+0:9]):[c:2]:[c:3]
null
[]
null
null
40
MINUTE
This 3.21 g of 2-bromo-3-hexyl-5,5-dimethyl-6,7,8,9-tetrahydro-5H-benzocycloheptene were placed in 30 ml of abs. tetrahydrofuran under Ar and treated at -78° with 6.75 ml of 1.55M nBuLi (hexane) (1.1 eq.). The metal/halogen exchange was followed by gas chromatography (GC). After 40 min., a large excess of CO2 gas was i...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carbon dioxide
Carboxylic acid
c1ccc2c(c1)CCCCC2
c1ccc2c(c1)CCCCC2
c1ccc2c(c1)CCCCC2
Br-
O1CCCC1
null
0.666667
CCCCCCc1cc2c(cc1Br)CCCCC2(C)C.O=C=O>O1CCCC1>CCCCCCc1cc2c(cc1C(=O)O)CCCCC2(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-998b94bdae2a4efb8c11261a196e92e3
C[Si](C)(C)C/C=C/CO.O=C(O)c1ccc(O)nc1>>C[Si](C)(C)C/C=C/COC(=O)c1ccc(O)nc1
C[Si](C/C=C/CO)(C)C.OC1=NC=C(C(=O)O)C=C1.C1(CCCCC1)N=C=NC1CCCCC1>>OC1=NC=C(C(=O)OC\C=C\C[Si](C)(C)C)C=C1
[CH3:1][Si:2]([CH3:3])([CH3:4])[CH2:5]/[CH:6]=[CH:7]/[CH2:8][OH:9].O[C:10](=[O:11])[c:12]1[cH:13][cH:14][c:15]([OH:16])[n:17][cH:18]1>>[CH3:1][Si:2]([CH3:3])([CH3:4])[CH2:5]/[CH:6]=[CH:7]/[CH2:8][O:9][C:10](=[O:11])[c:12]1[cH:13][cH:14][c:15]([OH:16])[n:17][cH:18]1
C[Si](C)(C)C/C=C/CO.O=C(O)c1ccc(O)nc1
C[Si](C)(C)C/C=C/COC(=O)c1ccc(O)nc1
null
CN(C1=CC=NC=C1)C
CN(C=O)C
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
c1ccncc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7].[C:8]/[C:9]=[C:10]/[C:11]-[OH;D1;+0:12]>>[C:8]/[C:9]=[C:10]/[C:11]-[O;H0;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]
38
[{"value": 38.0, "product": "OC1=NC=C(C(=O)OC\\C=C\\C[Si](C)(C)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
1.3 g of 4-trimethylsilyl-(E)-but-2-en-1-ol (synthesis described in J. Org. Chem. 1984, 49, 4092), 1.08 g of 6-hydroxy-nicotinic acid and 178 mg of 4-dimethylaminopyridine were placed in succession in 30 ml of abs. dimethylformamide. 1.77 g (1.1 eq.) of dicyclohexylcarbodiimide were added thereto at 0° and the mixture ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
c1ccncc1
HO-
CN(C1=CC=NC=C1)C.CN(C=O)C
null
null
C[Si](C)(C)C/C=C/CO.O=C(O)c1ccc(O)nc1>CN(C1=CC=NC=C1)C.CN(C=O)C>C[Si](C)(C)C/C=C/COC(=O)c1ccc(O)nc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-93220ca147a845ff95c1f6c722b6fe11
CCCC/C=C\c1cc2c(cc1Br)C(C)(C)CCC2(C)C.O=C=O>>CCCC/C=C\c1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C
[Li]CCCC.BrC=1C=C2C(CCC(C2=CC1\C=C/CCCC)(C)C)(C)C.C(=O)=O>>C(=C/CCCC)/C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C(=O)O
Br[c:12]1[c:7](/[CH:6]=[CH:5]\[CH2:4][CH2:3][CH2:2][CH3:1])[cH:8][c:9]2[c:10]([cH:11]1)[C:16]([CH3:17])([CH3:18])[CH2:19][CH2:20][C:21]2([CH3:22])[CH3:23].[C:13](=[O:14])=[O:15]>>[CH3:1][CH2:2][CH2:3][CH2:4]/[CH:5]=[CH:6]\[c:7]1[cH:8][c:9]2[c:10]([cH:11][c:12]1[C:13](=[O:14])[OH:15])[C:16]([CH3:17])([CH3:18])[CH2:19][C...
CCCC/C=C\c1cc2c(cc1Br)C(C)(C)CCC2(C)C.O=C=O
CCCC/C=C\c1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C
null
null
O1CCCC1
Acylation
OtherReaction
2c77db6aaec596a76b7a465634b3055972748ecc9b259d7fb098a14192761a6e
d0d963f3850574b1f0fda744314036458b2dd627cb0c4e2f893b9c52a88ad449
c1ccc2c(c1)CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](/[C:5]=[C:6]\[C:7]):[c:8].[O;D1;H0:9]=[C;H0;D2;+0:10]=[O;H0;D1;+0:11]>>[C:7]/[C:6]=[C:5]\[c:4](:[c:8]):[c;H0;D3;+0:1](-[C;H0;D3;+0:10](=[O;D1;H0:9])-[OH;D1;+0:11]):[c:2]:[c:3]
null
[]
null
null
null
null
3.72 g of (Z)-6-bromo-7-hex-1-enyl-1,1,4,4-tetramethyl-1,2,3,4-tetrahydro-naphthalene (75% pure) were placed in 25 ml of abs. tetrahydrofuran and treated at -75° with 8.25 ml of 1.55M n-BuLi (hexane) (1.2 eq.). After 1/2h., a CO2 stream was conducted vigorously through the solution for 30 min., with the temperature ris...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carbon dioxide
Carboxylic acid
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
Br-
O1CCCC1
null
null
CCCC/C=C\c1cc2c(cc1Br)C(C)(C)CCC2(C)C.O=C=O>O1CCCC1>CCCC/C=C\c1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-34b88de89a834c5b93af8ffabf69f38c
CCCCCOc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C.O=C(OCc1ccccc1)c1ccc(O)nc1>>CCCCCOc1cc2c(cc1C(=O)Oc1ccc(C(=O)OCc3ccccc3)cn1)C(C)(C)CCC2(C)C
C(CCCC)OC=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C(=O)O.BrC=1C=C2C(CCC(C2=CC1OCCCCC)(C)C)(C)C.C(C)(C)(C)[Li].OC1=NC=C(C(=O)OCC2=CC=CC=C2)C=C1.C(=O)=O>>C(CCCC)OC=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C(=O)OC1=NC=C(C(=O)OCC2=CC=CC=C2)C=C1
O[C:13]([c:12]1[c:7]([O:6][CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[cH:8][c:9]2[c:10]([cH:11]1)[C:32]([CH3:33])([CH3:34])[CH2:35][CH2:36][C:37]2([CH3:38])[CH3:39])=[O:14].[OH:15][c:16]1[cH:17][cH:18][c:19]([C:20](=[O:21])[O:22][CH2:23][c:24]2[cH:25][cH:26][cH:27][cH:28][cH:29]2)[cH:30][n:31]1>>[CH3:1][CH2:2][CH2:3][CH2:4][C...
CCCCCOc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C.O=C(OCc1ccccc1)c1ccc(O)nc1
CCCCCOc1cc2c(cc1C(=O)Oc1ccc(C(=O)OCc3ccccc3)cn1)C(C)(C)CCC2(C)C
null
null
null
Acylation
Mitsunobu esterification
f18451ac648b00cb7c6684a3e64bee855b0320c7eb0f62b757b29d5fb6745560
1489fe0065c6531b60fda87a3857d7da1cd21873868856f058c20706f927fa08
O=C(OCc1ccccc1)c1ccc(OC(=O)c2ccc3c(c2)CCCC3)nc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[O;H0;D2;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
In analogy to Example 1, by metallating 6-bromo-7-pentoxy-1,1,4,4-tetramethyl-1,2,3,4-tetrahydro-naphthalene with tert.butyl-lithium and reacting with carbon dioxide gas there was prepared 3-pentoxy-5,5,8,8-tetramethyl-5,6,7,8-tetrahydro-naphthalene-2-carboxylic acid (m.p. 67°-68° C., from hexane). Reaction of this aci...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Aromatic alcohol
Ester
null
null
c1ccncc1.c1ccccc1.c1ccc2c(c1)CCCC2
HO-
null
null
null
CCCCCOc1cc2c(cc1C(=O)O)C(C)(C)CCC2(C)C.O=C(OCc1ccccc1)c1ccc(O)nc1>>CCCCCOc1cc2c(cc1C(=O)Oc1ccc(C(=O)OCc3ccccc3)cn1)C(C)(C)CCC2(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0833dde5dcd44e279ff441b2ca2671fd
CC(C)(C)[Si](C)(C)Oc1ccc(Br)cc1C12CC3CC(CC(C3)C1)C2.O=C=O>>CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)O)cc1C12CC3CC(CC(C3)C1)C2
C(=O)=O.Cl.C(CCC)[Li].[Cl-].[NH4+].C12(CC3CC(CC(C1)C3)C2)C2=C(O[Si](C)(C)C(C)(C)C)C=CC(=C2)Br>>C12(CC3CC(CC(C1)C3)C2)C=2C=C(C(=O)O)C=CC2O[Si](C)(C)C(C)(C)C
Br[c:12]1[cH:11][cH:10][c:9]([O:8][Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7])[c:17]([C:18]23[CH2:19][CH:20]4[CH2:21][CH:22]([CH2:23][CH:24]([CH2:25]4)[CH2:26]2)[CH2:27]3)[cH:16]1.[C:13](=[O:14])=[O:15]>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][c:9]1[cH:10][cH:11][c:12]([C:13](=[O:14])[OH:...
CC(C)(C)[Si](C)(C)Oc1ccc(Br)cc1C12CC3CC(CC(C3)C1)C2.O=C=O
CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)O)cc1C12CC3CC(CC(C3)C1)C2
null
null
CCCCCC.O1CCCC1
Acylation
OtherReaction
07ac4a201d363784a28677e85b547e572f4793f5010c94050885192cae13600e
d0d963f3850574b1f0fda744314036458b2dd627cb0c4e2f893b9c52a88ad449
c1ccc(C23CC4CC(CC(C4)C2)C3)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[O;D1;H0:6]=[C;H0;D2;+0:7]=[O;H0;D1;+0:8]>>[O;D1;H0:6]=[C;H0;D3;+0:7](-[OH;D1;+0:8])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
-78
CELSIUS
1.5
HOUR
9.3 g of (2-adamantan-1-yl-4-bromo-phenoxy)-tert-butyl-dimethylsilane were dissolved in 120 ml of absolute tetrahydrofuran and treated dropwise at -78° C. with 15.5 ml of a 1.6 molar solution of n-butyl-lithium in hexane. After stirring at -78° C. for 1.5 hours, a vigorous stream of carbon dioxide was introduced for on...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carbon dioxide
Carboxylic acid
c1ccccc1
c1ccccc1
c1ccccc1.C1C2CC3CC1CC(C2)C3
Br-
CCCCCC.O1CCCC1
-78
1.5
CC(C)(C)[Si](C)(C)Oc1ccc(Br)cc1C12CC3CC(CC(C3)C1)C2.O=C=O>CCCCCC.O1CCCC1>CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)O)cc1C12CC3CC(CC(C3)C1)C2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-429d4cda5f5a43799ceb5fbb3c399100
C=CCOC(=O)c1ccc(OC(=O)c2ccc(O[Si](C)(C)C(C)(C)C)c(C34CC5CC(CC(C5)C3)C4)c2)nc1>>CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)Oc2ccc(C(=O)O)cn2)cc1C12CC3CC(CC(C3)C1)C2
C(CCC)[SnH](CCCC)CCCC.C12(CC3CC(CC(C1)C3)C2)C=2C=C(C(=O)OC3=NC=C(C(=O)OCC=C)C=C3)C=CC2O[Si](C)(C)C(C)(C)C.Cl>>C12(CC3CC(CC(C1)C3)C2)C=2C=C(C(=O)OC3=NC=C(C(=O)O)C=C3)C=CC2O[Si](C)(C)C(C)(C)C
C=CC[O:22][C:20]([c:19]1[cH:18][cH:17][c:16]([O:15][C:13]([c:12]2[cH:11][cH:10][c:9]([O:8][Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7])[c:26]([C:27]34[CH2:28][CH:29]5[CH2:30][CH:31]([CH2:32][CH:33]([CH2:34]5)[CH2:35]3)[CH2:36]4)[cH:25]2)=[O:14])[n:24][cH:23]1)=[O:21]>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3...
C=CCOC(=O)c1ccc(OC(=O)c2ccc(O[Si](C)(C)C(C)(C)C)c(C34CC5CC(CC(C5)C3)C4)c2)nc1
CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)Oc2ccc(C(=O)O)cn2)cc1C12CC3CC(CC(C3)C1)C2
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
O1CCCC1
Deprotection
Ester saponification (alkyl deprotection)
ed269ca55aec5bff4b12be2d0b3de5ee7266c084a9f8e361574d4479e760fc9a
9247ae44385773b8f4b33d9727786bed234278529a98c511521a502ffe365790
O=C(Oc1ccccn1)c1cccc(C23CC4CC(CC(C4)C2)C3)c1
C=C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
22.7
[{"value": 22.7, "product": "C12(CC3CC(CC(C1)C3)C2)C=2C=C(C(=O)OC3=NC=C(C(=O)O)C=C3)C=CC2O[Si](C)(C)C(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
100 mg of this ester were dissolved in 5 ml of absolute tetrahydrofuran and treated under argon with 104 mg of tetrakis-(triphenylphosphine)-palladium and 61 mg of tributyltin hydride. After stirring at room temperature for 30 min., the reaction mixture was poured on to ice/saturated ammonium chloride solution, acidifi...
10.6084/m9.figshare.5104873.v1
null
Ester.Allyl
Carboxylic acid
null
null
c1ccccc1.c1ccncc1.C1C2CC3CC1CC(C2)C3
Other
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O1CCCC1
null
0.5
C=CCOC(=O)c1ccc(OC(=O)c2ccc(O[Si](C)(C)C(C)(C)C)c(C34CC5CC(CC(C5)C3)C4)c2)nc1>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O1CCCC1>CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)Oc2ccc(C(=O)O)cn2)cc1C12CC3CC(CC(C3)C1)C2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7d998b7fe2794f36a0da66f08e6c5190
CN=C=O.C[C@H]1[C@@H](O)O[C@@H]2OC3(C)CC[C@H]4[C@H](C)CC[C@@H]1[C@@]24OO3>>CNC(=O)[O-].C[C@H]1[C@@H](O)O[C@@H]2OC3(C)CC[C@H]4[C@H](C)CC[C@@H]1[C@@]24OO3
C[C@@H]1CC[C@H]2[C@H]([C@H](O[C@H]3[C@@]24[C@H]1CCC(O3)(OO4)C)O)C.CN=C=O>>C[C@@H]1CC[C@H]2[C@H]([C@H](O[C@H]3[C@@]24[C@H]1CCC(O3)(OO4)C)O)C.CNC([O-])=O
[CH3:1][N:2]=[C:3]=[O:4].[OH:5][C@@H:8]1[C@H:7]([CH3:6])[C@@H:22]2[CH2:21][CH2:20][C@@H:18]([CH3:19])[C@@H:17]3[CH2:16][CH2:15][C:13]4([CH3:14])[O:12][C@@H:11]([O:10]1)[C@@:23]32[O:24][O:25]4>>[CH3:1][NH:2][C:3](=[O:4])[O-:5].[CH3:6][C@H:7]1[C@@H:8]([OH:9])[O:10][C@@H:11]2[O:12][C:13]3([CH3:14])[CH2:15][CH2:16][C@H:17]...
CN=C=O.C[C@H]1[C@@H](O)O[C@@H]2OC3(C)CC[C@H]4[C@H](C)CC[C@@H]1[C@@]24OO3
CNC(=O)[O-].C[C@H]1[C@@H](O)O[C@@H]2OC3(C)CC[C@H]4[C@H](C)CC[C@@H]1[C@@]24OO3
null
null
C(Cl)Cl
Acylation
OtherReaction
7daf814dac15ef7d283e5348fdd3c8b2fc54980ade315ce55b0bdc7532f8d52b
324b9b0d41dbdbd0410a7ca73b88d13aa195b02e8c8e5363c25d974e101242aa
C1C[C@@H]2CCC3OO[C@@]24[C@@H](C1)CCO[C@@H]4O3
[#8:1]-[C:2]-[#8:3]-[C@H;D3;+0:4](-[OH;D1;+0:5])-[C:6](-[C;D1;H3:7])-[C:8].[C;D1;H3:9]-[N;H0;D2;+0:10]=[C;H0;D2;+0:11]=[O;D1;H0:12]>>[#8:1]-[C:2]-[#8:3]-[C@H;D3;+0:4](-[O;D1;H1:13])-[C:6](-[C;D1;H3:7])-[C:8].[C;D1;H3:9]-[NH;D2;+0:10]-[C;H0;D3;+0:11](-[O-;H0;D1:5])=[O;D1;H0:12]
121.4
[{"value": 121.4, "product": "C[C@@H]1CC[C@H]2[C@H]([C@H](O[C@H]3[C@@]24[C@H]1CCC(O3)(OO4)C)O)C.CNC([O-])=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of dihydroqinghaosu (284 mg, 1 mmol) in dry CH2Cl2 (6 ml) and methyl isocyanate (63 mg, 1.1 mmol) was refluxed for ca. 2 days. The solution was filtered and evaporated in vacuo at 40° C. to give a solid, which was chromatographed on a silica-gel column with petroleumether/AcOEt 8:2. The fraction obtained was...
10.6084/m9.figshare.5104873.v1
null
Ether.Isocyanate.Secondary alcohol
Carbamic acid.Ether.Secondary alcohol
C1C[C@@H]2CCC3OO[C@@]24[C@@H](C1)CCO[C@@H]4O3
C1C[C@@H]2CCC3OO[C@@]24[C@@H](C1)CCO[C@@H]4O3
C1C[C@@H]2CCC3OO[C@@]24[C@@H](C1)CCO[C@@H]4O3
Other
C(Cl)Cl
null
null
CN=C=O.C[C@H]1[C@@H](O)O[C@@H]2OC3(C)CC[C@H]4[C@H](C)CC[C@@H]1[C@@]24OO3>C(Cl)Cl>CNC(=O)[O-].C[C@H]1[C@@H](O)O[C@@H]2OC3(C)CC[C@H]4[C@H](C)CC[C@@H]1[C@@]24OO3
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e14621919a904c08b3c9d56e77154681
O=C=Nc1cccc([N+](=O)[O-])c1>>O=C([O-])Nc1cccc([N+](=O)[O-])c1
C[C@@H]1CC[C@H]2[C@H]([C@H](O[C@H]3[C@@]24[C@H]1CCC(O3)(OO4)C)O)C.[N+](=O)([O-])C=1C=C(C=CC1)N=C=O>>C[C@@H]1CC[C@H]2[C@H]([C@H](O[C@H]3[C@@]24[C@H]1CCC(O3)(OO4)C)O)C.[N+](=O)([O-])C=1C=C(C=CC1)NC(=O)[O-]
[O:21]=[C:22]=[N:24][c:25]1[cH:26][cH:27][cH:28][c:29]([N+:30](=[O:23])[O-:32])[cH:33]1>>[O:21]=[C:22]([O-:23])[NH:24][c:25]1[cH:26][cH:27][cH:28][c:29]([N+:30](=[O:31])[O-:32])[cH:33]1
O=C=Nc1cccc([N+](=O)[O-])c1
O=C([O-])Nc1cccc([N+](=O)[O-])c1
null
null
null
Functional Group Addition
OtherReaction
420c7c4fe30cfc3fffb8332defbfeb637efb89651ae26c0575d9d088ab57e86b
6d26e3011880c7a427aadbc9aa67cdb6ed04eaa3210d938c9f2b8a36bf6fd25a
c1ccccc1
[O;-;D1;H0:1]-[N+;H0;D3:2](=[O;H0;D1;+0:3])-[c:4](:[c:5]):[c:6]:[c:7](-[N;H0;D2;+0:8]=[C;H0;D2;+0:9]=[O;D1;H0:10]):[c:11]>>[O-;H0;D1:3]-[C;H0;D3;+0:9](=[O;D1;H0:10])-[NH;D2;+0:8]-[c:7](:[c:11]):[c:6]:[c:4](-[N+;H0;D3:2](-[O;-;D1;H0:1])=[O;D1;H0:12]):[c:5]
null
[]
null
null
null
null
The title compound was similarly prepared from dihydroqinghaosu and m-nitrophenyl isocyanate as Example 3. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Nitro group.Isocyanate
Carbamic acid.Nitro group
null
null
c1ccccc1
Other
null
null
null
O=C=Nc1cccc([N+](=O)[O-])c1>>O=C([O-])Nc1cccc([N+](=O)[O-])c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b0029680d3ec4bf2ada8460d535c1585
CN(C)Cc1ccc(C2CCC(=O)CC2)cc1>>CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1
CN(C)CC1=CC=C(C=C1)C1CCC(CC1)=O.[BH4-].[Na+]>>CN(C)CC1=CC=C(C=C1)[C@@H]1CC[C@H](CC1)O
[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([CH:9]2[CH2:10][CH2:11][C:12](=[O:13])[CH2:14][CH2:15]2)[cH:16][cH:17]1>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([OH:13])[CH2:14][CH2:15]2)[cH:16][cH:17]1
CN(C)Cc1ccc(C2CCC(=O)CC2)cc1
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1
null
null
CO
Reduction
Reduction of ketone to secondary alcohol
2851cada23ce4ae5bca04d1ef48c1473fe285273d9a82803d040df273fff8e79
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1ccc(C2CCCCC2)cc1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[C:5]-[C:6]>>[C:1]-[C:2]-[C@H;D3;+0:3](-[OH;D1;+0:4])-[C:5]-[C:6]
null
[]
null
null
null
null
To a solution of 11.1 g (0.048 mol) of 4-(4-dimethylaminomethylphenyl)-cyclohexanone in 100 ml of absolute methanol, which has been cooled to -10° C., is added 1.82 g (0.048 mol) of sodium borohydride in batches with stirring. The reaction mixture is allowed to react for 1.5 hours at ambient temperature and then evapor...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
C1CCCCC1
C1CCCCC1
c1ccccc1.C1CCCCC1
null
CO
null
null
CN(C)Cc1ccc(C2CCC(=O)CC2)cc1>CO>CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-106a0c8f6a4340dd99e577e214caf696
CN(C)Cc1ccc(C2CCC(=O)CC2)cc1>>CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1
C(C)O.OO.CN(C)CC1=CC=C(C=C1)C1CCC(CC1)=O.C(C)(CC)[BH-](C(C)CC)C(C)CC.[Li+]>>CN(C)CC1=CC=C(C=C1)[C@H]1CC[C@H](CC1)O
[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([CH:9]2[CH2:10][CH2:11][C:12](=[O:13])[CH2:14][CH2:15]2)[cH:16][cH:17]1>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@@H:12]([OH:13])[CH2:14][CH2:15]2)[cH:16][cH:17]1
CN(C)Cc1ccc(C2CCC(=O)CC2)cc1
CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1
null
null
O1CCCC1
Reduction
Reduction of ketone to secondary alcohol
2851cada23ce4ae5bca04d1ef48c1473fe285273d9a82803d040df273fff8e79
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1ccc(C2CCCCC2)cc1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[C:5]-[C:6]>>[C:1]-[C:2]-[C@@H;D3;+0:3](-[OH;D1;+0:4])-[C:5]-[C:6]
null
[]
null
null
10
MINUTE
50 ml (0.05 mol) of a 1 molar solution of lithium tri-sec.-butyl-borohydride in absolute tetrahydrofuran are diluted with 100 ml of absolute tetrahydrofuran under a nitrogen atmosphere and then, at -65° C. to -70° C., with stirring and within 10 minutes, a solution of 5.8 g (0.025 mol) of 4-(4-dimethylaminomethylphenyl...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
C1CCCCC1
C1CCCCC1
c1ccccc1.C1CCCCC1
null
O1CCCC1
null
0.166667
CN(C)Cc1ccc(C2CCC(=O)CC2)cc1>O1CCCC1>CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-59ad5f10a39944bab640d9fbd6671548
O=C1CCC(c2ccccc2)CC1>>OC1CCC(c2ccccc2)CC1
C1(=CC=CC=C1)C1CCC(CC1)=O.[BH4-].[Na+]>>C1(=CC=CC=C1)C1CCC(CC1)O
[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[CH2:12][CH2:13]1>>[OH:1][CH:2]1[CH2:3][CH2:4][CH:5]([c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[CH2:12][CH2:13]1
O=C1CCC(c2ccccc2)CC1
OC1CCC(c2ccccc2)CC1
null
null
CO
Reduction
Reduction of ketone to secondary alcohol
2851cada23ce4ae5bca04d1ef48c1473fe285273d9a82803d040df273fff8e79
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1ccc(C2CCCCC2)cc1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[C:5]-[C:6]>>[C:1]-[C:2]-[CH;D3;+0:3](-[OH;D1;+0:4])-[C:5]-[C:6]
66.2
[{"value": 66.0, "product": "C1(=CC=CC=C1)C1CCC(CC1)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.2, "product": "C1(=CC=CC=C1)C1CCC(CC1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 31.4 g (0.18 mol) of 4-phenylcyclohexanone in 500 ml of absolute methanol, which is cooled to -10° C., are added 6.8 g (0.18 mol) of sodium borohydride in batches with stirring. The reaction mixture is allowed to react for 0.5 hours at -10° C. and for 3 hours at ambient temperature and then evaporated ...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
C1CCCCC1
C1CCCCC1
C1CCCCC1.c1ccccc1
null
CO
null
null
O=C1CCC(c2ccccc2)CC1>CO>OC1CCC(c2ccccc2)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9d8b4bad4cfc4f6f9993dde1eca90539
CC(=O)OC(C)=O.OC1CCC(c2ccccc2)CC1>>CC(=O)OC1CCC(c2ccccc2)CC1
C1(=CC=CC=C1)C1CCC(CC1)O.CC(=O)OC(=O)C>>C(C)(=O)OC1CCC(CC1)C1=CC=CC=C1
CC(=O)O[C:2]([CH3:1])=[O:3].[OH:4][CH:5]1[CH2:6][CH2:7][CH:8]([c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[CH2:15][CH2:16]1>>[CH3:1][C:2](=[O:3])[O:4][CH:5]1[CH2:6][CH2:7][CH:8]([c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[CH2:15][CH2:16]1
CC(=O)OC(C)=O.OC1CCC(c2ccccc2)CC1
CC(=O)OC1CCC(c2ccccc2)CC1
null
CN(C1=CC=NC=C1)C
C(C)N(CC)CC
Acylation
Transesterification
a7ad17dd333d7246e42d4632a0a7042db0b0d3b7f2adb7cdb2c46498a22ac4db
c98fee24664998fb42388f3a4804f79d763c5043c4f5565ea3b46913e3a86a6e
c1ccc(C2CCCCC2)cc1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](-[OH;D1;+0:6])-[C:7]>>[C:4]-[C:5](-[O;H0;D2;+0:6]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[C:7]
92
[{"value": 92.0, "product": "C(C)(=O)OC1CCC(CC1)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.6, "product": "C(C)(=O)OC1CCC(CC1)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a mixture of 20.3 g (0.115 mol) of 4-phenylcyclohexanol, 14.2 ml (0.15 mol) of acetanhydride and 29 ml of triethylamine are added, with stirring and at ambient temperature, 2.3 g (0.02 mol) of 4-dimethylaminopyridine, a clear solution being produced in an exothermic reaction. This is heated to 80° C. for 3 hours and...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Secondary alcohol
Ester
null
null
C1CCCCC1.c1ccccc1
HO-
CN(C1=CC=NC=C1)C.C(C)N(CC)CC
null
null
CC(=O)OC(C)=O.OC1CCC(c2ccccc2)CC1>CN(C1=CC=NC=C1)C.C(C)N(CC)CC>CC(=O)OC1CCC(c2ccccc2)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-989f1c45e316471198b7f2d873102bdb
C=O.CC(=O)OC1CCC(c2ccccc2)CC1.Cl>>CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1
C(Cl)Cl.C(C)(=O)OC1CCC(CC1)C1=CC=CC=C1.C=O.Cl>>C(C)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CCl
O=[CH2:13].[CH3:1][C:2](=[O:3])[O:4][CH:5]1[CH2:6][CH2:7][CH:8]([c:9]2[cH:10][cH:11][cH:12][cH:15][cH:16]2)[CH2:17][CH2:18]1.[ClH:14]>>[CH3:1][C:2](=[O:3])[O:4][C@H:5]1[CH2:6][CH2:7][C@H:8]([c:9]2[cH:10][cH:11][c:12]([CH2:13][Cl:14])[cH:15][cH:16]2)[CH2:17][CH2:18]1
C=O.CC(=O)OC1CCC(c2ccccc2)CC1.Cl
CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1
null
[Cl-].[Zn+2].[Cl-]
null
C-C Coupling
OtherReaction
8fe6a9acd6712eceb303cec1f37294821c7a3812792483df6fdf1f25e3f9d768
9040382df3c5c738c70f57f2da5c03057ad8ce8a09c32bd12c78827f9fd1b464
c1ccc(C2CCCCC2)cc1
O=[CH2;D1;+0:1].[ClH;D0;+0:2].[c:3]:[c:4]:[cH;D2;+0:5]:[c:6]:[c:7]>>[Cl;H0;D1;+0:2]-[CH2;D2;+0:1]-[c;H0;D3;+0:5](:[c:4]:[c:3]):[c:6]:[c:7]
null
[]
null
null
2.5
HOUR
A solution of 24.3 g (0.11 mol) of O-acetyl-4-phenylcyclohexanol in 1300 ml of methylene chloride is combined with 26.0 g (0.86 mol) of paraformaldehyde and 26.0 g (0.19 mol) of zinc chloride. Hydrogen chloride is introduced into this suspension, with stirring, for 2.5 hours, whilst the temperature rises to about 30° C...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde
Primary halide
c1ccccc1
c1ccccc1
C1CCCCC1.c1ccccc1
HO-
[Cl-].[Zn+2].[Cl-]
null
2.5
C=O.CC(=O)OC1CCC(c2ccccc2)CC1.Cl>[Cl-].[Zn+2].[Cl-]>CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-fe8da988a6f64ed0968009c91353edde
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)c1ccc(Cl)cc1>>CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)c3ccc(Cl)cc3)CC2)cc1
[OH-].[Na+].CN(C)CC1=CC=C(C=C1)[C@@H]1CC[C@H](CC1)O.C(C)N(CC)CC.ClC1=CC=C(C(=O)Cl)C=C1>>ClC1=CC=C(C(=O)O[C@@H]2CC[C@H](CC2)C2=CC=C(C=C2)CN(C)C)C=C1
[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([OH:13])[CH2:23][CH2:24]2)[cH:25][cH:26]1.Cl[C:14](=[O:15])[c:16]1[cH:17][cH:18][c:19]([Cl:20])[cH:21][cH:22]1>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([O:13][C:14](=[O:15])[c:16]3[cH:17][cH...
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)c1ccc(Cl)cc1
CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)c3ccc(Cl)cc3)CC2)cc1
null
null
C(Cl)Cl.O
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
O=C(O[C@H]1CC[C@H](c2ccccc2)CC1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7](-[OH;D1;+0:8])-[C:9]>>[C:6]-[C:7](-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:9]
null
[]
null
null
null
null
A solution of 1.0 g (0.0043 mol) of trans-4-(4-dimethylaminomethylphenyl)-cyclohexanol and 0.6 ml of triethylamine in 50 ml of methylene chloride is combined, dropwise, with 0.75 g (0.0043 mol) of 4-chlorobenzoylchloride, with stirring, and refluxed for 3 hours. After cooling, 50 ml of water are added, the mixture is a...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
c1ccccc1.C1CCCCC1.c1ccccc1
HCl
C(Cl)Cl.O
null
null
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)c1ccc(Cl)cc1>C(Cl)Cl.O>CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)c3ccc(Cl)cc3)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-98aa976f41dc49e1bd5ec855777b801d
CC(=O)Cl.CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1>>CC(=O)O[C@@H]1CC[C@@H](c2ccc(CN(C)C)cc2)CC1
CN(C)CC1=CC=C(C=C1)[C@@H]1CC[C@H](CC1)O.C(C)(=O)Cl.C(C)N(CC)CC>>C(C)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C
Cl[C:2]([CH3:1])=[O:3].[OH:4][C@H:5]1[CH2:6][CH2:7][C@H:8]([c:9]2[cH:10][cH:11][c:12]([CH2:13][N:14]([CH3:15])[CH3:16])[cH:17][cH:18]2)[CH2:19][CH2:20]1>>[CH3:1][C:2](=[O:3])[O:4][C@H:5]1[CH2:6][CH2:7][C@H:8]([c:9]2[cH:10][cH:11][c:12]([CH2:13][N:14]([CH3:15])[CH3:16])[cH:17][cH:18]2)[CH2:19][CH2:20]1
CC(=O)Cl.CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1
CC(=O)O[C@@H]1CC[C@@H](c2ccc(CN(C)C)cc2)CC1
null
null
null
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
c1ccc(C2CCCCC2)cc1
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](-[OH;D1;+0:6])-[C:7]>>[C:4]-[C:5](-[O;H0;D2;+0:6]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[C:7]
null
[]
null
null
null
null
from trans-4-(4-dimethylaminomethylphenyl)-cyclohexanol and acetylchloride/triethylamine. Colourless syrup. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
C1CCCCC1.c1ccccc1
HCl
null
null
null
CC(=O)Cl.CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1>>CC(=O)O[C@@H]1CC[C@@H](c2ccc(CN(C)C)cc2)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e78195adcc9b4f1e92d9c95ef4fa295b
CCCC(=O)Cl.CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1>>CCCC(=O)O[C@@H]1CC[C@@H](c2ccc(CN(C)C)cc2)CC1
CN(C)CC1=CC=C(C=C1)[C@@H]1CC[C@H](CC1)O.C(CCC)(=O)Cl.C(C)N(CC)CC>>C(CCC)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C
Cl[C:4]([CH2:3][CH2:2][CH3:1])=[O:5].[OH:6][C@H:7]1[CH2:8][CH2:9][C@H:10]([c:11]2[cH:12][cH:13][c:14]([CH2:15][N:16]([CH3:17])[CH3:18])[cH:19][cH:20]2)[CH2:21][CH2:22]1>>[CH3:1][CH2:2][CH2:3][C:4](=[O:5])[O:6][C@H:7]1[CH2:8][CH2:9][C@H:10]([c:11]2[cH:12][cH:13][c:14]([CH2:15][N:16]([CH3:17])[CH3:18])[cH:19][cH:20]2)[CH...
CCCC(=O)Cl.CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1
CCCC(=O)O[C@@H]1CC[C@@H](c2ccc(CN(C)C)cc2)CC1
null
null
null
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
c1ccc(C2CCCCC2)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[C:5]-[C:6](-[OH;D1;+0:7])-[C:8]>>[C:5]-[C:6](-[O;H0;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4])-[C:8]
null
[]
null
null
null
null
from trans-4-(4-dimethylaminomethylphenyl)-cyclohexanol and butyric acid chloride/triethylamine. Colourless oil. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
C1CCCCC1.c1ccccc1
HCl
null
null
null
CCCC(=O)Cl.CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1>>CCCC(=O)O[C@@H]1CC[C@@H](c2ccc(CN(C)C)cc2)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7f6c0cb8ddf545bda5b486eb8435608e
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)C1CC1>>CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)C3CC3)CC2)cc1
CN(C)CC1=CC=C(C=C1)[C@@H]1CC[C@H](CC1)O.C1(CC1)C(=O)Cl.C(C)N(CC)CC>>C1(CC1)C(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C
[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([OH:13])[CH2:19][CH2:20]2)[cH:21][cH:22]1.Cl[C:14](=[O:15])[CH:16]1[CH2:17][CH2:18]1>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([O:13][C:14](=[O:15])[CH:16]3[CH2:17][CH2:18]3)[CH2:19][CH2:20]2...
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)C1CC1
CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)C3CC3)CC2)cc1
null
null
null
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
O=C(O[C@H]1CC[C@H](c2ccccc2)CC1)C1CC1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[C:5]-1.[C:6]-[C:7](-[OH;D1;+0:8])-[C:9]>>[C:6]-[C:7](-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[C:5]-1)-[C:9]
null
[]
null
null
null
null
from trans-4-(4-dimethylaminomethylphenyl)-cyclohexanol and cyclopropane carboxylic acid chloride/triethylamine. Colourless wax. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
c1ccccc1.C1CCCCC1.C1CC1
HCl
null
null
null
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)C1CC1>>CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)C3CC3)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-65d0d248651b4777b9672b8046a54da0
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)C1CCCCC1>>CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)C3CCCCC3)CC2)cc1
CN(C)CC1=CC=C(C=C1)[C@@H]1CC[C@H](CC1)O.C1(CCCCC1)C(=O)Cl.C(C)N(CC)CC>>C1(CCCCC1)C(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C
[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([OH:13])[CH2:22][CH2:23]2)[cH:24][cH:25]1.Cl[C:14](=[O:15])[CH:16]1[CH2:17][CH2:18][CH2:19][CH2:20][CH2:21]1>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([O:13][C:14](=[O:15])[CH:16]3[CH2:17][CH...
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)C1CCCCC1
CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)C3CCCCC3)CC2)cc1
null
null
null
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
O=C(O[C@H]1CC[C@H](c2ccccc2)CC1)C1CCCCC1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5].[C:6]-[C:7](-[OH;D1;+0:8])-[C:9]>>[C:6]-[C:7](-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5])-[C:9]
null
[]
null
null
null
null
from trans-4-(4-dimethylaminomethylphenyl)-cyclohexanol and cyclohexane carboxylic acid chloride/triethylamine. White crystals. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
c1ccccc1.C1CCCCC1.C1CCCCC1
HCl
null
null
null
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)C1CCCCC1>>CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)C3CCCCC3)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-fb382a38ecde4b3498d73cf8d48e3315
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)CC=Cc1ccccc1>>CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)CC=Cc3ccccc3)CC2)cc1
CN(C)CC1=CC=C(C=C1)[C@@H]1CC[C@H](CC1)O.C1(=CC=CC=C1)C=CCC(=O)Cl.C(C)N(CC)CC>>C1(=CC=CC=C1)C=CCC(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C
[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([OH:13])[CH2:25][CH2:26]2)[cH:27][cH:28]1.Cl[C:14](=[O:15])[CH2:16][CH:17]=[CH:18][c:19]1[cH:20][cH:21][cH:22][cH:23][cH:24]1>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@H:12]([O:13][C:14](=[O:15])[C...
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)CC=Cc1ccccc1
CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)CC=Cc3ccccc3)CC2)cc1
null
null
null
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
O=C(CC=Cc1ccccc1)O[C@H]1CC[C@H](c2ccccc2)CC1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]=[C:5]-[c:6].[C:7]-[C:8](-[OH;D1;+0:9])-[C:10]>>[C:7]-[C:8](-[O;H0;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]=[C:5]-[c:6])-[C:10]
null
[]
null
null
null
null
from trans-4-(4-dimethylaminomethylphenyl)-cyclohexanol and 4-phenyl-3-butenoic acid chloride/triethylamine. White crystals. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
c1ccccc1.C1CCCCC1.c1ccccc1
HCl
null
null
null
CN(C)Cc1ccc([C@@H]2CC[C@@H](O)CC2)cc1.O=C(Cl)CC=Cc1ccccc1>>CN(C)Cc1ccc([C@@H]2CC[C@@H](OC(=O)CC=Cc3ccccc3)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-558c9a0ee99e4a3bb4ba4d9621782c8f
CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1.O=C(Cl)CC=Cc1ccccc1>>CN(C)Cc1ccc([C@@H]2CC[C@H](OC(=O)CC=Cc3ccccc3)CC2)cc1
CN(C)CC1=CC=C(C=C1)[C@H]1CC[C@H](CC1)O.C1(=CC=CC=C1)C=CCC(=O)Cl.C(C)N(CC)CC>>C1(=CC=CC=C1)C=CCC(=O)O[C@@H]1CC[C@@H](CC1)C1=CC=C(C=C1)CN(C)C
[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@@H:12]([OH:13])[CH2:25][CH2:26]2)[cH:27][cH:28]1.Cl[C:14](=[O:15])[CH2:16][CH:17]=[CH:18][c:19]1[cH:20][cH:21][cH:22][cH:23][cH:24]1>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@@H:12]([O:13][C:14](=[O:15])...
CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1.O=C(Cl)CC=Cc1ccccc1
CN(C)Cc1ccc([C@@H]2CC[C@H](OC(=O)CC=Cc3ccccc3)CC2)cc1
null
null
null
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
O=C(CC=Cc1ccccc1)O[C@H]1CC[C@@H](c2ccccc2)CC1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]=[C:5]-[c:6].[C:7]-[C:8](-[OH;D1;+0:9])-[C:10]>>[C:7]-[C:8](-[O;H0;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]=[C:5]-[c:6])-[C:10]
null
[]
null
null
null
null
from cis-4-(4-dimethylaminomethylphenyl)-cyclohexanol and 4-phenyl-3-butenoic acid chloride/triethylamine. White crystals. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
c1ccccc1.C1CCCCC1.c1ccccc1
HCl
null
null
null
CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1.O=C(Cl)CC=Cc1ccccc1>>CN(C)Cc1ccc([C@@H]2CC[C@H](OC(=O)CC=Cc3ccccc3)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-46545033cfa54ccfbfeb9970eade577f
CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1.O=C(Cl)c1ccc(Cl)cc1>>CN(C)Cc1ccc([C@@H]2CC[C@H](OC(=O)c3ccc(Cl)cc3)CC2)cc1
ClC1=CC=C(C(=O)Cl)C=C1.CN(C)CC1=CC=C(C=C1)[C@H]1CC[C@H](CC1)O.C(C)N(CC)CC.CN(C)C1=NC=CC=C1.[OH-].[Na+]>>ClC1=CC=C(C(=O)O[C@@H]2CC[C@@H](CC2)C2=CC=C(C=C2)CN(C)C)C=C1
[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@@H:12]([OH:13])[CH2:23][CH2:24]2)[cH:25][cH:26]1.Cl[C:14](=[O:15])[c:16]1[cH:17][cH:18][c:19]([Cl:20])[cH:21][cH:22]1>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]([C@H:9]2[CH2:10][CH2:11][C@@H:12]([O:13][C:14](=[O:15])[c:16]3[cH:17][...
CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1.O=C(Cl)c1ccc(Cl)cc1
CN(C)Cc1ccc([C@@H]2CC[C@H](OC(=O)c3ccc(Cl)cc3)CC2)cc1
null
null
C(Cl)Cl.O
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
O=C(O[C@H]1CC[C@@H](c2ccccc2)CC1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7](-[OH;D1;+0:8])-[C:9]>>[C:6]-[C:7](-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:9]
null
[]
null
null
12
HOUR
0.24 g (0.001 mol) of cis-4-(4-dimethylaminomethylphenyl)-cyclohexanol, 0,34 ml (0.0025 mol) of triethylamine and 0.12 g (0.001 mol) of dimethylaminopyridine are dissolved in 20 ml of methylene chloride, mixed with 0.175 g (0.001 mol) of 4-chlorobenzoylchloride and stirred for 12 hours at ambient temperature. The react...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
c1ccccc1.C1CCCCC1.c1ccccc1
HCl
C(Cl)Cl.O
null
12
CN(C)Cc1ccc([C@@H]2CC[C@H](O)CC2)cc1.O=C(Cl)c1ccc(Cl)cc1>C(Cl)Cl.O>CN(C)Cc1ccc([C@@H]2CC[C@H](OC(=O)c3ccc(Cl)cc3)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d5a8195f23794884af3a23a8c8f6148d
CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1.CCNCC>>CCN(CC)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
O.C(C)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CCl.C([O-])([O-])=O.[K+].[K+].C(C)NCC>>C(C)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(CC)CC
Cl[CH2:6][c:7]1[cH:8][cH:9][c:10]([C@H:11]2[CH2:12][CH2:13][C@H:14]([O:15][C:16]([CH3:17])=[O:18])[CH2:19][CH2:20]2)[cH:21][cH:22]1.[CH3:1][CH2:2][NH:3][CH2:4][CH3:5]>>[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[CH2:6][c:7]1[cH:8][cH:9][c:10]([C@H:11]2[CH2:12][CH2:13][C@H:14]([O:15][C:16]([CH3:17])=[O:18])[CH2:19][CH2:20]2)[cH...
CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1.CCNCC
CCN(CC)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
6d58cac08ccced0a33ed16fbca180bc12aa011288d6476106d98a7b2cbc3d709
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc(C2CCCCC2)cc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C;D1;H3:9]>>[C;D1;H3:5]-[C:6]-[N;H0;D3;+0:7](-[C:8]-[C;D1;H3:9])-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
50
CELSIUS
null
null
A solution of 1 g (3.75 mmol) of trans-O-acetyl-4-(4-chloromethylphenyl)-cyclohexanol in 10 ml of dimethylformamide is mixed with 0.52 g (3.75 mmol) of potassium carbonate and 0.27 g (3.75 mmol) of diethylamine. This mixture is heated to 50° C. for 6 hours with stirring, then water is added and the mixture is extracted...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
null
null
c1ccccc1.C1CCCCC1
HCl
CN(C=O)C
50
null
CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1.CCNCC>CN(C=O)C>CCN(CC)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-f2d5dfa3dcc34983a499f39832ce5301
CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1.CCCNCCC>>CCCN(CCC)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
C(C)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CCl.C(CC)NCCC>>C(C)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(CCC)CCC
Cl[CH2:8][c:9]1[cH:10][cH:11][c:12]([C@H:13]2[CH2:14][CH2:15][C@H:16]([O:17][C:18]([CH3:19])=[O:20])[CH2:21][CH2:22]2)[cH:23][cH:24]1.[CH3:1][CH2:2][CH2:3][NH:4][CH2:5][CH2:6][CH3:7]>>[CH3:1][CH2:2][CH2:3][N:4]([CH2:5][CH2:6][CH3:7])[CH2:8][c:9]1[cH:10][cH:11][c:12]([C@H:13]2[CH2:14][CH2:15][C@H:16]([O:17][C:18]([CH3:1...
CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1.CCCNCCC
CCCN(CCC)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
6d58cac08ccced0a33ed16fbca180bc12aa011288d6476106d98a7b2cbc3d709
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc(C2CCCCC2)cc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]>>[C:5]-[C:6]-[N;H0;D3;+0:7](-[C:8]-[C:9])-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
from trans-O-acetyl-4-(4-chloromethylphenyl)-cyclohexanol and dipropylamine. Colourless oil. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
null
null
c1ccccc1.C1CCCCC1
HCl
null
null
null
CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1.CCCNCCC>>CCCN(CCC)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2c57a2e6edd64e5e962d5636e0b02f36
C=CCNCC=C.CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1>>C=CCN(CC=C)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
C(C)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CCl.C(C=C)NCC=C>>C(C)(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(CC=C)CC=C
[CH2:1]=[CH:2][CH2:3][NH:4][CH2:5][CH:6]=[CH2:7].Cl[CH2:8][c:9]1[cH:10][cH:11][c:12]([C@H:13]2[CH2:14][CH2:15][C@H:16]([O:17][C:18]([CH3:19])=[O:20])[CH2:21][CH2:22]2)[cH:23][cH:24]1>>[CH2:1]=[CH:2][CH2:3][N:4]([CH2:5][CH:6]=[CH2:7])[CH2:8][c:9]1[cH:10][cH:11][c:12]([C@H:13]2[CH2:14][CH2:15][C@H:16]([O:17][C:18]([CH3:1...
C=CCNCC=C.CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1
C=CCN(CC=C)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
6d58cac08ccced0a33ed16fbca180bc12aa011288d6476106d98a7b2cbc3d709
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc(C2CCCCC2)cc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H2:5]=[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]=[C;D1;H2:11]>>[C;D1;H2:5]=[C:6]-[C:7]-[N;H0;D3;+0:8](-[C:9]-[C:10]=[C;D1;H2:11])-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
from trans-O-acetyl-4-(4-chloromethylphenyl)-cyclohexanol and diallylamine. Colourless oil. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
null
null
c1ccccc1.C1CCCCC1
HCl
null
null
null
C=CCNCC=C.CC(=O)O[C@@H]1CC[C@@H](c2ccc(CCl)cc2)CC1>>C=CCN(CC=C)Cc1ccc([C@@H]2CC[C@@H](OC(C)=O)CC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-cf6dff211f2249548afbc224153b66a4
Cl>>Cl
ClC1=CC=C(C=C1)CC(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C.Cl>>Cl.ClC1=CC=C(C=C1)CC(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C
[ClH:28]>>[ClH:28]
Cl
Cl
null
null
C(C)(C)O.C(C)OCC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
null
[]
null
null
1
HOUR
A solution of 0.39 g (0.001 mol) of trans-O-(4-chlorophenylacetyl)-4-(4-dimethylaminomethylphenyl)-cyclohexanol in 10 ml of diethyl ether is combined at ambient temperature, with stirring, with a 1.5 times equimolar amount of hydrogen chloride in isopropanol added dropwise. The precipitate formed is left for 1 hour at ...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O.C(C)OCC
null
1
Cl>C(C)(C)O.C(C)OCC>Cl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-55aacc7a80b0419cab9d2c65fa6adadb
O=C(O)C(O)C(O)C(=O)O>>O=C([O-])C(O)C(O)C(=O)[O-]
C(C(O)C(O)C(=O)O)(=O)O.ClC1=CC=C(C=C1)CC(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C.C(C)OCC>>ClC1=CC=C(C=C1)CC(=O)O[C@@H]1CC[C@H](CC1)C1=CC=C(C=C1)CN(C)C.C(=O)([O-])C(O)C(O)C(=O)[O-]
[O:28]=[C:29]([OH:30])[CH:31]([OH:32])[CH:33]([OH:34])[C:35](=[O:36])[OH:37]>>[O:28]=[C:29]([O-:30])[CH:31]([OH:32])[CH:33]([OH:34])[C:35](=[O:36])[O-:37]
O=C(O)C(O)C(O)C(=O)O
O=C([O-])C(O)C(O)C(=O)[O-]
null
null
C(C)O
Oxidation
OtherReaction
4af04878ecd22d61c6d7d46db52e672904d5e72408231940a5cea872324a16a2
4e878a1fdc9370141a3ed00507bdfaa037f36d163bb15c5076375a9835c80b8f
null
[O;D1;H0:1]=[C:2](-[OH;D1;+0:3])-[C:4]-[C:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]>>[O-;H0;D1:3]-[C:2](=[O;D1;H0:1])-[C:4]-[C:5]-[C:6](-[O-;H0;D1:8])=[O;D1;H0:7]
null
[]
null
null
8
HOUR
First 0.15 g (0.001 mol) of anhydrous tartaric acid and then 0.39 g (0.001 mol) of trans-O-(4-chlorophenylacetyl)-4-(4-dimethylaminomethylphenyl)-cyclohexanol are dissolved in 7 ml of absolute ethanol. Diethyl ether is then added to the clear solution until it becomes slightly cloudy and it is then left to stand for 8 ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid
null
null
null
null
null
C(C)O
null
8
O=C(O)C(O)C(O)C(=O)O>C(C)O>O=C([O-])C(O)C(O)C(=O)[O-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b8ac393b893c42cfb6d34015ef8c6939
N#Cc1ccc(CBr)cc1.O=C1NCCN1>>N#Cc1ccc(CN2CCN(Cc3ccc(C#N)cc3)C2=O)cc1
O.BrCC1=CC=C(C#N)C=C1.[H-].[Na+].N1C(NCC1)=O>>O=C1N(CCN1CC1=CC=C(C#N)C=C1)CC1=CC=C(C#N)C=C1
Br[CH2:7][c:6]1[cH:5][cH:4][c:3]([C:2]#[N:1])[cH:24][cH:23]1.[NH:8]1[CH2:9][CH2:15][NH:11][C:21]1=[O:22]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][N:8]2[CH2:9][CH2:10][N:11]([CH2:12][c:13]3[cH:14][cH:15][c:16]([C:17]#[N:18])[cH:19][cH:20]3)[C:21]2=[O:22])[cH:23][cH:24]1
N#Cc1ccc(CBr)cc1.O=C1NCCN1
N#Cc1ccc(CN2CCN(Cc3ccc(C#N)cc3)C2=O)cc1
null
null
CN(C=O)C
Aromatic Heterocycle Formation
OtherReaction
39571f641692bae0ab2e4fb7e56baf0a046bbe68e5d15065d8f936b61702d85c
04064b000c1f037cb6379c4a9b891971302bcd094d2302ea56061b3b37327222
O=C1N(Cc2ccccc2)CCN1Cc1ccccc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H0:5]=[C:6]1-[NH;D2;+0:7]-[CH2;D2;+0:8]-[CH2;D2;+0:9]-[NH;D2;+0:10]-1>>[C:11]-[c:12](:[c:13]):[cH;D2;+0:8]:[c:14]:[c:15]-[C:16]-[N;H0;D3;+0:7]1-[C:17]-[CH2;D2;+0:9]-[N;H0;D3;+0:10](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[C:6]-1=[O;D1;H0:5]
null
[]
null
null
1
HOUR
To sodium hydride (2.4 g, 60 mmol) in dimethylformamide (50 mL) at 0° C. was added imidazolin-2-one (2.6 g, 30 mmol). After stirring for 20 minutes 4-(bromomethyl)benzonitrile (13 g, 66 mmol) was added and the mixture was warmed to ambient temperature. After stirring for 1 hour the reaction was poured into water and a ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Urea
Urea.Nitrile
C1CNCN1
C1C[NH]C[NH]1.c1ccccc1
c1ccccc1.C1C[NH]C[NH]1.c1ccccc1
Br-
CN(C=O)C
null
1
N#Cc1ccc(CBr)cc1.O=C1NCCN1>CN(C=O)C>N#Cc1ccc(CN2CCN(Cc3ccc(C#N)cc3)C2=O)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d53ccc1fdb224edc9a97f3bf1af38c7c
CN(C)c1ccc(C(O)C(=O)c2ccccc2)cc1.NC(N)=O>>CN(C)c1ccc(-c2[nH]c(=O)[nH]c2-c2ccccc2)cc1
NC(=O)N.CN(C1=CC=C(C=C1)C(C(=O)C1=CC=CC=C1)O)C>>CN(C1=CC=C(C=C1)C=1NC(NC1C1=CC=CC=C1)=O)C
O=[C:13]([CH:8](O)[c:7]1[cH:6][cH:5][c:4]([N:2]([CH3:1])[CH3:3])[cH:21][cH:20]1)[c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1.[NH2:9][C:10](=[O:11])[NH2:12]>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[nH:9][c:10](=[O:11])[nH:12][c:13]2-[c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[cH:20][cH:21]1
CN(C)c1ccc(C(O)C(=O)c2ccccc2)cc1.NC(N)=O
CN(C)c1ccc(-c2[nH]c(=O)[nH]c2-c2ccccc2)cc1
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
7a04490902783a9d1d6099ad78b95538301d0ef7b8b6cc364284d393dbdf37cd
19da97726e6dc44d537eff971a50046c3e80ca62fdecca0b64533a3c10927d47
O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)[nH]1
O-[CH;D3;+0:1](-[C;H0;D3;+0:2](=O)-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6]:[c:7])-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12].[NH2;D1;+0:13]-[C;H0;D3;+0:14](-[NH2;D1;+0:15])=[O;D1;H0:16]>>[O;D1;H0:16]=[c;H0;D3;+0:14]1:[nH;D2;+0:13]:[c;H0;D3;+0:2](-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6]:[c:7]):[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:...
null
[]
120
CELSIUS
2
HOUR
To acetic acid (2 mL) was added urea (0.6 g, 10 mmol) and 2-(4-dimethylaminophenyl)-2-hydroxy-1-phenylethanone (2.6 g, 10 mmol). After stirring for 2 hours at 120° C., the reaction was cooled to ambient temperature. The resulting solid was filtered, washed with ether, and dried in vacuo to give 4-(4-dimethylaminophenyl...
10.6084/m9.figshare.5104873.v1
null
Ketone.Urea.Secondary alcohol
null
null
c1c[nH]cn1
c1ccccc1.c1c[nH]cn1.c1ccccc1
HO-
C(C)(=O)O
120
2
CN(C)c1ccc(C(O)C(=O)c2ccccc2)cc1.NC(N)=O>C(C)(=O)O>CN(C)c1ccc(-c2[nH]c(=O)[nH]c2-c2ccccc2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b724f3ac05e046b9b06047e61353e43e
N#Cc1cccc(CBr)c1.O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)[nH]1>>N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1
C1(=CC=CC=C1)C=1NC(NC1C1=CC=CC=C1)=O.BrCC=1C=C(C#N)C=CC1.[H-].[Na+]>>C1(=CC=CC=C1)C=1NC(N(C1C1=CC=CC=C1)CC=1C=C(C#N)C=CC1)=O
Br[CH2:8][c:7]1[cH:6][cH:5][cH:4][c:3]([C:2]#[N:1])[cH:27]1.[nH:9]1[c:10](-[c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[nH:24][c:25]1=[O:26]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([CH2:8][n:9]2[c:10](-[c:11]3[cH:12][cH:13][cH:14][cH:15][cH:16]3)[c:17](-[c:18]3[cH:1...
N#Cc1cccc(CBr)c1.O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)[nH]1
N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
b9d84e1ee028da6e8c5d8924d45fbf8f3755d9adc2caf0035bd5ed7f30f5ee03
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)n1Cc1ccccc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H0:5]=[c:6]1:[#7;a:7]:[c:8](-[c:9]):[c:10](-[c:11]):[nH;D2;+0:12]:1>>[O;D1;H0:5]=[c:6]1:[#7;a:7]:[c:8](-[c:9]):[c:10](-[c:11]):[n;H0;D3;+0:12]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
In a manner similar to Preparation 1 above, 2,3-dihydro-4,5-diphenyl-1H-imidazol-2-one (1.2 g, 5 mmol) was reacted with 3-(bromomethyl)benzonitrile (0.39 g, mmol) and sodium hydride (0.18 g, 5 mmol) in dimethylformamide (20 mL) to give 3-[(2,3-dihydro-4,5-diphenyl-2-oxo-1H-imidazol-1-yl)methyl]benzonitrile after chroma...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1c[nH]cn1
c1c[nH]cn1
c1ccccc1.c1ccccc1.c1ccccc1.c1c[nH]cn1
HBr
CN(C=O)C
null
null
N#Cc1cccc(CBr)c1.O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)[nH]1>CN(C=O)C>N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-5dd855de65c9493aa839d921f58ac95c
COC(=O)c1cccc(CBr)c1.O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)[nH]1>>COC(=O)c1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1
Cl.C1(=CC=CC=C1)C=1NC(NC1C1=CC=CC=C1)=O.[H-].[Na+].BrCC=1C=C(C(=O)OC)C=CC1>>COC(=O)C=1C=C(C=CC1)CN1C(NC(=C1C1=CC=CC=C1)C1=CC=CC=C1)=O
Br[CH2:10][c:9]1[cH:8][cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:29]1.[nH:11]1[c:12](-[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[c:19](-[c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[nH:26][c:27]1=[O:28]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([CH2:10][n:11]2[c:12](-[c:13]3[cH:14][cH:15][cH:16][cH:...
COC(=O)c1cccc(CBr)c1.O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)[nH]1
COC(=O)c1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
b9d84e1ee028da6e8c5d8924d45fbf8f3755d9adc2caf0035bd5ed7f30f5ee03
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)n1Cc1ccccc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H0:5]=[c:6]1:[#7;a:7]:[c:8](-[c:9]):[c:10](-[c:11]):[nH;D2;+0:12]:1>>[O;D1;H0:5]=[c:6]1:[#7;a:7]:[c:8](-[c:9]):[c:10](-[c:11]):[n;H0;D3;+0:12]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
25
[{"value": 25.0, "product": "COC(=O)C=1C=C(C=CC1)CN1C(NC(=C1C1=CC=CC=C1)C1=CC=CC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
30
MINUTE
To 2,3-dihydro-4,5-diphenyl-1H-imidazol-2-one (4.76 g, 20 mmol) in 50 mL DMF was added to a suspension of NaH (0.8 g, 20 mmol) in 25 mL DMF. The suspension was stirred at ambient temperatures for 30 minutes, then heated to 50° C. for 30 minutes. A solution of methyl 3-bromomethylbenzoate (2.86 g, 12.5 mmol) in 20 mL DM...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1c[nH]cn1
c1c[nH]cn1
c1ccccc1.c1ccccc1.c1ccccc1.c1c[nH]cn1
HBr
CN(C)C=O
50
0.5
COC(=O)c1cccc(CBr)c1.O=c1[nH]c(-c2ccccc2)c(-c2ccccc2)[nH]1>CN(C)C=O>COC(=O)c1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-786127000a804395a2a606287fdb5b82
N#Cc1ccc2ccc(CBr)cc2c1.N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1>>N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)n(Cc3ccc4ccc(C#N)cc4c3)c2=O)c1
C1(=CC=CC=C1)C=1NC(N(C1C1=CC=CC=C1)CC=1C=C(C#N)C=CC1)=O.BrCC1=CC=C2C=CC(=CC2=C1)C#N>>C(#N)C=1C=C(C=CC1)CN1C(N(C(=C1C1=CC=CC=C1)C1=CC=CC=C1)CC1=CC=C2C=CC(=CC2=C1)C#N)=O
Br[CH2:25][c:26]1[cH:27][cH:28][c:29]2[cH:30][cH:31][c:32]([C:33]#[N:34])[cH:35][c:36]2[cH:37]1.[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([CH2:8][n:9]2[c:10](-[c:11]3[cH:12][cH:13][cH:14][cH:15][cH:16]3)[c:17](-[c:18]3[cH:19][cH:20][cH:21][cH:22][cH:23]3)[nH:24][c:38]2=[O:39])[cH:40]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6...
N#Cc1ccc2ccc(CBr)cc2c1.N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1
N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)n(Cc3ccc4ccc(C#N)cc4c3)c2=O)c1
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
b9d84e1ee028da6e8c5d8924d45fbf8f3755d9adc2caf0035bd5ed7f30f5ee03
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
O=c1n(Cc2ccccc2)c(-c2ccccc2)c(-c2ccccc2)n1Cc1ccc2ccccc2c1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[#7;a:6]1:[c:7](-[c:8]):[c:9](-[c:10]):[nH;D2;+0:11]:[c:12]:1=[O;D1;H0:13]>>[C:5]-[#7;a:6]1:[c:7](-[c:8]):[c:9](-[c:10]):[n;H0;D3;+0:11](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]):[c:12]:1=[O;D1;H0:13]
null
[]
null
null
null
null
In a manner similar to Preparation 2 above, 3-[(2,3-dihydro-4,5-diphenyl-2-oxo-1H-imidazol-1-yl)methyl]benzonitrile was reacted with 7-(bromomethyl)naphthalene-2-carbonitrile to give 7-[[3-(3-cyanophenyl)methyl-2,3-dihydro-4,5-diphenyl-2-oxo-1H-imidazol-1-yl]methyl]naphthalene-2-carbonitrile; NMR (CDCl3) 8.05 (s, 1), 7...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1c[nH]cn1
c1c[nH]cn1
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2ccccc2c1.c1c[nH]cn1
HBr
null
null
null
N#Cc1ccc2ccc(CBr)cc2c1.N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)[nH]c2=O)c1>>N#Cc1cccc(Cn2c(-c3ccccc3)c(-c3ccccc3)n(Cc3ccc4ccc(C#N)cc4c3)c2=O)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-308160af0fe341559cc3cb76dcacfde8
C=CC(=O)OC.CCCN(CCC)C1CCc2cc(Br)ccc2C1>>CCCN(CCC)C1CCc2cc(/C=C/C(=O)OC)ccc2C1
BrC=1C=C2CCC(CC2=CC1)N(CCC)CCC.C(C=C)(=O)OC.C1(=C(C=CC=C1)P(C1=C(C=CC=C1)C)C1=C(C=CC=C1)C)C.C(C)N(CC)CC>>COC(\C=C\C=1C=C2CCC(CC2=CC1)N(CCC)CCC)=O
[CH2:14]=[CH:15][C:16](=[O:17])[O:18][CH3:19].Br[c:13]1[cH:12][c:11]2[c:22]([cH:21][cH:20]1)[CH2:23][CH:8]([N:4]([CH2:3][CH2:2][CH3:1])[CH2:5][CH2:6][CH3:7])[CH2:9][CH2:10]2>>[CH3:1][CH2:2][CH2:3][N:4]([CH2:5][CH2:6][CH3:7])[CH:8]1[CH2:9][CH2:10][c:11]2[cH:12][c:13](/[CH:14]=[CH:15]/[C:16](=[O:17])[O:18][CH3:19])[cH:20...
C=CC(=O)OC.CCCN(CCC)C1CCc2cc(Br)ccc2C1
CCCN(CCC)C1CCc2cc(/C=C/C(=O)OC)ccc2C1
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
CN(C=O)C.O
C-C Coupling
Heck terminal vinyl
7d54f98603f982a766802e8a50fd3c154a20a496d1d88bfc154a88f37c1a4dfc
4b186811a4930853b446d93d9faa39b267bddb9ce0b8021bda5c5a3b2bc69f0b
c1ccc2c(c1)CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C;D1;H3:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C:10]=[CH2;D1;+0:11]>>[C;D1;H3:6]-[#8:7]-[C:8](=[O;D1;H0:9])/[C:10]=[CH;D2;+0:11]/[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
28.5
[{"value": 28.5, "product": "COC(\\C=C\\C=1C=C2CCC(CC2=CC1)N(CCC)CCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
3.1 g (0.01 mol) of 6-bromo-2-(N,N-dipropylamino)-1,2,3,4-tetrahydronaphthalene are dissolved in 50 ml of dimethylformamide. There are added in succession to that solution 0.94 g (0.011 mol) of methyl acrylate, 22.4 mg (0.1 mmol) of palladium acetate, 121 mg (0.4 mmol) of tri-ortho-tolylphosphine and 1.6 ml (0.011 mol)...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl
null
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
HBr
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CN(C=O)C.O
null
null
C=CC(=O)OC.CCCN(CCC)C1CCc2cc(Br)ccc2C1>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CN(C=O)C.O>CCCN(CCC)C1CCc2cc(/C=C/C(=O)OC)ccc2C1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b4fd402e735143d2ba1df2c8a9a0fe8f
BrCc1ccccc1.COC(=O)c1ccc(O)cc1O>>COC(=O)c1ccc(OCc2ccccc2)cc1O
OC1=C(C(=O)OC)C=CC(=C1)O.C(=O)([O-])[O-].[K+].[K+].C(C1=CC=CC=C1)Br>>C(C1=CC=CC=C1)OC1=CC(=C(C(=O)OC)C=C1)O
Br[CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1.[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([OH:9])[cH:17][c:18]1[OH:19]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([O:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[cH:17][c:18]1[OH:19]
BrCc1ccccc1.COC(=O)c1ccc(O)cc1O
COC(=O)c1ccc(OCc2ccccc2)cc1O
null
null
CC(=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccc(COc2ccccc2)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[c:3]:[c:2](-[CH2;D2;+0:1]-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8]):[c:4]
null
[]
null
null
null
null
To a stirred, 0° C. solution of methyl 2,4-dihydroxybenzoate (50 g, 300 mmol) in acetone (1000 mL) was added K2CO3 (150 g, 1000 mmol) and benzyl bromide (330 mmol, 39 mL). The solution was allowed to warm to ambient temperature over 48 h. The reaction solution was filtered through celite and the acetone solution stripp...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.c1ccccc1
HBr
CC(=O)C
null
null
BrCc1ccccc1.COC(=O)c1ccc(O)cc1O>CC(=O)C>COC(=O)c1ccc(OCc2ccccc2)cc1O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c4670bc17b3d4dddbc6d0f72787fbc62
CI.COC(=O)c1ccc(OCc2ccccc2)cc1O>>COC(=O)c1ccc(OCc2ccccc2)cc1OC
C(C1=CC=CC=C1)OC1=CC(=C(C(=O)OC)C=C1)O.[H-].[Na+].CI>>C(C1=CC=CC=C1)OC1=CC(=C(C(=O)OC)C=C1)OC
I[CH3:20].[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([O:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[cH:17][c:18]1[OH:19]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([O:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[cH:17][c:18]1[O:19][CH3:20]
CI.COC(=O)c1ccc(OCc2ccccc2)cc1O
COC(=O)c1ccc(OCc2ccccc2)cc1OC
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
b8b041187bac58376aae824630608e7deb49a01db3d652291f8b379c10d4e434
0f0966e3597a58033417ecee71659f4d0c082f95d46b1e52c95541e6e4a59086
c1ccc(COc2ccccc2)cc1
I-[CH3;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]:[c:6](-[OH;D1;+0:7]):[c:8]>>[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]:[c:6](-[O;H0;D2;+0:7]-[CH3;D1;+0:1]):[c:8]
null
[]
null
null
null
null
To a stirred, 0° C. solution of methyl 4-benzyloxy-2-hydroxybenzoate (12 g, 46 mmol) in DMF (150 mL) was added NaH (2.76 g, 69 mmol) and methyl iodide (7.2 mL, 116 mmol). The solution was allowed to warm to ambient temperature overnight with stirring. The reaction mixture was poured onto ice and the resulting aqueous s...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol
Ether
null
null
c1ccccc1.c1ccccc1
HI
CN(C)C=O
null
null
CI.COC(=O)c1ccc(OCc2ccccc2)cc1O>CN(C)C=O>COC(=O)c1ccc(OCc2ccccc2)cc1OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c1656a56b0b84177904d3a04b5264874
COC(=O)c1ccc(O)cc1OC>>COc1cc(O)ccc1C(=O)O
Cl.OC1=CC(=C(C(=O)OC)C=C1)OC.O.O[Li].O>>OC1=CC(=C(C(=O)O)C=C1)OC
C[O:12][C:10]([c:9]1[c:3]([O:2][CH3:1])[cH:4][c:5]([OH:6])[cH:7][cH:8]1)=[O:11]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([OH:6])[cH:7][cH:8][c:9]1[C:10](=[O:11])[OH:12]
COC(=O)c1ccc(O)cc1OC
COc1cc(O)ccc1C(=O)O
null
null
C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccccc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
null
null
24
HOUR
To a stirred solution of methyl 4-hydroxy-2-methoxybenzoate (11 g, 60 mmol) in THF:H2O (100 mL:10 mL) was added LiOH.H2O (3 g, 71 mmol). The solution was stirred over 24 h and then made slightly acidic (pH 5) with 10% HCl (approx 15 mL). The reaction solution was extracted with CH2Cl2 (3×50 mL). The organic phase was d...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1
Other
C1CCOC1
null
24
COC(=O)c1ccc(O)cc1OC>C1CCOC1>COc1cc(O)ccc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-48df0370b6c1448ea65c1fd6355a24c2
COC(=O)c1ccc(O)cc1OC>>COC(=O)c1cc(F)c(O)cc1OC
OC1=CC(=C(C(=O)OC)C=C1)OC.[O-]S(=O)(=O)C(F)(F)F.ClC=1C=[N+](C=C(C1)Cl)F>>FC=1C(=CC(=C(C(=O)OC)C1)OC)O
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:9]([OH:10])[cH:11][c:12]1[O:13][CH3:14]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([F:8])[c:9]([OH:10])[cH:11][c:12]1[O:13][CH3:14]
COC(=O)c1ccc(O)cc1OC
COC(=O)c1cc(F)c(O)cc1OC
null
null
C(Cl)Cl
Functional Group Addition
Aromatic fluorination
2e63a9b91d60f82a8e59b7c72ed55b9aec048f26be2f5eb9ca65b1b73867743c
0a2f22058f27970cef4a98a778644dbe9c44e91f66c74cd24db321993177608a
c1ccccc1
[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[cH;D2;+0:6]:[c:7](-[O;D1;H1:8]):[c:9]>>[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[c;H0;D3;+0:6](-[F;D1;H0:10]):[c:7](-[O;D1;H1:8]):[c:9]
null
[]
null
null
null
null
To a stirred solution of the methyl 4-hydroxy-2-methoxybenzoate (1 g, 5 mmol, from Step 3) in CH2Cl2 (20 mL) was added 3,5-dichloro-1-fluoropyridinium triflate (2.25 g, 6 mmol). The solution was refluxed for 48 h and then cooled to ambient temperature and stripped down under reduced pressure. The crude oil was purified...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1
Other
C(Cl)Cl
null
null
COC(=O)c1ccc(O)cc1OC>C(Cl)Cl>COC(=O)c1cc(F)c(O)cc1OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2e02459c44114d51802676f652203008
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.OC1CCOCC1>>COC(=O)c1ccc(OC(=O)C2CCOCC2)cc1OC
O1CCC(CC1)O.N(=NC(=O)OCC)C(=O)OCC.OC1=CC(=C(C(=O)OC)C=C1)OC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>O1CCC(CC1)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC
CCOC(=O)N=N[C:10](OCC)=[O:11].[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([OH:9])[cH:18][c:19]1[O:20][CH3:21].O[CH:12]1[CH2:13][CH2:14][O:15][CH2:16][CH2:17]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([O:9][C:10](=[O:11])[CH:12]2[CH2:13][CH2:14][O:15][CH2:16][CH2:17]2)[cH:18][c:19]1[O:20][CH3:21]
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.OC1CCOCC1
COC(=O)c1ccc(OC(=O)C2CCOCC2)cc1OC
null
null
C1CCOC1
Acylation
OtherReaction
c4890e071978b0b6e02f922f3692bc2e5bc322d64b2e3a6224c530fe8f3a9533
99cbc1de664ce75fe7841777e00c71bc93fd4ae2bce0b73a15911d06040840b5
O=C(Oc1ccccc1)C1CCOCC1
C-C-O-C(=O)-N=N-[C;H0;D3;+0:1](=[O;D1;H0:2])-O-C-C.O-[CH;D3;+0:3]1-[C:4]-[C:5]-[#8:6]-[C:7]-[C:8]-1.[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[O;H0;D2;+0:9]-[c:10](:[c:11]):[c:12])-[CH;D3;+0:3]1-[C:4]-[C:5]-[#8:6]-[C:7]-[C:8]-1
null
[]
0
CELSIUS
null
null
To a stirred solution of methyl 4-hydroxy-2-methoxybenzoate (713 mg, 3.92 mmol) in dry THF (7.5 mL) was added triphenylphosphine (1.42 g, 5.4 mmol) and the solution was cooled to 0° C. A 2.5 mL volume of tetrahydro-4H-pyran-4-ol (466 mL, 4.90 mmol) and diethyl azodicarboxylate (850 μL, 5.4 mmol) in THF was added dropwi...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Diazene.Secondary alcohol.Aromatic alcohol
Ester
C1CCOCC1
C1CCOCC1
c1ccccc1.C1CCOCC1
HO-
C1CCOC1
0
null
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.OC1CCOCC1>C1CCOC1>COC(=O)c1ccc(OC(=O)C2CCOCC2)cc1OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-effcf6e5366a4bfca9b4bac40907f32c
COC(=O)c1ccc(OC(=O)C2CCOCC2)cc1OC>>COc1cc(OC(=O)C2CCOCC2)ccc1C(=O)O
O1CCC(CC1)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC.O.O[Li].O>>O1CCC(CC1)C(=O)OC1=CC(=C(C(=O)O)C=C1)OC
C[O:20][C:18]([c:17]1[c:3]([O:2][CH3:1])[cH:4][c:5]([O:6][C:7](=[O:8])[CH:9]2[CH2:10][CH2:11][O:12][CH2:13][CH2:14]2)[cH:15][cH:16]1)=[O:19]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][C:7](=[O:8])[CH:9]2[CH2:10][CH2:11][O:12][CH2:13][CH2:14]2)[cH:15][cH:16][c:17]1[C:18](=[O:19])[OH:20]
COC(=O)c1ccc(OC(=O)C2CCOCC2)cc1OC
COc1cc(OC(=O)C2CCOCC2)ccc1C(=O)O
null
null
C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(Oc1ccccc1)C1CCOCC1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
45
CELSIUS
null
null
To a stirred solution of methyl 4-(4-tetrahydropyranoyloxy)-2-methoxy-benzoate (369 mg, 1.38 mmol) in THF:H2O (2.5 mL: 0.5 mL) was added LiOH.H2O (116.4 mg, 2.77 mmol). The reaction was heated to 45° C. over 12 h and then cooled to ambient temperature. The solvent was removed under reduced pressure. The crude solid was...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.C1CCOCC1
Other
C1CCOC1
45
null
COC(=O)c1ccc(OC(=O)C2CCOCC2)cc1OC>C1CCOC1>COc1cc(OC(=O)C2CCOCC2)ccc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7d1e263a61084d54a5924ad814549c11
COC(=O)c1ccc(OC(=O)C2CCc3ccccc32)cc1OC>>COc1cc(OC(=O)C2CCc3ccccc32)ccc1C(=O)O
C1(CCC2=CC=CC=C12)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC.O.O[Li].O>>C1(CCC2=CC=CC=C12)C(=O)OC1=CC(=C(C(=O)O)C=C1)OC
C[O:23][C:21]([c:20]1[c:3]([O:2][CH3:1])[cH:4][c:5]([O:6][C:7](=[O:8])[CH:9]2[CH2:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]32)[cH:18][cH:19]1)=[O:22]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][C:7](=[O:8])[CH:9]2[CH2:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]32)[cH:18][cH:19][c:20]1[C:21](=[O:22])[OH:23]
COC(=O)c1ccc(OC(=O)C2CCc3ccccc32)cc1OC
COc1cc(OC(=O)C2CCc3ccccc32)ccc1C(=O)O
null
null
C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(Oc1ccccc1)C1CCc2ccccc21
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
45
CELSIUS
null
null
To a stirred solution of methyl 4-(1-indanoyloxy)-2-methoxy-benzoate (125 mg, 0.43 mmol) in THF:H2O (1 mL: 0.2 mL) was added LiOH.H2O (35.2 mg, 0.84 mmol). The reaction was heated to 45° C. over 12 h and then cooled to ambient temperature. The solvent was removed under reduced pressure. The crude solid was passed throu...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccc2c(c1)CCC2
Other
C1CCOC1
45
null
COC(=O)c1ccc(OC(=O)C2CCc3ccccc32)cc1OC>C1CCOC1>COc1cc(OC(=O)C2CCc3ccccc32)ccc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e05a7f6ef00b40218847ea8339f5616a
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.O[C@@H]1CCCC[C@H]1c1ccccc1>>COC(=O)c1ccc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)cc1OC
C1(=CC=CC=C1)[C@H]1[C@@H](CCCC1)O.N(=NC(=O)OCC)C(=O)OCC.OC1=CC(=C(C(=O)OC)C=C1)OC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>C1(=CC=CC=C1)[C@@H]1[C@@H](CCCC1)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC
CCOC(=O)N=N[C:10](OCC)=[O:11].[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([OH:9])[cH:24][c:25]1[O:26][CH3:27].O[C@@H:12]1[CH2:13][CH2:14][CH2:15][CH2:16][C@H:17]1[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([O:9][C:10](=[O:11])[C@@H:12]2[CH2:13][CH2:14][CH2:15][CH2:...
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.O[C@@H]1CCCC[C@H]1c1ccccc1
COC(=O)c1ccc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)cc1OC
null
null
C1CCOC1
Acylation
OtherReaction
8e7f7aec30b10cb52f82d427bef98ab15d43a92fc5e2b024cb3b9ec94ed6a028
99cbc1de664ce75fe7841777e00c71bc93fd4ae2bce0b73a15911d06040840b5
O=C(Oc1ccccc1)[C@@H]1CCCC[C@@H]1c1ccccc1
C-C-O-C(=O)-N=N-[C;H0;D3;+0:1](=[O;D1;H0:2])-O-C-C.O-[C@H;D3;+0:3](-[C:4]-[C:5])-[C:6](-[c:7])-[C:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[C:5]-[C:4]-[C@@H;D3;+0:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:9]-[c:10](:[c:11]):[c:12])-[C:6](-[c:7])-[C:8]
null
[]
0
CELSIUS
null
null
To a stirred solution of methyl 4-hydroxy-2-methoxybenzoate (310 mg, 1.7 mmol) in dry THF (1.25 mL) was added triphenylphosphine (446 mg, 1.7 mmol) and the solution was cooled to 0° C. A 500 mL volume of trans-2-phenyl-1-cyclohexanol (200 mg, 1.35 mmol) and diethyl azodicarboxylate (319 μL, 2.02 mmol) in THF was added ...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Diazene.Secondary alcohol.Aromatic alcohol
Ester
C1CCCCC1
C1CCCCC1
c1ccccc1.C1CCCCC1.c1ccccc1
HO-
C1CCOC1
0
null
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.O[C@@H]1CCCC[C@H]1c1ccccc1>C1CCOC1>COC(=O)c1ccc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)cc1OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9cf6d25d3c4e47a1a40710053bd23b71
COC(=O)c1ccc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)cc1OC>>COc1cc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)ccc1C(=O)O
C1(=CC=CC=C1)[C@@H]1[C@@H](CCCC1)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC.O.O[Li].O>>C1(=CC=CC=C1)[C@@H]1[C@@H](CCCC1)C(=O)OC1=CC(=C(C(=O)O)C=C1)OC
C[O:26][C:24]([c:23]1[c:3]([O:2][CH3:1])[cH:4][c:5]([O:6][C:7](=[O:8])[C@@H:9]2[CH2:10][CH2:11][CH2:12][CH2:13][C@@H:14]2[c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[cH:21][cH:22]1)=[O:25]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][C:7](=[O:8])[C@@H:9]2[CH2:10][CH2:11][CH2:12][CH2:13][C@@H:14]2[c:15]2[cH:16][cH:17][cH:18][cH...
COC(=O)c1ccc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)cc1OC
COc1cc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)ccc1C(=O)O
null
null
C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(Oc1ccccc1)[C@@H]1CCCC[C@@H]1c1ccccc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
45
CELSIUS
null
null
To a stirred solution of methyl 4-(cis-2-phenyl- 1-cyclohexanoyloxy)-2-methoxybenzoate (230 mg, 0.64 mmol) in THF:H2O (5 mL:1 mL) was added LiOH.H2O (113.5 mg, 2.7 mmol). The reaction was heated to 45° C. over 12 h and then cooled to ambient temperature. The solvent was removed under reduced pressure. The crude solid w...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.C1CCCCC1.c1ccccc1
Other
C1CCOC1
45
null
COC(=O)c1ccc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)cc1OC>C1CCOC1>COc1cc(OC(=O)[C@@H]2CCCC[C@@H]2c2ccccc2)ccc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0a806a2b38c847b7b222d09354336829
CCOC(=O)c1cccnc1C>>Cc1ncccc1CO
Cl.CC1=C(C(=O)OCC)C=CC=N1.[H-].C(C(C)C)[Al+]CC(C)C.[OH-].[Na+]>>OCC=1C(=NC=CC1)C
CCO[C:8]([c:7]1[c:2]([CH3:1])[n:3][cH:4][cH:5][cH:6]1)=[O:9]>>[CH3:1][c:2]1[n:3][cH:4][cH:5][cH:6][c:7]1[CH2:8][OH:9]
CCOC(=O)c1cccnc1C
Cc1ncccc1CO
null
null
C1(=CC=CC=C1)C.C1CCOC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccncc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]>>[C;D1;H3:6]-[c:5](:[#7;a:7]:[c:8]):[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:4]
null
[]
0
CELSIUS
6
HOUR
To a stirred solution of ethyl 2-methylnicotinate (1.50 g, 9.09 mmol) in freshly distilled THF (100 mL) at 0° C. was added diisobutylaluminum hydride (11.2 mL of a 1.5M solution in toluene, 16.9 mmol). The solution was stirred for 6 h at 0° C. and then warmed to ambient temperature. After 1 h, the solution was cooled i...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccncc1
HO-
C1(=CC=CC=C1)C.C1CCOC1
0
6
CCOC(=O)c1cccnc1C>C1(=CC=CC=C1)C.C1CCOC1>Cc1ncccc1CO
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b03b7005ae0f4e16a4358a35620a3d77
Cc1ncccc1CO.O=S(Cl)Cl>>Cc1ncccc1CCl
OCC=1C(=NC=CC1)C.O=S(Cl)Cl>>ClCC=1C(=NC=CC1)C
O[CH2:8][c:7]1[c:2]([CH3:1])[n:3][cH:4][cH:5][cH:6]1.O=S(Cl)[Cl:9]>>[CH3:1][c:2]1[n:3][cH:4][cH:5][cH:6][c:7]1[CH2:8][Cl:9]
Cc1ncccc1CO.O=S(Cl)Cl
Cc1ncccc1CCl
null
null
C(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
bb752b9027dc4488ba075e5955118a819f80cabd751a7497b67c2eeb1db6b071
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
c1ccncc1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]>>[C;D1;H3:6]-[c:5](:[#7;a:7]:[c:8]):[c:3](-[CH2;D2;+0:2]-[Cl;H0;D1;+0:1]):[c:4]
null
[]
null
null
4
HOUR
To a stirred solution of 3-hydroxymethyl-2-methylpyridine from Step 1 above (1.00 g, 8.13 mmol) in 40 mL of CH2Cl2 at ambient temperature was added SOCl2 (9.0 mL, 123 mmol). The reaction mixture was stirred for 4 hours, and the solvent and excess SOCl2 were evaporated under reduced pressure. The residue was partitioned...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
null
null
c1ccncc1
HCl
C(Cl)Cl
null
4
Cc1ncccc1CO.O=S(Cl)Cl>C(Cl)Cl>Cc1ncccc1CCl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b8dbba8e74ff4118bc3513f530757669
Cc1ncccc1CCl.O=C(OO)c1cccc(Cl)c1>>Cc1c(CCl)ccc[n+]1[O-]
ClCC=1C(=NC=CC1)C.ClC=1C=C(C(=O)OO)C=CC1>>ClCC=1C(=[N+](C=CC1)[O-])C
[CH3:1][c:2]1[c:3]([CH2:4][Cl:5])[cH:6][cH:7][cH:8][n:9]1.O=C(O[OH:10])c1cccc(Cl)c1>>[CH3:1][c:2]1[c:3]([CH2:4][Cl:5])[cH:6][cH:7][cH:8][n+:9]1[O-:10]
Cc1ncccc1CCl.O=C(OO)c1cccc(Cl)c1
Cc1c(CCl)ccc[n+]1[O-]
null
null
C(Cl)(Cl)Cl
Miscellaneous
OtherReaction
5b2b5a1eb88c9671c4a604b6f76054cc01cd86a1985fc147f7e56f19c4844d35
98b338a9d01476c0929fd5672e7509121bfe69600fd72e4d1cc6f1782e2d05d9
c1cc[nH+]cc1
Cl-c1:c:c:c:c(-C(=O)-O-[OH;D1;+0:1]):c:1.[C;D1;H3:2]-[c:3](:[c:4]):[n;H0;D2;+0:5]:[c:6]:[c:7]>>[C;D1;H3:2]-[c:3](:[c:4]):[n+;H0;D3:5](-[O-;H0;D1:1]):[c:6]:[c:7]
null
[]
null
null
1.5
HOUR
To a stirred solution of 3-chloromethyl-2-methylpyridine from Step 2 above (0.50 g; 3.5 mmol) in CHCl3 (40 mL) was added m-chloroperoxybenzoic acid (1.1 g of 55:45 mCPBA:mCBA; 3.5 mmol). After 1.5 h, TLC analysis indicated complete conversion to a lower Rf product. The solution was extracted with equal volumes of satur...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide
null
c1ccncc1.c1ccccc1
C1=CC=[NH+]C=C1
C1=CC=[NH+]C=C1
HCl
C(Cl)(Cl)Cl
null
1.5
Cc1ncccc1CCl.O=C(OO)c1cccc(Cl)c1>C(Cl)(Cl)Cl>Cc1c(CCl)ccc[n+]1[O-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c76a22e184294ef893b6fc5df9e611d7
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.OC1CCOc2ccccc21>>COC(=O)c1ccc(OC(=O)C2CCOc3ccccc32)cc1OC
O1CCC(C2=CC=CC=C12)O.N(=NC(=O)OCC)C(=O)OCC.OC1=CC(=C(C(=O)OC)C=C1)OC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>O1CCC(C2=CC=CC=C12)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC
CCOC(=O)N=N[C:10](OCC)=[O:11].[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([OH:9])[cH:22][c:23]1[O:24][CH3:25].O[CH:12]1[CH2:13][CH2:14][O:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]21>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([O:9][C:10](=[O:11])[CH:12]2[CH2:13][CH2:14][O:15][c:16]3[cH:17][cH:18][cH:19][c...
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.OC1CCOc2ccccc21
COC(=O)c1ccc(OC(=O)C2CCOc3ccccc32)cc1OC
null
null
C1CCOC1
Acylation
OtherReaction
f5703f0bb6d4de4f021493fee785ea9b023c9960545798c80ef6df53e039ff97
99cbc1de664ce75fe7841777e00c71bc93fd4ae2bce0b73a15911d06040840b5
O=C(Oc1ccccc1)C1CCOc2ccccc21
C-C-O-C(=O)-N=N-[C;H0;D3;+0:1](=[O;D1;H0:2])-O-C-C.O-[CH;D3;+0:3]1-[C:4]-[C:5]-[#8:6]-[c:7]:[c:8]-1:[c:9].[OH;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[O;H0;D2;+0:10]-[c:11](:[c:12]):[c:13])-[CH;D3;+0:3]1-[C:4]-[C:5]-[#8:6]-[c:7]:[c:8]-1:[c:9]
null
[]
0
CELSIUS
null
null
To a stirred solution of methyl 4-hydroxy-2-methoxybenzoate (364 mg, 2.0 mmol) in dry THF (1.25 mL) was added triphenylphosphine (525 mg, 2.0 mmol) and the solution was cooled to 0° C. A 500 mL volume of 4-chromanol (200 mg, 1.33 mmol) and diethyl azodicarboxylate (315 mL, 2.0 mmol) in THF was added dropwise via syring...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Diazene.Secondary alcohol.Aromatic alcohol
Ester
c1ccc2c(c1)CCCO2
c1ccc2c(c1)CCCO2
c1ccccc1.c1ccc2c(c1)CCCO2
HO-
C1CCOC1
0
null
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.OC1CCOc2ccccc21>C1CCOC1>COC(=O)c1ccc(OC(=O)C2CCOc3ccccc32)cc1OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-319ce102069542b08b0f9d0be725ed30
COC(=O)c1ccc(OC(=O)C2CCOc3ccccc32)cc1OC>>COc1cc(OC(=O)C2CCOc3ccccc32)ccc1C(=O)O
O1CCC(C2=CC=CC=C12)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC.O.O[Li].O>>O1CCC(C2=CC=CC=C12)C(=O)OC1=CC(=C(C(=O)O)C=C1)OC
C[O:24][C:22]([c:21]1[c:3]([O:2][CH3:1])[cH:4][c:5]([O:6][C:7](=[O:8])[CH:9]2[CH2:10][CH2:11][O:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]32)[cH:19][cH:20]1)=[O:23]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][C:7](=[O:8])[CH:9]2[CH2:10][CH2:11][O:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]32)[cH:19][cH:20][c:21]1[C:22](=[O...
COC(=O)c1ccc(OC(=O)C2CCOc3ccccc32)cc1OC
COc1cc(OC(=O)C2CCOc3ccccc32)ccc1C(=O)O
null
null
C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(Oc1ccccc1)C1CCOc2ccccc21
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
45
CELSIUS
null
null
To a stirred solution of methyl 4-(4-chromanoyloxy)-2-methoxybenzoate (260 mg, 0.82 mmol) in THF:H2O (4 mL:0.8 mL) was added LiOH.H2O (172 mg, 4.1 mmol). The reaction was heated to 45° C. over 12 h and then cooled to ambient temperature. The solvent was removed under reduced pressure. The crude solid was passed through...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccc2c(c1)CCCO2
Other
C1CCOC1
45
null
COC(=O)c1ccc(OC(=O)C2CCOc3ccccc32)cc1OC>C1CCOC1>COc1cc(OC(=O)C2CCOc3ccccc32)ccc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-997799bff2054cbcbc860fbe74d39dc5
Cc1cnc2c(c1)C(=O)CC(C)(C)C2>>Cc1cnc2c(c1)C(O)CC(C)(C)C2
CC=1C=NC=2CC(CC(C2C1)=O)(C)C.[BH4-].[Na+]>>CC=1C=NC=2CC(CC(C2C1)O)(C)C
[CH3:1][c:2]1[cH:3][n:4][c:5]2[c:6]([cH:7]1)[C:8](=[O:9])[CH2:10][C:11]([CH3:12])([CH3:13])[CH2:14]2>>[CH3:1][c:2]1[cH:3][n:4][c:5]2[c:6]([cH:7]1)[CH:8]([OH:9])[CH2:10][C:11]([CH3:12])([CH3:13])[CH2:14]2
Cc1cnc2c(c1)C(=O)CC(C)(C)C2
Cc1cnc2c(c1)C(O)CC(C)(C)C2
null
null
CO
Reduction
Reduction of ketone to secondary alcohol
82dfffcf6439c6136c0fbf9d7fad4a584d93f84eff1938ce9f23f430baa33464
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1cnc2c(c1)CCCC2
[O;H0;D1;+0:1]=[C;H0;D3;+0:2]1-[C:3]-[C:4]-[C:5]-[c:6](:[#7;a:7]:[c:8]):[c:9]-1:[c:10]>>[OH;D1;+0:1]-[CH;D3;+0:2]1-[C:3]-[C:4]-[C:5]-[c:6](:[#7;a:7]:[c:8]):[c:9]-1:[c:10]
null
[]
null
null
14
HOUR
A stirred solution of 5,6,7,8-tetrahydro-3,7,7-trimethylquinoline-5-one (240 mg, 1.3 mmol) in MeOH (6.5 mL) was cooled to 0° C. under Argon and treated with NaBH4 (48 mg, 1.3 mmol). The reaction was stirred over 14 h and allowed to warm to ambient temperature. The solvent was removed under reduced pressure and the crud...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
c1cnc2c(c1)CCCC2
c1cnc2c(c1)CCCC2
c1cnc2c(c1)CCCC2
null
CO
null
14
Cc1cnc2c(c1)C(=O)CC(C)(C)C2>CO>Cc1cnc2c(c1)C(O)CC(C)(C)C2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-aaa0ddfbf41e452299afe064a36ec3cd
CCc1ncccc1C(=O)[O-]>>CCc1ncccc1CO
[Li+].C(C)C1=C(C(=O)[O-])C=CC=N1.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>C(C)C1=NC=CC=C1CO
[O-][C:9]([c:8]1[c:3]([CH2:2][CH3:1])[n:4][cH:5][cH:6][cH:7]1)=[O:10]>>[CH3:1][CH2:2][c:3]1[n:4][cH:5][cH:6][cH:7][c:8]1[CH2:9][OH:10]
CCc1ncccc1C(=O)[O-]
CCc1ncccc1CO
null
null
C1CCOC1
Reduction
OtherReaction
3ee00ae8302f5a9cabfd43f47c90c2bc696c7c0e2b77ca13873c453d0520692e
c2c13922fe3c9358e6ba38897f2383764691ea247b267e6643408d03716a3879
c1ccncc1
[C:1]-[c:2](:[#7;a:3]:[c:4]):[c:5](-[C;H0;D3;+0:6](-[O-])=[O;H0;D1;+0:7]):[c:8]>>[C:1]-[c:2](:[#7;a:3]:[c:4]):[c:5](-[CH2;D2;+0:6]-[OH;D1;+0:7]):[c:8]
null
[]
null
null
3
HOUR
The 2-ethyl nicotinic acid lithium salt (5 g, 3.18 mmol) in distilled THF (400 mL) under nitrogen was cooled to 0° C. and lithium aluminum hydride (1M in THF) (25 mL) was added dropwise. The reaction was stirred for 3 hours at room temperature then cooled to 0° C. and quenched with EtOAc (949 μL), then H2O (949 μL), th...
10.6084/m9.figshare.5104873.v1
null
null
Primary alcohol
null
null
c1ccncc1
Other
C1CCOC1
null
3
CCc1ncccc1C(=O)[O-]>C1CCOC1>CCc1ncccc1CO
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-090d23f63738479ca8c99ffd51c34f39
CCc1ncccc1CO.O=S(Cl)Cl>>CCc1ncccc1CCl
C(C)C1=NC=CC=C1CO.S(=O)(Cl)Cl>>C(C)C1=NC=CC=C1CCl
O[CH2:9][c:8]1[c:3]([CH2:2][CH3:1])[n:4][cH:5][cH:6][cH:7]1.O=S(Cl)[Cl:10]>>[CH3:1][CH2:2][c:3]1[n:4][cH:5][cH:6][cH:7][c:8]1[CH2:9][Cl:10]
CCc1ncccc1CO.O=S(Cl)Cl
CCc1ncccc1CCl
null
null
C(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
bb752b9027dc4488ba075e5955118a819f80cabd751a7497b67c2eeb1db6b071
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
c1ccncc1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5](-[C:6]):[#7;a:7]:[c:8]>>[C:6]-[c:5](:[#7;a:7]:[c:8]):[c:3](-[CH2;D2;+0:2]-[Cl;H0;D1;+0:1]):[c:4]
null
[]
0
CELSIUS
3
HOUR
The 2-ethyl-3-hydroxymethylpyridine (2.3 g, 16.8 mmol) was dissolved in CH2Cl2 (100 mL) and cooled under nitrogen to 0° C. and thionyl chloride (7.0 mL) was slowly added and the reaction was stirred for 3 hours. The solvent was removed under reduced pressure and the residue was partitioned between CH2Cl2 (100 mL) and s...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
null
null
c1ccncc1
HCl
C(Cl)Cl
0
3
CCc1ncccc1CO.O=S(Cl)Cl>C(Cl)Cl>CCc1ncccc1CCl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-50b5f885709f4236b5aee536d764bea9
CCc1ncccc1CCl.O=C(OO)c1cccc(Cl)c1>>CCc1c(CCl)ccc[n+]1[O-]
C(C)C1=NC=CC=C1CCl.ClC1=CC(=CC=C1)C(=O)OO>>C(C)C1=[N+](C=CC=C1CCl)[O-]
[CH3:1][CH2:2][c:3]1[c:4]([CH2:5][Cl:6])[cH:7][cH:8][cH:9][n:10]1.O=C(O[OH:11])c1cccc(Cl)c1>>[CH3:1][CH2:2][c:3]1[c:4]([CH2:5][Cl:6])[cH:7][cH:8][cH:9][n+:10]1[O-:11]
CCc1ncccc1CCl.O=C(OO)c1cccc(Cl)c1
CCc1c(CCl)ccc[n+]1[O-]
null
null
C(Cl)(Cl)Cl
Miscellaneous
OtherReaction
5b2b5a1eb88c9671c4a604b6f76054cc01cd86a1985fc147f7e56f19c4844d35
98b338a9d01476c0929fd5672e7509121bfe69600fd72e4d1cc6f1782e2d05d9
c1cc[nH+]cc1
Cl-c1:c:c:c:c(-C(=O)-O-[OH;D1;+0:1]):c:1.[C:2]-[c:3](:[c:4]):[n;H0;D2;+0:5]:[c:6]:[c:7]>>[C:2]-[c:3](:[c:4]):[n+;H0;D3:5](-[O-;H0;D1:1]):[c:6]:[c:7]
null
[]
0
CELSIUS
2
HOUR
The 2-ethyl-3-chloromethylpyridine (2.4 g, 15.4 mmol) was dissolved in CHCl3 (100 mL) and cooled under nitrogen to 0° C. and m-chloroperbenzoic acid (55%, 4.2 g) was added in small portions. The reaction was stirred for 2 hours. The reaction was extracted twice with saturated aqueous sodium bicarbonate (100 mL). The or...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide
null
c1ccncc1.c1ccccc1
C1=CC=[NH+]C=C1
C1=CC=[NH+]C=C1
HCl
C(Cl)(Cl)Cl
0
2
CCc1ncccc1CCl.O=C(OO)c1cccc(Cl)c1>C(Cl)(Cl)Cl>CCc1c(CCl)ccc[n+]1[O-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-13eeac45e3ff4344b45ee3f41e200838
CCOC(=O)c1cccnc1C(C)C>>CC(C)c1ncccc1CO
C(C)(C)C1=NC=CC=C1C(=O)OCC.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>C(C)(C)C1=NC=CC=C1CO
CCO[C:10]([c:9]1[c:4]([CH:2]([CH3:1])[CH3:3])[n:5][cH:6][cH:7][cH:8]1)=[O:11]>>[CH3:1][CH:2]([CH3:3])[c:4]1[n:5][cH:6][cH:7][cH:8][c:9]1[CH2:10][OH:11]
CCOC(=O)c1cccnc1C(C)C
CC(C)c1ncccc1CO
null
null
C1CCOC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccncc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5](-[C:6]):[#7;a:7]:[c:8]>>[C:6]-[c:5](:[#7;a:7]:[c:8]):[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:4]
null
[]
null
null
18
HOUR
The 2-isopropyl-3-carboethoxypyridine (400 mg, 2 mmol) in distilled THF (50 mL) under nitrogen was cooled to 0° C. and lithium aluminum hydride (1M in THF) (2.07 mL) was added dropwise. The reaction was stirred for 18 hours at room temperature then cooled to 0° C. and quenched with EtOAc (100 μL), then H2O (100 μL), th...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccncc1
HO-
C1CCOC1
null
18
CCOC(=O)c1cccnc1C(C)C>C1CCOC1>CC(C)c1ncccc1CO
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4bba085d9504420e80535135054ff927
CC(C)c1ncccc1CO.O=S(Cl)Cl>>CC(C)c1ncccc1CCl
C(C)(C)C1=NC=CC=C1CO.S(=O)(Cl)Cl>>C(C)(C)C1=NC=CC=C1CCl
O[CH2:10][c:9]1[c:4]([CH:2]([CH3:1])[CH3:3])[n:5][cH:6][cH:7][cH:8]1.O=S(Cl)[Cl:11]>>[CH3:1][CH:2]([CH3:3])[c:4]1[n:5][cH:6][cH:7][cH:8][c:9]1[CH2:10][Cl:11]
CC(C)c1ncccc1CO.O=S(Cl)Cl
CC(C)c1ncccc1CCl
null
null
C(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
bb752b9027dc4488ba075e5955118a819f80cabd751a7497b67c2eeb1db6b071
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
c1ccncc1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5](-[C:6]):[#7;a:7]:[c:8]>>[C:6]-[c:5](:[#7;a:7]:[c:8]):[c:3](-[CH2;D2;+0:2]-[Cl;H0;D1;+0:1]):[c:4]
null
[]
0
CELSIUS
3
HOUR
The 2-isopropyl-3-hydroxymethylpyridine (240 mg, 1.59 mmol) was dissolved in CH2Cl2 (15 mL) and cooled under nitrogen to 0° C. and thionyl chloride (1.0 mL) was slowly added and the reaction was stirred for 3 hours. The solvent was removed under reduced pressure and the residue was partitioned between CH2Cl2 and satura...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
null
null
c1ccncc1
HCl
C(Cl)Cl
0
3
CC(C)c1ncccc1CO.O=S(Cl)Cl>C(Cl)Cl>CC(C)c1ncccc1CCl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-52cbceab19b44bab836d091fb3264cf6
CC(C)c1ncccc1CCl.O=C(OO)c1cccc(Cl)c1>>CC(C)c1c(CCl)ccc[n+]1[O-]
C(C)(C)C1=NC=CC=C1CCl.ClC1=CC(=CC=C1)C(=O)OO>>C(C)(C)C1=[N+](C=CC=C1CCl)[O-]
[CH3:1][CH:2]([CH3:3])[c:4]1[c:5]([CH2:6][Cl:7])[cH:8][cH:9][cH:10][n:11]1.O=C(O[OH:12])c1cccc(Cl)c1>>[CH3:1][CH:2]([CH3:3])[c:4]1[c:5]([CH2:6][Cl:7])[cH:8][cH:9][cH:10][n+:11]1[O-:12]
CC(C)c1ncccc1CCl.O=C(OO)c1cccc(Cl)c1
CC(C)c1c(CCl)ccc[n+]1[O-]
null
null
C(Cl)(Cl)Cl
Miscellaneous
OtherReaction
5b2b5a1eb88c9671c4a604b6f76054cc01cd86a1985fc147f7e56f19c4844d35
98b338a9d01476c0929fd5672e7509121bfe69600fd72e4d1cc6f1782e2d05d9
c1cc[nH+]cc1
Cl-c1:c:c:c:c(-C(=O)-O-[OH;D1;+0:1]):c:1.[C:2]-[c:3](:[c:4]):[n;H0;D2;+0:5]:[c:6]:[c:7]>>[C:2]-[c:3](:[c:4]):[n+;H0;D3:5](-[O-;H0;D1:1]):[c:6]:[c:7]
null
[]
0
CELSIUS
2
HOUR
The 2-isopropyl-3-hydroxymethylpyridine (240 mg, 1.59 mmol) was dissolved in CH2Cl2 (15 mL) and cooled under nitrogen to 0° C. and thionyl chloride (1.0 mL) was slowly added and the reaction was stirred for 3 hours. The solvent was removed under reduced pressure and the residue was partitioned between CH2Cl2 and satura...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide
null
c1ccncc1.c1ccccc1
C1=CC=[NH+]C=C1
C1=CC=[NH+]C=C1
HCl
C(Cl)(Cl)Cl
0
2
CC(C)c1ncccc1CCl.O=C(OO)c1cccc(Cl)c1>C(Cl)(Cl)Cl>CC(C)c1c(CCl)ccc[n+]1[O-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4b7921c79135478487a5a927dd9e4a45
CCOC(=O)c1c(C)ccnc1C>>Cc1ccnc(C)c1CO
CC1=NC=CC(=C1C(=O)OCC)C.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>CC1=NC=CC(=C1CO)C
CCO[C:9]([c:8]1[c:2]([CH3:1])[cH:3][cH:4][n:5][c:6]1[CH3:7])=[O:10]>>[CH3:1][c:2]1[cH:3][cH:4][n:5][c:6]([CH3:7])[c:8]1[CH2:9][OH:10]
CCOC(=O)c1c(C)ccnc1C
Cc1ccnc(C)c1CO
null
null
C1CCOC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccncc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]>>[C;D1;H3:6]-[c:5](:[#7;a:7]:[c:8]):[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:4]
null
[]
null
null
18
HOUR
The 2,4-dimethyl-3-carboethoxypyridine (11.3 g, 63.1 mmol) in distilled THF (375 mL) under nitrogen was cooled to 0° C. and lithium aluminum hydride (1M in THF, 63.1 mL) was added dropwise. The reaction was stirred for 18 hours at room temperature then cooled to 0° C. and quenched with EtOAc (2.5 mL), then H2O (2.5 mL)...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccncc1
HO-
C1CCOC1
null
18
CCOC(=O)c1c(C)ccnc1C>C1CCOC1>Cc1ccnc(C)c1CO
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-bfc9e545236f4da9864ea3f99c2d6fe8
Cc1ccnc(C)c1CO.O=S(Cl)Cl>>Cc1ccnc(C)c1CCl
CC1=NC=CC(=C1CO)C.S(=O)(Cl)Cl>>CC1=NC=CC(=C1CCl)C
O[CH2:9][c:8]1[c:2]([CH3:1])[cH:3][cH:4][n:5][c:6]1[CH3:7].O=S(Cl)[Cl:10]>>[CH3:1][c:2]1[cH:3][cH:4][n:5][c:6]([CH3:7])[c:8]1[CH2:9][Cl:10]
Cc1ccnc(C)c1CO.O=S(Cl)Cl
Cc1ccnc(C)c1CCl
null
null
C(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
bb752b9027dc4488ba075e5955118a819f80cabd751a7497b67c2eeb1db6b071
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
c1ccncc1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5](-[C;D1;H3:6]):[#7;a:7]:[c:8]>>[C;D1;H3:6]-[c:5](:[#7;a:7]:[c:8]):[c:3](-[CH2;D2;+0:2]-[Cl;H0;D1;+0:1]):[c:4]
null
[]
0
CELSIUS
18
HOUR
The 2,4-dimethyl-3-hydroxymethylpyridine (19.2 g, 140 mmol) was dissolved in CH2Cl2 (800 mL) and cooled under nitrogen to 0° C. and thionyl chloride (125 mL) was slowly added and the reaction was stirred for 18 hours. The solvent was removed under reduced pressure and the residue was partitioned between CH2Cl2 and satu...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
null
null
c1ccncc1
HCl
C(Cl)Cl
0
18
Cc1ccnc(C)c1CO.O=S(Cl)Cl>C(Cl)Cl>Cc1ccnc(C)c1CCl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-bc2379efbe054eccaf35ae30843004da
Cc1ccnc(C)c1CCl>>Cc1cc[n+]([O-])c(C)c1CCl
CC1=NC=CC(=C1CCl)C.ClC1=CC(=CC=C1)C(=O)OO>>CC1=[N+](C=CC(=C1CCl)C)[O-]
[CH3:1][c:2]1[cH:3][cH:4][n:5][c:7]([CH3:8])[c:9]1[CH2:10][Cl:11]>>[CH3:1][c:2]1[cH:3][cH:4][n+:5]([O-:6])[c:7]([CH3:8])[c:9]1[CH2:10][Cl:11]
Cc1ccnc(C)c1CCl
Cc1cc[n+]([O-])c(C)c1CCl
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
OtherReaction
54415aed4bb61f76efee9ed140374352608210a9fed7c372975c12eb7023cea2
f1bbf9aa3c82f5e49be9f6d53533b6bb152f359232b6d32090c168949766aa71
c1cc[nH+]cc1
[C;D1;H3:1]-[c:2](:[c:3]):[n;H0;D2;+0:4]:[c:5]:[c:6]>>[C;D1;H3:1]-[c:2](:[c:3]):[n+;H0;D3:4](-[O;-;D1;H0:7]):[c:5]:[c:6]
null
[]
0
CELSIUS
4
HOUR
The 2,4-dimethyl-3-chloromethylpyridine (21.5 g, 138 mmol) was dissolved in CHCl3 (800 mL) and cooled under nitrogen to 0° C. and m-chloroperbenzoic acid (55%, 35 g) was added in small portions. The reaction was stirred for 4 hours. The solution was extracted twice with saturated aqueous sodium bicarbonate (500 mL). Th...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccncc1
C1=CC=[NH+]C=C1
C1=CC=[NH+]C=C1
null
C(Cl)(Cl)Cl
0
4
Cc1ccnc(C)c1CCl>C(Cl)(Cl)Cl>Cc1cc[n+]([O-])c(C)c1CCl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-75cd419ae27e4e64877635a7083429d0
CC(C)(C)OC(=O)N[C@@H]1CC[C@@H](O)CC1.CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC>>COC(=O)c1ccc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)cc1OC
C(=O)(OC(C)(C)C)N[C@@H]1CC[C@H](CC1)O.N(=NC(=O)OCC)C(=O)OCC.OC1=CC(=C(C(=O)OC)C=C1)OC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>C(=O)(OC(C)(C)C)N[C@@H]1CC[C@@H](CC1)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC
O[C@H:12]1[CH2:13][CH2:14][C@H:15]([NH:16][C:17](=[O:18])[O:19][C:20]([CH3:21])([CH3:22])[CH3:23])[CH2:24][CH2:25]1.CCOC(=O)N=N[C:10](OCC)=[O:11].[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([OH:9])[cH:26][c:27]1[O:28][CH3:29]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([O:9][C:10](=[O:11])[C@H:12]2[CH2:13][C...
CC(C)(C)OC(=O)N[C@@H]1CC[C@@H](O)CC1.CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC
COC(=O)c1ccc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)cc1OC
null
null
C1CCOC1
Acylation
OtherReaction
8e7f7aec30b10cb52f82d427bef98ab15d43a92fc5e2b024cb3b9ec94ed6a028
99cbc1de664ce75fe7841777e00c71bc93fd4ae2bce0b73a15911d06040840b5
O=C(Oc1ccccc1)C1CCCCC1
C-C-O-C(=O)-N=N-[C;H0;D3;+0:1](=[O;D1;H0:2])-O-C-C.O-[C@@H;D3;+0:3](-[C:4]-[C:5])-[C:6]-[C:7].[OH;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[C:5]-[C:4]-[C@@H;D3;+0:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:8]-[c:9](:[c:10]):[c:11])-[C:6]-[C:7]
null
[]
0
CELSIUS
null
null
To a stirred solution of methyl 4-hydroxy-2-methoxybenzoate (1.09 g, 6.0 mmol) in dry THF (7 mL) was added triphenylphosphine (1.57 g, 6.0 mmol) and the solution was cooled to 0° C. A 4.0 mL volume of N-Boc-trans-1-amino-4-cyclohexanol (1 g, 4.0 mmol) and diethyl azodicarboxylate (945 μL, 6.0 mmol) in THF was added dro...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Diazene.Secondary alcohol.Aromatic alcohol
Ester
C1CCCCC1
C1CCCCC1
c1ccccc1.C1CCCCC1
HO-
C1CCOC1
0
null
CC(C)(C)OC(=O)N[C@@H]1CC[C@@H](O)CC1.CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC>C1CCOC1>COC(=O)c1ccc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)cc1OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c883c9ea34ed4863b03fce02c544723e
COC(=O)c1ccc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)cc1OC>>COc1cc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)ccc1C(=O)O
C(=O)(OC(C)(C)C)N[C@@H]1CC[C@@H](CC1)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC.O.O[Li].O>>C(=O)(OC(C)(C)C)N[C@@H]1CC[C@@H](CC1)C(=O)OC1=CC(=C(C(=O)O)C=C1)OC
C[O:28][C:26]([c:25]1[c:3]([O:2][CH3:1])[cH:4][c:5]([O:6][C:7](=[O:8])[C@H:9]2[CH2:10][CH2:11][C@@H:12]([NH:13][C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20])[CH2:21][CH2:22]2)[cH:23][cH:24]1)=[O:27]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][C:7](=[O:8])[C@H:9]2[CH2:10][CH2:11][C@@H:12]([NH:13][C:14](=[O:15])[O:16]...
COC(=O)c1ccc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)cc1OC
COc1cc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)ccc1C(=O)O
null
null
C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(Oc1ccccc1)C1CCCCC1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
45
CELSIUS
null
null
To a stirred solution of methyl 4-[N-Boc-cis-1-amino-4-cyclohexanoyloxy]-2-methoxybenzoate (220 mg, 0.52 mmol) in THF:H2O (5 mL: 1 mL) was added LiOH.H2O (67.6 mg, 1.59 mmol). The reaction was heated to 45° C. over 12 h and then cooled to ambient temperature. The solvent was removed under reduced pressure. The crude so...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.C1CCCCC1
Other
C1CCOC1
45
null
COC(=O)c1ccc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)cc1OC>C1CCOC1>COc1cc(OC(=O)[C@@H]2CC[C@H](NC(=O)OC(C)(C)C)CC2)ccc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a131d665a87f4613af62e1177a8607d3
O=C1C=COC(=S(=O)=O)C1>>O=S(=O)=c1cc(O)cco1
S(=O)(=O)=C1OC=CC(C1)=O.[BH4-].[Na+]>>S(=O)(=O)=C1OC=CC(=C1)O
[O:1]=[S:2](=[O:3])=[C:4]1[CH2:5][C:6](=[O:7])[CH:8]=[CH:9][O:10]1>>[O:1]=[S:2](=[O:3])=[c:4]1[cH:5][c:6]([OH:7])[cH:8][cH:9][o:10]1
O=C1C=COC(=S(=O)=O)C1
O=S(=O)=c1cc(O)cco1
null
null
CO
Aromatic Heterocycle Formation
OtherReaction
48f6a1ae20952a8d41bee1c84e0d2ca7d83fe14adec55c711dcca672b806b331
809a3d08c9122e2f3c0270c24e439deaab1c0993f94d7d2072d61ea347b6388c
S=c1cccco1
[O;D1;H0:1]=[#16:2](=[O;D1;H0:3])=[C;H0;D3;+0:4]1-[CH2;D2;+0:5]-[C;H0;D3;+0:6](=[O;H0;D1;+0:7])-[CH;D2;+0:8]=[CH;D2;+0:9]-[O;H0;D2;+0:10]-1>>[O;D1;H0:1]=[#16:2](=[O;D1;H0:3])=[c;H0;D3;+0:4]1:[cH;D2;+0:5]:[c;H0;D3;+0:6](-[OH;D1;+0:7]):[cH;D2;+0:8]:[cH;D2;+0:9]:[o;H0;D2;+0:10]:1
null
[]
null
null
16
HOUR
A stirred solution of sulfonylpyran-4-one (1.2 g, 8.1 mmol) in MeOH (20 mL) was cooled to 0° C. under Argon and treated with NaBH4 (331 mg, 9.0 mmol). The reaction was stirred over 16 h and allowed to warm to ambient temperature. The solvent was removed under reduced pressure and the crude oil was chromatographed on a ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ether
Aromatic alcohol
C1=COCCC1
c1ccocc1
c1ccocc1
null
CO
null
16
O=C1C=COC(=S(=O)=O)C1>CO>O=S(=O)=c1cc(O)cco1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e3ff06e7d5dc4790a4038ff5d1f041f4
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.O=S(=O)=c1cc(O)cco1>>COC(=O)c1ccc(OC(=O)c2cc(=S(=O)=O)cco2)cc1OC
S(=O)(=O)=C1OC=CC(=C1)O.N(=NC(=O)OCC)C(=O)OCC.C1CCOC1.OC1=CC(=C(C(=O)OC)C=C1)OC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1>>S(=O)(=O)=C1C=C(OC=C1)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC
CCOC(=O)N=N[C:10](OCC)=[O:11].[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([OH:9])[cH:21][c:22]1[O:23][CH3:24].O[c:14]1[cH:13][c:12](=[S:15](=[O:16])=[O:17])[o:20][cH:19][cH:18]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([O:9][C:10](=[O:11])[c:12]2[cH:13][c:14](=[S:15](=[O:16])=[O:17])[cH:18][cH:19][o:20]2)...
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.O=S(=O)=c1cc(O)cco1
COC(=O)c1ccc(OC(=O)c2cc(=S(=O)=O)cco2)cc1OC
null
null
null
Acylation
OtherReaction
82d3e3db198980f8c67f3eef4d9a4d912866b4f02d668a9bb06a72a6b1dd6d52
e265b1a668f6a16830e4b2b8abe472d5c9a52f6819ca25184b71f87b06186734
O=C(Oc1ccccc1)c1cc(=S)cco1
C-C-O-C(=O)-N=N-[C;H0;D3;+0:1](=[O;D1;H0:2])-O-C-C.O-[c;H0;D3;+0:3]1:[c:4]:[c;H0;D3;+0:5](=[S;H0;D3;+0:6](=[O;D1;H0:7])=[O;D1;H0:8]):[#8;a:9]:[c:10]:[c:11]:1.[OH;D1;+0:12]-[c:13](:[c:14]):[c:15]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[O;H0;D2;+0:12]-[c:13](:[c:14]):[c:15])-[c;H0;D3;+0:5]1:[#8;a:9]:[c:10]:[c:11]:[c;H0;D3;+0:3](=[...
null
[]
0
CELSIUS
null
null
To a stirred solution of methyl 4-hydroxy-2-methoxybenzoate (364 mg, 2.0 mmol) in dry THF (4 mL) was added triphenylphosphine (524.6 mg, 2.0 mmol) and the solution was cooled to 0° C. A 2.5 mL volume of sulfonylpyran-4-ol (200 mg, 1.33 mmol) and diethyl azodicarboxylate (315 μL, 2.0 mmol) in THF was added dropwise via ...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Diazene.Aromatic alcohol.Aromatic alcohol
Ester
c1ccocc1
c1ccocc1
c1ccccc1.c1ccocc1
HO-
null
0
null
CCOC(=O)N=NC(=O)OCC.COC(=O)c1ccc(O)cc1OC.O=S(=O)=c1cc(O)cco1>>COC(=O)c1ccc(OC(=O)c2cc(=S(=O)=O)cco2)cc1OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-633f98fd12d84e92930ec5dccc1d3957
COC(=O)c1ccc(OC(=O)c2cc(=S(=O)=O)cco2)cc1OC>>COc1cc(OC(=O)c2cc(=S(=O)=O)cco2)ccc1C(=O)O
S(=O)(=O)=C1C=C(OC=C1)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC.O.O[Li].O>>S(=O)(=O)=C1C=C(OC=C1)C(=O)OC1=CC(=C(C(=O)O)C=C1)OC
C[O:23][C:21]([c:20]1[c:3]([O:2][CH3:1])[cH:4][c:5]([O:6][C:7](=[O:8])[c:9]2[cH:10][c:11](=[S:12](=[O:13])=[O:14])[cH:15][cH:16][o:17]2)[cH:18][cH:19]1)=[O:22]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][C:7](=[O:8])[c:9]2[cH:10][c:11](=[S:12](=[O:13])=[O:14])[cH:15][cH:16][o:17]2)[cH:18][cH:19][c:20]1[C:21](=[O:22])[OH:23]
COC(=O)c1ccc(OC(=O)c2cc(=S(=O)=O)cco2)cc1OC
COc1cc(OC(=O)c2cc(=S(=O)=O)cco2)ccc1C(=O)O
null
null
C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(Oc1ccccc1)c1cc(=S)cco1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
45
CELSIUS
null
null
To a stirred solution of methyl 4-[4-sulfonylpyranoyloxy]-2-methoxybenzoate (470 mg, 1.5 mmol)in THF:H2O (18 mL: 2 mL) was added LiOH.H2O (128 mg, 3 mmol). The reaction was heated to 45° C. over 12 h and then cooled to ambient temperature. The solvent was removed under reduced pressure. The crude solid passed through a...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccocc1
Other
C1CCOC1
45
null
COC(=O)c1ccc(OC(=O)c2cc(=S(=O)=O)cco2)cc1OC>C1CCOC1>COc1cc(OC(=O)c2cc(=S(=O)=O)cco2)ccc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-46bdac7b5dca4dd2b9ea60dfb2c0fdfb
COC(=O)c1ccc(OC(=O)C2CC(=S(=O)=O)c3ccccc3O2)cc1OC>>COc1cc(OC(=O)C2CC(=S(=O)=O)c3ccccc3O2)ccc1C(=O)O
S(=O)(=O)=C1CC(OC2=CC=CC=C12)C(=O)OC1=CC(=C(C(=O)OC)C=C1)OC.O.O[Li].O>>S(=O)(=O)=C1CC(OC2=CC=CC=C12)C(=O)OC1=CC(=C(C(=O)O)C=C1)OC
C[O:27][C:25]([c:24]1[c:3]([O:2][CH3:1])[cH:4][c:5]([O:6][C:7](=[O:8])[CH:9]2[CH2:10][C:11](=[S:12](=[O:13])=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19][c:20]3[O:21]2)[cH:22][cH:23]1)=[O:26]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][C:7](=[O:8])[CH:9]2[CH2:10][C:11](=[S:12](=[O:13])=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19]...
COC(=O)c1ccc(OC(=O)C2CC(=S(=O)=O)c3ccccc3O2)cc1OC
COc1cc(OC(=O)C2CC(=S(=O)=O)c3ccccc3O2)ccc1C(=O)O
null
null
C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(Oc1ccccc1)C1CC(=S)c2ccccc2O1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
45
CELSIUS
null
null
To a stirred solution of methyl 4-[4-sulfonylchromanoyloxy]-2-methoxybenzoate (500 mg, 1.38 mmol) in THF:H2O (18 mL: 2 mL) was added LiOH.H2O (175 mg, 4.14 mmol). The reaction was heated to 45° C. over 12 h and then cooled to ambient temperature. The solvent was removed under reduced pressure. The crude solid was passe...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccc2c(c1)CCCO2
Other
C1CCOC1
45
null
COC(=O)c1ccc(OC(=O)C2CC(=S(=O)=O)c3ccccc3O2)cc1OC>C1CCOC1>COc1cc(OC(=O)C2CC(=S(=O)=O)c3ccccc3O2)ccc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-69fd522121284a219b8d7faaa6a44613
COc1c(C(=O)O)cc(F)c(O)c1C.C[C@H](O)c1ccncc1>>COC(=O)c1cc(F)c(O[C@@H](C)c2ccncc2)cc1OC
CC=1C(=C(C(=O)O)C=C(C1O)F)OC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.N1=CC=C(C=C1)[C@H](C)O>>FC=1C(=CC(=C(C(=O)OC)C1)OC)O[C@@H](C)C1=CC=NC=C1
[CH3:1][c:19]1[c:9]([OH:10])[c:7]([F:8])[cH:6][c:5]([C:3]([OH:2])=[O:4])[c:20]1[O:21][CH3:22].O[C@@H:11]([CH3:12])[c:13]1[cH:14][cH:15][n:16][cH:17][cH:18]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([F:8])[c:9]([O:10][C@@H:11]([CH3:12])[c:13]2[cH:14][cH:15][n:16][cH:17][cH:18]2)[cH:19][c:20]1[O:21][CH3:22]
COc1c(C(=O)O)cc(F)c(O)c1C.C[C@H](O)c1ccncc1
COC(=O)c1cc(F)c(O[C@@H](C)c2ccncc2)cc1OC
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
8a8724ed8fc380edd0de18f8c85c3981a493ec1ce8a1f1b33cae45dc36c4c406
f169f08614001d3d83f7341aab0dfd0af402046a91ce1b341334937672ec5630
c1ccc(OCc2ccncc2)cc1
O-[C@@H;D3;+0:1](-[C;D1;H3:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1.[#8:9]-[c:10](:[c:11]-[C:12](=[O;D1;H0:13])-[OH;D1;+0:14]):[c;H0;D3;+0:15](-[CH3;D1;+0:16]):[c:17](-[OH;D1;+0:18]):[c:19]>>[#8:9]-[c:10](:[c:11]-[C:12](=[O;D1;H0:13])-[O;H0;D2;+0:14]-[CH3;D1;+0:16]):[cH;D2;+0:15]:[c:17](-[O;H0;D2;+0:18]-[C@@H;D3;+...
null
[]
0
CELSIUS
null
null
A stirred solution of methyl 5-fluoro-2-methoxy-4-hydroxybenzoic acid (250 mg, 1.25 mmol, see Scheme II) in THF (15 mL) was treated with triphenylphosphine (494 mg, 1.88 mmol) and cooled to 0° C. under Argon. To this was added, dropwise over a period of 1 h, a solution of (S)-(-)-1-(4-pyridyl)-ethanol (232 mg, 1.88 mmo...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary alcohol.Aromatic alcohol
Ester.Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccncc1
HO-
C1CCOC1
0
null
COc1c(C(=O)O)cc(F)c(O)c1C.C[C@H](O)c1ccncc1>C1CCOC1>COC(=O)c1cc(F)c(O[C@@H](C)c2ccncc2)cc1OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-71a42b3bba7745d89371d9c19ddb7d49
COC(=O)c1cc(F)c(O[C@@H](C)c2ccncc2)cc1OC>>COc1cc(O[C@@H](C)c2ccncc2)c(F)cc1C(=O)O
O.CC#N.Cl.FC=1C(=CC(=C(C(=O)OC)C1)OC)O[C@@H](C)C1=CC=NC=C1.[OH-].[Na+]>>FC=1C(=CC(=C(C(=O)O)C1)OC)O[C@@H](C)C1=CC=NC=C1
C[O:21][C:19]([c:18]1[c:3]([O:2][CH3:1])[cH:4][c:5]([O:6][C@@H:7]([CH3:8])[c:9]2[cH:10][cH:11][n:12][cH:13][cH:14]2)[c:15]([F:16])[cH:17]1)=[O:20]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][C@@H:7]([CH3:8])[c:9]2[cH:10][cH:11][n:12][cH:13][cH:14]2)[c:15]([F:16])[cH:17][c:18]1[C:19](=[O:20])[OH:21]
COC(=O)c1cc(F)c(O[C@@H](C)c2ccncc2)cc1OC
COc1cc(O[C@@H](C)c2ccncc2)c(F)cc1C(=O)O
null
null
CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(OCc2ccncc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
null
null
8
HOUR
To a stirred solution of methyl 5-fluoro-2-methoxy-4-[1-(S)-(4-pyridyl)ethoxy]benzoate (290 mg, 0.95 mmol) in methanol (5 mL) was added aqueous NaOH (396 μL, 3.6M). The reaction was stirred at ambient temperature overnight and then heated to 45° C. in an oil bath for another 24 h. The reaction pH was lowered to pH 3 us...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccncc1
Other
CO
null
8
COC(=O)c1cc(F)c(O[C@@H](C)c2ccncc2)cc1OC>CO>COc1cc(O[C@@H](C)c2ccncc2)c(F)cc1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9773b48b03f44090887256b458e3e63d
O=S(=O)(Cl)C(F)(F)F.OCC(F)(F)F>>O=S(=O)(OCC(F)(F)F)C(F)(F)F
FC(S(=O)(=O)Cl)(F)F.C(=O)=O.FC(CO)(F)F.C(C)N(CC)CC>>FC(COS(=O)(=O)C(F)(F)F)(F)F
Cl[S:2](=[O:1])(=[O:3])[C:10]([F:11])([F:12])[F:13].[OH:4][CH2:5][C:6]([F:7])([F:8])[F:9]>>[O:1]=[S:2](=[O:3])([O:4][CH2:5][C:6]([F:7])([F:8])[F:9])[C:10]([F:11])([F:12])[F:13]
O=S(=O)(Cl)C(F)(F)F.OCC(F)(F)F
O=S(=O)(OCC(F)(F)F)C(F)(F)F
null
null
CCOCC.CC(C)O.C(Cl)Cl
Acylation
Formation of Sulfonic Esters
48fe3ab9ea419cabd2d3de445d20daee08ec8a66d593e83c888de3f63cb35bc2
90c05d4caa9001bd1d36ec239cccc93846c698579e9e88faf7db9bc82dbd1926
null
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7].[F;D1;H0:8]-[C:9](-[F;D1;H0:10])(-[F;D1;H0:11])-[C:12]-[OH;D1;+0:13]>>[F;D1;H0:5]-[C:4](-[F;D1;H0:6])(-[F;D1;H0:7])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[O;H0;D2;+0:13]-[C:12]-[C:9](-[F;D1;H0:8])(-[F;D1;H0:10])-[F;D1;H0:11...
null
[]
0
CELSIUS
1.5
HOUR
A solution of trifluoromethanesulfonyl chloride (640 μL, 6 mmol) in CH2Cl2 (5 mL) was cooled under argon to -78° C. (IPA:dry ice bath). 2,2,2-Trifluoroethanol was added (365 μL, 5 mmol) and triethylamine (834 μL, 6 mmol) was added dropwise. The reaction was stirred for 1.5 hours then warmed to 0° C. for 1 hour. Anhydro...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Sulfonyl halide
Triflate
null
null
null
HCl
CCOCC.CC(C)O.C(Cl)Cl
0
1.5
O=S(=O)(Cl)C(F)(F)F.OCC(F)(F)F>CCOCC.CC(C)O.C(Cl)Cl>O=S(=O)(OCC(F)(F)F)C(F)(F)F
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c1eb50330c204669ac80b93517bb8dec
O=S(=O)(Cl)C(F)(F)F.OCC(F)(F)F>>O=S(=O)(OCC(F)(F)F)C(F)(F)F
FC(S(=O)(=O)Cl)(F)F.C(=O)=O.FC(CO)(F)F.C(C)N(CC)CC>>FC(COS(=O)(=O)C(F)(F)F)(F)F
Cl[S:2](=[O:1])(=[O:3])[C:10]([F:11])([F:12])[F:13].[OH:4][CH2:5][C:6]([F:7])([F:8])[F:9]>>[O:1]=[S:2](=[O:3])([O:4][CH2:5][C:6]([F:7])([F:8])[F:9])[C:10]([F:11])([F:12])[F:13]
O=S(=O)(Cl)C(F)(F)F.OCC(F)(F)F
O=S(=O)(OCC(F)(F)F)C(F)(F)F
null
null
CCOCC.CC(C)O.C(Cl)Cl
Acylation
Formation of Sulfonic Esters
48fe3ab9ea419cabd2d3de445d20daee08ec8a66d593e83c888de3f63cb35bc2
90c05d4caa9001bd1d36ec239cccc93846c698579e9e88faf7db9bc82dbd1926
null
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7].[F;D1;H0:8]-[C:9](-[F;D1;H0:10])(-[F;D1;H0:11])-[C:12]-[OH;D1;+0:13]>>[F;D1;H0:5]-[C:4](-[F;D1;H0:6])(-[F;D1;H0:7])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[O;H0;D2;+0:13]-[C:12]-[C:9](-[F;D1;H0:8])(-[F;D1;H0:10])-[F;D1;H0:11...
null
[]
0
CELSIUS
1.5
HOUR
A solution of trifluoromethanesulfonyl chloride (800 uL, 7.5 mmole) in CH2Cl2 (6 mL) was cooled under argon to -60° C. (IPA:dry ice bath). 2,2,2-Trifluoroethanol was added (456 uL, 6 mmol) and triethylamine (1.04 uL, 7.5 mmol) was added dropwise. The reaction was stirred for 1.5 hours then warmed to 0° C. for 1 hour. A...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Sulfonyl halide
Triflate
null
null
null
HCl
CCOCC.CC(C)O.C(Cl)Cl
0
1.5
O=S(=O)(Cl)C(F)(F)F.OCC(F)(F)F>CCOCC.CC(C)O.C(Cl)Cl>O=S(=O)(OCC(F)(F)F)C(F)(F)F
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-1e6b8897562d412183a40fa3b1ae7fd3
COc1cc(OCC(F)(F)F)c(F)cc1C(=O)[O-]>>O=C(O)c1ccc(OCC(F)(F)F)c(F)c1
COC1=C(C(=O)[O-])C=C(C(=C1)OCC(F)(F)F)F.[OH-].[Na+].Cl>>FC(COC1=CC=C(C(=O)O)C=C1F)(F)F
CO[c:5]1[c:4]([C:2](=[O:1])[O-:3])[cH:16][c:14]([F:15])[c:7]([O:8][CH2:9][C:10]([F:11])([F:12])[F:13])[cH:6]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([O:8][CH2:9][C:10]([F:11])([F:12])[F:13])[c:14]([F:15])[cH:16]1
COc1cc(OCC(F)(F)F)c(F)cc1C(=O)[O-]
O=C(O)c1ccc(OCC(F)(F)F)c(F)c1
null
null
C1CCOC1.O
Reduction
OtherReaction
1429fe65d6db718c9183c85d60c34e1d02dcb32f985a35486f4318002b1dab1d
fc36b78de76f2c5141892df769222d9a793f25ecdae731308a2cae6bc6b43b17
c1ccccc1
C-O-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C:5](-[O-;H0;D1:6])=[O;D1;H0:7]):[c:8]>>[O;D1;H0:7]=[C:5](-[OH;D1;+0:6])-[c:4](:[c:8]):[cH;D2;+0:1]:[c:2]:[c:3]
null
[]
50
CELSIUS
18
HOUR
The above methoxy-4-trifluoroethoxy-5-fluorobenzoate (420 mg, 1.7 mmol) was dissolved in freshly distilled THF (50 mL) and water was added (20 mL) and 2N NaOH (2 mL) was dropped into the rapidly stirring solution at room temperature. The solution was warmed to 50° C. and stirred rapidly for 18 hours. The biphasic resul...
10.6084/m9.figshare.5104873.v1
null
Ether
Carboxylic acid
c1ccccc1
c1ccccc1
c1ccccc1
HO-
C1CCOC1.O
50
18
COc1cc(OCC(F)(F)F)c(F)cc1C(=O)[O-]>C1CCOC1.O>O=C(O)c1ccc(OCC(F)(F)F)c(F)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-68830d19234b4026807695ab721a68e9
CN(C)C(=O)N(C)C.O=C(Cl)C(=O)Cl>>CN(C)C(Cl)=[N+](C)C.[Cl-]
C(=O)=O.C(C(=O)Cl)(=O)Cl.CN(C(N(C)C)=O)C>>[Cl-].CN(C(=[N+](C)C)Cl)C
O=[C:4]([N:2]([CH3:1])[CH3:3])[N:6]([CH3:7])[CH3:8].O=C(C(=O)[Cl:9])[Cl:5]>>[CH3:1][N:2]([CH3:3])[C:4]([Cl:5])=[N+:6]([CH3:7])[CH3:8].[Cl-:9]
CN(C)C(=O)N(C)C.O=C(Cl)C(=O)Cl
CN(C)C(Cl)=[N+](C)C.[Cl-]
null
null
C(Cl)(Cl)(Cl)Cl
Miscellaneous
OtherReaction
343921b6cff5b43b8473a5520afb84d0f50313d1265a93af30b50408e3de339a
acce834eaacd8ad844a742ace5a164ab68132488e5eb9b0306e028af44623650
null
O=C(-[Cl;H0;D1;+0:1])-C(=O)-[Cl;H0;D1;+0:2].O=[C;H0;D3;+0:3](-[#7:4](-[C;D1;H3:5])-[C;D1;H3:6])-[N;H0;D3;+0:7](-[C;D1;H3:8])-[C;D1;H3:9]>>[C;D1;H3:5]-[#7:4](-[C;D1;H3:6])-[C;H0;D3;+0:3](-[Cl;H0;D1;+0:1])=[N+;H0;D3:7](-[C;D1;H3:8])-[C;D1;H3:9].[Cl-;H0;D0:2]
null
[]
null
null
null
null
A solution of 3.2 ml (0.037 mol) of oxalyl chloride in 30 ml of anhydrous carbon tetrachloride is added dropwise to a solution of 4.4 ml (0.037 mol) of tetramethylurea in 20 ml of anhydrous carbon tetrachloride with stirring. The reaction medium is maintained at reflux, with continued stirring, until the evolution of g...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Urea
Alkenyl halide.Amidinium
null
null
null
Other
C(Cl)(Cl)(Cl)Cl
null
null
CN(C)C(=O)N(C)C.O=C(Cl)C(=O)Cl>C(Cl)(Cl)(Cl)Cl>CN(C)C(Cl)=[N+](C)C.[Cl-]