dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-71828877dd4a46a7a0bca4e4e2ebc272
COc1ccc2cc(N(C)C)sc2c1>>COc1ccc2c(c1)SC(=O)C2
CN(C1=CC2=C(S1)C=C(C=C2)OC)C.O1CCCC1.Cl>>COC1=CC2=C(CC(=O)S2)C=C1
CN(C)[c:10]1[s:9][c:7]2[c:6]([cH:5][cH:4][c:3]([O:2][CH3:1])[cH:8]2)[cH:12]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[S:9][C:10](=[O:11])[CH2:12]2
COc1ccc2cc(N(C)C)sc2c1
COc1ccc2c(c1)SC(=O)C2
null
null
null
Miscellaneous
OtherReaction
7ec91e72ad4514f96d10825f092a3f78fdb6234593bffc93605e8ff2e9a497de
b4305623bf739174ef5934db06197c51126cdafe031b92baeff8df43c46cbb25
O=C1Cc2ccccc2S1
C-N(-C)-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[c:3](:[c:4]):[c:5](:[c:6]):[s;H0;D2;+0:7]:1>>[O;D1;H0:8]=[C;H0;D3;+0:1]1-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5](:[c:6])-[S;H0;D2;+0:7]-1
80
[{"value": 80.0, "product": "COC1=CC2=C(CC(=O)S2)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To tetrahydrofuran (200 mL) containing 2-dimethylamino-6-methoxybenzo-[b]-thiophene (cf. U.S. Pat. No. 5,420,349) (20.00 g, 96.5 mmol) was added 1N aqueous HCl (200 mL) and the resulting mixture was heated to reflux for 3 h. The mixture was cooled, the layers were separated, and the aqueous layer was extracted with dic...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
Carbo-thioester
c1ccc2sccc2c1
c1ccc2c(c1)CCS2
c1ccc2c(c1)CCS2
Other
null
null
null
COc1ccc2cc(N(C)C)sc2c1>>COc1ccc2c(c1)SC(=O)C2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-121fc81dc41c4c78b8c1bded1233dd08
COc1ccc(C=O)c(O)c1.COc1ccc2c(c1)SC(=O)C2>>COc1ccc2c(c1)OC(=O)C1c3ccc(OC)cc3SC21
COC1=CC2=C(CC(=O)S2)C=C1.COC=1C=C(C(C=O)=CC1)O>>COC1=CC2=C(C3C(C(O2)=O)C2=C(S3)C=C(C=C2)OC)C=C1
O=[CH:22][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:8][c:7]1[OH:9].[C:10]1(=[O:11])[CH2:12][c:13]2[cH:14][cH:15][c:16]([O:17][CH3:18])[cH:19][c:20]2[S:21]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[O:9][C:10](=[O:11])[CH:12]1[c:13]3[cH:14][cH:15][c:16]([O:17][CH3:18])[cH:19][c:20]3[S:21][CH:22]21
COc1ccc(C=O)c(O)c1.COc1ccc2c(c1)SC(=O)C2
COc1ccc2c(c1)OC(=O)C1c3ccc(OC)cc3SC21
null
C(C)N(CC)CC
C(C)O.C(Cl)Cl
Acylation
OtherReaction
e8fbc487563db87775f9ef5b53c3692d363b1a0498769b64bd7c794649742d9d
7259bf0e4ba555fe66049920a15c643fe90ace826f32b0be86332a42da8e3e0d
O=C1Oc2ccccc2C2Sc3ccccc3C12
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4](-[OH;D1;+0:5]):[c:6].[O;D1;H0:7]=[C;H0;D3;+0:8]1-[CH2;D2;+0:9]-[c:10](:[c:11]):[c:12](:[c:13])-[S;H0;D2;+0:14]-1>>[O;D1;H0:7]=[C;H0;D3;+0:8]1-[O;H0;D2;+0:5]-[c:4](:[c:6]):[c:2](:[c:3])-[CH;D3;+0:1]2-[S;H0;D2;+0:14]-[c:12](:[c:13]):[c:10](:[c:11])-[CH;D3;+0:9]-1-2
82.3
[{"value": 82.0, "product": "COC1=CC2=C(C3C(C(O2)=O)C2=C(S3)C=C(C=C2)OC)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 82.3, "product": "COC1=CC2=C(C3C(C(O2)=O)C2=C(S3)C=C(C=C2)OC)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a stirred solution of 6-methoxythianaphthen-2-one (see Docket B-9459) (20 g, 111 mmol) in a mixture of ethanol (100 mL) and methylene chloride (50 mL) was added 4-methoxysalicylaldehyde (17.5 g, 115 mmol) followed by triethylamine (567 mg, 784 mL, 5.6 mmol) at room temperature. After 30 min, a solid began to precipi...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Aromatic alcohol.Carbo-thioester
Ester.Monosulfide
c1ccc2c(c1)CCS2
c1ccc2c(c1)OCC1c3ccccc3SC21
c1ccc2c(c1)OCC1c3ccccc3SC21
HO-
C(C)N(CC)CC.C(C)O.C(Cl)Cl
null
0.5
COc1ccc(C=O)c(O)c1.COc1ccc2c(c1)SC(=O)C2>C(C)N(CC)CC.C(C)O.C(Cl)Cl>COc1ccc2c(c1)OC(=O)C1c3ccc(OC)cc3SC21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-37dabead809445b0a1f66e1d5ecbac91
O=S(=O)(Oc1ccc2c(c1)OC(c1ccc(OCCN3CCCCC3)cc1)c1c-2sc2cc(OS(=O)(=O)C(F)(F)F)ccc12)C(F)(F)F>>c1ccc2c(c1)OC(c1ccc(OCCN3CCCCC3)cc1)c1c-2sc2ccccc12
FC(S(=O)(=O)OC1=CC2=C(C3=C(C(O2)C2=CC=C(C=C2)OCCN2CCCCC2)C2=C(S3)C=C(C=C2)OS(=O)(=O)C(F)(F)F)C=C1)(F)F.C1(=CC=CC=C1)P(C1=CC=CC=C1)CCC.C(=O)O.C(C)N(CC)CC>>N1(CCCCC1)CCOC1=CC=C(C=C1)C1OC2=C(C3=C1C1=C(S3)C=CC=C1)C=CC=C2
O=S(=O)(O[c:1]1[cH:2][cH:3][c:4]2[c:5]([cH:6]1)[O:7][CH:8]([c:9]1[cH:10][cH:11][c:12]([O:13][CH2:14][CH2:15][N:16]3[CH2:17][CH2:18][CH2:19][CH2:20][CH2:21]3)[cH:22][cH:23]1)[c:24]1[c:25]-2[s:26][c:27]2[cH:28][c:29](OS(=O)(=O)C(F)(F)F)[cH:30][cH:31][c:32]12)C(F)(F)F>>[cH:1]1[cH:2][cH:3][c:4]2[c:5]([cH:6]1)[O:7][CH:8]([c...
O=S(=O)(Oc1ccc2c(c1)OC(c1ccc(OCCN3CCCCC3)cc1)c1c-2sc2cc(OS(=O)(=O)C(F)(F)F)ccc12)C(F)(F)F
c1ccc2c(c1)OC(c1ccc(OCCN3CCCCC3)cc1)c1c-2sc2ccccc12
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
CN(C=O)C
Functional Group Interconversion
OtherReaction
988f610538c90607221e55e921999ae11469ded1c50793c97c36afbad156792b
e253988a7a940b0d8f3e3d18b6e23b919f63a40009ea6501e6258cd32fcc6067
c1ccc2c(c1)OC(c1ccc(OCCN3CCCCC3)cc1)c1c-2sc2ccccc12
F-C(-F)(-F)-S(=O)(=O)-O-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]-[#8:6].F-C(-F)(-F)-S(=O)(=O)-O-[c;H0;D3;+0:7]1:[c:8]:[c:9](:[#16;a:10]:[c:11]):[c:12]:[c:13]:[c:14]:1>>[#8:6]-[c:5]:[c:4]:[cH;D2;+0:1]:[c:2]:[c:3].[c:11]:[#16;a:10]:[c:9]1:[c:8]:[cH;D2;+0:7]:[c:14]:[c:13]:[c:12]:1
57
[{"value": 57.0, "product": "N1(CCCCC1)CCOC1=CC=C(C=C1)C1OC2=C(C3=C1C1=C(S3)C=CC=C1)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.0, "product": "N1(CCCCC1)CCOC1=CC=C(C=C1)C1OC2=C(C3=C1C1=C(S3)C=CC=C1)C=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of the product of Example 6 (780 mg, 1.06 mmol), palladium(II) acetate (42 mg, 0.19 mmol), 1,2-bis(diphenylphosphinopropane (149 mg, 0.36 mmol), formic acid (0.6 mL), and triethylamine (3.0 mL) in anhydrous dimethylformamide (40 mL) was stirred at ambient temperature for 4 d. After concentration, the residue...
10.6084/m9.figshare.5104873.v1
null
Triflate.Triflate
null
c1ccc2c(c1)OCc1c3ccccc3sc12
c1ccc2c(c1)OCc1c3ccccc3sc12
c1ccccc1.C1CC[NH]CC1.c1ccc2c(c1)OCc1c3ccccc3sc12
TfOH
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CN(C=O)C
null
null
O=S(=O)(Oc1ccc2c(c1)OC(c1ccc(OCCN3CCCCC3)cc1)c1c-2sc2cc(OS(=O)(=O)C(F)(F)F)ccc12)C(F)(F)F>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CN(C=O)C>c1ccc2c(c1)OC(c1ccc(OCCN3CCCCC3)cc1)c1c-2sc2ccccc12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2e1c1509e9854bccbce85b7561bd70a2
COC(=O)C1C(=O)CCc2cc(OC)ccc21.Oc1cccc(O)c1>>COc1ccc2c(c1)CCc1c-2c(=O)oc2cc(O)ccc12
O.C(=O)(OC)C1C(CCC2=CC(=CC=C12)OC)=O.C1(O)=CC(O)=CC=C1.P(=O)(Cl)(Cl)Cl>>COC=1C=C2CCC=3C4=C(OC(C3C2=CC1)=O)C=C(C=C4)O
CO[C:13]([CH:12]1[c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:8][c:7]2[CH2:9][CH2:10][C:11]1=O)=[O:14].[OH:15][c:16]1[cH:17][c:18]([OH:19])[cH:20][cH:21][cH:22]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[CH2:9][CH2:10][c:11]1[c:12]-2[c:13](=[O:14])[o:15][c:16]2[cH:17][c:18]([OH:19])[cH:20][cH:21][c:22]12
COC(=O)C1C(=O)CCc2cc(OC)ccc21.Oc1cccc(O)c1
COc1ccc2c(c1)CCc1c-2c(=O)oc2cc(O)ccc12
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
4d3aeb8ad75885a43a483a2b4c96b3e7b33057d5f173c48e07c290188732a993
89a9e45776dbe9070f40025f4f55f2a7b9907ff5b9cebad1727718d85938e303
O=c1oc2ccccc2c2c1-c1ccccc1CC2
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH;D3;+0:3]1-[C;H0;D3;+0:4](=O)-[C:5]-[C:6]-[c:7](:[c:8]):[c;H0;D3;+0:9]-1:[c:10]:[c:11].[OH;D1;+0:12]-[c:13](:[c:14]):[cH;D2;+0:15]:[c:16]:[c:17]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[o;H0;D2;+0:12]:[c:13](:[c:14]):[c;H0;D3;+0:15](:[c:16]:[c:17]):[c;H0;D3;+0:4]2:[c;H0;D3;+0:3]:1-[c;H0;D3;+0:9...
70.8
[{"value": 70.8, "product": "COC=1C=C2CCC=3C4=C(OC(C3C2=CC1)=O)C=C(C=C4)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
To a solution of 1-carbomethoxy-6-methoxy-2-tetralone (see, Colvin, Martin, and Shroot, Chemistry and Industry, 2130 (1966)) (18.0 g, 76.8 mmol) and resorcinol (8.9 g, 80.7 mmol) stirring at ambient temperature in toluene (450 mL) was added phosphorus oxychloride (12.0 g, 7.3 mL, 18.3 mmol) dropwise, and the mixture wa...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Aromatic alcohol
null
c1ccc2c(c1)CCCC2.c1ccccc1
c1ccc2c(c1)CCc1c2coc2ccccc12
c1ccc2c(c1)CCc1c2coc2ccccc12
HO-
C1(=CC=CC=C1)C
80
null
COC(=O)C1C(=O)CCc2cc(OC)ccc21.Oc1cccc(O)c1>C1(=CC=CC=C1)C>COc1ccc2c(c1)CCc1c-2c(=O)oc2cc(O)ccc12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9257a86a9c6c4200ba96f6bf32445239
COc1ccc2c(c1)CCCC2=O.Nc1ccc(O)cc1>>COc1ccc2c(c1)CCCC2=Nc1ccc(O)cc1
COC=1C=C2CCCC(C2=CC1)=O.OC1=CC=C(N)C=C1>>COC=1C=C2CCCC(C2=CC1)=NC1=CC=C(C=C1)O
O=[C:12]1[c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:8][c:7]2[CH2:9][CH2:10][CH2:11]1.[NH2:13][c:14]1[cH:15][cH:16][c:17]([OH:18])[cH:19][cH:20]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[CH2:9][CH2:10][CH2:11][C:12]2=[N:13][c:14]1[cH:15][cH:16][c:17]([OH:18])[cH:19][cH:20]1
COc1ccc2c(c1)CCCC2=O.Nc1ccc(O)cc1
COc1ccc2c(c1)CCCC2=Nc1ccc(O)cc1
null
null
null
Heteroatom Alkylation and Arylation
Addition of primary amines to ketones/thiocarbonyls
b14ccdda6d8ec09f2623d3e2d2e8e272a424167acc06de88631d823acb29461f
009cc6a97ebe0dc96c669f0ef59b95bcc20de7cae20b1b648ce8f8fa82309e57
c1ccc(N=C2CCCc3ccccc32)cc1
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[C:3]-[C:2]-[C;H0;D3;+0:1](=[N;H0;D2;+0:7]-[c:8](:[c:9]):[c:10])-[c:4](:[c:5]):[c:6]
null
[]
180
CELSIUS
null
null
A mixture of 6-methoxytetralone (25 g, 142 mmol) and 4-hydroxyaniline (16.3 g, 149 mmol) was heated to 180° C. under a nitrogen stream for 2 h. After cooling to ambient temperature, the solid mass was recrystallized from toluene/methanol: 1H NMR (300 MHz) d 8.15 (d, J=9.7 Hz, 1H), 6.5-7.9 (m, 6H), 3.80 (s, 3H), 2.84 (t...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Substituted imine
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2.c1ccccc1
HO-
null
180
null
COc1ccc2c(c1)CCCC2=O.Nc1ccc(O)cc1>>COc1ccc2c(c1)CCCC2=Nc1ccc(O)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3b73803622b24e07932df49f9cb1154a
COc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)c1c-2ccc2cc(OC)ccc12>>Oc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)c1c-2ccc2cc(O)ccc12
COC=1C=CC2=C(C=CC=3C4=CC=C(C=C4CN(C23)C2=CC=C(C=C2)OCCN2CCCCC2)OC)C1.C(C)S.[Cl-].[Al+3].[Cl-].[Cl-]>>OC=1C=CC2=C(C=CC=3C4=CC=C(C=C4CN(C23)C2=CC=C(C=C2)OCCN2CCCCC2)O)C1
C[O:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[CH2:8][N:9]([c:10]1[cH:11][cH:12][c:13]([O:14][CH2:15][CH2:16][N:17]3[CH2:18][CH2:19][CH2:20][CH2:21][CH2:22]3)[cH:23][cH:24]1)[c:25]1[c:26]-2[cH:27][cH:28][c:29]2[cH:30][c:31]([O:32]C)[cH:33][cH:34][c:35]12>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[CH2:8][N:9]([c:10]1[c...
COc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)c1c-2ccc2cc(OC)ccc12
Oc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)c1c-2ccc2cc(O)ccc12
null
null
C(Cl)Cl
Deprotection
OtherReaction
a0f05885bbc65ae2846cad0ac34029941211b2ef3a426958b0c8aa83bb16fe86
9df751cd682ad9d54ed75d7313aaead6a019c5d37ede15c4672866d319b900ff
c1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)c1c-2ccc2ccccc12
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4].C-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4].[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]
60.5
[{"value": 60.0, "product": "OC=1C=CC2=C(C=CC=3C4=CC=C(C=C4CN(C23)C2=CC=C(C=C2)OCCN2CCCCC2)O)C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.5, "product": "OC=1C=CC2=C(C=CC=3C4=CC=C(C=C4CN(C23)C2=CC=C(C=C2)OCCN2CCCCC2)O)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A solution of the product of Example 13 (195 mg, 0.39 mmol) in methylene chloride (25 mL) was treated with ethanethiol (200 mg, 220 mL, 3.2 mmol) and aluminum chloride (320 mg, 2.4 mmol). After stirring for 4 h at ambient temperature, the mixture was quenched carefully with THF (25 mL) and saturated sodium bicarbonate ...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Aromatic alcohol.Aromatic alcohol
null
null
c1ccccc1.C1CC[NH]CC1.c1ccc2c(c1)C[NH]c1c3ccccc3ccc12
Other
C(Cl)Cl
null
4
COc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)c1c-2ccc2cc(OC)ccc12>C(Cl)Cl>Oc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)c1c-2ccc2cc(O)ccc12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-5ac5c62883484e62b790bfad4bc5e3bb
COc1ccc2c(c1)SC(=O)C2.O=Cc1ccccc1O>>COc1ccc2c(c1)SC1c3ccccc3OC(=O)C21
COC1=CC2=C(CC(=O)S2)C=C1.C(C=1C(O)=CC=CC1)=O>>COC1=CC2=C(C=C1)C1C(OC3=C(C1S2)C=CC=C3)=O
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[S:9][C:18](=[O:19])[CH2:20]2.O=[CH:10][c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[OH:17]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[S:9][CH:10]1[c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[O:17][C:18](=[O:19])[CH:20]21
COc1ccc2c(c1)SC(=O)C2.O=Cc1ccccc1O
COc1ccc2c(c1)SC1c3ccccc3OC(=O)C21
null
C(C)N(CC)CC
C(C)O.C(Cl)Cl
Acylation
OtherReaction
e8fbc487563db87775f9ef5b53c3692d363b1a0498769b64bd7c794649742d9d
7259bf0e4ba555fe66049920a15c643fe90ace826f32b0be86332a42da8e3e0d
O=C1Oc2ccccc2C2Sc3ccccc3C12
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4](-[OH;D1;+0:5]):[c:6].[O;D1;H0:7]=[C;H0;D3;+0:8]1-[CH2;D2;+0:9]-[c:10](:[c:11]):[c:12](:[c:13])-[S;H0;D2;+0:14]-1>>[O;D1;H0:7]=[C;H0;D3;+0:8]1-[O;H0;D2;+0:5]-[c:4](:[c:6]):[c:2](:[c:3])-[CH;D3;+0:1]2-[S;H0;D2;+0:14]-[c:12](:[c:13]):[c:10](:[c:11])-[CH;D3;+0:9]-1-2
83
[{"value": 83.0, "product": "COC1=CC2=C(C=C1)C1C(OC3=C(C1S2)C=CC=C3)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 82.8, "product": "COC1=CC2=C(C=C1)C1C(OC3=C(C1S2)C=CC=C3)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a stirred solution of 6-methoxythianaphthen-2-one (52.6 g, 290 mmol) in a mixture of ethanol (260 mL) and methylene chloride (130 mL) was added triethylamine (2.0 mL, 14.8 mmol) followed by salicylaldehyde (32 mL, 300 mmol) at room temperature. After 1 h, a solid began to precipitate and stirring was continued for 3...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Aromatic alcohol.Carbo-thioester
Ester.Monosulfide
c1ccc2c(c1)CCS2
c1ccc2c(c1)OCC1c3ccccc3SC21
c1ccc2c(c1)OCC1c3ccccc3SC21
HO-
C(C)N(CC)CC.C(C)O.C(Cl)Cl
null
1
COc1ccc2c(c1)SC(=O)C2.O=Cc1ccccc1O>C(C)N(CC)CC.C(C)O.C(Cl)Cl>COc1ccc2c(c1)SC1c3ccccc3OC(=O)C21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9870787f9e3f4d56b73d33d54187af4f
COc1ccc2c(c1)CCc1c-2n(-c2ccc(OCCN3CCCCC3)cc2)c(=O)c2cc(OC)ccc12>>COc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)C1=C2CCc2cc(OC)ccc21
COC=1C=CC2=C(CCC=3C4=CC=C(C=C4C(N(C23)C2=CC=C(C=C2)OCCN2CCCCC2)=O)OC)C1.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>COC=1C=CC2=C(CCC=3C4=CC=C(C=C4CN(C23)C2=CC=C(C=C2)OCCN2CCCCC2)OC)C1
O=[c:9]1[n:10](-[c:11]2[cH:12][cH:13][c:14]([O:15][CH2:16][CH2:17][N:18]3[CH2:19][CH2:20][CH2:21][CH2:22][CH2:23]3)[cH:24][cH:25]2)[c:27]2[c:26]([c:37]3[c:30]1[cH:31][c:32]([O:33][CH3:34])[cH:35][cH:36]3)[CH2:28][CH2:29][c:7]1[c:6]-2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:8]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8...
COc1ccc2c(c1)CCc1c-2n(-c2ccc(OCCN3CCCCC3)cc2)c(=O)c2cc(OC)ccc12
COc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)C1=C2CCc2cc(OC)ccc21
null
null
C1CCOC1
Reduction
OtherReaction
cb18ab27282d46f4a41097f59a4cd81ab68f1c74c5369f5c346d3507faec4980
b253d4575341720f8cb1bb1880f1e68453d6628d64a267e66737eafe44470ded
c1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)C1=C2CCc2ccccc21
O=[c;H0;D3;+0:1]1:[c;H0;D3;+0:2](:[c:3]:[c:4]):[c:5](:[c:6]):[c;H0;D3;+0:7]2:[c;H0;D3;+0:8](:[n;H0;D3;+0:9]:1-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14])-[c;H0;D3;+0:15]1:[c:16]:[c:17]:[c:18]:[c:19]:[c;H0;D3;+0:20]:1-[CH2;D2;+0:21]-[CH2;D2;+0:22]-2>>[c:12]:[c:11]:[c;H0;D3;+0:10](-[N;H0;D3;+0:9]1-[CH2;D2;+0:1]-[c;H0;...
72.4
[{"value": 64.0, "product": "COC=1C=CC2=C(CCC=3C4=CC=C(C=C4CN(C23)C2=CC=C(C=C2)OCCN2CCCCC2)OC)C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.4, "product": "COC=1C=CC2=C(CCC=3C4=CC=C(C=C4CN(C23)C2=CC=C(C=C2)OCCN2CCCCC2)OC)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of the product of Example 12 (350 mg, 0.69 mmol) in THF (25 mL) was treated with lithium aluminum hydride (129 mg, 3.4 mmol) inducing a moderate exotherm. The mixture was allowed to return to room temperature and stirred for 2 h, then briefly warmed to reflux, cooled, and quenched with ethyl acetate (50 mL) ...
10.6084/m9.figshare.5104873.v1
null
null
Enamine
c1ccc2c(c1)CCc1c3ccccc3cnc12
c1ccc2c(c1)C[NH]C1=C2CCc2ccccc21
c1ccccc1.C1CC[NH]CC1.c1ccc2c(c1)C[NH]C1=C2CCc2ccccc21
Other
C1CCOC1
null
2
COc1ccc2c(c1)CCc1c-2n(-c2ccc(OCCN3CCCCC3)cc2)c(=O)c2cc(OC)ccc12>C1CCOC1>COc1ccc2c(c1)CN(c1ccc(OCCN3CCCCC3)cc1)C1=C2CCc2cc(OC)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8c93a62461734d1c98f9eb63bc7a7f2a
CN(C)C=O.NNCC(=O)N[C@@H](CC(=O)OCc1ccccc1)C(=O)N[C@@H](Cc1ccccc1)C(=O)OCc1ccccc1.On1nnc2ccccc21>>Nc1cccc(CCC(=O)NCC(=O)N[C@@H](CC(=O)O)C(=O)N[C@@H](Cc2ccccc2)C(=O)O)n1
C(CCl)Cl.N(CC(=O)N[C@@H](CC(OCC1=CC=CC=C1)=O)C(=O)N[C@@H](CC1=CC=CC=C1)C(=O)OCC1=CC=CC=C1)N.Cl.C(C)(C)N(CC)C(C)C.CN(C=O)C.C=1C=CC2=C(C1)N=NN2O>>NC1=CC=CC(=N1)CCC(=O)NCC(=O)N[C@@H](CC(O)=O)C(=O)N[C@@H](CC1=CC=CC=C1)C(=O)O
CN(C)[CH:9]=[O:10].c1ccc(C[O:20][C:18]([CH2:17][C@H:16]([NH:15][C:13]([CH2:12][NH:11][NH2:1])=[O:14])[C:21](=[O:22])[NH:23][C@@H:24]([CH2:25][c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[C:32](=[O:33])[O:34]Cc2ccccc2)=[O:19])cc1.O[n:35]1nnc2[c:2]1[cH:3][cH:4][cH:5][cH:6]2>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][c:6]([CH2:7][CH...
CN(C)C=O.NNCC(=O)N[C@@H](CC(=O)OCc1ccccc1)C(=O)N[C@@H](Cc1ccccc1)C(=O)OCc1ccccc1.On1nnc2ccccc21
Nc1cccc(CCC(=O)NCC(=O)N[C@@H](CC(=O)O)C(=O)N[C@@H](Cc2ccccc2)C(=O)O)n1
null
[Pd]
C(C)O
C-C Coupling
OtherReaction
aa57fac1c9d9cb97858634258eb1a7fe21fcb884d41c6750757f83562faf70e2
e666beabd03b26d2855b8e8d5725ec0e57b2ce795c53b22bd9e1f0737e7ba1bc
O=C(CCc1ccccn1)NCC(=O)NCC(=O)NCCc1ccccc1
C-N(-C)-[CH;D2;+0:1]=[O;D1;H0:2].O-[n;H0;D3;+0:3]1:n:n:c2:[cH;D2;+0:4]:[c:5]:[c:6]:[c:7]:[c;H0;D3;+0:8]:1:2.[NH2;D1;+0:9]-[NH;D2;+0:10]-[C:11]-[C:12](=[O;D1;H0:13])-[#7:14]-[C:15](-[C:16]-[C:17](=[O;D1;H0:18])-[O;H0;D2;+0:19]-C-c1:c:c:c:c:c:1)-[C:20](=[O;D1;H0:21])-[#7:22]-[C:23]-[C:24](=[O;D1;H0:25])-[O;H0;D2;+0:26]-C...
10
[{"value": 10.0, "product": "NC1=CC=CC(=N1)CCC(=O)NCC(=O)N[C@@H](CC(O)=O)C(=O)N[C@@H](CC1=CC=CC=C1)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
18
HOUR
3-(2-[6-Aminopyridyl])-propionic acid (63 mg, 0.28 mmol), HOBT (50 mg, 0.37 mmol), HCl.H2N-Gly-Asp(OBn)-Phe-OBn (155 mg, 0.28 mmol) and diisopropylethylamine were combined in 7 ml of dry dimethylformamide. The reaction mixture was cooled to 0° C. EDC (68 mg, 0.35 mmol) was added in one portion, the reaction mixture all...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Ester.Ester.Tertiary amide
Carboxylic acid.Carboxylic acid.Secondary amide.Primary amine
c1ccccc1.c1ccccc1.c1ccc2[nH]nnc2c1
c1ccncc1
c1ccncc1.c1ccccc1
HO-
[Pd].C(C)O
0
18
CN(C)C=O.NNCC(=O)N[C@@H](CC(=O)OCc1ccccc1)C(=O)N[C@@H](Cc1ccccc1)C(=O)OCc1ccccc1.On1nnc2ccccc21>[Pd].C(C)O>Nc1cccc(CCC(=O)NCC(=O)N[C@@H](CC(=O)O)C(=O)N[C@@H](Cc2ccccc2)C(=O)O)n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-37d4e94f18a64572955158f797a738e8
COC(CN=C=S)OC.N>>COC(CNC(N)=S)OC
N.COC(CN=C=S)OC>>COC(CNC(=S)N)OC
[CH3:1][O:2][CH:3]([CH2:4][N:5]=[C:6]=[S:8])[O:9][CH3:10].[NH3:7]>>[CH3:1][O:2][CH:3]([CH2:4][NH:5][C:6]([NH2:7])=[S:8])[O:9][CH3:10]
COC(CN=C=S)OC.N
COC(CNC(N)=S)OC
null
null
CO
Heteroatom Alkylation and Arylation
OtherReaction
9ea44f258f40d07ea72818ac0d167217e6d11d32357aad8e81d4f079b5cbad85
8a79caa9356d3b30a3b61a9504f2b151cec34b3b4ac7afcdd36f0060d08e7701
null
[C:1]-[C:2]-[N;H0;D2;+0:3]=[C;H0;D2;+0:4]=[S;D1;H0:5].[NH3;D0;+0:6]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:4](-[NH2;D1;+0:6])=[S;D1;H0:5]
null
[]
null
null
null
null
Methanol (200 mL) was saturated with ammonia and stirred with isothiocyanatoacetaldehyde dimethyl acetal (5.0 g) for 2 h. The mixture was concentrated and the residue was chromatographed (silica gel, 5% methanol/dichloromethane) to give the title compound. Conditions: See reaction.notes.procedure_details. Workup: The m...
10.6084/m9.figshare.5104873.v1
null
Isothiocyanate
Thiourea
null
null
null
null
CO
null
null
COC(CN=C=S)OC.N>CO>COC(CNC(N)=S)OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-ccae603003f14fca9668b5a8da6d0d4d
CNCC(=O)OCc1ccccc1.O=C1CCC(=O)O1>>CN(CC(=O)OCc1ccccc1)C(=O)CCC(=O)O
C(C1=CC=CC=C1)OC(CNC)=O.C1(CCC(=O)O1)=O>>C(C1=CC=CC=C1)OC(CN(C)C(CCC(=O)O)=O)=O
[CH3:1][NH:2][CH2:3][C:4](=[O:5])[O:6][CH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1.[C:14]1(=[O:15])[CH2:16][CH2:17][C:18](=[O:19])[O:20]1>>[CH3:1][N:2]([CH2:3][C:4](=[O:5])[O:6][CH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)[C:14](=[O:15])[CH2:16][CH2:17][C:18](=[O:19])[OH:20]
CNCC(=O)OCc1ccccc1.O=C1CCC(=O)O1
CN(CC(=O)OCc1ccccc1)C(=O)CCC(=O)O
null
null
C1(=CC=CC=C1)C
Protection
OtherReaction
75be88e6b83c45fccbc410b13860a053f9023d8701f41828baea71b5452e7745
95d83cdac3a1d5509861e8b6462ab8c8218ba78b52ab99766013cb9b1af0d20d
c1ccccc1
[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[C:5]-[NH;D2;+0:6]-[C;D1;H3:7].[O;D1;H0:8]=[C;H0;D3;+0:9]1-[C:10]-[C:11]-[C:12](=[O;D1;H0:13])-[O;H0;D2;+0:14]-1>>[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[C:5]-[N;H0;D3;+0:6](-[C;D1;H3:7])-[C;H0;D3;+0:9](=[O;D1;H0:8])-[C:10]-[C:11]-[C:12](=[O;D1;H0:13])-[OH;D1;+0:14]
86.3
[{"value": 67.5, "product": "C(C1=CC=CC=C1)OC(CN(C)C(CCC(=O)O)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.3, "product": "C(C1=CC=CC=C1)OC(CN(C)C(CCC(=O)O)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of sarcosine benzyl ester (3.0 g, 30.7 mmol) and succinic anhydride (5.5 g, 30.7 mmol) in toluene (75 mL) was heated to reflux for 3 h, cooled, filtered, and the filtrate was concentrated. The residue was taken up in 5% aqueous sodium carbonate and extracted with ethyl acetate. The aqueous phase was adjusted ...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Secondary amine
Carboxylic acid.Tertiary amide
C1CCOC1
null
c1ccccc1
null
C1(=CC=CC=C1)C
null
null
CNCC(=O)OCc1ccccc1.O=C1CCC(=O)O1>C1(=CC=CC=C1)C>CN(CC(=O)OCc1ccccc1)C(=O)CCC(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-bcef87ed7a7043ef86ee001ff10769ae
CC(C)(C)OC(=O)NCC(=O)O.N[C@@H](CC(=O)OC1CCCCC1)C(=O)O>>CC(C)(C)OC(=O)NCC(=O)N[C@@H](CC(=O)OC1CCCCC1)C(=O)O
N(CC(=O)O)C(=O)OC(C)(C)C.C(C)N=C=NCCCN(C)C.N[C@@H](CC(OC1CCCCC1)=O)C(=O)O.OC1[C@@H](O)[C@@H](O)[C@H](OCC2=CC=C(C)C=C2)[C@H](O1)CO.CN(C)C=O.ON1N=NC2=C1C=CC=C2>>N(CC(=O)N[C@@H](CC(OC1CCCCC1)=O)C(=O)O)C(=O)OC(C)(C)C.OC1[C@@H](O)[C@@H](O)[C@H](OCC2=CC=C(C)C=C2)[C@H](O1)CO
O[C:10]([CH2:9][NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])=[O:11].[NH2:12][C@@H:13]([CH2:14][C:15](=[O:16])[O:17][CH:18]1[CH2:19][CH2:20][CH2:21][CH2:22][CH2:23]1)[C:24](=[O:25])[OH:26]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][CH2:9][C:10](=[O:11])[NH:12][C@@H:13]([CH2:14][C:15](=[O:16])[O:17...
CC(C)(C)OC(=O)NCC(=O)O.N[C@@H](CC(=O)OC1CCCCC1)C(=O)O
CC(C)(C)OC(=O)NCC(=O)N[C@@H](CC(=O)OC1CCCCC1)C(=O)O
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
C1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4]-[C:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11].[#8:12]-[C:13](=[O;D1;H0:14])-[C:15]-[C:16](-[NH2;D1;+0:17])-[C:18](=[O;D1;H0:19])-[O;D1;H1:20]>>[#8:12]-[C:13](=[O;D1;H0:14])-[C:15]-[C:16](-[NH;D2;+0:17]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4]-[C:...
89.2
[{"value": 89.2, "product": "N(CC(=O)N[C@@H](CC(OC1CCCCC1)=O)C(=O)O)C(=O)OC(C)(C)C.OC1[C@@H](O)[C@@H](O)[C@H](OCC2=CC=C(C)C=C2)[C@H](O1)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a cold solution of Asp(O-cHex)-Man(4-MBzl) (46.7 g, 86.4 mmol) in DMF (100 mL) diisopropylethylamine (15 mL, 86.1 mmol) was added. N-Hydroxybezotriazole (14.0 g, 104 mmol) was added followed by Boc-Gly (16.6 g, 94.8 mmol). The reaction mixture was stirred in the cold for a few minutes, and N-ethyl-N'(dimethylaminopr...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CCCCC1
HO-
null
null
null
CC(C)(C)OC(=O)NCC(=O)O.N[C@@H](CC(=O)OC1CCCCC1)C(=O)O>>CC(C)(C)OC(=O)NCC(=O)N[C@@H](CC(=O)OC1CCCCC1)C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-49f6270560624c5e98c775fdae86e129
Nc1ccc(-c2ccc(N)c(N)c2)cc1N.O=C(O)/C=C/C=C/C(=O)O>>C#C.C#C.c1ccc2[nH]cnc2c1.c1ccc2[nH]cnc2c1
NC=1C=C(C=CC1N)C1=CC(=C(N)C=C1)N.C(\C=C\C=C\C(=O)O)(=O)O>>C#C.C#C.N1=CNC2=C1C=CC=C2.N2=CNC1=C2C=CC=C1
[c:5]1(-[c:14]2[cH:15][cH:16][c:17]([NH2:18])[c:21]([NH2:20])[cH:22]2)[cH:6][cH:7][c:8]([NH2:9])[c:12]([NH2:11])[cH:13]1.O=[C:10](O)/[CH:4]=[CH:2]/[CH:1]=[CH:3]/[C:19](=O)O>>[CH:1]#[CH:2].[CH:3]#[CH:4].[cH:5]1[cH:6][cH:7][c:8]2[nH:9][cH:10][n:11][c:12]2[cH:13]1.[cH:14]1[cH:15][cH:16][c:17]2[nH:18][cH:19][n:20][c:21]2[c...
Nc1ccc(-c2ccc(N)c(N)c2)cc1N.O=C(O)/C=C/C=C/C(=O)O
C#C.C#C.c1ccc2[nH]cnc2c1.c1ccc2[nH]cnc2c1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
64aee3e13525c08a2cbef9993db4cf018b917c6ee7971e6ae287c4630fdee485
ad0a0f5871c13b069ca26b80b625bdedff486cbebfe95426d60993b066e77137
c1ccc2[nH]cnc2c1.c1ccc2[nH]cnc2c1
O-[C;H0;D3;+0:1](=O)/[CH;D2;+0:2]=[CH;D2;+0:3]/[CH;D2;+0:4]=[CH;D2;+0:5]/[C;H0;D3;+0:6](-O)=O.[NH2;D1;+0:7]-[c:8]1:[c:9]:[c;H0;D3;+0:10](-[c;H0;D3;+0:11]2:[c:12]:[c:13]:[c:14](-[NH2;D1;+0:15]):[c:16](-[NH2;D1;+0:17]):[c:18]:2):[c:19]:[c:20]:[c:21]:1-[NH2;D1;+0:22]>>[CH;D1;+0:4]#[CH;D1;+0:3].[CH;D1;+0:5]#[CH;D1;+0:2].[c...
null
[]
null
null
null
null
3,3'-Diaminobenzidine (1.508 g, 7.04 mmol) was dehydrochlorinated with 83.3 wt % deaerated PPA in accordance with the procedure enumerated in Example 1. The product of this dehydrochlorination was reacted with trans,trans-muconic acid (1.0 g, 7.04 mmol) in accordance with the procedure of Example 1. This polymerization...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid.Primary amine.Primary amine.Primary amine.Primary amine.Conjugated diene
Alkyne.Alkyne
c1ccccc1.c1ccccc1
c1ccc2[nH]cnc2c1.c1ccc2[nH]cnc2c1
c1ccc2[nH]cnc2c1.c1ccc2[nH]cnc2c1
HO-
null
null
null
Nc1ccc(-c2ccc(N)c(N)c2)cc1N.O=C(O)/C=C/C=C/C(=O)O>>C#C.C#C.c1ccc2[nH]cnc2c1.c1ccc2[nH]cnc2c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b158250efe4c40eebdb1b21930a1a3f4
CCO.CCOC(=O)OCC.Cc1ccccc1.Cc1ccccc1.O>>O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
C(C)O.C1(=CC=CC=C1)C.C(OCC)(OCC)=O.[H-].[Na+].C1(=CC=CC=C1)C.O>>C(C1=CC=CC=C1)OC1=CC=C2C(=CC(OC2=C1)=O)O
C[CH2:11][OH:10].CCO[C:2](=[O:1])[O:20]C[CH3:3].[CH3:4][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1.C[c:9]1[cH:8][cH:7][cH:6][cH:19][cH:18]1.[OH2:5]>>[O:1]=[c:2]1[cH:3][c:4]([OH:5])[c:6]2[cH:7][cH:8][c:9]([O:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][cH:17]3)[cH:18][c:19]2[o:20]1
CCO.CCOC(=O)OCC.Cc1ccccc1.Cc1ccccc1.O
O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
be35ef74b40b7d957ec8047d8dc673b1caff4483920f29c19cc5b15deebfce29
dbd17518751cc08c5e0fc4e9f0128fc615bc09bcdbd2410dc38bce2febf6d1b1
O=c1ccc2ccc(OCc3ccccc3)cc2o1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:3]-C-[CH3;D1;+0:4].C-[CH2;D2;+0:5]-[OH;D1;+0:6].C-[c;H0;D3;+0:7]1:[c:8]:[cH;D2;+0:9]:[cH;D2;+0:10]:[c:11]:[c:12]:1.[CH3;D1;+0:13]-[c;H0;D3;+0:14](:[c:15]:[c:16]):[c:17]:[c:18].[OH2;D0;+0:19]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[cH;D2;+0:4]:[c;H0;D3;+0:13](-[OH;D1;+0:19]):[c;H0;D3...
84
[{"value": 84.0, "product": "C(C1=CC=CC=C1)OC1=CC=C2C(=CC(OC2=C1)=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
4-Benzyloxy-2-hydroxy-acetophenone (20 g, 0.0825 mol), prepared in accordance with Example 4, was dissolved in 150 mL of toluene. To this solution was added diethyl carbonate (25.3 g, 0.21 mol) and the entire contents taken in a beaker was heated while stirring to dissolve the starting material. This solution was then ...
10.6084/m9.figshare.5104873.v1
null
Carbonic Ester.Primary alcohol
Ether.Aromatic alcohol
c1ccccc1.c1ccccc1
c1ccc2cccoc2c1.c1ccccc1
c1ccc2cccoc2c1.c1ccccc1
HO-
null
null
null
CCO.CCOC(=O)OCC.Cc1ccccc1.Cc1ccccc1.O>>O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-fc45e6d9775a4f599ceedc6dcd5fe8bc
O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1>>O=c1cc(O)c2ccc(O)cc2o1
C(C1=CC=CC=C1)OC1=CC=C2C(=CC(OC2=C1)=O)O>>OC1=CC(OC2=CC(=CC=C12)O)=O
c1ccc(C[O:10][c:9]2[cH:8][cH:7][c:6]3[c:4]([OH:5])[cH:3][c:2](=[O:1])[o:13][c:12]3[cH:11]2)cc1>>[O:1]=[c:2]1[cH:3][c:4]([OH:5])[c:6]2[cH:7][cH:8][c:9]([OH:10])[cH:11][c:12]2[o:13]1
O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
O=c1cc(O)c2ccc(O)cc2o1
null
[Pd]
CO
Deprotection
Hydroxyl benzyl deprotection
36869d1fe85185a14d9eb30bf05178c600a9b6eca277ffaf3803578c30e0bf5d
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=c1ccc2ccccc2o1
[#8;a:1]:[c:2]:[c:3]:[c:4](-[O;H0;D2;+0:5]-C-c1:c:c:c:c:c:1):[c:6]>>[#8;a:1]:[c:2]:[c:3]:[c:4](-[OH;D1;+0:5]):[c:6]
90
[{"value": 90.0, "product": "OC1=CC(OC2=CC(=CC=C12)O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A 300 cc autoclave was charged with 7-benzyloxy-4-hydroxycoumarin (3 g, 3.7 mmol), prepared in accordance with Example 5, 5% Pd on carbon (0.18 g) and 85 mL of methanol and the autoclave was purged with N2. The autoclave was pressurized with H2 to a pressure of about 100 psi and maintained at that pressure. The exother...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
c1ccccc1
null
c1ccc2cccoc2c1
Other
[Pd].CO
null
null
O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1>[Pd].CO>O=c1cc(O)c2ccc(O)cc2o1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-eafe799634bf413884245083d524cea5
Cc1ccc(S(=O)(=O)N=[N+]=[N-])cc1.O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1>>[N-]=[N+]=C1C(=O)Oc2cc(OCc3ccccc3)ccc2C1=O
C1(=CC=C(C=C1)S(=O)(=O)N=[N+]=[N-])C.C(C1=CC=CC=C1)OC1=CC=C2C(=CC(OC2=C1)=O)O.C(C)N(CC)CC>>[N+](=[N-])=C1C(OC2=CC(=CC=C2C1=O)OCC1=CC=CC=C1)=O
Cc1ccc(S(=O)(=O)[N:1]=[N+:2]=[N-])cc1.[cH:3]1[c:4](=[O:5])[o:6][c:7]2[cH:8][c:9]([O:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][cH:17]3)[cH:18][cH:19][c:20]2[c:21]1[OH:22]>>[N-:1]=[N+:2]=[C:3]1[C:4](=[O:5])[O:6][c:7]2[cH:8][c:9]([O:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][cH:17]3)[cH:18][cH:19][c:20]2[C:21]1=[...
Cc1ccc(S(=O)(=O)N=[N+]=[N-])cc1.O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
[N-]=[N+]=C1C(=O)Oc2cc(OCc3ccccc3)ccc2C1=O
null
null
C1CCOC1
Acylation
OtherReaction
a588281ee0712866d01012f4c8cf674cc1e86d876933bcbee61aed4605b28980
16c5bfe4e75246e5d41e0c1283cd592a9e824171ae59abf49dae1b6957964ef9
[N+]=C1C(=O)Oc2cc(OCc3ccccc3)ccc2C1=O
C-c1:c:c:c(-S(=O)(=O)-[N;H0;D2;+0:1]=[N+;H0;D2:2]=[N-]):c:c:1.[O;D1;H0:3]=[c;H0;D3;+0:4]1:[cH;D2;+0:5]:[c;H0;D3;+0:6](-[OH;D1;+0:7]):[c:8](:[c:9]):[c:10](:[c:11]):[o;H0;D2;+0:12]:1>>[N-;H0;D1:1]=[N+;H0;D2:2]=[C;H0;D3;+0:5]1-[C;H0;D3;+0:6](=[O;H0;D1;+0:7])-[c:8](:[c:9]):[c:10](:[c:11])-[O;H0;D2;+0:12]-[C;H0;D3;+0:4]-1=[...
90
[{"value": 90.0, "product": "[N+](=[N-])=C1C(OC2=CC(=CC=C2C1=O)OCC1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A solution of 7-benzyloxy -4-hydroxy coumarin (2.5 g, 9.3 mmol; prepared in accordance with Example 5) in anhydrous THF (40 mL) was mixed with triethylamine (0.9 g, 9 mmol) taken in a 100 mL 3-neck round-bottom flask under an atmosphere of N2. A solution of p-toluenesulfonyl azide (2.8 g, 14 mmol) in dry THF (20 mL) wa...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Azide.Aromatic alcohol
Ketone.Ester.Diazo
c1ccccc1.c1ccc2cccoc2c1
c1ccc2c(c1)CCCO2
c1ccc2c(c1)CCCO2.c1ccccc1
TsOH.HO-
C1CCOC1
null
3
Cc1ccc(S(=O)(=O)N=[N+]=[N-])cc1.O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1>C1CCOC1>[N-]=[N+]=C1C(=O)Oc2cc(OCc3ccccc3)ccc2C1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d813d0f041e246f1a6849017f99fae8a
CCO.CCOC(=O)OCC.Cc1ccccc1.Cc1ccccc1.O>>O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
C(C)O.C1(=CC=CC=C1)C.C(OCC)(OCC)=O.[H-].[Na+].C1(=CC=CC=C1)C.O>>C(C1=CC=CC=C1)OC1=CC=C2C(=CC(OC2=C1)=O)O
C[CH2:11][OH:10].CCO[C:2](=[O:1])[O:20]C[CH3:3].[CH3:4][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1.C[c:9]1[cH:8][cH:7][cH:6][cH:19][cH:18]1.[OH2:5]>>[O:1]=[c:2]1[cH:3][c:4]([OH:5])[c:6]2[cH:7][cH:8][c:9]([O:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][cH:17]3)[cH:18][c:19]2[o:20]1
CCO.CCOC(=O)OCC.Cc1ccccc1.Cc1ccccc1.O
O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
be35ef74b40b7d957ec8047d8dc673b1caff4483920f29c19cc5b15deebfce29
dbd17518751cc08c5e0fc4e9f0128fc615bc09bcdbd2410dc38bce2febf6d1b1
O=c1ccc2ccc(OCc3ccccc3)cc2o1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:3]-C-[CH3;D1;+0:4].C-[CH2;D2;+0:5]-[OH;D1;+0:6].C-[c;H0;D3;+0:7]1:[c:8]:[cH;D2;+0:9]:[cH;D2;+0:10]:[c:11]:[c:12]:1.[CH3;D1;+0:13]-[c;H0;D3;+0:14](:[c:15]:[c:16]):[c:17]:[c:18].[OH2;D0;+0:19]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[cH;D2;+0:4]:[c;H0;D3;+0:13](-[OH;D1;+0:19]):[c;H0;D3...
84
[{"value": 84.0, "product": "C(C1=CC=CC=C1)OC1=CC=C2C(=CC(OC2=C1)=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
4-Benzyloxy-2-hydroxy-acetophenone (20 g, 0.0825 mol), prepared in accordance with Example 4, was dissolved in 150 mL of toluene. To this solution was added diethyl carbonate (25.3 g, 0.21 mol) and the entire contents taken in a beaker was heated while stirring to dissolve the starting material. This solution was then ...
10.6084/m9.figshare.5104873.v1
null
Carbonic Ester.Primary alcohol
Ether.Aromatic alcohol
c1ccccc1.c1ccccc1
c1ccc2cccoc2c1.c1ccccc1
c1ccc2cccoc2c1.c1ccccc1
HO-
null
null
null
CCO.CCOC(=O)OCC.Cc1ccccc1.Cc1ccccc1.O>>O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0732293e181346eba1ff8d891ce02cf4
O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1>>O=c1cc(O)c2ccc(O)cc2o1
C(C1=CC=CC=C1)OC1=CC=C2C(=CC(OC2=C1)=O)O>>OC1=CC(OC2=CC(=CC=C12)O)=O
c1ccc(C[O:10][c:9]2[cH:8][cH:7][c:6]3[c:4]([OH:5])[cH:3][c:2](=[O:1])[o:13][c:12]3[cH:11]2)cc1>>[O:1]=[c:2]1[cH:3][c:4]([OH:5])[c:6]2[cH:7][cH:8][c:9]([OH:10])[cH:11][c:12]2[o:13]1
O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
O=c1cc(O)c2ccc(O)cc2o1
null
[Pd]
CO
Deprotection
Hydroxyl benzyl deprotection
36869d1fe85185a14d9eb30bf05178c600a9b6eca277ffaf3803578c30e0bf5d
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=c1ccc2ccccc2o1
[#8;a:1]:[c:2]:[c:3]:[c:4](-[O;H0;D2;+0:5]-C-c1:c:c:c:c:c:1):[c:6]>>[#8;a:1]:[c:2]:[c:3]:[c:4](-[OH;D1;+0:5]):[c:6]
90
[{"value": 90.0, "product": "OC1=CC(OC2=CC(=CC=C12)O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A 300 cc autoclave was charged with 7-benzyloxy-4-hydroxycoumarin (3 g, 3.7 mmol), prepared in accordance with Example 5, 5% Pd on carbon (0.18 g) and 85 mL of methanol and the autoclave was purged with N2. The autoclave was pressurized with H2 to a pressure of about 100 psi and maintained at that pressure. The exother...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
c1ccccc1
null
c1ccc2cccoc2c1
Other
[Pd].CO
null
null
O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1>[Pd].CO>O=c1cc(O)c2ccc(O)cc2o1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2be13a8581c44d4eb5c7cef82a7c8e6c
Cc1ccc(S(=O)(=O)N=[N+]=[N-])cc1.O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1>>[N-]=[N+]=C1C(=O)Oc2cc(OCc3ccccc3)ccc2C1=O
C1(=CC=C(C=C1)S(=O)(=O)N=[N+]=[N-])C.C(C1=CC=CC=C1)OC1=CC=C2C(=CC(OC2=C1)=O)O.C(C)N(CC)CC>>[N+](=[N-])=C1C(OC2=CC(=CC=C2C1=O)OCC1=CC=CC=C1)=O
Cc1ccc(S(=O)(=O)[N:1]=[N+:2]=[N-])cc1.[cH:3]1[c:4](=[O:5])[o:6][c:7]2[cH:8][c:9]([O:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][cH:17]3)[cH:18][cH:19][c:20]2[c:21]1[OH:22]>>[N-:1]=[N+:2]=[C:3]1[C:4](=[O:5])[O:6][c:7]2[cH:8][c:9]([O:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][cH:17]3)[cH:18][cH:19][c:20]2[C:21]1=[...
Cc1ccc(S(=O)(=O)N=[N+]=[N-])cc1.O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1
[N-]=[N+]=C1C(=O)Oc2cc(OCc3ccccc3)ccc2C1=O
null
null
C1CCOC1
Acylation
OtherReaction
a588281ee0712866d01012f4c8cf674cc1e86d876933bcbee61aed4605b28980
16c5bfe4e75246e5d41e0c1283cd592a9e824171ae59abf49dae1b6957964ef9
[N+]=C1C(=O)Oc2cc(OCc3ccccc3)ccc2C1=O
C-c1:c:c:c(-S(=O)(=O)-[N;H0;D2;+0:1]=[N+;H0;D2:2]=[N-]):c:c:1.[O;D1;H0:3]=[c;H0;D3;+0:4]1:[cH;D2;+0:5]:[c;H0;D3;+0:6](-[OH;D1;+0:7]):[c:8](:[c:9]):[c:10](:[c:11]):[o;H0;D2;+0:12]:1>>[N-;H0;D1:1]=[N+;H0;D2:2]=[C;H0;D3;+0:5]1-[C;H0;D3;+0:6](=[O;H0;D1;+0:7])-[c:8](:[c:9]):[c:10](:[c:11])-[O;H0;D2;+0:12]-[C;H0;D3;+0:4]-1=[...
90
[{"value": 90.0, "product": "[N+](=[N-])=C1C(OC2=CC(=CC=C2C1=O)OCC1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A solution of7-benzyloxy-4-hydroxy coumarin (2.5 g, 9.3 mmol; prepared in accordance with Example 5) in anhydrous THF (40 mL) was mixed with triethylamine (0.9 g, 9 mmol) taken in a 100 mL 3-neck round-bottom flask under an atmosphere of N2. A solution of p-toluenesulfonyl azide (2.8 g, 14 mmol) in dry THF (20 mL) was ...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Azide.Aromatic alcohol
Ketone.Ester.Diazo
c1ccccc1.c1ccc2cccoc2c1
c1ccc2c(c1)CCCO2
c1ccc2c(c1)CCCO2.c1ccccc1
TsOH.HO-
C1CCOC1
null
3
Cc1ccc(S(=O)(=O)N=[N+]=[N-])cc1.O=c1cc(O)c2ccc(OCc3ccccc3)cc2o1>C1CCOC1>[N-]=[N+]=C1C(=O)Oc2cc(OCc3ccccc3)ccc2C1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-61e90dfc436e46c68b3d763ba8118cbb
CC(=O)OC(C)=O.Nc1ccn([C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)n1>>CC(=O)Nc1ccn([C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)n1
[C@@H]1(C[C@H](O)[C@@H](CO)O1)N1C(=O)N=C(N)C=C1.C(C)(=O)OC(C)=O>>C(C)(=O)NC1=NC(N([C@H]2C[C@H](O)[C@@H](CO)O2)C=C1)=O
CC(=O)O[C:2]([CH3:1])=[O:3].[NH2:4][c:5]1[cH:6][cH:7][n:8]([C@H:9]2[CH2:10][C@H:11]([OH:12])[C@@H:13]([CH2:14][OH:15])[O:16]2)[c:17](=[O:18])[n:19]1>>[CH3:1][C:2](=[O:3])[NH:4][c:5]1[cH:6][cH:7][n:8]([C@H:9]2[CH2:10][C@H:11]([OH:12])[C@@H:13]([CH2:14][OH:15])[O:16]2)[c:17](=[O:18])[n:19]1
CC(=O)OC(C)=O.Nc1ccn([C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)n1
CC(=O)Nc1ccn([C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)n1
null
null
CN(C=O)C
Acylation
Aminolysis of esters
87d35e51b477fc9a658a6f307eb56d84c8879182772c9dd3a42ec0d584fd2684
627cbc0550c9f51ad0105d9fcf46677e8c93bed87ee95bfe69292a82550c95b7
O=c1ncccn1[C@H]1CCCO1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[NH2;D1;+0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:[c:10]:1>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[NH;D2;+0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:[c:10]:1
98.2
[{"value": 98.0, "product": "C(C)(=O)NC1=NC(N([C@H]2C[C@H](O)[C@@H](CO)O2)C=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.2, "product": "C(C)(=O)NC1=NC(N([C@H]2C[C@H](O)[C@@H](CO)O2)C=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
HOUR
To 61.29 g (270 mmol) of the material of Example I dissolved in 1300 ml of anhydrous N,N-dimethylformamide ("DMF") (Aldrich; Cat. No. 22, 70506), was added 28 ml (296 mmol) of acetic anhydride (Aldrich; Cat. No. 11,004-3), and the resulting mixture was stirred at room temperature for 20 hrs. DMF was removed under reduc...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary amine
Secondary amide
null
null
c1cncnc1.C1CCOC1
HO-
CN(C=O)C
null
20
CC(=O)OC(C)=O.Nc1ccn([C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)n1>CN(C=O)C>CC(=O)Nc1ccn([C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3780dab8e7fc4abdb18faae656691afb
OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO>>OC[C@H]1O[C@@H](O[C@@H]2[C@@H](CO)O[C@](O)(CO)[C@H]2O)[C@H](O)[C@@H](O)[C@H]1O
C([C@@H]1[C@@H]([C@@H]([C@H]([C@@H](O1)O[C@H]([C@@H](CO)O)[C@@H]([C@H](CO)O)O)O)O)O)O.O.C([C@@H]1[C@@H]([C@@H]([C@H]([C@@H](O1)O[C@H]([C@@H](CO)O)[C@@H]([C@H](CO)O)O)O)O)O)O.O.O>>C([C@@H]1[C@@H]([C@@H]([C@H]([C@@H](O1)O[C@@H]2[C@H](O[C@@]([C@H]2O)(CO)O)CO)O)O)O)O
[OH:1][CH2:2][C@H:3]1[O:4][C@@H:5]([O:6][C@H:7]([C@@H:8]([CH2:9][OH:10])[OH:11])[C@@H:16]([C@@H:12]([OH:13])[CH2:14][OH:15])[OH:17])[C@H:18]([OH:19])[C@@H:20]([OH:21])[C@H:22]1[OH:23]>>[OH:1][CH2:2][C@H:3]1[O:4][C@@H:5]([O:6][C@@H:7]2[C@@H:8]([CH2:9][OH:10])[O:11][C@:12]([OH:13])([CH2:14][OH:15])[C@H:16]2[OH:17])[C@H:1...
OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO
OC[C@H]1O[C@@H](O[C@@H]2[C@@H](CO)O[C@](O)(CO)[C@H]2O)[C@H](O)[C@@H](O)[C@H]1O
null
null
null
Oxidation
OtherReaction
278cf296da9870749f18ed71f2bfd7f7f5f66e19da4bee88ccbf5f43b75dda7b
5da3fb1ebb4c17ae961f305629feaf8cfc0c08c33829d24f3e8bbd94478beb9a
C1CC[C@H](O[C@H]2CCOC2)OC1
[C:1]-[C:2](-[OH;D1;+0:3])-[C:4]-[C:5](-[O;D1;H1:6])-[C@@H;D3;+0:7](-[O;D1;H1:8])-[C:9]-[O;D1;H1:10]>>[C:1]-[C:2]1-[C:4]-[C:5](-[O;D1;H1:6])-[C@@;H0;D4;+0:7](-[O;D1;H1:8])(-[C:9]-[O;D1;H1:10])-[O;H0;D2;+0:3]-1
null
[]
null
null
null
null
Examples XII-XXVII elucidate the conditions at which lactitol monohydrate and lactitol dihydrate, respectively, may be obtained from aqueous solutions of lactitol. In each instance 200 g lactitol dihydrate was used as the starting material which wasd dissolved in an amount of water varying from 40 g to 50 g at 100° C. ...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol.Secondary alcohol
Ether
null
C1CCOC1
C1CCOCC1.C1CCOC1
null
null
null
null
OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO>>OC[C@H]1O[C@@H](O[C@@H]2[C@@H](CO)O[C@](O)(CO)[C@H]2O)[C@H](O)[C@@H](O)[C@H]1O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-19ef8b5233de4220a1842b9d3ce2334f
OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO>>OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO
C([C@@H]1[C@@H]([C@@H]([C@H]([C@@H](O1)O[C@@H]2[C@H](O[C@@]([C@H]2O)(CO)O)CO)O)O)O)O.C([C@@H]1[C@@H]([C@@H]([C@H]([C@@H](O1)O[C@@H]2[C@H](O[C@@]([C@H]2O)(CO)O)CO)O)O)O)O.C([C@@H]1[C@@H]([C@@H]([C@H]([C@@H](O1)O[C@H]([C@@H](CO)O)[C@@H]([C@H](CO)O)O)O)O)O)O.O.O>>C([C@@H]1[C@@H]([C@@H]([C@H]([C@@H](O1)O[C@H]([C@@H](CO)O)[...
[OH:2][CH2:3][C@@H:4]([OH:5])[C@@H:6]([O:7][C@@H:8]1[O:9][C@H:10]([CH2:11][OH:12])[C@H:13]([OH:14])[C@H:15]([OH:16])[C@H:17]1[OH:18])[C@H:19]([OH:20])[C@@H:21]([OH:22])[CH2:23][OH:24]>>[OH:2][CH2:3][C@@H:4]([OH:5])[C@@H:6]([O:7][C@@H:8]1[O:9][C@H:10]([CH2:11][OH:12])[C@H:13]([OH:14])[C@H:15]([OH:16])[C@H:17]1[OH:18])[C...
OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO
OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO
null
null
O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
C1CCOCC1
null
4.9
[{"value": 4.9, "product": "C([C@@H]1[C@@H]([C@@H]([C@H]([C@@H](O1)O[C@H]([C@@H](CO)O)[C@@H]([C@H](CO)O)O)O)O)O)O.O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
950 g lactitol dihydrate (860 g anhydric lactitol) were dissolved in 125 g water at 100° C. Upon cooling to 50° C. the 80 percent by weight lactitol solution was seeded with 9.5 g ground dihydrate (1 percent by weight based on the lactitol dissolves). After crystallization for 48 hours at 45° C. the crystals formed wer...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
C1CCOCC1
null
O
null
null
OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO>O>OC[C@@H](O)[C@@H](O[C@@H]1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O)[C@H](O)[C@@H](O)CO
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3d49ae6f297d47999ae3e523cd23084d
Cc1cccc(C)c1.Clc1nc(Cl)nc(Cl)n1>>Cc1ccc(-c2nc(Cl)nc(-c3ccc(C)cc3C)n2)c(C)c1
N1=C(Cl)N=C(Cl)N=C1Cl.C1(=CC(=CC=C1)C)C>>ClC1=NC(=NC(=N1)C1=C(C=C(C=C1)C)C)C1=C(C=C(C=C1)C)C
[CH3:1][c:2]1[cH:3][cH:4][cH:23][c:18]([CH3:16])[cH:17]1.Cl[c:5]1[n:7][c:15]([Cl:9])[n:20][c:22](Cl)[n:10]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[n:7][c:8]([Cl:9])[n:10][c:11](-[c:12]3[cH:13][cH:14][c:15]([CH3:16])[cH:17][c:18]3[CH3:19])[n:20]2)[c:21]([CH3:22])[cH:23]1
Cc1cccc(C)c1.Clc1nc(Cl)nc(Cl)n1
Cc1ccc(-c2nc(Cl)nc(-c3ccc(C)cc3C)n2)c(C)c1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
d95917990c8fa34e930db780b5436b0e53bbf37db4f64a5de5e7ed86f3153274
61b0a5599977a22af270e7bf51ae98dbf8841255d4777bc8dbf1a0b3a43dd3ed
c1ccc(-c2ncnc(-c3ccccc3)n2)cc1
Cl-[c;H0;D3;+0:1]1:[n;H0;D2;+0:2]:[c;H0;D3;+0:3](-Cl):[n;H0;D2;+0:4]:[c;H0;D3;+0:5](-[Cl;H0;D1;+0:6]):[n;H0;D2;+0:7]:1.[C;D1;H3:8]-[c;H0;D3;+0:9]1:[c:10]:[cH;D2;+0:11]:[cH;D2;+0:12]:[c;H0;D3;+0:13](-[CH3;D1;+0:14]):[cH;D2;+0:15]:1>>[C;D1;H3:16]-[c;H0;D3;+0:13]1:[cH;D2;+0:15]:[c;H0;D3;+0:5](-[CH3;D1;+0:14]):[c:17]:[c:18...
null
[]
null
null
null
null
The reaction of cyanuric chloride with 1,3-xylene under Friedel-Crafts conditions to give 2-chloro-4,6-bis(2,4-dimethylphenyl)-s-triazine is known, e.g. from DE-A-1 169 947 and Helv. Chim. Acta 55, 1589 (1972). However, the product can also be obtained using an appropriate Grignard reagent, such as described in Helv. C...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Aromatic halide
Aromatic halide
c1ccccc1.c1ncncn1
c1ccccc1.c1ncncn1.c1ccccc1
c1ccccc1.c1ncncn1.c1ccccc1
null
null
null
null
Cc1cccc(C)c1.Clc1nc(Cl)nc(Cl)n1>>Cc1ccc(-c2nc(Cl)nc(-c3ccc(C)cc3C)n2)c(C)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a23a2974ba3941e79b71f0f690cd1e1b
O=C(O)c1ccc(I)cc1>>COC(=O)c1ccc(I)cc1
[N+](=[N-])=C.IC1=CC=C(C(=O)O)C=C1.CCOCC>>COC(C1=CC=C(C=C1)I)=O
[OH:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([I:9])[cH:10][cH:11]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([I:9])[cH:10][cH:11]1
O=C(O)c1ccc(I)cc1
COC(=O)c1ccc(I)cc1
null
null
O1CCCC1
Miscellaneous
Protection of carboxylic acid
56520e0abb4535dce9a663824ca803b71c2c0dd72dfd246317d953596a987bd2
2ccc7a30191c2c171b49e8a0217bee87430687dd0f567141eca025a75b7e3136
c1ccccc1
[O;D1;H0:1]=[C:2](-[OH;D1;+0:3])-[c:4]>>[C;D1;H3:5]-[O;H0;D2;+0:3]-[C:2](=[O;D1;H0:1])-[c:4]
99.3
[{"value": 99.3, "product": "COC(C1=CC=C(C=C1)I)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Fifty (50) mmol (12.4 g) of commercially available 4-iodobenzoic acid was dissolved in 200 ml of tetrahydrofuran and then added to an ether solution containing freshly prepared diazomethane. The excess diazomethane was subsequently consumed by addition of glacial acetic acid and the resultant solution was concentrated ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ester
null
null
c1ccccc1
Other
O1CCCC1
null
null
O=C(O)c1ccc(I)cc1>O1CCCC1>COC(=O)c1ccc(I)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6c41a6072d6542949567036d24ed5e23
C#CCO.COC(=O)c1ccc(I)cc1>>COC(=O)c1ccc(C#CCO)cc1
IC1=CC=C(C(=O)OC)C=C1.C(C#C)O>>OCC#CC1=CC=C(C(=O)OC)C=C1
[CH:9]#[C:10][CH2:11][OH:12].I[c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:14][cH:13]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9]#[C:10][CH2:11][OH:12])[cH:13][cH:14]1
C#CCO.COC(=O)c1ccc(I)cc1
COC(=O)c1ccc(C#CCO)cc1
null
[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
C(C)NCC
C-C Coupling
Sonogashira alkyne_aryl halide
15c08902746c61a960c314898ce6bb5fcc5e189f9e057388c59dba9ec9d0c81c
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
c1ccccc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[C:7]#[CH;D1;+0:8]>>[C:6]-[C:7]#[C;H0;D2;+0:8]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
83.1
[{"value": 83.0, "product": "OCC#CC1=CC=C(C(=O)OC)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.1, "product": "OCC#CC1=CC=C(C(=O)OC)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Methyl 4-iodobenzoate (9.0 g, 34.4 mmol) was dissolved in 90 ml of diethylamine. The solution was stirred vigorously and, sequentially, 121 milligrams of bis(triphenylphosphine) palladium chloride and 65 milligrams of cuprous iodide were added, each in a single portion, followed by 1.93 grams of propargyl alcohol. The ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1ccccc1
c1ccccc1
c1ccccc1
HI
[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(C)NCC
null
null
C#CCO.COC(=O)c1ccc(I)cc1>[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(C)NCC>COC(=O)c1ccc(C#CCO)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d7d51544825c4bb7a548bd1885f197b6
O=C(CC(C(=O)O)C(=O)O)c1ccsc1>>O=C(O)CCCc1ccsc1
[Na+].[Cl-].O.NN.[OH-].[K+].O=C(CC(C(=O)O)C(=O)O)C1=CSC=C1.Cl>>S1C=C(C=C1)CCCC(=O)O
O=C(O)[CH:4]([C:2](=[O:1])[OH:3])[CH2:5][C:6](=O)[c:7]1[cH:8][cH:9][s:10][cH:11]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][CH2:6][c:7]1[cH:8][cH:9][s:10][cH:11]1
O=C(CC(C(=O)O)C(=O)O)c1ccsc1
O=C(O)CCCc1ccsc1
null
null
C(CO)O
Reduction
OtherReaction
5b8f0395946b243f5d5c516ddfd2c7b17767fe5a6bd4d01b8d36e05474913824
a54c4ff227377b63a7e5600277363bb31869ae720888ac22a37508be1aa77a21
c1ccsc1
O-C(=O)-[CH;D3;+0:1](-[C:2]-[C;H0;D3;+0:3](=O)-[c:4]1:[c:5]:[#16;a:6]:[c:7]:[c:8]:1)-[C:9](=[O;D1;H0:10])-[O;D1;H1:11]>>[O;D1;H0:10]=[C:9](-[O;D1;H1:11])-[CH2;D2;+0:1]-[C:2]-[CH2;D2;+0:3]-[c:4]1:[c:5]:[#16;a:6]:[c:7]:[c:8]:1
87.6
[{"value": 87.6, "product": "S1C=C(C=C1)CCCC(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Hydrazine hydrate (1.3 mL, 1.34 g, 26.8 mmol) was added dropwise to a solution of KOH (3.54 g, 63 mmol) and 2-[2-oxo-2-(3-thienyl) ethyl]malonic acid 8(c) (4.00 g, 17.5 mmol) in ethylene glycol (30 mL). This solution was heated at reflux for 6 hours. After cooling to room temperature, the crude reaction mixture was pou...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ketone
null
null
null
c1ccsc1
Other
C(CO)O
null
null
O=C(CC(C(=O)O)C(=O)O)c1ccsc1>C(CO)O>O=C(O)CCCc1ccsc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-377a459ff6984e289cfcd5758d18e946
NO.O=C1CCCc2ccccc21>>ON=C1CCCc2ccccc21
C1(CCCC2=CC=CC=C12)=O.O.C(C)(=O)[O-].[Na+].Cl.NO>>C1(CCCC2=CC=CC=C12)=NO
[OH:1][NH2:2].O=[C:3]1[CH2:4][CH2:5][CH2:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]21>>[OH:1][N:2]=[C:3]1[CH2:4][CH2:5][CH2:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]21
NO.O=C1CCCc2ccccc21
ON=C1CCCc2ccccc21
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
98df1d319842c80da69615da3a5ce7c9aa877051ff6e5b7391db85d01092ee6d
1a0ef15294bdb221fb8888b5d4c7fcf00473b11e53da288791d32747daa48d23
N=C1CCCc2ccccc21
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[O;D1;H1:8]>>[C:3]-[C:2]-[C;H0;D3;+0:1](=[N;H0;D2;+0:7]-[O;D1;H1:8])-[c:4](:[c:5]):[c:6]
95
[{"value": 95.0, "product": "C1(CCCC2=CC=CC=C12)=NO", "details": "PERCENTYIELD", "is_desired": false}]
75
CELSIUS
15
MINUTE
To 4.6 L of water at room temperature in a 4-neck 50 L flask sitting in a steam bath apparatus equipped with an overhead stirrer, a temperature probe and reflux condenser was added 3.72 Kg (27.36 mol) of sodium acetate with stirring, followed by 1.9 Kg of hydroxylamine hydrochloride (27.36 mol). To this slurry at room ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Oxime
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
HO-
C(C)O
75
0.25
NO.O=C1CCCc2ccccc21>C(C)O>ON=C1CCCc2ccccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-bcec0cf5870e4b4b8e57365233ab30d8
ON=C1CCCc2ccccc21>>O=C1CCCc2ccccc2N1
C1(CCCC2=CC=CC=C12)=NO.CS(=O)(=O)O.O=P12OP3(=O)OP(=O)(O1)OP(=O)(O2)O3.[OH-].[Na+].CS(=O)(=O)O>>N1C(CCCC2=C1C=CC=C2)=O
[OH:1][N:12]=[C:2]1[CH2:3][CH2:4][CH2:5][c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]21>>[O:1]=[C:2]1[CH2:3][CH2:4][CH2:5][c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[NH:12]1
ON=C1CCCc2ccccc21
O=C1CCCc2ccccc2N1
null
null
null
Miscellaneous
OtherReaction
3063b294f7182a0341159c5a5ab6dd2b1163127b2f088d9184b9c29e8afcfd24
810ed199c446b7a720678de08fbd331169d64180af03f0e0c66326af0c16570f
O=C1CCCc2ccccc2N1
[OH;D1;+0:1]-[N;H0;D2;+0:2]=[C;H0;D3;+0:3]1-[C:4]-[C:5]-[C:6]-[c:7](:[c:8]):[c;H0;D3;+0:9]-1:[c:10]:[c:11]>>[O;H0;D1;+0:1]=[C;H0;D3;+0:3]1-[C:4]-[C:5]-[C:6]-[c:7](:[c:8]):[c;H0;D3;+0:9](:[c:10]:[c:11])-[NH;D2;+0:2]-1
95
[{"value": 95.0, "product": "N1C(CCCC2=C1C=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}]
90
CELSIUS
3
HOUR
To 10 L of methanesulfonic acid in a 22 L 3-neck flask equipped with an overhead stirrer, a temperature probe, nitrogen inlet and reflux condenser was added 2.6 Kg (18.61 mol) of phosphorus pentoxide. An additional 1.6 L of methanesulfonic acid was used to wash all the phosphorus pentoxide into the vessel. The mixture ...
10.6084/m9.figshare.5104873.v1
null
Oxime
Secondary amide
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCCN2
c1ccc2c(c1)CCCCN2
null
null
90
3
ON=C1CCCc2ccccc21>>O=C1CCCc2ccccc2N1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6d7bcd1e14f74813ae3d55bd0a8bbec4
II.O=C1CCCc2ccccc2N1>>O=C1Nc2ccccc2CCC1I
N1C(CCCC2=C1C=CC=C2)=O.S(=O)([O-])[O-].[Na+].[Na+].S(=O)([O-])[O-].[Na+].[Na+].C[Si](N[Si](C)(C)C)(C)C.II>>IC1C(NC2=C(CC1)C=CC=C2)=O
I[I:13].[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH2:10][CH2:11][CH2:12]1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH2:10][CH2:11][CH:12]1[I:13]
II.O=C1CCCc2ccccc2N1
O=C1Nc2ccccc2CCC1I
null
null
C(Cl)Cl.O
Functional Group Interconversion
OtherReaction
73a4b8101accc5821bcd407bb00b0d5a1b99828e455f6ca75099f6d3708d4163
0c353a1260488c22c3ffb72de5623420c3ec35470a0b3a2045b11c29224f458e
O=C1CCCc2ccccc2N1
I-[I;H0;D1;+0:1].[C:2]-[C:3]-[CH2;D2;+0:4]-[C:5](=[O;D1;H0:6])-[#7:7]-[c:8]>>[C:2]-[C:3]-[CH;D3;+0:4](-[I;H0;D1;+0:1])-[C:5](=[O;D1;H0:6])-[#7:7]-[c:8]
57.5
[{"value": 57.0, "product": "IC1C(NC2=C(CC1)C=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.5, "product": "IC1C(NC2=C(CC1)C=CC=C2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
30
CELSIUS
null
null
A suspension of 1.8 Kg (11.17 mol) of 2,3,4,5-tetrahydro-1H-1-benzazepin-2-one in a mixture of 22.33 L of methylene chloride and 11.78 L (55.83 mol) of hexamethyldisilazane was heated at reflux for 10 minutes then cooled to 30° C. and treated with 8.503 Kg (33.5 mol) of iodine in one portion. The mixture was heated at ...
10.6084/m9.figshare.5104873.v1
null
null
Secondary halide
c1ccc2c(c1)CCCCN2
c1ccc2c(c1)CCCCN2
c1ccc2c(c1)CCCCN2
HI
C(Cl)Cl.O
30
null
II.O=C1CCCc2ccccc2N1>C(Cl)Cl.O>O=C1Nc2ccccc2CCC1I
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c735dcd09dc84541aa910c31a66677ea
CC(C)(C)OC(=O)N1C(=O)CC1(C)C.[OH-]>>CC(C)(CC(=O)O)NC(=O)OC(C)(C)C
C(C)(C)(C)OC(=O)N1C(CC1(C)C)=O.[OH-].[Li+]>>C(C)(C)(C)OC(=O)NC(CC(=O)O)(C)C
[CH3:1][C:2]1([CH3:3])[CH2:4][C:5](=[O:6])[N:8]1[C:9](=[O:10])[O:11][C:12]([CH3:13])([CH3:14])[CH3:15].[OH-:7]>>[CH3:1][C:2]([CH3:3])([CH2:4][C:5](=[O:6])[OH:7])[NH:8][C:9](=[O:10])[O:11][C:12]([CH3:13])([CH3:14])[CH3:15]
CC(C)(C)OC(=O)N1C(=O)CC1(C)C.[OH-]
CC(C)(CC(=O)O)NC(=O)OC(C)(C)C
null
null
CCOCC.O.O1CCCC1
Protection
OtherReaction
699e354eb5730d20a794b83d5cd440f6d8fa1c94b8fdaa5e255e70e482a7e50d
d205f1320160ea6fd9f0bda4863ee5979f7ad336699029216ee1832d3dc0743f
null
[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C:6](=[O;D1;H0:7])-[N;H0;D3;+0:8]1-[C;H0;D3;+0:9](=[O;D1;H0:10])-[C:11]-[C:12]-1(-[C;D1;H3:13])-[C;D1;H3:14].[OH-;D0:15]>>[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C:6](=[O;D1;H0:7])-[NH;D2;+0:8]-[C:12](-[C;D1;H3:13])(-[C;D1;H3:14])-[C:11]-[C;H0;D3;+0:9]...
87
[{"value": 87.0, "product": "C(C)(C)(C)OC(=O)NC(CC(=O)O)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A 3 L, 3-neck round bottom flask equipped with a magnetic stirrer, thermometer, nitrogen bubbler and addition funnel was charged with 180.3 g (0.89 mol) of N-(t-butoxycarbonyl)-4,4-dimethylazetidin-2-one dissolved in 1 L of tetrahydrofuran. The solution was cooled to 0°-5° C. and treated dropwise with 890 mL of 1.0M aq...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Substituted dicarboximide
Carbamic ester.Carboxylic acid
C1C[NH]C1
null
null
null
CCOCC.O.O1CCCC1
null
2
CC(C)(C)OC(=O)N1C(=O)CC1(C)C.[OH-]>CCOCC.O.O1CCCC1>CC(C)(CC(=O)O)NC(=O)OC(C)(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-48cc48b39ac845098b60f3e2837e0e56
CC(C)(CC(=O)O)NC(=O)OC(C)(C)C.N[C@@H]1CCc2ccccc2NC1=O>>CC(C)(CC(=O)N[C@@H]1CCc2ccccc2NC1=O)NC(=O)OC(C)(C)C
F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.N[C@H]1C(NC2=C(CC1)C=CC=C2)=O.C(C)(C)(C)OC(=O)NC(CC(=O)O)(C)C.C(C)N(CC)CC>>C(C)(C)(C)OC(=O)NC(CC(=O)N[C@H]1C(NC2=C(CC1)C=CC=C2)=O)(C)C
O[C:5]([CH2:4][C:2]([CH3:1])([CH3:3])[NH:20][C:21](=[O:22])[O:23][C:24]([CH3:25])([CH3:26])[CH3:27])=[O:6].[NH2:7][C@@H:8]1[CH2:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]2[NH:17][C:18]1=[O:19]>>[CH3:1][C:2]([CH3:3])([CH2:4][C:5](=[O:6])[NH:7][C@@H:8]1[CH2:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]2[NH...
CC(C)(CC(=O)O)NC(=O)OC(C)(C)C.N[C@@H]1CCc2ccccc2NC1=O
CC(C)(CC(=O)N[C@@H]1CCc2ccccc2NC1=O)NC(=O)OC(C)(C)C
null
null
C(Cl)Cl.C(C)(=O)OCC
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C1CCCc2ccccc2N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8](=[O;D1;H0:9])-[#7:10]-[c:11]>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[C:6](-[C:5])-[C:8](=[O;D1;H0:9])-[#7:10]-[c:11]
94
[{"value": 94.0, "product": "C(C)(C)(C)OC(=O)NC(CC(=O)N[C@H]1C(NC2=C(CC1)C=CC=C2)=O)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.9, "product": "C(C)(C)(C)OC(=O)NC(CC(=O)N[C@H]1C(NC2=C(CC1)C=CC=C2)=O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of 8.70 g (49.4 mmol) of 3(R)-amino-2,3,4,5-tetrahydro-1H-1-benzazepin-2-one (Step E) in 100 mL of methylene chloride was treated with 10.73 g (49.4 mmol) of 3-t-butoxycarbonylamino-3-methylbutanoic acid (Step H) and 13.8 mL of triethylamine (10.0 g, 99 mmol, 2 eq.). The reaction flask was immersed in an amb...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2c(c1)CCCCN2
HO-
C(Cl)Cl.C(C)(=O)OCC
null
2
CC(C)(CC(=O)O)NC(=O)OC(C)(C)C.N[C@@H]1CCc2ccccc2NC1=O>C(Cl)Cl.C(C)(=O)OCC>CC(C)(CC(=O)N[C@@H]1CCc2ccccc2NC1=O)NC(=O)OC(C)(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-ead516c1b5b84915b6f58d3f44f1f181
C=O.Cc1ccc(O)cc1>>Cc1ccc(O)c(C=O)c1
C1(=CC=CC=C1)C.C=O.C[Mg]Cl.C1=CC(=CC=C1O)C>>OC1=C(C=O)C=C(C=C1)C
[CH2:8]=[O:9].[CH3:1][c:2]1[cH:3][cH:4][c:5]([OH:6])[cH:7][cH:10]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([OH:6])[c:7]([CH:8]=[O:9])[cH:10]1
C=O.Cc1ccc(O)cc1
Cc1ccc(O)c(C=O)c1
null
CN1C(N(CCC1)C)=O
O1CCCC1
C-C Coupling
OtherReaction
6bafee88871e7df55b2a6a706a8a62d4f54a2873abef1ac73ed67da72b977665
0102b88d9700d39435e06971744797a0ad3df95b36c61ce095d6702bc41b05ed
c1ccccc1
[CH2;D1;+0:1]=[O;D1;H0:2].[O;D1;H1:3]-[c:4](:[c:5]):[cH;D2;+0:6]:[c:7]:[c:8]>>[O;D1;H0:2]=[CH;D2;+0:1]-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:4](-[O;D1;H1:3]):[c:5]
18
[{"value": 18.0, "product": "OC1=C(C=O)C=C(C=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 18.0, "product": "OC1=C(C=O)C=C(C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Methylmagnesium chloride solution in tetrahydrofuran (100 mL, 3.0M, 300 mmol) at room temperature was treated dropwise over 30 minutes with a solution of 32.3 g (300 mmol) of p-cresol in 30 mL of tetrahydrofuran. An additional 70 mL of tetrahydrofuran was added to moderate the exothermic reaction. The mixture was aged ...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde
Aldehyde
c1ccccc1
c1ccccc1
c1ccccc1
null
CN1C(N(CCC1)C)=O.O1CCCC1
null
2
C=O.Cc1ccc(O)cc1>CN1C(N(CCC1)C)=O.O1CCCC1>Cc1ccc(O)c(C=O)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6c59e00fa9b34294a8339d168dc3dcaa
Cc1ccc(O)c(C=O)c1.N#Cc1ccccc1CBr>>Cc1ccc2oc(-c3ccccc3C#N)cc2c1
C[O-].[Na+].BrCC=1C(=CC=CC1)C#N.OC1=C(C=O)C=C(C=C1)C.C[O-].[Na+].C(C)O>>C(#N)C1=C(C=CC=C1)C=1OC2=C(C1)C=C(C=C2)C
O=[CH:16][c:17]1[c:5]([OH:6])[cH:4][cH:3][c:2]([CH3:1])[cH:18]1.Br[CH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][c:13]1[C:14]#[N:15]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]2[o:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3[C:14]#[N:15])[cH:16][c:17]2[cH:18]1
Cc1ccc(O)c(C=O)c1.N#Cc1ccccc1CBr
Cc1ccc2oc(-c3ccccc3C#N)cc2c1
null
null
CN(C=O)C.O
Aromatic Heterocycle Formation
OtherReaction
ae0d8af73753cd90bad163caf180a20dbba0089f4ad123713353f52ec702d104
92cc8b0a92f96eb9b03a03a2ee19d09e7e6c24351b1bf5fbd10085af3332d8a0
c1ccc(-c2cc3ccccc3o2)cc1
Br-[CH2;D2;+0:1]-[c;H0;D3;+0:2](:[c:3]:[c:4]):[c:5](-[C:6]#[N;D1;H0:7]):[c:8].O=[CH;D2;+0:9]-[c:10](:[c:11]):[c:12](-[OH;D1;+0:13]):[c:14]>>[N;D1;H0:7]#[C:6]-[c:5](:[c:8]):[c;H0;D3;+0:2](-[c;H0;D3;+0:1]1:[cH;D2;+0:9]:[c:10](:[c:11]):[c:12](:[c:14]):[o;H0;D2;+0:13]:1):[c:3]:[c:4]
63.3
[{"value": 63.0, "product": "C(#N)C1=C(C=CC=C1)C=1OC2=C(C1)C=C(C=C2)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.3, "product": "C(#N)C1=C(C=CC=C1)C=1OC2=C(C1)C=C(C=C2)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
75
CELSIUS
20
MINUTE
A 500 mL 3-neck round bottom flask equipped with a magnetic stirrer, dropping funnel, thermometer and nitrogen bubbler was charged with 10.7 g (108 mmol) of sodium methoxide and 75 mL of absolute ethanol. A solution of 24.9 g (183 mmol) of 2-hydroxy-5-methylbenzaldehyde in 75 mL of dry dimethylformamide was added dropw...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aldehyde.Aromatic alcohol
null
c1ccccc1
c1ccc2occc2c1
c1ccc2occc2c1.c1ccccc1
HBr
CN(C=O)C.O
75
0.333333
Cc1ccc(O)c(C=O)c1.N#Cc1ccccc1CBr>CN(C=O)C.O>Cc1ccc2oc(-c3ccccc3C#N)cc2c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a70c972de63c48c88aee846896f01c2b
Cc1ccc2oc(-c3ccccc3C#N)cc2c1.[CH3][Sn]([CH3])([CH3])[N]=[N+]=[N-]>>Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)cc2c1
C[Sn](C)(C)N=[N+]=[N-].C[Sn](C)(C)N=[N+]=[N-].C(#N)C1=C(C=CC=C1)C=1OC2=C(C1)C=C(C=C2)C.C[Sn](C)(C)N=[N+]=[N-]>>N1N=NN=C1C1=C(C=CC=C1)C=1OC2=C(C1)C=C(C=C2)C
[CH3:1][c:2]1[cH:3][cH:4][c:5]2[o:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3[C:14]#[N:15])[cH:19][c:20]2[cH:21]1.[CH3][Sn]([CH3])([CH3])[N:18]=[N+:17]=[N-:16]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]2[o:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3-[c:14]3[n:15][n:16][n:17][nH:18]3)[cH:19][c:20]2[cH:21]1
Cc1ccc2oc(-c3ccccc3C#N)cc2c1.[CH3][Sn]([CH3])([CH3])[N]=[N+]=[N-]
Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)cc2c1
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
d793d4dee9d5a39dbd122d04a35a5f691674657d5f6e422ae31ce158ea438a57
95e338ac8e3158e8ab88ebe03ba7338cec0c32ed80de2cb9f73834a6f54aede3
c1ccc(-c2cc3ccccc3o2)c(-c2nnn[nH]2)c1
[#8;a:1]:[c:2]-[c:3](:[c:4]):[c;H0;D3;+0:5](-[C;H0;D2;+0:6]#[N;H0;D1;+0:7]):[c:8]:[c:9].[CH3]-[Sn](-[CH3])(-[CH3])-[N;H0;D2;+0:10]=[N+;H0;D2:11]=[N-;H0;D1:12]>>[#8;a:1]:[c:2]-[c:3](:[c:4]):[c;H0;D3;+0:5](-[c;H0;D3;+0:6]1:[n;H0;D2;+0:7]:[n;H0;D2;+0:12]:[n;H0;D2;+0:11]:[nH;D2;+0:10]:1):[c:8]:[c:9]
57.3
[{"value": 57.0, "product": "N1N=NN=C1C1=C(C=CC=C1)C=1OC2=C(C1)C=C(C=C2)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.3, "product": "N1N=NN=C1C1=C(C=CC=C1)C=1OC2=C(C1)C=C(C=C2)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
A 500 mL 3-neck round bottom flask equipped with a magnetic stirrer, condenser, thermometer and nitrogen bubbler was charged with 19.1 g (82 mmol) of 2-(2-cyanophenyl)-5-methylbenzofuran, 200 mL of toluene and 25.6 g (124 mmol) of trimethyltin azide. The suspension was heated at reflux for 20 hours, then an additional ...
10.6084/m9.figshare.5104873.v1
null
Azide.Nitrile.Tin
null
null
c1nnn[nH]1
c1ccc2occc2c1.c1ccccc1.c1nnn[nH]1
Sn
C1(=CC=CC=C1)C
null
24
Cc1ccc2oc(-c3ccccc3C#N)cc2c1.[CH3][Sn]([CH3])([CH3])[N]=[N+]=[N-]>C1(=CC=CC=C1)C>Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)cc2c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c9728215e0934ce58de5aa5e0e1a5863
BrBr.Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)cc2c1>>Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)c(Br)c2c1
C1=CCCCC1.BrBr.N1N=NN=C1C1=C(C=CC=C1)C=1OC2=C(C1)C=C(C=C2)C.O1CCOCC1>>BrC1=C(OC2=C1C=C(C=C2)C)C2=C(C=CC=C2)C2=NN=NN2
Br[Br:20].[CH3:1][c:2]1[cH:3][cH:4][c:5]2[o:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3-[c:14]3[n:15][n:16][n:17][nH:18]3)[cH:19][c:21]2[cH:22]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]2[o:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3-[c:14]3[n:15][n:16][n:17][nH:18]3)[c:19]([Br:20])[c:21]2[cH:22]1
BrBr.Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)cc2c1
Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)c(Br)c2c1
null
null
C(Cl)(Cl)(Cl)Cl
Functional Group Interconversion
Bromination
aef34a534a5357a8d8d24e91d8c0597ba5461b904c5f6750301da171e41c6efd
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc(-c2cc3ccccc3o2)c(-c2nnn[nH]2)c1
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]1:[cH;D2;+0:4]:[c:5](-[c:6]):[#8;a:7]:[c:8]:1:[c:9]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4]1:[c:3](:[c:2]):[c:8](:[c:9]):[#8;a:7]:[c:5]:1-[c:6]
85
[{"value": 85.0, "product": "BrC1=C(OC2=C1C=C(C=C2)C)C2=C(C=CC=C2)C2=NN=NN2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.6, "product": "BrC1=C(OC2=C1C=C(C=C2)C)C2=C(C=CC=C2)C2=NN=NN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A 1 L 3-neck round bottom flask equipped with a magnetic stirrer, thermometer, dropping funnel and nitrogen bubbler was charged with 12.97 g (46.9 mmol) of 2-[2-(1H-tetrazol-5-yl)phenyl]-5-methylbenzofuran and 500 mL of 1,4-dioxane. To the well-stirred solution at room temperature was added a solution of 4.8 mL (93.2 m...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2occc2c1
c1ccc2occc2c1
c1ccc2occc2c1.c1ccccc1.c1nnn[nH]1
HBr
C(Cl)(Cl)(Cl)Cl
null
null
BrBr.Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)cc2c1>C(Cl)(Cl)(Cl)Cl>Cc1ccc2oc(-c3ccccc3-c3nnn[nH]3)c(Br)c2c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-29db157c047e49c9aec1fa6bbd5e3bdc
O=C(O)CNC(=O)c1nc2cc(Cl)c(OCC(F)(F)F)cc2cc1O>>Cl.O=C(O)CNC(=O)c1nc2ccc(OCC(F)(F)F)cc2cc1O
ClC1=C(C=C2C=C(C(=NC2=C1)C(=O)NCC(=O)O)O)OCC(F)(F)F>>Cl.OC=1C(=NC2=CC=C(C=C2C1)OCC(F)(F)F)C(=O)NCC(=O)O
[Cl:1][c:13]1[cH:12][c:11]2[n:10][c:9]([C:7]([NH:6][CH2:5][C:3](=[O:2])[OH:4])=[O:8])[c:24]([OH:25])[cH:23][c:22]2[cH:21][c:14]1[O:15][CH2:16][C:17]([F:18])([F:19])[F:20]>>[ClH:1].[O:2]=[C:3]([OH:4])[CH2:5][NH:6][C:7](=[O:8])[c:9]1[n:10][c:11]2[cH:12][cH:13][c:14]([O:15][CH2:16][C:17]([F:18])([F:19])[F:20])[cH:21][c:22...
O=C(O)CNC(=O)c1nc2cc(Cl)c(OCC(F)(F)F)cc2cc1O
Cl.O=C(O)CNC(=O)c1nc2ccc(OCC(F)(F)F)cc2cc1O
null
null
C(=O)O
Reduction
Aromatic dehalogenation
eb8f97868eda2cc61388d201749d19c211b03c524acdc08748ef282eeabfb54b
32dd8b99ef466a65369cb3d0423332250d968cb6028b4894311fd2c39ad8dfd2
c1ccc2ncccc2c1
[#7:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#7;a:5]:[c:6]1:[c:7]:[c;H0;D3;+0:8](-[Cl;H0;D1;+0:9]):[c:10](-[#8:11]):[c:12]:[c:13]:1>>[#7:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#7;a:5]:[c:6]1:[c:7]:[cH;D2;+0:8]:[c:10](-[#8:11]):[c:12]:[c:13]:1.[ClH;D0;+0:9]
null
[]
null
null
null
null
0.5 g (1.3 mmol) of N-((7-chloro-3-hydroxy-6-(2,2,2-trifluoroethyloxy)quinolin-2-yl)carbonyl)glycine (title compound from Example 31) was dissolved in 26 ml of methanolic formic acid (4.4% strength), and a further 26 ml of methanolic formic acid were added at 20° C. After addition of 0.5 g of Pd/C (10%), the mixture wa...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
null
C(=O)O
null
null
O=C(O)CNC(=O)c1nc2cc(Cl)c(OCC(F)(F)F)cc2cc1O>C(=O)O>Cl.O=C(O)CNC(=O)c1nc2ccc(OCC(F)(F)F)cc2cc1O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a19347c988eb4c1c9861adc66fd17858
O=C(O)c1cccc(OC(F)(F)F)c1.O=[N+]([O-])O>>O=C(O)c1cc(OC(F)(F)F)ccc1[N+](=O)[O-]
[N+](=O)(O)[O-].S(O)(O)(=O)=O.FC(OC=1C=C(C(=O)O)C=CC1)(F)F>>[N+](=O)([O-])C1=C(C(=O)O)C=C(C=C1)OC(F)(F)F
[O:1]=[C:2]([OH:3])[c:4]1[cH:5][c:6]([O:7][C:8]([F:9])([F:10])[F:11])[cH:12][cH:13][cH:14]1.O[N+:15](=[O:16])[O-:17]>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][c:6]([O:7][C:8]([F:9])([F:10])[F:11])[cH:12][cH:13][c:14]1[N+:15](=[O:16])[O-:17]
O=C(O)c1cccc(OC(F)(F)F)c1.O=[N+]([O-])O
O=C(O)c1cc(OC(F)(F)F)ccc1[N+](=O)[O-]
null
null
null
Functional Group Addition
Aromatic nitration with HNO3
53848b8b2bb4e867226e49db2e60519b24be9379900e3ad7c56af54fe8fde7a5
ddce49825c02b8965f10c8d99e3c841d26e1f136da6037b417c09313e6d73097
c1ccccc1
O-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3].[O;D1;H0:4]=[C:5](-[O;D1;H1:6])-[c:7](:[c:8]):[cH;D2;+0:9]:[c:10]:[c:11]>>[O;-;D1;H0:2]-[N+;H0;D3:1](=[O;D1;H0:3])-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:7](-[C:5](=[O;D1;H0:4])-[O;D1;H1:6]):[c:8]
null
[]
null
null
null
null
29.7 ml of nitric acid were added dropwise to 76.5 ml of concentrated sulfuric acid, while cooling and stirring, and 9.0 g (43.7 mmol) of 3-trifluoromethoxybenzoic acid were then added. The reaction mixture was heated at 50°-55° C. for 1 hour and, after cooling, was poured onto ice, and the residue was filtered off wit...
10.6084/m9.figshare.5104873.v1
null
Nitrate
Nitro group
c1ccccc1
c1ccccc1
c1ccccc1
HO-
null
null
null
O=C(O)c1cccc(OC(F)(F)F)c1.O=[N+]([O-])O>>O=C(O)c1cc(OC(F)(F)F)ccc1[N+](=O)[O-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-61857a4aa4ad49af8aac9e9223a18f71
CC(C)I.O=[N+]([O-])c1ccc(O)cc1CO>>CC(C)Oc1ccc([N+](=O)[O-])c(CO)c1
OC=1C=CC(=C(CO)C1)[N+](=O)[O-].C(C)(C)I>>[N+](=O)([O-])C1=C(CO)C=C(C=C1)OC(C)C
I[CH:2]([CH3:1])[CH3:3].[OH:4][c:5]1[cH:6][cH:7][c:8]([N+:9](=[O:10])[O-:11])[c:12]([CH2:13][OH:14])[cH:15]1>>[CH3:1][CH:2]([CH3:3])[O:4][c:5]1[cH:6][cH:7][c:8]([N+:9](=[O:10])[O-:11])[c:12]([CH2:13][OH:14])[cH:15]1
CC(C)I.O=[N+]([O-])c1ccc(O)cc1CO
CC(C)Oc1ccc([N+](=O)[O-])c(CO)c1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
bff4876be49b448135c783dd3eeeb68ab3cc5bdc91beadda8a9095106cd5c747
cf768afb66ed5041aefdce1fa6d1e40995a1ab7c4b4a4ca47544fe49ee1e629f
c1ccccc1
I-[CH;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3].[OH;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C;D1;H3:2]-[CH;D3;+0:1](-[C;D1;H3:3])-[O;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]
null
[]
null
null
null
null
10 g (60 mmol) of 5-hydroxy-2-nitrobenzyl alcohol were reacted with 7.0 ml (70 mmol) of isopropyl iodide analogously to Example 4a); after purification over silica gel with n-heptane/ethyl acetate (3:2), 10.3 g of oily crude product. Conditions: See reaction.notes.procedure_details. Workup: after purification over sili...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HI
null
null
null
CC(C)I.O=[N+]([O-])c1ccc(O)cc1CO>>CC(C)Oc1ccc([N+](=O)[O-])c(CO)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-dd95acbc02174382a8fb617b567ae3bb
CCCCCCC.NCC(=O)OCc1ccccc1.O=C(O)c1ccc2ccccc2n1>>CC(C)Oc1ccc2nc(C(=O)O)c(OCc3ccccc3)cc2c1
CCCCCCC.C(C)(=O)OCC.N1=C(C=CC2=CC=CC=C12)C(=O)O.S(=O)(=O)(O)C1=CC=C(C)C=C1.C(C1=CC=CC=C1)OC(CN)=O.C=1C=CC2=C(C1)N=NN2O>>C(C1=CC=CC=C1)OC=1C(=NC2=CC=C(C=C2C1)OC(C)C)C(=O)O
CCCC[CH2:3][CH2:2][CH3:1].NC[C:14](=[O:4])[O:15][CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1.c1[c:10]([C:11](=[O:12])[OH:13])[n:9][c:8]2[cH:7][cH:6][cH:5][cH:25][c:24]2[cH:23]1>>[CH3:1][CH:2]([CH3:3])[O:4][c:5]1[cH:6][cH:7][c:8]2[n:9][c:10]([C:11](=[O:12])[OH:13])[c:14]([O:15][CH2:16][c:17]3[cH:18][cH:19][cH:20]...
CCCCCCC.NCC(=O)OCc1ccccc1.O=C(O)c1ccc2ccccc2n1
CC(C)Oc1ccc2nc(C(=O)O)c(OCc3ccccc3)cc2c1
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
2b199ec13aedb354aa0e3cdfe102b222aae079ed256cd671f480c20ceec4f336
5769fcad2252788e49992e3c2acac5e3ae32b3811010bcf6e71d6b058fc9a9df
c1ccc(COc2cnc3ccccc3c2)cc1
C-C-C-C-[CH2;D2;+0:1]-[CH2;D2;+0:2]-[C;D1;H3:3].N-C-[C;H0;D3;+0:4](=[O;H0;D1;+0:5])-[#8:6]-[C:7].[O;D1;H0:8]=[C:9](-[O;D1;H1:10])-[c;H0;D3;+0:11]1:[#7;a:12]:[c:13]2:[c:14]:[c:15]:[cH;D2;+0:16]:[c:17]:[c:18]:2:[cH;D2;+0:19]:c:1>>[C:7]-[#8:6]-[c;H0;D3;+0:4]1:[cH;D2;+0:19]:[c:18]2:[c:17]:[c;H0;D3;+0:16](-[O;H0;D2;+0:5]-[C...
129.7
[{"value": 129.7, "product": "C(C1=CC=CC=C1)OC=1C(=NC2=CC=C(C=C2C1)OC(C)C)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2.7 g (8 mmol) of the above quinolinecarboxylic acid were reacted with 2.7 g (8 mmol) of glycine benzyl ester tosylate, 4.4 ml (32 mmol) of NEM, 1.35 g (10 mmol) of HOBT and 3.6 g (8.8 mmol) of CMC in 300 ml of anhydrous methylene chloride at 20° C. for 24 hours, analogously to Example 25g). After working up and chroma...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Ether.Ether
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1.c1ccccc1
Other
C(Cl)Cl
null
null
CCCCCCC.NCC(=O)OCc1ccccc1.O=C(O)c1ccc2ccccc2n1>C(Cl)Cl>CC(C)Oc1ccc2nc(C(=O)O)c(OCc3ccccc3)cc2c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7ccd2207c11e4dc982df4da8ca022082
Cc1cc(F)ccc1[N+](=O)[O-].Oc1ccccc1>>Cc1cc(Oc2ccccc2)ccc1[N+](=O)[O-]
C1(=CC=CC=C1)O.C([O-])([O-])=O.[K+].[K+].FC=1C=CC(=C(C1)C)[N+](=O)[O-]>>[N+](=O)([O-])C1=C(C=C(C=C1)OC1=CC=CC=C1)C
F[c:4]1[cH:3][c:2]([CH3:1])[c:14]([N+:15](=[O:16])[O-:17])[cH:13][cH:12]1.[OH:5][c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1>>[CH3:1][c:2]1[cH:3][c:4]([O:5][c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[cH:12][cH:13][c:14]1[N+:15](=[O:16])[O-:17]
Cc1cc(F)ccc1[N+](=O)[O-].Oc1ccccc1
Cc1cc(Oc2ccccc2)ccc1[N+](=O)[O-]
null
null
CN(C(C)=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
e4ea1e38252bc3b9c5ec04486386725e6570ab3860d45e337a1d131319bbf0fc
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccccc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:8]:[c:7](-[O;H0;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]
null
[]
20
CELSIUS
null
null
14.1 g (150 mmol) of phenol were dissolved in 120 ml of anhydrous N,N-dimethylacetamide, while stirring, 20.6 g (150 mmol) of finely powdered potassium carbonate were added and the mixture was stirred at 70°-80° C. for 30 minutes. After cooling to 20° C., 23.25 g (18.3 ml, 150 mmol) of 5-fluoro-2-nitrotoluene were adde...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HF
CN(C(C)=O)C
20
null
Cc1cc(F)ccc1[N+](=O)[O-].Oc1ccccc1>CN(C(C)=O)C>Cc1cc(Oc2ccccc2)ccc1[N+](=O)[O-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9998629522e842d089f0d1c3f6b90263
Cc1ccc(Cl)c(Cl)c1.O=[N+]([O-])O>>Cc1cc(Cl)c(Cl)cc1[N+](=O)[O-]
ClC=1C=C(C=CC1Cl)C.S(O)(O)(=O)=O.[N+](=O)(O)[O-]>>ClC1=CC(=C(C=C1Cl)C)[N+](=O)[O-]
[CH3:1][c:2]1[cH:3][c:4]([Cl:5])[c:6]([Cl:7])[cH:8][cH:9]1.O[N+:10](=[O:11])[O-:12]>>[CH3:1][c:2]1[cH:3][c:4]([Cl:5])[c:6]([Cl:7])[cH:8][c:9]1[N+:10](=[O:11])[O-:12]
Cc1ccc(Cl)c(Cl)c1.O=[N+]([O-])O
Cc1cc(Cl)c(Cl)cc1[N+](=O)[O-]
null
null
null
Functional Group Addition
Aromatic nitration with HNO3
53848b8b2bb4e867226e49db2e60519b24be9379900e3ad7c56af54fe8fde7a5
ddce49825c02b8965f10c8d99e3c841d26e1f136da6037b417c09313e6d73097
c1ccccc1
O-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3].[C;D1;H3:4]-[c:5](:[c:6]):[cH;D2;+0:7]:[c:8]:[c:9]>>[C;D1;H3:4]-[c:5](:[c:6]):[c;H0;D3;+0:7](-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3]):[c:8]:[c:9]
null
[]
null
null
null
null
3,4-Dichlorotoluene was nitrated with concentrated sulfuric acid and fuming nitric acid (d=1.52). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Nitrate
Nitro group
c1ccccc1
c1ccccc1
c1ccccc1
HO-
null
null
null
Cc1ccc(Cl)c(Cl)c1.O=[N+]([O-])O>>Cc1cc(Cl)c(Cl)cc1[N+](=O)[O-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-5c297b4a87b04776a1276a465dc94abc
Cc1cc(Cl)c(Cl)cc1[N+](=O)[O-].OCC(F)(F)F>>Cc1cc(OCC(F)(F)F)c(Cl)cc1[N+](=O)[O-]
CC(C)(C)[O-].[K+].C(C(F)(F)F)O.ClC1=CC(=C(C=C1Cl)C)[N+](=O)[O-]>>ClC1=CC(=C(C=C1OCC(F)(F)F)C)[N+](=O)[O-]
Cl[c:4]1[cH:3][c:2]([CH3:1])[c:14]([N+:15](=[O:16])[O-:17])[cH:13][c:11]1[Cl:12].[OH:5][CH2:6][C:7]([F:8])([F:9])[F:10]>>[CH3:1][c:2]1[cH:3][c:4]([O:5][CH2:6][C:7]([F:8])([F:9])[F:10])[c:11]([Cl:12])[cH:13][c:14]1[N+:15](=[O:16])[O-:17]
Cc1cc(Cl)c(Cl)cc1[N+](=O)[O-].OCC(F)(F)F
Cc1cc(OCC(F)(F)F)c(Cl)cc1[N+](=O)[O-]
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
4821d6d7238522ee9ef4538c00647e855becf4de3d9c939c0cec2b01c1e5e915
a4cafa7bcd156e21cca6eaac1b32e28ec8540642a31181122e6957f3d7559631
c1ccccc1
Cl-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Cl;D1;H0:5]):[c:6].[F;D1;H0:7]-[C:8](-[F;D1;H0:9])(-[F;D1;H0:10])-[C:11]-[OH;D1;+0:12]>>[Cl;D1;H0:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[O;H0;D2;+0:12]-[C:11]-[C:8](-[F;D1;H0:7])(-[F;D1;H0:9])-[F;D1;H0:10]):[c:2]:[c:3]
null
[]
null
null
null
null
40.4 g (360 mmol) of potassium tert-butylate were added in portions to 60 ml of trifluoroethanol, while stirring and cooling, and the mixture was heated to 80°-90° C. After cooling, 14.4 g (70 mmol) of 4,5-dichloro-2-nitrotoluene were added and the mixture was stirred at 105° C. for 1 hour. It was concentrated in vacuo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1
HCl
null
null
null
Cc1cc(Cl)c(Cl)cc1[N+](=O)[O-].OCC(F)(F)F>>Cc1cc(OCC(F)(F)F)c(Cl)cc1[N+](=O)[O-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0d0cde9f744f4003bee69dc9e97ec82e
NCC(=O)N1CCC[C@H]1C(=O)N1C[C@H](O)C[C@H]1C(=O)O.O=C(OCC1c2ccccc2-c2ccccc21)ON1C(=O)CCC1=O>>O=C(NCC(=O)N1CCC[C@H]1C(=O)N1C[C@H](O)C[C@H]1C(=O)O)OCC1c2ccccc2-c2ccccc21
C(=O)([O-])[O-].[Na+].[Na+].C(OCC1C2=CC=CC=C2C=2C=CC=CC12)(ON1C(CCC1=O)=O)=O.NCC(=O)N1[C@H](C(=O)N2[C@H](C(=O)O)C[C@@H](O)C2)CCC1.NCC(=O)N1[C@H](C(=O)N2[C@H](C(=O)O)C[C@@H](O)C2)CCC1>>N(CC(=O)N1[C@H](C(=O)N2[C@H](C(=O)O)C[C@@H](O)C2)CCC1)C(=O)OCC1C2=CC=CC=C2C2=CC=CC=C12
[NH2:3][CH2:4][C:5](=[O:6])[N:7]1[CH2:8][CH2:9][CH2:10][C@H:11]1[C:12](=[O:13])[N:14]1[CH2:15][C@H:16]([OH:17])[CH2:18][C@H:19]1[C:20](=[O:21])[OH:22].O=C1CCC(=O)N1O[C:2](=[O:1])[O:23][CH2:24][CH:25]1[c:26]2[cH:27][cH:28][cH:29][cH:30][c:31]2-[c:32]2[cH:33][cH:34][cH:35][cH:36][c:37]21>>[O:1]=[C:2]([NH:3][CH2:4][C:5](=...
NCC(=O)N1CCC[C@H]1C(=O)N1C[C@H](O)C[C@H]1C(=O)O.O=C(OCC1c2ccccc2-c2ccccc21)ON1C(=O)CCC1=O
O=C(NCC(=O)N1CCC[C@H]1C(=O)N1C[C@H](O)C[C@H]1C(=O)O)OCC1c2ccccc2-c2ccccc21
null
null
C(OC)COC.C(=O)([O-])[O-].[Na+].[Na+].O
Protection
OtherReaction
90f1cd2cfb4916c247fdb0b8c4bcd653fe37fb375d251f3afd49969111cee737
f7ec1d72774a3155b06d1cf24e018b58f69117ddf4d9559df84efc3ecef0f4d7
O=C(NCC(=O)N1CCC[C@H]1C(=O)N1CCCC1)OCC1c2ccccc2-c2ccccc21
O=C1-C-C-C(=O)-N-1-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4].[#7:5]-[C:6](=[O;D1;H0:7])-[C:8]-[#7:9](-[C:10](=[O;D1;H0:11])-[C:12]-[NH2;D1;+0:13])-[C:14]>>[#7:5]-[C:6](=[O;D1;H0:7])-[C:8]-[#7:9](-[C:10](=[O;D1;H0:11])-[C:12]-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4])-[C:14]
null
[]
4
CELSIUS
21
HOUR
Fmoc-Gly-Pro-Hyp was synthesized from Gly-Pro-Hyp as follows: 3.0 g Gly-Pro-Hyp (10.5 mmol) was dissolved in 54 mL Na2CO3 --H2O (1:9) and stored at 4° C. 4.05 g 9-fluorenylmethyl succinimidyl carbonate (12.0 mmol) was dissolved in 45 mL dimethoxyethane and stirred at 4° C. The aqueous Na2CO3 solution was added slowly t...
10.6084/m9.figshare.5104873.v1
null
Ether.Tertiary amide.Tertiary amide.Primary amine
Carbamic ester
C1CCNC1
null
C1CC[NH]C1.C1CC[NH]C1.c1ccc2c(c1)Cc1ccccc12
HO-
C(OC)COC.C(=O)([O-])[O-].[Na+].[Na+].O
4
21
NCC(=O)N1CCC[C@H]1C(=O)N1C[C@H](O)C[C@H]1C(=O)O.O=C(OCC1c2ccccc2-c2ccccc21)ON1C(=O)CCC1=O>C(OC)COC.C(=O)([O-])[O-].[Na+].[Na+].O>O=C(NCC(=O)N1CCC[C@H]1C(=O)N1C[C@H](O)C[C@H]1C(=O)O)OCC1c2ccccc2-c2ccccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c1ba761e373b418eb88a318c26b3d7f2
CCCC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O.O=C(O)CNC(=O)OCC1c2ccccc2-c2ccccc21>>C=CCC(=O)CNC(=O)OCC1c2ccccc2-c2ccccc21
N(CC(=O)O)C(=O)OCC1C2=CC=CC=C2C2=CC=CC=C12.C=1C=CC2=C(C1)N=NN2O.CC(C)N=C=NC(C)C.N([C@@H](CCCC)C(=O)O)C(=O)OCC1C2=CC=CC=C2C2=CC=CC=C12.CC1=CC=C(C=C1)C(C2=CC=CC=C2)N.C=CC1=CC=CC=C1.C=CC1=CC=C(C=C1)C=C.Cl.C=1C=CC2=C(C1)N=NN2O.CC(C)N=C=NC(C)C.C=1C=CC2=C(C1)N=NN2O.CC(C)N=C=NC(C)C>>N(CC(=O)CC=C)C(=O)OCC1C2=CC=CC=C2C2=CC=CC=C...
CC[CH2:2][CH2:3][C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O.O[C:4](=[O:5])[CH2:6][NH:7][C:8](=[O:9])[O:10][CH2:11][CH:12]1[c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]2-[c:19]2[cH:20][cH:21][cH:22][cH:23][c:24]21>>[CH2:1]=[CH:2][CH2:3][C:4](=[O:5])[CH2:6][NH:7][C:8](=[O:9])[O:10][CH2:11][CH:12]1[c:13]2[cH:14][cH:15][cH:16][c...
CCCC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O.O=C(O)CNC(=O)OCC1c2ccccc2-c2ccccc21
C=CCC(=O)CNC(=O)OCC1c2ccccc2-c2ccccc21
null
CN(C)C=1C=CN=CC1
CN(C)C=O.C(Cl)Cl.CN(C)C=O
C-C Coupling
OtherReaction
0eca1684da96ab67dce1b14f1cbf2209808af72c025b7fb12a2f1f73d35240c3
3eae7e4d25d89a062e55e5b9951a7233e3647040f5b5a06988852b724cfdebae
c1ccc2c(c1)Cc1ccccc1-2
C-C-[CH2;D2;+0:1]-[CH2;D2;+0:2]-[C@H](-N-C(=O)-O-C-C1-c2:c:c:c:c:c:2-c2:c:c:c:c:c:2-1)-C(-O)=O.O-[C;H0;D3;+0:3](=[O;D1;H0:4])-[C:5]-[#7:6]-[C:7]=[O;D1;H0:8]>>[C;D1;H2:9]=[CH;D2;+0:1]-[CH2;D2;+0:2]-[C;H0;D3;+0:3](=[O;D1;H0:4])-[C:5]-[#7:6]-[C:7]=[O;D1;H0:8]
null
[]
null
null
30
MINUTE
0.848 g Fmoc-Nle (2.4 mmol) was coupled to 2.0 g MBHA resin (1.6 mmol) with 0.367 g HOBt (2.4 mmol) and 0.373 mL DIPCDI (2.4 mmol) in 20 mL DCM-DMF (1:1) for 2.3 h. The resin was washed 3 times with DMF, deprotected with 20 mL piperidine-DMF (1:1) for 30 min, and washed 3 times with DMF. 1.82 g allyl linker (3.2 mmol) ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Carboxylic acid.Carboxylic acid.Ether
Ketone.Allyl
c1ccc2c(c1)Cc1ccccc12
null
c1ccc2c(c1)Cc1ccccc12
HO-
CN(C)C=1C=CN=CC1.CN(C)C=O.C(Cl)Cl.CN(C)C=O
null
0.5
CCCC[C@H](NC(=O)OCC1c2ccccc2-c2ccccc21)C(=O)O.O=C(O)CNC(=O)OCC1c2ccccc2-c2ccccc21>CN(C)C=1C=CN=CC1.CN(C)C=O.C(Cl)Cl.CN(C)C=O>C=CCC(=O)CNC(=O)OCC1c2ccccc2-c2ccccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-f12406699295447fa245b2a1d83d7703
BrCCBr.COc1ccc(Br)cc1.[Mg]>>COc1ccc([CH2][Mg][Br])cc1
BrC1=CC=C(C=C1)OC.[Mg].II.C1CCOC1.BrCCBr>>C(C1=CC=C(C=C1)OC)[Mg]Br
BrC[CH2:7][Br:9].Br[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:11][cH:10]1.[Mg:8]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][Mg:8][Br:9])[cH:10][cH:11]1
BrCCBr.COc1ccc(Br)cc1.[Mg]
COc1ccc([CH2][Mg][Br])cc1
null
null
null
C-C Coupling
OtherReaction
9715e07751be3d7cadbe1fdc48e97bed4ac08db10902529fa702981c6f96e883
798737e906b6055cdcd851af3dddf5a764921f9651ccac6f32257884e0fa16b2
c1ccccc1
Br-C-[CH2;D2;+0:1]-[Br;H0;D1;+0:2].Br-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6]:[c:7].[Mg;H0;D0;+0:8]>>[Br;H0;D1;+0:2]-[Mg;H0;D2;+0:8]-[CH2;D2;+0:1]-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6]:[c:7]
null
[]
20
CELSIUS
10
MINUTE
Magnesium (36 g, 1.5 mol), iodine (a few crystals) and THF (1 L) were heated under nitrogen, with stirring, at reflux for 15 min. The mixture was cooled to 20° C., stirring stopped, and 1,2-dibromoethane (2.5 ml) added. After an exothermic reaction was observed (a few min) stirring was restarted which was accompanied b...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary halide.Primary halide
Magnesium halide
c1ccccc1
c1ccccc1
c1ccccc1
HBr
null
20
0.166667
BrCCBr.COc1ccc(Br)cc1.[Mg]>>COc1ccc([CH2][Mg][Br])cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6534326785de4d64a16466ff2b37b899
C=O.Oc1cccnc1Br>>OCc1ccc(O)c(Br)n1
[OH-].[K+].BrC1=NC=CC=C1O.[Na].C=O>>BrC1=NC(=CC=C1O)CO
[O:1]=[CH2:2].[cH:3]1[cH:4][cH:5][c:6]([OH:7])[c:8]([Br:9])[n:10]1>>[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6]([OH:7])[c:8]([Br:9])[n:10]1
C=O.Oc1cccnc1Br
OCc1ccc(O)c(Br)n1
null
null
C(C)(=O)O.O
C-C Coupling
OtherReaction
e828e08512136a1006e7ed8edf3ea1a358c5687d4ea7b00d12d245f1aeb515aa
4396295d899f5d4f5de2e844a80fc7d194b4da158f49df3d2717206b401b59bd
c1ccncc1
[CH2;D1;+0:1]=[O;H0;D1;+0:2].[c:3]:[c:4]:[cH;D2;+0:5]:[#7;a:6]:[c:7]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c;H0;D3;+0:5](:[#7;a:6]:[c:7]):[c:4]:[c:3]
null
[]
null
null
2
HOUR
Potassium hydroxide (85% assay, 113.8 g, 1.73 mol) was dissolved in distilled water (750 ml) and to the solution was added 2-bromo-3-hydroxypyridine (300 g, 1.72 mol), ethylenediaminetetraaeetic acid sodium salt (2 mol %, 13.1 g, 0.034 mol) and formalin (37-41% w/v 470 ml, 5.95 mol). The stirred mixture was heated at 9...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde
Primary alcohol
c1ccncc1
c1ccncc1
c1ccncc1
null
C(C)(=O)O.O
null
2
C=O.Oc1cccnc1Br>C(C)(=O)O.O>OCc1ccc(O)c(Br)n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-518c5ae80b704ac1999ffc9853c652ad
C=CC(=O)OC(C)(C)C.COc1ccc(CCCCCCCCOc2ccc(CO)nc2Br)cc1>>COc1ccc(CCCCCCCCOc2ccc(CO)nc2C=CC(=O)OC(C)(C)C)cc1
BrC1=NC(=CC=C1OCCCCCCCCC1=CC=C(C=C1)OC)CO.C(C)(=O)[O-].[K+].C(C=C)(=O)OC(C)(C)C.CCOCC>>OCC1=CC=C(C(=N1)C=CC(=O)OC(C)(C)C)OCCCCCCCCC1=CC=C(C=C1)OC
[CH2:24]=[CH:25][C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32].Br[c:23]1[c:16]([O:15][CH2:14][CH2:13][CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:34][cH:33]2)[cH:17][cH:18][c:19]([CH2:20][OH:21])[n:22]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][CH2:8][CH2:9][CH2:10][...
C=CC(=O)OC(C)(C)C.COc1ccc(CCCCCCCCOc2ccc(CO)nc2Br)cc1
COc1ccc(CCCCCCCCOc2ccc(CO)nc2C=CC(=O)OC(C)(C)C)cc1
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
ClCCl.CN(C)C=O.O
C-C Coupling
Heck terminal vinyl
6ff9a103c54245e6fd54f5e5a1a2869a152f70eb90c7b0a9e978953fb523505e
4b186811a4930853b446d93d9faa39b267bddb9ce0b8021bda5c5a3b2bc69f0b
c1ccc(CCCCCCCCOc2cccnc2)cc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[#8:5]):[c:6].[C;D1;H3:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[#8:11]-[C:12](=[O;D1;H0:13])-[C:14]=[CH2;D1;+0:15]>>[#8:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[CH;D2;+0:15]=[C:14]-[C:12](=[O;D1;H0:13])-[#8:11]-[C:8](-[C;D1;H3:7])(-[C;D1;H3:9])-[C;D1;H3:10]):[#7;a:2]:[c:3]
null
[]
120
CELSIUS
null
null
To a solution of 2-bromo-6-hydroxymethyl-[8(4-methoxyphenyl)octyloxy]pyridine (5.00 g, 11.8 mmol) in DMF (22.8 ml) and water (1.2 ml) were added potassium acetate (3.00 g, 30.6 mmol), tetra-n-butylammonium iodide (4.36 g, 11.8 mmol), bis(triphenylphosphine)palladium dichloride (0.33 g, 0.47 mmol) and t-butyl acrylate (...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl
null
c1ccncc1
c1ccncc1
c1ccccc1.c1ccncc1
HBr
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.ClCCl.CN(C)C=O.O
120
null
C=CC(=O)OC(C)(C)C.COc1ccc(CCCCCCCCOc2ccc(CO)nc2Br)cc1>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.ClCCl.CN(C)C=O.O>COc1ccc(CCCCCCCCOc2ccc(CO)nc2C=CC(=O)OC(C)(C)C)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d167806c04b646d4b1c49664d0f6f7f3
C=CC(=O)[O-].COc1ccc(CCCCCCCCOc2ccc(CO)nc2Br)cc1>>COc1ccc(CCCCCCCCOc2ccc(CO)nc2C=CC(=O)O)cc1
C(C=C)(=O)[O-].[K+].BrC1=NC(=CC=C1OCCCCCCCCC1=CC=C(C=C1)OC)CO.C(C)(=O)[O-].[K+].C(C=C)(=O)[O-].[K+].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>OCC1=CC=C(C(=N1)C=CC(=O)O)OCCCCCCCCC1=CC=C(C=C1)OC
[CH2:24]=[CH:25][C:26](=[O:27])[O-:28].Br[c:23]1[c:16]([O:15][CH2:14][CH2:13][CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:30][cH:29]2)[cH:17][cH:18][c:19]([CH2:20][OH:21])[n:22]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][O...
C=CC(=O)[O-].COc1ccc(CCCCCCCCOc2ccc(CO)nc2Br)cc1
COc1ccc(CCCCCCCCOc2ccc(CO)nc2C=CC(=O)O)cc1
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.[Pd](Cl)Cl
CN(C)C=O.O
C-C Coupling
OtherReaction
3b41ec1889793db9e086d930ee817d7e17590040116fe3ea8390760f5b59a649
96c1c356cfda99239d83270c8639c030c1984d01ddd836a1f89bde5e602ad450
c1ccc(CCCCCCCCOc2cccnc2)cc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[#8:5]):[c:6].[CH2;D1;+0:7]=[C:8]-[C:9](-[O-;H0;D1:10])=[O;D1;H0:11]>>[#8:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[CH;D2;+0:7]=[C:8]-[C:9](=[O;D1;H0:11])-[OH;D1;+0:10]):[#7;a:2]:[c:3]
null
[]
120
CELSIUS
null
null
To a solution of 2-bromo-6-hydroxymethyl-[8(4-methoxyphenyl)octyloxy]pyridine (5.00 g, 11.8 mmol) in DMF (22.8 ml) and water (1.2 ml) were added potassium acetate (2.91 g, 29.7 mmol), tetra-n-butylammonium iodide (4.37 g, 11.8 mmol); triphenylphosphine (0.245 g, 0.94 mmol), palladium chloride (83 mg, 0.47 mmol) and pot...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl
Carboxylic acid
c1ccncc1
c1ccncc1
c1ccccc1.c1ccncc1
Br-
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.[Pd](Cl)Cl.CN(C)C=O.O
120
null
C=CC(=O)[O-].COc1ccc(CCCCCCCCOc2ccc(CO)nc2Br)cc1>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.[Pd](Cl)Cl.CN(C)C=O.O>COc1ccc(CCCCCCCCOc2ccc(CO)nc2C=CC(=O)O)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-daea2679130c4e96a69efc91647c4537
C=CC(=O)OCC.Cc1ccc(O)c(I)n1>>C=C(C(=O)OCC)c1nc(C)ccc1O
OC=1C(=NC(=CC1)C)I.C(C)(=O)[O-].[K+].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(C=C)(=O)OCC>>OC=1C(=NC(=CC1)C)C(C(=O)OCC)=C
[CH2:1]=[CH:2][C:3](=[O:4])[O:5][CH2:6][CH3:7].I[c:8]1[n:9][c:10]([CH3:11])[cH:12][cH:13][c:14]1[OH:15]>>[CH2:1]=[C:2]([C:3](=[O:4])[O:5][CH2:6][CH3:7])[c:8]1[n:9][c:10]([CH3:11])[cH:12][cH:13][c:14]1[OH:15]
C=CC(=O)OCC.Cc1ccc(O)c(I)n1
C=C(C(=O)OCC)c1nc(C)ccc1O
null
[Pd](Cl)Cl
CN(C)C=O.O
C-C Coupling
OtherReaction
8d3cfa690cead9dcdb5f0a1f56e2ac08c5de55d1454f6c77dc7ae2812b1acf3d
0148cae362ae1ae42dbb9a3b681759839c81f4c02b0942bce45e45dd2b0b9c70
c1ccncc1
I-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[O;D1;H1:5]):[c:6].[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[CH;D2;+0:11]=[C;D1;H2:12]>>[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[C;H0;D3;+0:11](=[C;D1;H2:12])-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[O;D1;H1:5]):[c:6]
null
[]
120
CELSIUS
null
null
To a solution of 3-hydroxy-2-iodo-6-methylpyridine (1.175 g, 5.0 mmol) in DMF (9.5 ml) and water (0.5 ml) were added potassium acetate (1.23 g, 12.5 mmol), triphenylphosphine (105 mg, 0.40 mmol), palladium chloride (36 mg, 0.20 mmol) and ethyl acrylate (1.63 ml, 1.50 g, 15.0 mmol). The mixture was placed under nitrogen...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester
Ester.Vinyl
c1ccncc1
c1ccncc1
c1ccncc1
HI
[Pd](Cl)Cl.CN(C)C=O.O
120
null
C=CC(=O)OCC.Cc1ccc(O)c(I)n1>[Pd](Cl)Cl.CN(C)C=O.O>C=C(C(=O)OCC)c1nc(C)ccc1O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-33f5c2c61cec497c9cae12b9bafc104f
C=CC(=O)OCC.OCc1ccc(O)c(I)n1>>CCOC(=O)C=Cc1nc(CO)ccc1O
OC=1C(=NC(=CC1)CO)I.C(C)(=O)[O-].[K+].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(C=C)(=O)OCC>>OC=1C(=NC(=CC1)CO)C=CC(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[CH2:7].I[c:8]1[n:9][c:10]([CH2:11][OH:12])[cH:13][cH:14][c:15]1[OH:16]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[CH:7][c:8]1[n:9][c:10]([CH2:11][OH:12])[cH:13][cH:14][c:15]1[OH:16]
C=CC(=O)OCC.OCc1ccc(O)c(I)n1
CCOC(=O)C=Cc1nc(CO)ccc1O
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
CN(C)C=O.O
C-C Coupling
Heck terminal vinyl
6ff9a103c54245e6fd54f5e5a1a2869a152f70eb90c7b0a9e978953fb523505e
4b186811a4930853b446d93d9faa39b267bddb9ce0b8021bda5c5a3b2bc69f0b
c1ccncc1
I-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[O;D1;H1:5]):[c:6].[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[C:11]=[CH2;D1;+0:12]>>[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[C:11]=[CH;D2;+0:12]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[O;D1;H1:5]):[c:6]
null
[]
120
CELSIUS
null
null
To a solution of 3-hydroxy-6-hydroxymethyl-2-iodopyridine (708 mg, 2.82 mmol) in DMF (5.7 ml) and water (0.3 ml) were added potassium acetate (0.74 g, 7.5 mmol), triphenylphosphine (63 mg, 0.24 mmol), ethyl acrylate (0.98 ml, 0.90 g, 9.0 mmol) and palladium acetate (27 mg, 0.12 mmol). The mixture was placed under nitro...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl
null
c1ccncc1
c1ccncc1
c1ccncc1
HI
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CN(C)C=O.O
120
null
C=CC(=O)OCC.OCc1ccc(O)c(I)n1>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CN(C)C=O.O>CCOC(=O)C=Cc1nc(CO)ccc1O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7962bc1b7397448eac87976efef7cca2
C=CC(=O)OCC.OCc1ccc(OCc2ccccc2)c(I)n1>>C=C(C(=O)OCC)c1nc(CO)ccc1OCc1ccccc1
C(C1=CC=CC=C1)OC=1C(=NC(=CC1)CO)I.C(C)(=O)[O-].[K+].C(C=C)(=O)OCC>>C(C1=CC=CC=C1)OC=1C(=NC(=CC1)CO)C(C(=O)OCC)=C
[CH2:1]=[CH:2][C:3](=[O:4])[O:5][CH2:6][CH3:7].I[c:8]1[n:9][c:10]([CH2:11][OH:12])[cH:13][cH:14][c:15]1[O:16][CH2:17][c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[CH2:1]=[C:2]([C:3](=[O:4])[O:5][CH2:6][CH3:7])[c:8]1[n:9][c:10]([CH2:11][OH:12])[cH:13][cH:14][c:15]1[O:16][CH2:17][c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]...
C=CC(=O)OCC.OCc1ccc(OCc2ccccc2)c(I)n1
C=C(C(=O)OCC)c1nc(CO)ccc1OCc1ccccc1
null
null
CN(C)C=O.O
C-C Coupling
OtherReaction
8d3cfa690cead9dcdb5f0a1f56e2ac08c5de55d1454f6c77dc7ae2812b1acf3d
0148cae362ae1ae42dbb9a3b681759839c81f4c02b0942bce45e45dd2b0b9c70
c1ccc(COc2cccnc2)cc1
I-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[#8:5]):[c:6].[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[CH;D2;+0:11]=[C;D1;H2:12]>>[#8:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[C;H0;D3;+0:11](=[C;D1;H2:12])-[C:9](=[O;D1;H0:10])-[#8:8]-[C:7]):[#7;a:2]:[c:3]
62
[{"value": 62.0, "product": "C(C1=CC=CC=C1)OC=1C(=NC(=CC1)CO)C(C(=O)OCC)=C", "details": "PERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
To a solution of 3-benzyloxy-6-hydroxymethyl-2-iodopyridine (1.20 g, 3.50 mmol) in DMF (6.4 ml) and water (0.32 ml) were added potassium acetate (0.83 g, 8.5 mmol) palladium acetate (32 mg, 0.14 mmol) and ethyl acrylate (1.1 ml, 1.01 g, 10 mmol). The mixture was placed under nitrogen and stirred and heated at 120° C. f...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester
Ester.Vinyl
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1
HI
CN(C)C=O.O
120
null
C=CC(=O)OCC.OCc1ccc(OCc2ccccc2)c(I)n1>CN(C)C=O.O>C=C(C(=O)OCC)c1nc(CO)ccc1OCc1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-cbc402db79bd4ddea3a7284194868b01
C=CC(=O)OCCCC.OCc1ccc(OCc2ccccc2)c(Br)n1>>C=C(C(=O)OCCCC)c1nc(CO)ccc1OCc1ccccc1
BrC1=NC(=CC=C1OCC1=CC=CC=C1)CO.C(C)(=O)[O-].[K+].C(C=C)(=O)OCCCC>>C(C1=CC=CC=C1)OC=1C(=NC(=CC1)CO)C(C(=O)OCCCC)=C
[CH2:1]=[CH:2][C:3](=[O:4])[O:5][CH2:6][CH2:7][CH2:8][CH3:9].Br[c:10]1[n:11][c:12]([CH2:13][OH:14])[cH:15][cH:16][c:17]1[O:18][CH2:19][c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1>>[CH2:1]=[C:2]([C:3](=[O:4])[O:5][CH2:6][CH2:7][CH2:8][CH3:9])[c:10]1[n:11][c:12]([CH2:13][OH:14])[cH:15][cH:16][c:17]1[O:18][CH2:19][c:20]1[c...
C=CC(=O)OCCCC.OCc1ccc(OCc2ccccc2)c(Br)n1
C=C(C(=O)OCCCC)c1nc(CO)ccc1OCc1ccccc1
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
CN(C)C=O.O
C-C Coupling
OtherReaction
8d3cfa690cead9dcdb5f0a1f56e2ac08c5de55d1454f6c77dc7ae2812b1acf3d
0148cae362ae1ae42dbb9a3b681759839c81f4c02b0942bce45e45dd2b0b9c70
c1ccc(COc2cccnc2)cc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[#8:5]):[c:6].[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[CH;D2;+0:11]=[C;D1;H2:12]>>[#8:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[C;H0;D3;+0:11](=[C;D1;H2:12])-[C:9](=[O;D1;H0:10])-[#8:8]-[C:7]):[#7;a:2]:[c:3]
null
[]
120
CELSIUS
null
null
To a solution of 2-bromo-3-benzyloxy-6-hydroxymethylpyridine (2.94 g, 10.0 mmol) in DMF (19 ml) and water (1 ml) were added potassium acetate (2.45 g, 25.0 mmol), tetra-n-butylammonium iodide (3.69 g, 10.0 mmol), bis(triphenylphosphine)palladium dichloride (281 mg, 0.4 mmol) and n-butyl acrylate (4.31 ml, 3.84 g, 30 mm...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester
Ester.Vinyl
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1
HBr
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O.O
120
null
C=CC(=O)OCCCC.OCc1ccc(OCc2ccccc2)c(Br)n1>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O.O>C=C(C(=O)OCCCC)c1nc(CO)ccc1OCc1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a748f251ca1d423aa7e17eaf3d09ac7f
C=CC(=O)OC.OCc1ccc(OCc2ccccc2)c(Br)n1>>C=C(C(=O)OC)c1nc(CO)ccc1OCc1ccccc1
BrC1=NC(=CC=C1OCC1=CC=CC=C1)CO.C(C)(=O)[O-].[K+].C(C=C)(=O)OC>>C(C1=CC=CC=C1)OC=1C(=NC(=CC1)CO)C(C(=O)OC)=C
[CH2:1]=[CH:2][C:3](=[O:4])[O:5][CH3:6].Br[c:7]1[n:8][c:9]([CH2:10][OH:11])[cH:12][cH:13][c:14]1[O:15][CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1>>[CH2:1]=[C:2]([C:3](=[O:4])[O:5][CH3:6])[c:7]1[n:8][c:9]([CH2:10][OH:11])[cH:12][cH:13][c:14]1[O:15][CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1
C=CC(=O)OC.OCc1ccc(OCc2ccccc2)c(Br)n1
C=C(C(=O)OC)c1nc(CO)ccc1OCc1ccccc1
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
CN(C)C=O.O
C-C Coupling
OtherReaction
8d3cfa690cead9dcdb5f0a1f56e2ac08c5de55d1454f6c77dc7ae2812b1acf3d
0148cae362ae1ae42dbb9a3b681759839c81f4c02b0942bce45e45dd2b0b9c70
c1ccc(COc2cccnc2)cc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](-[#8:5]):[c:6].[C;D1;H2:7]=[CH;D2;+0:8]-[C:9](=[O;D1;H0:10])-[#8:11]-[C;D1;H3:12]>>[#8:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[C;H0;D3;+0:8](=[C;D1;H2:7])-[C:9](=[O;D1;H0:10])-[#8:11]-[C;D1;H3:12]):[#7;a:2]:[c:3]
84.1
[{"value": 84.0, "product": "C(C1=CC=CC=C1)OC=1C(=NC(=CC1)CO)C(C(=O)OC)=C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.1, "product": "C(C1=CC=CC=C1)OC=1C(=NC(=CC1)CO)C(C(=O)OC)=C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
To a solution of 2-bromo-3-benzyloxy-6-hydroxymethylpyridine (2.94 g, 10 mmol) in DMF (19 ml) and water (1 ml) were added potassium acetate (2.45 g, 10.0 mmol), tetra-n-butylammonium iodide (3.69 g. 10.0 mmol), bis(triphenyl-phosphine)palladium dichloride (281 mg, 0.4 mmol) and methyl acrylate (2.70 ml. 2.58 g, 30 mmol...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester
Ester.Vinyl
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1
HBr
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O.O
120
null
C=CC(=O)OC.OCc1ccc(OCc2ccccc2)c(Br)n1>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O.O>C=C(C(=O)OC)c1nc(CO)ccc1OCc1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-10d91779e086461aa563e2a37737f0b8
CC(C)(C)OC(=O)NCC/C=C/c1cncnc1.CI>>CN(CC/C=C/c1cncnc1)C(=O)OC(C)(C)C
[H-].[Na+].C(C)(C)(C)OC(=O)NCC\C=C\C=1C=NC=NC1.IC.C(C)(C)NC(C)C>>CN(CC\C=C\C=1C=NC=NC1)C(=O)OC(C)(C)C
[NH:2]([CH2:3][CH2:4]/[CH:5]=[CH:6]/[c:7]1[cH:8][n:9][cH:10][n:11][cH:12]1)[C:13](=[O:14])[O:15][C:16]([CH3:17])([CH3:18])[CH3:19].I[CH3:1]>>[CH3:1][N:2]([CH2:3][CH2:4]/[CH:5]=[CH:6]/[c:7]1[cH:8][n:9][cH:10][n:11][cH:12]1)[C:13](=[O:14])[O:15][C:16]([CH3:17])([CH3:18])[CH3:19]
CC(C)(C)OC(=O)NCC/C=C/c1cncnc1.CI
CN(CC/C=C/c1cncnc1)C(=O)OC(C)(C)C
null
null
COCCOC.O.CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
29c841ae076cb6ee785aad2a4e3ce1a9b47357d7ad25657b8d9991b1347f5721
c485eddcb40c5a0d396ffdb624041effa09ee4f5ca2ecce3fe13077cf65004ed
c1cncnc1
I-[CH3;D1;+0:1].[C:2]=[C:3]/[C:4]-[C:5]-[NH;D2;+0:6]-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13]>>[C:2]=[C:3]/[C:4]-[C:5]-[N;H0;D3;+0:6](-[CH3;D1;+0:1])-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13]
76.1
[{"value": 76.1, "product": "CN(CC\\C=C\\C=1C=NC=NC1)C(=O)OC(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
45
MINUTE
Under a nitrogen atmosphere, sodium hydride (0.78 g, 19.5 mmol, 60% dispersion in oil) was added to a stirring solution of IV (0.50 g, 2.0 mmol), 1,2-dimethyoxyethane (20 mL), DMF (25 mL), and a trace of diisopropylamine. The mixture was stirred at ambient temperature for 45 min, and a solution of iodomethane (2.59 g, ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester
Carbamic ester
null
null
c1cncnc1
HI
COCCOC.O.CN(C)C=O
null
0.75
CC(C)(C)OC(=O)NCC/C=C/c1cncnc1.CI>COCCOC.O.CN(C)C=O>CN(CC/C=C/c1cncnc1)C(=O)OC(C)(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b463cdcceaba4202b2513724f75023cf
BrC(Br)(Br)Br.O=Cc1cccnc1>>BrC(Br)=Cc1cccnc1
BrC(Br)(Br)Br.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.N1=CC(=CC=C1)C=O>>BrC(=CC=1C=NC=CC1)Br
Br[C:2](Br)([Br:1])[Br:3].O=[CH:4][c:5]1[cH:6][cH:7][cH:8][n:9][cH:10]1>>[Br:1][C:2]([Br:3])=[CH:4][c:5]1[cH:6][cH:7][cH:8][n:9][cH:10]1
BrC(Br)(Br)Br.O=Cc1cccnc1
BrC(Br)=Cc1cccnc1
null
null
C(Cl)Cl
C-C Coupling
OtherReaction
b27e55226bb2edd452ae488b95081b2b03421ee27be6c3935dbea4c7a5eeb5f6
695d5d1b30a064e72a7d907baf677e910730421b6580cc4e59d378cd6f0be898
c1ccncc1
Br-[C;H0;D4;+0:1](-Br)(-[Br;D1;H0:2])-[Br;D1;H0:3].O=[CH;D2;+0:4]-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]>>[Br;D1;H0:2]-[C;H0;D3;+0:1](-[Br;D1;H0:3])=[CH;D2;+0:4]-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]
70
[{"value": 70.0, "product": "BrC(=CC=1C=NC=CC1)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.0, "product": "BrC(=CC=1C=NC=CC1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
45
MINUTE
Tetrabromomethane (24.82 g, 0.747 mole) and triphenylphosphine (39.17 g, 0.149 mole) were stirred together in dry methylene chloride (100 mL) for 5 min. at 0° C. under a nitrogen atmosphere. To this mixture was added dropwise pyridine 3-carboxaldehyde (4 g, 0.0373 mole). The solution was then stirred for 45 min. at amb...
10.6084/m9.figshare.5104873.v1
null
Tertiary halide.Tertiary halide.Tertiary halide.Tertiary halide.Aldehyde
Alkenyl halide.Alkenyl halide
null
null
c1ccncc1
Br-
C(Cl)Cl
null
0.75
BrC(Br)(Br)Br.O=Cc1cccnc1>C(Cl)Cl>BrC(Br)=Cc1cccnc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-acfd98fbecaf4acda872324b5f557a19
C=O.Cc1ccc(C2CCCN2)cn1>>Cc1ccc(C2CCCN2C)cn1
CC1=NC=C(C=C1)C2CCCN2.C=O.[OH-].[Na+]>>CC1=NC=C(C=C1)C2CCCN2C
O=[CH2:11].[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH:6]2[CH2:7][CH2:8][CH2:9][NH:10]2)[cH:12][n:13]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH:6]2[CH2:7][CH2:8][CH2:9][N:10]2[CH3:11])[cH:12][n:13]1
C=O.Cc1ccc(C2CCCN2)cn1
Cc1ccc(C2CCCN2C)cn1
null
null
C(=O)O
Heteroatom Alkylation and Arylation
Eschweiler-Clarke Secondary Amine Methylation
91bb2ea8aeb046c2c7c6bbf5485a7fce0a359aeb3adea3549d5b06757bc9a669
e1fdef8fde1c506d7c9deb8fd5e6f322eceea2abce3167abcf412a1fa4fd5443
c1cncc(C2CCCN2)c1
O=[CH2;D1;+0:1].[#7;a:2]:[c:3]:[c:4]-[C:5]1-[C:6]-[C:7]-[C:8]-[NH;D2;+0:9]-1>>[#7;a:2]:[c:3]:[c:4]-[C:5]1-[C:6]-[C:7]-[C:8]-[N;H0;D3;+0:9]-1-[CH3;D1;+0:1]
92
[{"value": 92.0, "product": "CC1=NC=C(C=C1)C2CCCN2C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Into a round bottom flask was placed XVI (2.0 g), and formaldehyde (37% w/v in water, 20 mL) and formic acid (95-97% w/v, 45 mL), both a 0° C., were added. The mixture then was refluxed under nitrogen for 8 hr. The cooled reaction mixture was basified with aqueous sodium hydroxide (50% w/v) to pH 8-9, and the solution ...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Secondary amine
Tertiary amine
C1CCNC1
C1CC[NH]C1
c1ccncc1.C1CC[NH]C1
Other
C(=O)O
null
null
C=O.Cc1ccc(C2CCCN2)cn1>C(=O)O>Cc1ccc(C2CCCN2C)cn1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-73e83470040446eba51ba941b5338013
NCCc1ccc(O)c(O)c1.O=S(=O)(O)CCN1CCN(CCO)CC1.O=S(=O)(O)CCN1CCN(CCO)CC1>>CN1CCC[C@H]1c1cccnc1
C1CN(CCN1CCO)CCS(=O)(=O)O.NCCC1=CC(O)=C(O)C=C1.C1CN(CCN1CCO)CCS(=O)(=O)O.NCCC1=CC(O)=C(O)C=C1>>N1=CC=CC(=C1)[C@H]1N(C)CCC1
N[CH2:5][CH2:6][c:7]1[cH:8][cH:9][c:10](O)c(O)[cH:12]1.O=S(=O)(O)CCN1CC[N:11](CCO)CC1.O=S(=O)(O)CCN1CC[N:2]([CH2:1]CO)[CH2:3][CH2:4]1>>[CH3:1][N:2]1[CH2:3][CH2:4][CH2:5][C@H:6]1[c:7]1[cH:8][cH:9][cH:10][n:11][cH:12]1
NCCc1ccc(O)c(O)c1.O=S(=O)(O)CCN1CCN(CCO)CC1.O=S(=O)(O)CCN1CCN(CCO)CC1
CN1CCC[C@H]1c1cccnc1
null
null
C([C@@H]1[C@H]([C@@H]([C@H]([C@H](O1)O[C@]2([C@H]([C@@H]([C@H](O2)CO)O)O)CO)O)O)O)O
Heteroatom Alkylation and Arylation
OtherReaction
19fc9a872b549396d811b42e2ef2bc61edfc6ad753a9b784038fcb2d26d8bd1b
22424af31acac19f7bdb5717c7b71b423c8772246143962540fd1af6bf911444
c1cncc([C@@H]2CCCN2)c1
N-[CH2;D2;+0:1]-[CH2;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[c;H0;D3;+0:6](-O):c(-O):[cH;D2;+0:7]:1.O-C-C-[N;H0;D3;+0:8]1-C-C-N(-C-C-S(-O)(=O)=O)-C-C-1.O-C-[CH2;D2;+0:9]-[N;H0;D3;+0:10]1-C-C-N(-C-C-S(-O)(=O)=O)-[CH2;D2;+0:11]-[C:12]-1>>[CH3;D1;+0:9]-[N;H0;D3;+0:10]1-[C:12]-[CH2;D2;+0:11]-[CH2;D2;+0:1]-[C@H;D3;+0:2]-1-[c:3]1:[c:4]...
null
[]
null
null
10
MINUTE
Dopamine release was measured by preparing synaptosomes from the striatal area of rat brain obtained from Sprague-Dawley rats generally according to the procedures set forth by Nagy et al., J. Neurochem., Vol. 43, pp. 1114-1123 (1984). Striata from 4 rats were homogenized in 2 ml of 0.32M sucrose buffered with 5 mM HEP...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Primary alcohol.Aromatic alcohol.Aromatic alcohol.Primary amine.Tertiary amine.Tertiary amine.Tertiary amine.Tertiary amine.Sulfonic acid.Sulfonic acid
Tertiary amine
c1ccccc1.C1CNCC[NH]1.C1CNCC[NH]1
C1CC[NH]C1.c1ccncc1
C1CC[NH]C1.c1ccncc1
HO-
C([C@@H]1[C@H]([C@@H]([C@H]([C@H](O1)O[C@]2([C@H]([C@@H]([C@H](O2)CO)O)O)CO)O)O)O)O
null
0.166667
NCCc1ccc(O)c(O)c1.O=S(=O)(O)CCN1CCN(CCO)CC1.O=S(=O)(O)CCN1CCN(CCO)CC1>C([C@@H]1[C@H]([C@@H]([C@H]([C@H](O1)O[C@]2([C@H]([C@@H]([C@H](O2)CO)O)O)CO)O)O)O)O>CN1CCC[C@H]1c1cccnc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2efa0157f0794899ae4b9b6277f9cfd2
COC(=O)[C@H](O)[C@@H](NC(=O)OC(C)(C)C)c1ccccc1.O=CC(Cl)(Cl)Cl>>COC(=O)[C@@H]1OC(C(Cl)(Cl)Cl)N[C@H]1c1ccccc1
C(C)(C)(C)OC(=O)N[C@H]([C@H](C(=O)OC)O)C1=CC=CC=C1.O=CC(Cl)(Cl)Cl.C1(=CC=C(C=C1)S(=O)(=O)[O-])C.[NH+]1=CC=CC=C1>>COC(=O)[C@H]1[C@@H](NC(O1)C(Cl)(Cl)Cl)C1=CC=CC=C1
CC(C)(C)O[C:7](=O)[NH:12][C@H:13]([C@H:5]([C:3]([O:2][CH3:1])=[O:4])[OH:6])[c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1.O=C[C:8]([Cl:9])([Cl:10])[Cl:11]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[O:6][CH:7]([C:8]([Cl:9])([Cl:10])[Cl:11])[NH:12][C@H:13]1[c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1
COC(=O)[C@H](O)[C@@H](NC(=O)OC(C)(C)C)c1ccccc1.O=CC(Cl)(Cl)Cl
COC(=O)[C@@H]1OC(C(Cl)(Cl)Cl)N[C@H]1c1ccccc1
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
875f311f15254ab0306d385b68a0217cd66c4ae0dba2b1f601a96620dbad3fb4
8f365cb6871fb0212098d3b154969febdc519bee26d88c8a0ee935c154eca887
c1ccc([C@H]2COCN2)cc1
C-C(-C)(-C)-O-[C;H0;D3;+0:1](=O)-[#7:2]-[C:3]-[C:4](-[OH;D1;+0:5])-[C:6](=[O;D1;H0:7])-[#8:8]-[C;D1;H3:9].O=C-[C;H0;D4;+0:10](-[Cl;D1;H0:11])(-[Cl;D1;H0:12])-[Cl;D1;H0:13]>>[C;D1;H3:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[C:4]1-[C:3]-[#7:2]-[CH;D3;+0:1](-[C;H0;D4;+0:10](-[Cl;D1;H0:11])(-[Cl;D1;H0:12])-[Cl;D1;H0:13])-[O;H0;D2;+0...
91
[{"value": 91.0, "product": "COC(=O)[C@H]1[C@@H](NC(O1)C(Cl)(Cl)Cl)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
20
CELSIUS
null
null
A solution of 3.0 g of methyl (2R,3S)-3-(tert-butoxycarbonylamino)-2-hydroxy-3-phenylpropionate, of 5 cm3 of chloral and of 0.05 g of pyridinium p-toluenesulphonate in 40 cm3 of anhydrous toluene is heated at reflux with distillation of the solvent. 15 cm3 of solvent are distilled and then 5 cm3 of chloral and 0.05 g o...
10.6084/m9.figshare.5104873.v1
null
Trichloro group.Aldehyde.Carbamic ester.Ether.Secondary alcohol.Boc
Trichloro group.Ether
null
C1COCN1
C1COCN1.c1ccccc1
HO-
C1(=CC=CC=C1)C
20
null
COC(=O)[C@H](O)[C@@H](NC(=O)OC(C)(C)C)c1ccccc1.O=CC(Cl)(Cl)Cl>C1(=CC=CC=C1)C>COC(=O)[C@@H]1OC(C(Cl)(Cl)Cl)N[C@H]1c1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d735999e237040e79efd9e34aa9e36bf
CCOC(=O)CBr.CSC>>CCOC(=O)C[S+](C)C.[Br-]
BrCC(=O)OCC.CSC>>[Br-].C(=O)(OCC)C[S+](C)C
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][Br:10].[S:7]([CH3:8])[CH3:9]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][S+:7]([CH3:8])[CH3:9].[Br-:10]
CCOC(=O)CBr.CSC
CCOC(=O)C[S+](C)C.[Br-]
null
null
CC(=O)C
Functional Group Interconversion
OtherReaction
330ba230541c446579322dd1f88c2db776aefe9bd80c8cf1780c2ef11bd721f7
7219c7e59d7b4e04c52ec17fd1785ce10066175f9fdee39a2b95a7cdf0cce07b
null
[Br;H0;D1;+0:1]-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6].[C;D1;H3:7]-[S;H0;D2;+0:8]-[C;D1;H3:9]>>[Br-;H0;D0:1].[C:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[CH2;D2;+0:2]-[S+;H0;D3:8](-[C;D1;H3:7])-[C;D1;H3:9]
null
[]
null
null
3
DAY
A solution of ethyl bromoacetate (265 g) and dimethyl sulfide (114 g) in acetone (500 mL) was stirred at room temperature. After three days, the title compound was isolated by filtration of the reaction mixture. Melting point 88°-90° C. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Monosulfide
Ester
null
null
null
null
CC(=O)C
null
72
CCOC(=O)CBr.CSC>CC(=O)C>CCOC(=O)C[S+](C)C.[Br-]
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8fef71afc98949c49bc84e25d6876698
CCOC(=O)C[S+](C)C.O=C1C=CCC1>>CCOC(=O)C1C2CCC(=O)C21
Cl.[Cl-].[Na+].N12CCCCCC2=NCCC1.[Br-].C(=O)(OCC)C[S+](C)C.C1(C=CCC1)=O>>O=C1C2C(C2CC1)C(=O)OCC
C[S+](C)[CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].[CH:7]1=[CH:12][C:10](=[O:11])[CH2:9][CH2:8]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH:7]2[CH2:8][CH2:9][C:10](=[O:11])[CH:12]12
CCOC(=O)C[S+](C)C.O=C1C=CCC1
CCOC(=O)C1C2CCC(=O)C21
null
null
C1(=CC=CC=C1)C
C-C Coupling
OtherReaction
12efc71b43a52362bb5f8e0d3581ffe17688ff325d048d90483f02a1e254244b
94c7364692188ef8ef531518cf74a9fca9728a2aa5d4b3e96a01bb7b82219171
O=C1CCC2CC12
C-[S+](-C)-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5].[O;D1;H0:6]=[C:7]1-[C:8]-[C:9]-[CH;D2;+0:10]=[CH;D2;+0:11]-1>>[C:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[CH;D3;+0:1]1-[CH;D3;+0:11]2-[C:7](=[O;D1;H0:6])-[C:8]-[C:9]-[CH;D3;+0:10]-2-1
68.3
[{"value": 68.3, "product": "O=C1C2C(C2CC1)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A suspension of carboethoxymethyl dimethylsulfonium bromide (45.5 g) in toluene (350 mL) was treated with 1,8-diazabicyclo[5.4.0]undec-7-ene (30.2 g). The resulting mixture was stirred at room temperature. After one hour, the reaction mixture was treated with 2-cyclopenten-1-one (19.57 g). After an additional 18 hours,...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester
Ketone.Ester
C1=CCCC1
C1CC2CC2C1
C1CC2CC2C1
Other
C1(=CC=CC=C1)C
null
1
CCOC(=O)C[S+](C)C.O=C1C=CCC1>C1(=CC=CC=C1)C>CCOC(=O)C1C2CCC(=O)C21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-07beb0ec388f43cd9ac71486ee726a73
CCOC(=O)C1C2CCC(=O)C21>>O=C(O)C1C2CCC(=O)C21
O=C1C2C(C2CC1)C(=O)OCC.Cl>>O=C1C2C(C2CC1)C(=O)O
CC[O:3][C:2](=[O:1])[CH:4]1[CH:5]2[CH2:6][CH2:7][C:8](=[O:9])[CH:10]12>>[O:1]=[C:2]([OH:3])[CH:4]1[CH:5]2[CH2:6][CH2:7][C:8](=[O:9])[CH:10]12
CCOC(=O)C1C2CCC(=O)C21
O=C(O)C1C2CCC(=O)C21
null
null
[OH-].[Na+]
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C1CCC2CC12
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
2.5
HOUR
A mixture of 60 g of ethyl 2-oxobicyclo[3.1.0]hexane-6-carboxylate and 300 ml of 1N sodium hydroxide was stirred at 25°-30° C. After 2.5 hours, concentrated hydrochloric acid was added to adjust the pH to 0.8-1.2. The resulting solution was extracted with ethyl acetate. The extracts were dried over magnesium sulfate, f...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
C1CC2CC2C1
Other
[OH-].[Na+]
null
2.5
CCOC(=O)C1C2CCC(=O)C21>[OH-].[Na+]>O=C(O)C1C2CCC(=O)C21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8b32fa3382184901ae70790edf4034ba
CC(Br)C(=O)Br.CNc1cccc(OC)c1>>COc1cccc(N(C)C(=O)C(C)Br)c1
CNC=1C=C(OC)C=CC1.C(C)N(CC)CC.C1(=CC=CC=C1)C.BrC(C(=O)Br)C>>BrC(C(=O)N(C)C1=CC(=CC=C1)OC)C
Br[C:10](=[O:11])[CH:12]([CH3:13])[Br:14].[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][CH3:9])[cH:15]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([N:8]([CH3:9])[C:10](=[O:11])[CH:12]([CH3:13])[Br:14])[cH:15]1
CC(Br)C(=O)Br.CNc1cccc(OC)c1
COc1cccc(N(C)C(=O)C(C)Br)c1
null
null
O
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
c1ccccc1
Br-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[Br;D1;H0:4])-[C;D1;H3:5].[C;D1;H3:6]-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]>>[Br;D1;H0:4]-[C:3](-[C;D1;H3:5])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:7](-[C;D1;H3:6])-[c:8](:[c:9]):[c:10]
null
[]
null
null
8
HOUR
A solution of N-methyl-m-anisidine (265 g), triethylamine (269 ml) and toluene (550 ml) was stirred at 0° C. as 2-bromopropionyl bromide (202.6 ml) was added dropwise. The mixture was mechanically stirred overnight at room temperature. Water was added to the reaction and the aqueous layer was collected and extracted wi...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccccc1
HBr
O
null
8
CC(Br)C(=O)Br.CNc1cccc(OC)c1>O>COc1cccc(N(C)C(=O)C(C)Br)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-81f17a5f0c63408184ecd6ae2c164668
COc1cc2c(cc1Br)[C@]1(C)CCN(C)[C@@H]1N2C>>CN1CC[C@@]2(C)c3cc(Br)c(O)cc3N(C)[C@@H]12
BrC=1C=C2[C@]3([C@@H](N(C2=CC1OC)C)N(CC3)C)C.B(Br)(Br)Br>>BrC=1C=C2[C@]3([C@@H](N(C2=CC1O)C)N(CC3)C)C
C[O:12][c:11]1[c:9]([Br:10])[cH:8][c:7]2[c:14]([cH:13]1)[N:15]([CH3:16])[C@H:17]1[N:2]([CH3:1])[CH2:3][CH2:4][C@@:5]21[CH3:6]>>[CH3:1][N:2]1[CH2:3][CH2:4][C@@:5]2([CH3:6])[c:7]3[cH:8][c:9]([Br:10])[c:11]([OH:12])[cH:13][c:14]3[N:15]([CH3:16])[C@@H:17]12
COc1cc2c(cc1Br)[C@]1(C)CCN(C)[C@@H]1N2C
CN1CC[C@@]2(C)c3cc(Br)c(O)cc3N(C)[C@@H]12
null
null
C(Cl)Cl
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
c1ccc2c(c1)N[C@H]1NCCC21
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
8
HOUR
cis-(±)-5-Bromo-1,2,3,3a,8,8a-hexahydro-6-methoxy- 1,3a,8-trimethyl-pyrrolo[2,3-b]indole (11 g) was dissolved in dry DCM (200 ml) and added dropwise at 0° C. to a stirred solution of BBr3 in DCM (300 ml). The mixture was warmed to room temperature and stirred overnight under nitrogen. The mixture was quenched with aq. ...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccc2c(c1)[NH][C@H]1[NH]CC[C@@H]21
Other
C(Cl)Cl
null
8
COc1cc2c(cc1Br)[C@]1(C)CCN(C)[C@@H]1N2C>C(Cl)Cl>CN1CC[C@@]2(C)c3cc(Br)c(O)cc3N(C)[C@@H]12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0f8c43802c60460ab93e17f76623a594
CC1C(=O)N(C)c2cccc(O)c21.COS(=O)(=O)OC>>COc1cccc2c1C(C)C(=O)N2C
OC1=C2C(C(N(C2=CC=C1)C)=O)C.C([O-])([O-])=O.[K+].[K+].COS(=O)(=O)OC>>COC1=C2C(C(N(C2=CC=C1)C)=O)C
[OH:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]1[CH:9]([CH3:10])[C:11](=[O:12])[N:13]2[CH3:14].COS(=O)(=O)O[CH3:1]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]1[CH:9]([CH3:10])[C:11](=[O:12])[N:13]2[CH3:14]
CC1C(=O)N(C)c2cccc(O)c21.COS(=O)(=O)OC
COc1cccc2c1C(C)C(=O)N2C
null
null
CC(=O)C
Heteroatom Alkylation and Arylation
Methylation of OH with DMS
b8b041187bac58376aae824630608e7deb49a01db3d652291f8b379c10d4e434
0f0966e3597a58033417ecee71659f4d0c082f95d46b1e52c95541e6e4a59086
O=C1Cc2ccccc2N1
C-O-S(=O)(=O)-O-[CH3;D1;+0:1].[OH;D1;+0:2]-[c:3](:[c:4]):[c:5]>>[CH3;D1;+0:1]-[O;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]
86.2
[{"value": 86.2, "product": "COC1=C2C(C(N(C2=CC=C1)C)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A slurry of 1,3-dihydro-4-hydroxy-1,3-dimethyl-2H-indol-2-one (50 g), milled potassium carbonate (60.1 g) and HPLC grade acetone (400 ml) was mechanically stirred at room temperature as dimethylsulfate (41.4 ml) was added dropwise. The addition funnel was replaced with a condenser and the slurry was refluxed for 18 hou...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol
Ether
null
null
c1ccc2c(c1)CC[NH]2
HO-
CC(=O)C
null
null
CC1C(=O)N(C)c2cccc(O)c21.COS(=O)(=O)OC>CC(=O)C>COc1cccc2c1C(C)C(=O)N2C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-cb9d1bc99b9b4ab18c65744a87225d92
CC(N=C=O)c1ccccc1.CN1CC[C@@]2(C)c3c(O)cccc3N(C)[C@@H]12>>C[C@@H](NC(=O)Oc1cccc2c1[C@@]1(C)CCN(C)[C@H]1N2C)c1ccccc1
CN1CC[C@@]2([C@H]1N(C=1C=CC=C(C21)O)C)C.C1CCC2=NCCCN2CC1.CC(C1=CC=CC=C1)N=C=O>>C[C@H](C1=CC=CC=C1)NC(OC1=C2[C@@]3([C@H](N(C2=CC=C1)C)N(CC3)C)C)=O
[CH3:1][CH:2]([N:3]=[C:4]=[O:5])[c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1.[OH:6][c:7]1[cH:8][cH:9][cH:10][c:11]2[c:12]1[C@:13]1([CH3:14])[CH2:15][CH2:16][N:17]([CH3:18])[C@@H:19]1[N:20]2[CH3:21]>>[CH3:1][C@@H:2]([NH:3][C:4](=[O:5])[O:6][c:7]1[cH:8][cH:9][cH:10][c:11]2[c:12]1[C@@:13]1([CH3:14])[CH2:15][CH2:16][N:17]([...
CC(N=C=O)c1ccccc1.CN1CC[C@@]2(C)c3c(O)cccc3N(C)[C@@H]12
C[C@@H](NC(=O)Oc1cccc2c1[C@@]1(C)CCN(C)[C@H]1N2C)c1ccccc1
null
null
C1CCOC1
Protection
OtherReaction
1cd060f96f1d4acffc14539274a5df6a214938373877da5ea80bcb2e30d74918
55864cdc06e9526eaed7216ed2cc57ef652f1657070e16ae5b01f42ad254cf4b
O=C(NCc1ccccc1)Oc1cccc2c1C1CCN[C@H]1N2
[C;D1;H3:1]-[CH;D3;+0:2](-[N;H0;D2;+0:3]=[C;H0;D2;+0:4]=[O;D1;H0:5])-[c:6](:[c:7]):[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[C;D1;H3:1]-[C@@H;D3;+0:2](-[NH;D2;+0:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[O;H0;D2;+0:9]-[c:10](:[c:11]):[c:12])-[c:6](:[c:7]):[c:8]
null
[]
null
null
8
HOUR
cis-(±)-1,2,3,3a,8,8a-Hexahydro-1,3a,8-trimethylpyrrolo [2,3-b]indol-4-ol (2g) was dissolved in degassed THF (200 ml). DBU (0.8 ml) was added to the mixture followed by R-(+)-α-methylbenzyl isocyanate (2 g). The reaction was stirred at room temperature overnight under nitrogen. The solvent was evaporated under reduced ...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Aromatic alcohol
Carbamic ester
null
null
c1ccc2c(c1)[NH][C@@H]1[NH]CC[C@H]21.c1ccccc1
null
C1CCOC1
null
8
CC(N=C=O)c1ccccc1.CN1CC[C@@]2(C)c3c(O)cccc3N(C)[C@@H]12>C1CCOC1>C[C@@H](NC(=O)Oc1cccc2c1[C@@]1(C)CCN(C)[C@H]1N2C)c1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-157fb9c3937847cf98e7bf4bb5a1bfb6
CC(C)(C)C(=O)OCCl.CC(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>>CC(C)CN1C(=O)[C@@H](CC(=O)OCOC(=O)C(C)(C)C)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)C)=O)CC(=O)O)C2=C(C=CC=C2)Cl)C1.C(C(C)(C)C)(=O)OCCl.C(C(C)C)N(CC(C)C)CC.O>>C(C(C)(C)C)(=O)OCOC(C[C@@H]1C(N(C2=C([C@H](O1)C1=C(C=CC=C1)Cl)C=C(C=C2)Cl)CC(C)C)=O)=O
Cl[CH2:13][O:14][C:15](=[O:16])[C:17]([CH3:18])([CH3:19])[CH3:20].[CH3:1][CH:2]([CH3:3])[CH2:4][N:5]1[C:6](=[O:7])[C@@H:8]([CH2:9][C:10](=[O:11])[OH:12])[O:21][C@H:22]([c:23]2[cH:24][cH:25][cH:26][cH:27][c:28]2[Cl:29])[c:30]2[cH:31][c:32]([Cl:33])[cH:34][cH:35][c:36]21>>[CH3:1][CH:2]([CH3:3])[CH2:4][N:5]1[C:6](=[O:7])[...
CC(C)(C)C(=O)OCCl.CC(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
CC(C)CN1C(=O)[C@@H](CC(=O)OCOC(=O)C(C)(C)C)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
null
CN(C=O)C.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
d0f2e7dd04291aff91491624f6ba09bd6ae2852adc109edeabfddd534d9ccfd8
ebb133741743004d799d6738504ddfd5b4a53248a4f85602c0fff1c33566ad58
O=C1CO[C@H](c2ccccc2)c2ccccc2N1
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3](-[C:4])=[O;D1;H0:5].[C:6]-[C:7](=[O;D1;H0:8])-[OH;D1;+0:9]>>[C:4]-[C:3](=[O;D1;H0:5])-[#8:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:9]-[C:7](-[C:6])=[O;D1;H0:8]
null
[]
null
null
8
HOUR
In N,N-dimethylformamide (10 ml) was dissolved trans- 7-chloro-5-(2-chlorophenyl)-1-isobutyl-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-acetic acid (0.5 g) obtained in Example 2. To the solution were added pivaloyloxymethyl chloride (0.43 ml), N,N-diisobutyl ethylamine (0.52 ml) and KI (0.2 g). The mixture was stirre...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester.Ester
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2
HCl
CN(C=O)C.C(C)(=O)OCC
null
8
CC(C)(C)C(=O)OCCl.CC(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>CN(C=O)C.C(C)(=O)OCC>CC(C)CN1C(=O)[C@@H](CC(=O)OCOC(=O)C(C)(C)C)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8208d819f879448fbecf7d2aa5f1ad04
COc1ccc(C=O)c(OC)c1.Nc1ccc(Cl)cc1C(O)c1ccccc1Cl>>COc1ccc(CNc2ccc(Cl)cc2C(O)c2ccccc2Cl)c(OC)c1
O.NC1=C(C(C2=C(C=CC=C2)Cl)O)C=C(C=C1)Cl.COC1=C(C=O)C=CC(=C1)OC.[BH4-].[Na+]>>ClC=1C=CC(=C(C(C2=C(C=CC=C2)Cl)O)C1)NCC1=C(C=C(C=C1)OC)OC
O=[CH:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:28][c:25]1[O:26][CH3:27].[NH2:8][c:9]1[cH:10][cH:11][c:12]([Cl:13])[cH:14][c:15]1[CH:16]([OH:17])[c:18]1[cH:19][cH:20][cH:21][cH:22][c:23]1[Cl:24]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][NH:8][c:9]2[cH:10][cH:11][c:12]([Cl:13])[cH:14][c:15]2[CH:16]([OH:17])[c:18]2[c...
COc1ccc(C=O)c(OC)c1.Nc1ccc(Cl)cc1C(O)c1ccccc1Cl
COc1ccc(CNc2ccc(Cl)cc2C(O)c2ccccc2Cl)c(OC)c1
null
null
C(C)(=O)O
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
c1ccc(CNc2ccccc2Cc2ccccc2)cc1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[c:7]:[c:6](-[NH;D2;+0:5]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]):[c:8]
96.1
[{"value": 96.1, "product": "ClC=1C=CC(=C(C(C2=C(C=CC=C2)Cl)O)C1)NCC1=C(C=C(C=C1)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 2-amino-5-chloro-α-(2-chloro phenyl)benzyl alcohol (5.0 g) and 2,4-dimethoxy benzaldehyde (3.72 g) in acetic acid (50 ml) was added, under ice-cooling, sodium borohydride (0.94 g). The mixture was stirred for one hour at room temperature, which was poured into water (200 ml), followed by extraction wit...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccccc1.c1ccccc1
Other
C(C)(=O)O
null
1
COc1ccc(C=O)c(OC)c1.Nc1ccc(Cl)cc1C(O)c1ccccc1Cl>C(C)(=O)O>COc1ccc(CNc2ccc(Cl)cc2C(O)c2ccccc2Cl)c(OC)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c2d7b50a1bd84d1e8cef8cf871d36f05
O=C1CCC(C(=O)O)O1.O=S(Cl)Cl>>O=C1CCC(C(=O)Cl)O1
O=C1CCC(O1)C(=O)O.S(=O)(Cl)Cl>>O=C1CCC(O1)C(=O)Cl
O[C:6]([CH:5]1[CH2:4][CH2:3][C:2](=[O:1])[O:9]1)=[O:7].O=S(Cl)[Cl:8]>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([C:6](=[O:7])[Cl:8])[O:9]1
O=C1CCC(C(=O)O)O1.O=S(Cl)Cl
O=C1CCC(C(=O)Cl)O1
null
null
null
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
O=C1CCCO1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[C:4](-[C:5])-[#8:6]-[C:7]=[O;D1;H0:8]>>[C:5]-[C:4](-[C;H0;D3;+0:2](-[Cl;H0;D1;+0:1])=[O;D1;H0:3])-[#8:6]-[C:7]=[O;D1;H0:8]
null
[]
null
null
null
null
A mixture of 4.9 g of 5-oxotetrahydrofuran-2-carboxylic acid and 5.5 ml of thionyl chloride was subjected to reflux for 2 hours. Thionyl chloride was then distilled off under reduced pressure to leave 5-oxotetrahydrofuran-2-carbonyl chloride. This product was mixed with 5.0 g of 2-aminobenzophenone, 200 ml of ethyl ace...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
C1CCOC1
HCl
null
null
null
O=C1CCC(C(=O)O)O1.O=S(Cl)Cl>>O=C1CCC(C(=O)Cl)O1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-947d3e4afae94a0b8dd4f97535b58d90
Nc1ccccc1C(=O)c1ccccc1.O=C([O-])O>>O=C1CCC(C(=O)Nc2ccccc2C(=O)c2ccccc2)O1
NC1=C(C(=O)C2=CC=CC=C2)C=CC=C1.C(O)([O-])=O.[Na+]>>O=C1CCC(O1)C(=O)NC1=C(C(=O)C2=CC=CC=C2)C=CC=C1
[cH:2]1[c:17]([C:15]([c:14]2[c:9]([NH2:8])[cH:10][cH:11][cH:12][cH:13]2)=[O:16])[cH:18][cH:19][cH:20][cH:21]1.[O-:1][C:6](=[O:7])[OH:23]>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[C:15](=[O:16])[c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[O:23]1
Nc1ccccc1C(=O)c1ccccc1.O=C([O-])O
O=C1CCC(C(=O)Nc2ccccc2C(=O)c2ccccc2)O1
null
null
C(C)(=O)OCC
Aromatic Heterocycle Formation
OtherReaction
3b8ba0f8d519b260eb86a1b85cbd2a09fe48860e12a159295ca3a0782b453820
8ce2a5a806393bd18c953b6c97fbcdd6719072ce11d36a47b3c99f1b34ed4c0a
O=C1CCC(C(=O)Nc2ccccc2C(=O)c2ccccc2)O1
[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]-[C:5](=[O;D1;H0:6])-[c;H0;D3;+0:7]1:[c:8]:[c:9]:[c:10]:[cH;D2;+0:11]:[cH;D2;+0:12]:1.[O-;H0;D1:13]-[C;H0;D3;+0:14](=[O;D1;H0:15])-[OH;D1;+0:16]>>[O;D1;H0:6]=[C:5](-[c:4]:[c:2](-[NH;D2;+0:1]-[C;H0;D3;+0:14](=[O;D1;H0:15])-[C:17]1-[C:18]-[C:19]-[C;H0;D3;+0:12](=[O;H0;D1;+0:13])-[O;H0;D2;...
null
[]
null
null
1
HOUR
A mixture of 4.9 g of 5-oxotetrahydrofuran-2-carboxylic acid and 5.5 ml of thionyl chloride was subjected to reflux for 2 hours. Thionyl chloride was then distilled off under reduced pressure to leave 5-oxotetrahydrofuran-2-carbonyl chloride. This product was mixed with 5.0 g of 2-aminobenzophenone, 200 ml of ethyl ace...
10.6084/m9.figshare.5104873.v1
null
Carbonic Acid.Ketone.Primary amine
Ketone.Ester.Secondary amide
c1ccccc1
C1CCOC1.c1ccccc1
C1CCOC1.c1ccccc1.c1ccccc1
null
C(C)(=O)OCC
null
1
Nc1ccccc1C(=O)c1ccccc1.O=C([O-])O>C(C)(=O)OCC>O=C1CCC(C(=O)Nc2ccccc2C(=O)c2ccccc2)O1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b0c5b510b8454987be8e23400859a420
Nc1ccc(Cl)cc1C(=O)c1ccccc1Cl.O=C1CCC(C(=O)Cl)O1>>O=C1CCC(C(=O)Nc2ccc(Cl)cc2C(=O)c2ccccc2Cl)O1
NC1=C(C(=O)C2=C(C=CC=C2)Cl)C=C(C=C1)Cl.O=C1CCC(O1)C(=O)Cl>>ClC1=C(C=CC=C1)C(C1=C(C=CC(=C1)Cl)NC(=O)C1OC(CC1)=O)=O
[NH2:8][c:9]1[cH:10][cH:11][c:12]([Cl:13])[cH:14][c:15]1[C:16](=[O:17])[c:18]1[cH:19][cH:20][cH:21][cH:22][c:23]1[Cl:24].Cl[C:6]([CH:5]1[CH2:4][CH2:3][C:2](=[O:1])[O:25]1)=[O:7]>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12]([Cl:13])[cH:14][c:15]2[C:16](=[O:17])[c:18]2[cH:19][cH:20][cH:...
Nc1ccc(Cl)cc1C(=O)c1ccccc1Cl.O=C1CCC(C(=O)Cl)O1
O=C1CCC(C(=O)Nc2ccc(Cl)cc2C(=O)c2ccccc2Cl)O1
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C1CCC(C(=O)Nc2ccccc2C(=O)c2ccccc2)O1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#8:5]-[C:6]=[O;D1;H0:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]-[C:12]=[O;D1;H0:13]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]-[C:12]=[O;D1;H0:13])-[#8:5]-[C:6]=[O;D1;H0:7]
null
[]
null
null
null
null
In substantially the same manner as in Example 8 (1), 15 g of 2-amino-2',5-dichlorobenzophenone was allowed to react with 5-oxotetrahydrofuran-2-carbonyl chloride to afford 18.1 g of 2',5-dichloro-2-(5-oxotetrahydrofuran-2-carbonyl) aminobenzophenone, m.p. 170° C.-173° C. Conditions: See reaction.notes.procedure_detail...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
C1CCOC1.c1ccccc1.c1ccccc1
HCl
null
null
null
Nc1ccc(Cl)cc1C(=O)c1ccccc1Cl.O=C1CCC(C(=O)Cl)O1>>O=C1CCC(C(=O)Nc2ccc(Cl)cc2C(=O)c2ccccc2Cl)O1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9e9ed99cddf843adaf7a03857e42c160
COc1ccc(C(=O)c2ccccc2N)cc1.O=C1CCC(C(=O)Cl)O1>>COc1ccc(C(=O)c2ccccc2NC(=O)C2CCC(=O)O2)cc1
NC1=C(C(=O)C2=CC=C(C=C2)OC)C=CC=C1.O=C1CCC(O1)C(=O)Cl>>COC1=CC=C(C=C1)C(C1=C(C=CC=C1)NC(=O)C1OC(CC1)=O)=O
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[NH2:15])[cH:24][cH:25]1.Cl[C:16](=[O:17])[CH:18]1[CH2:19][CH2:20][C:21](=[O:22])[O:23]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[NH:15][C:16](=[O:17])[CH:18]2[CH2:19][CH2:20][C:2...
COc1ccc(C(=O)c2ccccc2N)cc1.O=C1CCC(C(=O)Cl)O1
COc1ccc(C(=O)c2ccccc2NC(=O)C2CCC(=O)O2)cc1
null
null
null
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C1CCC(C(=O)Nc2ccccc2C(=O)c2ccccc2)O1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#8:5]-[C:6]=[O;D1;H0:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]-[C:12]=[O;D1;H0:13]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]-[C:12]=[O;D1;H0:13])-[#8:5]-[C:6]=[O;D1;H0:7]
null
[]
null
null
null
null
In substantially the same manner as in Example 8 (1), 8 g of 2-amino-4'-methoxybenzophenone was allowed to react with 5-oxotetrahydrofuran-2-carbonyl chloride to give 12 g of 4'-methoxy-2-(5-oxotetrahydrofuran-2-carbonyl)aminobenzophenone as an oily product. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.C1CCOC1
HCl
null
null
null
COc1ccc(C(=O)c2ccccc2N)cc1.O=C1CCC(C(=O)Cl)O1>>COc1ccc(C(=O)c2ccccc2NC(=O)C2CCC(=O)O2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9645ae5ef13440c58b9e8e3877a34a9d
COC(=O)C(C)CC(Cl)C(=O)O.O=S(Cl)Cl>>COC(=O)CCC(Cl)C(=O)Cl
ClC(C(=O)O)CC(C)C(=O)OC.S(=O)(Cl)Cl>>ClC(C(=O)Cl)CCC(=O)OC
C[CH:5]([C:3]([O:2][CH3:1])=[O:4])[CH2:6][CH:7]([Cl:8])[C:9](O)=[O:10].O=S(Cl)[Cl:11]>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][CH:7]([Cl:8])[C:9](=[O:10])[Cl:11]
COC(=O)C(C)CC(Cl)C(=O)O.O=S(Cl)Cl
COC(=O)CCC(Cl)C(=O)Cl
null
null
C1(=CC=CC=C1)C
Functional Group Interconversion
OtherReaction
71853bac5dd0732e3d60bec8e19996dc831d229d490544ad9bbbb3710b2dc130
f24a3ae28a4ec4bb4dccac7a59b48cf750266c146d0631e1527a9b06ebcd084a
null
C-[CH;D3;+0:1](-[C:2]-[C:3](-[Cl;D1;H0:4])-[C;H0;D3;+0:5](-O)=[O;D1;H0:6])-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10].Cl-S(=O)-[Cl;H0;D1;+0:11]>>[C;D1;H3:10]-[#8:9]-[C:7](=[O;D1;H0:8])-[CH2;D2;+0:1]-[C:2]-[C:3](-[Cl;D1;H0:4])-[C;H0;D3;+0:5](-[Cl;H0;D1;+0:11])=[O;D1;H0:6]
null
[]
80
CELSIUS
30
MINUTE
A mixture of 7.6 g of 2-chloro-4-methoxycarbonyl valeric acid, 9.2 ml of thionyl chloride and 30 ml of toluene was stirred for 30 minutes at 80° C., followed by distilling off the solvent under reduced pressure to leave 2-chloro-4-methoxycarbonyl butyryl chloride. A mixture of this compound, 5.0 g of 2-benzylaminobenzo...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ester
Acyl halide.Ester
null
null
null
HCl
C1(=CC=CC=C1)C
80
0.5
COC(=O)C(C)CC(Cl)C(=O)O.O=S(Cl)Cl>C1(=CC=CC=C1)C>COC(=O)CCC(Cl)C(=O)Cl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a9d5932f47fc470faf0612928f6d7003
COC(=O)C(C)CC(Cl)C(=O)O.O=S(Cl)Cl>>COC(=O)CCC(Cl)C(=O)Cl
ClC(C(=O)O)CC(C)C(=O)OC.S(=O)(Cl)Cl>>ClC(C(=O)Cl)CCC(=O)OC
C[CH:5]([C:3]([O:2][CH3:1])=[O:4])[CH2:6][CH:7]([Cl:8])[C:9](O)=[O:10].O=S(Cl)[Cl:11]>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][CH:7]([Cl:8])[C:9](=[O:10])[Cl:11]
COC(=O)C(C)CC(Cl)C(=O)O.O=S(Cl)Cl
COC(=O)CCC(Cl)C(=O)Cl
null
null
null
Functional Group Interconversion
OtherReaction
71853bac5dd0732e3d60bec8e19996dc831d229d490544ad9bbbb3710b2dc130
f24a3ae28a4ec4bb4dccac7a59b48cf750266c146d0631e1527a9b06ebcd084a
null
C-[CH;D3;+0:1](-[C:2]-[C:3](-[Cl;D1;H0:4])-[C;H0;D3;+0:5](-O)=[O;D1;H0:6])-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10].Cl-S(=O)-[Cl;H0;D1;+0:11]>>[C;D1;H3:10]-[#8:9]-[C:7](=[O;D1;H0:8])-[CH2;D2;+0:1]-[C:2]-[C:3](-[Cl;D1;H0:4])-[C;H0;D3;+0:5](-[Cl;H0;D1;+0:11])=[O;D1;H0:6]
null
[]
null
null
null
null
A mixture of 6.2 g of 2-chloro-4-methoxycarbonyl valeric acid and 12.6 ml of thionyl chloride was refluxed for 30 minutes, then the solvent was distilled off under reduced pressure to leave 2-chloro-4-methoxycarbonyl butyryl chloride. A mixture of this product, 5.0 g of 2-benzylaminodiphenyl methanol, 100 ml of ethyl a...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ester
Acyl halide.Ester
null
null
null
HCl
null
null
null
COC(=O)C(C)CC(Cl)C(=O)O.O=S(Cl)Cl>>COC(=O)CCC(Cl)C(=O)Cl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b5522d18fb004b81842dc376c274bba5
COc1ccc(CN2C(=O)[C@@H](CC(=O)O)O[C@H](c3ccccc3Cl)c3cc(Cl)ccc32)c(OC)c1>>O=C(O)CC[C@H]1O[C@@H](c2ccccc2)c2ccccc2N(Cc2ccccc2)C1=O
Cl.ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC2=C(C=C(C=C2)OC)OC)=O)CC(=O)O)C2=C(C=CC=C2)Cl)C1.[OH-].[Na+]>>C(C1=CC=CC=C1)N1C([C@H](O[C@H](C2=C1C=CC=C2)C2=CC=CC=C2)CCC(=O)O)=O
CO[c:2]1[cH:25][c:24](O[CH3:26])[c:23]([CH2:22][N:21]2[c:20]3[c:15]([cH:16][c:17](Cl)[cH:18][cH:19]3)[C@@H:8]([c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]3Cl)[O:7][C@H:6]([CH2:5][C:4](=[O:1])[OH:3])[C:29]2=[O:30])[cH:28][cH:27]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][C@H:6]1[O:7][C@@H:8]([c:9]2[cH:10][cH:11][cH:12][cH:13][cH:1...
COc1ccc(CN2C(=O)[C@@H](CC(=O)O)O[C@H](c3ccccc3Cl)c3cc(Cl)ccc32)c(OC)c1
O=C(O)CC[C@H]1O[C@@H](c2ccccc2)c2ccccc2N(Cc2ccccc2)C1=O
null
null
CO
Miscellaneous
OtherReaction
43bebc7a1611e70b5b5e71e81d8b4d741d8b8d1e70d6756d788764865343cbfc
4ec579fe1c565a8ac8dd28a6e233bf9ed5ac66403ad6d60a497ae7f2aaa21688
O=C1CO[C@@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
C-O-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[c;H0;D3;+0:3](-O-[CH3;D1;+0:4]):[c:5](-[C:6]-[#7:7]-[C:8](=[O;D1;H0:9])-[C:10](-[C:11]-[C;H0;D3;+0:12](=[O;H0;D1;+0:13])-[OH;D1;+0:14])-[#8:15]-[C:16](-[c:17](:[c:18]):[c;H0;D3;+0:19](-Cl):[c:20]:[c:21])-[c:22]:[c:23]:[c;H0;D3;+0:24](-Cl):[c:25]:[c:26]):[c:27]:[cH;D2;+0:28]:1>>[O;D1;H0...
null
[]
null
null
30
MINUTE
In 20 ml of methanol was dissolved 0.5 g of ethyl ester of cis-1-benzyl-2-oxo-5-phenyl-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-propionic acid obtained in Example 8. To the solution was added 7 ml of 1N sodium hydroxide, and the mixture was stirred for 30 minutes at room temperature. The reaction mixture was acidified wi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Carboxylic acid.Ether.Ether
Carboxylic acid
c1ccccc1.c1ccccc1.c1ccc2c(c1)COCC[NH]2
c1ccccc1.c1ccc2c(c1)COCC[NH]2.c1ccccc1
c1ccccc1.c1ccc2c(c1)COCC[NH]2.c1ccccc1
Other
CO
null
0.5
COc1ccc(CN2C(=O)[C@@H](CC(=O)O)O[C@H](c3ccccc3Cl)c3cc(Cl)ccc32)c(OC)c1>CO>O=C(O)CC[C@H]1O[C@@H](c2ccccc2)c2ccccc2N(Cc2ccccc2)C1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-14c74de0439b4c7ab9a7a1cfbae36b8f
O=C(O)CC[C@H]1O[C@H](c2ccccc2)c2ccccc2N(Cc2ccccc2)C1=O>>O=C1[C@@H](CCCO)O[C@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC=C2)C2=CC=CC=C2)CCC(=O)O)=O.[BH4-].[Na+].[Cl-].[Li+].Cl>>C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC=C2)C2=CC=CC=C2)CCCO)=O
O=[C:6]([CH2:5][CH2:4][C@@H:3]1[C:2](=[O:1])[N:22]([CH2:23][c:24]2[cH:25][cH:26][cH:27][cH:28][cH:29]2)[c:21]2[c:16]([cH:17][cH:18][cH:19][cH:20]2)[C@@H:9]([c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[O:8]1)[OH:7]>>[O:1]=[C:2]1[C@@H:3]([CH2:4][CH2:5][CH2:6][OH:7])[O:8][C@H:9]([c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2...
O=C(O)CC[C@H]1O[C@H](c2ccccc2)c2ccccc2N(Cc2ccccc2)C1=O
O=C1[C@@H](CCCO)O[C@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
null
null
C(C)O.C(C)(=O)OCC.O1CCCC1
Reduction
Reduction of carboxylic acid to primary alcohol
0db83a5ebe1e318b78b55461cf7eb8f7c004eef0f9e3b6666d3df4c96b5f665e
93b4621647b04d2ad2f2825215b1567f171ba61fe10d136b5db6ea0470aa4932
O=C1CO[C@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
O=[C;H0;D3;+0:1](-[O;D1;H1:2])-[C:3]-[C:4]>>[C:4]-[C:3]-[CH2;D2;+0:1]-[O;D1;H1:2]
null
[]
null
null
10
MINUTE
The mixture of 0.4 g of methyl ester of trans-1-benzyl2-oxo-5-phenyl-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-propionic acid obtained in Example 12, 0.16 g of sodium borohydride and 0.16 g of lithium chloride in 15 ml of tetrahydrofuran were stirred for 10 minutes at room temperature. To the resultant was added 30 ml of ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary alcohol
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2.c1ccccc1
Other
C(C)O.C(C)(=O)OCC.O1CCCC1
null
0.166667
O=C(O)CC[C@H]1O[C@H](c2ccccc2)c2ccccc2N(Cc2ccccc2)C1=O>C(C)O.C(C)(=O)OCC.O1CCCC1>O=C1[C@@H](CCCO)O[C@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b53797564a374067960a6e48c29544d3
O=C(O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1>>Cl.NC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC(=C2)Cl)C2=C(C=CC=C2)Cl)CC(=O)O)=O.C(C)N(CC)CC.C1(=CC=CC=C1)P(=O)(C1=CC=CC=C1)N=[N+]=[N-]>>Cl.C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC(=C2)Cl)C2=C(C=CC=C2)Cl)CN)=O
O=C(O)[CH2:3][C@H:4]1[O:5][C@H:6]([c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[Cl:1])[c:14]2[cH:15][c:16]([Cl:17])[cH:18][cH:19][c:20]2[N:21]([CH2:22][c:23]2[cH:24][cH:25][cH:26][cH:27][cH:28]2)[C:29]1=[O:30].[N-]=[N+]=[N:2]P(=O)(c1ccccc1)c1ccccc1>>[ClH:1].[NH2:2][CH2:3][C@H:4]1[O:5][C@H:6]([c:7]2[cH:8][cH:9][cH:10][cH:11][...
O=C(O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1
Cl.NC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
1f1b04abeaffa1cd0dbeadbc846df91a86d79cd0794def0b7d63e085a5b52d11
ace9751e95272b0dafda873c7583ab20489d68697a41c7be5b84ad07fe14a502
O=C1CO[C@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
O-C(=O)-[CH2;D2;+0:1]-[C:2](-[#8:3]-[C:4]-[c:5](:[c:6]):[c;H0;D3;+0:7](-[Cl;H0;D1;+0:8]):[c:9]:[c:10])-[C:11](=[O;D1;H0:12])-[#7:13](-[C:14])-[c:15].O=P(-[N;H0;D2;+0:16]=[N+]=[N-])(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[C:14]-[#7:13](-[c:15])-[C:11](=[O;D1;H0:12])-[C:2](-[CH2;D2;+0:1]-[NH2;D1;+0:16])-[#8:3]-[C:4]-[c:5](:[c:...
null
[]
null
null
null
null
In 5 ml of dimethylformamide was dissolved 1.0 g of trans-1-benzyl-7-chloro-5-(2-chlorophenyl)-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-acetic acid obtained obtained in Reference Example 5. To the solution was added 0.3 ml of triethylamine, to which was added dropwise, while stirring under ice-cooling, 0.6 g of dip...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carboxylic acid.Azide
Aromatic halide.Primary amine
c1ccccc1.c1ccccc1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccc2c(c1)COCC[NH]2.c1ccccc1
HO-
CN(C=O)C
null
null
O=C(O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1>CN(C=O)C>Cl.NC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e1cdebf350904ceba1f779d1bab6a752
C=O.O=C(O)CNC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O>>CN(CC(=O)O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC(=C2)Cl)C2=C(C=CC=C2)Cl)CNCC(=O)O)=O.C=O.C(C(=O)O)(=O)O>>C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC(=C2)Cl)C2=C(C=CC=C2)Cl)CN(CC(=O)O)C)=O
O=[CH2:1].[NH:2]([CH2:3][C:4](=[O:5])[OH:6])[CH2:7][C@H:8]1[O:9][C@H:10]([c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]2[Cl:17])[c:18]2[cH:19][c:20]([Cl:21])[cH:22][cH:23][c:24]2[N:25]([CH2:26][c:27]2[cH:28][cH:29][cH:30][cH:31][cH:32]2)[C:33]1=[O:34]>>[CH3:1][N:2]([CH2:3][C:4](=[O:5])[OH:6])[CH2:7][C@H:8]1[O:9][C@H:10]([c:...
C=O.O=C(O)CNC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
CN(CC(=O)O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
null
null
null
Heteroatom Alkylation and Arylation
Eschweiler-Clarke Secondary Amine Methylation
deb0f39510ff32c3bd75ceaf7ece4070b1f686ff120d798ccd640765025dab3c
e1fdef8fde1c506d7c9deb8fd5e6f322eceea2abce3167abcf412a1fa4fd5443
O=C1CO[C@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
O=[CH2;D1;+0:1].[#7:2]-[C:3](=[O;D1;H0:4])-[C:5](-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9](=[O;D1;H0:10])-[O;D1;H1:11])-[#8:12]>>[#7:2]-[C:3](=[O;D1;H0:4])-[C:5](-[C:6]-[N;H0;D3;+0:7](-[CH3;D1;+0:1])-[C:8]-[C:9](=[O;D1;H0:10])-[O;D1;H1:11])-[#8:12]
null
[]
80
CELSIUS
2
HOUR
To 0.13 g of ethyl ester of N-[trans-1-benzyl-7-chloro-5-(2-chlorophenyl)-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepin-3-ylmethyl]glycine obtained in Example 40 were added 2 ml of formalin and 2 ml of oxalic acid: The mixture was heated at 80° C. for 2 hours. The reaction mixture was concentrated under reduced pressure, a...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Secondary amine
Tertiary amine
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2.c1ccccc1
Other
null
80
2
C=O.O=C(O)CNC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O>>CN(CC(=O)O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-55b206274ba64afda97796f6ecfc93a5
CC(=O)OC(C)=O.O=C(O)CNC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O>>CC(=O)N(CC(=O)O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC(=C2)Cl)C2=C(C=CC=C2)Cl)CNCC(=O)O)=O.C(C)(=O)OC(C)=O.C(C)N(CC)CC>>C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC(=C2)Cl)C2=C(C=CC=C2)Cl)CN(CC(=O)O)C(C)=O)=O
CC(=O)O[C:2]([CH3:1])=[O:3].[NH:4]([CH2:5][C:6](=[O:7])[OH:8])[CH2:9][C@H:10]1[O:11][C@H:12]([c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]2[Cl:19])[c:20]2[cH:21][c:22]([Cl:23])[cH:24][cH:25][c:26]2[N:27]([CH2:28][c:29]2[cH:30][cH:31][cH:32][cH:33][cH:34]2)[C:35]1=[O:36]>>[CH3:1][C:2](=[O:3])[N:4]([CH2:5][C:6](=[O:7])[OH:8]...
CC(=O)OC(C)=O.O=C(O)CNC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
CC(=O)N(CC(=O)O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
null
null
CO
Acylation
Aminolysis of esters
72a6d1966b6b15ac7195d4682af251dc9ffac857f784a4242970ab5c7a529369
6593c6062585994f02076cd3c86920ae7244b86659eab65c21b5a8628c6d4bb8
O=C1CO[C@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#7:4]-[C:5](=[O;D1;H0:6])-[C:7](-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11](=[O;D1;H0:12])-[O;D1;H1:13])-[#8:14]>>[#7:4]-[C:5](=[O;D1;H0:6])-[C:7](-[C:8]-[N;H0;D3;+0:9](-[C:10]-[C:11](=[O;D1;H0:12])-[O;D1;H1:13])-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[#8:14]
null
[]
null
null
null
null
In 4 ml of methanol was dissolved 60 mg of ethyl ester of N-[trans-1-benzyl-7-chloro-5-(2-chlorophenyl)-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepin-3-ylmethyl]glycine obtained in Example 40. To the solution were added 0.2 ml of acetic anhydride and 0.2 ml of triethylamine. The mixture was heated for one hour under reflux...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Secondary amine
Tertiary amide
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2.c1ccccc1
HO-
CO
null
null
CC(=O)OC(C)=O.O=C(O)CNC[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O>CO>CC(=O)N(CC(=O)O)C[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-42aca8051c1945bf90df0b26f4fe3c47
O=C1[C@@H](CO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N1Cc1ccccc1>>O=C(O)[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC(=C2)Cl)C2=C(C=CC=C2)Cl)CO)=O.CC(=O)C.OS(=O)(=O)O.O=[Cr](=O)=O>>C(C1=CC=CC=C1)N1C([C@H](O[C@@H](C2=C1C=CC(=C2)Cl)C2=C(C=CC=C2)Cl)C(=O)O)=O
[CH2:2]([OH:3])[C@H:4]1[O:5][C@H:6]([c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[Cl:13])[c:14]2[cH:15][c:16]([Cl:17])[cH:18][cH:19][c:20]2[N:21]([CH2:22][c:23]2[cH:24][cH:25][cH:26][cH:27][cH:28]2)[C:29]1=[O:30]>>[O:1]=[C:2]([OH:3])[C@H:4]1[O:5][C@H:6]([c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[Cl:13])[c:14]2[cH:15][c:16]([Cl:...
O=C1[C@@H](CO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N1Cc1ccccc1
O=C(O)[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
null
null
CC(=O)C
Oxidation
Oxidation of alcohol to carboxylic acid
b709baac44a995a9a8f6386a6b5d87f98c32eb5a0636340abc1f778fae827230
4454822e22dc2dc24e7495385256bfce456e337c240bb764261f81dbeda1aaa1
O=C1CO[C@H](c2ccccc2)c2ccccc2N1Cc1ccccc1
[C:1]-[#7:2](-[c:3])-[C:4](=[O;D1;H0:5])-[C:6](-[CH2;D2;+0:7]-[O;D1;H1:8])-[#8:9]-[C:10]>>[C:1]-[#7:2](-[c:3])-[C:4](=[O;D1;H0:5])-[C:6](-[C;H0;D3;+0:7](=[O;D1;H0:11])-[O;D1;H1:8])-[#8:9]-[C:10]
null
[]
null
null
null
null
In 20 ml of acetone was dissolved 0.5 g of trans-1-benzyl-7-chloro-5-(2-chlorophenyl)-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-methanol obtained in Example 46. To the solution was added dropwise, while stirring at room temperature, 0.5 ml of a Jones reagent. The reaction mixture was stirred for one hour at room tem...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Carboxylic acid
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2.c1ccccc1
Other
CC(=O)C
null
null
O=C1[C@@H](CO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N1Cc1ccccc1>CC(=O)C>O=C(O)[C@H]1O[C@H](c2ccccc2Cl)c2cc(Cl)ccc2N(Cc2ccccc2)C1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a28f563304e54fffb04c32e3c16b18c3
CCOC(=O)CNC(=O)C[C@H]1O[C@@H](c2ccccc2)c2cc(Cl)ccc2N(C(C)C)C1=O>>CC(C)N1C(=O)[C@@H](CC(=O)NCC(=O)O)O[C@@H](c2ccccc2)c2cc(Cl)ccc21
C(C)OC(CNC(C[C@@H]1C(N(C2=C([C@@H](O1)C1=CC=CC=C1)C=C(C=C2)Cl)C(C)C)=O)=O)=O.C([O-])([O-])=O.[K+].[K+].Cl>>ClC=1C=CC2=C([C@@H](O[C@@H](C(N2C(C)C)=O)CC(=O)NCC(=O)O)C2=CC=CC=C2)C1
CC[O:15][C:13]([CH2:12][NH:11][C:9]([CH2:8][C@@H:7]1[C:5](=[O:6])[N:4]([CH:2]([CH3:1])[CH3:3])[c:30]2[c:24]([cH:25][c:26]([Cl:27])[cH:28][cH:29]2)[C@H:17]([c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[O:16]1)=[O:10])=[O:14]>>[CH3:1][CH:2]([CH3:3])[N:4]1[C:5](=[O:6])[C@@H:7]([CH2:8][C:9](=[O:10])[NH:11][CH2:12][C:13](=[O...
CCOC(=O)CNC(=O)C[C@H]1O[C@@H](c2ccccc2)c2cc(Cl)ccc2N(C(C)C)C1=O
CC(C)N1C(=O)[C@@H](CC(=O)NCC(=O)O)O[C@@H](c2ccccc2)c2cc(Cl)ccc21
null
null
CO.O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C1CO[C@@H](c2ccccc2)c2ccccc2N1
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
64.4
[{"value": 64.4, "product": "ClC=1C=CC2=C([C@@H](O[C@@H](C(N2C(C)C)=O)CC(=O)NCC(=O)O)C2=CC=CC=C2)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
6
HOUR
In a mixture of 2 ml of methanol and 1 ml of water was suspended 48 mg of N-(trans-7-chloro-1-isopropyl-5-phenyl-1,2,3,5-tetrahydro-2-oxo-4,1-benzoxazepin-3-ylacetyl)glycine ethyl ester obtained in Example 55. To the suspension was added 0.1 g of potassium carbonate. The mixture was stirred for 6 hours at room temperat...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2
Other
CO.O
null
6
CCOC(=O)CNC(=O)C[C@H]1O[C@@H](c2ccccc2)c2cc(Cl)ccc2N(C(C)C)C1=O>CO.O>CC(C)N1C(=O)[C@@H](CC(=O)NCC(=O)O)O[C@@H](c2ccccc2)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-848ec5bd613e4f5c9be2f2b670bc528c
CC(C)N1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>>CC(C)N1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
CS(=O)C.C(C(=O)Cl)(=O)Cl.ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)CCO)C2=C(C=CC=C2)Cl)C1.C(C)N(CC)CC>>ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)CC=O)C2=C(C=CC=C2)Cl)C1
[CH3:1][CH:2]([CH3:3])[N:4]1[C:5](=[O:6])[C@@H:7]([CH2:8][CH2:9][OH:10])[O:11][C@H:12]([c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]2[Cl:19])[c:20]2[cH:21][c:22]([Cl:23])[cH:24][cH:25][c:26]21>>[CH3:1][CH:2]([CH3:3])[N:4]1[C:5](=[O:6])[C@@H:7]([CH2:8][CH:9]=[O:10])[O:11][C@H:12]([c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]2[C...
CC(C)N1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
CC(C)N1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
null
C(Cl)Cl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
O=C1CO[C@H](c2ccccc2)c2ccccc2N1
[#7:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[CH2;D2;+0:6]-[OH;D1;+0:7])-[#8:8]>>[#7:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[CH;D2;+0:6]=[O;H0;D1;+0:7])-[#8:8]
92.5
[{"value": 92.5, "product": "ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)CC=O)C2=C(C=CC=C2)Cl)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
A solution of oxalyl chloride (0.72 ml) in methylene chloride (10 ml) was cooled to -65° C., to which was added dropwise a solution of dimethyl sulfoxide (0.63 ml) in methylene chloride (2 ml) taking 5 minutes, followed by stirring for 5 minutes. To the mixture was added dropwise, taking 15 minutes, a solution of trans...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2
null
C(Cl)Cl
null
0.083333
CC(C)N1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>C(Cl)Cl>CC(C)N1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7891886a1dce4bd98201a13284a39c9a
CC(C)N1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.CCOC(=O)C=P(c1ccccc1)(c1ccccc1)c1ccccc1>>CC(C)N1C(=O)[C@@H](C/C=C/C(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)CC=O)C2=C(C=CC=C2)Cl)C1.C(C)OC(=O)C=P(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1>>ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)C/C=C/C(=O)O)C2=C(C=CC=C2)Cl)C1
O=[CH:9][CH2:8][C@@H:7]1[C:5](=[O:6])[N:4]([CH:2]([CH3:1])[CH3:3])[c:29]2[c:23]([cH:24][c:25]([Cl:26])[cH:27][cH:28]2)[C@@H:15]([c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[Cl:22])[O:14]1.CC[O:13][C:11]([CH:10]=P(c1ccccc1)(c1ccccc1)c1ccccc1)=[O:12]>>[CH3:1][CH:2]([CH3:3])[N:4]1[C:5](=[O:6])[C@@H:7]([CH2:8]/[CH:9]=[CH:10]...
CC(C)N1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.CCOC(=O)C=P(c1ccccc1)(c1ccccc1)c1ccccc1
CC(C)N1C(=O)[C@@H](C/C=C/C(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
null
C1(=CC=CC=C1)C
C-C Coupling
OtherReaction
c06f441329a1c85dd58b67c3ed7dca4f2b4838e56125ed608c5d39ebec591cc0
04a7a14866317f7132eb69ea35ca8b6703c51b03c0c51c392001b195de1edfe7
O=C1CO[C@H](c2ccccc2)c2ccccc2N1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[CH;D2;+0:4]=P(-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1.O=[CH;D2;+0:5]-[C:6]-[C:7](-[#8:8])-[C:9](=[O;D1;H0:10])-[#7:11]>>[#7:11]-[C:9](=[O;D1;H0:10])-[C:7](-[C:6]/[CH;D2;+0:5]=[CH;D2;+0:4]/[C:2](=[O;D1;H0:3])-[OH;D1;+0:1])-[#8:8]
77.1
[{"value": 77.1, "product": "ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)C/C=C/C(=O)O)C2=C(C=CC=C2)Cl)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
3
HOUR
In toluene (20 ml) was dissolved trans-7-chloro-5-(2-chlorophenyl)-1-isopropyl-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-acetaldehyde (1.5 g). To the solution was added (ethoxycarbonylmethylene)-triphenylphosphorane (2.0 g), and the mixture was stirred for 3 hours at 90° C. The solvent was distilled off, and the res...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Ester
Carboxylic acid
c1ccccc1.c1ccccc1.c1ccccc1
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2
HO-
C1(=CC=CC=C1)C
90
3
CC(C)N1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.CCOC(=O)C=P(c1ccccc1)(c1ccccc1)c1ccccc1>C1(=CC=CC=C1)C>CC(C)N1C(=O)[C@@H](C/C=C/C(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a2fcb8e364ca4dd2ada72db56fde3611
CC(C)N1C(=O)[C@@H](C/C=C/C(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>>CC(C)N1C(=O)[C@@H](CCCC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)C/C=C/C(=O)O)C2=C(C=CC=C2)Cl)C1.[H][H]>>ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)CCCC(=O)O)C2=C(C=CC=C2)Cl)C1
[CH3:1][CH:2]([CH3:3])[N:4]1[C:5](=[O:6])[C@@H:7]([CH2:8]/[CH:9]=[CH:10]/[C:11](=[O:12])[OH:13])[O:14][C@H:15]([c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[Cl:22])[c:23]2[cH:24][c:25]([Cl:26])[cH:27][cH:28][c:29]21>>[CH3:1][CH:2]([CH3:3])[N:4]1[C:5](=[O:6])[C@@H:7]([CH2:8][CH2:9][CH2:10][C:11](=[O:12])[OH:13])[O:14][C@H:...
CC(C)N1C(=O)[C@@H](C/C=C/C(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
CC(C)N1C(=O)[C@@H](CCCC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
[C].[Pd]
C(C)(=O)OCC
Reduction
Hydrogenation (double to single)
0bc3968b35f0839c230afb4215314da278abd4e1f10e42ec3012c5512de49ea5
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
O=C1CO[C@H](c2ccccc2)c2ccccc2N1
[#7:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]/[CH;D2;+0:6]=[CH;D2;+0:7]/[C:8](=[O;D1;H0:9])-[O;D1;H1:10])-[#8:11]>>[#7:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[CH2;D2;+0:6]-[CH2;D2;+0:7]-[C:8](=[O;D1;H0:9])-[O;D1;H1:10])-[#8:11]
81.8
[{"value": 81.8, "product": "ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)CCCC(=O)O)C2=C(C=CC=C2)Cl)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In ethyl acetate (20 ml) was dissolved ethyl ester of trans-7-chloro-5-(2-chlorophenyl)-1-isopropyl-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-crotonic acid (0.45 g). To the solution was added 10% palladium carbon (0.1 g), and the mixture was subjected to catalytic reduction at room temperatures under atmospheric pre...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2
null
[C].[Pd].C(C)(=O)OCC
null
null
CC(C)N1C(=O)[C@@H](C/C=C/C(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>[C].[Pd].C(C)(=O)OCC>CC(C)N1C(=O)[C@@H](CCCC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-058d1ba117d240a89d29098d17908733
COc1cc(OC)c(C(=O)c2cc(Cl)ccc2NC(C)=O)c(OC)c1>>COc1cc(OC)c(C(=O)c2cc(Cl)ccc2N)c(OC)c1
C(C)(=O)NC1=C(C(=O)C2=C(C=C(C=C2OC)OC)OC)C=C(C=C1)Cl.Cl>>NC1=C(C(=O)C2=C(C=C(C=C2OC)OC)OC)C=C(C=C1)Cl
CC(=O)[NH:18][c:17]1[c:11]([C:9]([c:8]2[c:5]([O:6][CH3:7])[cH:4][c:3]([O:2][CH3:1])[cH:22][c:19]2[O:20][CH3:21])=[O:10])[cH:12][c:13]([Cl:14])[cH:15][cH:16]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][CH3:7])[c:8]([C:9](=[O:10])[c:11]2[cH:12][c:13]([Cl:14])[cH:15][cH:16][c:17]2[NH2:18])[c:19]([O:20][CH3:21])[cH:22]1
COc1cc(OC)c(C(=O)c2cc(Cl)ccc2NC(C)=O)c(OC)c1
COc1cc(OC)c(C(=O)c2cc(Cl)ccc2N)c(OC)c1
null
null
C(C)O
Reduction
Hydrogenolysis of amides/imides/carbamates
755df58c254dea764fdda078ffd678ec540bba057c83683be04c253f1270ac7b
025f7cefe51e71668ad5d09fca32df168e9b538347403e4d5c1748073e538adc
O=C(c1ccccc1)c1ccccc1
C-C(=O)-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5]=[O;D1;H0:6]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]-[C:5]=[O;D1;H0:6]
90.2
[{"value": 90.2, "product": "NC1=C(C(=O)C2=C(C=C(C=C2OC)OC)OC)C=C(C=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 4.7 g of 2-acetylamino-5-chloro-2',4',6'-trimethoxybenzophenone, 50 ml of 6N hydrochloric acid and 50 ml of ethanol was refluxed for 1 hour while heating. After the solvent was distilled off, the residue was basefied with an aqueous solution of sodium hydrogen carbonate and then extracted with ethyl acetat...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Primary amine
null
null
c1ccccc1.c1ccccc1
HO-
C(C)O
null
null
COc1cc(OC)c(C(=O)c2cc(Cl)ccc2NC(C)=O)c(OC)c1>C(C)O>COc1cc(OC)c(C(=O)c2cc(Cl)ccc2N)c(OC)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4ec01e77712840338ca5e710ce372103
COc1cc(OC)c(C(=O)c2cc(Cl)ccc2N)c(OC)c1>>COc1cc(OC)c(C(O)c2cc(Cl)ccc2N)c(OC)c1
O.NC1=C(C(=O)C2=C(C=C(C=C2OC)OC)OC)C=C(C=C1)Cl.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>NC1=C(C(C2=C(C=C(C=C2OC)OC)OC)O)C=C(C=C1)Cl
[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][CH3:7])[c:8]([C:9](=[O:10])[c:11]2[cH:12][c:13]([Cl:14])[cH:15][cH:16][c:17]2[NH2:18])[c:19]([O:20][CH3:21])[cH:22]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][CH3:7])[c:8]([CH:9]([OH:10])[c:11]2[cH:12][c:13]([Cl:14])[cH:15][cH:16][c:17]2[NH2:18])[c:19]([O:20][CH3:21])[cH:22]1
COc1cc(OC)c(C(=O)c2cc(Cl)ccc2N)c(OC)c1
COc1cc(OC)c(C(O)c2cc(Cl)ccc2N)c(OC)c1
null
null
O1CCCC1
Reduction
Reduction of ketone to secondary alcohol
02790ac194d8bf7ccb13d6247c59412024d87f77d2c906ef7804f021f57d5070
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1ccc(Cc2ccccc2)cc1
[O;H0;D1;+0:1]=[C;H0;D3;+0:2](-[c:3](:[c:4]):[c:5])-[c:6](:[c:7]):[c:8]>>[OH;D1;+0:1]-[CH;D3;+0:2](-[c:3](:[c:4]):[c:5])-[c:6](:[c:7]):[c:8]
96.1
[{"value": 96.1, "product": "NC1=C(C(C2=C(C=C(C=C2OC)OC)OC)O)C=C(C=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 3.0 g of 2-amino-5-chloro-2',4',6'-trimethoxybenzophenone in 50 ml of tetrahydrofuran, 0.43 g of lithium aluminum hydride was added, followed by stirring for 1 hour. After water was added, the solution was extracted with ethyl acetate and dried over anhydrous sodium sulfate, after which the solvent was...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
null
null
c1ccccc1.c1ccccc1
null
O1CCCC1
null
1
COc1cc(OC)c(C(=O)c2cc(Cl)ccc2N)c(OC)c1>O1CCCC1>COc1cc(OC)c(C(O)c2cc(Cl)ccc2N)c(OC)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-775bed0ad28c49fbb6c1ce5df50c6d65
CC(C)(C)C=O.COc1cc(OC)c(C(O)c2cc(Cl)ccc2N)c(OC)c1>>COc1cc(OC)c(C(O)c2cc(Cl)ccc2NCC(C)(C)C)c(OC)c1
C(#N)[BH3-].[Na+].NC1=C(C(C2=C(C=C(C=C2OC)OC)OC)O)C=C(C=C1)Cl.CC(C=O)(C)C.C(C)(=O)O>>ClC=1C=CC(=C(C(C2=C(C=C(C=C2OC)OC)OC)O)C1)NCC(C)(C)C
O=[CH:19][C:20]([CH3:21])([CH3:22])[CH3:23].[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][CH3:7])[c:8]([CH:9]([OH:10])[c:11]2[cH:12][c:13]([Cl:14])[cH:15][cH:16][c:17]2[NH2:18])[c:24]([O:25][CH3:26])[cH:27]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][CH3:7])[c:8]([CH:9]([OH:10])[c:11]2[cH:12][c:13]([Cl:14])[cH:15][cH:16][c:17]2[NH:18]...
CC(C)(C)C=O.COc1cc(OC)c(C(O)c2cc(Cl)ccc2N)c(OC)c1
COc1cc(OC)c(C(O)c2cc(Cl)ccc2NCC(C)(C)C)c(OC)c1
null
null
C(C)O
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
c1ccc(Cc2ccccc2)cc1
O=[CH;D2;+0:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[C;D1;H3:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[C;D1;H3:3]-[C:2](-[C;D1;H3:4])(-[C;D1;H3:5])-[CH2;D2;+0:1]-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]
null
[]
null
null
8
HOUR
After a solution of 2.5 g of 2-amino-5-chloro-α-(2,4,6-trimethoxyphenyl)benzyl alcohol, 1.01 ml of trimethylacetaldehyde and 0.56 g of acetic acid in 30 ml of ethanol was stirred at room temperature for 1.5 hours, 0.81 g of sodium cyanoborohydride was added, followed by stirring overnight. After concentration and subse...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccccc1
Other
C(C)O
null
8
CC(C)(C)C=O.COc1cc(OC)c(C(O)c2cc(Cl)ccc2N)c(OC)c1>C(C)O>COc1cc(OC)c(C(O)c2cc(Cl)ccc2NCC(C)(C)C)c(OC)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-1fc2f1e399f34cafb24dd477e3e8aa29
CC(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[NH4+]>>CC(C)CN1C(=O)[C@@H](CC(N)=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)C)=O)CC(=O)O)C2=C(C=CC=C2)Cl)C1.[Cl-].[NH4+].Cl.C(C)N=C=NCCCN(C)C.C(C)N(CC)CC>>ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)C)=O)CC(=O)N)C2=C(C=CC=C2)Cl)C1
O[C:10]([CH2:9][C@@H:8]1[C:6](=[O:7])[N:5]([CH2:4][CH:2]([CH3:1])[CH3:3])[c:28]2[c:22]([cH:23][c:24]([Cl:25])[cH:26][cH:27]2)[C@@H:14]([c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[Cl:21])[O:13]1)=[O:12].[NH4+:11]>>[CH3:1][CH:2]([CH3:3])[CH2:4][N:5]1[C:6](=[O:7])[C@@H:8]([CH2:9][C:10]([NH2:11])=[O:12])[O:13][C@H:14]([c:15...
CC(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[NH4+]
CC(C)CN1C(=O)[C@@H](CC(N)=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
null
CN(C=O)C.O
Acylation
Carboxylic acid to amide conversion
1283aef55d7ee699f097a8e5267689198c76ba671644401547f902657820236d
cb0a71c3fb37a76e96fbd81aae6f95a28398a03d1ad2c8e877085e735efb98f1
O=C1CO[C@H](c2ccccc2)c2ccccc2N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4](-[#8:5])-[C:6](=[O;D1;H0:7])-[#7:8].[NH4+;D0:9]>>[#7:8]-[C:6](=[O;D1;H0:7])-[C:4](-[C:3]-[C;H0;D3;+0:1](-[NH2;D1;+0:9])=[O;D1;H0:2])-[#8:5]
75.2
[{"value": 75.2, "product": "ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)C)=O)CC(=O)N)C2=C(C=CC=C2)Cl)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
1.0 g of trans-7-chloro-5-(2-chlorophenyl)-1-isobutyl-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-acetic acid and 0.5 g of ammonium chloride were dissolved in 8 mi of dimethylformamide, and 0.46 g of 1-ethyl-3-(3-dimethylaminopropyl)carbodiimide hydrochloride and 0.7 ml of triethylamine were added, followed by stirrin...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary amide
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2
HO-
CN(C=O)C.O
null
0.5
CC(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[NH4+]>CN(C=O)C.O>CC(C)CN1C(=O)[C@@H](CC(N)=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-39af1e12beb24e17a8267182051aa7af
Nc1ccc(Cl)cc1C(O)c1ccccc1Cl.O=C(O)C(F)(F)F>>O=C(Nc1ccc(Cl)cc1C(O)c1ccccc1Cl)C(F)(F)F
NC1=C(C(C2=C(C=CC=C2)Cl)O)C=C(C=C1)Cl.FC(C(=O)O)(F)F.C(O)([O-])=O.[Na+]>>ClC=1C=CC(=C(C(C2=C(C=CC=C2)Cl)O)C1)NC(C(F)(F)F)=O
[NH2:3][c:4]1[cH:5][cH:6][c:7]([Cl:8])[cH:9][c:10]1[CH:11]([OH:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][c:18]1[Cl:19].O[C:2](=[O:1])[C:20]([F:21])([F:22])[F:23]>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][c:7]([Cl:8])[cH:9][c:10]1[CH:11]([OH:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][c:18]1[Cl:19])[C:20]([F:21])([F:22])[F:23]
Nc1ccc(Cl)cc1C(O)c1ccccc1Cl.O=C(O)C(F)(F)F
O=C(Nc1ccc(Cl)cc1C(O)c1ccccc1Cl)C(F)(F)F
null
null
ClCCl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
c1ccc(Cc2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[F;D1;H0:4])(-[F;D1;H0:5])-[F;D1;H0:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[F;D1;H0:4]-[C:3](-[F;D1;H0:5])(-[F;D1;H0:6])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]
95.7
[{"value": 95.7, "product": "ClC=1C=CC(=C(C(C2=C(C=CC=C2)Cl)O)C1)NC(C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 1.0 g of 2-amino-5-chloro-α-(2-chlorophenyl)benzyl alcohol in 12 ml of dichloromethane, a solution of 0.8 g of anhydrous trifluoroacetic acid in 2 ml of dichloromethane was added. After reaction, an aqueous solution of sodium hydrogen carbonate was added, and the organic layer was dried, after which th...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1
HO-
ClCCl
null
null
Nc1ccc(Cl)cc1C(O)c1ccccc1Cl.O=C(O)C(F)(F)F>ClCCl>O=C(Nc1ccc(Cl)cc1C(O)c1ccccc1Cl)C(F)(F)F
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-043e8eba8ec84c2aabee85de8361dc19
O=C(Nc1ccc(Cl)cc1C(O)c1ccccc1Cl)C(F)(F)F>>OC(c1ccccc1Cl)c1cc(Cl)ccc1NCC(F)(F)F
[H-].[Al+3].[Li+].[H-].[H-].[H-].ClC=1C=CC(=C(C(C2=C(C=CC=C2)Cl)O)C1)NC(C(F)(F)F)=O.O>>ClC=1C=CC(=C(C(C2=C(C=CC=C2)Cl)O)C1)NCC(F)(F)F
O=[C:18]([NH:17][c:16]1[c:10]([CH:2]([OH:1])[c:3]2[cH:4][cH:5][cH:6][cH:7][c:8]2[Cl:9])[cH:11][c:12]([Cl:13])[cH:14][cH:15]1)[C:19]([F:20])([F:21])[F:22]>>[OH:1][CH:2]([c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1[Cl:9])[c:10]1[cH:11][c:12]([Cl:13])[cH:14][cH:15][c:16]1[NH:17][CH2:18][C:19]([F:20])([F:21])[F:22]
O=C(Nc1ccc(Cl)cc1C(O)c1ccccc1Cl)C(F)(F)F
OC(c1ccccc1Cl)c1cc(Cl)ccc1NCC(F)(F)F
null
null
O1CCCC1.C(C)OCC
Reduction
Reduction of secondary amides to amines
85b757f1833edc9e5c6365ee6b904683f414e7b9a5f9bfcfd7addca401447058
ab40188eef2f825df7003af0ffae31d0ce53d126542122535627d3d354cbc9fe
c1ccc(Cc2ccccc2)cc1
O=[C;H0;D3;+0:1](-[#7:2]-[c:3])-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7]>>[F;D1;H0:5]-[C:4](-[F;D1;H0:6])(-[F;D1;H0:7])-[CH2;D2;+0:1]-[#7:2]-[c:3]
86.7
[{"value": 86.7, "product": "ClC=1C=CC(=C(C(C2=C(C=CC=C2)Cl)O)C1)NCC(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a suspension of 0.25 g of lithium aluminum hydride in 20 ml of absolute ethyl ether, a solution of 1.2 g of 5-chloro-α-(2-chlorophenyl)-2-(trifluoroacetylamino)benzyl alcohol in 5 ml of tetrahydrofuran was added dropwise. After mixture stirring at room temperature for 1 hour, water was added, and the organic layer w...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
null
null
null
c1ccccc1.c1ccccc1
Other
O1CCCC1.C(C)OCC
null
1
O=C(Nc1ccc(Cl)cc1C(O)c1ccccc1Cl)C(F)(F)F>O1CCCC1.C(C)OCC>OC(c1ccccc1Cl)c1cc(Cl)ccc1NCC(F)(F)F
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-757632750487427b80394903b6f82440
CC(C)(C)CN1C(=O)[C@@H](CC(=O)Nc2cccc(C#N)c2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[N-]=[N+]=[N-]>>CC(C)(C)CN1C(=O)[C@@H](CC(=O)Nc2cccc(-c3nnn[nH]3)c2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC(=O)NC2=CC(=CC=C2)C#N)C2=C(C=CC=C2)Cl)C1.[N-]=[N+]=[N-].[Na+].O>>ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC(=O)NC2=CC(=CC=C2)C2=NN=NN2)C2=C(C=CC=C2)Cl)C1
[CH3:1][C:2]([CH3:3])([CH3:4])[CH2:5][N:6]1[C:7](=[O:8])[C@@H:9]([CH2:10][C:11](=[O:12])[NH:13][c:14]2[cH:15][cH:16][cH:17][c:18]([C:19]#[N:20])[cH:24]2)[O:25][C@H:26]([c:27]2[cH:28][cH:29][cH:30][cH:31][c:32]2[Cl:33])[c:34]2[cH:35][c:36]([Cl:37])[cH:38][cH:39][c:40]21.[N-:21]=[N+:22]=[N-:23]>>[CH3:1][C:2]([CH3:3])([CH...
CC(C)(C)CN1C(=O)[C@@H](CC(=O)Nc2cccc(C#N)c2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[N-]=[N+]=[N-]
CC(C)(C)CN1C(=O)[C@@H](CC(=O)Nc2cccc(-c3nnn[nH]3)c2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
null
CN(C=O)C
Aromatic Heterocycle Formation
OtherReaction
237b84aaa459abf427f233dc6a07a1d9de824f980714e458423189bb68f60f12
d8c808528b7ee68720aaeebd35cb6a2a30e344748d0066102cdae99843b93cf0
O=C(C[C@H]1O[C@H](c2ccccc2)c2ccccc2NC1=O)Nc1cccc(-c2nnn[nH]2)c1
[N-;H0;D1:1]=[N+;H0;D2:2]=[N-;H0;D1:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:10]:[c:9]:[c;H0;D3;+0:6](-[c;H0;D3;+0:5]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:1]:[n;H0;D2;+0:2]:[nH;D2;+0:3]:1):[c:7]:[c:8]
50.9
[{"value": 50.9, "product": "ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC(=O)NC2=CC(=CC=C2)C2=NN=NN2)C2=C(C=CC=C2)Cl)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 0.2 g of trans-7-chloro-5-(2-chlorophenyl)-3-(3-cyanophenylaminocarbonylmethyl)-1-neopentyl-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine and 80 mg of sodium azide in 5 ml of dimethylformamide was stirred at 90° C. for 60 hours. After water was added, the mixture was washed with water, after which the solven...
10.6084/m9.figshare.5104873.v1
null
Nitrile
null
null
c1nnn[nH]1
c1ccccc1.c1nnn[nH]1.c1ccccc1.c1ccc2c(c1)COCC[NH]2
null
CN(C=O)C
null
null
CC(C)(C)CN1C(=O)[C@@H](CC(=O)Nc2cccc(C#N)c2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[N-]=[N+]=[N-]>CN(C=O)C>CC(C)(C)CN1C(=O)[C@@H](CC(=O)Nc2cccc(-c3nnn[nH]3)c2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-450e99beb381497883ffdb50182f2603
CC(C)N1C(=O)[C@@H](CC(=O)NCC#N)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[N-]=[N+]=[N-]>>CC(C)N1C(=O)[C@@H](CC(=O)NCc2nnn[nH]2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)CC(=O)NCC#N)C2=C(C=CC=C2)Cl)C1.[N-]=[N+]=[N-].[Na+]>>ClC=1C=CC2=C([C@H](O[C@@H](C(N2C(C)C)=O)CC(=O)NCC2=NN=NN2)C2=C(C=CC=C2)Cl)C1
[CH3:1][CH:2]([CH3:3])[N:4]1[C:5](=[O:6])[C@@H:7]([CH2:8][C:9](=[O:10])[NH:11][CH2:12][C:13]#[N:14])[O:18][C@H:19]([c:20]2[cH:21][cH:22][cH:23][cH:24][c:25]2[Cl:26])[c:27]2[cH:28][c:29]([Cl:30])[cH:31][cH:32][c:33]21.[N-:15]=[N+:16]=[N-:17]>>[CH3:1][CH:2]([CH3:3])[N:4]1[C:5](=[O:6])[C@@H:7]([CH2:8][C:9](=[O:10])[NH:11]...
CC(C)N1C(=O)[C@@H](CC(=O)NCC#N)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[N-]=[N+]=[N-]
CC(C)N1C(=O)[C@@H](CC(=O)NCc2nnn[nH]2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
null
null
Aromatic Heterocycle Formation
OtherReaction
237b84aaa459abf427f233dc6a07a1d9de824f980714e458423189bb68f60f12
d8c808528b7ee68720aaeebd35cb6a2a30e344748d0066102cdae99843b93cf0
O=C(C[C@H]1O[C@H](c2ccccc2)c2ccccc2NC1=O)NCc1nnn[nH]1
[N-;H0;D1:1]=[N+;H0;D2:2]=[N-;H0;D1:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[C:6]-[#7:7]-[C:8]=[O;D1;H0:9]>>[O;D1;H0:9]=[C:8]-[#7:7]-[C:6]-[c;H0;D3;+0:5]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:1]:[n;H0;D2;+0:2]:[nH;D2;+0:3]:1
null
[]
null
null
null
null
Trans-7-chloro-5-(2-chlorophenyl)-3-(cyanomethylaminocarbonylmethyl)-1-isopropyl-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine and sodium azide were subjected to the same procedure as in Example 102 to yield a crystal. Conditions: See reaction.notes.procedure_details. Workup: to yield a crystal
10.6084/m9.figshare.5104873.v1
null
Nitrile
null
null
c1nnn[nH]1
c1nnn[nH]1.c1ccccc1.c1ccc2c(c1)COCC[NH]2
null
null
null
null
CC(C)N1C(=O)[C@@H](CC(=O)NCC#N)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21.[N-]=[N+]=[N-]>>CC(C)N1C(=O)[C@@H](CC(=O)NCc2nnn[nH]2)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b12632ff90da4c7fbf9aead0149dd2e8
COc1ccccc1C(=O)c1cc(Cl)ccc1N>>Nc1ccc(Cl)cc1C(=O)c1ccccc1O
NC1=C(C(=O)C2=C(C=CC=C2)OC)C=C(C=C1)Cl.C([O-])(O)=O.[Na+]>>NC1=C(C(=O)C2=C(C=CC=C2)O)C=C(C=C1)Cl
C[O:17][c:16]1[c:11]([C:9]([c:8]2[c:2]([NH2:1])[cH:3][cH:4][c:5]([Cl:6])[cH:7]2)=[O:10])[cH:12][cH:13][cH:14][cH:15]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[cH:7][c:8]1[C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[OH:17]
COc1ccccc1C(=O)c1cc(Cl)ccc1N
Nc1ccc(Cl)cc1C(=O)c1ccccc1O
null
null
Br
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=C(c1ccccc1)c1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5]=[O;D1;H0:6]>>[O;D1;H0:6]=[C:5]-[c:4]:[c:2](-[OH;D1;+0:1]):[c:3]
93.4
[{"value": 93.4, "product": "NC1=C(C(=O)C2=C(C=CC=C2)O)C=C(C=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 2.15 g of 2-amino-5-chloro-2'-methoxybenzophenone and 20 ml of 47% hydrogen bromide was heated for 1 hour under reflux. The solution was rendered neutral with sodium bicarbonate, and subjected to extraction with 100 ml of ethyl acetate. The extract solution was washed with water and dried over anhydrous ma...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccccc1.c1ccccc1
Other
Br
null
null
COc1ccccc1C(=O)c1cc(Cl)ccc1N>Br>Nc1ccc(Cl)cc1C(=O)c1ccccc1O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-64bedfb59dbe42709ee67ad4aa0bd72c
COc1ccccc1C(=O)c1cc(Cl)ccc1NC(C)=O>>Nc1ccc(Cl)cc1C(=O)c1ccccc1O
C(C)(=O)NC1=C(C(=O)C2=C(C=CC=C2)OC)C=C(C=C1)Cl.[OH-].[Na+]>>NC1=C(C(=O)C2=C(C=CC=C2)O)C=C(C=C1)Cl
CC(=O)[NH:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[cH:7][c:8]1[C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[O:17]C>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[cH:7][c:8]1[C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[OH:17]
COc1ccccc1C(=O)c1cc(Cl)ccc1NC(C)=O
Nc1ccc(Cl)cc1C(=O)c1ccccc1O
null
null
Br
Reduction
OtherReaction
d3424ce4719989ec8362730265a7804ca73064ec84ab7f078c118d035fcf0f68
6cc30ba1c20e73143a62ef8b67c89f5e4f4048975da64c393eca7e8942cb91f2
O=C(c1ccccc1)c1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5](=[O;D1;H0:6])-[c:7]:[c:8](-[NH;D2;+0:9]-C(-C)=O):[c:10]>>[NH2;D1;+0:9]-[c:8](:[c:10]):[c:7]-[C:5](=[O;D1;H0:6])-[c:4]:[c:2](-[OH;D1;+0:1]):[c:3]
98.1
[{"value": 98.1, "product": "NC1=C(C(=O)C2=C(C=CC=C2)O)C=C(C=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 10 g of 2-acetylamino-5-chloro-2'-methoxybenzophenone and 100 ml of 47% hydrogen bromide was heated for 2 hours under reflux. The solution was rendered neutral with sodium hydroxide, and was subjected to extraction with 200 ml of ethyl acetate. The extract solution was washed with water and dried over anhy...
10.6084/m9.figshare.5104873.v1
null
Ether.Secondary amide
Aromatic alcohol.Primary amine
null
null
c1ccccc1.c1ccccc1
HO-
Br
null
null
COc1ccccc1C(=O)c1cc(Cl)ccc1NC(C)=O>Br>Nc1ccc(Cl)cc1C(=O)c1ccccc1O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c2eabdf1be4f4a81a4b9a839ae6cea53
BrCc1ccccc1.Nc1ccc(Cl)cc1C(=O)c1ccccc1O>>Nc1ccc(Cl)cc1C(=O)c1ccccc1OCc1ccccc1
NC1=C(C(=O)C2=C(C=CC=C2)O)C=C(C=C1)Cl.C([O-])([O-])=O.[K+].[K+].C(C1=CC=CC=C1)Br>>NC1=C(C(=O)C2=C(C=CC=C2)OCC2=CC=CC=C2)C=C(C=C1)Cl
Br[CH2:18][c:19]1[cH:20][cH:21][cH:22][cH:23][cH:24]1.[NH2:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[cH:7][c:8]1[C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[OH:17]>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([Cl:6])[cH:7][c:8]1[C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[O:17][CH2:18][c:19]1[cH:20][cH:21][cH:22][cH...
BrCc1ccccc1.Nc1ccc(Cl)cc1C(=O)c1ccccc1O
Nc1ccc(Cl)cc1C(=O)c1ccccc1OCc1ccccc1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
O=C(c1ccccc1)c1ccccc1OCc1ccccc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H0:5]=[C:6]-[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[O;D1;H0:5]=[C:6]-[c:7]:[c:8](-[O;H0;D2;+0:9]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]):[c:10]
null
[]
null
null
2
HOUR
In 30 ml of N,N-dimethylformamide was dissolved 5.0 g of 2-amino-5-chloro-2'-hydroxybenzophenone, as obtained in Example 123 (1), to which were added 4.2 g of potassium carbonate and 2.9 ml of benzyl bromide; the mixture was then stirred for 2 hours at room temperature. The mixture was subjected to extraction with 150 ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.c1ccccc1.c1ccccc1
HBr
CN(C=O)C
null
2
BrCc1ccccc1.Nc1ccc(Cl)cc1C(=O)c1ccccc1O>CN(C=O)C>Nc1ccc(Cl)cc1C(=O)c1ccccc1OCc1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-776f36934446481dab0bf262aa25a497
CC(C)CN(C(=O)C=CC(=O)O)c1ccc(Cl)cc1C(O)c1ccccc1OCc1ccccc1>>CCOc1ccccc1C(O)c1cc(Cl)ccc1NCC(C)C
ClC1=CC(=C(C=C1)N(C(=O)C=CC(=O)O)CC(C)C)C(C1=C(C=CC=C1)OCC1=CC=CC=C1)O>>ClC=1C=CC(=C(C(C2=C(C=CC=C2)OCC)O)C1)NCC(C)C
O=C(O)C=CC(=O)[N:19]([c:18]1[c:12]([CH:10]([c:9]2[c:4]([O:3][CH2:2][c:1]3ccccc3)[cH:5][cH:6][cH:7][cH:8]2)[OH:11])[cH:13][c:14]([Cl:15])[cH:16][cH:17]1)[CH2:20][CH:21]([CH3:22])[CH3:23]>>[CH3:1][CH2:2][O:3][c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1[CH:10]([OH:11])[c:12]1[cH:13][c:14]([Cl:15])[cH:16][cH:17][c:18]1[NH:19][CH2:...
CC(C)CN(C(=O)C=CC(=O)O)c1ccc(Cl)cc1C(O)c1ccccc1OCc1ccccc1
CCOc1ccccc1C(O)c1cc(Cl)ccc1NCC(C)C
null
null
C(C)O
Reduction
OtherReaction
e461f252a26fa4b93ac220a17d32fd647954cf89489e8e27e35f099185cd9545
5ccb3bfdfb46dce5bb2696293a6757e412fd4dc56a89e9e787541a08ac1a1541
c1ccc(Cc2ccccc2)cc1
O-C(=O)-C=C-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[c:4](:[c:5]):[c:6].[#8:7]-[C:8]-[c;H0;D3;+0:9]1:c:c:c:c:c:1>>[#8:7]-[C:8]-[CH3;D1;+0:9].[C:3]-[C:2]-[NH;D2;+0:1]-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
In 150 ml of ethanol was dissolved 6.0 g of ethyl ester of 3-[N-[4-chloro-2-[2-benzyloxy-α-hydroxybenzyl]phenyl]-N-isobutylcarbamoyl]acrylic acid, as obtained in (4), to which was added 3.18 g of potassium carbonate; the mixture was then stirred overnight. The solvent was distilled off under reduced pressure, and the r...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Tertiary amide
Secondary amine
c1ccccc1
null
c1ccccc1.c1ccccc1
HO-
C(C)O
null
null
CC(C)CN(C(=O)C=CC(=O)O)c1ccc(Cl)cc1C(O)c1ccccc1OCc1ccccc1>C(C)O>CCOc1ccccc1C(O)c1cc(Cl)ccc1NCC(C)C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b73af90813ea458ca97a1404afcbed16
Nc1ccc(Br)cc1-c1cccnc1C(=O)c1ncccc1-c1cc(Br)ccc1N>>Nc1ccc(Br)cc1C(O)c1ccccn1
NC1=C(C=C(C=C1)Br)C=1C(=NC=CC1)C(=O)C1=NC=CC=C1C1=C(C=CC(=C1)Br)N.CO.[BH4-].[Na+]>>NC1=C(C(C2=NC=CC=C2)O)C=C(C=C1)Br
Nc1ccc(Br)cc1-c1cccnc1[C:9](=[O:10])[c:11]1[c:12](-[c:8]2[c:2]([NH2:1])[cH:3][cH:4][c:5]([Br:6])[cH:7]2)[cH:13][cH:14][cH:15][n:16]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([Br:6])[cH:7][c:8]1[CH:9]([OH:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][n:16]1
Nc1ccc(Br)cc1-c1cccnc1C(=O)c1ncccc1-c1cc(Br)ccc1N
Nc1ccc(Br)cc1C(O)c1ccccn1
null
null
null
Miscellaneous
OtherReaction
dbf8b9843a4aa59d2ff28f14ba8c3dbca059945b8b4b47a76899cf54da6edf1f
7f88d98f489d3609ee025be1dc002fcd7725e29ffaaad7fff2cd12b3660f666b
c1ccc(Cc2ccccn2)cc1
Br-c1:c:c:c(-N):c(-c2:c:c:c:n:c:2-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3]2:[#7;a:4]:[c:5]:[c:6]:[c:7]:[c;H0;D3;+0:8]:2-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[N;D1;H2:13]):[c:14]):c:1>>[N;D1;H2:13]-[c:12](:[c:14]):[c;H0;D3;+0:9](-[CH;D3;+0:1](-[OH;D1;+0:2])-[c:3]1:[#7;a:4]:[c:5]:[c:6]:[c:7]:[cH;D2;+0:8]:1):[c:10]:[c:11]
null
[]
null
null
30
MINUTE
In 100 ml of methanol was dissolved 10 g of 2-amino-5-bromophenyl-2-pyridylketone. To the solution was added 1.7 g of sodium borohydride and stirred for 30 minutes. The solvent methanol was evaporated off under reduced pressure. The residue was treated with an aqueous solution of hydrochloric acid. The decomposed resid...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ketone.Primary amine
Secondary alcohol
c1ccccc1.c1ccncc1.c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HBr
null
null
0.5
Nc1ccc(Br)cc1-c1cccnc1C(=O)c1ncccc1-c1cc(Br)ccc1N>>Nc1ccc(Br)cc1C(O)c1ccccn1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-5873d336793841adad5cbcf873b625c5
CC(=O)O>>CC(C)(C)C=O
NC1=C(C(C2=NC=CC=C2)O)C=C(C=C1)Br.C(C)(=O)O>>NC1=C(C(C2=NC=CC=C2)O)C=C(C=C1)Br.CC(C=O)(C)C
O[C:2]([CH3:1])=[O:6]>>[CH3:1][C:2]([CH3:3])([CH3:4])[CH:5]=[O:6]
CC(=O)O
CC(C)(C)C=O
null
null
null
Functional Group Interconversion
OtherReaction
3adc515926529d8c940a7d5ba1c36d7bcade4bebf82afc0a58508096be2f2fac
a68c8c362a41a1ec68d8543ede8c2ecdd4269a0402da828bb76b860809c088c0
null
O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;H0;D1;+0:3]>>[C;D1;H3:2]-[C;H0;D4;+0:1](-[C;D1;H3:4])(-[C;D1;H3:5])-[C:6]=[O;H0;D1;+0:3]
null
[]
null
null
null
null
In 20 ml of acetic acid was dissolved 2.0 g of 2-amino-5-bromo-α-(2-pyridyl)benzyl alcohol obtained in (1) together with 0.86 ml of trimethylacetoaldehyde. To the solution was added 0.36 g of sodium borohydride under ice-cooling. The reaction mixture was stirred for 30 minutes at room temperature and then subjected to ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Aldehyde
null
null
null
null
null
null
null
CC(=O)O>>CC(C)(C)C=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2f947493a0ee4631a9cc6d66588aa9d1
CCOC(=O)C[C@H]1O[C@H](c2ccccn2)c2cc(Br)ccc2N(CC(C)(C)C)C1=O>>CC(C)(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccn2)c2cc(Br)ccc21
BrC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC(=O)OCC)C2=NC=CC=C2)C1.C([O-])([O-])=O.[K+].[K+]>>BrC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC(=O)O)C2=NC=CC=C2)C1
CC[O:13][C:11]([CH2:10][C@@H:9]1[C:7](=[O:8])[N:6]([CH2:5][C:2]([CH3:1])([CH3:3])[CH3:4])[c:28]2[c:22]([cH:23][c:24]([Br:25])[cH:26][cH:27]2)[C@@H:15]([c:16]2[cH:17][cH:18][cH:19][cH:20][n:21]2)[O:14]1)=[O:12]>>[CH3:1][C:2]([CH3:3])([CH3:4])[CH2:5][N:6]1[C:7](=[O:8])[C@@H:9]([CH2:10][C:11](=[O:12])[OH:13])[O:14][C@H:15...
CCOC(=O)C[C@H]1O[C@H](c2ccccn2)c2cc(Br)ccc2N(CC(C)(C)C)C1=O
CC(C)(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccn2)c2cc(Br)ccc21
null
null
CO
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C1CO[C@H](c2ccccn2)c2ccccc2N1
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
69.9
[{"value": 69.9, "product": "BrC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC(=O)O)C2=NC=CC=C2)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In 20 ml of methanol was dissolved 1.9 g of ethyl trans-7-bromo-1-neopentyl-5-(2-pyridyl)-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-acetate obtained in Example 131. To the solution was added 10 ml of an aqueous solution containing 1.1 g of potassium carbonate. The mixture was heated and refluxed for 30 minutes, and ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccncc1.c1ccc2c(c1)COCC[NH]2
Other
CO
null
null
CCOC(=O)C[C@H]1O[C@H](c2ccccn2)c2cc(Br)ccc2N(CC(C)(C)C)C1=O>CO>CC(C)(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccn2)c2cc(Br)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-daf4ba5367694338ab2591f41b1c75e1
CC(C)(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>>CC(C)(C)CN1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC(=O)O)C2=C(C=CC=C2)Cl)C1.CN1CCOCC1.[BH4-].[Na+].C(OCC)(=O)Cl>>ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CCO)C2=C(C=CC=C2)Cl)C1
O[C:11]([CH2:10][C@@H:9]1[C:7](=[O:8])[N:6]([CH2:5][C:2]([CH3:1])([CH3:3])[CH3:4])[c:28]2[c:22]([cH:23][c:24]([Cl:25])[cH:26][cH:27]2)[C@@H:14]([c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[Cl:21])[O:13]1)=[O:12]>>[CH3:1][C:2]([CH3:3])([CH3:4])[CH2:5][N:6]1[C:7](=[O:8])[C@@H:9]([CH2:10][CH2:11][OH:12])[O:13][C@H:14]([c:15...
CC(C)(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
CC(C)(C)CN1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
null
CO.O1CCCC1
Reduction
Reduction of carboxylic acid to primary alcohol
0db83a5ebe1e318b78b55461cf7eb8f7c004eef0f9e3b6666d3df4c96b5f665e
93b4621647b04d2ad2f2825215b1567f171ba61fe10d136b5db6ea0470aa4932
O=C1CO[C@H](c2ccccc2)c2ccccc2N1
O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3]-[C:4](-[#8:5])-[C:6](=[O;D1;H0:7])-[#7:8]>>[#7:8]-[C:6](=[O;D1;H0:7])-[C:4](-[C:3]-[CH2;D2;+0:1]-[OH;D1;+0:2])-[#8:5]
99.8
[{"value": 99.8, "product": "ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CCO)C2=C(C=CC=C2)Cl)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
In 200 ml of tetrahydrofuran was dissolved 14.7 g of trans-7-chloro-5-(2-chlorophenyl)-1-neopentyl-2-oxo-1,2,3,5-tetrahydro-4,1-benzoxazepine-3-acetic acid obtained in Example 2 and 4.51 ml of N-methylmorpholine. To the solution was added 3.92 ml of ethyl chlorocarbonate at -10° C.; the mixture was then stirred for 15 ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary alcohol
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2
Other
CO.O1CCCC1
null
0.25
CC(C)(C)CN1C(=O)[C@@H](CC(=O)O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>CO.O1CCCC1>CC(C)(C)CN1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-77f2d3d356f745ffa41558ea6f3bd9f3
CC(C)(C)CN1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>>CC(C)(C)CN1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CCO)C2=C(C=CC=C2)Cl)C1.CS(=O)C.C(C(=O)Cl)(=O)Cl>>ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC=O)C2=C(C=CC=C2)Cl)C1
[CH3:1][C:2]([CH3:3])([CH3:4])[CH2:5][N:6]1[C:7](=[O:8])[C@@H:9]([CH2:10][CH2:11][OH:12])[O:13][C@H:14]([c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[Cl:21])[c:22]2[cH:23][c:24]([Cl:25])[cH:26][cH:27][c:28]21>>[CH3:1][C:2]([CH3:3])([CH3:4])[CH2:5][N:6]1[C:7](=[O:8])[C@@H:9]([CH2:10][CH:11]=[O:12])[O:13][C@H:14]([c:15]2[cH...
CC(C)(C)CN1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
CC(C)(C)CN1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21
null
null
ClCCl.O.C(C)N(CC)CC
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
O=C1CO[C@H](c2ccccc2)c2ccccc2N1
[#7:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[CH2;D2;+0:6]-[OH;D1;+0:7])-[#8:8]>>[#7:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[CH;D2;+0:6]=[O;H0;D1;+0:7])-[#8:8]
64.2
[{"value": 64.2, "product": "ClC=1C=CC2=C([C@H](O[C@@H](C(N2CC(C)(C)C)=O)CC=O)C2=C(C=CC=C2)Cl)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
To 25 ml of dichloromethane solution containing 0.70 ml of oxalyl chloride was added 5 ml of dichloromethane solution containing 0.71 ml of dimethylsulfoxide at -78° C., followed by stirring for 5 minutes. To the solution was slowly added 10 ml of dichloromethane solution containing 1.69 g of trans-7-chloro-5-(2-chloro...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccccc1.c1ccc2c(c1)COCC[NH]2
null
ClCCl.O.C(C)N(CC)CC
null
0.083333
CC(C)(C)CN1C(=O)[C@@H](CCO)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21>ClCCl.O.C(C)N(CC)CC>CC(C)(C)CN1C(=O)[C@@H](CC=O)O[C@H](c2ccccc2Cl)c2cc(Cl)ccc21