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414 values
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large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e56469efe4574f2b8684abbf187dfa1c
CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(=O)c2ccccc2)C1>>CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCNC1
C(C1=CC=CC=C1)(=O)N1C[C@@H](CC1)N(C(CN(C1=CC=CC=C1)C1=CC=CC=C1)=O)C>>C1(=CC=CC=C1)N(CC(=O)N([C@H]1CNCC1)C)C1=CC=CC=C1
O=C(c1ccccc1)[N:22]1[CH2:21][CH2:20][C@@H:19]([N:2]([CH3:1])[C:3](=[O:4])[CH2:5][N:6]([c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[CH2:23]1>>[CH3:1][N:2]([C:3](=[O:4])[CH2:5][N:6]([c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1)[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[C@@H:19]1[CH2...
CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(=O)c2ccccc2)C1
CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCNC1
null
[Pd]
CO
Reduction
Hydrogenolysis of tertiary amines
f31a24fac1247652ffb9d16bd05f6451f460ef232d259564a837b8998ec61ef8
62cf08a8ae6315067a063b5b3495125ccbdaff6b2340ce1d3e1c7b6cde962ae4
O=C(CN(c1ccccc1)c1ccccc1)N[C@@H]1CCNC1
O=C(-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-1)-c1:c:c:c:c:c:1>>[C:4]1-[C:3]-[C:2]-[NH;D2;+0:1]-[C:5]-1
114.1
[{"value": 114.1, "product": "C1(=CC=CC=C1)N(CC(=O)N([C@H]1CNCC1)C)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
To a solution of (R)—N-(1-benzoyl-pyrrolidin-3-yl)-2-diphenylamino-N-methyl-acetamide (0.68 g, 1.7 mmol) in CH3OH (30 ml) was added Pd/C 20% (170 mg). The resulting slurry was hydrogenated at 50 psi for 24 hours. The catalyst was filtered through Celite and filtrate evaporated under reduced pressure to give 0.6 g of de...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide
Secondary amine
c1ccccc1.C1CC[NH]C1
C1CCNC1
c1ccccc1.c1ccccc1.C1CCNC1
HO-
[Pd].CO
null
24
CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(=O)c2ccccc2)C1>[Pd].CO>CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCNC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-85194727a3bc4855a7dda35f5106f763
BrC(c1ccccc1)c1ccccc1.CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCNC1>>CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(c2ccccc2)c2ccccc2)C1
BrC(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)N(CC(=O)N([C@H]1CNCC1)C)C1=CC=CC=C1.C(=O)([O-])[O-].[K+].[K+]>>C(C1=CC=CC=C1)(C1=CC=CC=C1)N1C[C@@H](CC1)N(C(CN(C1=CC=CC=C1)C1=CC=CC=C1)=O)C
Br[CH:23]([c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1)[c:30]1[cH:31][cH:32][cH:33][cH:34][cH:35]1.[CH3:1][N:2]([C:3](=[O:4])[CH2:5][N:6]([c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1)[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[C@@H:19]1[CH2:20][CH2:21][NH:22][CH2:36]1>>[CH3:1][N:2]([C:3](=[O:4])[CH2:5][N:6]([c:7]1[cH:8][cH...
BrC(c1ccccc1)c1ccccc1.CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCNC1
CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(c2ccccc2)c2ccccc2)C1
null
null
CC(CC)=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
10cc789bcfe0ae11c7b2b474c79d3cdda850354ad720004a77dedb66c0fbd515
fb63ba09935e18320be03869002f6d5d0f0321fe7dbcd94a5ae956c3effd182d
O=C(CN(c1ccccc1)c1ccccc1)N[C@@H]1CCN(C(c2ccccc2)c2ccccc2)C1
Br-[CH;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7].[C:8]1-[C:9]-[C:10]-[NH;D2;+0:11]-[C:12]-1>>[c:3]:[c:2](-[CH;D3;+0:1](-[N;H0;D3;+0:11]1-[C:10]-[C:9]-[C:8]-[C:12]-1)-[c:5](:[c:6]):[c:7]):[c:4]
null
[]
null
null
null
null
To a solution of bromodiphenylmethane (0.3 g, 1.23 mmol) in butanone (10 ml) was added (R)-2-diphenylamino-N-methyl-N-pyrrolidin-3-yl-acetamide (0.46 g, 1.5 mmol), K2CO3 (0.17 g, 1.23 mmol) and KI (0.2 g, 1.23 mmol). The mixture was heated under reflux for 18 hours, then filtered and the solvent was removed in vacuo. T...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Secondary amine
Tertiary amine
C1CCNC1
C1CC[NH]C1
c1ccccc1.c1ccccc1.C1CC[NH]C1.c1ccccc1.c1ccccc1
HBr
CC(CC)=O
null
null
BrC(c1ccccc1)c1ccccc1.CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCNC1>CC(CC)=O>CN(C(=O)CN(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(c2ccccc2)c2ccccc2)C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b9d361fa95a640f9a04b086442faf109
CN[C@@H]1CCN(C(=O)c2ccccc2)C1.O=C(CBr)N(c1ccccc1)c1ccccc1>>O=C(CNC[C@H]1CCN(Cc2ccccc2)C1)N(c1ccccc1)c1ccccc1
C(C1=CC=CC=C1)(=O)N1C[C@@H](CC1)NC.BrCC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1.C(=O)(O)[O-].[Na+].CC#N>>C(C1=CC=CC=C1)N1C[C@H](CC1)CNCC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1
O=[C:10]([N:9]1[CH2:8][CH2:7][C@@H:6]([NH:4][CH3:5])[CH2:17]1)[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1.Br[CH2:3][C:2](=[O:1])[N:18]([c:19]1[cH:20][cH:21][cH:22][cH:23][cH:24]1)[c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1>>[O:1]=[C:2]([CH2:3][NH:4][CH2:5][C@H:6]1[CH2:7][CH2:8][N:9]([CH2:10][c:11]2[cH:12][cH:13][cH:14]...
CN[C@@H]1CCN(C(=O)c2ccccc2)C1.O=C(CBr)N(c1ccccc1)c1ccccc1
O=C(CNC[C@H]1CCN(Cc2ccccc2)C1)N(c1ccccc1)c1ccccc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
c66894eac9ef615d3b141f01122e8f9823ff344d499c205c62c1b3cf49e74ba3
378c54a7d08ff33f29940783d7d340c21eaa54954287ff0d36ce8b1eb86b6057
O=C(CNC[C@H]1CCN(Cc2ccccc2)C1)N(c1ccccc1)c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#7:4](-[c:5])-[c:6].O=[C;H0;D3;+0:7](-[#7:8]1-[C:9]-[C@H;D3;+0:10](-[NH;D2;+0:11]-[CH3;D1;+0:12])-[C:13]-[C:14]-1)-[c:15](:[c:16]):[c:17]>>[O;D1;H0:3]=[C:2](-[CH2;D2;+0:1]-[NH;D2;+0:11]-[CH2;D2;+0:12]-[C@@H;D3;+0:10]1-[C:9]-[#7:8](-[CH2;D2;+0:7]-[c:15](:[c:16]):[c:17])-[C:14]-[C:13...
null
[]
null
null
null
null
To a solution of (R)-(1-benzoyl-pyrrolidin-3-yl)-methyl-amine(0.32 g, 1.68 mmol) in dry CH3CN (10 ml) was added 2-bromo-N,N-diphenyl acetamide(0.49 g, 1.68 mmol) and NaHCO3 (0.28 g, 3.36 mmol) under nitrogen. The reaction mixture was refluxed overnight. After cooling, the solvent was evaporated. The residue was taken u...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Tertiary amide.Secondary amine
Secondary amine
C1CC[NH]C1
C1CC[NH]C1
C1CC[NH]C1.c1ccccc1.c1ccccc1.c1ccccc1
Br-
null
null
null
CN[C@@H]1CCN(C(=O)c2ccccc2)C1.O=C(CBr)N(c1ccccc1)c1ccccc1>>O=C(CNC[C@H]1CCN(Cc2ccccc2)C1)N(c1ccccc1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a1bf7b07a6e84b91be3f4ef0d347f994
CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(=O)c2ccccc2)C1>>CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCNC1
C(C1=CC=CC=C1)(=O)N1C[C@@H](CC1)N(CC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1)C>>CN(CC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1)[C@H]1CNCC1
O=C(c1ccccc1)[N:22]1[CH2:21][CH2:20][C@@H:19]([N:2]([CH3:1])[CH2:3][C:4](=[O:5])[N:6]([c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[CH2:23]1>>[CH3:1][N:2]([CH2:3][C:4](=[O:5])[N:6]([c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1)[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[C@@H:19]1[CH2...
CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(=O)c2ccccc2)C1
CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCNC1
null
[Pd]
CO
Reduction
Hydrogenolysis of tertiary amines
f31a24fac1247652ffb9d16bd05f6451f460ef232d259564a837b8998ec61ef8
62cf08a8ae6315067a063b5b3495125ccbdaff6b2340ce1d3e1c7b6cde962ae4
O=C(CN[C@@H]1CCNC1)N(c1ccccc1)c1ccccc1
O=C(-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-1)-c1:c:c:c:c:c:1>>[C:4]1-[C:3]-[C:2]-[NH;D2;+0:1]-[C:5]-1
95.1
[{"value": 95.1, "product": "CN(CC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1)[C@H]1CNCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
To a solution of (R)-2-[(1-benzoyl-pyrrolidin-3-yl)-methyl-amino]-N,N-diphenyl acetamide(0.68 g, 1.70 mmol) in CH3OH (30 ml) was added Pd/C 20% (170 mg). The resulting slurry was hydrogenated at 50 psi for 24 hours. The catalyst was filtered through Celite and filtrate evaporated under reduced pressure to give 0.5 g of...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide
Secondary amine
c1ccccc1.C1CC[NH]C1
C1CCNC1
c1ccccc1.c1ccccc1.C1CCNC1
HO-
[Pd].CO
null
24
CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(=O)c2ccccc2)C1>[Pd].CO>CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCNC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bdf3f775b9a54da7b287838161695a5b
BrC(c1ccccc1)c1ccccc1.CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCNC1>>CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(c2ccccc2)c2ccccc2)C1
BrC(C1=CC=CC=C1)C1=CC=CC=C1.CN(CC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1)[C@H]1CNCC1.C(=O)([O-])[O-].[K+].[K+]>>C(C1=CC=CC=C1)(C1=CC=CC=C1)N1C[C@@H](CC1)N(CC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1)C
Br[CH:23]([c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1)[c:30]1[cH:31][cH:32][cH:33][cH:34][cH:35]1.[CH3:1][N:2]([CH2:3][C:4](=[O:5])[N:6]([c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1)[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[C@@H:19]1[CH2:20][CH2:21][NH:22][CH2:36]1>>[CH3:1][N:2]([CH2:3][C:4](=[O:5])[N:6]([c:7]1[cH:8][cH...
BrC(c1ccccc1)c1ccccc1.CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCNC1
CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(c2ccccc2)c2ccccc2)C1
null
null
CC(CC)=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
10cc789bcfe0ae11c7b2b474c79d3cdda850354ad720004a77dedb66c0fbd515
fb63ba09935e18320be03869002f6d5d0f0321fe7dbcd94a5ae956c3effd182d
O=C(CN[C@@H]1CCN(C(c2ccccc2)c2ccccc2)C1)N(c1ccccc1)c1ccccc1
Br-[CH;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7].[C:8]1-[C:9]-[C:10]-[NH;D2;+0:11]-[C:12]-1>>[c:3]:[c:2](-[CH;D3;+0:1](-[N;H0;D3;+0:11]1-[C:10]-[C:9]-[C:8]-[C:12]-1)-[c:5](:[c:6]):[c:7]):[c:4]
null
[]
null
null
null
null
To a solution of bromodiphenylmethane (0.33 g, 1.34 mmol) in butanone (10 ml) was added (R)-2-(methyl-pyrrolidin-3-yl-amino)-N,N-diphenyl acetamide(0.5 g, 1.61 mmol), K2CO3 (0.18 g, 1.34 mmol) and KI (0.22 g, 1.34 mmol). The mixture was, heated under reflux for 18 hours, then filtered and the solvent was removed in vac...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Secondary amine
Tertiary amine
C1CCNC1
C1CC[NH]C1
c1ccccc1.c1ccccc1.C1CC[NH]C1.c1ccccc1.c1ccccc1
HBr
CC(CC)=O
null
null
BrC(c1ccccc1)c1ccccc1.CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCNC1>CC(CC)=O>CN(CC(=O)N(c1ccccc1)c1ccccc1)[C@@H]1CCN(C(c2ccccc2)c2ccccc2)C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-822d7d076ac1463281ca632d166946dc
CC(C)(C)OC(=O)N1C[C@H](O)C[C@H]1C(=O)O.CCO>>CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)OC(C)(C)C
C1CCC(CC1)N=C=NC2CCCCC2.C(C)(C)(C)OC(=O)N1[C@H](C(=O)O)C[C@H](C1)O.C(C)O>>CCOC(=O)[C@H]1N(C[C@@H](C1)O)C(=O)OC(C)(C)C
O[C:4](=[O:5])[C@@H:6]1[CH2:7][C@@H:8]([OH:9])[CH2:10][N:11]1[C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18].[CH3:1][CH2:2][OH:3]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@@H:8]([OH:9])[CH2:10][N:11]1[C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18]
CC(C)(C)OC(=O)N1C[C@H](O)C[C@H]1C(=O)O.CCO
CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)OC(C)(C)C
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
C1CCNC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5](-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12])-[C:13].[C;D1;H3:14]-[C:15]-[OH;D1;+0:16]>>[C:13]-[#7:5](-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12])-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:16]-[C:1...
173.5
[{"value": 173.5, "product": "CCOC(=O)[C@H]1N(C[C@@H](C1)O)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of (4R)-(tert-Butoxycarbonyl)-4-hydroxy-L-proline (26) (0.92 g, 4.0 mmol) in dry CH2Cl2 (30 ml) was added ethanol (1 ml, 21 mmol). To the reaction was added DCC (1.64 g, 8.0 mmol) and DMAP (cat) and the reaction mixture was, stirred under nitrogen at room temperature overnight. The reaction was then conce...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
C1CC[NH]C1
HO-
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
8
CC(C)(C)OC(=O)N1C[C@H](O)C[C@H]1C(=O)O.CCO>CN(C)C=1C=CN=CC1.C(Cl)Cl>CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5dc719d2fa02420b85b134fb57840152
CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)OC(C)(C)C.Cc1ccc(S(=O)(=O)Cl)cc1>>CCOC(=O)[C@@H]1C[C@@H](OS(=O)(=O)c2ccc(C)cc2)CN1C(=O)OC(C)(C)C
CCOC(=O)[C@H]1N(C[C@@H](C1)O)C(=O)OC(C)(C)C.C1(=CC=C(C=C1)S(=O)(=O)Cl)C>>CCOC(=O)[C@H]1N(C[C@@H](C1)OS(=O)(=O)C1=CC=C(C=C1)C)C(=O)OC(C)(C)C
[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@@H:8]([OH:9])[CH2:20][N:21]1[C:22](=[O:23])[O:24][C:25]([CH3:26])([CH3:27])[CH3:28].Cl[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][c:16]([CH3:17])[cH:18][cH:19]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@@H:8]([O:9][S:10](=[O:11])(=[O:12])[c:13]2[cH:14][cH:1...
CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)OC(C)(C)C.Cc1ccc(S(=O)(=O)Cl)cc1
CCOC(=O)[C@@H]1C[C@@H](OS(=O)(=O)c2ccc(C)cc2)CN1C(=O)OC(C)(C)C
null
null
N1=CC=CC=C1
Acylation
Formation of Sulfonic Esters
ad3deb6f5d4dc7823aa3ad2bfe24985be1f3e6860ff8cc0ba215d7624074ef69
ec645297cfd3107bffb1a4753ac125e48856598e58005e939bb2f0e91bf5e57c
O=S(=O)(O[C@@H]1CCNC1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[#7:7]-[C:8]-[C:9](-[OH;D1;+0:10])-[C:11]>>[#7:7]-[C:8]-[C:9](-[O;H0;D2;+0:10]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[C:11]
89.8
[{"value": 89.8, "product": "CCOC(=O)[C@H]1N(C[C@@H](C1)OS(=O)(=O)C1=CC=C(C=C1)C)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
DAY
To the solution of (2S,4R)-4-hydroxy-pyrrolidine-1,2-dicarboxylic acid-1-tert-butyl ester-2-ethyl ester (27) (1.8 g, 7 mmol) in dry pyridine (40 ml) was added p-toluenesulfonyl chloride (4.0 g, 21 mmol) under nitrogen at 0° C. The reaction mixture was kept refrigerated at 0° C. for 2 days. The reaction was then concent...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Secondary alcohol.Sulfonyl halide
Tosylate
null
null
C1CC[NH]C1.c1ccccc1
HCl
N1=CC=CC=C1
null
48
CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)OC(C)(C)C.Cc1ccc(S(=O)(=O)Cl)cc1>N1=CC=CC=C1>CCOC(=O)[C@@H]1C[C@@H](OS(=O)(=O)c2ccc(C)cc2)CN1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8f69ce2be3a64ab4ba0c5693a2c95f75
CCOC(=O)[C@@H]1C[C@@H](OS(=O)(=O)c2ccc(C)cc2)CN1C(=O)OC(C)(C)C.[N-]=[N+]=[N-]>>CCOC(=O)[C@@H]1C[C@H](N=[N+]=[N-])CN1C(=O)OC(C)(C)C
CCOC(=O)[C@H]1N(C[C@@H](C1)OS(=O)(=O)C1=CC=C(C=C1)C)C(=O)OC(C)(C)C.[N-]=[N+]=[N-].[Na+]>>CCOC(=O)[C@H]1N(C[C@H](C1)N=[N+]=[N-])C(=O)OC(C)(C)C
Cc1ccc(S(=O)(=O)O[C@@H:8]2[CH2:7][C@@H:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[N:13]([C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20])[CH2:12]2)cc1.[N-:9]=[N+:10]=[N-:11]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@H:8]([N:9]=[N+:10]=[N-:11])[CH2:12][N:13]1[C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3...
CCOC(=O)[C@@H]1C[C@@H](OS(=O)(=O)c2ccc(C)cc2)CN1C(=O)OC(C)(C)C.[N-]=[N+]=[N-]
CCOC(=O)[C@@H]1C[C@H](N=[N+]=[N-])CN1C(=O)OC(C)(C)C
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
cf780355dc56581e8d37046459aa1a19ddbf607b31eb6c95196e260e01e63476
6961229e10e0db3c410e97098a5b94923cb09bb1c069f267ae4410afd98cc24e
C1CCNC1
C-c1:c:c:c(-S(=O)(=O)-O-[C@H;D3;+0:1]2-[C:2]-[#7:3](-[C:4](=[O;D1;H0:5])-[#8:6]-[C:7](-[C;D1;H3:8])(-[C;D1;H3:9])-[C;D1;H3:10])-[C:11](-[C:12](-[#8:13])=[O;D1;H0:14])-[C:15]-2):c:c:1.[N-;H0;D1:16]=[#7;+:17]=[N;-;D1;H0:18]>>[#8:13]-[C:12](=[O;D1;H0:14])-[C:11]1-[C:15]-[C@H;D3;+0:1](-[N;H0;D2;+0:16]=[#7;+:17]=[N;-;D1;H0:...
null
[]
null
null
8
HOUR
To the solution of (2S,4R)-4-(toluene-4-sulfonyloxy)-pyrrolidine-1,2-dicarboxylic acid-1-tert-butyl ester-2-ethyl ester) (28) (2.6 g, 6.3 mmol) in dry DMF (15 ml) was added NaN3 (0.41 g, 6.3 mmol). The reaction mixture was stirred at room temperature overnight. The reaction mixture was then concentrated under reduced p...
10.6084/m9.figshare.5104873.v1
null
Tosylate
Azide
c1ccccc1.C1CC[NH]C1
C1CC[NH]C1
C1CC[NH]C1
TsOH.HO-
CN(C)C=O
null
8
CCOC(=O)[C@@H]1C[C@@H](OS(=O)(=O)c2ccc(C)cc2)CN1C(=O)OC(C)(C)C.[N-]=[N+]=[N-]>CN(C)C=O>CCOC(=O)[C@@H]1C[C@H](N=[N+]=[N-])CN1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0eb52d540c8643569b4e14c25cf6b4c8
CCOC(=O)[C@@H]1C[C@H](N=[N+]=[N-])CN1C(=O)OC(C)(C)C>>CCOC(=O)[C@@H]1C[C@H](N)CN1C(=O)OC(C)(C)C
CCOC(=O)[C@H]1N(C[C@H](C1)N=[N+]=[N-])C(=O)OC(C)(C)C>>CCOC(=O)[C@H]1N(C[C@H](C1)N)C(=O)OC(C)(C)C
[N-]=[N+]=[N:9][C@H:8]1[CH2:7][C@@H:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[N:11]([C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18])[CH2:10]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@H:8]([NH2:9])[CH2:10][N:11]1[C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18]
CCOC(=O)[C@@H]1C[C@H](N=[N+]=[N-])CN1C(=O)OC(C)(C)C
CCOC(=O)[C@@H]1C[C@H](N)CN1C(=O)OC(C)(C)C
null
[Pd]
CO
Reduction
Azide to amine reduction (Staudinger)
4c9e4990dae2bb965dec06bd45e318560989ee3681b61e443f7aa363b7cfa222
cd009d687d606bf351eac9390a176d16be38f2c8216a599b398641009c215027
C1CCNC1
[#7:1]-[C:2]-[C:3](-[N;H0;D2;+0:4]=[N+]=[N-])-[C:5]>>[#7:1]-[C:2]-[C:3](-[NH2;D1;+0:4])-[C:5]
175.1
[{"value": 175.1, "product": "CCOC(=O)[C@H]1N(C[C@H](C1)N)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
To the solution of (2S,4S)-4-azido-pyrrolidin-1,2-dicarboxylic acid-1-tert-butyl ester-2-ethyl ester (29) (1.8 g, 2.1 mmol) in CH3OH (40 ml) was added Pd/C 10% (50 mg). The resulting slurry was hydrogenated at 1 atm for 24 hours. The catalyst was filtered through Celite and filtrate evaporated under reduced pressure to...
10.6084/m9.figshare.5104873.v1
null
Azide
Primary amine
null
null
C1CC[NH]C1
Other
[Pd].CO
null
24
CCOC(=O)[C@@H]1C[C@H](N=[N+]=[N-])CN1C(=O)OC(C)(C)C>[Pd].CO>CCOC(=O)[C@@H]1C[C@H](N)CN1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a777f1168cba4253ad0ab4561a06139a
CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1.COc1c(C(C)(C)C)cc(C(=O)O)cc1C(C)(C)C>>CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1C(=O)c1cc(C(C)(C)C)c(OC)c(C(C)(C)C)c1
C(CCl)Cl.C(C)OC(=O)[C@H]1NC[C@H](C1)NC(CCCCC(C1=CC=C(C=C1)F)C1=CC=C(C=C1)F)=O.C(C)(C)(C)C=1C=C(C(=O)O)C=C(C1OC)C(C)(C)C>>C(C)OC(=O)[C@H]1N(C[C@H](C1)NC(CCCCC(C1=CC=C(C=C1)F)C1=CC=C(C=C1)F)=O)C(C1=CC(=C(C(=C1)C(C)(C)C)OC)C(C)(C)C)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@H:8]([NH:9][C:10](=[O:11])[CH2:12][CH2:13][CH2:14][CH2:15][CH:16]([c:17]2[cH:18][cH:19][c:20]([F:21])[cH:22][cH:23]2)[c:24]2[cH:25][cH:26][c:27]([F:28])[cH:29][cH:30]2)[CH2:31][NH:32]1.O[C:33](=[O:34])[c:35]1[cH:36][c:37]([C:38]([CH3:39])([CH3:40])[CH3:41])[c:42]([O:43...
CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1.COc1c(C(C)(C)C)cc(C(=O)O)cc1C(C)(C)C
CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1C(=O)c1cc(C(C)(C)C)c(OC)c(C(C)(C)C)c1
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
a590d96426a2fbaed42913d9daf8a16471a16de4978200f1d35a30a10009ebe7
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CCCCC(c1ccccc1)c1ccccc1)N[C@H]1CCN(C(=O)c2ccccc2)C1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C:10]1-[C:11]-[C:12]-[C:13]-[NH;D2;+0:14]-1>>[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C:10]1-[C:11]-[C:12]-[C:13]-[N;H0;D3;+0:14]-1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
75.7
[{"value": 75.7, "product": "C(C)OC(=O)[C@H]1N(C[C@H](C1)NC(CCCCC(C1=CC=C(C=C1)F)C1=CC=C(C=C1)F)=O)C(C1=CC(=C(C(=C1)C(C)(C)C)OC)C(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To the solution of (2S,4S)-4-[6,6-Bis-(4-fluoro-phenyl)-hexanoylamino]-pyrrolidine-2-carboxylic acid ethyl ester (32) (0.39 g, 0.88 mmol) in dry CH2Cl2 (20 ml) was added 3,5-di-tert-butyl-4-methoxy benzoic acid (0.23 g, 0.88 mmol). To the reaction was added EDC (0.34 g, 1.76 mmol) and DMAP (cat), and the reaction mixtu...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNC1
C1CC[NH]C1
C1CC[NH]C1.c1ccccc1.c1ccccc1.c1ccccc1
HO-
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
8
CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1.COc1c(C(C)(C)C)cc(C(=O)O)cc1C(C)(C)C>CN(C)C=1C=CN=CC1.C(Cl)Cl>CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1C(=O)c1cc(C(C)(C)C)c(OC)c(C(C)(C)C)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7f009c52032d459bb8dea3aedafca017
CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1C(=O)c1cc(C(C)(C)C)c(OC)c(C(C)(C)C)c1>>COc1c(C(C)(C)C)cc(C(=O)N2C[C@@H](NC(=O)CCCCC(c3ccc(F)cc3)c3ccc(F)cc3)C[C@H]2C(=O)O)cc1C(C)(C)C
C(C)OC(=O)[C@H]1N(C[C@H](C1)NC(CCCCC(C1=CC=C(C=C1)F)C1=CC=C(C=C1)F)=O)C(C1=CC(=C(C(=C1)C(C)(C)C)OC)C(C)(C)C)=O.[Li+].[OH-]>>FC1=CC=C(C=C1)C(CCCCC(=O)N[C@H]1C[C@H](N(C1)C(C1=CC(=C(C(=C1)C(C)(C)C)OC)C(C)(C)C)=O)C(=O)O)C1=CC=C(C=C1)F
CC[O:42][C:40]([C@H:39]1[N:13]([C:11]([c:10]2[cH:9][c:4]([C:5]([CH3:6])([CH3:7])[CH3:8])[c:3]([O:2][CH3:1])[c:44]([C:45]([CH3:46])([CH3:47])[CH3:48])[cH:43]2)=[O:12])[CH2:14][C@@H:15]([NH:16][C:17](=[O:18])[CH2:19][CH2:20][CH2:21][CH2:22][CH:23]([c:24]2[cH:25][cH:26][c:27]([F:28])[cH:29][cH:30]2)[c:31]2[cH:32][cH:33][c...
CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1C(=O)c1cc(C(C)(C)C)c(OC)c(C(C)(C)C)c1
COc1c(C(C)(C)C)cc(C(=O)N2C[C@@H](NC(=O)CCCCC(c3ccc(F)cc3)c3ccc(F)cc3)C[C@H]2C(=O)O)cc1C(C)(C)C
null
null
O.CO.C1CCOC1
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(CCCCC(c1ccccc1)c1ccccc1)N[C@H]1CCN(C(=O)c2ccccc2)C1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4]-[#7:5]>>[#7:5]-[C:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
75.4
[{"value": 75.4, "product": "FC1=CC=C(C=C1)C(CCCCC(=O)N[C@H]1C[C@H](N(C1)C(C1=CC(=C(C(=C1)C(C)(C)C)OC)C(C)(C)C)=O)C(=O)O)C1=CC=C(C=C1)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To the solution of (2S,4S)-4-[6,6-Bis-(4-fluoro-phenyl)-hexanoylamino]-1-(3,5-di-tert-butyl-4-methoxy-benzoyl)-pyrrolidine-2-carboxylic acid ethyl ester (33) (0.32 g, 0.52 mmol) in THF (15 ml), MeOH (5 ml) and water (5 ml) was added LiOH (0.1 g, 2.45 mmol), and the reaction mixture was stirred at room temperature overn...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.C1CC[NH]C1.c1ccccc1.c1ccccc1
Other
O.CO.C1CCOC1
null
8
CCOC(=O)[C@@H]1C[C@H](NC(=O)CCCCC(c2ccc(F)cc2)c2ccc(F)cc2)CN1C(=O)c1cc(C(C)(C)C)c(OC)c(C(C)(C)C)c1>O.CO.C1CCOC1>COc1c(C(C)(C)C)cc(C(=O)N2C[C@@H](NC(=O)CCCCC(c3ccc(F)cc3)c3ccc(F)cc3)C[C@H]2C(=O)O)cc1C(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bac9ddbcb8d04a9bba676089661f1a08
BrC(c1ccccc1)c1ccccc1.CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1>>CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1C(c1ccccc1)c1ccccc1
BrC(C1=CC=CC=C1)C1=CC=CC=C1.C(C)OC(=O)[C@H]1NC[C@H](C1)NC(CC(C1=CC=CC=C1)C1=CC=CC=C1)=O.C(=O)([O-])[O-].[K+].[K+]>>C(C)OC(=O)[C@H]1N(C[C@H](C1)NC(CC(C1=CC=CC=C1)C1=CC=CC=C1)=O)C(C1=CC=CC=C1)C1=CC=CC=C1
Br[CH:28]([c:29]1[cH:30][cH:31][cH:32][cH:33][cH:34]1)[c:35]1[cH:36][cH:37][cH:38][cH:39][cH:40]1.[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@H:8]([NH:9][C:10](=[O:11])[CH2:12][CH:13]([c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[CH2:26][NH:27]1>>[CH3:1][CH2:2][O:3][C:4...
BrC(c1ccccc1)c1ccccc1.CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1
CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1C(c1ccccc1)c1ccccc1
null
null
CC(CC)=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
10cc789bcfe0ae11c7b2b474c79d3cdda850354ad720004a77dedb66c0fbd515
fb63ba09935e18320be03869002f6d5d0f0321fe7dbcd94a5ae956c3effd182d
O=C(CC(c1ccccc1)c1ccccc1)N[C@H]1CCN(C(c2ccccc2)c2ccccc2)C1
Br-[CH;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7].[C:8]-[#8:9]-[C:10](=[O;D1;H0:11])-[C:12]1-[C:13]-[C:14]-[C:15]-[NH;D2;+0:16]-1>>[C:8]-[#8:9]-[C:10](=[O;D1;H0:11])-[C:12]1-[C:13]-[C:14]-[C:15]-[N;H0;D3;+0:16]-1-[CH;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7]
57.2
[{"value": 57.2, "product": "C(C)OC(=O)[C@H]1N(C[C@H](C1)NC(CC(C1=CC=CC=C1)C1=CC=CC=C1)=O)C(C1=CC=CC=C1)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of bromodiphenylmethane (0.4 g, 1.64 mmol) in butanone (10 ml) was added (2S,4S)-4-(3,3-diphenyl-propionylamino)-pyrrolidine-2-carboxylic acid ethyl ester (36) (0.6 g, 1.64 mmol), K2CO3 (0.23 g, 1.64 mmol) and KI (0.27 g, 1.64 mmol). The mixture was heated under reflux for 18 hours, and then filtered and ...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Secondary amine
Tertiary amine
C1CCNC1
C1CC[NH]C1
C1CC[NH]C1.c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
HBr
CC(CC)=O
null
null
BrC(c1ccccc1)c1ccccc1.CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1>CC(CC)=O>CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1C(c1ccccc1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-796be2c3ca244a2cbb9c89a0b40f9d1a
CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1C(c1ccccc1)c1ccccc1>>O=C(CC(c1ccccc1)c1ccccc1)N[C@H]1C[C@@H](C(=O)O)N(C(c2ccccc2)c2ccccc2)C1
C(C)OC(=O)[C@H]1N(C[C@H](C1)NC(CC(C1=CC=CC=C1)C1=CC=CC=C1)=O)C(C1=CC=CC=C1)C1=CC=CC=C1.[Li+].[OH-]>>C(C1=CC=CC=C1)(C1=CC=CC=C1)N1[C@@H](C[C@@H](C1)NC(CC(C1=CC=CC=C1)C1=CC=CC=C1)=O)C(=O)O
CC[O:23][C:21]([C@@H:20]1[CH2:19][C@H:18]([NH:17][C:2](=[O:1])[CH2:3][CH:4]([c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[CH2:38][N:24]1[CH:25]([c:26]1[cH:27][cH:28][cH:29][cH:30][cH:31]1)[c:32]1[cH:33][cH:34][cH:35][cH:36][cH:37]1)=[O:22]>>[O:1]=[C:2]([CH2:3][CH:4]([c:5]1[cH:6][cH...
CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1C(c1ccccc1)c1ccccc1
O=C(CC(c1ccccc1)c1ccccc1)N[C@H]1C[C@@H](C(=O)O)N(C(c2ccccc2)c2ccccc2)C1
null
null
O.CO.C1CCOC1
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(CC(c1ccccc1)c1ccccc1)N[C@H]1CCN(C(c2ccccc2)c2ccccc2)C1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4]-[#7:5]>>[#7:5]-[C:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
47.6
[{"value": 47.6, "product": "C(C1=CC=CC=C1)(C1=CC=CC=C1)N1[C@@H](C[C@@H](C1)NC(CC(C1=CC=CC=C1)C1=CC=CC=C1)=O)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To the solution of (2S,4S)-1-benzhydryl-4-(3,3-diphenyl-propionylamino)-pyrrolidine-2-carboxylic acid ethyl ester (37) (0.25 g, 0.5 mmol) in THF (15 ml), MeOH (5 ml) and water (5 ml) was added LiOH (0.1 g, 2.45 mmol), and the reaction mixture was stirred at room temperature overnight. The reaction was then concentrated...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.C1CC[NH]C1.c1ccccc1.c1ccccc1
Other
O.CO.C1CCOC1
null
8
CCOC(=O)[C@@H]1C[C@H](NC(=O)CC(c2ccccc2)c2ccccc2)CN1C(c1ccccc1)c1ccccc1>O.CO.C1CCOC1>O=C(CC(c1ccccc1)c1ccccc1)N[C@H]1C[C@@H](C(=O)O)N(C(c2ccccc2)c2ccccc2)C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-13e9753f36934bee8bf2fae8a1e16e7b
CC(C)(C)OC(=O)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O>>NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
C(C)(C)(C)OC(NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O)=O.C(F)(F)(F)C(=O)O>>NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O
CC(C)(C)OC(=O)[NH:1][CH:2]1[CH2:3][CH2:4][N:5]([CH:6]([c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[C:19]1=[O:20]>>[NH2:1][CH:2]1[CH2:3][CH2:4][N:5]([CH:6]([c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[C:19]1=[O:20]
CC(C)(C)OC(=O)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
null
null
C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=C1CCCN1C(c1ccccc1)c1ccccc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]1-[C:3]-[C:4]-[#7:5](-[C:6])-[C:7]-1=[O;D1;H0:8]>>[C:6]-[#7:5]1-[C:4]-[C:3]-[C:2](-[NH2;D1;+0:1])-[C:7]-1=[O;D1;H0:8]
97
[{"value": 97.0, "product": "NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To the solution of (1-benzhydryl-2-oxo-pyrrollidin-3-yl)-carbamic acid tert-butyl ester (41) (1.2 g, 3.26 mmol) in CH2Cl2 (20 ml) was added CF3CO2H (8 ml). The resulting mixture was stirred under nitrogen at room temperature overnight. The reaction was then concentrated under reduced pressure. The residue was dissolved...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
C1CC[NH]C1.c1ccccc1.c1ccccc1
HO-
C(Cl)Cl
null
8
CC(C)(C)OC(=O)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O>C(Cl)Cl>NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c05a6af839be4448b137432d6475a7b3
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(O)CC(c1ccccc1)c1ccccc1>>O=C(CC(c1ccccc1)c1ccccc1)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
C(CCl)Cl.NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O.C1(=CC=CC=C1)C(CC(=O)O)C1=CC=CC=C1>>C(C1=CC=CC=C1)(C1=CC=CC=C1)N1C(C(CC1)NC(CC(C1=CC=CC=C1)C1=CC=CC=C1)=O)=O
[NH2:17][CH:18]1[CH2:19][CH2:20][N:21]([CH:22]([c:23]2[cH:24][cH:25][cH:26][cH:27][cH:28]2)[c:29]2[cH:30][cH:31][cH:32][cH:33][cH:34]2)[C:35]1=[O:36].O[C:2](=[O:1])[CH2:3][CH:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[O:1]=[C:2]([CH2:3][CH:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][c...
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(O)CC(c1ccccc1)c1ccccc1
O=C(CC(c1ccccc1)c1ccccc1)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(CC(c1ccccc1)c1ccccc1)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[C:5]-[#7:6]1-[C:7]-[C:8]-[C:9](-[NH2;D1;+0:10])-[C:11]-1=[O;D1;H0:12]>>[C:5]-[#7:6]1-[C:7]-[C:8]-[C:9](-[NH;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4])-[C:11]-1=[O;D1;H0:12]
70
[{"value": 70.0, "product": "C(C1=CC=CC=C1)(C1=CC=CC=C1)N1C(C(CC1)NC(CC(C1=CC=CC=C1)C1=CC=CC=C1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 3-amino-1-benzhydryl-pyrrolidin-2-one (42) (0.2 g, 0.75 mmol) in dry CH2Cl2 (20 ml)was added 3,3-diphenylpropionic acid (0.19 g, 0.82 mmol) under nitrogen. To the reaction was added EDC (0.18 g, 0.9 mmol) and DMAP (cat), and the reaction mixture was stirred under nitrogen at room temperature overnight....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.C1CC[NH]C1.c1ccccc1.c1ccccc1
HO-
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
8
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(O)CC(c1ccccc1)c1ccccc1>CN(C)C=1C=CN=CC1.C(Cl)Cl>O=C(CC(c1ccccc1)c1ccccc1)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-90252da0f3144d0e85fb42da01f4d4d5
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C=NC(c1ccccc1)c1ccccc1>>O=C(NC1CCN(C(c2ccccc2)c2ccccc2)C1=O)NC(c1ccccc1)c1ccccc1
NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O.C1(=CC=CC=C1)C(C1=CC=CC=C1)N=C=O>>C(C1=CC=CC=C1)(C1=CC=CC=C1)NC(=O)NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O
[NH2:3][CH:4]1[CH2:5][CH2:6][N:7]([CH:8]([c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[C:21]1=[O:22].[O:1]=[C:2]=[N:23][CH:24]([c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1)[c:31]1[cH:32][cH:33][cH:34][cH:35][cH:36]1>>[O:1]=[C:2]([NH:3][CH:4]1[CH2:5][CH2:6][N:7]([CH:8]([c:9]2[cH:...
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C=NC(c1ccccc1)c1ccccc1
O=C(NC1CCN(C(c2ccccc2)c2ccccc2)C1=O)NC(c1ccccc1)c1ccccc1
null
null
C(Cl)Cl
Acylation
Urea synthesis via isocyanate and primary amine
d39cd7dc52a79bb265ff8ef61ef7bf9dc7f7b5fb0150fcb4881bdfb18ab9c380
a5dc801930c765d2a435a0a2973e50163c305ba8e7641d6adbcc1550b7b96de7
O=C(NC1CCN(C(c2ccccc2)c2ccccc2)C1=O)NC(c1ccccc1)c1ccccc1
[C:1]-[#7:2]1-[C:3]-[C:4]-[C:5](-[NH2;D1;+0:6])-[C:7]-1=[O;D1;H0:8].[O;D1;H0:9]=[C;H0;D2;+0:10]=[N;H0;D2;+0:11]-[C:12](-[c:13])-[c:14]>>[C:1]-[#7:2]1-[C:3]-[C:4]-[C:5](-[NH;D2;+0:6]-[C;H0;D3;+0:10](=[O;D1;H0:9])-[NH;D2;+0:11]-[C:12](-[c:13])-[c:14])-[C:7]-1=[O;D1;H0:8]
65
[{"value": 65.0, "product": "C(C1=CC=CC=C1)(C1=CC=CC=C1)NC(=O)NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
DAY
To a solution of 3-amino-1-benzhydryl-pyrrolidin-2-one (42) (0.2 g, 0.75 mmol) in dry CH2Cl2 (15 ml) was added diphenylmethyl isocyanate (0.17 mg, 0.82 mmol) dropwise under nitrogen. The resulting mixture was stirred at room temperature for two days followed by refluxing for 5 hours. Removal of solvent under reduced pr...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Primary amine
Urea
null
null
C1CC[NH]C1.c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
null
C(Cl)Cl
null
48
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C=NC(c1ccccc1)c1ccccc1>C(Cl)Cl>O=C(NC1CCN(C(c2ccccc2)c2ccccc2)C1=O)NC(c1ccccc1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-14563a3db8c14122aafee18220f7b5df
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(O)CN(c1ccccc1)c1ccccc1>>O=C(CN(c1ccccc1)c1ccccc1)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
C(CCl)Cl.NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O.C1(=CC=CC=C1)N(C1=CC=CC=C1)CC(=O)O>>C(C1=CC=CC=C1)(C1=CC=CC=C1)N1C(C(CC1)NC(CN(C1=CC=CC=C1)C1=CC=CC=C1)=O)=O
[NH2:17][CH:18]1[CH2:19][CH2:20][N:21]([CH:22]([c:23]2[cH:24][cH:25][cH:26][cH:27][cH:28]2)[c:29]2[cH:30][cH:31][cH:32][cH:33][cH:34]2)[C:35]1=[O:36].O[C:2](=[O:1])[CH2:3][N:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[O:1]=[C:2]([CH2:3][N:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:...
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(O)CN(c1ccccc1)c1ccccc1
O=C(CN(c1ccccc1)c1ccccc1)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(CN(c1ccccc1)c1ccccc1)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[C:5]-[#7:6]1-[C:7]-[C:8]-[C:9](-[NH2;D1;+0:10])-[C:11]-1=[O;D1;H0:12]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:10]-[C:9]1-[C:8]-[C:7]-[#7:6](-[C:5])-[C:11]-1=[O;D1;H0:12]
69
[{"value": 69.0, "product": "C(C1=CC=CC=C1)(C1=CC=CC=C1)N1C(C(CC1)NC(CN(C1=CC=CC=C1)C1=CC=CC=C1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 3-amino-1-benzhydryl-pyrrolidin-2-one (42) (0.2 g, 0.75 mmol) in dry CH2Cl2 (20 ml)was added diphenylamino ethanoic acid (0.19 g, 0.82 mmol) under nitrogen. To the reaction was added EDC (0.18 g, 0.9 mmol) and DMAP (cat) and the reaction mixture was stirred under nitrogen at room temperature overnight....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.C1CC[NH]C1.c1ccccc1.c1ccccc1
HO-
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
8
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(O)CN(c1ccccc1)c1ccccc1>CN(C)C=1C=CN=CC1.C(Cl)Cl>O=C(CN(c1ccccc1)c1ccccc1)NC1CCN(C(c2ccccc2)c2ccccc2)C1=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f49a2e9c3a4b49999eae65a12fbe610b
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(CBr)N(c1ccccc1)c1ccccc1>>O=C(CNC1CCN(C(c2ccccc2)c2ccccc2)C1=O)N(c1ccccc1)c1ccccc1
NC1C(N(CC1)C(C1=CC=CC=C1)C1=CC=CC=C1)=O.BrCC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1.[H-].[Na+]>>C(C1=CC=CC=C1)(C1=CC=CC=C1)N1C(C(CC1)NCC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1)=O
[NH2:4][CH:5]1[CH2:6][CH2:7][N:8]([CH:9]([c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[C:22]1=[O:23].Br[CH2:3][C:2](=[O:1])[N:24]([c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1)[c:31]1[cH:32][cH:33][cH:34][cH:35][cH:36]1>>[O:1]=[C:2]([CH2:3][NH:4][CH:5]1[CH2:6][CH2:7][N:8]([CH:9]...
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(CBr)N(c1ccccc1)c1ccccc1
O=C(CNC1CCN(C(c2ccccc2)c2ccccc2)C1=O)N(c1ccccc1)c1ccccc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of primary amines with alkyl halides
fc19a1445ff204e66e51735d0191465bda3c6691fd233624a54742c9d4828411
0b1d32f56ad00f1e5bdae9390f9227bbea012fa2f8203aac34726b8a6761cc7c
O=C(CNC1CCN(C(c2ccccc2)c2ccccc2)C1=O)N(c1ccccc1)c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#7:4](-[c:5])-[c:6].[C:7]-[#7:8]1-[C:9]-[C:10]-[C:11](-[NH2;D1;+0:12])-[C:13]-1=[O;D1;H0:14]>>[C:7]-[#7:8]1-[C:9]-[C:10]-[C:11](-[NH;D2;+0:12]-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#7:4](-[c:5])-[c:6])-[C:13]-1=[O;D1;H0:14]
73
[{"value": 73.0, "product": "C(C1=CC=CC=C1)(C1=CC=CC=C1)N1C(C(CC1)NCC(=O)N(C1=CC=CC=C1)C1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 3-amino-1-benzhydryl-pyrrolidin-2-one (42) (0.2 g, 0.75 mmol in dry DMF (15 ml) was added 2-bromo-N,N-diphenyl acetamide (0.24 g, 0.82 mmol) and NaH (50 mg) under nitrogen. The reaction mixture was heated at 100 degrees overnight. After cooling, the solvent was evaporated and residue was taken up with ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary amine
Secondary amine
null
null
C1CC[NH]C1.c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
HBr
CN(C)C=O
null
null
NC1CCN(C(c2ccccc2)c2ccccc2)C1=O.O=C(CBr)N(c1ccccc1)c1ccccc1>CN(C)C=O>O=C(CNC1CCN(C(c2ccccc2)c2ccccc2)C1=O)N(c1ccccc1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e83a7c5d5f0b4d529f6aaf0097ae6224
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1.NS(=O)(=O)c1ccccc1>>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccccc4)oc3C)cc2)cc1
COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O.Cl.CN(CCCN=C=NCC)C.C1(=CC=CC=C1)S(=O)(=O)N>>COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=CC=CC=C1
O[C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:34][cH:33]3)[cH:32][cH:31]2)[c:29]([CH3:30])[o:28]1)=[O:17].[NH2:18][S:19](=[O:20])(=[O:21])[c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([O:11][CH2:...
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1.NS(=O)(=O)c1ccccc1
COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccccc4)oc3C)cc2)cc1
null
CN(C)C1=CC=NC=C1
ClCCl
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(COc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[c:3](:[c:4]):[#8;a:5]:[c:6]
8.5
[{"value": 8.5, "product": "COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A stirred solution of 4-(4′-methoxy-biphenyl-4-yloxymethyl)-5-methyl-furan-2-carboxylic acid (4) (250 mg) in dichloromethane (50 mL) was treated with 1-(3-dimethylaminopropyl)-3-ethylcarbodiimide hydrochloride (142 mg), 4-(N,N-dimethylamino)pyridine (2 mg) and benzenesulfonamide (232 mg). After 16 hours the reaction mi...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccoc1.c1ccccc1
HO-
CN(C)C1=CC=NC=C1.ClCCl
null
null
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1.NS(=O)(=O)c1ccccc1>CN(C)C1=CC=NC=C1.ClCCl>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccccc4)oc3C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-14da1013d149444fadc18cb28ff0aae9
CC(C)(C)OC(=O)NCc1ccc(S(N)(=O)=O)cc1.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1>>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccc(CN)cc4)oc3C)cc2)cc1
COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O.C(C)(C)(C)OC(NCC1=CC=C(C=C1)S(N)(=O)=O)=O.C(N)(OC(C)(C)C)=O.FC(C(=O)O)(F)F.ClCCl>>FC(C(=O)O)(F)F.NCC1=CC=C(C=C1)S(=O)(=O)NC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=C(C=C1)OC)C
CC(C)(C)OC(=O)[NH:27][CH2:26][c:25]1[cH:24][cH:23][c:22]([S:19]([NH2:18])(=[O:20])=[O:21])[cH:29][cH:28]1.O[C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:36][cH:35]3)[cH:34][cH:33]2)[c:31]([CH3:32])[o:30]1)=[O:17]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2...
CC(C)(C)OC(=O)NCc1ccc(S(N)(=O)=O)cc1.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccc(CN)cc4)oc3C)cc2)cc1
null
null
null
Acylation
OtherReaction
a760ca44badae53cef3a44d9b0c4e8bf45a42ef421ec54275506cdd614b80a67
840e1f09c3507b8ae193cb274981cf3e3bee243853f088474eb17d6f0eb72564
O=C(NS(=O)(=O)c1ccccc1)c1cc(COc2ccc(-c3ccccc3)cc2)co1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]-[c:3].[NH2;D1;+0:4]-[#16:5](=[O;D1;H0:6])(=[O;D1;H0:7])-[c:8].O-[C;H0;D3;+0:9](=[O;D1;H0:10])-[c:11](:[c:12]):[#8;a:13]:[c:14]>>[NH2;D1;+0:1]-[C:2]-[c:3].[O;D1;H0:10]=[C;H0;D3;+0:9](-[NH;D2;+0:4]-[#16:5](=[O;D1;H0:6])(=[O;D1;H0:7])-[c:8])-[c:11](:[c:12]):[#8;a:13]:[c:14]
null
[]
null
null
null
null
4-(4′-Methoxy-biphenyl-4-yloxymethyl)-5-methyl-furan-2-carboxylic acid (4) (50 mg) was reacted with (4-sulphamoyl-benzyl)-carbamic acid tert-butyl ester (85 mg) in an analogous manner to that described in Example 2A. The intermediate tert-butyl carbamate was hydrolysed with 1% trifluoroacetic acid/dichloromethane over ...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carbamic ester.Carboxylic acid.Ether.Boc
Sulfonamide.Secondary amide.Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccoc1.c1ccccc1
HO-
null
null
null
CC(C)(C)OC(=O)NCc1ccc(S(N)(=O)=O)cc1.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1>>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccc(CN)cc4)oc3C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cda13cc1515e4528b0f71e0e93e8c05c
CC(=O)Oc1ccc(S(N)(=O)=O)cc1.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1>>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccc(O)cc4)oc3C)cc2)cc1
C[O-].[Na+].COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O.S(N)(=O)(=O)C1=CC=C(C=C1)OC(C)=O>>OC1=CC=C(C=C1)S(=O)(=O)NC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=C(C=C1)OC)C
CC(=O)[O:26][c:25]1[cH:24][cH:23][c:22]([S:19]([NH2:18])(=[O:20])=[O:21])[cH:28][cH:27]1.O[C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:35][cH:34]3)[cH:33][cH:32]2)[c:30]([CH3:31])[o:29]1)=[O:17]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10...
CC(=O)Oc1ccc(S(N)(=O)=O)cc1.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccc(O)cc4)oc3C)cc2)cc1
null
null
O.CO
Acylation
OtherReaction
ccf63ed2558f3e347d41fcbfdfe7add29165cbb3f81591cb16bdfafb45c4bfd8
97f370026ca06570a9ea0c7cfeec3690633e89955cf72b7ca0b6e4c204c30702
O=C(NS(=O)(=O)c1ccccc1)c1cc(COc2ccc(-c3ccccc3)cc2)co1
C-C(=O)-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4].[NH2;D1;+0:5]-[#16:6](=[O;D1;H0:7])(=[O;D1;H0:8])-[c:9].O-[C;H0;D3;+0:10](=[O;D1;H0:11])-[c:12](:[c:13]):[#8;a:14]:[c:15]>>[O;D1;H0:11]=[C;H0;D3;+0:10](-[NH;D2;+0:5]-[#16:6](=[O;D1;H0:7])(=[O;D1;H0:8])-[c:9])-[c:12](:[c:13]):[#8;a:14]:[c:15].[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
20.6
[{"value": 20.6, "product": "OC1=CC=C(C=C1)S(=O)(=O)NC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=C(C=C1)OC)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
4-(4′-Methoxy-biphenyl-4-yloxymethyl)-5-methyl-furan-2-carboxylic acid (4) (50 mg) was reacted with acetic acid 4-sulphamoyl-phenyl ester (64 mg) in an analogous manner to that described in Example 2A. The acetic ester intermediate was hydrolysed with sodium methoxide (80 mg) in a mixture of methanol (10 mL) and water ...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid.Ester
Sulfonamide.Secondary amide.Aromatic alcohol
null
null
c1ccccc1.c1ccccc1.c1ccoc1.c1ccccc1
HO-
O.CO
null
null
CC(=O)Oc1ccc(S(N)(=O)=O)cc1.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1>O.CO>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccc(O)cc4)oc3C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-dd218db336c3408d83fea32600257830
COC(=O)Cl.Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C>>COC(=O)c1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
[Cl-].[NH4+].C(C)(CC)[Li].C(C)(C)[Si](OCC1=C(OC=C1)C)(C(C)C)C(C)C.ClC(=O)OC>>COC(=O)C=1OC(=C(C1)CO[Si](C(C)C)(C(C)C)C(C)C)C
Cl[C:3]([O:2][CH3:1])=[O:4].[cH:5]1[cH:6][c:7]([CH2:8][O:9][Si:10]([CH:11]([CH3:12])[CH3:13])([CH:14]([CH3:15])[CH3:16])[CH:17]([CH3:18])[CH3:19])[c:20]([CH3:21])[o:22]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][Si:10]([CH:11]([CH3:12])[CH3:13])([CH:14]([CH3:15])[CH3:16])[CH:17]([CH3:18])[CH3:19])[c:20](...
COC(=O)Cl.Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C
COC(=O)c1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
null
null
O1CCCC1
C-C Coupling
Friedel-Crafts acylation
1c39f06f701be9363365d1994407a43ecc223155f8d909b9c19badfc90d9f29d
25d9bd8621b941df428c033fedc648334f6dc6f4157dff30f33212e6bac7f1de
c1ccoc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].[#8;a:5]1:[c:6]:[c:7]:[c:8]:[cH;D2;+0:9]:1>>[C;D1;H3:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c;H0;D3;+0:9]1:[#8;a:5]:[c:6]:[c:7]:[c:8]:1
null
[]
null
null
1
HOUR
A solution of triisopropyl-(2-methyl-furan-3-ylmethoxy)-silane (14) (10.0 g) in tetrahydrofuran (300 mL) was cooled to −78° C. with stirring was treated drop-wise with sec-butyllithium (3.0 M in cyclohexane, 37 mL). After 1 hour the reaction mixture was treated drop-wise with a solution of methyl chloroformate (5.2 g) ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether
Ester
c1ccoc1
c1ccoc1
c1ccoc1
HCl
O1CCCC1
null
1
COC(=O)Cl.Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C>O1CCCC1>COC(=O)c1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ac2ef776a5ec4e41aedf2abf920d3586
COC(=O)c1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1>>COC(=O)c1cc(CO)c(C)o1
COC(=O)C=1OC(=C(C1)CO[Si](C(C)C)(C(C)C)C(C)C)C.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC>>COC(=O)C=1OC(=C(C1)CO)C
CC(C)[Si](C(C)C)(C(C)C)[O:9][CH2:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:12][c:10]1[CH3:11]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][OH:9])[c:10]([CH3:11])[o:12]1
COC(=O)c1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
COC(=O)c1cc(CO)c(C)o1
null
null
O1CCCC1
Deprotection
Alcohol deprotection from silyl ethers
488547c1043a845c08188be7baa01e2ee1f8d7661927552d481c2d214b18b6c0
5c02ee98cb6b210a313993bea9e102110eb73637a50746f5457590f98613069b
c1ccoc1
C-C(-C)-[Si](-[O;H0;D2;+0:1]-[C:2]-[c:3]:[c:4]:[#8;a:5])(-C(-C)-C)-C(-C)-C>>[#8;a:5]:[c:4]:[c:3]-[C:2]-[OH;D1;+0:1]
null
[]
null
null
16
HOUR
A stirred solution of 5-methyl-4-triisopropylsilanyloxymethyl-furan-2-carboxylic acid methyl ester (15) (5.2 g) in tetrahydrofuran (200 mL) was treated with tetrabutylammonium fluoride (1.0 M solution in tetrahydrofuran, 3.2 mL) and stirring continued for 16 hours. The reaction mixture was concentrated in vacuo and the...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
Primary alcohol
null
null
c1ccoc1
Other
O1CCCC1
null
16
COC(=O)c1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1>O1CCCC1>COC(=O)c1cc(CO)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a7d0d0205801432b8fa8e525235e33f4
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(-c2ccccc2)cc1>>COC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
OC1=CC=C(C=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.COC(=O)C=1OC(=C(C1)CO)C.OC1=CC=C(C=C1)C1=CC=CC=C1>>COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=CC=C1)C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][OH:9])[c:22]([CH3:23])[o:24]1.O[c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[cH:20][cH:21]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][cH:18][cH:19]3)[cH:20][cH:21]2)[c:2...
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(-c2ccccc2)cc1
COC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
8915084acbaaf997bf0f89ff5187cb2f89c25dc683fffc57b3391298c8430dd9
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
O-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#8;a:6]:[c:7]:[c:8]-[C:9]-[OH;D1;+0:10]>>[#8;a:6]:[c:7]:[c:8]-[C:9]-[O;H0;D2;+0:10]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
0
CELSIUS
10
MINUTE
A solution of 4-hydroxymethyl-5-methyl-furan-2-carboxylic acid methyl ester (16) (1 g) in anhydrous tetrahydrofuran (20 mL) was cooled to 0° C. under a nitrogen atmosphere. 4-Hydroxybiphenyl (3 g) and triphenylphosphine (4.61 g) were added and the mixture was treated with di-isopropylazodicarboxylate (3.46 mL) dropwise...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HO-
O1CCCC1
0
0.166667
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(-c2ccccc2)cc1>O1CCCC1>COC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d25e81af639241ea95fb0a8d026f08b5
COC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2)cc1
[OH-].[Li+].COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=CC=C1)C>>C1(=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O)C1=CC=CC=C1
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][O:11][c:12]2[cH:13][cH:14][c:15](-[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[cH:22][cH:23]2)[cH:8]1)=[O:6]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[cH:22][cH:23]1
COC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2)cc1
null
null
O1CCCC1.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
22
[{"value": 22.0, "product": "C1(=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
1M Aqueous lithium hydroxide (18 mL) was added to solution of 4-(biphenyl-4-yloxymethyl)-5-methyl-furan-2-carboxylic acid methyl ester (17) (1 g) in tetrahydrofuran/methanol (2:1 by volume, 100 mL) and the mixture stirred at room temperature for 5 h. The solvent was removed in vacuo, the residue dissolved in water (20 ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccoc1.c1ccccc1.c1ccccc1
Other
O1CCCC1.CO
null
5
COC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1>O1CCCC1.CO>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1f48ae5b0846442abf06d18edea5ee6e
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(I)cc1>>COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1
COC(=O)C=1OC(=C(C1)CO)C.IC1=CC=C(C=C1)O.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.CC(C)OC(=O)/N=N/C(=O)OC(C)C>>COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][OH:9])[c:17]([CH3:18])[o:19]1.O[c:10]1[cH:11][cH:12][c:13]([I:14])[cH:15][cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13]([I:14])[cH:15][cH:16]2)[c:17]([CH3:18])[o:19]1
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(I)cc1
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
8915084acbaaf997bf0f89ff5187cb2f89c25dc683fffc57b3391298c8430dd9
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1ccc(OCc2ccoc2)cc1
O-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#8;a:6]:[c:7]:[c:8]-[C:9]-[OH;D1;+0:10]>>[#8;a:6]:[c:7]:[c:8]-[C:9]-[O;H0;D2;+0:10]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
63.4
[{"value": 63.4, "product": "COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-hydroxymethyl-5-methyl-furan-2-carboxylic acid methyl ester (16) (1.14 g) in tetrahydrofuran (15 mL) was cooled to 0° C. with stirring and treated with 4-iodophenol (4.6 g), triphenylphosphine (5.5 g) and diisopropylazodicarboxylate (4.2 g). After 10 minutes the cooling bath was removed. After 3 hours t...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccoc1.c1ccccc1
HO-
O1CCCC1
null
null
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(I)cc1>O1CCCC1>COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a3ea5e46e05a4ac28b7ebc9fb4b6d5dc
CC(=O)c1ccc(B(O)O)cc1.COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1>>CC(=O)c1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.C(C)(=O)C1=CC=C(C=C1)B(O)O.CN(C=O)C.C(C)(=O)[O-].[K+]>>C(C)(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
OB(O)[c:7]1[cH:6][cH:5][c:4]([C:2]([CH3:1])=[O:3])[cH:26][cH:25]1.C[O:19][C:17]([c:16]1[cH:15][c:14]([CH2:13][O:12][c:11]2[cH:10][cH:9][c:8](I)[cH:24][cH:23]2)[c:21]([CH3:22])[o:20]1)=[O:18]>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([O:12][CH2:13][c:14]3[cH:15][c:16]([C:17](=[O:18])[OH:19]...
CC(=O)c1ccc(B(O)O)cc1.COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1
CC(=O)c1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
null
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2]
ClCCl
C-C Coupling
OtherReaction
04157bef51d5543c035526858b11d2af2b78e75d38cd85edf56b617e6aebc946
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1].[c:10]:[c:9]:[c;H0;D3;+0:6](-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]):[c:7]:[c:8]
20.4
[{"value": 20.4, "product": "C(C)(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
16
HOUR
A stirred mixture of 4-(4-iodo-phenoxymethyl)-5-methyl-furan-2-carboxylic acid methyl ester (20) (0.26 g), 4-acetylphenylboronic acid (0.15 g), N,N-dimethylformamide (30 mL), potassium acetate (0.26 g) and [1,1′-bis(diphenylphosphino)ferrocene]dichloropalladium(II), complex with dichloromethane (1:1) (40 mg) was heated...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccoc1
HI.B
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].ClCCl
90
16
CC(=O)c1ccc(B(O)O)cc1.COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1>C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].ClCCl>CC(=O)c1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-df684f31504c41af9b9ddc8343cecf7c
COC(=O)c1cc(CO)c(C)o1>>COC(=O)c1cc(C(=O)O)c(C)o1
CC(=O)C.OS(=O)(=O)O.O=[Cr](=O)=O.COC(=O)C=1OC(=C(C1)CO)C>>COC(=O)C=1OC(=C(C1)C(=O)O)C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][OH:10])[c:11]([CH3:12])[o:13]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([C:8](=[O:9])[OH:10])[c:11]([CH3:12])[o:13]1
COC(=O)c1cc(CO)c(C)o1
COC(=O)c1cc(C(=O)O)c(C)o1
null
null
CC(=O)C.C(C)OCC
Oxidation
Oxidation of alcohol to carboxylic acid
b709baac44a995a9a8f6386a6b5d87f98c32eb5a0636340abc1f778fae827230
4454822e22dc2dc24e7495385256bfce456e337c240bb764261f81dbeda1aaa1
c1ccoc1
[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#8;a:5]:[c:6](-[C;D1;H3:7]):[c:8](-[CH2;D2;+0:9]-[O;D1;H1:10]):[c:11]:1>>[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#8;a:5]:[c:6](-[C;D1;H3:7]):[c:8](-[C;H0;D3;+0:9](=[O;D1;H0:12])-[O;D1;H1:10]):[c:11]:1
null
[]
null
null
5
HOUR
Jones' reagent (Prepared according to Fieser and Fieser, Reagents for Organic Synthesis, Volume 1, page 142, 1967) was added drop-wise to a stirred solution of 4-hydroxymethyl-5-methyl-furan-2-carboxylic acid methyl ester (16) (100 mg) in acetone (10 mL) until the orange colouration just remained. Stirring was continue...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Carboxylic acid
null
null
c1ccoc1
Other
CC(=O)C.C(C)OCC
null
5
COC(=O)c1cc(CO)c(C)o1>CC(=O)C.C(C)OCC>COC(=O)c1cc(C(=O)O)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-05d5003fdcd942298997f09dcba031a1
COC(=O)c1cc(C(=O)O)c(C)o1.COc1ccc(-c2ccc(N)cc2)cc1>>COc1ccc(-c2ccc(NC(=O)c3cc(C(=O)O)oc3C)cc2)cc1
COC(=O)C=1OC(=C(C1)C(=O)O)C.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1N=CC=C2)OC(=[N+](C)C)N(C)C.C(C)(C)N(CC)C(C)C.COC1=CC=C(C=C1)C1=CC=C(C=C1)N>>COC1=CC=C(C=C1)C1=CC=C(C=C1)NC(=O)C=1C=C(OC1C)C(=O)O
C[O:19][C:17]([c:16]1[cH:15][c:14]([C:12](O)=[O:13])[c:21]([CH3:22])[o:20]1)=[O:18].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([NH2:11])[cH:23][cH:24]2)[cH:25][cH:26]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([NH:11][C:12](=[O:13])[c:14]3[cH:15][c:16]([C:17](=[O:18])[OH:19])[o:2...
COC(=O)c1cc(C(=O)O)c(C)o1.COc1ccc(-c2ccc(N)cc2)cc1
COc1ccc(-c2ccc(NC(=O)c3cc(C(=O)O)oc3C)cc2)cc1
null
null
CN(C=O)C.C(C)(=O)OCC
Acylation
OtherReaction
2f4be8b14ede2d52c920d439e5f741d97aa4249f4c57807152c62994aca84307
87a69d5ad38be49e96448ab38c6e7071a2232ada5542b6b62a2f1e1b1e6e076f
O=C(Nc1ccc(-c2ccccc2)cc1)c1ccoc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#8;a:5]:[c:6](-[C;D1;H3:7]):[c:8](-[C;H0;D3;+0:9](-O)=[O;D1;H0:10]):[c:11]:1.[NH2;D1;+0:12]-[c:13](:[c:14]):[c:15]>>[C;D1;H3:7]-[c:6]1:[#8;a:5]:[c:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]):[c:11]:[c:8]:1-[C;H0;D3;+0:9](=[O;D1;H0:10])-[NH;D2;+0:12]-[c:13](:[c:14]):[c:15]
null
[]
null
null
2
HOUR
To a solution of 5-methyl-furan-2,4-dicarboxylic acid-2-methyl ester (23) (100 mg) in N,N-dimethylformamide (3.0 mL) was added O-(7-azabenzotriazol-1-yl)-N,N,N′,N′-tetramethyluronium hexafluorophosphate (228 mg), diisopropylethylamine (0.56 mL) and 4′-methoxy-biphenyl-4-ylamine (120 mg). The resulting solution was stir...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ester.Primary amine
Carboxylic acid.Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccoc1
HO-
CN(C=O)C.C(C)(=O)OCC
null
2
COC(=O)c1cc(C(=O)O)c(C)o1.COc1ccc(-c2ccc(N)cc2)cc1>CN(C=O)C.C(C)(=O)OCC>COc1ccc(-c2ccc(NC(=O)c3cc(C(=O)O)oc3C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-01f9e44084024917a8d3449096b9c05f
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1>>Cc1oc(C(=O)O)cc1COc1ccc(I)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.[OH-].[Li+].Cl>>IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][O:11][c:12]2[cH:13][cH:14][c:15]([I:16])[cH:17][cH:18]2)[cH:8]1)=[O:6]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15]([I:16])[cH:17][cH:18]1
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1
null
null
O1CCCC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(OCc2ccoc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
70.4
[{"value": 70.4, "product": "IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A stirred solution of 4-(4-iodo-phenoxymethyl)-5-methyl-furan-2-carboxylic acid methyl ester (20) (2.7 g) in tetrahydrofuran (25 mL) was treated with a solution of lithium hydroxide (1.5 g) in water (2 mL). After 3 hours the reaction mixture was diluted with water and acidified to pH 2 with 1.0 M hydrochloric acid. The...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccoc1.c1ccccc1
Other
O1CCCC1.O
null
null
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1>O1CCCC1.O>Cc1oc(C(=O)O)cc1COc1ccc(I)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b39b01417a2b446bb848c76274443639
CCOC(=O)CBr.Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C>>CCOC(=O)Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
BrCC(=O)OCC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(C)(C)[Si](OCC1=C(OC=C1)C)(C(C)C)C(C)C.C(CCC)[Li].[Cl-].O1C(=CC=C1)[Zn+]>>C(C)OC(CC=1OC(=C(C1)CO[Si](C(C)C)(C(C)C)C(C)C)C)=O
Br[CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].[cH:7]1[cH:8][c:9]([CH2:10][O:11][Si:12]([CH:13]([CH3:14])[CH3:15])([CH:16]([CH3:17])[CH3:18])[CH:19]([CH3:20])[CH3:21])[c:22]([CH3:23])[o:24]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][c:7]1[cH:8][c:9]([CH2:10][O:11][Si:12]([CH:13]([CH3:14])[CH3:15])([CH:16]([CH3:17])[CH3:18])[...
CCOC(=O)CBr.Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C
CCOC(=O)Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
null
C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2].[Cl-].[Zn+2].[Cl-]
O1CCCC1
C-C Coupling
Friedel-Crafts alkylation with halide
93fdde097896472bfc12eb49e0fb34940611c3ffece494af1ba9bc1fd805c2ea
0061a06af9fc64155952582b91b574e4abd8908ca14244f15179c2400b24dd08
c1ccoc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5].[#8;a:6]1:[c:7]:[c:8]:[c:9]:[cH;D2;+0:10]:1>>[C:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[CH2;D2;+0:1]-[c;H0;D3;+0:10]1:[#8;a:6]:[c:7]:[c:8]:[c:9]:1
null
[]
0
CELSIUS
30
MINUTE
A solution of triisopropyl-(2-methyl-furan-3-ylmethoxy)-silane (14) (5.0 g) in tetrahydrofuran (15 mL) was cooled to −78° C. with stirring. This solution was treated drop-wise with n-butyl lithium (2.5 M in hexanes, 8.94 mL). The resulting solution was warmed to 0° C. and allowed to stand for 30 minutes after which a s...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Ester
c1ccoc1
c1ccoc1
c1ccoc1
HBr
C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2].[Cl-].[Zn+2].[Cl-].O1CCCC1
0
0.5
CCOC(=O)CBr.Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C>C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2].[Cl-].[Zn+2].[Cl-].O1CCCC1>CCOC(=O)Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8d40e02461f94836b554b430ff35d267
CCOC(=O)Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1>>CCOC(=O)Cc1cc(CO)c(C)o1
C(C)OC(CC=1OC(=C(C1)CO[Si](C(C)C)(C(C)C)C(C)C)C)=O.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC>>C(C)OC(CC=1OC(=C(C1)CO)C)=O
CC(C)[Si](C(C)C)(C(C)C)[O:11][CH2:10][c:9]1[cH:8][c:7]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[o:14][c:12]1[CH3:13]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][c:7]1[cH:8][c:9]([CH2:10][OH:11])[c:12]([CH3:13])[o:14]1
CCOC(=O)Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
CCOC(=O)Cc1cc(CO)c(C)o1
null
null
O1CCCC1
Deprotection
Alcohol deprotection from silyl ethers
488547c1043a845c08188be7baa01e2ee1f8d7661927552d481c2d214b18b6c0
5c02ee98cb6b210a313993bea9e102110eb73637a50746f5457590f98613069b
c1ccoc1
C-C(-C)-[Si](-[O;H0;D2;+0:1]-[C:2]-[c:3]:[c:4]:[#8;a:5])(-C(-C)-C)-C(-C)-C>>[#8;a:5]:[c:4]:[c:3]-[C:2]-[OH;D1;+0:1]
67.3
[{"value": 67.3, "product": "C(C)OC(CC=1OC(=C(C1)CO)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A solution of (5-methyl-4-triisopropylsilanyloxymethyl-furan-2-yl)-acetic acid ethyl ester (29) (0.5 g) in tetrahydrofuran (3.0 mL) was cooled to 0° C. with stirring and treated with tetrabutylammonium fluoride (1.0 M solution in tetrahydrofuran, 2.82 mL) under argon. After 30 minutes, the resulting solution was concen...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
Primary alcohol
null
null
c1ccoc1
Other
O1CCCC1
null
0.5
CCOC(=O)Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1>O1CCCC1>CCOC(=O)Cc1cc(CO)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e39fb497513b41a8a2dc3023a8229f53
Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C>>Cc1oc(C=O)cc1CO[Si](C(C)C)(C(C)C)C(C)C
C(C)(C)[Si](OCC1=C(OC=C1)C)(C(C)C)C(C)C.O1CCCC1.C(C)(CC)[Li].[Cl-].[NH4+]>>CC1=C(C=C(O1)C=O)CO[Si](C(C)C)(C(C)C)C(C)C
[CH3:1][c:2]1[o:3][cH:4][cH:7][c:8]1[CH2:9][O:10][Si:11]([CH:12]([CH3:13])[CH3:14])([CH:15]([CH3:16])[CH3:17])[CH:18]([CH3:19])[CH3:20]>>[CH3:1][c:2]1[o:3][c:4]([CH:5]=[O:6])[cH:7][c:8]1[CH2:9][O:10][Si:11]([CH:12]([CH3:13])[CH3:14])([CH:15]([CH3:16])[CH3:17])[CH:18]([CH3:19])[CH3:20]
Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C
Cc1oc(C=O)cc1CO[Si](C(C)C)(C(C)C)C(C)C
null
null
null
Miscellaneous
OtherReaction
cae1cf39610b30a86caac44da7f4804528832aa7a233d782930e12364457f524
3cccf922e74135722ee21a46ad7578302a8603e1f71d6f2113cd42de4ba0cf73
c1ccoc1
[#8;a:1]1:[c:2]:[c:3]:[c:4]:[cH;D2;+0:5]:1>>[O;D1;H0:6]=[C:7]-[c;H0;D3;+0:5]1:[#8;a:1]:[c:2]:[c:3]:[c:4]:1
null
[]
null
null
null
null
A solution of triisopropyl-(2-methyl-furan-3-ylmethoxy)-silane (14) (10 g) in tetrahydrofuran (250 mL) was cooled to −78° C. with stirring, and then sec-butyllithium (1.3 M in cyclohexane; 37.25 mL) was added drop-wise over 10 mins. After stirring for 45 mins at −78° C., the cooling bath was removed for a period of 15 ...
10.6084/m9.figshare.5104873.v1
null
null
Aldehyde
c1ccoc1
c1ccoc1
c1ccoc1
Other
null
null
null
Cc1occc1CO[Si](C(C)C)(C(C)C)C(C)C>>Cc1oc(C=O)cc1CO[Si](C(C)C)(C(C)C)C(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-31f961aec1ce4f748b4be3af38423464
CCOC(=O)C=Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1>>CCOC(=O)CCc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
C(C)OC(C=CC=1OC(=C(C1)CO[Si](C(C)C)(C(C)C)C(C)C)C)=O>>C(C)OC(CCC=1OC(=C(C1)CO[Si](C(C)C)(C(C)C)C(C)C)C)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[CH:7][c:8]1[cH:9][c:10]([CH2:11][O:12][Si:13]([CH:14]([CH3:15])[CH3:16])([CH:17]([CH3:18])[CH3:19])[CH:20]([CH3:21])[CH3:22])[c:23]([CH3:24])[o:25]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][c:8]1[cH:9][c:10]([CH2:11][O:12][Si:13]([CH:14]([CH3:15])[CH3:16])([CH:17]([CH3:18]...
CCOC(=O)C=Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
CCOC(=O)CCc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
null
[Pd]
C(C)(=O)OCC
Reduction
Hydrogenation (double to single)
c04c38f95d7b746e5bdb99c368a7a33956c97b95b54c7ad89be2a85526386ec9
9a50abf8d2e4cd9195d7a0cadbe97483a261a81cf70b653cfddd5ecf76d383a6
c1ccoc1
[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH;D2;+0:5]=[CH;D2;+0:6]-[c:7](:[c:8]):[#8;a:9]:[c:10]>>[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH2;D2;+0:5]-[CH2;D2;+0:6]-[c:7](:[c:8]):[#8;a:9]:[c:10]
104.4
[{"value": 104.4, "product": "C(C)OC(CCC=1OC(=C(C1)CO[Si](C(C)C)(C(C)C)C(C)C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-(5-methyl-4-triisopropylsilanyloxymethyl-furan-2-yl)-acrylic acid ethyl ester (34) (1.0 g) in ethyl acetate (70 mL) was treated with 5% w/w palladium on carbon (350 mg) and hydrogenated at 1 atmosphere for exactly 1¼ hours at room temperature. The reaction mixture was filtered through filter-aid and the...
10.6084/m9.figshare.5104873.v1
null
Ester
Ester
null
null
c1ccoc1
null
[Pd].C(C)(=O)OCC
null
null
CCOC(=O)C=Cc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1>[Pd].C(C)(=O)OCC>CCOC(=O)CCc1cc(CO[Si](C(C)C)(C(C)C)C(C)C)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4701f04e25814d9fb2341f2dae6ce08f
CCOC(=O)CCc1cc(CO)c(C)o1.Oc1ccc(-c2ccccc2)cc1>>Cc1oc(CCC(=O)O)cc1COc1ccc(-c2ccccc2)cc1
C(C)OC(CCC=1OC(=C(C1)CO)C)=O.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=C(C=C1)O)C1=CC=CC=C1.CC(C)OC(=O)/N=N/C(=O)OC(C)C>>C1(=CC=C(C=C1)OCC=1C=C(OC1C)CCC(=O)O)C1=CC=CC=C1
CC[O:9][C:7]([CH2:6][CH2:5][c:4]1[o:3][c:2]([CH3:1])[c:11]([CH2:12][OH:13])[cH:10]1)=[O:8].O[c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[cH:24][cH:25]1>>[CH3:1][c:2]1[o:3][c:4]([CH2:5][CH2:6][C:7](=[O:8])[OH:9])[cH:10][c:11]1[CH2:12][O:13][c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][c...
CCOC(=O)CCc1cc(CO)c(C)o1.Oc1ccc(-c2ccccc2)cc1
Cc1oc(CCC(=O)O)cc1COc1ccc(-c2ccccc2)cc1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
OtherReaction
387928e2999368eba02196099cabcd9fef681a6c27addbdc8240d657651def8d
9653d63179b641796999681486e0249947865421087fe94dd6954f3668089e9b
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4].[#8;a:5]:[c:6]:[c:7]-[C:8]-[OH;D1;+0:9].O-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[#8;a:5]:[c:6]:[c:7]-[C:8]-[O;H0;D2;+0:9]-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14].[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
3.9
[{"value": 3.9, "product": "C1(=CC=C(C=C1)OCC=1C=C(OC1C)CCC(=O)O)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
10
MINUTE
To a stirred, cooled 0° C. solution, in tetrahydrofuran (2.5 mL), a solution of 3-(4-hydroxymethyl-5-methyl-furan-2-yl)-propionic acid ethyl ester (36) (400 mg) in tetrahydrofuran (2.5 mL) was cooled to 0° C. and treated successively with triphenylphosphine (542 mg), biphenyl-4-ol (353 mg) and diisopropylazodicarboxyla...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary alcohol.Aromatic alcohol
Carboxylic acid.Ether
c1ccccc1
c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HO-
O1CCCC1
0
0.166667
CCOC(=O)CCc1cc(CO)c(C)o1.Oc1ccc(-c2ccccc2)cc1>O1CCCC1>Cc1oc(CCC(=O)O)cc1COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6c2940245aaf4bbfa62e61b4eb37787a
Cc1occc1CO.Oc1ccc(-c2ccccc2)cc1>>Cc1occc1COc1ccc(-c2ccccc2)cc1
CC(C)OC(=O)/N=N/C(=O)OC(C)C.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=C(C=C1)O)C1=CC=CC=C1.CC=1OC=CC1CO>>C1(=CC=C(C=C1)OCC1=C(OC=C1)C)C1=CC=CC=C1
[CH3:1][c:2]1[o:3][cH:4][cH:5][c:6]1[CH2:7][OH:8].O[c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[cH:19][cH:20]1>>[CH3:1][c:2]1[o:3][cH:4][cH:5][c:6]1[CH2:7][O:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[cH:19][cH:20]1
Cc1occc1CO.Oc1ccc(-c2ccccc2)cc1
Cc1occc1COc1ccc(-c2ccccc2)cc1
null
null
C(C)OCC
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
8915084acbaaf997bf0f89ff5187cb2f89c25dc683fffc57b3391298c8430dd9
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
O-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#8;a:6]:[c:7]:[c:8]-[C:9]-[OH;D1;+0:10]>>[#8;a:6]:[c:7]:[c:8]-[C:9]-[O;H0;D2;+0:10]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
59.4
[{"value": 59.4, "product": "C1(=CC=C(C=C1)OCC1=C(OC=C1)C)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of (2-methyl-furan-3-yl)-methanol (1) (5.0 g) in diethyl ether (75 mL) was cooled to 0° C. with stirring and treated with triphenylphosphine (12.85 g) and biphenyl-4-ol (7.59 g). The resulting solution was then treated drop-wise with diisopropylazodicarboxylate (9.75 mL). After stirring for 10 minutes at 0° ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HO-
C(C)OCC
null
null
Cc1occc1CO.Oc1ccc(-c2ccccc2)cc1>C(C)OCC>Cc1occc1COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-19f2272b9fd148bc8448f74140c8d61c
Cc1oc(S(N)(=O)=O)cc1COc1ccc(-c2ccccc2)cc1.O=C(O)c1ccccc1>>Cc1oc(S(=O)(=O)NC(=O)c2ccccc2)cc1COc1ccc(-c2ccccc2)cc1
Cl.CN(CCCN=C=NCC)C.C1(=CC=C(C=C1)OCC=1C=C(OC1C)S(=O)(=O)N)C1=CC=CC=C1.C(C1=CC=CC=C1)(=O)O>>C(C1=CC=CC=C1)(=O)NS(=O)(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=CC=C1)C
[CH3:1][c:2]1[o:3][c:4]([S:5](=[O:6])(=[O:7])[NH2:8])[cH:17][c:18]1[CH2:19][O:20][c:21]1[cH:22][cH:23][c:24](-[c:25]2[cH:26][cH:27][cH:28][cH:29][cH:30]2)[cH:31][cH:32]1.O[C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][c:2]1[o:3][c:4]([S:5](=[O:6])(=[O:7])[NH:8][C:9](=[O:10])[c:11]2[cH:12][cH:13][cH:...
Cc1oc(S(N)(=O)=O)cc1COc1ccc(-c2ccccc2)cc1.O=C(O)c1ccccc1
Cc1oc(S(=O)(=O)NC(=O)c2ccccc2)cc1COc1ccc(-c2ccccc2)cc1
null
CN(C)C1=CC=NC=C1
O1CCCC1.CN(C=O)C
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1cc(COc2ccc(-c3ccccc3)cc2)co1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#8;a:6]:[c:7]-[#16:8](-[NH2;D1;+0:9])(=[O;D1;H0:10])=[O;D1;H0:11]>>[#8;a:6]:[c:7]-[#16:8](=[O;D1;H0:10])(=[O;D1;H0:11])-[NH;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
To a stirred solution of benzoic acid (61 mg) in a mixture of tetrahydrofuran (10 mL) and N,N-dimethylformamide (5 mL) was added 4-(N,N-dimethylamino)pyridine (3.0 mg), 1-(3-dimethylaminopropyl)-3-ethylcarbodiimide hydrochloride (118 mg) and 4-(biphenyl-4-yloxymethyl)-5-methyl-furan-2-sulfonic acid amide (45) (206 mg)....
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccoc1.c1ccccc1.c1ccccc1.c1ccccc1
HO-
CN(C)C1=CC=NC=C1.O1CCCC1.CN(C=O)C
null
null
Cc1oc(S(N)(=O)=O)cc1COc1ccc(-c2ccccc2)cc1.O=C(O)c1ccccc1>CN(C)C1=CC=NC=C1.O1CCCC1.CN(C=O)C>Cc1oc(S(=O)(=O)NC(=O)c2ccccc2)cc1COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-02dc82f64f374c8c91b15f796bec0e0c
CCCC(=O)Cl.Cc1oc(S(N)(=O)=O)cc1COc1ccc(-c2ccccc2)cc1>>CCCC(=O)NS(=O)(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
C1(=CC=C(C=C1)OCC=1C=C(OC1C)S(=O)(=O)N)C1=CC=CC=C1.C(C)N(CC)CC.C(CCC)(=O)Cl>>C(CCC)(=O)NS(=O)(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=CC=C1)C
Cl[C:4]([CH2:3][CH2:2][CH3:1])=[O:5].[NH2:6][S:7](=[O:8])(=[O:9])[c:10]1[cH:11][c:12]([CH2:13][O:14][c:15]2[cH:16][cH:17][c:18](-[c:19]3[cH:20][cH:21][cH:22][cH:23][cH:24]3)[cH:25][cH:26]2)[c:27]([CH3:28])[o:29]1>>[CH3:1][CH2:2][CH2:3][C:4](=[O:5])[NH:6][S:7](=[O:8])(=[O:9])[c:10]1[cH:11][c:12]([CH2:13][O:14][c:15]2[cH...
CCCC(=O)Cl.Cc1oc(S(N)(=O)=O)cc1COc1ccc(-c2ccccc2)cc1
CCCC(=O)NS(=O)(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
null
CN(C1=CC=NC=C1)C
ClCCl
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
403eb34e708e50f7077a9da490b1654c837258ce901614ddd1204eb6f2a10a27
37dfa12f19cd8cec29206fb8a18b7504935d92bc326a2084e9ef8a13076d3b87
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[#8;a:5]:[c:6]-[#16:7](-[NH2;D1;+0:8])(=[O;D1;H0:9])=[O;D1;H0:10]>>[#8;a:5]:[c:6]-[#16:7](=[O;D1;H0:9])(=[O;D1;H0:10])-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]
79.5
[{"value": 79.5, "product": "C(CCC)(=O)NS(=O)(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=CC=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
To a stirred solution of 4-(biphenyl-4-yloxymethyl)-5-methyl-furan-2-sulphonic acid amide (45) (50 mg, 0.146 mmoles) in dichloromethane (5.0 ml) was added triethylamine (26 μl, 0.189 mmoles), dimethyl-pyridin-4-yl-amine (1 mg) and butyryl chloride (19 μl, 0.184 mmoles). After stirring for 16 hours at room temperature t...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Sulfonamide
Sulfonamide.Secondary amide
null
null
c1ccoc1.c1ccccc1.c1ccccc1
HCl
CN(C1=CC=NC=C1)C.ClCCl
null
16
CCCC(=O)Cl.Cc1oc(S(N)(=O)=O)cc1COc1ccc(-c2ccccc2)cc1>CN(C1=CC=NC=C1)C.ClCCl>CCCC(=O)NS(=O)(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7deec222c1444263b279988f5b822d56
CC1(C)OB(c2ccc(O)cc2)OC1(C)C.COC(=O)c1cc(CO)c(C)o1>>COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1
COC(=O)C=1OC(=C(C1)CO)C.CC1(OB(OC1(C)C)C1=CC=C(C=C1)O)C.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)B1OC(C(O1)(C)C)(C)C)C
[OH:9][c:10]1[cH:11][cH:12][c:13]([B:14]2[O:15][C:16]([CH3:17])([CH3:18])[C:19]([CH3:20])([CH3:21])[O:22]2)[cH:23][cH:24]1.O[CH2:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:27][c:25]1[CH3:26]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13]([B:14]3[O:15][C:16]([CH3:17])([CH3:18])...
CC1(C)OB(c2ccc(O)cc2)OC1(C)C.COC(=O)c1cc(CO)c(C)o1
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1
null
null
null
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
86bfb73617450d22f9456ed5ce4d96a73f1f8fc0c016bebae57fda68e2da86a2
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1cc(COc2ccc(B3OCCO3)cc2)co1
O-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4](-[C:5](-[#8:6])=[O;D1;H0:7]):[#8;a:8]:[c:9]:1-[C;D1;H3:10].[OH;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#8;a:8]:[c:9](-[C;D1;H3:10]):[c:2](-[CH2;D2;+0:1]-[O;H0;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:3]:1
null
[]
0
CELSIUS
72
HOUR
A mixture of 4-hydroxymethyl-5-methyl-furan-2-carboxylic acid methyl ester (16) (0.5 g), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-phenol (1.9 g) and triphenylphosphine (2.3 g) in dry tetrahydrofuan (20 mL) under a nitrogen atmosphere was cooled to 0° C. Di-isopropylazodicarboxylate (1.8 mL) was added drop-wise ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
null
null
c1ccoc1.c1ccccc1.[B]1OCCO1
HO-
null
0
72
CC1(C)OB(c2ccc(O)cc2)OC1(C)C.COC(=O)c1cc(CO)c(C)o1>>COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8fd90a8774c149268ada582b7a92c9ed
COC(=O)c1cc(COc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1>>COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)nc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=NC=C(C=C1)OC)C>>COC=1C=CC(=NC1)C1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1
C[O:18][C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:25][n:24]3)[cH:23][cH:22]2)[c:20]([CH3:21])[o:19]1)=[O:17]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([O:11][CH2:12][c:13]3[cH:14][c:15]([C:16](=[O:17])[OH:18])[o:19][c:20]3[CH3:21])[c...
COC(=O)c1cc(COc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)nc1
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(OCc3ccoc3)cc2)nc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
53.6
[{"value": 53.6, "product": "COC=1C=CC(=NC1)C1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of 4-[4-(5-methoxy-pyridin-2-yl)-phenoxymethyl]-5-methyl-furan-2-carboxylic acid methyl ester (52) (118 mg, 0.33 mmoles) in dry tetrahydrofuran (10 ml) was treated with potassium trimethylsilanoate (260 mg, 2.0 mmoles) and the mixture stirred under an argon atmosphere for 2 hours. After evaporation of the so...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccncc1.c1ccccc1.c1ccoc1
Other
O1CCCC1
null
2
COC(=O)c1cc(COc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1>O1CCCC1>COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fe66121b7403479f809e32a3e651e0d7
COC(=O)c1cc(COc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1>>COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)nc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=NC=C(C=C1)OC)C.[OH-].[Li+]>>COC=1C=CC(=NC1)C1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1
C[O:18][C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:25][n:24]3)[cH:23][cH:22]2)[c:20]([CH3:21])[o:19]1)=[O:17]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([O:11][CH2:12][c:13]3[cH:14][c:15]([C:16](=[O:17])[OH:18])[o:19][c:20]3[CH3:21])[c...
COC(=O)c1cc(COc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)nc1
null
null
O1CCCC1.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(OCc3ccoc3)cc2)nc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
16
HOUR
A mixture of 4-[4-(5-methoxy-pyridin-2-yl)-phenoxymethyl]-5-methyl-furan-2-carboxylic acid methyl ester (52) (70 mg) and 1M aqueous lithium hydroxide (1 mL) in tetrahydrofuran/methanol (2:1 by volume) (12 mL) was stirred at room temperature for 16 hours. The reaction mixture was acidified to between pH6 and pH7, and pa...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccncc1.c1ccccc1.c1ccoc1
Other
O1CCCC1.CO
null
16
COC(=O)c1cc(COc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1>O1CCCC1.CO>COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-56a99a1d74b947438319981ba013fc7b
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(I)nc1>>COC(=O)c1cc(COc2ccc(I)nc2)c(C)o1
COC(=O)C=1OC(=C(C1)CO)C.IC1=NC=C(C=C1)O>>COC(=O)C=1OC(=C(C1)COC=1C=NC(=CC1)I)C
O[CH2:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:19][c:17]1[CH3:18].[OH:9][c:10]1[cH:11][cH:12][c:13]([I:14])[n:15][cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13]([I:14])[n:15][cH:16]2)[c:17]([CH3:18])[o:19]1
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(I)nc1
COC(=O)c1cc(COc2ccc(I)nc2)c(C)o1
null
null
null
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
86bfb73617450d22f9456ed5ce4d96a73f1f8fc0c016bebae57fda68e2da86a2
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1cncc(OCc2ccoc2)c1
O-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4](-[C:5](-[#8:6])=[O;D1;H0:7]):[#8;a:8]:[c:9]:1-[C;D1;H3:10].[OH;D1;+0:11]-[c:12](:[c:13]):[c:14]:[#7;a:15]:[c:16]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#8;a:8]:[c:9](-[C;D1;H3:10]):[c:2](-[CH2;D2;+0:1]-[O;H0;D2;+0:11]-[c:12](:[c:13]):[c:14]:[#7;a:15]:[c:16]):[c:3]:1
null
[]
null
null
null
null
Compound (54) was prepared from compound (16) and 2-iodo-5-hydroxy-pyridine in a manner analagous to that described in Example 5(a). LC/MS System A: Rt=3.52 mins, m/z=374 ((M+H) for C13H12INO4) Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
null
null
c1ccoc1.c1ccncc1
HO-
null
null
null
COC(=O)c1cc(CO)c(C)o1.Oc1ccc(I)nc1>>COC(=O)c1cc(COc2ccc(I)nc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6dee0ec125d049e8b6c4550813e014e9
N.O=S(=O)(Cl)CCCN1CCOCC1>>NS(=O)(=O)CCCN1CCOCC1
N.C(=O)=O.CC(=O)C.N1(CCOCC1)CCCS(=O)(=O)Cl>>N1(CCOCC1)CCCS(=O)(=O)N
[NH3:1].Cl[S:2](=[O:3])(=[O:4])[CH2:5][CH2:6][CH2:7][N:8]1[CH2:9][CH2:10][O:11][CH2:12][CH2:13]1>>[NH2:1][S:2](=[O:3])(=[O:4])[CH2:5][CH2:6][CH2:7][N:8]1[CH2:9][CH2:10][O:11][CH2:12][CH2:13]1
N.O=S(=O)(Cl)CCCN1CCOCC1
NS(=O)(=O)CCCN1CCOCC1
null
null
ClCCl
Acylation
OtherReaction
672a14b4f1ef0b966898e1b4c118f241f21df1d6e087372155b9d0c840dac61f
29e1633db8f1f00444181a0bcac91d574ed806fddf9165be4c8478fc32a80994
C1COCCN1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[C:4]-[C:5].[NH3;D0;+0:6]>>[C:5]-[C:4]-[S;H0;D4;+0:1](-[NH2;D1;+0:6])(=[O;D1;H0:2])=[O;D1;H0:3]
null
[]
null
null
24
HOUR
Dichloromethane (40 ml) was saturated with ammonia gas with cooling (dry ice/acetone), and then 3-morpholin-4-yl-propane-1-sulphonyl chloride (279 mg, 1.23 mmoles) was added. The mixture was stirred at room temperature for 24 hours. The mixture was filtered, the filtrate evaporated and the residue was dried at 40° C. i...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
Sulfonamide
null
null
C1COCC[NH]1
HCl
ClCCl
null
24
N.O=S(=O)(Cl)CCCN1CCOCC1>ClCCl>NS(=O)(=O)CCCN1CCOCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7ad047b539f64ba7879af67e63b2cabb
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1.NS(=O)(=O)CCCN1CCOCC1>>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)CCCN4CCOCC4)oc3C)cc2)cc1
COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O.N1(CCOCC1)CCCS(=O)(=O)N>>COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)CCCN1CCOCC1
O[C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:37][cH:36]3)[cH:35][cH:34]2)[c:32]([CH3:33])[o:31]1)=[O:17].[NH2:18][S:19](=[O:20])(=[O:21])[CH2:22][CH2:23][CH2:24][N:25]1[CH2:26][CH2:27][O:28][CH2:29][CH2:30]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH...
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1.NS(=O)(=O)CCCN1CCOCC1
COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)CCCN4CCOCC4)oc3C)cc2)cc1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)CCCN1CCOCC1)c1cc(COc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[C:7]-[#16:8](-[NH2;D1;+0:9])(=[O;D1;H0:10])=[O;D1;H0:11]>>[C:7]-[#16:8](=[O;D1;H0:10])(=[O;D1;H0:11])-[NH;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6]
null
[]
null
null
null
null
Compound (59) was prepared from compounds (4) and (58) by adapting the procedure of Example 2A. LC/MS System D; Rt=4.97 mins, m/z (ES+)=529 (M+H for C27H32N2O7S). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccoc1.C1COCC[NH]1
HO-
null
null
null
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1.NS(=O)(=O)CCCN1CCOCC1>>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)CCCN4CCOCC4)oc3C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-560f3b6afd6544568b40a77d5eba2f20
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2)cc1>>Cc1ccccc1S(=O)(=O)NC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
C1(=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O)C1=CC=CC=C1.CC1=C(C=CC=C1)S(=O)(=O)N.Cl.CN(CCCN=C=NCC)C>>C1(=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=C(C=CC=C1)C)C1=CC=CC=C1
[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:9])(=[O:10])[NH2:11].O[C:12](=[O:13])[c:14]1[cH:15][c:16]([CH2:17][O:18][c:19]2[cH:20][cH:21][c:22](-[c:23]3[cH:24][cH:25][cH:26][cH:27][cH:28]3)[cH:29][cH:30]2)[c:31]([CH3:32])[o:33]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:9])(=[O:10])[NH:11][C:12](=[...
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2)cc1
Cc1ccccc1S(=O)(=O)NC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
null
CN(C)C1=CC=NC=C1
O1CCCC1.C(C)#N
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(COc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:9]=[#16:8](=[O;D1;H0:10])(-[c:11])-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6]
26.7
[{"value": 26.7, "product": "C1(=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=C(C=CC=C1)C)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
A stirred solution of 4-(biphenyl-4-yloxymethyl)-5-methyl-furan-2-carboxylic acid (18) (50 mg, 0.162 mmoles), 2-methyl-benzenesulphonamide (42 mg, 0.243 mmoles) and 4-(N,N-dimethylamino)-pyridine (2.5 mg) in a mixture of tetrahydrofuran (8 ml) and acetonitrile (2 ml) was treated with 1-(3-dimethylaminopropyl)-3-ethylca...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.c1ccoc1.c1ccccc1.c1ccccc1
HO-
CN(C)C1=CC=NC=C1.O1CCCC1.C(C)#N
null
16
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2)cc1>CN(C)C1=CC=NC=C1.O1CCCC1.C(C)#N>Cc1ccccc1S(=O)(=O)NC(=O)c1cc(COc2ccc(-c3ccccc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8a2e8f2af4d64aa7aa985cdd5f35656f
CCOC(=O)Cc1ccoc1C>>Cc1occc1CCO
C(C)OC(CC1=C(OC=C1)C)=O.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>CC=1OC=CC1CCO
CCO[C:8]([CH2:7][c:6]1[c:2]([CH3:1])[o:3][cH:4][cH:5]1)=[O:9]>>[CH3:1][c:2]1[o:3][cH:4][cH:5][c:6]1[CH2:7][CH2:8][OH:9]
CCOC(=O)Cc1ccoc1C
Cc1occc1CCO
null
null
O1CCCC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccoc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3]-[c:4]:[c:5]:[#8;a:6]>>[#8;a:6]:[c:5]:[c:4]-[C:3]-[CH2;D2;+0:1]-[OH;D1;+0:2]
null
[]
0
CELSIUS
3
HOUR
A solution of (2-methyl-furan-3-yl)-acetic acid ethyl ester (11.8 g, 70.2 mmoles) in tetrahydrofuran (50 ml) was added to a stirred suspension of lithium aluminium hydride (2.66 g, 70.2 mmoles) under a nitrogen atmosphere and with cooling to 0° C. When the addition was complete the mixture was stirred at room temperatu...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccoc1
HO-
O1CCCC1
0
3
CCOC(=O)Cc1ccoc1C>O1CCCC1>Cc1occc1CCO
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d8ebeacd351047e682146583a90b1d2f
CCOC(=O)CC(=O)C(C)C>>CCOC(=O)c1ccoc1C(C)C
[OH-].[Na+].C(C)OC(CC(C(C)C)=O)=O.ClC(CCl)OCC>>C(C)OC(=O)C1=C(OC=C1)C(C)C
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][C:10](=[O:9])[CH:11]([CH3:12])[CH3:13]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][o:9][c:10]1[CH:11]([CH3:12])[CH3:13]
CCOC(=O)CC(=O)C(C)C
CCOC(=O)c1ccoc1C(C)C
null
null
O.C(C)OCC
Aromatic Heterocycle Formation
OtherReaction
3d59eca64d9e08f3f2cf41a13f93be1239ae749d285b221a48e58749a8dba3ab
0ee4fb987ebeea21a9d50ac911d0f83c8450e9a26ef48746d74554271dcaf444
c1ccoc1
[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH2;D2;+0:5]-[C;H0;D3;+0:6](=[O;H0;D1;+0:7])-[C:8](-[C;D1;H3:9])-[C;D1;H3:10]>>[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[c;H0;D3;+0:5]1:[c:11]:[c:12]:[o;H0;D2;+0:7]:[c;H0;D3;+0:6]:1-[C:8](-[C;D1;H3:9])-[C;D1;H3:10]
69.5
[{"value": 69.5, "product": "C(C)OC(=O)C1=C(OC=C1)C(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
An ice-chilled solution of sodium hydroxide (1.9 g) in water (25 ml) was added, during 40 minutes, to a stirred solution of 4-methyl-3-oxo-pentanoic acid ethyl ester (3 g, 18.96 mmoles) and 1,2-dichloro-1-ethoxy-ethane (3.3 g, 35.19 mmole) in diethyl ether (15 ml) with ice bath cooling. When the addition was complete t...
10.6084/m9.figshare.5104873.v1
null
Ketone
Ester
null
c1ccoc1
c1ccoc1
Other
O.C(C)OCC
null
1
CCOC(=O)CC(=O)C(C)C>O.C(C)OCC>CCOC(=O)c1ccoc1C(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-96c7f09801eb4099a5dddb1b85969f7e
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.COc1ccc(B(O)O)cc1OC>>COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1OC
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.COC=1C=C(C=CC1OC)B(O)O.CN(C=O)C.C(C)(=O)[O-].[K+]>>COC=1C=C(C=CC1OC)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
C[O:18][C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](I)[cH:23][cH:22]2)[c:20]([CH3:21])[o:19]1)=[O:17].OB(O)[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[c:25]([O:26][CH3:27])[cH:24]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([O:11][CH2:12][c:13]3[cH:14][c:15]([C:16](=[O:17])[OH:18])[o...
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.COc1ccc(B(O)O)cc1OC
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1OC
null
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2]
ClCCl.O
C-C Coupling
OtherReaction
04157bef51d5543c035526858b11d2af2b78e75d38cd85edf56b617e6aebc946
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1].[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]):[c:9]:[c:10]
60.8
[{"value": 60.8, "product": "COC=1C=C(C=CC1OC)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
A stirred mixture of 4-(4-iodo-phenoxymethyl)-5-methyl-furan-2-carboxylic acid methyl ester (20) (0.025 g, 0.067 mmoles), (3,4-dimethoxyphenyl)-boronic acid (0.017 g, 0.093 mmoles), N,N-dimethylformamide (3 mL), potassium acetate (0.026 g) and [1,1′-bis(diphenylphosphino) ferrocene]dichloropalladium(II), complex with d...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccoc1
HI.B
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].ClCCl.O
null
24
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.COc1ccc(B(O)O)cc1OC>C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].ClCCl.O>COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-52c36e7502654e76aab4d4a760d58f29
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccc2c(c1)OCO2>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc3c(c2)OCO3)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.C1OC=2C=C(C=CC2O1)B(O)O>>O1COC2=C1C=CC(=C2)C2=CC=C(OCC=1C=C(OC1C)C(=O)O)C=C2
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][O:11][c:12]2[cH:13][cH:14][c:15](I)[cH:25][cH:26]2)[cH:8]1)=[O:6].OB(O)[c:16]1[cH:17][cH:18][c:19]2[c:20]([cH:21]1)[O:22][CH2:23][O:24]2>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][c:19]3[c:...
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccc2c(c1)OCO2
Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc3c(c2)OCO3)cc1
null
null
null
C-C Coupling
OtherReaction
6edcd9e2b402dbd56bbc75a03f0214d18a4609f841b039e42a77bd180cb3ab1f
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1cc(COc2ccc(-c3ccc4c(c3)OCO4)cc2)co1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]-[#8:16]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1].[#8:16]-[c:15]:[c:14]:[c;H0;D3;+0:11](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:12]:[c:13]
null
[]
null
null
null
null
Compound (28) was prepared from compound (20) and (3,4-methylenedioxyphenyl)-boronic acid by adapting the procedure of Example 24A. LC/MS System B; Rt=1.76 mins, m/z (ES−)=351 (M−H for C20H16O6). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccc2c(c1)OCO2
c1ccccc1.c1ccc2c(c1)OCO2
c1ccoc1.c1ccccc1.c1ccc2c(c1)OCO2
HI.B
null
null
null
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccc2c(c1)OCO2>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc3c(c2)OCO3)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-529eedf26bf44583bbaeb734051aec2e
CCOc1ccc(B(O)O)cc1.COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1>>CCOc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.C(C)OC1=CC=C(C=C1)B(O)O>>C(C)OC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
OB(O)[c:7]1[cH:6][cH:5][c:4]([O:3][CH2:2][CH3:1])[cH:26][cH:25]1.C[O:19][C:17]([c:16]1[cH:15][c:14]([CH2:13][O:12][c:11]2[cH:10][cH:9][c:8](I)[cH:24][cH:23]2)[c:21]([CH3:22])[o:20]1)=[O:18]>>[CH3:1][CH2:2][O:3][c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([O:12][CH2:13][c:14]3[cH:15][c:16]([C:17](=[O:18])[OH:19])[...
CCOc1ccc(B(O)O)cc1.COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1
CCOc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
null
null
null
C-C Coupling
OtherReaction
04157bef51d5543c035526858b11d2af2b78e75d38cd85edf56b617e6aebc946
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1].[c:10]:[c:9]:[c;H0;D3;+0:6](-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]):[c:7]:[c:8]
null
[]
null
null
null
null
Compound (98) was prepared from compound (20) and (4-ethoxyphenyl)-boronic acid by an adapting the procedure of Example 24A. LC/MS System B; Rt=1.86 mins, m/z (ES−) 351 (M−H for C21H20O5). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccoc1
HI.B
null
null
null
CCOc1ccc(B(O)O)cc1.COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1>>CCOc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f0d31306041240e0a3ebdf610ed46d30
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccccc1Cl>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2Cl)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.ClC1=C(C=CC=C1)B(O)O>>ClC1=C(C=CC=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][O:11][c:12]2[cH:13][cH:14][c:15](I)[cH:23][cH:24]2)[cH:8]1)=[O:6].OB(O)[c:16]1[cH:17][cH:18][cH:19][cH:20][c:21]1[Cl:22]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[Cl:2...
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccccc1Cl
Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2Cl)cc1
null
null
null
C-C Coupling
OtherReaction
04157bef51d5543c035526858b11d2af2b78e75d38cd85edf56b617e6aebc946
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14](-[Cl;D1;H0:15]):[c:16]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1].[Cl;D1;H0:15]-[c:14](:[c:16]):[c;H0;D3;+0:11](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:12]:[c:13]
null
[]
null
null
null
null
Compound (99) was prepared from compound (20) and (2-chlorophenyl)-boronic acid by adapting the procedure of Example 5(b). LC/MS System B; Rt=1.86 mins, m/z (ES−)=341 and 343 (M−H for C19H15ClO4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccccc1Cl>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2Cl)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-28dbdc5ae2cc4f0c8a4912c54813641b
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1c(F)cccc1F>>Cc1oc(C(=O)O)cc1COc1ccc(-c2c(F)cccc2F)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.FC1=C(C(=CC=C1)F)B(O)O>>FC1=C(C(=CC=C1)F)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][O:11][c:12]2[cH:13][cH:14][c:15](I)[cH:24][cH:25]2)[cH:8]1)=[O:6].OB(O)[c:16]1[c:17]([F:18])[cH:19][cH:20][cH:21][c:22]1[F:23]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[c:17]([F:18])[cH:19][cH:20][cH:21...
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1c(F)cccc1F
Cc1oc(C(=O)O)cc1COc1ccc(-c2c(F)cccc2F)cc1
null
null
null
C-C Coupling
OtherReaction
04157bef51d5543c035526858b11d2af2b78e75d38cd85edf56b617e6aebc946
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12](-[F;D1;H0:13]):[c:14]):[c:15](-[F;D1;H0:16]):[c:17]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1].[F;D1;H0:13]-[c:12](:[c:14]):[c;H0;D3;+0:11](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c...
null
[]
null
null
null
null
Compound (100) was prepared from compound (20) and (2,6-difluorophenyl)-boronic acid by adapting the procedure of Example 5(b). LC/MS System B; Rt=1.83 mins, m/z (ES−)=343 (M−H for C19H14F2O4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1c(F)cccc1F>>Cc1oc(C(=O)O)cc1COc1ccc(-c2c(F)cccc2F)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cc13d83cc9ed4a93a4e80f4f170d6d88
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccccc1C(F)(F)F>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2C(F)(F)F)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.FC(C1=C(C=CC=C1)B(O)O)(F)F>>CC1=C(C=C(O1)C(=O)O)COC1=CC=C(C=C1)C1=C(C=CC=C1)C(F)(F)F
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][O:11][c:12]2[cH:13][cH:14][c:15](I)[cH:26][cH:27]2)[cH:8]1)=[O:6].OB(O)[c:16]1[cH:17][cH:18][cH:19][cH:20][c:21]1[C:22]([F:23])([F:24])[F:25]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][cH:1...
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccccc1C(F)(F)F
Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2C(F)(F)F)cc1
null
null
null
C-C Coupling
OtherReaction
04157bef51d5543c035526858b11d2af2b78e75d38cd85edf56b617e6aebc946
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14](-[C:15](-[F;D1;H0:16])(-[F;D1;H0:17])-[F;D1;H0:18]):[c:19]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1].[F;D1;H0:16]-[C:15](-[F;D1;H0:17])(-[F;D1;H0:18])-[c:14](:[c:19]):[c;...
null
[]
null
null
null
null
Compound (102) was prepared from compound (20) and (2-trifluoromethyl-phenyl)-boronic acid by adapting the procedure of Example 5(b). LC/MS System B; Rt=1.93 mins, m/z (ES−)=375 (M−H for C20H15F3O4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccccc1C(F)(F)F>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2C(F)(F)F)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a327e610d9b4437480c441c754af1547
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccc(Cl)cc1>>O=C(O)c1cc(COc2ccc(-c3ccccc3)cc2)co1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.ClC1=CC=C(C=C1)B(O)O>>C1(=CC=C(C=C1)OCC=1C=C(OC1)C(=O)O)C1=CC=CC=C1
C[O:3][C:2](=[O:1])[c:4]1[cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][cH:11][c:12](I)[cH:19][cH:20]2)[c:21](C)[o:22]1.OB(O)[c:13]1[cH:14][cH:15][c:16](Cl)[cH:17][cH:18]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][cH:11][c:12](-[c:13]3[cH:14][cH:15][cH:16][cH:17][cH:18]3)[cH:19][cH:20]2)[cH:21][o:22]1
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccc(Cl)cc1
O=C(O)c1cc(COc2ccc(-c3ccccc3)cc2)co1
null
null
null
C-C Coupling
OtherReaction
208d7cb8553b4a8de62b809cfc13cdf69831a49eaa82f1183e0589cc9f7bb8ce
57e36285fe5e46d1b7fb6bd126f751f9e7245cbcf73856b9176889fbc17d553c
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#8;a:5]:[c;H0;D3;+0:6](-C):[c:7](-[C:8]):[c:9]:1.I-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14].Cl-[c;H0;D3;+0:15]1:[c:16]:[c:17]:[c;H0;D3;+0:18](-B(-O)-O):[c:19]:[c:20]:1>>[C:8]-[c:7]1:[c:9]:[c:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]):[#8;a:5]:[cH;D2;+0:6]:1.[c:12]:[c:11]:[c;...
null
[]
null
null
null
null
Compound (77) was prepared from compound (20) and (4-chloro-phenyl)-boronic acid by adapting the procedure of Example 5(b). LC/MS System B; Rt=1.93 mins, m/z (ES−)=341 and 343 (M−H for C19H15ClO4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccoc1.c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HCl.I-.B
null
null
null
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1ccc(Cl)cc1>>O=C(O)c1cc(COc2ccc(-c3ccccc3)cc2)co1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8577508583384178b30a1ef53df52204
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1cccc(F)c1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2cccc(F)c2)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.FC=1C=C(C=CC1)B(O)O>>FC=1C=C(C=CC1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][O:11][c:12]2[cH:13][cH:14][c:15](I)[cH:23][cH:24]2)[cH:8]1)=[O:6].OB(O)[c:16]1[cH:17][cH:18][cH:19][c:20]([F:21])[cH:22]1>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][cH:19][c:20]([F:21])[cH:...
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1cccc(F)c1
Cc1oc(C(=O)O)cc1COc1ccc(-c2cccc(F)c2)cc1
null
null
null
C-C Coupling
OtherReaction
04157bef51d5543c035526858b11d2af2b78e75d38cd85edf56b617e6aebc946
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1].[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]):[c:9]:[c:10]
null
[]
null
null
null
null
Compound (104) was prepared from compound (20) and (3-fluoro-phenyl)-boronic acid by adapting the procedure of Example 5(b). LC/MS System B; Rt=1.83 mins, m/z (ES−)=325 (M−H for C19H15FO4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.OB(O)c1cccc(F)c1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2cccc(F)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-01bea476d7a24691adbcc38b526e3118
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.CSc1ccccc1B(O)O>>CSc1ccccc1-c1ccc(OCc2cc(C(=O)O)oc2C)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)I)C.CSC1=C(C=CC=C1)B(O)O>>CC1=C(C=C(O1)C(=O)O)COC1=CC=C(C=C1)C1=C(C=CC=C1)SC
C[O:20][C:18]([c:17]1[cH:16][c:15]([CH2:14][O:13][c:12]2[cH:11][cH:10][c:9](I)[cH:25][cH:24]2)[c:22]([CH3:23])[o:21]1)=[O:19].OB(O)[c:8]1[c:3]([S:2][CH3:1])[cH:4][cH:5][cH:6][cH:7]1>>[CH3:1][S:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[c:9]1[cH:10][cH:11][c:12]([O:13][CH2:14][c:15]2[cH:16][c:17]([C:18](=[O:19])[OH:20])[o:...
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.CSc1ccccc1B(O)O
CSc1ccccc1-c1ccc(OCc2cc(C(=O)O)oc2C)cc1
null
null
null
C-C Coupling
OtherReaction
04157bef51d5543c035526858b11d2af2b78e75d38cd85edf56b617e6aebc946
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5].I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14](-[#16:15]):[c:16]>>[#16:15]-[c:14](:[c:16]):[c;H0;D3;+0:11](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:12]:[c:13].[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
null
null
Compound (105) was prepared from compound (20) and (2-methylsulphanyl-phenyl)-boronic acid by adapting the procedure of Example 5(b). LC/MS System B; Rt=1.86 mins, m/z (ES−)=353 (M−H for C20H18O4S). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccoc1
HI.B
null
null
null
COC(=O)c1cc(COc2ccc(I)cc2)c(C)o1.CSc1ccccc1B(O)O>>CSc1ccccc1-c1ccc(OCc2cc(C(=O)O)oc2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3d6ea64c5ed048f68628e533251ab5c5
COC(=O)c1cc(CO)c(C)o1.Oc1cccc(I)c1>>COC(=O)c1cc(COc2cccc(I)c2)c(C)o1
CC(C)OC(=O)/N=N/C(=O)OC(C)C.COC(=O)C=1OC(=C(C1)CO)C.IC=1C=C(C=CC1)O.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>COC(=O)C=1OC(=C(C1)COC1=CC(=CC=C1)I)C
O[CH2:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:19][c:17]1[CH3:18].[OH:9][c:10]1[cH:11][cH:12][cH:13][c:14]([I:15])[cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][cH:13][c:14]([I:15])[cH:16]2)[c:17]([CH3:18])[o:19]1
COC(=O)c1cc(CO)c(C)o1.Oc1cccc(I)c1
COC(=O)c1cc(COc2cccc(I)c2)c(C)o1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
86bfb73617450d22f9456ed5ce4d96a73f1f8fc0c016bebae57fda68e2da86a2
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1ccc(OCc2ccoc2)cc1
O-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4](-[C:5](-[#8:6])=[O;D1;H0:7]):[#8;a:8]:[c:9]:1-[C;D1;H3:10].[OH;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#8;a:8]:[c:9](-[C;D1;H3:10]):[c:2](-[CH2;D2;+0:1]-[O;H0;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:3]:1
69
[{"value": 69.0, "product": "COC(=O)C=1OC(=C(C1)COC1=CC(=CC=C1)I)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
72
HOUR
A mixture of 4-hydroxymethyl-5-methyl-furan-2-carboxylic acid methyl ester (16) (1.85 g, 10.9 mmoles), 3-iodophenol (3.6 g, 16.35 mmoles), triphenylphosphine (4.3 g, 16.35 mmoles) in tetrahydrofuran (15 mL) was cooled to 0° C. Diisopropylazodicarboxylate (3.3 g, 16.35 mmoles) was added and the mixture was allowed to wa...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
null
null
c1ccoc1.c1ccccc1
HO-
O1CCCC1
0
72
COC(=O)c1cc(CO)c(C)o1.Oc1cccc(I)c1>O1CCCC1>COC(=O)c1cc(COc2cccc(I)c2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4a2158331057488e93cfd7699c144d36
COC(=O)c1cc(COc2cccc(I)c2)c(C)o1>>Cc1oc(C(=O)O)cc1COc1cccc(I)c1
COC(=O)C=1OC(=C(C1)COC1=CC(=CC=C1)I)C.[OH-].[Li+].O>>IC=1C=C(OCC=2C=C(OC2C)C(=O)O)C=CC1
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][O:11][c:12]2[cH:13][cH:14][cH:15][c:16]([I:17])[cH:18]2)[cH:8]1)=[O:6]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][cH:15][c:16]([I:17])[cH:18]1
COC(=O)c1cc(COc2cccc(I)c2)c(C)o1
Cc1oc(C(=O)O)cc1COc1cccc(I)c1
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(OCc2ccoc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
67.8
[{"value": 67.8, "product": "IC=1C=C(OCC=2C=C(OC2C)C(=O)O)C=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A mixture of 4-(3-iodo-phenoxymethyl)-5-methyl-furan-2-carboxylic acid methyl ester (106) (2.7 g, 7.25 mmoles) and lithium hydroxide (1.5 g, 36.25 mmoles) in tetrahydrofuran (25 ml) containing water (2 ml) was stirred at room temperature for 3 h. The tetrahydrofuran was evaporated, the residue was diluted with water an...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccoc1.c1ccccc1
Other
O1CCCC1
null
3
COC(=O)c1cc(COc2cccc(I)c2)c(C)o1>O1CCCC1>Cc1oc(C(=O)O)cc1COc1cccc(I)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1e64fadabc8040509211bab2ca1d8aa8
Cc1oc(C(=O)O)cc1COc1cccc(I)c1.OB(O)c1cccc(C(F)(F)F)c1>>Cc1oc(C(=O)O)cc1COc1cccc(-c2cccc(C(F)(F)F)c2)c1
IC=1C=C(OCC=2C=C(OC2C)C(=O)O)C=CC1.FC(C=1C=C(C=CC1)B(O)O)(F)F>>CC1=C(C=C(O1)C(=O)O)COC=1C=C(C=CC1)C1=CC(=CC=C1)C(F)(F)F
I[c:16]1[cH:15][cH:14][cH:13][c:12]([O:11][CH2:10][c:9]2[c:2]([CH3:1])[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8]2)[cH:27]1.OB(O)[c:17]1[cH:18][cH:19][cH:20][c:21]([C:22]([F:23])([F:24])[F:25])[cH:26]1>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][cH:15][c:16](-[c:17]2[cH:18][cH...
Cc1oc(C(=O)O)cc1COc1cccc(I)c1.OB(O)c1cccc(C(F)(F)F)c1
Cc1oc(C(=O)O)cc1COc1cccc(-c2cccc(C(F)(F)F)c2)c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cccc(OCc3ccoc3)c2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:2]:[c:3]
null
[]
null
null
null
null
Compound (109) was prepared from compound (107) and (3-trifluoromethyl-phenyl)-boronic acid by adapting the procedure of Example 26A(c). LC/MS System B; Rt=1.97 mins, m/z (ES−)=375 (M−H for C20H15F3O4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
Cc1oc(C(=O)O)cc1COc1cccc(I)c1.OB(O)c1cccc(C(F)(F)F)c1>>Cc1oc(C(=O)O)cc1COc1cccc(-c2cccc(C(F)(F)F)c2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-92ddf5af190d4c29a69761cabcfddae3
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1cccc(O)c1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2cccc(O)c2)cc1
IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1.OC=1C=C(C=CC1)B(O)O>>OC=1C=C(C=CC1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
I[c:15]1[cH:14][cH:13][c:12]([O:11][CH2:10][c:9]2[c:2]([CH3:1])[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8]2)[cH:24][cH:23]1.OB(O)[c:16]1[cH:17][cH:18][cH:19][c:20]([OH:21])[cH:22]1>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][cH:19][c:20]([OH:21])[c...
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1cccc(O)c1
Cc1oc(C(=O)O)cc1COc1ccc(-c2cccc(O)c2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
null
null
null
null
Compound (112) was prepared from compound (26) and (3-hydroxy-phenyl)-boronic acid by adapting the procedure of Example 27A. LC/MS System B; Rt=1.23 mins, m/z (ES−)=323 (M−H for C19H16O5). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1cccc(O)c1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2cccc(O)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c93c2c2b2c82485bbc72c0e49d1a1560
CN(C)c1ccc(B(O)O)cc1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(N(C)C)cc2)cc1
IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1.CN(C1=CC=C(C=C1)B(O)O)C>>CN(C1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O)C
OB(O)[c:16]1[cH:17][cH:18][c:19]([N:20]([CH3:21])[CH3:22])[cH:23][cH:24]1.I[c:15]1[cH:14][cH:13][c:12]([O:11][CH2:10][c:9]2[c:2]([CH3:1])[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8]2)[cH:26][cH:25]1>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][c:19](...
CN(C)c1ccc(B(O)O)cc1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1
Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(N(C)C)cc2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
null
null
null
null
Compound (113) was prepared from compound (26) and (4-dimethylamino-phenyl)-boronic acid by adapting the procedure of Example 27B. LC/MS System B; Rt=1.83 mins, m/z (ES−)=350 (M−H for C21H21NO4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
CN(C)c1ccc(B(O)O)cc1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(N(C)C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7035b38a01324b5d8ca19f4b9f3ffd87
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccc(OC(F)(F)F)cc1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(OC(F)(F)F)cc2)cc1
IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1.FC(OC1=CC=C(C=C1)B(O)O)(F)F>>CC1=C(C=C(O1)C(=O)O)COC1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)(F)F
I[c:15]1[cH:14][cH:13][c:12]([O:11][CH2:10][c:9]2[c:2]([CH3:1])[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8]2)[cH:28][cH:27]1.OB(O)[c:16]1[cH:17][cH:18][c:19]([O:20][C:21]([F:22])([F:23])[F:24])[cH:25][cH:26]1>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:...
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccc(OC(F)(F)F)cc1
Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(OC(F)(F)F)cc2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
null
null
null
null
Compound (114) was prepared from compound (26) and (4-trifluoromethoxy-phenyl)-boronic acid by adapting the procedure of Example 27B. LC/MS System C; Rt=11.01 mins, m/z (ES−)=391 (M−H for C20H15F3O5). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccc(OC(F)(F)F)cc1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(OC(F)(F)F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a445ee1ffded4aad94a53923cae7e2c0
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccccc1OC(F)(F)F>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2OC(F)(F)F)cc1
IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1.FC(OC1=C(C=CC=C1)B(O)O)(F)F>>CC1=C(C=C(O1)C(=O)O)COC1=CC=C(C=C1)C1=C(C=CC=C1)OC(F)(F)F
I[c:15]1[cH:14][cH:13][c:12]([O:11][CH2:10][c:9]2[c:2]([CH3:1])[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8]2)[cH:28][cH:27]1.OB(O)[c:16]1[cH:17][cH:18][cH:19][cH:20][c:21]1[O:22][C:23]([F:24])([F:25])[F:26]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18...
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccccc1OC(F)(F)F
Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2OC(F)(F)F)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](-[#8:10]):[c:11]>>[#8:10]-[c:9](:[c:11]):[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:7]:[c:8]
null
[]
null
null
null
null
Compound (115) was prepared from compound (26) and (2-trifluoromethoxy-phenyl)-boronic acid by adapting the procedure of Example 27B. LC/MS System B; Rt=1.97 mins, m/z (ES−)=391 (M−H for C20H15F3O5). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccccc1OC(F)(F)F>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccccc2OC(F)(F)F)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a745ebe2cec542bea3f976d0ccc14e07
COc1cccc(B(O)O)c1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1>>COc1cccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c1
IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1.COC=1C=C(C=CC1)B(O)O>>COC=1C=C(C=CC1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
OB(O)[c:7]1[cH:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:25]1.I[c:8]1[cH:9][cH:10][c:11]([O:12][CH2:13][c:14]2[cH:15][c:16]([C:17](=[O:18])[OH:19])[o:20][c:21]2[CH3:22])[cH:23][cH:24]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([O:12][CH2:13][c:14]3[cH:15][c:16]([C:17](=[O:18])[OH:19])[o:20][c:21]...
COc1cccc(B(O)O)c1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1
COc1cccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:2]:[c:3]
null
[]
null
null
null
null
Compound (116) was prepared from compound (26) and (3-methoxy-phenyl)-boronic acid by adapting the procedure of Example 27B. LC/MS System B; Rt=1.79 mins, m/z (ES−)=337 (M−H for C20H18O5). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccoc1
HI.B
null
null
null
COc1cccc(B(O)O)c1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1>>COc1cccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-75029e6729194d0fb444b8fba2204342
CC(=O)c1cccc(B(O)O)c1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1>>CC(=O)c1cccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c1
IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1.C(C)(=O)C=1C=C(C=CC1)B(O)O>>C(C)(=O)C=1C=C(C=CC1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
OB(O)[c:8]1[cH:7][cH:6][cH:5][c:4]([C:2]([CH3:1])=[O:3])[cH:26]1.I[c:9]1[cH:10][cH:11][c:12]([O:13][CH2:14][c:15]2[cH:16][c:17]([C:18](=[O:19])[OH:20])[o:21][c:22]2[CH3:23])[cH:24][cH:25]1>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([O:13][CH2:14][c:15]3[cH:16][c:17]([C:18](=[O:19])[O...
CC(=O)c1cccc(B(O)O)c1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1
CC(=O)c1cccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]-[C:9](-[C;D1;H3:10])=[O;D1;H0:11]):[c:12]:[c:13]>>[C;D1;H3:10]-[C:9](=[O;D1;H0:11])-[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:12]:[c:13]
null
[]
null
null
null
null
Compound (117) was prepared from compound (26) and (3-acetyl-phenyl)-boronic acid by adapting the procedure of Example 27B. LC/MS System B; Rt=1.69 mins, m/z (ES−) 349 (M−H for C21H18O5). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccoc1
HI.B
null
null
null
CC(=O)c1cccc(B(O)O)c1.Cc1oc(C(=O)O)cc1COc1ccc(I)cc1>>CC(=O)c1cccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9c103d1d8e37431983902d7095198680
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccc(F)cc1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(F)cc2)cc1
IC1=CC=C(OCC=2C=C(OC2C)C(=O)O)C=C1.FC1=CC=C(C=C1)B(O)O>>FC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
I[c:15]1[cH:14][cH:13][c:12]([O:11][CH2:10][c:9]2[c:2]([CH3:1])[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8]2)[cH:24][cH:23]1.OB(O)[c:16]1[cH:17][cH:18][c:19]([F:20])[cH:21][cH:22]1>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][O:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][c:19]([F:20])[cH:21][cH:...
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccc(F)cc1
Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(F)cc2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
null
null
null
null
Compound (118) was prepared from compound (26) and (4-fluoro-phenyl)-boronic acid by adapting the procedure of Example 27B. LC/MS System B; Rt=1.79 mins, m/z (ES−)=325 (M−H for C19H15FO4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
null
null
null
Cc1oc(C(=O)O)cc1COc1ccc(I)cc1.OB(O)c1ccc(F)cc1>>Cc1oc(C(=O)O)cc1COc1ccc(-c2ccc(F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-210eee0a1b654d54865c2dd8538b0772
CN(C)S(N)(=O)=O.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1>>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)N(C)C)oc3C)cc2)cc1
CN(S(=O)(=O)N)C.Cl.CN(CCCN=C=NCC)C.COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O>>COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)N(C)C
[NH2:18][S:19](=[O:20])(=[O:21])[N:22]([CH3:23])[CH3:24].O[C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:31][cH:30]3)[cH:29][cH:28]2)[c:26]([CH3:27])[o:25]1)=[O:17]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([O:11][CH2:12][c:13]3[cH:14][c...
CN(C)S(N)(=O)=O.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1
COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)N(C)C)oc3C)cc2)cc1
null
CN(C1=CC=NC=C1)C
ClCCl
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[#7:7]-[#16:8](-[NH2;D1;+0:9])(=[O;D1;H0:10])=[O;D1;H0:11]>>[#7:7]-[#16:8](=[O;D1;H0:10])(=[O;D1;H0:11])-[NH;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6]
35.7
[{"value": 35.7, "product": "COC1=CC=C(C=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)N(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
N,N-Dimethylsulphamide (73 mg, 0.59 mmoles), 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (31 mg, 0.162 mmoles) and dimethyl-pyridin-4-yl-amine (1 mg) were added to a stirred solution of 4-(4′-methoxy-biphenyl-4-yloxymethyl)-5-methyl-furan-2-carboxylic acid (4) (50 mg, 0.148 mmoles) in dichloromethane ...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccoc1
HO-
CN(C1=CC=NC=C1)C.ClCCl
null
18
CN(C)S(N)(=O)=O.COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)cc1>CN(C1=CC=NC=C1)C.ClCCl>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)N(C)C)oc3C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b70a8f12d1c243739b8e0a7b71a61923
Cc1occc1CO.Oc1ccc(I)cc1>>Cc1occc1COc1ccc(I)cc1
CC=1OC=CC1CO.IC1=CC=C(C=C1)O>>IC1=CC=C(OCC2=C(OC=C2)C)C=C1
O[CH2:7][c:6]1[c:2]([CH3:1])[o:3][cH:4][cH:5]1.[OH:8][c:9]1[cH:10][cH:11][c:12]([I:13])[cH:14][cH:15]1>>[CH3:1][c:2]1[o:3][cH:4][cH:5][c:6]1[CH2:7][O:8][c:9]1[cH:10][cH:11][c:12]([I:13])[cH:14][cH:15]1
Cc1occc1CO.Oc1ccc(I)cc1
Cc1occc1COc1ccc(I)cc1
null
null
null
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
86bfb73617450d22f9456ed5ce4d96a73f1f8fc0c016bebae57fda68e2da86a2
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1ccc(OCc2ccoc2)cc1
O-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[#8;a:5]:[c:6]:1-[C;D1;H3:7].[OH;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[C;D1;H3:7]-[c:6]1:[#8;a:5]:[c:4]:[c:3]:[c:2]:1-[CH2;D2;+0:1]-[O;H0;D2;+0:8]-[c:9](:[c:10]):[c:11]
null
[]
null
null
null
null
3-(4-Iodo-phenoxymethyl)-2-methyl-furan was prepared from (2-methyl-furan-3-yl)-methanol and 4-iodo-phenol in an analogous manner to that described in Example 14(a). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
null
null
c1ccoc1.c1ccccc1
HO-
null
null
null
Cc1occc1CO.Oc1ccc(I)cc1>>Cc1occc1COc1ccc(I)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-30912a3d6da24e659691cf8a35221043
Cc1occc1COc1ccc(I)cc1.OB(O)c1ccc(F)cc1>>Cc1occc1COc1ccc(-c2ccc(F)cc2)cc1
FC1=CC=C(C=C1)B(O)O.IC1=CC=C(OCC2=C(OC=C2)C)C=C1.C(C)(=O)[O-].[K+]>>FC1=CC=C(C=C1)C1=CC=C(C=C1)OCC1=C(OC=C1)C
I[c:12]1[cH:11][cH:10][c:9]([O:8][CH2:7][c:6]2[c:2]([CH3:1])[o:3][cH:4][cH:5]2)[cH:21][cH:20]1.OB(O)[c:13]1[cH:14][cH:15][c:16]([F:17])[cH:18][cH:19]1>>[CH3:1][c:2]1[o:3][cH:4][cH:5][c:6]1[CH2:7][O:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][c:16]([F:17])[cH:18][cH:19]2)[cH:20][cH:21]1
Cc1occc1COc1ccc(I)cc1.OB(O)c1ccc(F)cc1
Cc1occc1COc1ccc(-c2ccc(F)cc2)cc1
null
null
CN(C=O)C
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
44.3
[{"value": 44.3, "product": "FC1=CC=C(C=C1)C1=CC=C(C=C1)OCC1=C(OC=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
95
CELSIUS
12
HOUR
A mixture of (4-fluoro-phenyl)-boronic acid (300 mg, 2.1 mmoles), 3-(4-iodophenoxymethyl)-2-methyl-furan (123) (500 mg, 1.6 mmoles) and potassium acetate (0.6 g) in N,N-dimethylformamide (70 mL) was degassed, treated with [1,1′-bis(diphenylphosphino) ferrocene]dichloropalladium(II) complex with dichloromethane (1:1) (9...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
CN(C=O)C
95
12
Cc1occc1COc1ccc(I)cc1.OB(O)c1ccc(F)cc1>CN(C=O)C>Cc1occc1COc1ccc(-c2ccc(F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7fb2007ee68c4b29b71708a42bf794c5
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccccc1Br>>COC(=O)c1cc(COc2ccc(-c3ccccc3OC)cc2)c(C)o1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)B1OC(C(O1)(C)C)(C)C)C.BrC1=C(C=CC=C1)OC.C([O-])([O-])=O.[Cs+].[Cs+].ClCCl>>COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=C(C=CC=C1)OC)C
CC1(C)OB([c:13]2[cH:12][cH:11][c:10]([O:9][CH2:8][c:7]3[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:26][c:24]3[CH3:25])[cH:23][cH:22]2)OC1(C)C.Br[c:14]1[cH:15][cH:16][cH:17][cH:18][c:19]1[O:20][CH3:21]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][cH:18][c...
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccccc1Br
COC(=O)c1cc(COc2ccc(-c3ccccc3OC)cc2)c(C)o1
null
null
O1CCOCC1
C-C Coupling
Suzuki coupling with boronic esters
8b44d63590c7228953eb9acb565338c9584155fdcec14c37f9f3f344e065dc2d
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[#8:5]):[c:6].C-C1(-C)-O-B(-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11])-O-C-1(-C)-C>>[#8:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]):[c:2]:[c:3]
21
[{"value": 21.0, "product": "COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=C(C=CC=C1)OC)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A degassed mixture of 5-methyl-4-[4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-phenoxymethyl]-furan-2-carboxylic acid methyl ester (119) (200 mg, 0.54 mmoles), 1-bromo-2-methoxy-benzene (80 μl, 0.65 mmoles), 2M aqueous cesium carbonate (11.0 ml) and), [1,1′-bis(diphenylphosphino) ferrocene]dichloropalladium(II) com...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HBr.B
O1CCOCC1
null
null
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccccc1Br>O1CCOCC1>COC(=O)c1cc(COc2ccc(-c3ccccc3OC)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-32c077bc389d4444b4569049d81dd19a
COC(=O)c1cc(COc2ccc(-c3ccccc3OC)cc2)c(C)o1>>COc1ccccc1-c1ccc(OCc2cc(C(=O)O)oc2C)cc1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=C(C=CC=C1)OC)C>>COC1=C(C=CC=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O
C[O:20][C:18]([c:17]1[cH:16][c:15]([CH2:14][O:13][c:12]2[cH:11][cH:10][c:9](-[c:8]3[c:3]([O:2][CH3:1])[cH:4][cH:5][cH:6][cH:7]3)[cH:25][cH:24]2)[c:22]([CH3:23])[o:21]1)=[O:19]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[c:9]1[cH:10][cH:11][c:12]([O:13][CH2:14][c:15]2[cH:16][c:17]([C:18](=[O:19])[OH:20])[o:21][c:...
COC(=O)c1cc(COc2ccc(-c3ccccc3OC)cc2)c(C)o1
COc1ccccc1-c1ccc(OCc2cc(C(=O)O)oc2C)cc1
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
77.9
[{"value": 77.9, "product": "COC1=C(C=CC=C1)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
A solution of 4-(2′-methoxy-biphenyl-4-yloxymethyl)-5-methyl-furan-2-carboxylic acid methyl ester (125) (40 mg, 0.11 mmoles) in dry tetrahydrofuran (25 ml) was treated with potassium trimethylsilanoate (73 mg, 0.56 mmoles) and the mixture stirred under an argon atmosphere for 16 h. After evaporation of the solvent the ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccoc1
Other
O1CCCC1
null
16
COC(=O)c1cc(COc2ccc(-c3ccccc3OC)cc2)c(C)o1>O1CCCC1>COc1ccccc1-c1ccc(OCc2cc(C(=O)O)oc2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8a13edad80be449c95a88f481f6b85d9
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.FC(F)Oc1ccc(I)cc1>>COC(=O)c1cc(COc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)B1OC(C(O1)(C)C)(C)C)C.FC(OC1=CC=C(C=C1)I)F.C([O-])([O-])=O.[Cs+].[Cs+].ClCCl.FC(OC1=CC=C(C=C1)I)F.ClCCl>>COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C
CC1(C)OB([c:13]2[cH:12][cH:11][c:10]([O:9][CH2:8][c:7]3[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:28][c:26]3[CH3:27])[cH:25][cH:24]2)OC1(C)C.I[c:14]1[cH:15][cH:16][c:17]([O:18][CH:19]([F:20])[F:21])[cH:22][cH:23]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][c...
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.FC(F)Oc1ccc(I)cc1
COC(=O)c1cc(COc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
null
null
O1CCOCC1
C-C Coupling
Suzuki coupling with boronic esters
8b44d63590c7228953eb9acb565338c9584155fdcec14c37f9f3f344e065dc2d
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
C-C1(-C)-O-B(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-O-C-1(-C)-C.I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
57.2
[{"value": 57.2, "product": "COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
4
HOUR
A degassed mixture of 5-methyl-4-[4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-phenoxymethyl]-furan-2-carboxylic acid methyl ester (119) (200 mg, 0.54 mmoles), 4-difluoromethoxy-1-iodo-benzene (175 mg, 0.65 mmoles), 2M aqueous cesium carbonate (0.81 ml) and), [1,1′-bis(diphenylphosphino) ferrocene]dichloropalladium...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
O1CCOCC1
80
4
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.FC(F)Oc1ccc(I)cc1>O1CCOCC1>COC(=O)c1cc(COc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5a847f4c405547528e5dae171d2c92c6
Brc1ncccn1.COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1>>COC(=O)c1cc(COc2ccc(-c3ncccn3)cc2)c(C)o1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)B1OC(C(O1)(C)C)(C)C)C.BrC1=NC=CC=N1>>COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=NC=CC=N1)C
Br[c:14]1[n:15][cH:16][cH:17][cH:18][n:19]1.CC1(C)OB([c:13]2[cH:12][cH:11][c:10]([O:9][CH2:8][c:7]3[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:24][c:22]3[CH3:23])[cH:21][cH:20]2)OC1(C)C>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[n:15][cH:16][cH:17][cH:18][n:19]3)[cH:20][cH...
Brc1ncccn1.COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1
COC(=O)c1cc(COc2ccc(-c3ncccn3)cc2)c(C)o1
null
null
null
C-C Coupling
Suzuki coupling with boronic esters
90181dd6ff486545b377979be4eda7b1ee93a9a36374e4157c8be739bec9f2e6
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1cnc(-c2ccc(OCc3ccoc3)cc2)nc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].C-C1(-C)-O-B(-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10])-O-C-1(-C)-C>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5]):[c:9]:[c:10]
null
[]
null
null
null
null
Compound (136) was prepared from compound (119) and 2-bromo-pyrimidine by adapting the procedure of Example 30(a). LC/MS System A; Rt=3.43 mins, m/z (ES+)=325 (M+H for C18H16N2O4). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1cncnc1.B1OCCO1.c1ccccc1
c1ccccc1.c1cncnc1
c1ccoc1.c1ccccc1.c1cncnc1
HBr.B
null
null
null
Brc1ncccn1.COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1>>COC(=O)c1cc(COc2ccc(-c3ncccn3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-79af233fa6814a859a89fefa6149c7f3
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccc(Br)c(OC)c1>>COC(=O)c1cc(COc2ccc(-c3ccc(OC)cc3OC)cc2)c(C)o1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)B1OC(C(O1)(C)C)(C)C)C.BrC1=C(C=C(C=C1)OC)OC>>COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=C(C=C(C=C1)OC)OC)C
CC1(C)OB([c:13]2[cH:12][cH:11][c:10]([O:9][CH2:8][c:7]3[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:28][c:26]3[CH3:27])[cH:25][cH:24]2)OC1(C)C.Br[c:14]1[cH:15][cH:16][c:17]([O:18][CH3:19])[cH:20][c:21]1[O:22][CH3:23]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][...
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccc(Br)c(OC)c1
COC(=O)c1cc(COc2ccc(-c3ccc(OC)cc3OC)cc2)c(C)o1
null
null
null
C-C Coupling
Suzuki coupling with boronic esters
8b44d63590c7228953eb9acb565338c9584155fdcec14c37f9f3f344e065dc2d
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[#8:5]):[c:6].C-C1(-C)-O-B(-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11])-O-C-1(-C)-C>>[#8:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]):[c:2]:[c:3]
null
[]
null
null
null
null
Compound (139) was prepared from compound (119) and 1-bromo-2,4-dimethoxy-benzene by adapting the procedure of Example 31(a). LC/MS System A; Rt=4.09 mins. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccc(Br)c(OC)c1>>COC(=O)c1cc(COc2ccc(-c3ccc(OC)cc3OC)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b22e48cec180493eb8ca108d7f33a7e3
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c(OC)c1.NS(=O)(=O)c1ccccc1>>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccccc4)oc3C)cc2)c(OC)c1
COC1=C(C=CC(=C1)OC)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)O.C1(=CC=CC=C1)S(=O)(=O)N.Cl.CN(CCCN=C=NCC)C>>COC1=C(C=CC(=C1)OC)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=CC=CC=C1
O[C:16]([c:15]1[cH:14][c:13]([CH2:12][O:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:36][c:33]3[O:34][CH3:35])[cH:32][cH:31]2)[c:29]([CH3:30])[o:28]1)=[O:17].[NH2:18][S:19](=[O:20])(=[O:21])[c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10...
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c(OC)c1.NS(=O)(=O)c1ccccc1
COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccccc4)oc3C)cc2)c(OC)c1
null
CN(C)C1=CC=NC=C1
O1CCCC1.C(C)#N
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(COc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[c:3](:[c:4]):[#8;a:5]:[c:6]
34.8
[{"value": 34.8, "product": "COC1=C(C=CC(=C1)OC)C1=CC=C(C=C1)OCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
A stirred solution of 4-(2′,4′-dimethoxy-biphenyl-4-yloxymethyl)-5-methyl-furan-2-carboxylic acid (140) (50 mg, 0.136 mmoles), benzenesulphonamide (32 mg, 0.204 mmoles) and 4-(N,N-dimethylamino)-pyridine (5 mg) in a mixture of tetrahydrofuran (8 ml) and acetonitrile (2 ml) was treated with 1-(3-dimethylaminopropyl)-3-e...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccoc1.c1ccccc1
HO-
CN(C)C1=CC=NC=C1.O1CCCC1.C(C)#N
null
16
COc1ccc(-c2ccc(OCc3cc(C(=O)O)oc3C)cc2)c(OC)c1.NS(=O)(=O)c1ccccc1>CN(C)C1=CC=NC=C1.O1CCCC1.C(C)#N>COc1ccc(-c2ccc(OCc3cc(C(=O)NS(=O)(=O)c4ccccc4)oc3C)cc2)c(OC)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-419665407b5e432f9d2e271fb35c29c6
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccc(Br)c(C)c1>>COC(=O)c1cc(COc2ccc(-c3ccc(OC)cc3C)cc2)c(C)o1
COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)B1OC(C(O1)(C)C)(C)C)C.BrC1=C(C=C(C=C1)OC)C>>COC(=O)C=1OC(=C(C1)COC1=CC=C(C=C1)C1=C(C=C(C=C1)OC)C)C
CC1(C)OB([c:13]2[cH:12][cH:11][c:10]([O:9][CH2:8][c:7]3[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:27][c:25]3[CH3:26])[cH:24][cH:23]2)OC1(C)C.Br[c:14]1[cH:15][cH:16][c:17]([O:18][CH3:19])[cH:20][c:21]1[CH3:22]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][c:17](...
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccc(Br)c(C)c1
COC(=O)c1cc(COc2ccc(-c3ccc(OC)cc3C)cc2)c(C)o1
null
null
null
C-C Coupling
Suzuki coupling with boronic esters
8b44d63590c7228953eb9acb565338c9584155fdcec14c37f9f3f344e065dc2d
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C;D1;H3:5]):[c:6].C-C1(-C)-O-B(-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11])-O-C-1(-C)-C>>[C;D1;H3:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]):[c:2]:[c:3]
null
[]
null
null
null
null
Compound (143) was prepared from compound (119) and 1-bromo-4-methoxy-2-methyl-benzene by adapting the procedure of Example 31(a). LC/MS System A; Rt=4.24 mins. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1cc(COc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.COc1ccc(Br)c(C)c1>>COC(=O)c1cc(COc2ccc(-c3ccc(OC)cc3C)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-27f5cc3427694e1da2beab85727cff68
Cc1oc(C#N)cc1CO.Oc1ccc(-c2ccccc2)cc1>>Cc1oc(C#N)cc1COc1ccc(-c2ccccc2)cc1
CC(C)OC(=O)/N=N/C(=O)OC(C)C.OCC=1C=C(OC1C)C#N.C1(=CC=C(C=C1)O)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>C1(=CC=C(C=C1)OCC=1C=C(OC1C)C#N)C1=CC=CC=C1
[CH3:1][c:2]1[o:3][c:4]([C:5]#[N:6])[cH:7][c:8]1[CH2:9][OH:10].O[c:11]1[cH:12][cH:13][c:14](-[c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[cH:21][cH:22]1>>[CH3:1][c:2]1[o:3][c:4]([C:5]#[N:6])[cH:7][c:8]1[CH2:9][O:10][c:11]1[cH:12][cH:13][c:14](-[c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[cH:21][cH:22]1
Cc1oc(C#N)cc1CO.Oc1ccc(-c2ccccc2)cc1
Cc1oc(C#N)cc1COc1ccc(-c2ccccc2)cc1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
8915084acbaaf997bf0f89ff5187cb2f89c25dc683fffc57b3391298c8430dd9
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1ccc(-c2ccc(OCc3ccoc3)cc2)cc1
O-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#8;a:6]:[c:7]:[c:8]-[C:9]-[OH;D1;+0:10]>>[#8;a:6]:[c:7]:[c:8]-[C:9]-[O;H0;D2;+0:10]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
79.2
[{"value": 79.2, "product": "C1(=CC=C(C=C1)OCC=1C=C(OC1C)C#N)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
5
MINUTE
Diisopropylazodicarboxylate (1.84 g, 10.6 mmoles) was added to a solution of 4-hydroxymethyl-5-methyl-furan-2-carbonitrile (147) (1.32 g, 9.6 mmoles), biphenyl-4-ol (1.63 g, 9.6 mmoles) and triphenylphosphine (4.3 g, 16.35 mmoles) in tetrahydrofuran (50 mL) with stirring and cooling to 0° C. under an argon atmosphere. ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HO-
O1CCCC1
0
0.083333
Cc1oc(C#N)cc1CO.Oc1ccc(-c2ccccc2)cc1>O1CCCC1>Cc1oc(C#N)cc1COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b8900bbc90f4450c81aefb0fb7deb8e5
Cc1oc(C#N)cc1COc1ccc(-c2ccccc2)cc1.[N-]=[N+]=[N-]>>Cc1oc(-c2nnn[nH]2)cc1COc1ccc(-c2ccccc2)cc1
C1(=CC=C(C=C1)OCC=1C=C(OC1C)C#N)C1=CC=CC=C1.[N-]=[N+]=[N-].[Na+].C([O-])([O-])=O.[K+].[K+]>>C1(=CC=C(C=C1)OCC=1C=C(OC1C)C1=NN=NN1)C1=CC=CC=C1
[CH3:1][c:2]1[o:3][c:4]([C:5]#[N:6])[cH:10][c:11]1[CH2:12][O:13][c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[cH:24][cH:25]1.[N+:7](=[N-:8])=[N-:9]>>[CH3:1][c:2]1[o:3][c:4](-[c:5]2[n:6][n:7][n:8][nH:9]2)[cH:10][c:11]1[CH2:12][O:13][c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:...
Cc1oc(C#N)cc1COc1ccc(-c2ccccc2)cc1.[N-]=[N+]=[N-]
Cc1oc(-c2nnn[nH]2)cc1COc1ccc(-c2ccccc2)cc1
null
null
CN(C=O)C
Aromatic Heterocycle Formation
OtherReaction
237b84aaa459abf427f233dc6a07a1d9de824f980714e458423189bb68f60f12
d8c808528b7ee68720aaeebd35cb6a2a30e344748d0066102cdae99843b93cf0
c1ccc(-c2ccc(OCc3coc(-c4nnn[nH]4)c3)cc2)cc1
[N-;H0;D1:1]=[N+;H0;D2:2]=[N-;H0;D1:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[c;H0;D3;+0:6]1:[#8;a:7]:[c:8]:[c:9]:[c:10]:1>>[#8;a:7]1:[c:8]:[c:9]:[c:10]:[c;H0;D3;+0:6]:1-[c;H0;D3;+0:5]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:2]:[n;H0;D2;+0:1]:[nH;D2;+0:3]:1
55
[{"value": 55.0, "product": "C1(=CC=C(C=C1)OCC=1C=C(OC1C)C1=NN=NN1)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
24
HOUR
A mixture of 4-(biphenyl-4-yloxymethyl)-5-methyl-furan-2-carbonitrile (148) (100 mg, 0.35 mmoles), sodium azide (27 mg, 0.415 mmoles) and potassium carbonate (62 mg, 0.45 mmoles) in dimethylformamide (5 ml) was heated at 90° C. for 96 hours then at 120° C. for 24 hours. The mixture was evaporated and the residue purifi...
10.6084/m9.figshare.5104873.v1
null
Nitrile
null
null
c1nnn[nH]1
c1ccoc1.c1nnn[nH]1.c1ccccc1.c1ccccc1
null
CN(C=O)C
90
24
Cc1oc(C#N)cc1COc1ccc(-c2ccccc2)cc1.[N-]=[N+]=[N-]>CN(C=O)C>Cc1oc(-c2nnn[nH]2)cc1COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fb1d3ffecd354896b31b0d389b91a1c5
COC(=O)c1cc(CO)c(C)o1.Sc1ccc(Br)cc1>>COC(=O)c1cc(CSc2ccc(Br)cc2)c(C)o1
CC(C)OC(=O)/N=N/C(=O)OC(C)C.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.COC(=O)C=1OC(=C(C1)CO)C.BrC1=CC=C(C=C1)S>>COC(=O)C=1OC(=C(C1)CSC1=CC=C(C=C1)Br)C
O[CH2:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:19][c:17]1[CH3:18].[SH:9][c:10]1[cH:11][cH:12][c:13]([Br:14])[cH:15][cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][S:9][c:10]2[cH:11][cH:12][c:13]([Br:14])[cH:15][cH:16]2)[c:17]([CH3:18])[o:19]1
COC(=O)c1cc(CO)c(C)o1.Sc1ccc(Br)cc1
COC(=O)c1cc(CSc2ccc(Br)cc2)c(C)o1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
S-alkylation of thiols with alcohols
c119424abb7b621e5fb126e8156c5e4310815e8f2d609f48f2eb427b327d29ac
c1ccf05c97341d9cf75acae4c03f7d5a8212340a35905af6c8d60b4ccc775d1f
c1ccc(SCc2ccoc2)cc1
O-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4](-[C:5](-[#8:6])=[O;D1;H0:7]):[#8;a:8]:[c:9]:1-[C;D1;H3:10].[SH;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#8;a:8]:[c:9](-[C;D1;H3:10]):[c:2](-[CH2;D2;+0:1]-[S;H0;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:3]:1
null
[]
null
null
null
null
Diisopropylazodicarboxylate (1.27 g, 6.3 mmoles) was added to a solution of triphenylphosphine (1.65 g, 6.3 mmoles) in tetrahydrofuran (15 ml) with stirring and cooling in an ice/water bath. A solution of 4-hydroxymethyl-5-methyl-furan-2-carboxylic acid methyl ester (16) (536 mg, 3.15 mmoles) and 4-bromo-thiophenol (58...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic thiol
Monosulfide
null
null
c1ccoc1.c1ccccc1
HO-
O1CCCC1
null
null
COC(=O)c1cc(CO)c(C)o1.Sc1ccc(Br)cc1>O1CCCC1>COC(=O)c1cc(CSc2ccc(Br)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-08dae77882a24fb899fc4358c13c2176
CC1(C)OBOC1(C)C.COC(=O)c1cc(CSc2ccc(Br)cc2)c(C)o1>>COC(=O)c1cc(CSc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1
ClCCl.CC1(OBOC1(C)C)C.COC(=O)C=1OC(=C(C1)CSC1=CC=C(C=C1)Br)C>>COC(=O)C=1OC(=C(C1)CSC1=CC=C(C=C1)B1OC(C(O1)(C)C)(C)C)C
[BH:14]1[O:15][C:16]([CH3:17])([CH3:18])[C:19]([CH3:20])([CH3:21])[O:22]1.Br[c:13]1[cH:12][cH:11][c:10]([S:9][CH2:8][c:7]2[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:27][c:25]2[CH3:26])[cH:24][cH:23]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][S:9][c:10]2[cH:11][cH:12][c:13]([B:14]3[O:15][C:16]([CH3:17])([CH3:18]...
CC1(C)OBOC1(C)C.COC(=O)c1cc(CSc2ccc(Br)cc2)c(C)o1
COC(=O)c1cc(CSc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1
null
null
O1CCCC1.O1CCOCC1
Miscellaneous
OtherReaction
ad2870ebdd035b36ca28b76fce8ec2fa1001820252a6151877804f04f83d958c
f1d1202adfbfb63cdbea2fa31eb5766b49914acb653b77a04e8043b460a99de7
c1cc(CSc2ccc(B3OCCO3)cc2)co1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#8:6]1-[BH;D2;+0:7]-[#8:8]-[C:9]-[C:10]-1>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[B;H0;D3;+0:7]1-[#8:6]-[C:10]-[C:9]-[#8:8]-1):[c:4]:[c:5]
null
[]
100
CELSIUS
null
null
[1,1′-Bis(diphenylphosphino)ferrocene]dichloropalladium(II) complex with dichloromethane (1:1) (30 mg) and 4,4,5,5-tetramethyl-[1,3,2]dioxaborolane (2.34 ml of a 1M solution in tetrahydrofuran) were added to a degassed solution of 4-(4-bromo-phenylsulphanylmethyl)-5-methyl-furan-2-carboxylic acid methyl ester (150) (40...
10.6084/m9.figshare.5104873.v1
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Aromatic halide
Boronic ester
B1OCCO1.c1ccccc1
c1ccccc1.[B]1OCCO1
c1ccoc1.c1ccccc1.[B]1OCCO1
HBr
O1CCCC1.O1CCOCC1
100
null
CC1(C)OBOC1(C)C.COC(=O)c1cc(CSc2ccc(Br)cc2)c(C)o1>O1CCCC1.O1CCOCC1>COC(=O)c1cc(CSc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8f007f3003364e23bbbf9a999df757cb
COC(=O)c1cc(CSc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.FC(F)Oc1ccc(I)cc1>>COC(=O)c1cc(CSc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
ClCCl.COC(=O)C=1OC(=C(C1)CSC1=CC=C(C=C1)B1OC(C(O1)(C)C)(C)C)C.FC(OC1=CC=C(C=C1)I)F.C([O-])([O-])=O.[Cs+].[Cs+]>>COC(=O)C=1OC(=C(C1)CSC1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C
CC1(C)OB([c:13]2[cH:12][cH:11][c:10]([S:9][CH2:8][c:7]3[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:28][c:26]3[CH3:27])[cH:25][cH:24]2)OC1(C)C.I[c:14]1[cH:15][cH:16][c:17]([O:18][CH:19]([F:20])[F:21])[cH:22][cH:23]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][S:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][c...
COC(=O)c1cc(CSc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.FC(F)Oc1ccc(I)cc1
COC(=O)c1cc(CSc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
null
null
O1CCOCC1
C-C Coupling
Suzuki coupling with boronic esters
8b44d63590c7228953eb9acb565338c9584155fdcec14c37f9f3f344e065dc2d
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(-c2ccc(SCc3ccoc3)cc2)cc1
C-C1(-C)-O-B(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-O-C-1(-C)-C.I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
60.4
[{"value": 60.4, "product": "COC(=O)C=1OC(=C(C1)CSC1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
[1,1′-Bis(diphenylphosphino) ferrocene]dichloropalladium(II) complex with dichloromethane (1:1) (12.8 mg) was added to a degassed mixture of 5-methyl-4-[4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-phenylsulphanylmethyl]-furan-2-carboxylic acid methyl ester (151) (200 mg, 0.516 mmoles), 1-difluoromethoxy-4-iodo-ben...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccoc1.c1ccccc1.c1ccccc1
HI.B
O1CCOCC1
100
null
COC(=O)c1cc(CSc2ccc(B3OC(C)(C)C(C)(C)O3)cc2)c(C)o1.FC(F)Oc1ccc(I)cc1>O1CCOCC1>COC(=O)c1cc(CSc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-21b55cf35030424cb7583962d1272e3c
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CSc1ccc(-c2ccc(OC(F)F)cc2)cc1>>Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CSc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)SCC=1C=C(OC1C)C(=O)O)F.CC1=C(C=CC=C1)S(=O)(=O)N>>FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)SCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=C(C=CC=C1)C)F
[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:9])(=[O:10])[NH2:11].O[C:12](=[O:13])[c:14]1[cH:15][c:16]([CH2:17][S:18][c:19]2[cH:20][cH:21][c:22](-[c:23]3[cH:24][cH:25][c:26]([O:27][CH:28]([F:29])[F:30])[cH:31][cH:32]3)[cH:33][cH:34]2)[c:35]([CH3:36])[o:37]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:...
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CSc1ccc(-c2ccc(OC(F)F)cc2)cc1
Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CSc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(CSc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:9]=[#16:8](=[O;D1;H0:10])(-[c:11])-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6]
null
[]
null
null
null
null
Compound (154) was prepared from compound (153) and 2-methyl-benzenesulphonamide by adapting the procedure of Example 34(c). LC/MS System D; Rt=11.61 mins, m/z (ES+)=544 (M+H for C27H23F2NO5S2). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.c1ccoc1.c1ccccc1.c1ccccc1
HO-
null
null
null
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CSc1ccc(-c2ccc(OC(F)F)cc2)cc1>>Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CSc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-546f1a850b5743a5a9dda2d130876e8d
COC(=O)c1cc(CO)c(C)o1>>COC(=O)c1cc(C=O)c(C)o1
O.O.O.O.O.S(=S)(=O)([O-])[O-].[Na+].[Na+].C(C)(=O)OI1(OC(C2=CC=CC=C12)=O)(OC(C)=O)OC(C)=O.COC(=O)C=1OC(=C(C1)CO)C.C([O-])(O)=O.[Na+]>>COC(=O)C=1OC(=C(C1)C=O)C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][OH:9])[c:10]([CH3:11])[o:12]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH:8]=[O:9])[c:10]([CH3:11])[o:12]1
COC(=O)c1cc(CO)c(C)o1
COC(=O)c1cc(C=O)c(C)o1
null
null
ClCCl.C(C)OCC
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccoc1
[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#8;a:5]:[c:6](-[C;D1;H3:7]):[c:8](-[CH2;D2;+0:9]-[OH;D1;+0:10]):[c:11]:1>>[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#8;a:5]:[c:6](-[C;D1;H3:7]):[c:8](-[CH;D2;+0:9]=[O;H0;D1;+0:10]):[c:11]:1
70.8
[{"value": 70.8, "product": "COC(=O)C=1OC(=C(C1)C=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
20
MINUTE
Acetic acid 1,1-diacetoxy-3-oxo-1λ5-ioda-2-oxa-indan-1-yl ester (Dess-Martin reagent) (549 mg, 1.293 mmoles) in dry dichloromethane was added to a solution of 4-hydroxymethyl-5-methyl-furan-2-carboxylic acid methyl ester (16) (200 mg, 1.176 mmoles) in dry dichloromethane (9 ml) with cooling to 0° C. under an argon atmo...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccoc1
null
ClCCl.C(C)OCC
0
0.333333
COC(=O)c1cc(CO)c(C)o1>ClCCl.C(C)OCC>COC(=O)c1cc(C=O)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-42862eee63924cddb9006d6a9ab1e024
COC(=O)c1cc(C=O)c(C)o1.Nc1ccc(-c2ccccc2)cc1>>COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
C1(=CC=C(C=C1)N)C1=CC=CC=C1.COC(=O)C=1OC(=C(C1)C=O)C.C(#N)[BH3-].[Na+]>>COC(=O)C=1OC(=C(C1)CNC1=CC=C(C=C1)C1=CC=CC=C1)C
O=[CH:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:24][c:22]1[CH3:23].[NH2:9][c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[cH:20][cH:21]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][NH:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][cH:18][cH:19]3)[cH:20][cH:21]2)[c:2...
COC(=O)c1cc(C=O)c(C)o1.Nc1ccc(-c2ccccc2)cc1
COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
null
null
CO
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
c1ccc(-c2ccc(NCc3ccoc3)cc2)cc1
O=[CH;D2;+0:1]-[c:2]1:[c:3]:[c:4](-[C:5](-[#8:6])=[O;D1;H0:7]):[#8;a:8]:[c:9]:1-[C;D1;H3:10].[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#8;a:8]:[c:9](-[C;D1;H3:10]):[c:2](-[CH2;D2;+0:1]-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:3]:1
29.1
[{"value": 29.1, "product": "COC(=O)C=1OC(=C(C1)CNC1=CC=C(C=C1)C1=CC=CC=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
A solution of biphenyl-4-ylamine (150 mg, 0.883 mmoles) and 4-formyl-5-methyl-furan-2-carboxylic acid methyl ester (157) (135 mg, 0.803 mmoles) in methanol (2.0 ml) was stirred over molecular sieves (type 3 Å) for 1 hour. Sodium cyanoborohydride (55 mg, 0.883 mmoles) was added and the mixture stirred for 18 hour at roo...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccoc1.c1ccccc1.c1ccccc1
Other
CO
null
18
COC(=O)c1cc(C=O)c(C)o1.Nc1ccc(-c2ccccc2)cc1>CO>COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e646003c904d4701a39f4a2a6e5f1e6f
COC(=O)c1cc(CO)c(C)o1.Cc1ccc(S(=O)(=O)Cl)cc1>>COC(=O)c1cc(CCl)c(C)o1
C(C)N(CC)CC.CC1=CC=C(C=C1)S(=O)(=O)Cl.COC(=O)C=1OC(=C(C1)CO)C>>COC(=O)C=1OC(=C(C1)CCl)C
O[CH2:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:12][c:10]1[CH3:11].Cc1ccc(S(=O)(=O)[Cl:9])cc1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][Cl:9])[c:10]([CH3:11])[o:12]1
COC(=O)c1cc(CO)c(C)o1.Cc1ccc(S(=O)(=O)Cl)cc1
COC(=O)c1cc(CCl)c(C)o1
null
null
ClCCl
Functional Group Interconversion
Alcohol to chloride_sulfonyl chloride
46eb49b1f728a0d336f2089cc941f1be7b941b4ddaef68327099a4e18f4b1c02
ebb4f73ae894ea29d308da9353b73dcd2a829947c5cd449c678fae1fc55ddffd
c1ccoc1
C-c1:c:c:c(-S(=O)(=O)-[Cl;H0;D1;+0:1]):c:c:1.O-[CH2;D2;+0:2]-[c:3]1:[c:4]:[c:5](-[C:6](-[#8:7])=[O;D1;H0:8]):[#8;a:9]:[c:10]:1-[C;D1;H3:11]>>[#8:7]-[C:6](=[O;D1;H0:8])-[c:5]1:[#8;a:9]:[c:10](-[C;D1;H3:11]):[c:3](-[CH2;D2;+0:2]-[Cl;H0;D1;+0:1]):[c:4]:1
33.8
[{"value": 33.8, "product": "COC(=O)C=1OC(=C(C1)CCl)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
15
MINUTE
Triethylamine (196 μl, 1.41 mmoles), followed by 4-methyl-benzenesulphonyl chloride (247 mg, 1.293 mmoles) were added to a stirred solution of 4-hydroxymethyl-5-methyl-furan-2-carboxylic acid methyl ester (16) (200 mg, 1.176 mmoles) in dry dichloromethane at 0° C. under an argon atmosphere. The reaction mixture was sti...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Primary alcohol.Sulfonyl halide
Primary halide
c1ccccc1
null
c1ccoc1
TsOH.HO-
ClCCl
0
0.25
COC(=O)c1cc(CO)c(C)o1.Cc1ccc(S(=O)(=O)Cl)cc1>ClCCl>COC(=O)c1cc(CCl)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-80ca010d9cf343f0a90c04484c6401ac
COC(=O)c1cc(CCl)c(C)o1.Nc1ccc(-c2ccccc2)cc1>>COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
[I-].[K+].C1(=CC=C(C=C1)N)C1=CC=CC=C1.COC(=O)C=1OC(=C(C1)CCl)C.C([O-])([O-])=O.[K+].[K+]>>COC(=O)C=1OC(=C(C1)CNC1=CC=C(C=C1)C1=CC=CC=C1)C
Cl[CH2:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:24][c:22]1[CH3:23].[NH2:9][c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[cH:20][cH:21]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][NH:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][cH:18][cH:19]3)[cH:20][cH:21]2)[c:...
COC(=O)c1cc(CCl)c(C)o1.Nc1ccc(-c2ccccc2)cc1
COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
N-alkylation of primary amines with alkyl halides
fc19a1445ff204e66e51735d0191465bda3c6691fd233624a54742c9d4828411
0b1d32f56ad00f1e5bdae9390f9227bbea012fa2f8203aac34726b8a6761cc7c
c1ccc(-c2ccc(NCc3ccoc3)cc2)cc1
Cl-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4](-[C:5](-[#8:6])=[O;D1;H0:7]):[#8;a:8]:[c:9]:1-[C;D1;H3:10].[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#8;a:8]:[c:9](-[C;D1;H3:10]):[c:2](-[CH2;D2;+0:1]-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:3]:1
71.1
[{"value": 71.1, "product": "COC(=O)C=1OC(=C(C1)CNC1=CC=C(C=C1)C1=CC=CC=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
Potassium iodide (32 mg) and a solution of biphenyl-4-ylamine (74 mg, 0.438 mmoles) in tetrahydrofuran (1 ml) was added to a mixture of 4-chloromethyl-5-methyl-furan-2-carboxylic acid methyl ester (159) (75 mg, 0.398 mmoles) and potassium carbonate (83 mg) in tetrahydrofuran (1 ml). The mixture was stirred at room temp...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary amine
Secondary amine
null
null
c1ccoc1.c1ccccc1.c1ccccc1
HCl
O1CCCC1
null
16
COC(=O)c1cc(CCl)c(C)o1.Nc1ccc(-c2ccccc2)cc1>O1CCCC1>COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ab09486afca74d20a134ba0fe5071a3c
COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1>>Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1
COC(=O)C=1OC(=C(C1)CNC1=CC=C(C=C1)C1=CC=CC=C1)C>>C1(=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O)C1=CC=CC=C1
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][NH:11][c:12]2[cH:13][cH:14][c:15](-[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[cH:22][cH:23]2)[cH:8]1)=[O:6]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][NH:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[cH:22][cH:23...
COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(NCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
40.2
[{"value": 40.2, "product": "C1(=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A solution of 4-(biphenyl-4-ylaminomethyl)-5-methyl-furan-2-carboxylic acid methyl ester (158) (91 mg, 0.283 mmoles) in dry tetrahydrofuran (5 ml) was treated with potassium trimethylsilanoate (182 mg, 1.42 mmoles) and the mixture stirred under an argon atmosphere for 3 hours. After evaporation of the solvent, the resi...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccoc1.c1ccccc1.c1ccccc1
Other
O1CCCC1
null
3
COC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1>O1CCCC1>Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1cc4c2ff67f945298a1bc699b95b927c
Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1.NS(=O)(=O)c1ccccc1>>Cc1oc(C(=O)NS(=O)(=O)c2ccccc2)cc1CNc1ccc(-c2ccccc2)cc1
C1(=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O)C1=CC=CC=C1.C1(=CC=CC=C1)S(=O)(=O)N.C(C)N(CC)CC.Cl.CN(CCCN=C=NCC)C>>C1(=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=CC=CC=C1)C1=CC=CC=C1
O[C:5]([c:4]1[o:3][c:2]([CH3:1])[c:18]([CH2:19][NH:20][c:21]2[cH:22][cH:23][c:24](-[c:25]3[cH:26][cH:27][cH:28][cH:29][cH:30]3)[cH:31][cH:32]2)[cH:17]1)=[O:6].[NH2:7][S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[NH:7][S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][...
Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1.NS(=O)(=O)c1ccccc1
Cc1oc(C(=O)NS(=O)(=O)c2ccccc2)cc1CNc1ccc(-c2ccccc2)cc1
null
CN(C)C1=CC=NC=C1
O1CCCC1.C(C)#N
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(CNc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:9]=[#16:8](=[O;D1;H0:10])(-[c:11])-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6]
49.8
[{"value": 49.8, "product": "C1(=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=CC=CC=C1)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
19
HOUR
A stirred solution of 4-(biphenyl-4-ylaminomethyl)-5-methyl-furan-2-carboxylic acid (160) (15 mg, 0.036 mmoles), benzenesulphonamide (17 mg, 0.107 mmoles) and 4-(N,N-dimethylamino)-pyridine (1 mg) in a mixture of tetrahydrofuran (3 ml) and acetonitrile (0.5 ml) was treated with triethylamine (5.5 μl, 0.039 mmoles) and ...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccoc1.c1ccccc1.c1ccccc1.c1ccccc1
HO-
CN(C)C1=CC=NC=C1.O1CCCC1.C(C)#N
null
19
Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1.NS(=O)(=O)c1ccccc1>CN(C)C1=CC=NC=C1.O1CCCC1.C(C)#N>Cc1oc(C(=O)NS(=O)(=O)c2ccccc2)cc1CNc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d1a83f1c9f9749bfadc7b099ff1d977e
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1>>Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
C1(=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O)C1=CC=CC=C1.CC1=C(C=CC=C1)S(=O)(=O)N>>C1(=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=C(C=CC=C1)C)C1=CC=CC=C1
[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:9])(=[O:10])[NH2:11].O[C:12](=[O:13])[c:14]1[cH:15][c:16]([CH2:17][NH:18][c:19]2[cH:20][cH:21][c:22](-[c:23]3[cH:24][cH:25][cH:26][cH:27][cH:28]3)[cH:29][cH:30]2)[c:31]([CH3:32])[o:33]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:9])(=[O:10])[NH:11][C:12](=...
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1
Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(CNc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:9]=[#16:8](=[O;D1;H0:10])(-[c:11])-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6]
null
[]
null
null
null
null
Compound (162) was prepared from compound (160) and 2-methyl-benzenesulphonamide by adapting the procedure of Example 38(f). LC/MS System D; Rt=10.39 mins, m/z (ES+)=461 (M+H for C26H24N2O4S). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.c1ccoc1.c1ccccc1.c1ccccc1
HO-
null
null
null
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccccc2)cc1>>Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccccc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e9597d101bd24d74a58afd7c9a04f7fb
COC(=O)c1cc(CNc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1>>COc1ccc(-c2ccc(NCc3cc(C(=O)O)oc3C)cc2)nc1
Cl.FC(C(=O)O)(F)F.COC(=O)C=1OC(=C(C1)CNC1=CC=C(C=C1)C1=NC=C(C=C1)OC)C>>Cl.COC=1C=CC(=NC1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O
C[O:18][C:16]([c:15]1[cH:14][c:13]([CH2:12][NH:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:25][n:24]3)[cH:23][cH:22]2)[c:20]([CH3:21])[o:19]1)=[O:17]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([NH:11][CH2:12][c:13]3[cH:14][c:15]([C:16](=[O:17])[OH:18])[o:19][c:20]3[CH3:21])...
COC(=O)c1cc(CNc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1
COc1ccc(-c2ccc(NCc3cc(C(=O)O)oc3C)cc2)nc1
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(NCc3ccoc3)cc2)nc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
16
HOUR
A solution of 4-{[4-(5-methoxy-pyridin-2-yl)-phenylamino]-methyl}-5-methyl-furan-2-carboxylic acid methyl ester trifluoroacetic acid salt (165) (38 mg, 0.082 mmoles) in tetrahydrofuran (4 ml) was treated with potassium trimethylsilanoate (63 mg, 0.049 mmoles) and the mixture stirred at room temperature for 16 hours. Th...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccncc1.c1ccccc1.c1ccoc1
Other
O1CCCC1
null
16
COC(=O)c1cc(CNc2ccc(-c3ccc(OC)cn3)cc2)c(C)o1>O1CCCC1>COc1ccc(-c2ccc(NCc3cc(C(=O)O)oc3C)cc2)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d1db7f0365564cd88479d02ef3124c02
COc1ccc(-c2ccc(NCc3cc(C(=O)O)oc3C)cc2)nc1.Cc1ccccc1S(N)(=O)=O>>COc1ccc(-c2ccc(NCc3cc(C(=O)NS(=O)(=O)c4ccccc4C)oc3C)cc2)nc1
C(C)N(CC)CC.C=1(C(=CC=CC1)S(=O)(=O)N)C.Cl.CN(CCCN=C=NCC)C.Cl.COC=1C=CC(=NC1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O>>COC=1C=CC(=NC1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=C(C=CC=C1)C
O[C:16]([c:15]1[cH:14][c:13]([CH2:12][NH:11][c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:35][n:34]3)[cH:33][cH:32]2)[c:30]([CH3:31])[o:29]1)=[O:17].[NH2:18][S:19](=[O:20])(=[O:21])[c:22]1[cH:23][cH:24][cH:25][cH:26][c:27]1[CH3:28]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([NH:...
COc1ccc(-c2ccc(NCc3cc(C(=O)O)oc3C)cc2)nc1.Cc1ccccc1S(N)(=O)=O
COc1ccc(-c2ccc(NCc3cc(C(=O)NS(=O)(=O)c4ccccc4C)oc3C)cc2)nc1
null
CN(C)C1=CC=NC=C1
O1CCCC1
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(CNc2ccc(-c3ccccn3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[c:3](:[c:4]):[#8;a:5]:[c:6]
2.8
[{"value": 2.8, "product": "COC=1C=CC(=NC1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=C(C=CC=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
A suspension of 4-{[4-(5-methoxy-pyridin-2-yl)-phenylamino]-methyl}-5-methyl-furan-2-carboxylic acid hydrochloride salt (166) (30 mg, 0.08 mmoles) in tetrahydrofuran (5 ml) was treated with toluene-2-sulphonamide (41 mg, 0.24 mmoles), 1-(3-dimethylaminopropyl)-3-ethylcarbodiimide hydrochloride (34 mg, 0.176 mmoles) and...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccncc1.c1ccccc1.c1ccoc1.c1ccccc1
HO-
CN(C)C1=CC=NC=C1.O1CCCC1
null
16
COc1ccc(-c2ccc(NCc3cc(C(=O)O)oc3C)cc2)nc1.Cc1ccccc1S(N)(=O)=O>CN(C)C1=CC=NC=C1.O1CCCC1>COc1ccc(-c2ccc(NCc3cc(C(=O)NS(=O)(=O)c4ccccc4C)oc3C)cc2)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ccf9008942794e5aa78e6b6850432f5b
COC(=O)c1cc(CCl)c(C)o1.Nc1ccc(-c2ccc(OC(F)F)cc2)cc1>>COC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
COC(=O)C=1OC(=C(C1)CCl)C.FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)N)F>>COC(=O)C=1OC(=C(C1)CNC1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C
Cl[CH2:8][c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[o:28][c:26]1[CH3:27].[NH2:9][c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][c:17]([O:18][CH:19]([F:20])[F:21])[cH:22][cH:23]2)[cH:24][cH:25]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][NH:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][c:17]([O:18][...
COC(=O)c1cc(CCl)c(C)o1.Nc1ccc(-c2ccc(OC(F)F)cc2)cc1
COC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
null
null
C(C)#N
Heteroatom Alkylation and Arylation
N-alkylation of primary amines with alkyl halides
fc19a1445ff204e66e51735d0191465bda3c6691fd233624a54742c9d4828411
0b1d32f56ad00f1e5bdae9390f9227bbea012fa2f8203aac34726b8a6761cc7c
c1ccc(-c2ccc(NCc3ccoc3)cc2)cc1
Cl-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4](-[C:5](-[#8:6])=[O;D1;H0:7]):[#8;a:8]:[c:9]:1-[C;D1;H3:10].[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#8;a:8]:[c:9](-[C;D1;H3:10]):[c:2](-[CH2;D2;+0:1]-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:3]:1
null
[]
null
null
null
null
Compound (170) was prepared from compounds (159) and (169) by adapting the procedure of Example 38(d). (420 mg). LC/MS System A; Rt=4.00 mins, m/z (ES+)=388 (M+H) and 429 (M+H acetonitrile adduct) for C21H19F2NO3. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary amine
Secondary amine
null
null
c1ccoc1.c1ccccc1.c1ccccc1
HCl
C(C)#N
null
null
COC(=O)c1cc(CCl)c(C)o1.Nc1ccc(-c2ccc(OC(F)F)cc2)cc1>C(C)#N>COC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ce63af510995437e92187b6693f28e47
Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1.NS(=O)(=O)c1ccccc1>>Cc1oc(C(=O)NS(=O)(=O)c2ccccc2)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1
FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O)F.C1(=CC=CC=C1)S(=O)(=O)N>>FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=CC=CC=C1)F
O[C:5]([c:4]1[o:3][c:2]([CH3:1])[c:18]([CH2:19][NH:20][c:21]2[cH:22][cH:23][c:24](-[c:25]3[cH:26][cH:27][c:28]([O:29][CH:30]([F:31])[F:32])[cH:33][cH:34]3)[cH:35][cH:36]2)[cH:17]1)=[O:6].[NH2:7][S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[NH:7][S:8](=[O:9])(=[...
Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1.NS(=O)(=O)c1ccccc1
Cc1oc(C(=O)NS(=O)(=O)c2ccccc2)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(CNc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:9]=[#16:8](=[O;D1;H0:10])(-[c:11])-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6]
null
[]
null
null
null
null
Compound (172) was prepared from compound (171) and benzenesulphonamide by adapting the procedure of Example 38(f). LC/MS System D; Rt=10.38 mins, m/z (ES+)=513 (M+H for C26H22F2N2O5S). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccoc1.c1ccccc1.c1ccccc1.c1ccccc1
HO-
null
null
null
Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1.NS(=O)(=O)c1ccccc1>>Cc1oc(C(=O)NS(=O)(=O)c2ccccc2)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5258ab6b08134b9dac12a009777659f1
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1>>Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O)F.CC1=C(C=CC=C1)S(=O)(=O)N>>FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C1=C(C=CC=C1)C)F
[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:9])(=[O:10])[NH2:11].O[C:12](=[O:13])[c:14]1[cH:15][c:16]([CH2:17][NH:18][c:19]2[cH:20][cH:21][c:22](-[c:23]3[cH:24][cH:25][c:26]([O:27][CH:28]([F:29])[F:30])[cH:31][cH:32]3)[cH:33][cH:34]2)[c:35]([CH3:36])[o:37]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O...
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1
Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1ccccc1)c1cc(CNc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[O;D1;H0:9]=[#16:8](=[O;D1;H0:10])(-[c:11])-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6]
null
[]
null
null
null
null
Compound (173) was prepared from compound (171) and 2-methyl-benzenesulphonamide by adapting the procedure of Example 38(f). LC/MS System D; Rt=10.63 mins, m/z (ES+)=527 (M+H for C27H24F2N2O5S). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.c1ccoc1.c1ccccc1.c1ccccc1
HO-
null
null
null
Cc1ccccc1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1>>Cc1ccccc1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f252a2fcd224468bbd28488e1f44e8fc
Cc1noc(C)c1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1>>Cc1noc(C)c1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
F[P-](F)(F)(F)(F)F.N1(N=NC2=C1N=CC=C2)OC(=[N+](C)C)N(C)C.C(C)(C)N(CC)C(C)C.FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)O)F.CC1=NOC(=C1S(=O)(=O)N)C>>FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C=1C(=NOC1C)C)F
[CH3:1][c:2]1[n:3][o:4][c:5]([CH3:6])[c:7]1[S:8](=[O:9])(=[O:10])[NH2:11].O[C:12](=[O:13])[c:14]1[cH:15][c:16]([CH2:17][NH:18][c:19]2[cH:20][cH:21][c:22](-[c:23]3[cH:24][cH:25][c:26]([O:27][CH:28]([F:29])[F:30])[cH:31][cH:32]3)[cH:33][cH:34]2)[c:35]([CH3:36])[o:37]1>>[CH3:1][c:2]1[n:3][o:4][c:5]([CH3:6])[c:7]1[S:8](=[O...
Cc1noc(C)c1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1
Cc1noc(C)c1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
null
null
CN(C=O)C
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1cnoc1)c1cc(CNc2ccc(-c3ccccc3)cc2)co1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]1:[c:12]:[#7;a:13]:[#8;a:14]:[c:15]:1>>[O;D1;H0:9]=[#16:8](=[O;D1;H0:10])(-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6])-[c:11]1:[c:12]:[#7;a:13]:[#8;a:14]:[c:15]:1
3.7
[{"value": 3.7, "product": "FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)NCC=1C=C(OC1C)C(=O)NS(=O)(=O)C=1C(=NOC1C)C)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
Diisopropylethylamine (60 μl, 0.339 mmoles) and a solution of 4-(4′-difluoromethoxy-biphenyl-4-ylaminomethyl)-5-methyl-furan-2-carboxylic acid (171) (50 mg, 0.103 mmoles) in N,N-dimethylformamide (1.0 ml) were added to a stirred solution of 3,5-dimethyl-isoxazole-4-sulphonic acid amide (55 mg, 0.308 mmoles) in N,N-dime...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1cnoc1.c1ccoc1.c1ccccc1.c1ccccc1
HO-
CN(C=O)C
null
16
Cc1noc(C)c1S(N)(=O)=O.Cc1oc(C(=O)O)cc1CNc1ccc(-c2ccc(OC(F)F)cc2)cc1>CN(C=O)C>Cc1noc(C)c1S(=O)(=O)NC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2e3d54351f6e4043af52017d3c0c5e4d
CI.COC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1>>COC(=O)c1cc(CN(C)c2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
IC.C([O-])([O-])=O.[K+].[K+].COC(=O)C=1OC(=C(C1)CNC1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C>>COC(=O)C=1OC(=C(C1)CN(C)C1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C
I[CH3:10].[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][NH:9][c:11]2[cH:12][cH:13][c:14](-[c:15]3[cH:16][cH:17][c:18]([O:19][CH:20]([F:21])[F:22])[cH:23][cH:24]3)[cH:25][cH:26]2)[c:27]([CH3:28])[o:29]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([CH2:8][N:9]([CH3:10])[c:11]2[cH:12][cH:13][c:14](-[c:15]3[cH:16][cH:...
CI.COC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
COC(=O)c1cc(CN(C)c2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
e1587a52a1bca6a80c6048d43276d8bccf8d3e94e692e6b210e5fd3b22494187
7cc25fba33369069673bac5bd8fc404dc064da8d6c8cf4a77f21f4df0a617fe3
c1ccc(-c2ccc(NCc3ccoc3)cc2)cc1
I-[CH3;D1;+0:1].[#8;a:2]:[c:3]:[c:4]-[C:5]-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]>>[#8;a:2]:[c:3]:[c:4]-[C:5]-[N;H0;D3;+0:6](-[CH3;D1;+0:1])-[c:7](:[c:8]):[c:9]
63.8
[{"value": 63.8, "product": "COC(=O)C=1OC(=C(C1)CN(C)C1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
36
HOUR
Iodomethane (91 mg, 0.64 mmoles) and potassium carbonate (88 mg, 0.64 mmoles) were added to a solution of 4-(4′-difluoromethoxy-biphenyl-4-ylaminomethyl)-5-methyl-furan-2-carboxylic acid methyl ester (170) (62 mg, 0.16 mmoles) in N,N-dimethylformamide (10 ml) and the mixture stirred at room temperature for 36 hours und...
10.6084/m9.figshare.5104873.v1
null
Secondary amine
Tertiary amine
null
null
c1ccoc1.c1ccccc1.c1ccccc1
HI
CN(C=O)C
null
36
CI.COC(=O)c1cc(CNc2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1>CN(C=O)C>COC(=O)c1cc(CN(C)c2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1f696ea19d0d449caca1cf27cb196449
COC(=O)c1cc(CN(C)c2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1>>Cc1oc(C(=O)O)cc1CN(C)c1ccc(-c2ccc(OC(F)F)cc2)cc1
FC(C(=O)O)(F)F.COC(=O)C=1OC(=C(C1)CN(C)C1=CC=C(C=C1)C1=CC=C(C=C1)OC(F)F)C>>FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)N(C)CC=1C=C(OC1C)C(=O)O)F
C[O:7][C:5]([c:4]1[o:3][c:2]([CH3:1])[c:9]([CH2:10][N:11]([CH3:12])[c:13]2[cH:14][cH:15][c:16](-[c:17]3[cH:18][cH:19][c:20]([O:21][CH:22]([F:23])[F:24])[cH:25][cH:26]3)[cH:27][cH:28]2)[cH:8]1)=[O:6]>>[CH3:1][c:2]1[o:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][c:9]1[CH2:10][N:11]([CH3:12])[c:13]1[cH:14][cH:15][c:16](-[c:17]2[cH:...
COC(=O)c1cc(CN(C)c2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1
Cc1oc(C(=O)O)cc1CN(C)c1ccc(-c2ccc(OC(F)F)cc2)cc1
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(NCc3ccoc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
17.7
[{"value": 17.7, "product": "FC(OC1=CC=C(C=C1)C1=CC=C(C=C1)N(C)CC=1C=C(OC1C)C(=O)O)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
HOUR
A solution of 4-{[(4′-difluoromethoxy-biphenyl-4-yl)-methyl-amino]-methyl}-5-methyl-furan-2-carboxylic acid methyl ester (175) (30 mg, 0.07 mmoles) in dry tetrahydrofuran (20 ml) was treated with potassium trimethylsilanoate (19 mg, 0.15 mmoles) and the mixture stirred under an argon atmosphere for 30 hours. Trifluoroa...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccoc1.c1ccccc1.c1ccccc1
Other
O1CCCC1
null
30
COC(=O)c1cc(CN(C)c2ccc(-c3ccc(OC(F)F)cc3)cc2)c(C)o1>O1CCCC1>Cc1oc(C(=O)O)cc1CN(C)c1ccc(-c2ccc(OC(F)F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-281f019ab44e493bac9d647da6402ad8
CC(C)=CCC/C(C)=C/C(=O)O.N[C@H]1C(O)O[C@H](CO)[C@H](O)[C@@H]1O>>CC(C)=CCC/C(C)=C/C(=O)NC1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O
C(\C=C(/C)\CCC=C(C)C)(=O)O.C(C)N(CC)CC.Cl.OC1[C@H](N)[C@@H](O)[C@@H](O)[C@H](O1)CO.ClC(=O)OCC(C)C>>C1([C@H](O)[C@@H](O)[C@@H](O)[C@H](O1)CO)NC(\C=C(/C)\CCC=C(C)C)=O
O[C:10](/[CH:9]=[C:7](/[CH2:6][CH2:5][CH:4]=[C:2]([CH3:1])[CH3:3])[CH3:8])=[O:11].[NH2:12][C@H:22]1[CH:13]([OH:23])[O:14][C@H:15]([CH2:16][OH:17])[C@H:18]([OH:19])[C@@H:20]1[OH:21]>>[CH3:1][C:2]([CH3:3])=[CH:4][CH2:5][CH2:6]/[C:7]([CH3:8])=[CH:9]/[C:10](=[O:11])[NH:12][CH:13]1[O:14][C@H:15]([CH2:16][OH:17])[C@H:18]([OH...
CC(C)=CCC/C(C)=C/C(=O)O.N[C@H]1C(O)O[C@H](CO)[C@H](O)[C@@H]1O
CC(C)=CCC/C(C)=C/C(=O)NC1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O
null
null
O.CC(=O)C.[OH-].[Na+].C1CCOC1
Acylation
OtherReaction
2a67fc59999fd518505897134e5e714168f09ef3b0471e4d1831375d1302921f
ef5d2f42d27e953f00e3f1ba0755384ec25f145a166ad3265dce19707549d74a
C1CCOCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])/[C:3]=[C:4](\[C;D1;H3:5])-[C:6]-[C:7]-[C:8]=[C:9].[NH2;D1;+0:10]-[C@@H;D3;+0:11]1-[C:12](-[O;D1;H1:13])-[C:14]-[C:15]-[#8:16]-[CH;D3;+0:17]-1-[OH;D1;+0:18]>>[C:9]=[C:8]-[C:7]-[C:6]/[C:4](-[C;D1;H3:5])=[C:3]/[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:10]-[CH;D3;+0:17]1-[#8:16]-[C:15]-[C:14]-[C...
46
[{"value": 46.0, "product": "C1([C@H](O)[C@@H](O)[C@@H](O)[C@H](O1)CO)NC(\\C=C(/C)\\CCC=C(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 45.8, "product": "C1([C@H](O)[C@@H](O)[C@@H](O)[C@H](O1)CO)NC(\\C=C(/C)\\CCC=C(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
To a THF (20 ml) solution containing geranic acid (0.84 g, 5 mmols), triethylamine (0.51 g, 5 mmols) was added and cooled to 0° C., into which a THF (5 ml) solution containing isobutyl chloroformate (0.68 g, 5 mmols) was added dropwise, followed by 30 minutes' stirring at 0° C. Then galactosamine hydrochloride (1.08 g,...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ether.Secondary alcohol.Primary amine
Ether.Secondary amide.Secondary alcohol
C1CCOCC1
C1CCOCC1
C1CCOCC1
HO-
O.CC(=O)C.[OH-].[Na+].C1CCOC1
0
0.5
CC(C)=CCC/C(C)=C/C(=O)O.N[C@H]1C(O)O[C@H](CO)[C@H](O)[C@@H]1O>O.CC(=O)C.[OH-].[Na+].C1CCOC1>CC(C)=CCC/C(C)=C/C(=O)NC1O[C@H](CO)[C@H](O)[C@H](O)[C@H]1O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d5316dfe55c3453a90a3327d5fe4fda0
CC(C)=CCC/C(C)=C/CN.CC(C)COC(=O)Cl.CCN(CC)CC.O=C(O)/C=C/C(=O)O>>CC(C)=CCC/C(C)=C/CNC(=O)/C=C/C(=O)NC/C=C(\C)CCC=C(C)C
C(\C=C\C(=O)O)(=O)O.C(C)N(CC)CC.C(\C=C(/C)\CCC=C(C)C)N.ClC(=O)OCC(C)C>>C(\C=C(/C)\CCC=C(C)C)NC(\C=C\C(=O)NC\C=C(/C)\CCC=C(C)C)=O
[CH3:1][C:2](=[CH:4][CH2:5][CH2:6]/[C:7]([CH3:8])=[CH:9]/[CH2:10][NH2:11])[CH3:28].Cl[C:12](O[CH2:25][CH:26]([CH3:3])[CH3:27])=[O:13].C[CH2:16][N:18]([CH2:19][CH3:20])[CH2:22][CH3:24].O=[C:21](O)/[CH:23]=[CH:15]/[C:14](O)=[O:17]>>[CH3:1][C:2]([CH3:3])=[CH:4][CH2:5][CH2:6]/[C:7]([CH3:8])=[CH:9]/[CH2:10][NH:11][C:12](=[O...
CC(C)=CCC/C(C)=C/CN.CC(C)COC(=O)Cl.CCN(CC)CC.O=C(O)/C=C/C(=O)O
CC(C)=CCC/C(C)=C/CNC(=O)/C=C/C(=O)NC/C=C(\C)CCC=C(C)C
null
null
O1CCCC1.O
C-C Coupling
OtherReaction
bc8288f693b3f5e1f83ea0c7d2621a7bdbc8ff31868257930c3cf41a0e293c05
9b04b435d4909f27aba13de39436efd4f6dbf84886a2b40e0be7f7a8729de693
null
C-[CH2;D2;+0:1]-[N;H0;D3;+0:2](-[C:3]-[CH3;D1;+0:4])-[CH2;D2;+0:5]-[CH3;D1;+0:6].Cl-[C;H0;D3;+0:7](=[O;D1;H0:8])-O-[CH2;D2;+0:9]-[CH;D3;+0:10](-[C;D1;H3:11])-[CH3;D1;+0:12].O-[C;H0;D3;+0:13](=[O;H0;D1;+0:14])/[CH;D2;+0:15]=[CH;D2;+0:16]/[C;H0;D3;+0:17](-O)=O.[C;D1;H3:18]-[C;H0;D3;+0:19](-[CH3;D1;+0:20])=[C:21]-[C:22]-[...
110.7
[{"value": 55.0, "product": "C(\\C=C(/C)\\CCC=C(C)C)NC(\\C=C\\C(=O)NC\\C=C(/C)\\CCC=C(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 110.7, "product": "C(\\C=C(/C)\\CCC=C(C)C)NC(\\C=C\\C(=O)NC\\C=C(/C)\\CCC=C(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
To a tetrahydrofuran (THF) (20 ml) solution containing fumaric acid (0.58 g, 5 mmols), triethylamine (1.01 g, 10 mmols) was added and the solution was cooled to 0° C., into which a THF (5 ml) solution containing isobutyl chloroformate (1.53 g, 10 mmols) was added dropwise. As the addition was continued, white precipita...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Carboxylic acid.Carboxylic acid.Ether.Primary amine.Tertiary amine
Secondary amide.Secondary amide
null
null
null
HCl
O1CCCC1.O
0
0.5
CC(C)=CCC/C(C)=C/CN.CC(C)COC(=O)Cl.CCN(CC)CC.O=C(O)/C=C/C(=O)O>O1CCCC1.O>CC(C)=CCC/C(C)=C/CNC(=O)/C=C/C(=O)NC/C=C(\C)CCC=C(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8a95bc2602d14bacb8ec28deb740f57f
CC(C)=CCC/C(C)=C/C(=O)O.N[C@@H](CS)C(=O)O>>CC(C)=CCC/C(C)=C/C(=O)N[C@@H](CS)C(=O)O
C(\C=C(/C)\CCC=C(C)C)(=O)O.C(C)N(CC)CC.ClC(=O)OCC(C)C.N[C@@H](CS)C(=O)O.Cl>>C(\C=C(/C)\CCC=C(C)C)(=O)N[C@@H](CS)C(=O)O
O[C:10](/[CH:9]=[C:7](/[CH2:6][CH2:5][CH:4]=[C:2]([CH3:1])[CH3:3])[CH3:8])=[O:11].[NH2:12][C@@H:13]([CH2:14][SH:15])[C:16](=[O:17])[OH:18]>>[CH3:1][C:2]([CH3:3])=[CH:4][CH2:5][CH2:6]/[C:7]([CH3:8])=[CH:9]/[C:10](=[O:11])[NH:12][C@@H:13]([CH2:14][SH:15])[C:16](=[O:17])[OH:18]
CC(C)=CCC/C(C)=C/C(=O)O.N[C@@H](CS)C(=O)O
CC(C)=CCC/C(C)=C/C(=O)N[C@@H](CS)C(=O)O
null
null
[OH-].[Na+].C1CCOC1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
null
O-[C;H0;D3;+0:1](=[O;D1;H0:2])/[C:3]=[C:4](\[C;D1;H3:5])-[C:6]-[C:7]-[C:8]=[C:9].[C:10]-[C:11](-[NH2;D1;+0:12])-[C:13](=[O;D1;H0:14])-[O;D1;H1:15]>>[C:10]-[C:11](-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])/[C:3]=[C:4](\[C;D1;H3:5])-[C:6]-[C:7]-[C:8]=[C:9])-[C:13](=[O;D1;H0:14])-[O;D1;H1:15]
20.5
[{"value": 19.5, "product": "C(\\C=C(/C)\\CCC=C(C)C)(=O)N[C@@H](CS)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 20.5, "product": "C(\\C=C(/C)\\CCC=C(C)C)(=O)N[C@@H](CS)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
To a THF (20 ml) solution containing geranic acid (1.68 g, 10 mmols), triethylamine (1.01 g, 10 mmols) was added and cooled to 0° C., into which a THF (5 ml) solution of isobutyl chloroformate (1.37 g, 10 mmols) was added dropwise, followed by 30 minutes' stirring at 0° C. To the reaction mixture a solution of cysteine...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
null
HO-
[OH-].[Na+].C1CCOC1
0
0.5
CC(C)=CCC/C(C)=C/C(=O)O.N[C@@H](CS)C(=O)O>[OH-].[Na+].C1CCOC1>CC(C)=CCC/C(C)=C/C(=O)N[C@@H](CS)C(=O)O