dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f7118650aa1c49b4a2a7fb581c794a93
O.O=S(Cl)Cl.c1ccc2c(c1)CCO2>>O=S(=O)(Cl)c1ccc2c(c1)CCO2
S(=O)(Cl)Cl.O1CCC2=C1C=CC=C2.C(Cl)Cl.O>>O1CCC2=C1C=CC(=C2)S(=O)(=O)Cl
[OH2:3].Cl[S:2](=[O:1])[Cl:4].[cH:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH2:11][CH2:12][O:13]2>>[O:1]=[S:2](=[O:3])([Cl:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH2:11][CH2:12][O:13]2
O.O=S(Cl)Cl.c1ccc2c(c1)CCO2
O=S(=O)(Cl)c1ccc2c(c1)CCO2
null
null
ClCCCl
Oxidation
OtherReaction
8b01ac9c5d7b697f016d7042f2d05a3b46d0d06f578fe0c90c8043196b5281a6
81690bf6214dfc87f1e80e37dd7a1b86738358b56ee49d58ce8b77a9699c92f8
c1ccc2c(c1)CCO2
Cl-[S;H0;D3;+0:1](-[Cl;D1;H0:2])=[O;D1;H0:3].[OH2;D0;+0:4].[c:5]:[c:6]:[cH;D2;+0:7]:[c:8]:[c:9]>>[Cl;D1;H0:2]-[S;H0;D4;+0:1](=[O;D1;H0:3])(=[O;H0;D1;+0:4])-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:6]:[c:5]
100
[{"value": 100.0, "product": "O1CCC2=C1C=CC(=C2)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}]
85
CELSIUS
null
null
3.56 g (29.6 mmol) 2,3-dihydrobenzofuran was added to a slurry of 5.44 g (35.5 mmol) sulfur trioxide-N,N-dimethylformamide complex in 12 mL 1,2-dichloroethane under argon. The reaction was heated to 85° C. for 1 hour and then cooled to room temperature. Thionyl chloride (2.6 mL, 35.5 mmol, 1.2 eq) was added dropwise an...
10.6084/m9.figshare.5104873.v1
null
null
Sulfonyl halide
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
HCl
ClCCCl
85
null
O.O=S(Cl)Cl.c1ccc2c(c1)CCO2>ClCCCl>O=S(=O)(Cl)c1ccc2c(c1)CCO2
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2c29efc0e55344048d0fc25f38879fed
BrCc1noc2ccccc12.O=S(=O)(O)Cl>>O=S(=O)(Cl)c1ccc2onc(CBr)c2c1
ClS(=O)(=O)O.BrCC1=NOC2=C1C=CC=C2>>BrCC1=NOC2=C1C=C(C=C2)S(=O)(=O)Cl
[cH:5]1[cH:6][cH:7][c:8]2[o:9][n:10][c:11]([CH2:12][Br:13])[c:14]2[cH:15]1.O[S:2](=[O:1])(=[O:3])[Cl:4]>>[O:1]=[S:2](=[O:3])([Cl:4])[c:5]1[cH:6][cH:7][c:8]2[o:9][n:10][c:11]([CH2:12][Br:13])[c:14]2[cH:15]1
BrCc1noc2ccccc12.O=S(=O)(O)Cl
O=S(=O)(Cl)c1ccc2onc(CBr)c2c1
null
null
null
Heteroatom Alkylation and Arylation
Aromatic sulfonyl chlorination
1de617f597940a4b1353fa427b486b905916e0273772c5a5239bad72a4ce2f2a
d32b60b8f9bfd187c6c9f1eef6a22a00f53525a7532b83aba763d5389c9e4280
c1ccc2oncc2c1
O-[S;H0;D4;+0:1](-[Cl;D1;H0:2])(=[O;D1;H0:3])=[O;D1;H0:4].[#7;a:5]1:[#8;a:6]:[c:7]2:[c:8]:[c:9]:[cH;D2;+0:10]:[c:11]:[c:12]:2:[c:13]:1>>[Cl;D1;H0:2]-[S;H0;D4;+0:1](=[O;D1;H0:3])(=[O;D1;H0:4])-[c;H0;D3;+0:10]1:[c:11]:[c:12]2:[c:13]:[#7;a:5]:[#8;a:6]:[c:7]:2:[c:8]:[c:9]:1
80.2
[{"value": 80.0, "product": "BrCC1=NOC2=C1C=C(C=C2)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.2, "product": "BrCC1=NOC2=C1C=C(C=C2)S(=O)(=O)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
6
HOUR
Chlorosulfonic acid (1.5 ml, 22 mmol) was slowly added to 3-Bromomethyl-benzo[d]isoxazole (1.0 g, 4.7 mmol) at RT under argon. The reaction was heated at 90° C. for 12 h and then left at RT for 6 h. The resulting viscous oil was quenched over ice, extracted with EtOAc, dried over MgSO4 and concentrated in vacuo to a br...
10.6084/m9.figshare.5104873.v1
null
null
Sulfonyl halide
c1ccc2oncc2c1
c1ccc2oncc2c1
c1ccc2oncc2c1
HO-
null
90
6
BrCc1noc2ccccc12.O=S(=O)(O)Cl>>O=S(=O)(Cl)c1ccc2onc(CBr)c2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bb936bcf86b84c1b9b86441df70ddda7
CC(=O)OC(C)=O.Cc1n[nH]c2ccccc12>>CC(=O)n1nc(C)c2ccccc21
CC1=NNC2=CC=CC=C12.N1=CC=CC=C1.CC(=O)OC(=O)C>>CC1=NN(C2=CC=CC=C12)C(C)=O
CC(=O)O[C:2]([CH3:1])=[O:3].[nH:4]1[n:5][c:6]([CH3:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12>>[CH3:1][C:2](=[O:3])[n:4]1[n:5][c:6]([CH3:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12
CC(=O)OC(C)=O.Cc1n[nH]c2ccccc12
CC(=O)n1nc(C)c2ccccc21
null
CN(C)C=1C=CN=CC1
C1CCOC1
Acylation
Ester with secondary amine to amide
d2d8e67de66decf6e048f203acc2705e43acc0e3e98f0fe3c6249b66ad1e328e
93289da630dbaf2d9339c4212dcd342dfbcc29df4e79a63418a0fd9f589abdc1
c1ccc2[nH]ncc2c1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[c:4]:[c:5]1:[c:6]:[c:7]:[#7;a:8]:[nH;D2;+0:9]:1>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[n;H0;D3;+0:9]1:[#7;a:8]:[c:7]:[c:6]:[c:5]:1:[c:4]
91
[{"value": 91.0, "product": "CC1=NN(C2=CC=CC=C12)C(C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.6, "product": "CC1=NN(C2=CC=CC=C12)C(C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
3-Methylindazole (1.00 g, 7.6 mmol) (J. Med. Chem. 2706 (1997)] was dissolved in 10 ml THF and stirred at room temperature under a blanket of argon. Pyridine (0.64 ml, 7.9 mmol) was added, followed by Ac2O (0.79 ml, 8.3 mmol) and catalytic DMAP (90 mg, 0.7 mmol). The reaction proceeded for 2 h and was then partitioned ...
10.6084/m9.figshare.5104873.v1
null
Anhydride
null
c1ccc2[nH]ncc2c1
c1n[nH]c2ccccc12
c1n[nH]c2ccccc12
HO-
CN(C)C=1C=CN=CC1.C1CCOC1
null
2
CC(=O)OC(C)=O.Cc1n[nH]c2ccccc12>CN(C)C=1C=CN=CC1.C1CCOC1>CC(=O)n1nc(C)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-53d1f816a897459a8db0121cd6ac7f8e
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC(C)(C)C)C(=O)OCc1ccccc1.O=C(OC1COC2OCCC12)ON1C(=O)CCC1=O>>CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)C(=O)OCc1ccccc1
C(C1=CC=CC=C1)OC(N(CC(C)C)CC(C(CC1=CC=CC=C1)NC(=O)OC(C)(C)C)O)=O.Cl.C(C)(C)N(C(C)C)CC.O1CC(C2C1OCC2)OC(ON2C(CCC2=O)=O)=O>>C(C1=CC=CC=C1)OC(N(CC(C)C)CC(C(CC1=CC=CC=C1)NC(=O)OC1COC2OCCC21)O)=O
CC(C)(C)OC(=O)[NH:17][CH:9]([CH:7]([CH2:6][N:5]([CH2:4][CH:2]([CH3:1])[CH3:3])[C:29](=[O:30])[O:31][CH2:32][c:33]1[cH:34][cH:35][cH:36][cH:37][cH:38]1)[OH:8])[CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1.O=C1CCC(=O)N1O[C:18](=[O:19])[O:20][CH:21]1[CH2:22][O:23][CH:24]2[O:25][CH2:26][CH2:27][CH:28]12>>[CH3:1][CH:2...
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC(C)(C)C)C(=O)OCc1ccccc1.O=C(OC1COC2OCCC12)ON1C(=O)CCC1=O
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)C(=O)OCc1ccccc1
null
null
O1CCOCC1
Protection
OtherReaction
1128a7ed8198894bb78897e6f497896066e6c904d8c783a7606c5f801ae7721e
c6b87d20dd468a6b1a3f862a783b52d5f603286c2fec0192cc836668a76ce046
O=C(NCCC(Cc1ccccc1)NC(=O)OC1COC2OCCC12)OCc1ccccc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4].O=C1-C-C-C(=O)-N-1-O-[C;H0;D3;+0:5](=[O;D1;H0:6])-[#8:7]-[C:8]>>[C:3]-[C:2](-[C:4])-[NH;D2;+0:1]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[#8:7]-[C:8]
73.4
[{"value": 73.0, "product": "C(C1=CC=CC=C1)OC(N(CC(C)C)CC(C(CC1=CC=CC=C1)NC(=O)OC1COC2OCCC21)O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.4, "product": "C(C1=CC=CC=C1)OC(N(CC(C)C)CC(C(CC1=CC=CC=C1)NC(=O)OC1COC2OCCC21)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
(3-tert-Butoxycarbonylamino-2-hydroxy-4-phenyl-butyl)-isobutyl-carbamic acid benzyl ester 16 (7.54 g, 15 mmol) and 35 ml of 4M HCl in dioxane were stirred 30 min under an argon atmosphere. The mixture was concentrated in vacuo, and co-evaporated twice with dichloromethane. The residue was dissolved in dichloromethane (...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Ether.Tertiary amide.Tertiary amide.Boc
Carbamic ester
C1CCNC1
null
c1ccccc1.C1CC2CCOC2O1.c1ccccc1
HO-
O1CCOCC1
null
8
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC(C)(C)C)C(=O)OCc1ccccc1.O=C(OC1COC2OCCC12)ON1C(=O)CCC1=O>O1CCOCC1>CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)C(=O)OCc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-da7c1d34ef7f4336bbb01a45cf299d6f
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)C(=O)OCc1ccccc1>>CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12
C(C1=CC=CC=C1)OC(N(CC(C)C)CC(C(CC1=CC=CC=C1)NC(=O)OC1COC2OCCC21)O)=O>>O1CC(C2C1OCC2)OC(NC(C(CNCC(C)C)O)CC2=CC=CC=C2)=O
O=C(OCc1ccccc1)[N:5]([CH2:4][CH:2]([CH3:1])[CH3:3])[CH2:6][CH:7]([OH:8])[CH:9]([CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)[NH:17][C:18](=[O:19])[O:20][CH:21]1[CH2:22][O:23][CH:24]2[O:25][CH2:26][CH2:27][CH:28]12>>[CH3:1][CH:2]([CH3:3])[CH2:4][NH:5][CH2:6][CH:7]([OH:8])[CH:9]([CH2:10][c:11]1[cH:12][cH:13][cH:14...
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)C(=O)OCc1ccccc1
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12
null
[Pd]
C(C)O
Reduction
Hydrogenolysis of tertiary amines
709a03512f2b36af470a6c002bf594696c9a8d9f4ff0ae82dddda03c8a91a358
20c36f41eeb07c3ba4437b51ba72e8ff3c22d0b27e7197b0e9af3127f331149f
O=C(NCCc1ccccc1)OC1COC2OCCC12
O=C(-O-C-c1:c:c:c:c:c:1)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5]
98
[{"value": 97.0, "product": "O1CC(C2C1OCC2)OC(NC(C(CNCC(C)C)O)CC2=CC=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.0, "product": "O1CC(C2C1OCC2)OC(NC(C(CNCC(C)C)O)CC2=CC=CC=C2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A mixture of [3-(hexahydro-furo[2,3-b]furan-3-yloxycarbonylamino)-2-hydroxy-4-phenyl-butyl]-isobutyl-carbamic acid benzyl ester 18 (5.5 g, 10.4 mmol) and 550 mg of 10% Pd/C in 130 ml of ethanol was stirred under a hydrogen atmosphere overnight. The catalyst was removed by filtration through Celite®, and the solution wa...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Secondary amine
c1ccccc1
null
c1ccccc1.C1CC2CCOC2O1
HO-
[Pd].C(C)O
null
8
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)C(=O)OCc1ccccc1>[Pd].C(C)O>CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-908a968d90344375b8c2b6508cbc7955
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12.O=S(=O)(Cl)c1ccc2occc2c1>>CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occc2c1
O1C=CC2=C1C=CC(=C2)S(=O)(=O)Cl.O1CC(C2C1OCC2)OC(NC(C(CNCC(C)C)O)CC2=CC=CC=C2)=O.C(=O)(O)[O-].[Na+]>>O1CC(C2C1OCC2)OC(NC(C(CN(CC(C)C)S(=O)(=O)C=2C=CC1=C(C=CO1)C2)O)CC2=CC=CC=C2)=O
[CH3:1][CH:2]([CH3:3])[CH2:4][NH:5][CH2:6][CH:7]([OH:8])[CH:9]([CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)[NH:17][C:18](=[O:19])[O:20][CH:21]1[CH2:22][O:23][CH:24]2[O:25][CH2:26][CH2:27][CH:28]12.Cl[S:29](=[O:30])(=[O:31])[c:32]1[cH:33][cH:34][c:35]2[o:36][cH:37][cH:38][c:39]2[cH:40]1>>[CH3:1][CH:2]([CH3:3])[C...
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12.O=S(=O)(Cl)c1ccc2occc2c1
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occc2c1
null
null
C(Cl)Cl
Acylation
Sulfonamide synthesis (Schotten-Baumann) secondary amine
abeb6d9a0c70fe5baef0a8e555c2cd55ac2317f763ce7a0831775db7a04777d8
b7aca5a5d690b0846685a854bc946849e1041bfc3965161290b5ffb2821af09e
O=C(NC(CCNS(=O)(=O)c1ccc2occc2c1)Cc1ccccc1)OC1COC2OCCC12
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]>>[C:7]-[C:8]-[N;H0;D3;+0:9](-[C:10]-[C:11])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
null
[]
null
null
16
HOUR
Benzofuran-5-sulfonyl chloride 148 mg (0.68 mmol) was dissolved in 5 mL of methylene chloride. (1-Benzyl-2-hydroxy-3-isobutylamino-propyl)-carbamic acid hexahydro-furo[2,3-b]furan-3-yl ester 19 (244 mg, 0.62 mmol) was added followed by 0.63 mL 10% NaHCO3 solution (0.75 mmol). The reaction was stirred at room temperatur...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
null
null
c1ccccc1.C1CC2CCOC2O1.c1ccc2occc2c1
HCl
C(Cl)Cl
null
16
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12.O=S(=O)(Cl)c1ccc2occc2c1>C(Cl)Cl>CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occc2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0b020d2e3819488f85be6834a110dbfb
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occ(CN)c2c1.O=C(Cl)c1ccccc1>>CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occ(CNC(=O)c3ccccc3)c2c1
O1CC(C2C1OCC2)OC(NC(C(CN(CC(C)C)S(=O)(=O)C=2C=CC1=C(C(=CO1)CN)C2)O)CC2=CC=CC=C2)=O.C(C1=CC=CC=C1)(=O)Cl.C(C)N(CC)CC>>O1CC(C2C1OCC2)OC(NC(C(CN(CC(C)C)S(=O)(=O)C=2C=CC1=C(C(=CO1)CNC(C1=CC=CC=C1)=O)C2)O)CC2=CC=CC=C2)=O
[CH3:1][CH:2]([CH3:3])[CH2:4][N:5]([CH2:6][CH:7]([OH:8])[CH:9]([CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)[NH:17][C:18](=[O:19])[O:20][CH:21]1[CH2:22][O:23][CH:24]2[O:25][CH2:26][CH2:27][CH:28]12)[S:29](=[O:30])(=[O:31])[c:32]1[cH:33][cH:34][c:35]2[o:36][cH:37][c:38]([CH2:39][NH2:40])[c:49]2[cH:50]1.Cl[C:41](=...
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occ(CN)c2c1.O=C(Cl)c1ccccc1
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occ(CNC(=O)c3ccccc3)c2c1
null
null
C1CCOC1
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(NC(CCNS(=O)(=O)c1ccc2occ(CNC(=O)c3ccccc3)c2c1)Cc1ccccc1)OC1COC2OCCC12
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#8;a:6]:[c:7]:[c:8]-[C:9]-[NH2;D1;+0:10]>>[#8;a:6]:[c:7]:[c:8]-[C:9]-[NH;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
52
[{"value": 52.0, "product": "O1CC(C2C1OCC2)OC(NC(C(CN(CC(C)C)S(=O)(=O)C=2C=CC1=C(C(=CO1)CNC(C1=CC=CC=C1)=O)C2)O)CC2=CC=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
{3-[(3-Aminomethyl-benzofuran-5-sulfonyl)-isobutyl-amino]-1-benzyl-2-hydroxy-propyl}-carbamic acid hexahydro-furo[2,3-b]furan-3-yl ester from the previous step (20 mg, 33 umol) was dissolved in 0.5 mL THF. 5.8 uL (50 umol) benzoyl chloride and 7 uL (50 umol) triethylamine were added and the reaction was stirred at room...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.C1CC2CCOC2O1.c1ccc2occc2c1.c1ccccc1
HCl
C1CCOC1
null
1
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occ(CN)c2c1.O=C(Cl)c1ccccc1>C1CCOC1>CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc2occ(CNC(=O)c3ccccc3)c2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c6c5ae1d98dc4816a328e83c31c6e97d
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12.N#Cc1cc(S(=O)(=O)Cl)ccc1F>>CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc(F)c(C#N)c1
C(=O)(O)[O-].[Na+].O1CC(C2C1OCC2)OC(NC(C(CNCC(C)C)O)CC2=CC=CC=C2)=O.FC1=C(C=C(C=C1)S(=O)(=O)Cl)C#N.C(=O)(O)[O-].[Na+]>>O1CC(C2C1OCC2)OC(NC(C(CN(CC(C)C)S(=O)(=O)C2=CC(=C(C=C2)F)C#N)O)CC2=CC=CC=C2)=O
[CH3:1][CH:2]([CH3:3])[CH2:4][NH:5][CH2:6][CH:7]([OH:8])[CH:9]([CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)[NH:17][C:18](=[O:19])[O:20][CH:21]1[CH2:22][O:23][CH:24]2[O:25][CH2:26][CH2:27][CH:28]12.Cl[S:29](=[O:30])(=[O:31])[c:32]1[cH:33][cH:34][c:35]([F:36])[c:37]([C:38]#[N:39])[cH:40]1>>[CH3:1][CH:2]([CH3:3])[...
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12.N#Cc1cc(S(=O)(=O)Cl)ccc1F
CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc(F)c(C#N)c1
null
null
C(C)(=O)OCC
Acylation
Sulfonamide synthesis (Schotten-Baumann) secondary amine
abeb6d9a0c70fe5baef0a8e555c2cd55ac2317f763ce7a0831775db7a04777d8
b7aca5a5d690b0846685a854bc946849e1041bfc3965161290b5ffb2821af09e
O=C(NC(CCNS(=O)(=O)c1ccccc1)Cc1ccccc1)OC1COC2OCCC12
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]>>[C:7]-[C:8]-[N;H0;D3;+0:9](-[C:10]-[C:11])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
92
[{"value": 92.0, "product": "O1CC(C2C1OCC2)OC(NC(C(CN(CC(C)C)S(=O)(=O)C2=CC(=C(C=C2)F)C#N)O)CC2=CC=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of (1-benzyl-2-hydroxy-3-isobutylamino-propyl)-carbamic acid hexahydro-furo[2,3-b]furan-3-yl ester 19 in CH2C12 (4 mL) was added 4-fluoro-3-cyanobenzenesulfonyl chloride (92 mg, 0.42 mmol) followed by NaHCO3 (40 mg) and satd. NaHCO3 (0.4 mL) and stirred at RT for 1 h. The reaction mixture was diluted with...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
null
null
c1ccccc1.C1CC2CCOC2O1.c1ccccc1
HCl
C(C)(=O)OCC
null
null
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12.N#Cc1cc(S(=O)(=O)Cl)ccc1F>C(C)(=O)OCC>CC(C)CN(CC(O)C(Cc1ccccc1)NC(=O)OC1COC2OCCC12)S(=O)(=O)c1ccc(F)c(C#N)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b6c91dcf2f8c47799cd42b39bfc4aba8
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC(C)(C)C.Cc1n[nH]c2ccc(S(=O)(=O)Cl)cc12>>Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC(C)(C)C)cc12
C(C)(C)(C)OC(NC(C(CNCC(C)C)O)CC1=CC=CC=C1)=O.CC1=NNC2=CC=C(C=C12)S(=O)(=O)Cl.C(=O)(O)[O-].[Na+].C(=O)(O)[O-].[Na+].CCCCCC>>C(C)(C)(C)OC(NC(C(CN(S(=O)(=O)C=1C=C2C(=NNC2=CC1)C)CC(C)C)O)CC1=CC=CC=C1)=O
[NH:12]([CH2:13][CH:14]([CH3:15])[CH3:16])[CH2:17][CH:18]([OH:19])[CH:20]([CH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1)[NH:28][C:29](=[O:30])[O:31][C:32]([CH3:33])([CH3:34])[CH3:35].Cl[S:9]([c:8]1[cH:7][cH:6][c:5]2[nH:4][n:3][c:2]([CH3:1])[c:37]2[cH:36]1)(=[O:10])=[O:11]>>[CH3:1][c:2]1[n:3][nH:4][c:5]2[cH:6][cH:...
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC(C)(C)C.Cc1n[nH]c2ccc(S(=O)(=O)Cl)cc12
Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC(C)(C)C)cc12
null
null
ClCCl
Acylation
Sulfonamide synthesis (Schotten-Baumann) secondary amine
abeb6d9a0c70fe5baef0a8e555c2cd55ac2317f763ce7a0831775db7a04777d8
b7aca5a5d690b0846685a854bc946849e1041bfc3965161290b5ffb2821af09e
O=S(=O)(NCCCCc1ccccc1)c1ccc2[nH]ncc2c1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]>>[C:7]-[C:8]-[N;H0;D3;+0:9](-[C:10]-[C:11])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
99.5
[{"value": 99.0, "product": "C(C)(C)(C)OC(NC(C(CN(S(=O)(=O)C=1C=C2C(=NNC2=CC1)C)CC(C)C)O)CC1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.5, "product": "C(C)(C)(C)OC(NC(C(CN(S(=O)(=O)C=1C=C2C(=NNC2=CC1)C)CC(C)C)O)CC1=CC=CC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To (1-Benzyl-2-hydroxy-3-isobutylamino-propyl)-carbamic acid tert-butyl ester 15 (60 mg, 0.18 mmol) and 3-methyl-1H-indazole-5-sulfonyl chloride (50 mg, 0.22 mmol) in 2 mL dichloromethane was added a 70 ul solution of a saturated NaHCO3 and 30 mg NaHCO3 and stirred overnight. The product was purified by preparative TLC...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
null
null
c1ccc2n[nH]cc2c1.c1ccccc1
HCl
ClCCl
null
8
CC(C)CNCC(O)C(Cc1ccccc1)NC(=O)OC(C)(C)C.Cc1n[nH]c2ccc(S(=O)(=O)Cl)cc12>ClCCl>Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC(C)(C)C)cc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ce026a901f9f47dc966a3a7150cbc0c2
Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC(C)(C)C)cc12.O=C(OC1COC2OCCC12)ON1C(=O)CCC1=O>>Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC3COC4OCCC34)cc12
O1CC(C2C1OCC2)OC(ON2C(CCC2=O)=O)=O.C(C)(C)(C)OC(NC(C(CN(S(=O)(=O)C=1C=C2C(=NNC2=CC1)C)CC(C)C)O)CC1=CC=CC=C1)=O.Cl.C(C)(C)N(CC)C(C)C>>O1CC(C2C1OCC2)OC(NC(C(CN(S(=O)(=O)C=2C=C1C(=NNC1=CC2)C)CC(C)C)O)CC2=CC=CC=C2)=O
CC(C)(C)OC(=O)[NH:28][CH:20]([CH:18]([CH2:17][N:12]([S:9]([c:8]1[cH:7][cH:6][c:5]2[nH:4][n:3][c:2]([CH3:1])[c:41]2[cH:40]1)(=[O:10])=[O:11])[CH2:13][CH:14]([CH3:15])[CH3:16])[OH:19])[CH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1.O=C1CCC(=O)N1O[C:29](=[O:30])[O:31][CH:32]1[CH2:33][O:34][CH:35]2[O:36][CH2:37][CH2:38...
Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC(C)(C)C)cc12.O=C(OC1COC2OCCC12)ON1C(=O)CCC1=O
Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC3COC4OCCC34)cc12
null
null
O1CCOCC1
Protection
OtherReaction
1128a7ed8198894bb78897e6f497896066e6c904d8c783a7606c5f801ae7721e
c6b87d20dd468a6b1a3f862a783b52d5f603286c2fec0192cc836668a76ce046
O=C(NC(CCNS(=O)(=O)c1ccc2[nH]ncc2c1)Cc1ccccc1)OC1COC2OCCC12
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4].O=C1-C-C-C(=O)-N-1-O-[C;H0;D3;+0:5](=[O;D1;H0:6])-[#8:7]-[C:8]>>[C:3]-[C:2](-[C:4])-[NH;D2;+0:1]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[#8:7]-[C:8]
null
[]
null
null
8
HOUR
{1-Benzyl-2-hydroxy-3-[isobutyl-(3-methyl-1H-indazole-5-sulfonyl)-amino]-propyl}-carbamic acid tert-butyl ester (25 mg, 0.047 mmol) was added to a solution of 4N HCl in dioxane (0.25 mL). Material precipitated out so 800 uL conc. HCl was added and the reaction heated at reflux for 2 h. The resulting solution was concen...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Ether.Tertiary amide.Tertiary amide.Boc
Carbamic ester
C1CCNC1
null
c1ccc2n[nH]cc2c1.c1ccccc1.C1CC2CCOC2O1
HO-
O1CCOCC1
null
8
Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC(C)(C)C)cc12.O=C(OC1COC2OCCC12)ON1C(=O)CCC1=O>O1CCOCC1>Cc1n[nH]c2ccc(S(=O)(=O)N(CC(C)C)CC(O)C(Cc3ccccc3)NC(=O)OC3COC4OCCC34)cc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-42112608490a425faa1ac1eff5a4ebd2
CC(=O)OC(C)=O.Cc1n[nH]c2ccccc12>>CC(=O)n1nc(C)c2ccccc21
CC1=NNC2=CC=CC=C12.N1=CC=CC=C1.CC(=O)OC(=O)C>>CC1=NN(C2=CC=CC=C12)C(C)=O
CC(=O)O[C:2]([CH3:1])=[O:3].[nH:4]1[n:5][c:6]([CH3:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12>>[CH3:1][C:2](=[O:3])[n:4]1[n:5][c:6]([CH3:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12
CC(=O)OC(C)=O.Cc1n[nH]c2ccccc12
CC(=O)n1nc(C)c2ccccc21
null
CN(C)C=1C=CN=CC1
C1CCOC1
Acylation
Ester with secondary amine to amide
d2d8e67de66decf6e048f203acc2705e43acc0e3e98f0fe3c6249b66ad1e328e
93289da630dbaf2d9339c4212dcd342dfbcc29df4e79a63418a0fd9f589abdc1
c1ccc2[nH]ncc2c1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[c:4]:[c:5]1:[c:6]:[c:7]:[#7;a:8]:[nH;D2;+0:9]:1>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[n;H0;D3;+0:9]1:[#7;a:8]:[c:7]:[c:6]:[c:5]:1:[c:4]
91
[{"value": 91.0, "product": "CC1=NN(C2=CC=CC=C12)C(C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.6, "product": "CC1=NN(C2=CC=CC=C12)C(C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
3-Methylindazole (1.00 g, 7.6 mmol) was dissolved in 10 ml THF and stirred at RT under a blanket of argon. Pyridine (0.64 ml, 7.9 mmol) was added followed by Ac2O (0.79 ml, 8.3 mmol) and catalytic DMAP (90 mg, 0.7 mmol). The reaction proceeded for 2 h and was then partitioned between 1N HCl and dichloromethane. The org...
10.6084/m9.figshare.5104873.v1
null
Anhydride
null
c1ccc2[nH]ncc2c1
c1n[nH]c2ccccc12
c1n[nH]c2ccccc12
HO-
CN(C)C=1C=CN=CC1.C1CCOC1
null
2
CC(=O)OC(C)=O.Cc1n[nH]c2ccccc12>CN(C)C=1C=CN=CC1.C1CCOC1>CC(=O)n1nc(C)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-838c87c92f474128935a7992ddabd067
CC(=O)n1nc(C)c2ccccc21.O=S(=O)(O)Cl>>Cc1n[nH]c2ccc(S(=O)(=O)Cl)cc12
ClS(=O)(=O)O.CC1=NN(C2=CC=CC=C12)C(C)=O>>CC1=NNC2=CC=C(C=C12)S(=O)(=O)Cl
CC(=O)[n:4]1[n:3][c:2]([CH3:1])[c:14]2[c:5]1[cH:6][cH:7][cH:8][cH:13]2.O=[S:9]([OH:10])(=[O:11])[Cl:12]>>[CH3:1][c:2]1[n:3][nH:4][c:5]2[cH:6][cH:7][c:8]([S:9](=[O:10])(=[O:11])[Cl:12])[cH:13][c:14]12
CC(=O)n1nc(C)c2ccccc21.O=S(=O)(O)Cl
Cc1n[nH]c2ccc(S(=O)(=O)Cl)cc12
null
null
null
Protection
OtherReaction
b9dc7c87f2f45dd86e8ff60e2a7adab0bd3bba51bbf50c644b30368bb0c3eb20
c731d053565135be022f3edbe36cf28a9b4364ca579bdb183b2db9578bab4695
c1ccc2[nH]ncc2c1
C-C(=O)-[n;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]2:[c:5]:[cH;D2;+0:6]:[c:7]:[c:8]:[c:9]:2:1.O=[S;H0;D4;+0:10](-[Cl;D1;H0:11])(=[O;D1;H0:12])-[OH;D1;+0:13]>>[Cl;D1;H0:11]-[S;H0;D4;+0:10](=[O;D1;H0:12])(=[O;H0;D1;+0:13])-[c;H0;D3;+0:6]1:[c:5]:[c:4]2:[c:3]:[#7;a:2]:[nH;D2;+0:1]:[c:9]:2:[c:8]:[c:7]:1
63.6
[{"value": 61.0, "product": "CC1=NNC2=CC=C(C=C12)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.6, "product": "CC1=NNC2=CC=C(C=C12)S(=O)(=O)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To chlorosulfonic acid (0.38 ml, 5.7 mmol) under a blanket of argon in an ice bath was added 1-(3-methyl-indazol-1-yl)-ethanone (200 mg, 1.1 mmol). The reaction was allowed to warm to RT and then was heated at 70° C. for 45 min. The reaction was cooled to rt, slowly quenched over ice and extracted with dichloromethane....
10.6084/m9.figshare.5104873.v1
null
null
Sulfonyl halide
c1n[nH]c2ccccc12
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1
HO-
null
null
null
CC(=O)n1nc(C)c2ccccc21.O=S(=O)(O)Cl>>Cc1n[nH]c2ccc(S(=O)(=O)Cl)cc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ce9520244ed44683b5e5b9d1e3bd3a1b
BrCc1noc2ccccc12.O=S(=O)(O)Cl>>O=S(=O)(Cl)c1ccc2onc(CBr)c2c1
ClS(=O)(=O)O.BrCC1=NOC2=C1C=CC=C2>>BrCC1=NOC2=C1C=C(C=C2)S(=O)(=O)Cl
[cH:5]1[cH:6][cH:7][c:8]2[o:9][n:10][c:11]([CH2:12][Br:13])[c:14]2[cH:15]1.O[S:2](=[O:1])(=[O:3])[Cl:4]>>[O:1]=[S:2](=[O:3])([Cl:4])[c:5]1[cH:6][cH:7][c:8]2[o:9][n:10][c:11]([CH2:12][Br:13])[c:14]2[cH:15]1
BrCc1noc2ccccc12.O=S(=O)(O)Cl
O=S(=O)(Cl)c1ccc2onc(CBr)c2c1
null
null
null
Heteroatom Alkylation and Arylation
Aromatic sulfonyl chlorination
1de617f597940a4b1353fa427b486b905916e0273772c5a5239bad72a4ce2f2a
d32b60b8f9bfd187c6c9f1eef6a22a00f53525a7532b83aba763d5389c9e4280
c1ccc2oncc2c1
O-[S;H0;D4;+0:1](-[Cl;D1;H0:2])(=[O;D1;H0:3])=[O;D1;H0:4].[#7;a:5]1:[#8;a:6]:[c:7]2:[c:8]:[c:9]:[cH;D2;+0:10]:[c:11]:[c:12]:2:[c:13]:1>>[Cl;D1;H0:2]-[S;H0;D4;+0:1](=[O;D1;H0:3])(=[O;D1;H0:4])-[c;H0;D3;+0:10]1:[c:11]:[c:12]2:[c:13]:[#7;a:5]:[#8;a:6]:[c:7]:2:[c:8]:[c:9]:1
80.2
[{"value": 80.0, "product": "BrCC1=NOC2=C1C=C(C=C2)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.2, "product": "BrCC1=NOC2=C1C=C(C=C2)S(=O)(=O)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
6
HOUR
Chlorosulfonic acid (1.5 ml, 22 mmol) was slowly added to 3-Bromomethyl-benzo[d]isoxazole (1.0 g, 4.7 mmol) at RT under argon. The reaction was heated at 90° C. for 12 h and then left at RT for 6 h. The resulting viscous oil was quenched over ice, extracted with EtOAc, dried over MgSO4 and concentrated in vacuo to a br...
10.6084/m9.figshare.5104873.v1
null
null
Sulfonyl halide
c1ccc2oncc2c1
c1ccc2oncc2c1
c1ccc2oncc2c1
HO-
null
90
6
BrCc1noc2ccccc12.O=S(=O)(O)Cl>>O=S(=O)(Cl)c1ccc2onc(CBr)c2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a72737089aaa4ad48c4a57342ae8adb2
C(=NC1CCCCC1)=NC1CCCCC1.O=C(O)CC(=O)O>>O=C(NC1CCCCC1)NC1CCCCC1
C1CCC(CC1)N=C=NC2CCCCC2.C(CC(=O)O)(=O)O>>C1(CCCCC1)NC(=O)NC1CCCCC1
[C:2](=[N:3][CH:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9]1)=[N:10][CH:11]1[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]1.O=C(O)CC(O)=[O:1]>>[O:1]=[C:2]([NH:3][CH:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9]1)[NH:10][CH:11]1[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]1
C(=NC1CCCCC1)=NC1CCCCC1.O=C(O)CC(=O)O
O=C(NC1CCCCC1)NC1CCCCC1
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Miscellaneous
OtherReaction
0642a6af5b16e884276bf15c9f7fe9e7381a3a91014ec4f6a4d25a56dfeaaf0f
3a965eba3098fd1a397f9a7f68b5522f39b7a7b91f2a5718e79d867e06da2a35
O=C(NC1CCCCC1)NC1CCCCC1
O-C(=O)-C-C(-O)=[O;H0;D1;+0:1].[C:2]-[C:3](-[N;H0;D2;+0:4]=[C;H0;D2;+0:5]=[N;H0;D2;+0:6]-[C:7](-[C:8])-[C:9])-[C:10]>>[C:2]-[C:3](-[NH;D2;+0:4]-[C;H0;D3;+0:5](=[O;H0;D1;+0:1])-[NH;D2;+0:6]-[C:7](-[C:8])-[C:9])-[C:10]
60
[{"value": 60.0, "product": "C1(CCCCC1)NC(=O)NC1CCCCC1", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
15
MINUTE
104 mg (1 mmol) of malonic acid and 1.23 g (2.2 mmol) of alcohol 7 were dissolved in dry CH2Cl2 under N2 protection and the solution cooled in an ice bath. 41.0 mg (0.20 mmol) DMAP (10 mol %) and 454 mg (2.20 mmol) DCC were added subsequently. After stirring under N2-protection for 15 min at 0° C. and 2 h at RT, TLC co...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid
Urea
null
null
C1CCCCC1.C1CCCCC1
HO-
CN(C)C=1C=CN=CC1.C(Cl)Cl
0
0.25
C(=NC1CCCCC1)=NC1CCCCC1.O=C(O)CC(=O)O>CN(C)C=1C=CN=CC1.C(Cl)Cl>O=C(NC1CCCCC1)NC1CCCCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bb51094371c24b66b89e385748086d88
C=C(C)C.C[SiH2]O[Si](C)(C)C.C[SiH2]O[Si](C)(C)C>>CC(C)C[Si](C)(C)O[SiH](C)C
C[SiH2]O[Si](C)(C)C.C1(=CC=CC=C1)C.CC(C)=C.C[SiH2]O[Si](C)(C)C>>CC(C[Si](O[SiH](C)C)(C)C)C
[CH3:1][C:2]([CH3:3])=[CH2:4].C[Si:9]([O:8][SiH2:5][CH3:6])([CH3:10])[CH3:11].C[SiH2]O[Si](C)(C)[CH3:7]>>[CH3:1][CH:2]([CH3:3])[CH2:4][Si:5]([CH3:6])([CH3:7])[O:8][SiH:9]([CH3:10])[CH3:11]
C=C(C)C.C[SiH2]O[Si](C)(C)C.C[SiH2]O[Si](C)(C)C
CC(C)C[Si](C)(C)O[SiH](C)C
null
C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]
null
Miscellaneous
OtherReaction
b4bff7b9dcd71eb005ee39656535d134dbcf321494767350d1f69e556c66a41c
ecf71ff1f33b95218682f89e2359975035d7e3510954631c0171914de0ec4fcf
null
C-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[#8:4]-[SiH2;D2;+0:5]-[C;D1;H3:6].C-[SiH2]-O-[Si](-C)(-C)-[CH3;D1;+0:7].[C;D1;H3:8]-[C;H0;D3;+0:9](-[C;D1;H3:10])=[CH2;D1;+0:11]>>[C;D1;H3:2]-[SiH;D3;+0:1](-[C;D1;H3:3])-[#8:4]-[Si;H0;D4;+0:5](-[C;D1;H3:6])(-[CH3;D1;+0:7])-[CH2;D2;+0:11]-[CH;D3;+0:9](-[C;D1;H3:8])-[C;D1;H3:...
null
[]
65
CELSIUS
null
null
An 80 mL Fischer-Porter high pressure bottle was charged with tetramethyldisiloxane (10.0 g), toluene (10.0 g) and Wilkinson's catalyst ((PPh3)3RhCl, 40 ppm), stirred and brought to 60° C. The bottle was attached to a manifold and pressurized with isobutylene (25 psig) and maintained at 60-70° C. for 8 h. The pressure ...
10.6084/m9.figshare.5104873.v1
null
Vinyl.Silyl protective group.Silyl protective group
Silyl protective group
null
null
null
HO-
C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]
65
null
C=C(C)C.C[SiH2]O[Si](C)(C)C.C[SiH2]O[Si](C)(C)C>C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]>CC(C)C[Si](C)(C)O[SiH](C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a084dd9163ef4076ab27ee0607da2c42
C=CC.C[SiH2]O[Si](C)(C)C>>CCC[Si](C)(C)O[SiH](C)C
C[SiH2]O[Si](C)(C)C.C1(=CC=CC=C1)C.C=CC>>C(CC)[Si](O[SiH](C)C)(C)C
[CH3:1][CH:2]=[CH2:3].[SiH2:4]([CH3:5])[O:7][Si:8]([CH3:6])([CH3:9])[CH3:10]>>[CH3:1][CH2:2][CH2:3][Si:4]([CH3:5])([CH3:6])[O:7][SiH:8]([CH3:9])[CH3:10]
C=CC.C[SiH2]O[Si](C)(C)C
CCC[Si](C)(C)O[SiH](C)C
null
C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]
null
Miscellaneous
OtherReaction
48aaa97344ecca5468aef29c7ae97b953b9270cac980ae6594ab741e32b388dd
a73aab15218d9f83236501cdc99718c52ca13cdc4d7f312ae7b6fa0d5a506e13
null
[C;D1;H3:1]-[CH;D2;+0:2]=[CH2;D1;+0:3].[C;D1;H3:4]-[Si;H0;D4;+0:5](-[C;D1;H3:6])(-[CH3;D1;+0:7])-[#8:8]-[SiH2;D2;+0:9]-[C;D1;H3:10]>>[C;D1;H3:4]-[SiH;D3;+0:5](-[C;D1;H3:6])-[#8:8]-[Si;H0;D4;+0:9](-[C;D1;H3:10])(-[CH3;D1;+0:7])-[CH2;D2;+0:3]-[CH2;D2;+0:2]-[C;D1;H3:1]
null
[]
50
CELSIUS
null
null
An 80 mL Fischer-Porter high pressure bottle was charged with tetramethyldisiloxane (10.0 g), toluene (10.0 g) and Wilkinson's catalyst ((PPh3)3RhCl, 40 ppm), stirred and brought to 50° C. The bottle was attached to a manifold and pressurized with propylene (40 psig) and maintained at 50° C. for 2 h. The pressure was v...
10.6084/m9.figshare.5104873.v1
null
Vinyl.Silyl protective group
Silyl protective group
null
null
null
null
C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]
50
null
C=CC.C[SiH2]O[Si](C)(C)C>C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]>CCC[Si](C)(C)O[SiH](C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c5c287dd7b134f45bb78154a1dee8a69
CC(C)(C)[Si](C)(C)Cl.C[SiH](C)Cl.O>>C[SiH](C)O[Si](C)(C)C(C)(C)C
O.C[SiH](Cl)C.[Si](C)(C)(C(C)(C)C)Cl.O>>C(C)(C)(C)[Si](O[SiH](C)C)(C)C
Cl[Si:5]([CH3:6])([CH3:7])[C:8]([CH3:9])([CH3:10])[CH3:11].Cl[SiH:2]([CH3:1])[CH3:3].[OH2:4]>>[CH3:1][SiH:2]([CH3:3])[O:4][Si:5]([CH3:6])([CH3:7])[C:8]([CH3:9])([CH3:10])[CH3:11]
CC(C)(C)[Si](C)(C)Cl.C[SiH](C)Cl.O
C[SiH](C)O[Si](C)(C)C(C)(C)C
null
null
C(C)(C)OC(C)C
Protection
OtherReaction
bcb384be6de101a88c51c45266569e6728cab9c6042ed1ac123bd15419519cd8
d3939d5b137968db9e591134356fa8e55d322b5352280788afd540e031d3a866
null
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].Cl-[SiH;D3;+0:8](-[C;D1;H3:9])-[C;D1;H3:10].[OH2;D0;+0:11]>>[C;D1;H3:5]-[C:4](-[C;D1;H3:6])(-[C;D1;H3:7])-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[O;H0;D2;+0:11]-[SiH;D3;+0:8](-[C;D1;H3:9])-[C;D1;H3:10]
null
[]
32.5
CELSIUS
null
null
A 1 L round bottom flask was charged with water (95 g) and diisopropyl ether (50 g) and stirred. A solution of tert-butyldimethylsilyl chloride (39.5 g) in isopropyl ether (50 g) was charged to an addition funnel, and added dropwise to the water/IPE mixture at a rate to maintain the reaction temperature between 30-35° ...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
TMS ether protective group
null
null
null
HCl
C(C)(C)OC(C)C
32.5
null
CC(C)(C)[Si](C)(C)Cl.C[SiH](C)Cl.O>C(C)(C)OC(C)C>C[SiH](C)O[Si](C)(C)C(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d454e0aadbda429e85a9206ac6fc1e6f
BrBr.c1ccc(C2CC2)cc1>>Brc1ccc(C2CC2)cc1
OS(=O)[O-].[Na+].BrBr.C1(CC1)C1=CC=CC=C1.C(C)(=O)[O-].[Na+]>>C1(CC1)C1=CC=C(C=C1)Br
Br[Br:1].[cH:2]1[cH:3][cH:4][c:5]([CH:6]2[CH2:7][CH2:8]2)[cH:9][cH:10]1>>[Br:1][c:2]1[cH:3][cH:4][c:5]([CH:6]2[CH2:7][CH2:8]2)[cH:9][cH:10]1
BrBr.c1ccc(C2CC2)cc1
Brc1ccc(C2CC2)cc1
null
null
O.C(C)(=O)O
Functional Group Interconversion
Bromination
f6effe61353895b318215d8bd9b6bb1105cafbf7be8c217d748df587260b32c3
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc(C2CC2)cc1
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]:[cH;D2;+0:4]:[c:5]:[c:6]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:3]:[c:2]
21
[{"value": 21.0, "product": "C1(CC1)C1=CC=C(C=C1)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 21.0, "product": "C1(CC1)C1=CC=C(C=C1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
Cyclopropyl benzene (48.5 g, 410 mmol), glacial acetic acid (510 mL), and sodium acetate (38.9 g, 474 mmol) were added to a round bottomed flask. The flask was cooled in an ice-water bath. A solution of bromine (66.3 g, 414 mmol) dissolved in 105 mL of acetic acid was added dropwise over 90 min. The reaction mixture wa...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1.C1CC1
HBr
O.C(C)(=O)O
null
5
BrBr.c1ccc(C2CC2)cc1>O.C(C)(=O)O>Brc1ccc(C2CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9116056894ee47a3b743e195d1a7d4bd
O=S(=O)(Cl)c1ccc(C2CC2)cc1.[F-]>>O=S(=O)(F)c1ccc(C2CC2)cc1
C1(CC1)C1=CC=C(C=C1)S(=O)(=O)Cl.[F-].[K+]>>C1(CC1)C1=CC=C(C=C1)S(=O)(=O)F
Cl[S:2](=[O:1])(=[O:3])[c:5]1[cH:6][cH:7][c:8]([CH:9]2[CH2:10][CH2:11]2)[cH:12][cH:13]1.[F-:4]>>[O:1]=[S:2](=[O:3])([F:4])[c:5]1[cH:6][cH:7][c:8]([CH:9]2[CH2:10][CH2:11]2)[cH:12][cH:13]1
O=S(=O)(Cl)c1ccc(C2CC2)cc1.[F-]
O=S(=O)(F)c1ccc(C2CC2)cc1
null
null
O.CC(=O)C.CCOC(=O)C
Functional Group Interconversion
OtherReaction
1a5adee7f1ba8844d3aeea23793c6ed559c5770364925cb0ebd2c7a72ae17659
100ecb262b71c25deadc3940d6f3c2c0e7443b2546e5e1649d38d873195b4540
c1ccc(C2CC2)cc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[F-;H0;D0:7]>>[F;H0;D1;+0:7]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
97
[{"value": 97.0, "product": "C1(CC1)C1=CC=C(C=C1)S(=O)(=O)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.7, "product": "C1(CC1)C1=CC=C(C=C1)S(=O)(=O)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Crude compound 45 (13.3 g) was dissolved in 200 mL of acetone and 60 mL of water. Potassium fluoride (7.12 g, 122 mmol) was added and the reaction mixture was stirred overnight at rt. The reaction mixture was diluted with EtOAc and washed with water. The organic layer was dried with Na2SO4, filtered, and concentrated t...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
Sulfonyl halide
null
null
c1ccccc1.C1CC1
Other
O.CC(=O)C.CCOC(=O)C
null
8
O=S(=O)(Cl)c1ccc(C2CC2)cc1.[F-]>O.CC(=O)C.CCOC(=O)C>O=S(=O)(F)c1ccc(C2CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-28df4cf85a8944b3854f43b6c60da1fe
CC(=O)c1ccncc1.NN.O=CC(=O)O>>O=c1ccc(-c2ccncc2)n[nH]1
C(C)(=O)C1=CC=NC=C1.C([O-])([O-])=O.[K+].[K+].O.C(C=O)(=O)O.C(=O)([O-])[O-].[K+].[K+].O.NN>>N1=CC=C(C=C1)C=1C=CC(NN1)=O
O=[C:5]([CH3:4])[c:6]1[cH:7][cH:8][n:9][cH:10][cH:11]1.[NH2:12][NH2:13].O=[CH:3][C:2](O)=[O:1]>>[O:1]=[c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[n:12][nH:13]1
CC(=O)c1ccncc1.NN.O=CC(=O)O
O=c1ccc(-c2ccncc2)n[nH]1
null
null
O.C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
0461b2f03bfc59a40676cd766082d1f571986553f759b05431b650a71f0fe88c
87635d623d9cacd54865f4e9739e35f5fc1294b1eab6c4ff3e83b38d330e008c
O=c1ccc(-c2ccncc2)n[nH]1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH;D2;+0:3]=O.O=[C;H0;D3;+0:4](-[CH3;D1;+0:5])-[c;H0;D3;+0:6]1:[c:7]:[c:8]:[#7;a:9]:[c:10]:[c:11]:1.[NH2;D1;+0:12]-[NH2;D1;+0:13]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[cH;D2;+0:3]:[cH;D2;+0:5]:[c;H0;D3;+0:4](-[c;H0;D3;+0:6]2:[c:7]:[c:8]:[#7;a:9]:[c:10]:[c:11]:2):[n;H0;D2;+0:12]:[nH;D2;+0:13]:1
64
[{"value": 64.0, "product": "N1=CC=C(C=C1)C=1C=CC(NN1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2.5
HOUR
99.5 g 4-Acetylpyridine is added to a cold (10° C.) solution of 222.4 potassium carbonate and 76.3 glyoxylic acid monohydrate in 1 L of water and the solution stirred at room temperature for 2.5 h. After cooling in to 0° C., 325 ml of acetic acid are added followed by 58.8 ml hydrazine hydrate, and the resulting soluti...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Aldehyde.Carboxylic acid.Ketone
null
null
c1cccnn1
c1cccnn1.c1ccncc1
HO-
O.C(C)(=O)O
null
2.5
CC(=O)c1ccncc1.NN.O=CC(=O)O>O.C(C)(=O)O>O=c1ccc(-c2ccncc2)n[nH]1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-df293d8948ca4d669724f7c80cc987c5
O=P(Cl)(Cl)Cl.O=c1ccc(-c2ccncc2)n[nH]1>>Clc1ccc(-c2ccncc2)nn1
N1=CC=C(C=C1)C=1C=CC(NN1)=O.P(=O)(Cl)(Cl)Cl>>ClC=1N=NC(=CC1)C1=CC=NC=C1
O=P(Cl)(Cl)[Cl:1].O=[c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[n:12][nH:13]1>>[Cl:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[n:12][n:13]1
O=P(Cl)(Cl)Cl.O=c1ccc(-c2ccncc2)n[nH]1
Clc1ccc(-c2ccncc2)nn1
null
null
null
Functional Group Interconversion
OtherReaction
980c777204deda72a9af5dde6575971b5f1222eda5e63e2dd187b0b667e1d6d9
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1cnnc(-c2ccncc2)c1
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[c:3]:[c:4]:[c:5]:[#7;a:6]:[nH;D2;+0:7]:1>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[c:3]:[c:4]:[c:5]:[#7;a:6]:[n;H0;D2;+0:7]:1
64.6
[{"value": 64.6, "product": "ClC=1N=NC(=CC1)C1=CC=NC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
1
HOUR
75.6 g 6-Pyridin-4-yl-2H-pyridazin-3-one is added in small portions to 234.5 g phosphorus oxychloride and the resulting mixture is stirred for 1 h at 100° C. Diluting into ice cold water, adjusting the pH 7 with aqueous sodium hydroxide and extraction with dichloromethane yielded 54 g 3-Chloro-6-pyridin-4-yl-pyridazine...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1cccnn1
c1ccnnc1
c1ccnnc1.c1ccncc1
HCl
null
100
1
O=P(Cl)(Cl)Cl.O=c1ccc(-c2ccncc2)n[nH]1>>Clc1ccc(-c2ccncc2)nn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-62fd159e83e5416fbdff63e700088ba2
C[O-].Clc1ccc(-c2ccncc2)nn1>>COc1ccc(-c2ccncc2)nn1
C[O-].[Na+].ClC=1N=NC(=CC1)C1=CC=NC=C1>>COC=1N=NC(=CC1)C1=CC=NC=C1
[CH3:1][O-:2].Cl[c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[n:13][n:14]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[n:13][n:14]1
C[O-].Clc1ccc(-c2ccncc2)nn1
COc1ccc(-c2ccncc2)nn1
null
null
CO
Heteroatom Alkylation and Arylation
OtherReaction
a9b48706c0031de50054078adf178cdb9c97933ae9a69eb837163dea0dd09084
51fd03eb6a688046e417b9ed09ea0e72062396d005af1318b9b5f376a97da959
c1cnnc(-c2ccncc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1.[C;D1;H3:7]-[O-;H0;D1:8]>>[C;D1;H3:7]-[O;H0;D2;+0:8]-[c;H0;D3;+0:1]1:[#7;a:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1
null
[]
null
null
null
null
63 ml of a 32% sodium methoxide solution in methanol are added to a solution of 57 g 3-Chloro-6-pyridin-4-yl-pyridazine in methanol, and the reaction mixture is stirred under reflux for 1.5 h. The solvent is removed under reduced pressure, the residue suspended in 0.7 L water and the pH adjusted to 7. Extraction with d...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Ether
c1ccnnc1
c1ccnnc1
c1ccnnc1.c1ccncc1
Other
CO
null
null
C[O-].Clc1ccc(-c2ccncc2)nn1>CO>COc1ccc(-c2ccncc2)nn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8abab3a4ad8a47a697141fbdebc2189e
COc1ccc(-c2ccncc2)nn1.II>>COc1nnc(-c2ccncc2)cc1I
C(CCC)[Li].CC1(NC(CCC1)(C)C)C.COC=1N=NC(=CC1)C1=CC=NC=C1.II>>IC1=C(N=NC(=C1)C1=CC=NC=C1)OC
[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][cH:14]1.I[I:15]>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1[I:15]
COc1ccc(-c2ccncc2)nn1.II
COc1nnc(-c2ccncc2)cc1I
null
null
CCCCCC.C1CCOC1
Functional Group Interconversion
OtherReaction
3b22a5d23572bfe9ad1502a182eb9a0357f308a16eb4f4f5e1618044bed6ab38
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1cnnc(-c2ccncc2)c1
I-[I;H0;D1;+0:1].[#8:2]-[c:3]1:[#7;a:4]:[#7;a:5]:[c:6](-[c:7]):[c:8]:[cH;D2;+0:9]:1>>[#8:2]-[c:3]1:[#7;a:4]:[#7;a:5]:[c:6](-[c:7]):[c:8]:[c;H0;D3;+0:9]:1-[I;H0;D1;+0:1]
76.9
[{"value": 76.9, "product": "IC1=C(N=NC(=C1)C1=CC=NC=C1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
45 ml 1.6M solution of n-Butyllithium in hexane are added at −30° C. to a 10.2 g 2,2,6,6-tetramethylpiperidine in 100 ml THF, and the mixture is stirred at 0° C. for 30 min. After cooling to −75° C., 11.2 g 3-Methoxy-6-pyridin-4-yl-pyridazine dissolved 300 ml THF are added, and the solution is stirred at −75° C. for 35...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccnnc1
c1ccnnc1
c1ccnnc1.c1ccncc1
HI
CCCCCC.C1CCOC1
0
0.5
COc1ccc(-c2ccncc2)nn1.II>CCCCCC.C1CCOC1>COc1nnc(-c2ccncc2)cc1I
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9c2f5754bafc4404a3db8a4e1aef1435
CC(C)(C)OC(=O)n1c(B(O)O)cc2ccccc21.COc1nnc(-c2ccncc2)cc1I>>COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C
IC1=C(N=NC(=C1)C1=CC=NC=C1)OC.C(C)(C)(C)OC(=O)N1C(=CC2=CC=CC=C12)B(O)O.C([O-])([O-])=O.[K+].[K+].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=CC=C12)C1=C(N=NC(=C1)C1=CC=NC=C1)OC
OB(O)[c:15]1[cH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]2[n:23]1[C:24](=[O:25])[O:26][C:27]([CH3:28])([CH3:29])[CH3:30].I[c:14]1[c:3]([O:2][CH3:1])[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1-[c:15]1[cH:1...
CC(C)(C)OC(=O)n1c(B(O)O)cc2ccccc21.COc1nnc(-c2ccncc2)cc1I
COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
O.COCCOC.C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
1825c39cd9e32be09658a13a21b34a56b6f1ce71f57a969c757b7ba9a84ebe00
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
I-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[c:4]):[#7;a:5]:[#7;a:6]:[c:7]:1-[#8:8].O-B(-O)-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[c:12]:[#7;a:13]:1-[C:14](=[O;D1;H0:15])-[#8:16]-[C:17](-[C;D1;H3:18])(-[C;D1;H3:19])-[C;D1;H3:20]>>[#8:8]-[c:7]1:[#7;a:6]:[#7;a:5]:[c:3](-[c:4]):[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[c:12]:[#7;a...
null
[]
null
null
null
null
Argon is passed for 30 min through a suspension of 55 mg 4-Iodo-3-methoxy-6-pyridin-4-yl-pyridazine, 55 mg 1-(tert-butoxycarbonyl)indole-2-boronic acid, 53.5 mg potassium carbonate, and 18.5 mg triphenylphosphine in 0.8 ml DME and 0.7 ml water. 4 mg palladium (II) acetate is added, and the mixture is stirred under refl...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc2ccccc2[nH]1.c1ccnnc1
c1ccnnc1.c1cc2ccccc2[nH]1
c1ccnnc1.c1ccncc1.c1cc2ccccc2[nH]1
HI.B
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.COCCOC.C(C)(=O)OCC
null
null
CC(C)(C)OC(=O)n1c(B(O)O)cc2ccccc21.COc1nnc(-c2ccncc2)cc1I>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.COCCOC.C(C)(=O)OCC>COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b550d42f4a41483788e567e509065321
COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C>>O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
Cl.C(C)(C)(C)OC(=O)N1C(=CC2=CC=CC=C12)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.C[Si](Cl)(C)C.CN(C)C=O.O>>N1C(=CC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O
CC(C)(C)OC(=O)[n:22]1[c:14](-[c:13]2[c:2]([O:1]C)[n:3][n:4][c:5](-[c:6]3[cH:7][cH:8][n:9][cH:10][cH:11]3)[cH:12]2)[cH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]21>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[cH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[nH:22]1
COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
null
null
O1CCOCC1.C(C)#N
Functional Group Interconversion
OtherReaction
ccff9e96bdfd7c95ea90e5e92eb38ee503eb19e38ebb19293d7570ec24d3836c
e4c2437726be227f3a4589d2c6c79cc20b165fa11361f93621036c026b9ea7bf
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]1:[c:9]:[c:10]:[c:11](:[c:12]):[n;H0;D3;+0:13]:1-C(=O)-O-C(-C)(-C)-C>>[O;H0;D1;+0:1]=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]1:[c:9]:[c:10]:[c:11](:[c:12]):[nH;D2;+0:13]:1
25.1
[{"value": 25.1, "product": "N1C(=CC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
2
HOUR
25 mg of 2-(3-Methoxy-6-pyridin-4-yl-pyridazin-4-yl) -indole-1-carboxylic acid tert-butyl ester, 7.4 mg trimethylchlorosilane and 11.3 mg KI dissolved in 1 ml of acetonitrile are stirred for 2 h at 60° C. Subsequently, 0.5 ml of a 4N solution of hydrochloric acid in dioxane is added and stirred for 2 h at room temperat...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Boc
null
c1ccnnc1.c1cc2ccccc2[nH]1
c1cnncc1.c1ccc2[nH]ccc2c1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1
HO-
O1CCOCC1.C(C)#N
60
2
COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C>O1CCOCC1.C(C)#N>O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-28d11d416310459daff1279f034bef16
CC(C)(C)OC(=O)n1c(B(O)O)cc2ccccc21.COc1nnc(Cl)cc1I>>COc1nnc(Cl)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C
ClC1=CC(=C(N=N1)OC)I.C(C)(C)(C)OC(=O)N1C(=CC2=CC=CC=C12)B(O)O.C([O-])([O-])=O.[K+].[K+].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=CC=C12)C1=C(N=NC(=C1)Cl)OC
OB(O)[c:10]1[cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[n:18]1[C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25].I[c:9]1[c:3]([O:2][CH3:1])[n:4][n:5][c:6]([Cl:7])[cH:8]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6]([Cl:7])[cH:8][c:9]1-[c:10]1[cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[n:18]1[C:19](=[O:20])[O:21]...
CC(C)(C)OC(=O)n1c(B(O)O)cc2ccccc21.COc1nnc(Cl)cc1I
COc1nnc(Cl)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
O.COCCOC.C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
1825c39cd9e32be09658a13a21b34a56b6f1ce71f57a969c757b7ba9a84ebe00
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc2[nH]c(-c3ccnnc3)cc2c1
I-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[Cl;D1;H0:4]):[#7;a:5]:[#7;a:6]:[c:7]:1-[#8:8].O-B(-O)-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[c:12]:[#7;a:13]:1-[C:14](=[O;D1;H0:15])-[#8:16]-[C:17](-[C;D1;H3:18])(-[C;D1;H3:19])-[C;D1;H3:20]>>[#8:8]-[c:7]1:[#7;a:6]:[#7;a:5]:[c:3](-[Cl;D1;H0:4]):[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9]1:[c:10]:[c:11...
null
[]
null
null
null
null
Argon is passed for 30 min through a suspension of 135 mg 6-Chloro-4-iodo-3-methoxy-pyridazine, 130.5 mg 1-(tert-butoxycarbonyl)indole-2-boronic acid, 152 mg potassium carbonate, and 52.5 mg triphenylphosphine in 2.2 ml DME and 1.1 ml water. 11.2 mg palladium (II) acetate is added, and the mixture is stirred under refl...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc2ccccc2[nH]1.c1ccnnc1
c1ccnnc1.c1cc2ccccc2[nH]1
c1ccnnc1.c1cc2ccccc2[nH]1
HI.B
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.COCCOC.C(C)(=O)OCC
null
null
CC(C)(C)OC(=O)n1c(B(O)O)cc2ccccc21.COc1nnc(Cl)cc1I>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.COCCOC.C(C)(=O)OCC>COc1nnc(Cl)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-47393936c874421891c1b4b0bc535d00
CC(C)OB1OC(C)(C)C(C)(C)O1.Cc1cn(C(=O)OC(C)(C)C)c2ccccc12>>Cc1c(B2OC(C)(C)C(C)(C)O2)n(C(=O)OC(C)(C)C)c2ccccc12
C(C)(C)(C)OC(=O)N1C=C(C2=CC=CC=C12)C.[Li+].CC(C)[N-]C(C)C.C(C)(C)OB1OC(C(O1)(C)C)(C)C>>C(C)(C)(C)OC(=O)N1C(=C(C2=CC=CC=C12)C)B1OC(C(O1)(C)C)(C)C
CC(C)O[B:4]1[O:5][C:6]([CH3:7])([CH3:8])[C:9]([CH3:10])([CH3:11])[O:12]1.[CH3:1][c:2]1[cH:3][n:13]([C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20])[c:21]2[cH:22][cH:23][cH:24][cH:25][c:26]12>>[CH3:1][c:2]1[c:3]([B:4]2[O:5][C:6]([CH3:7])([CH3:8])[C:9]([CH3:10])([CH3:11])[O:12]2)[n:13]([C:14](=[O:15])[O:16][C:17]...
CC(C)OB1OC(C)(C)C(C)(C)O1.Cc1cn(C(=O)OC(C)(C)C)c2ccccc12
Cc1c(B2OC(C)(C)C(C)(C)O2)n(C(=O)OC(C)(C)C)c2ccccc12
null
null
O1CCCC1.C1CCOC1.CCCCCC
Functional Group Interconversion
OtherReaction
6d7c7d3bd6b2a5cfde60b017fe21925e0baa18667a55bca89303f87003bc482b
55b2480301cea859d1218f23e11281559f3dfc2ef4b9f2ac7f38d4293c2fe6cc
c1ccc2[nH]c(B3OCCO3)cc2c1
C-C(-C)-O-[B;H0;D3;+0:1]1-[#8:2]-[C:3]-[C:4]-[#8:5]-1.[C;D1;H3:6]-[C:7](-[C;D1;H3:8])(-[C;D1;H3:9])-[#8:10]-[C:11](=[O;D1;H0:12])-[#7;a:13]1:[c:14]:[c:15]:[c:16](-[C;D1;H3:17]):[cH;D2;+0:18]:1>>[C;D1;H3:6]-[C:7](-[C;D1;H3:8])(-[C;D1;H3:9])-[#8:10]-[C:11](=[O;D1;H0:12])-[#7;a:13]1:[c:14]:[c:15]:[c:16](-[C;D1;H3:17]):[c;...
null
[]
0
CELSIUS
30
MINUTE
To a solution of 462 mg 3-Methyl-indole-1-carboxylic acid tert-butyl ester in 2.5 ml anhydrous tetrahydrofuran at −78° C. under argon is added 1.2 ml of a 2M LDA solution in THF/hexane and stirred at 0° C. for 30 min to complete the deprotonation. The reaction mixture is cooled to −78° C., 0.6 ml 2-Isopropoxy-4,4,5,5-t...
10.6084/m9.figshare.5104873.v1
null
null
Boronic ester
[B]1OCCO1.c1c[nH]c2ccccc12
[B]1OCCO1.c1cc2ccccc2[nH]1
[B]1OCCO1.c1cc2ccccc2[nH]1
HO-
O1CCCC1.C1CCOC1.CCCCCC
0
0.5
CC(C)OB1OC(C)(C)C(C)(C)O1.Cc1cn(C(=O)OC(C)(C)C)c2ccccc12>O1CCCC1.C1CCOC1.CCCCCC>Cc1c(B2OC(C)(C)C(C)(C)O2)n(C(=O)OC(C)(C)C)c2ccccc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ea2469830b4c4d03baee311161473058
COc1nnc(-c2ccncc2)cc1I.Cc1c(B2OC(C)(C)C(C)(C)O2)n(C(=O)OC(C)(C)C)c2ccccc12>>COc1nnc(-c2ccncc2)cc1-c1c(C)c2ccccc2n1C(=O)OC(C)(C)C
IC1=C(N=NC(=C1)C1=CC=NC=C1)OC.C(C)(C)(C)OC(=O)N1C(=C(C2=CC=CC=C12)C)B1OC(C(O1)(C)C)(C)C.C([O-])([O-])=O.[K+].[K+].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>C(C)(C)(C)OC(=O)N1C(=C(C2=CC=CC=C12)C)C1=C(N=NC(=C1)C1=CC=NC=C1)OC
I[c:14]1[c:3]([O:2][CH3:1])[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13]1.CC1(C)OB([c:15]2[c:16]([CH3:17])[c:18]3[cH:19][cH:20][cH:21][cH:22][c:23]3[n:24]2[C:25](=[O:26])[O:27][C:28]([CH3:29])([CH3:30])[CH3:31])OC1(C)C>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13...
COc1nnc(-c2ccncc2)cc1I.Cc1c(B2OC(C)(C)C(C)(C)O2)n(C(=O)OC(C)(C)C)c2ccccc12
COc1nnc(-c2ccncc2)cc1-c1c(C)c2ccccc2n1C(=O)OC(C)(C)C
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
O.COCCOC.C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic esters
950d74e7d32747b9e96a82a5735570544e464a4aae937bd81248abdfc2ab46de
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
C-C1(-C)-O-B(-[c;H0;D3;+0:1]2:[#7;a:2](-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6](-[C;D1;H3:7])(-[C;D1;H3:8])-[C;D1;H3:9]):[c:10]:[c:11]:[c:12]:2-[C;D1;H3:13])-O-C-1(-C)-C.I-[c;H0;D3;+0:14]1:[c:15]:[c:16](-[c:17]):[#7;a:18]:[#7;a:19]:[c:20]:1-[#8:21]>>[#8:21]-[c:20]1:[#7;a:19]:[#7;a:18]:[c:16](-[c:17]):[c:15]:[c;H0;D3;+0:14]:1-...
null
[]
null
null
null
null
Argon is passed for 30 min through a suspension of 333 mg 4-Iodo-3-methoxy-6-pyridin-4-yl-pyridazine, 380 mg 3-Methyl-2-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-indole-1-carb-oxylic acid tert-butyl ester, 294 mg potassium carbonate, and 111.6 mg triphenylphosphine in 4.8 ml DME and 2.4 ml water. 24 mg palladium (...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1ccnnc1.B1OCCO1.c1cc2ccccc2[nH]1
c1ccnnc1.c1cc2ccccc2[nH]1
c1ccnnc1.c1ccncc1.c1cc2ccccc2[nH]1
HI.B
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.COCCOC.C(C)(=O)OCC
null
null
COc1nnc(-c2ccncc2)cc1I.Cc1c(B2OC(C)(C)C(C)(C)O2)n(C(=O)OC(C)(C)C)c2ccccc12>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.COCCOC.C(C)(=O)OCC>COc1nnc(-c2ccncc2)cc1-c1c(C)c2ccccc2n1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-84e18a8e496b4d0886d03495ef54cd7d
COc1nnc(-c2ccncc2)cc1-c1c(C)c2ccccc2n1C(=O)OC(C)(C)C>>Cc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
C(C)(C)(C)OC(=O)N1C(=C(C2=CC=CC=C12)C)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.Cl>>CC1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O
CC(C)(C)OC(=O)[n:17]1[c:3](-[c:4]2[cH:5][c:6](-[c:7]3[cH:8][cH:9][n:10][cH:11][cH:12]3)[n:13][n:14][c:15]2[O:16]C)[c:2]([CH3:1])[c:23]2[c:18]1[cH:19][cH:20][cH:21][cH:22]2>>[CH3:1][c:2]1[c:3](-[c:4]2[cH:5][c:6](-[c:7]3[cH:8][cH:9][n:10][cH:11][cH:12]3)[n:13][nH:14][c:15]2=[O:16])[nH:17][c:18]2[cH:19][cH:20][cH:21][cH:2...
COc1nnc(-c2ccncc2)cc1-c1c(C)c2ccccc2n1C(=O)OC(C)(C)C
Cc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
null
null
[OH-].[Na+].C(C)O
Functional Group Interconversion
OtherReaction
ccff9e96bdfd7c95ea90e5e92eb38ee503eb19e38ebb19293d7570ec24d3836c
e4c2437726be227f3a4589d2c6c79cc20b165fa11361f93621036c026b9ea7bf
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]1:[c:9]:[c:10]:[c:11](:[c:12]):[n;H0;D3;+0:13]:1-C(=O)-O-C(-C)(-C)-C>>[O;H0;D1;+0:1]=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]1:[c:9]:[c:10]:[c:11](:[c:12]):[nH;D2;+0:13]:1
58.1
[{"value": 58.1, "product": "CC1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
150
CELSIUS
null
null
50 mg 2-(3-Methoxy-6-pyridin-4-yl-pyridazin-4-yl)-3-methyl-indole-1-carboxylic acid tert-butyl ester is dissolved in 0.75 ml ethanol and 0.75 ml 1N aqueous NaOH solution. The reaction mixture is stirred at 150° C. in microwave apparatus (200 W). The solution is neutralized by addition of 1N HCl, the solvent removed und...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Boc
null
c1ccnnc1.c1cc2ccccc2[nH]1
c1cnncc1.c1ccc2[nH]ccc2c1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1
HO-
[OH-].[Na+].C(C)O
150
null
COc1nnc(-c2ccncc2)cc1-c1c(C)c2ccccc2n1C(=O)OC(C)(C)C>[OH-].[Na+].C(C)O>Cc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b41063aa5f564adfb8c58a590b17be0b
CC=O.COc1ccc(Cl)nn1>>COc1nnc(Cl)cc1C(C)O
Cl.C(C)=O.C(CCC)[Li].ClC=1N=NC(=CC1)OC.C([O-])(O)=O.[Na+].CC1(NC(CCC1)(C)C)C>>ClC1=CC(=C(N=N1)OC)C(C)O
[CH:10]([CH3:11])=[O:12].[CH3:1][O:2][c:3]1[n:4][n:5][c:6]([Cl:7])[cH:8][cH:9]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6]([Cl:7])[cH:8][c:9]1[CH:10]([CH3:11])[OH:12]
CC=O.COc1ccc(Cl)nn1
COc1nnc(Cl)cc1C(C)O
null
null
O1CCCC1.CCCCCC.C(C)O
C-C Coupling
OtherReaction
a27fffed4aaf6d2a30bf6b0df69ab017955ce9c7a44f21694f8a14adcbb193f6
a7cae52d902b2812376f5459a7a8b7ead54e8ef31fd78982d2e99bec532613ba
c1ccnnc1
[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](-[Cl;D1;H0:6]):[c:7]:[cH;D2;+0:8]:1.[C;D1;H3:9]-[CH;D2;+0:10]=[O;H0;D1;+0:11]>>[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](-[Cl;D1;H0:6]):[c:7]:[c;H0;D3;+0:8]:1-[CH;D3;+0:10](-[C;D1;H3:9])-[OH;D1;+0:11]
null
[]
0
CELSIUS
30
MINUTE
47.7 ml of a 1.6M solution of n-Butyl lithium in hexane is added dropwise at −75° C. to 100 ml tetrahydrofuran followed by 12.9 ml 2,2,6,6-tetramethylpiperidine and the resulting solution is allowed to warm to 0° C. and stirred for 30 min. The solution is cooled to −75° C. and a solution of 5 g 3-chloro-6-methoxypyrida...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Secondary alcohol
c1ccnnc1
c1ccnnc1
c1ccnnc1
null
O1CCCC1.CCCCCC.C(C)O
0
0.5
CC=O.COc1ccc(Cl)nn1>O1CCCC1.CCCCCC.C(C)O>COc1nnc(Cl)cc1C(C)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4e0a1926184942ec9626622b11249023
COc1nnc(Cl)cc1C(C)O>>COc1nnc(Cl)cc1C(C)=O
ClC1=CC(=C(N=N1)OC)C(C)O>>ClC1=CC(=C(N=N1)OC)C(C)=O
[CH3:1][O:2][c:3]1[n:4][n:5][c:6]([Cl:7])[cH:8][c:9]1[CH:10]([CH3:11])[OH:12]>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6]([Cl:7])[cH:8][c:9]1[C:10]([CH3:11])=[O:12]
COc1nnc(Cl)cc1C(C)O
COc1nnc(Cl)cc1C(C)=O
null
[O-2].[O-2].[Mn+4]
O1CCCC1
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
c7c20d2959ac48847b03cc1265962cf99a8ec8a85900c087dabb30077298c66c
767cfd93f5821ebb9e1e72addd9cb404b20b0c821d246ae6b87a5776b74a455b
c1ccnnc1
[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[CH;D3;+0:8](-[C;D1;H3:9])-[OH;D1;+0:10]>>[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[C;H0;D3;+0:8](-[C;D1;H3:9])=[O;H0;D1;+0:10]
null
[]
null
null
48
HOUR
3.85 g 1-(6-Chloro-3-methoxy-pyridazin-4-yl)-ethanol is dissolved in 300 ml tetrahydrofuran and 35.5 g of manganese dioxide is added. The reaction is stirred for 48 h at RT. Solids are removed by filtration, and the solvent is removed under reduced pressure. The product is purified and separated from 1-(3-chloro-6-meth...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
Ketone
null
null
c1ccnnc1
null
[O-2].[O-2].[Mn+4].O1CCCC1
null
48
COc1nnc(Cl)cc1C(C)O>[O-2].[O-2].[Mn+4].O1CCCC1>COc1nnc(Cl)cc1C(C)=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-37ce4e5a8ef842b18b2e9b12bd3cff77
COc1nnc(Cl)cc1C(C)=O.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O>>COc1nnc(-c2cc(C)c(O)c(C)c2)cc1C(C)=O
CC1=C(C(=CC(=C1)B1OC(C(O1)(C)C)(C)C)C)O.C([O-])([O-])=O.[Na+].[Na+].ClC1=CC(=C(N=N1)OC)C(C)=O>>OC1=C(C=C(C=C1C)C1=CC(=C(N=N1)OC)C(C)=O)C
Cl[c:6]1[n:5][n:4][c:3]([O:2][CH3:1])[c:17]([C:18]([CH3:19])=[O:20])[cH:16]1.CC1(C)OB([c:7]2[cH:8][c:9]([CH3:10])[c:11]([OH:12])[c:13]([CH3:14])[cH:15]2)OC1(C)C>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][c:9]([CH3:10])[c:11]([OH:12])[c:13]([CH3:14])[cH:15]2)[cH:16][c:17]1[C:18]([CH3:19])=[O:20]
COc1nnc(Cl)cc1C(C)=O.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1C(C)=O
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
COCCOC
C-C Coupling
Suzuki coupling with boronic esters
7d3abbda54e933df9ff9dc39c70f4c4ada1c268870f29590395c2cc6bed1dda1
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(-c2cccnn2)cc1
C-C1(-C)-O-B(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-O-C-1(-C)-C.Cl-[c;H0;D3;+0:6]1:[#7;a:7]:[#7;a:8]:[c:9]:[c:10](-[C:11](-[C;D1;H3:12])=[O;D1;H0:13]):[c:14]:1>>[C;D1;H3:12]-[C:11](=[O;D1;H0:13])-[c:10]1:[c:14]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[#7;a:7]:[#7;a:8]:[c:9]:1
null
[]
null
null
5
MINUTE
250 mg of 1-(6-Chloro-3-methoxy-pyridazin-4-yl)-ethanone and 232 mg of tetrakis(triphenylphosphine) palladium (0) are dissolved in 5 ml DME and the solution is stirred for 5 min at RT under argon. 400 mg of 2,6-Dimethyl-4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-phenol and 1.4 ml of a 2M aqueous solution of sodiu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1ccnnc1.B1OCCO1.c1ccccc1
c1ccnnc1.c1ccccc1
c1ccnnc1.c1ccccc1
HCl.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.COCCOC
null
0.083333
COc1nnc(Cl)cc1C(C)=O.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.COCCOC>COc1nnc(-c2cc(C)c(O)c(C)c2)cc1C(C)=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-752f5172a1dc4c88aa70e977aa30f488
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1C(C)=O.Nc1ccccc1Br>>COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1cc2ccccc2[nH]1
BrC1=C(N)C=CC=C1.S(=O)(=O)([O-])[O-].[Mg+2].OC1=C(C=C(C=C1C)C1=CC(=C(N=N1)OC)C(C)=O)C.C(C)(=O)O>>N1C(=CC2=CC=CC=C12)C=1C=C(N=NC1OC)C1=CC(=C(C(=C1)C)O)C
O=[C:18]([c:17]1[c:3]([O:2][CH3:1])[n:4][n:5][c:6](-[c:7]2[cH:8][c:9]([CH3:10])[c:11]([OH:12])[c:13]([CH3:14])[cH:15]2)[cH:16]1)[CH3:19].Br[c:20]1[cH:21][cH:22][cH:23][cH:24][c:25]1[NH2:26]>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][c:9]([CH3:10])[c:11]([OH:12])[c:13]([CH3:14])[cH:15]2)[cH:16][c:17]1-[c:18]1[cH:1...
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1C(C)=O.Nc1ccccc1Br
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1cc2ccccc2[nH]1
null
null
CC(=O)N(C)C
Aromatic Heterocycle Formation
OtherReaction
2aeebda70d28950751bcff9d93d27d409a496c19f9c9b9893349a271b234d219
4e13c013c1ec63cb4e4f791be1390f390c40f8fc080e4593325e7876241ac282
c1ccc(-c2cc(-c3cc4ccccc4[nH]3)cnn2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[NH2;D1;+0:5]):[c:6].O=[C;H0;D3;+0:7](-[CH3;D1;+0:8])-[c;H0;D3;+0:9]1:[c:10]:[c:11](-[c:12]):[#7;a:13]:[#7;a:14]:[c:15]:1-[#8:16]>>[#8:16]-[c:15]1:[#7;a:14]:[#7;a:13]:[c:11](-[c:12]):[c:10]:[c;H0;D3;+0:9]:1-[c;H0;D3;+0:7]1:[cH;D2;+0:8]:[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:6]):[n...
null
[]
140
CELSIUS
null
null
205 mg of 2-bromoaniline and 72 mg of anhydrous magnesium sulfate are suspended in 7 ml dimethylacetamide. 325 mg of 1-[6-(4-Hydroxy-3,5-dimethyl-phenyl)-3-methoxy-pyridazin-4-yl]-ethanone and 86.6 μl acetic acid are added and the reaction is degassed with argon. 330 mg of tripotassium phosphate and 61 mg of bis(tri-te...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ketone.Primary amine
null
c1ccccc1
c1ccc2[nH]ccc2c1
c1ccnnc1.c1ccccc1.c1ccc2[nH]ccc2c1
HBr
CC(=O)N(C)C
140
null
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1C(C)=O.Nc1ccccc1Br>CC(=O)N(C)C>COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1cc2ccccc2[nH]1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7463c8b27b9b45fe987dd3e1d903dce1
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1cc2ccccc2[nH]1>>Cc1cc(-c2cc(-c3cc4ccccc4[nH]3)c(=O)[nH]n2)cc(C)c1O
N1C(=CC2=CC=CC=C12)C=1C=C(N=NC1OC)C1=CC(=C(C(=C1)C)O)C.C[Si](C)(C)Cl.[I-].[K+].C[Si](C)(C)Cl.[I-].[K+]>>OC1=C(C=C(C=C1C)C=1C=C(C(NN1)=O)C=1NC2=CC=CC=C2C1)C
C[O:18][c:17]1[c:7](-[c:8]2[cH:9][c:10]3[cH:11][cH:12][cH:13][cH:14][c:15]3[nH:16]2)[cH:6][c:5](-[c:4]2[cH:3][c:2]([CH3:1])[c:24]([OH:25])[c:22]([CH3:23])[cH:21]2)[n:20][n:19]1>>[CH3:1][c:2]1[cH:3][c:4](-[c:5]2[cH:6][c:7](-[c:8]3[cH:9][c:10]4[cH:11][cH:12][cH:13][cH:14][c:15]4[nH:16]3)[c:17](=[O:18])[nH:19][n:20]2)[cH:...
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1cc2ccccc2[nH]1
Cc1cc(-c2cc(-c3cc4ccccc4[nH]3)c(=O)[nH]n2)cc(C)c1O
null
null
C(C)#N.O
Miscellaneous
OtherReaction
3a907fa62544f46964e2b473ab8a45caedf80503ce5e705ae3da44b55acc0eb2
291cad8b6dfbbd2c823b5c9d45efc37a166dc3454a9f151ac48cb357f4bc155f
O=c1[nH]nc(-c2ccccc2)cc1-c1cc2ccccc2[nH]1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]-[c:7]1:[c:6]:[c:5]:[#7;a:4]:[nH;D2;+0:3]:[c;H0;D3;+0:2]:1=[O;H0;D1;+0:1]
null
[]
80
CELSIUS
16
HOUR
100 mg of 4-[5-(1H-Indol-2-yl)-6-methoxy-pyridazin-3-yl]-2,6-dimethyl-phenol is suspended in 2 ml acetonitrile and 40 μl of trimethylsilyl chloride and 53 mg of potassium iodide are added. The solution is heated to 80° C. for 3h, then a further 120 μl of trimethylsilyl chloride and 159 mg of potassium iodide are added....
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccnnc1
c1cnncc1
c1ccccc1.c1cnncc1.c1ccc2[nH]ccc2c1
Other
C(C)#N.O
80
16
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1cc2ccccc2[nH]1>C(C)#N.O>Cc1cc(-c2cc(-c3cc4ccccc4[nH]3)c(=O)[nH]n2)cc(C)c1O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5c6a509c1e8d4e2fa4db8389032a13af
COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C>>COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
C(C)(C)(C)OC(=O)N1C(=CC2=CC=CC=C12)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.C(=O)(C(F)(F)F)O>>FC(C(=O)O)(F)F.COC=1N=NC(=CC1C=1NC2=CC=CC=C2C1)C1=CC=NC=C1
CC(C)(C)OC(=O)[n:23]1[c:15](-[c:14]2[c:3]([O:2][CH3:1])[n:4][n:5][c:6](-[c:7]3[cH:8][cH:9][n:10][cH:11][cH:12]3)[cH:13]2)[cH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]21>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1-[c:15]1[cH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]2[...
COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C
COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
null
null
ClCCl
Reduction
Boc amine deprotection
eefd4487d640b2607d7a60d065f8822bc457add01d643b9dbf7d76d9b4bfeca6
e1bf5a54b1f87284564f107662531aec2aff7de801e4606340967b38924afb28
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
C-C(-C)(-C)-O-C(=O)-[n;H0;D3;+0:1]1:[c:2](-[c:3]:[c:4]:[#7;a:5]):[c:6]:[c:7]:[c:8]:1:[c:9]>>[#7;a:5]:[c:4]:[c:3]-[c:2]1:[c:6]:[c:7]:[c:8](:[c:9]):[nH;D2;+0:1]:1
null
[]
null
null
null
null
A solution of 5.5 g 2-(3-Methoxy-6-pyridin-4-yl-pyridazin-4-yl)-indole-1-carboxylic acid tert-butyl ester and 5 ml TFA in 10 ml dichloromethane stirred for 18 h at room temperature. The solvent is evaporated and the crude product purified by suspended in water and collecting the precipitate. Conditions: See reaction.no...
10.6084/m9.figshare.5104873.v1
null
Ether.Boc
null
c1cc2ccccc2[nH]1
c1ccc2[nH]ccc2c1
c1ccnnc1.c1ccncc1.c1ccc2[nH]ccc2c1
HO-
ClCCl
null
null
COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2n1C(=O)OC(C)(C)C>ClCCl>COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-df37e54e99184edb875ff4a1fcc24cfb
COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I.OB(O)c1ccccc1>>COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1
OC(=O)C(F)(F)F.IC1=C(NC2=CC=CC=C12)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.C1(=CC=CC=C1)B(O)O.C([O-])([O-])=O.[K+].[K+].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>COC=1N=NC(=CC1C=1NC2=CC=CC=C2C1C1=CC=CC=C1)C1=CC=NC=C1
I[c:23]1[c:15](-[c:14]2[c:3]([O:2][CH3:1])[n:4][n:5][c:6](-[c:7]3[cH:8][cH:9][n:10][cH:11][cH:12]3)[cH:13]2)[nH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]21.OB(O)[c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1-[c:15]1[nH:16][c:17]2...
COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I.OB(O)c1ccccc1
COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
O.COCCOC.C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2c(-c3cnnc(-c4ccncc4)c3)[nH]c3ccccc23)cc1
I-[c;H0;D3;+0:1]1:[c:2](-[c:3]:[c:4]:[#7;a:5]):[#7;a:6]:[c:7](:[c:8]):[c:9]:1:[c:10].O-B(-O)-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]>>[#7;a:5]:[c:4]:[c:3]-[c:2]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[c;H0;D3;+0:1]:1-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]
null
[]
null
null
null
null
Argon is passed for 30 min through a suspension of 270 mg 3-Iodo-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-1H-indole TFA salt, 73 mg phenylboronic acid, 220 mg potassium carbonate and 52.4 mg triphenylphosphine in 2 ml DME and 1 ml water. 11.2 mg palladium (II) acetate is added and the mixture stirred under reflux fo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccnnc1.c1ccncc1.c1ccc2[nH]ccc2c1.c1ccccc1
HI.B
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.COCCOC.C(C)(=O)OCC
null
null
COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I.OB(O)c1ccccc1>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.COCCOC.C(C)(=O)OCC>COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-babd983aec834ea392fb32d0044e7696
COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1>>O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1
COC=1N=NC(=CC1C=1NC2=CC=CC=C2C1C1=CC=CC=C1)C1=CC=NC=C1.C(C)#N.O.C(=O)O>>C1(=CC=CC=C1)C1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O
C[O:1][c:2]1[n:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[nH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[c:22]1-[c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[nH:15][c:16]2[cH:17][cH:18][cH:19][c...
COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1
O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1
null
null
[OH-].[Na+].C(C)O
Miscellaneous
OtherReaction
3a907fa62544f46964e2b473ab8a45caedf80503ce5e705ae3da44b55acc0eb2
291cad8b6dfbbd2c823b5c9d45efc37a166dc3454a9f151ac48cb357f4bc155f
O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]-[c:7]1:[c:6]:[c:5]:[#7;a:4]:[nH;D2;+0:3]:[c;H0;D3;+0:2]:1=[O;H0;D1;+0:1]
null
[]
150
CELSIUS
null
null
63 mg 2-(3-Methoxy-6-pyridin-4-yl-pyridazin-4-yl)-3-phenyl-1H-indole is dissolved in 0.75 ml ethanol and 0.75 ml 1N aqueous NaOH solution. The reaction mixture is stirred at 150° C. in microwave apparatus (200 W). The reaction mixture is directly applied to HPLC chromatography to isolate the product (RP18 column, aceto...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccnnc1
c1cnncc1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1.c1ccccc1
Other
[OH-].[Na+].C(C)O
150
null
COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1>[OH-].[Na+].C(C)O>O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b5645a3c8db242f59d774cd41912d028
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I>>C=Cc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12
IC1=C(NC2=CC=CC=C12)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.C(CCC)[Sn](C=C)(CCCC)CCCC.CCOC(=O)C.[F-].[K+]>>COC=1N=NC(=CC1C=1NC2=CC=CC=C2C1C=C)C1=CC=NC=C1
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[CH:2]=[CH2:1].I[c:3]1[c:4](-[c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][n:11][cH:12][cH:13]3)[n:14][n:15][c:16]2[O:17][CH3:18])[nH:19][c:20]2[cH:21][cH:22][cH:23][cH:24][c:25]12>>[CH2:1]=[CH:2][c:3]1[c:4](-[c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][n:11][cH:12][cH:13]3)[n:14][n:15][c:16]2[O:17][...
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I
C=Cc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12
null
[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
CN(C)C=O
C-C Coupling
Stille reaction_vinyl
f4ad649c74b7a6a35b0e84610492e238d5241d8eaf0ab45cca5db093924b7eac
ec03c739f58696d2a3659a73884744e1a490a20a587da6f115be382b663cf23d
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[CH;D2;+0:1]=[C;D1;H2:2].I-[c;H0;D3;+0:3]1:[c:4](:[c:5]):[c:6](:[c:7]):[#7;a:8]:[c:9]:1-[c:10]:[c:11]:[#7;a:12]>>[#7;a:12]:[c:11]:[c:10]-[c:9]1:[#7;a:8]:[c:6](:[c:7]):[c:4](:[c:5]):[c;H0;D3;+0:3]:1-[CH;D2;+0:1]=[C;D1;H2:2]
null
[]
80
CELSIUS
40
MINUTE
A mixture of 430 mg 3-Iodo-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-1H-indole, 490 mg tributyl(vinyl)tin, 165 mg tetraethylammonium-chloride and 35 mg bis(triphenylphosphine)palladium(II) chloride in DMF is stirred at 80° C. for 40 min. After cooling to room temperature, 15 ml aqueous potassium fluoride solution (30...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl.Tin
Vinyl
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccnnc1.c1ccncc1.c1ccc2[nH]ccc2c1
HI.Sn
[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O
80
0.666667
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.COc1nnc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I>[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O>C=Cc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-33ec444488544a8ebe118ee0146cd0ef
C=CC1c2ccccc2NC1(CO)c1cc(-c2ccncc2)nnc1OC>>CCc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12
COC=1N=NC(=CC1C1(NC2=CC=CC=C2C1C=C)CO)C1=CC=NC=C1>>C(C)C1=C(NC2=CC=CC=C12)C1=C(N=NC(=C1)C1=CC=NC=C1)OC
OC[C:4]1([c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][n:11][cH:12][cH:13]3)[n:14][n:15][c:16]2[O:17][CH3:18])[CH:3]([CH:2]=[CH2:1])[c:25]2[c:20]([cH:21][cH:22][cH:23][cH:24]2)[NH:19]1>>[CH3:1][CH2:2][c:3]1[c:4](-[c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][n:11][cH:12][cH:13]3)[n:14][n:15][c:16]2[O:17][CH3:18])[nH:19][c:20]2[cH:21...
C=CC1c2ccccc2NC1(CO)c1cc(-c2ccncc2)nnc1OC
CCc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12
null
[Pd]
null
Functional Group Interconversion
OtherReaction
b6d4453beea49d45807241e91d8288d0f248f4f4d05bbfb442e2a8540fe98ed6
b5345ac429e84e6be0df234cae5011cf4e71e4da6aa7f89ad313e9a0722024e2
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
O-C-[C;H0;D4;+0:1]1(-[c;H0;D3;+0:2]2:[c:3]:[c:4](-[c:5]):[#7;a:6]:[#7;a:7]:[c:8]:2-[#8:9])-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13](:[c:14])-[CH;D3;+0:15]-1-[CH;D2;+0:16]=[CH2;D1;+0:17]>>[#8:9]-[c:8]1:[#7;a:7]:[#7;a:6]:[c:4](-[c:5]):[c:3]:[c;H0;D3;+0:2]:1-[c;H0;D3;+0:1]1:[nH;D2;+0:10]:[c:11](:[c:12]):[c:13](:[c:14]):[c;H0;...
null
[]
null
null
4
HOUR
12 mg Palladium, 10% on charcoal are added to a solution of 70 mg 2-(3-Methoxy-6-pyridin-4-yl-pyridazin-4-yl)-3-vinyl-1H-indole methanol, and the reaction mixture is stirred under an hydrogen atmosphere for 4 hours. The catalyst is removed by filtration and the solvent by evaporation yielding the product which was used...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Secondary amine.Vinyl
null
c1ccc2c(c1)CCN2
c1ccc2[nH]ccc2c1
c1ccnnc1.c1ccncc1.c1ccc2[nH]ccc2c1
HO-
[Pd]
null
4
C=CC1c2ccccc2NC1(CO)c1cc(-c2ccncc2)nnc1OC>[Pd]>CCc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-abda347c2ef249bc8915db008f19ce56
CCc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12>>CCc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
C(C)C1=C(NC2=CC=CC=C12)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.C(C)#N.O.C(=O)O>>C(C)C1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O
C[O:17][c:16]1[c:5](-[c:4]2[c:3]([CH2:2][CH3:1])[c:24]3[c:19]([nH:18]2)[cH:20][cH:21][cH:22][cH:23]3)[cH:6][c:7](-[c:8]2[cH:9][cH:10][n:11][cH:12][cH:13]2)[n:14][n:15]1>>[CH3:1][CH2:2][c:3]1[c:4](-[c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][n:11][cH:12][cH:13]3)[n:14][nH:15][c:16]2=[O:17])[nH:18][c:19]2[cH:20][cH:21][cH:22]...
CCc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12
CCc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
null
null
[OH-].[Na+].C(C)O
Miscellaneous
OtherReaction
3a907fa62544f46964e2b473ab8a45caedf80503ce5e705ae3da44b55acc0eb2
291cad8b6dfbbd2c823b5c9d45efc37a166dc3454a9f151ac48cb357f4bc155f
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]-[c:7]1:[c:6]:[c:5]:[#7;a:4]:[nH;D2;+0:3]:[c;H0;D3;+0:2]:1=[O;H0;D1;+0:1]
null
[]
150
CELSIUS
null
null
60 mg 3-Ethyl-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-1H-indole is dissolved in 0.5 ml ethanol and 0.5 ml 1N aqueous NaOH solution. The reaction mixture is stirred at 150° C. in microwave apparatus (200 W). The reaction mixture is directly applied to HPLC chromatography to isolate the product (RP18 column, acetonit...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccnnc1
c1cnncc1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1
Other
[OH-].[Na+].C(C)O
150
null
CCc1c(-c2cc(-c3ccncc3)nnc2OC)[nH]c2ccccc12>[OH-].[Na+].C(C)O>CCc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-259b42023b664515a996f4294d8c1ae5
C1COCCN1.C=O.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1>>O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1CN1CCOCC1
[OH-].[Na+].C=O.N1CCOCC1.N1C(=CC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O>>N1(CCOCC1)CC1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O
[NH:24]1[CH2:25][CH2:26][O:27][CH2:28][CH2:29]1.O=[CH2:23].[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[nH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[cH:22]1>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[nH:15][c:16]2[cH:17...
C1COCCN1.C=O.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1CN1CCOCC1
null
null
O1CCOCC1.C(C)(=O)O
Heteroatom Alkylation and Arylation
OtherReaction
8fe770f617c873b341268f271197203396fa684d2848d3c06932569abea4d8be
e1fdef8fde1c506d7c9deb8fd5e6f322eceea2abce3167abcf412a1fa4fd5443
O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1CN1CCOCC1
O=[CH2;D1;+0:1].[#7;a:2]:[c:3]:[c:4]-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[cH;D2;+0:11]:1.[#8:12]1-[C:13]-[C:14]-[NH;D2;+0:15]-[C:16]-[C:17]-1>>[#7;a:2]:[c:3]:[c:4]-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[c;H0;D3;+0:11]:1-[CH2;D2;+0:1]-[N;H0;D3;+0:15]1-[C:14]-[C:13]-[#8:12]-[C:17]-[C:16]-1
null
[]
null
null
3
HOUR
A solution of 14 ul formaldehyde (37% solution in water) and 17 ul morpholine in 0.5 ml glacial acetic acid is added dropwise at 0° C. to 50 mg 4-(1H-Indol-2-yl)-6-pyridin-4-yl-2H-pyridazin-3-one suspended in 2.24 ml glacial acetic acid and 2.6 ml 1,4-Dioxan. The resulting mixture is stirred for 3 h at room temperature...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Secondary amine
Tertiary amine
C1COCCN1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.C1COCC[NH]1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1.C1COCC[NH]1
HO-
O1CCOCC1.C(C)(=O)O
null
3
C1COCCN1.C=O.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1>O1CCOCC1.C(C)(=O)O>O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1CN1CCOCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2d7ada8edbb44b57bbc24d685b7e8e78
O=C1CCC(=O)N1Br.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1>>O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1Br
N1C(=CC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O.BrN1C(CCC1=O)=O>>BrC1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O
O=C1CCC(=O)N1[Br:23].[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[nH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[cH:22]1>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[nH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[c:22]1[B...
O=C1CCC(=O)N1Br.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1Br
null
null
CC(=O)C
Functional Group Interconversion
Bromination
0754ae2664ff7ba9610e6f272707033ed8b7278ddd1c23d9264359692cf74d77
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[c:3]:[c:4]-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[cH;D2;+0:11]:1>>[#7;a:2]:[c:3]:[c:4]-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[c;H0;D3;+0:11]:1-[Br;H0;D1;+0:1]
null
[]
null
null
3
HOUR
22 mg 4-(1H-Indol-2-yl)-6-pyridin-4-yl-2H-pyridazin-3-one is suspended in 30 mL acetone and 2 mg N-bromosuccinimide is added. The reaction mixture is stirred for 3 hours at room temperature, the precipitated product isolated by filtration and washed with acetone. The product is purified by preparative RP-HPLC eluting w...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
C1CCNC1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1
HO-
CC(=O)C
null
3
O=C1CCC(=O)N1Br.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1>CC(=O)C>O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ef0d5160087c40a19b5856f0bc9e8161
CC=O.COc1ccc(-c2ccncc2)nn1>>COc1nnc(-c2ccncc2)cc1C(C)O
C(C)=O.COC=1N=NC(=CC1)C1=CC=NC=C1.CC1(NC(CCC1)(C)C)C.C(CCC)[Li]>>COC=1N=NC(=CC1C(C)O)C1=CC=NC=C1
[CH:15]([CH3:16])=[O:17].[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][cH:14]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1[CH:15]([CH3:16])[OH:17]
CC=O.COc1ccc(-c2ccncc2)nn1
COc1nnc(-c2ccncc2)cc1C(C)O
null
null
C1CCOC1
C-C Coupling
OtherReaction
a27fffed4aaf6d2a30bf6b0df69ab017955ce9c7a44f21694f8a14adcbb193f6
a7cae52d902b2812376f5459a7a8b7ead54e8ef31fd78982d2e99bec532613ba
c1cnnc(-c2ccncc2)c1
[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](-[c:6]):[c:7]:[cH;D2;+0:8]:1.[C;D1;H3:9]-[CH;D2;+0:10]=[O;H0;D1;+0:11]>>[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](-[c:6]):[c:7]:[c;H0;D3;+0:8]:1-[CH;D3;+0:10](-[C;D1;H3:9])-[OH;D1;+0:11]
66
[{"value": 66.0, "product": "COC=1N=NC(=CC1C(C)O)C1=CC=NC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.8, "product": "COC=1N=NC(=CC1C(C)O)C1=CC=NC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
To a solution of 0.93 g 2,2,6,6-tetramethylpiperidine in 30 ml THF is added 4.13 ml (15% solution in toluene) n-butyllithium at −30° C. After being stirred at 0° C. for 30 min, the reaction mixture is cooled to −78° C. and a solution of 1.12 g 3-methoxy-6-pyridin-4-yl-pyridazine in 30 ml THF is added and stirred at −78...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Secondary alcohol
c1ccnnc1
c1ccnnc1
c1ccnnc1.c1ccncc1
null
C1CCOC1
0
0.5
CC=O.COc1ccc(-c2ccncc2)nn1>C1CCOC1>COc1nnc(-c2ccncc2)cc1C(C)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fda2ba8339ae49b3950cb537d1f4f04f
COc1nnc(-c2ccncc2)cc1C(C)O>>COc1nnc(-c2ccncc2)cc1C(C)=O
COC=1N=NC(=CC1C(C)O)C1=CC=NC=C1.CC(=O)OI1(C2=CC=CC=C2C(=O)O1)(OC(=O)C)OC(=O)C>>COC=1N=NC(=CC1C(C)=O)C1=CC=NC=C1
[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1[CH:15]([CH3:16])[OH:17]>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1[C:15]([CH3:16])=[O:17]
COc1nnc(-c2ccncc2)cc1C(C)O
COc1nnc(-c2ccncc2)cc1C(C)=O
null
null
C(Cl)Cl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
c7c20d2959ac48847b03cc1265962cf99a8ec8a85900c087dabb30077298c66c
767cfd93f5821ebb9e1e72addd9cb404b20b0c821d246ae6b87a5776b74a455b
c1cnnc(-c2ccncc2)c1
[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[CH;D3;+0:8](-[C;D1;H3:9])-[OH;D1;+0:10]>>[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[C;H0;D3;+0:8](-[C;D1;H3:9])=[O;H0;D1;+0:10]
92
[{"value": 92.0, "product": "COC=1N=NC(=CC1C(C)=O)C1=CC=NC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.0, "product": "COC=1N=NC(=CC1C(C)=O)C1=CC=NC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a solution of 0.91 g 1-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-ethanol in 10 ml CH2Cl2 is added a suspension of 1.70 g Dess-Martin Periodane in 10 ml CH2Cl2 at room temperature. After being stirred for 3 h, the suspension is extracted with 5% aq. Na2S2O3 solution. The organic layer is washed with water, dried over...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
Ketone
null
null
c1ccnnc1.c1ccncc1
null
C(Cl)Cl
null
3
COc1nnc(-c2ccncc2)cc1C(C)O>C(Cl)Cl>COc1nnc(-c2ccncc2)cc1C(C)=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-30d999d6d5da476a805d170eef6c17db
COc1nnc(-c2ccncc2)cc1-c1cc2cc(C(C)C)ccc2[nH]1>>CC(C)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)cc2c1
C(C)(C)C=1C=C2C=C(NC2=CC1)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.[OH-].[Na+]>>C(C)(C)C=1C=C2C=C(NC2=CC1)C=1C(NN=C(C1)C1=CC=NC=C1)=O
C[O:22][c:21]1[c:10](-[c:9]2[nH:8][c:7]3[cH:6][cH:5][c:4]([CH:2]([CH3:1])[CH3:3])[cH:25][c:24]3[cH:23]2)[cH:11][c:12](-[c:13]2[cH:14][cH:15][n:16][cH:17][cH:18]2)[n:19][n:20]1>>[CH3:1][CH:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]2[nH:8][c:9](-[c:10]3[cH:11][c:12](-[c:13]4[cH:14][cH:15][n:16][cH:17][cH:18]4)[n:19][nH:20][c:21]...
COc1nnc(-c2ccncc2)cc1-c1cc2cc(C(C)C)ccc2[nH]1
CC(C)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)cc2c1
null
null
CCO
Miscellaneous
OtherReaction
3a907fa62544f46964e2b473ab8a45caedf80503ce5e705ae3da44b55acc0eb2
291cad8b6dfbbd2c823b5c9d45efc37a166dc3454a9f151ac48cb357f4bc155f
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]-[c:7]1:[c:6]:[c:5]:[#7;a:4]:[nH;D2;+0:3]:[c;H0;D3;+0:2]:1=[O;H0;D1;+0:1]
11
[{"value": 11.0, "product": "C(C)(C)C=1C=C2C=C(NC2=CC1)C=1C(NN=C(C1)C1=CC=NC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 10.5, "product": "C(C)(C)C=1C=C2C=C(NC2=CC1)C=1C(NN=C(C1)C1=CC=NC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
150
CELSIUS
null
null
To a solution of 139 mg (crude material) 5-isopropyl-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-1H-indole in 2.5 ml EtOH is added 2.5 ml aq. NaOH (1 M). The mixture is heated for 10 min at 150° C. using microwave. After cooling to room temperature the mixture is filtered and purified by HPLC to give 14 mg (11%) of the...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccnnc1
c1cnncc1
c1ccc2[nH]ccc2c1.c1cnncc1.c1ccncc1
Other
CCO
150
null
COc1nnc(-c2ccncc2)cc1-c1cc2cc(C(C)C)ccc2[nH]1>CCO>CC(C)c1ccc2[nH]c(-c3cc(-c4ccncc4)n[nH]c3=O)cc2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-24a8127de3a04e3592f183c34bbe44e8
CC(=O)Cl.COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1>>CC(=O)c1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
C(C)(=O)Cl.ClCCCl.[Cl-].[Al+3].[Cl-].[Cl-].FC(C(=O)O)(F)F.COC=1N=NC(=CC1C=1NC2=CC=CC=C2C1)C1=CC=NC=C1>>C(C)(=O)C1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O
Cl[C:2]([CH3:1])=[O:3].C[O:18][c:17]1[c:6](-[c:5]2[cH:4][c:25]3[c:20]([nH:19]2)[cH:21][cH:22][cH:23][cH:24]3)[cH:7][c:8](-[c:9]2[cH:10][cH:11][n:12][cH:13][cH:14]2)[n:15][n:16]1>>[CH3:1][C:2](=[O:3])[c:4]1[c:5](-[c:6]2[cH:7][c:8](-[c:9]3[cH:10][cH:11][n:12][cH:13][cH:14]3)[n:15][nH:16][c:17]2=[O:18])[nH:19][c:20]2[cH:2...
CC(=O)Cl.COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
CC(=O)c1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
null
null
null
Acylation
OtherReaction
20b7fe8fa1eec589fd08a2a4fea071d764dc4c09cfad5a5fb1f99f7540bb4b04
404ac493a92648b12d897060b845969d840d30aa4e379815a25f94ff447379d8
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]1:[#7;a:9]:[c:10](:[c:11]):[c:12](:[c:13]):[cH;D2;+0:14]:1.Cl-[C;H0;D3;+0:15](-[C;D1;H3:16])=[O;D1;H0:17]>>[C;D1;H3:16]-[C;H0;D3;+0:15](=[O;D1;H0:17])-[c;H0;D3;+0:14]1:[c:12](:[c:13]):[c:10](:[c:11]):[#7;a:9]:[c:8]:1-[c:7]1:[c:6]:[c:5]:[#...
48.1
[{"value": 48.1, "product": "C(C)(=O)C1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
4 mg acetyl chloride are added at 0° C. to a suspension of 80 mg aluminum chloride 1,2-Dichloroethane, followed by 208 mg 2-(3-Methoxy-6-pyridin-4-yl-pyridazin-4-yl)-1H-indole Trifluoroacetate. The reaction mixture is stirred for 4 h at room temperature and for 3h at 50° C. It is worked up pouring into an ice/water mix...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether
Ketone
c1ccnnc1.c1ccc2[nH]ccc2c1
c1cnncc1.c1ccc2[nH]ccc2c1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1
HCl
null
null
null
CC(=O)Cl.COc1nnc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1>>CC(=O)c1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9e5fc3ac1d3a4b60b4e53322e78f8a86
CC(C)(C)[Si](C)(C)Cl.Oc1ccc2cc[nH]c2c1>>CC(C)(C)[Si](C)(C)Oc1ccc2cc[nH]c2c1
OC1=CC=C2C=CNC2=C1.[Si](C)(C)(C(C)(C)C)Cl.N1C=NC=C1.CN(C=O)C>>O([Si](C)(C)C(C)(C)C)C1=CC=C2C=CNC2=C1
Cl[Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7].[OH:8][c:9]1[cH:10][cH:11][c:12]2[cH:13][cH:14][nH:15][c:16]2[cH:17]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][c:9]1[cH:10][cH:11][c:12]2[cH:13][cH:14][nH:15][c:16]2[cH:17]1
CC(C)(C)[Si](C)(C)Cl.Oc1ccc2cc[nH]c2c1
CC(C)(C)[Si](C)(C)Oc1ccc2cc[nH]c2c1
null
null
C(C)(=O)OCC
Protection
Alcohol protection with silyl ethers
91043baed1393f1ecd2302d7d0b31c01cf171d3977dd7c70afa1da52fa298c73
4a917c959d011f885a1269fa3c1f022ee5e09144996246d24e42e65634a451ac
c1ccc2[nH]ccc2c1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[#7;a:8]:[c:9]:[c:10]:[c:11](-[OH;D1;+0:12]):[c:13]>>[#7;a:8]:[c:9]:[c:10]:[c:11](-[O;H0;D2;+0:12]-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7]):[c:13]
88.6
[{"value": 88.0, "product": "O([Si](C)(C)C(C)(C)C)C1=CC=C2C=CNC2=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.6, "product": "O([Si](C)(C)C(C)(C)C)C1=CC=C2C=CNC2=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
HOUR
A mixture of 5.5 g 6-hydroxyindole, 7.47 g tert-butyldimethylsilyl chloride, 7.03 g imidazole, and 25 mL dimethylformamide is stirred at ambient temperature for 20 h. The reaction is diluted with ethyl acetate, washed with water (2×), dried (MgSO4), and the solvent removed under reduced pressure to provide an oil. The ...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol.Silyl protective group
TMS ether protective group
null
null
c1ccc2[nH]ccc2c1
HCl
C(C)(=O)OCC
null
20
CC(C)(C)[Si](C)(C)Cl.Oc1ccc2cc[nH]c2c1>C(C)(=O)OCC>CC(C)(C)[Si](C)(C)Oc1ccc2cc[nH]c2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bcaa333902f44bb3aba5645c7b8da4fa
CC(C)(C)OC(=O)n1ccc2ccc(O[Si](C)(C)C(C)(C)C)cc21>>CC(C)(C)OC(=O)n1c(B(O)O)cc2ccc(O[Si](C)(C)C(C)(C)C)cc21
[Cl-].[NH4+].COB(OC)OC.C(C)(C)(C)OC(=O)N1C=CC2=CC=C(C=C12)O[Si](C)(C)C(C)(C)C.C(C)(C)(C)[Li].OS(=O)(=O)[O-].[K+].OS(=O)(=O)O>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)O[Si](C)(C)C(C)(C)C)B(O)O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[n:8]1[cH:9][cH:13][c:14]2[cH:15][cH:16][c:17]([O:18][Si:19]([CH3:20])([CH3:21])[C:22]([CH3:23])([CH3:24])[CH3:25])[cH:26][c:27]12>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[n:8]1[c:9]([B:10]([OH:11])[OH:12])[cH:13][c:14]2[cH:15][cH:16][c:17]([O:18][Si:19]([CH3:20]...
CC(C)(C)OC(=O)n1ccc2ccc(O[Si](C)(C)C(C)(C)C)cc21
CC(C)(C)OC(=O)n1c(B(O)O)cc2ccc(O[Si](C)(C)C(C)(C)C)cc21
null
null
O1CCCC1.CCOCC.CCCCC
Functional Group Interconversion
OtherReaction
4b0e6aa4d1fd1c5214dd3931ca16cd67f94912c719f614bc8380822d6ecd3d94
d6d312d46f766d2774f96de1fd96fd8f98a20e51a20ef3280f850cd6a3c77869
c1ccc2[nH]ccc2c1
[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C:6](=[O;D1;H0:7])-[#7;a:8]1:[c:9]:[c:10]:[c:11]:[cH;D2;+0:12]:1>>[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C:6](=[O;D1;H0:7])-[#7;a:8]1:[c:9]:[c:10]:[c:11]:[c;H0;D3;+0:12]:1-[#5:13](-[O;D1;H1:14])-[O;D1;H1:15]
56
[{"value": 56.0, "product": "C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)O[Si](C)(C)C(C)(C)C)B(O)O", "details": "PERCENTYIELD", "is_desired": false}]
78
CELSIUS
32
MINUTE
To a solution of 1 g 1-(tert-butoxycarbonyl)-6-(tert-butyldimethylsiloxy)indole in 15 mL anhydrous tetrahydrofuran at −78° C. under nitrogen is added tert-butyllithium (2.30 mL of a 1.5 M solution in pentane) over 3 min, and the reaction is stirred at ˜78° C. After 32 min, 0.66 mL trimethylborate are added in one porti...
10.6084/m9.figshare.5104873.v1
null
null
Boronic acid
c1ccc2cc[nH]c2c1
c1ccc2cc[nH]c2c1
c1ccc2cc[nH]c2c1
null
O1CCCC1.CCOCC.CCCCC
78
0.533333
CC(C)(C)OC(=O)n1ccc2ccc(O[Si](C)(C)C(C)(C)C)cc21>O1CCCC1.CCOCC.CCCCC>CC(C)(C)OC(=O)n1c(B(O)O)cc2ccc(O[Si](C)(C)C(C)(C)C)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5b2c326aaee243048156ce6181409011
CN(C)CCO.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(O)cc2n1C(=O)OC(C)(C)C>>COc1nnc(-c2ccncc2)cc1-c1cc2ccc(OCCN(C)C)cc2n1C(=O)OC(C)(C)C
C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.CN(CCO)C.N(=NC(=O)OCC)C(=O)OCC>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)OCCN(C)C)C1=C(N=NC(=C1)C1=CC=NC=C1)OC
O[CH2:22][CH2:23][N:24]([CH3:25])[CH3:26].[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1-[c:15]1[cH:16][c:17]2[cH:18][cH:19][c:20]([OH:21])[cH:27][c:28]2[n:29]1[C:30](=[O:31])[O:32][C:33]([CH3:34])([CH3:35])[CH3:36]>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][...
CN(C)CCO.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(O)cc2n1C(=O)OC(C)(C)C
COc1nnc(-c2ccncc2)cc1-c1cc2ccc(OCCN(C)C)cc2n1C(=O)OC(C)(C)C
null
null
C1(=CC=CC=C1)C.C1CCOC1
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
86bfb73617450d22f9456ed5ce4d96a73f1f8fc0c016bebae57fda68e2da86a2
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
O-[CH2;D2;+0:1]-[C:2]-[#7:3].[#7;a:4]:[c:5]:[c:6]:[c:7](-[OH;D1;+0:8]):[c:9]>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:8]-[c:7](:[c:9]):[c:6]:[c:5]:[#7;a:4]
43
[{"value": 43.0, "product": "C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)OCCN(C)C)C1=C(N=NC(=C1)C1=CC=NC=C1)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
100 mg 6-hydroxy-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-indole-1-carboxylic acid tert-butyl ester and 175 mg triphenylphosphine are dissolved in 7 mL toluene and 2 mL THF. After dropwise addition of 84 μL 2-dimethylaminoethanol and 123 μL diethyl azodicarboxylate, the reaction mixture is stirred at room temperatur...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
null
null
c1ccnnc1.c1ccncc1.c1ccc2cc[nH]c2c1
HO-
C1(=CC=CC=C1)C.C1CCOC1
null
5
CN(C)CCO.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(O)cc2n1C(=O)OC(C)(C)C>C1(=CC=CC=C1)C.C1CCOC1>COc1nnc(-c2ccncc2)cc1-c1cc2ccc(OCCN(C)C)cc2n1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eb075f340d53495fa1b59f44d7390793
CCC=O.COc1ccc(Cl)nn1>>CCC(O)c1cc(Cl)nnc1OC
Cl.C(CC)=O.C(CCC)[Li].ClC=1N=NC(=CC1)OC.C([O-])(O)=O.[Na+].CC1(NC(CCC1)(C)C)C>>ClC1=CC(=C(N=N1)OC)C(CC)O
[CH3:1][CH2:2][CH:3]=[O:4].[cH:5]1[cH:6][c:7]([Cl:8])[n:9][n:10][c:11]1[O:12][CH3:13]>>[CH3:1][CH2:2][CH:3]([OH:4])[c:5]1[cH:6][c:7]([Cl:8])[n:9][n:10][c:11]1[O:12][CH3:13]
CCC=O.COc1ccc(Cl)nn1
CCC(O)c1cc(Cl)nnc1OC
null
null
O1CCCC1.CCCCCC.C(C)O
C-C Coupling
OtherReaction
a27fffed4aaf6d2a30bf6b0df69ab017955ce9c7a44f21694f8a14adcbb193f6
a7cae52d902b2812376f5459a7a8b7ead54e8ef31fd78982d2e99bec532613ba
c1ccnnc1
[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](-[Cl;D1;H0:6]):[c:7]:[cH;D2;+0:8]:1.[C;D1;H3:9]-[C:10]-[CH;D2;+0:11]=[O;H0;D1;+0:12]>>[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](-[Cl;D1;H0:6]):[c:7]:[c;H0;D3;+0:8]:1-[CH;D3;+0:11](-[OH;D1;+0:12])-[C:10]-[C;D1;H3:9]
null
[]
0
CELSIUS
30
MINUTE
104.6 ml of a 1.6M solution of n-Butyl lithium in hexane is added dropwise at −75° C. to 200 ml tetrahydrofuran followed by 28.3 ml 2,2,6,6-tetramethylpiperidine and the resulting solution is allowed to warm to 0° C. and stirred for 30 min. The solution is cooled to −75° C. and a solution of 11 g 3-chloro-6-methoxypyri...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Secondary alcohol
c1ccnnc1
c1ccnnc1
c1ccnnc1
null
O1CCCC1.CCCCCC.C(C)O
0
0.5
CCC=O.COc1ccc(Cl)nn1>O1CCCC1.CCCCCC.C(C)O>CCC(O)c1cc(Cl)nnc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-695cb214ce6b4accb0e739d2448d5410
CCC(O)c1cc(Cl)nnc1OC>>CCC(=O)c1cc(Cl)nnc1OC
ClC1=CC(=C(N=N1)OC)C(CC)O>>ClC1=CC(=C(N=N1)OC)C(CC)=O
[CH3:1][CH2:2][CH:3]([OH:4])[c:5]1[cH:6][c:7]([Cl:8])[n:9][n:10][c:11]1[O:12][CH3:13]>>[CH3:1][CH2:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([Cl:8])[n:9][n:10][c:11]1[O:12][CH3:13]
CCC(O)c1cc(Cl)nnc1OC
CCC(=O)c1cc(Cl)nnc1OC
null
[O-2].[O-2].[Mn+4]
O1CCCC1
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
c7c20d2959ac48847b03cc1265962cf99a8ec8a85900c087dabb30077298c66c
767cfd93f5821ebb9e1e72addd9cb404b20b0c821d246ae6b87a5776b74a455b
c1ccnnc1
[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[CH;D3;+0:8](-[OH;D1;+0:9])-[C:10]-[C;D1;H3:11]>>[#8:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[C;H0;D3;+0:8](=[O;H0;D1;+0:9])-[C:10]-[C;D1;H3:11]
null
[]
null
null
24
HOUR
12.25 g 1-(6-Chloro-3-methoxy-pyridazin-4-yl)-propan-1-ol is dissolved in 410 ml tetrahydrofuran and 105 g of manganese dioxide is added. The reaction is stirred for 24 h at RT. Solids are removed by filtration, and the solution is treated with a further 105 g of manganese dioxide for 16 h at RT. Solids are removed by ...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
Ketone
null
null
c1ccnnc1
null
[O-2].[O-2].[Mn+4].O1CCCC1
null
24
CCC(O)c1cc(Cl)nnc1OC>[O-2].[O-2].[Mn+4].O1CCCC1>CCC(=O)c1cc(Cl)nnc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-43eba2caeef14a1ea548eb0145350cad
CCC(=O)c1cc(Cl)nnc1OC.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O>>CCC(=O)c1cc(-c2cc(C)c(O)c(C)c2)nnc1OC
CC1=C(C(=CC(=C1)B1OC(C(O1)(C)C)(C)C)C)O.C([O-])([O-])=O.[Na+].[Na+].C(C)(=O)OCC.ClC1=CC(=C(N=N1)OC)C(CC)=O>>OC1=C(C=C(C=C1C)C1=CC(=C(N=N1)OC)C(CC)=O)C
Cl[c:7]1[cH:6][c:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:19]([O:20][CH3:21])[n:18][n:17]1.CC1(C)OB([c:8]2[cH:9][c:10]([CH3:11])[c:12]([OH:13])[c:14]([CH3:15])[cH:16]2)OC1(C)C>>[CH3:1][CH2:2][C:3](=[O:4])[c:5]1[cH:6][c:7](-[c:8]2[cH:9][c:10]([CH3:11])[c:12]([OH:13])[c:14]([CH3:15])[cH:16]2)[n:17][n:18][c:19]1[O:20][CH3:21]
CCC(=O)c1cc(Cl)nnc1OC.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O
CCC(=O)c1cc(-c2cc(C)c(O)c(C)c2)nnc1OC
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
COCCOC
C-C Coupling
Suzuki coupling with boronic esters
7d3abbda54e933df9ff9dc39c70f4c4ada1c268870f29590395c2cc6bed1dda1
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(-c2cccnn2)cc1
C-C1(-C)-O-B(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-O-C-1(-C)-C.Cl-[c;H0;D3;+0:6]1:[#7;a:7]:[#7;a:8]:[c:9]:[c:10](-[C:11]=[O;D1;H0:12]):[c:13]:1>>[O;D1;H0:12]=[C:11]-[c:10]1:[c:9]:[#7;a:8]:[#7;a:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:13]:1
null
[]
null
null
5
MINUTE
2 g of 1-(6-Chloro-3-methoxy-pyridazin-4-yl)-propan-1-one and 1.73 g of tetrakis(triphenylphosphine) palladium (0) are dissolved in 10 ml DME and the solution is stirred for 5 min at RT under argon. 3 g of 2,6-Dimethyl-4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-phenol and 10 ml of a 2M aqueous solution of sodium ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1ccnnc1.B1OCCO1.c1ccccc1
c1ccnnc1.c1ccccc1
c1ccnnc1.c1ccccc1
HCl.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.COCCOC
null
0.083333
CCC(=O)c1cc(Cl)nnc1OC.Cc1cc(B2OC(C)(C)C(C)(C)O2)cc(C)c1O>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.COCCOC>CCC(=O)c1cc(-c2cc(C)c(O)c(C)c2)nnc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-dfbd9f5c18534ceebd8b86e1288c2370
CCC(=O)c1cc(-c2cc(C)c(O)c(C)c2)nnc1OC.Nc1ccccc1Cl>>COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1[nH]c2ccccc2c1C
ClC1=C(N)C=CC=C1.S(=O)(=O)([O-])[O-].[Mg+2].OC1=C(C=C(C=C1C)C1=CC(=C(N=N1)OC)C(CC)=O)C.C(C)(=O)O>>COC1=C(C=C(N=N1)C1=CC(=C(C(=C1)C)O)C)C=1NC2=CC=CC=C2C1C
O=[C:18]([c:17]1[c:3]([O:2][CH3:1])[n:4][n:5][c:6](-[c:7]2[cH:8][c:9]([CH3:10])[c:11]([OH:12])[c:13]([CH3:14])[cH:15]2)[cH:16]1)[CH2:26][CH3:27].Cl[c:25]1[c:20]([NH2:19])[cH:21][cH:22][cH:23][cH:24]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][c:9]([CH3:10])[c:11]([OH:12])[c:13]([CH3:14])[cH:15]2)[cH:16][c:17]1-[c...
CCC(=O)c1cc(-c2cc(C)c(O)c(C)c2)nnc1OC.Nc1ccccc1Cl
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1[nH]c2ccccc2c1C
null
null
CC(=O)N(C)C
Aromatic Heterocycle Formation
OtherReaction
2aeebda70d28950751bcff9d93d27d409a496c19f9c9b9893349a271b234d219
4e13c013c1ec63cb4e4f791be1390f390c40f8fc080e4593325e7876241ac282
c1ccc(-c2cc(-c3cc4ccccc4[nH]3)cnn2)cc1
Cl-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[NH2;D1;+0:5]):[c:6].O=[C;H0;D3;+0:7](-[CH2;D2;+0:8]-[C;D1;H3:9])-[c;H0;D3;+0:10]1:[c:11]:[c:12](-[c:13]):[#7;a:14]:[#7;a:15]:[c:16]:1-[#8:17]>>[#8:17]-[c:16]1:[#7;a:15]:[#7;a:14]:[c:12](-[c:13]):[c:11]:[c;H0;D3;+0:10]:1-[c;H0;D3;+0:7]1:[nH;D2;+0:5]:[c:4](:[c:6]):[c;H0;D3;+0:1](:[...
null
[]
140
CELSIUS
null
null
73.4 μl of 2-chloroaniline and 21 mg of anhydrous magnesium sulfate are suspended in 3 ml dimethylacetamide. 100 mg of 1-[6-(4-Hydroxy-3,5-dimethyl-phenyl)-3-methoxy-pyridazin-4-yl]-propan-1-one and 31.4 mg acetic acid are added and the reaction is degassed with argon. 96 mg of tripotassium phosphate and 35.7 mg of bis...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ketone.Primary amine
null
c1ccccc1
c1ccc2[nH]ccc2c1
c1ccnnc1.c1ccccc1.c1ccc2[nH]ccc2c1
HCl
CC(=O)N(C)C
140
null
CCC(=O)c1cc(-c2cc(C)c(O)c(C)c2)nnc1OC.Nc1ccccc1Cl>CC(=O)N(C)C>COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1[nH]c2ccccc2c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0a7d41c35518413983d7f23b6fe8c52f
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1[nH]c2ccccc2c1C>>Cc1cc(-c2cc(-c3[nH]c4ccccc4c3C)c(=O)[nH]n2)cc(C)c1O
COC1=C(C=C(N=N1)C1=CC(=C(C(=C1)C)O)C)C=1NC2=CC=CC=C2C1C.C[Si](C)(C)Cl.[I-].[K+]>>OC1=C(C=C(C=C1C)C=1C=C(C(NN1)=O)C=1NC2=CC=CC=C2C1C)C
C[O:19][c:18]1[c:7](-[c:8]2[nH:9][c:10]3[cH:11][cH:12][cH:13][cH:14][c:15]3[c:16]2[CH3:17])[cH:6][c:5](-[c:4]2[cH:3][c:2]([CH3:1])[c:25]([OH:26])[c:23]([CH3:24])[cH:22]2)[n:21][n:20]1>>[CH3:1][c:2]1[cH:3][c:4](-[c:5]2[cH:6][c:7](-[c:8]3[nH:9][c:10]4[cH:11][cH:12][cH:13][cH:14][c:15]4[c:16]3[CH3:17])[c:18](=[O:19])[nH:2...
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1[nH]c2ccccc2c1C
Cc1cc(-c2cc(-c3[nH]c4ccccc4c3C)c(=O)[nH]n2)cc(C)c1O
null
null
C(C)#N.O
Miscellaneous
OtherReaction
3a907fa62544f46964e2b473ab8a45caedf80503ce5e705ae3da44b55acc0eb2
291cad8b6dfbbd2c823b5c9d45efc37a166dc3454a9f151ac48cb357f4bc155f
O=c1[nH]nc(-c2ccccc2)cc1-c1cc2ccccc2[nH]1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[c:8]:[#7;a:9]>>[#7;a:9]:[c:8]-[c:7]1:[c:6]:[c:5]:[#7;a:4]:[nH;D2;+0:3]:[c;H0;D3;+0:2]:1=[O;H0;D1;+0:1]
null
[]
80
CELSIUS
null
null
6 mg of 4-[6-Methoxy-5-(3-methyl-1H-indol-2-yl) -pyridazin-3-yl]-2,6-dimethyl-phenol is suspended in 2 ml acetonitrile and 6.5 mg of trimethylsilyl chloride and 9.96 mg of potassium iodide are added. The solution is heated to 80° C. for 3 h. The reaction solution is diluted with water and the product is purified by pre...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccnnc1
c1cnncc1
c1ccccc1.c1cnncc1.c1ccc2[nH]ccc2c1
Other
C(C)#N.O
80
null
COc1nnc(-c2cc(C)c(O)c(C)c2)cc1-c1[nH]c2ccccc2c1C>C(C)#N.O>Cc1cc(-c2cc(-c3[nH]c4ccccc4c3C)c(=O)[nH]n2)cc(C)c1O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f3bd3399003a4e82aa52d47a4c9b99e2
O=C1CCC(=O)N1I.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1>>O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I
N1C(=CC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O.C1CC(=O)N(C1=O)I>>IC1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O
O=C1CCC(=O)N1[I:23].[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[nH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[cH:22]1>>[O:1]=[c:2]1[nH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13]1-[c:14]1[nH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[c:22]1[I:...
O=C1CCC(=O)N1I.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I
null
null
CC(=O)C
Functional Group Interconversion
OtherReaction
0754ae2664ff7ba9610e6f272707033ed8b7278ddd1c23d9264359692cf74d77
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
O=C1-C-C-C(=O)-N-1-[I;H0;D1;+0:1].[#7;a:2]:[c:3]:[c:4]-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[cH;D2;+0:11]:1>>[#7;a:2]:[c:3]:[c:4]-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[c;H0;D3;+0:11]:1-[I;H0;D1;+0:1]
null
[]
null
null
3
HOUR
577 mg 4-(1H-Indol-2-yl)-6-pyridin-4-yl-2H-pyridazin-3-one is suspended in 30 mL acetone and 550 mg NIS is added. The reaction mixture is stirred for 3 hours at room temperature, the precipitated product isolated by filtration and washed with acetone. The material product is used without further purification Conditions...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
C1CCNC1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1
HO-
CC(=O)C
null
3
O=C1CCC(=O)N1I.O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1>CC(=O)C>O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4c08ebff04e74637bf2cec2accec9dc6
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I>>C=Cc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
IC1=C(NC2=CC=CC=C12)C=1C(NN=C(C1)C1=CC=NC=C1)=O.C(CCC)[Sn](C=C)(CCCC)CCCC.CCOC(=O)C.[F-].[K+]>>N1=CC=C(C=C1)C=1C=C(C(NN1)=O)C=1NC2=CC=CC=C2C1C=C
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[CH:2]=[CH2:1].I[c:3]1[c:4](-[c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][n:11][cH:12][cH:13]3)[n:14][nH:15][c:16]2=[O:17])[nH:18][c:19]2[cH:20][cH:21][cH:22][cH:23][c:24]12>>[CH2:1]=[CH:2][c:3]1[c:4](-[c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][n:11][cH:12][cH:13]3)[n:14][nH:15][c:16]2=[O:17])[nH:...
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I
C=Cc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
null
[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
CN(C)C=O
C-C Coupling
Stille reaction_vinyl
f4ad649c74b7a6a35b0e84610492e238d5241d8eaf0ab45cca5db093924b7eac
ec03c739f58696d2a3659a73884744e1a490a20a587da6f115be382b663cf23d
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccccc2[nH]1
C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[CH;D2;+0:1]=[C;D1;H2:2].I-[c;H0;D3;+0:3]1:[c:4](:[c:5]):[c:6](:[c:7]):[#7;a:8]:[c:9]:1-[c:10]:[c:11]:[#7;a:12]>>[#7;a:12]:[c:11]:[c:10]-[c:9]1:[#7;a:8]:[c:6](:[c:7]):[c:4](:[c:5]):[c;H0;D3;+0:3]:1-[CH;D2;+0:1]=[C;D1;H2:2]
null
[]
80
CELSIUS
40
MINUTE
A mixture of 104 mg 4-(3-Iodo-1H-indol-2-yl)-6-pyridin-4-yl-2H-pyridazin-3-one (example 25), 123 mg tributyl(vinyl)tin, 41 mg tetraethylammonium-chloride and 9 mg bis(triphenylphosphine)palladium(II) chloride in DMF is stirred at 80° C. for 40 min. After cooling to room temperature, 4 ml aqueous potassium fluoride solu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl.Tin
Vinyl
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1cnncc1.c1ccncc1.c1ccc2[nH]ccc2c1
HI.Sn
[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O
80
0.666667
C=[CH][Sn]([CH2]CCC)([CH2]CCC)[CH2]CCC.O=c1[nH]nc(-c2ccncc2)cc1-c1[nH]c2ccccc2c1I>[Cl-].C(C)[N+](CC)(CC)CC.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O>C=Cc1c(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]c2ccccc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8e9388745e8c40c88dfe425586cb5534
COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CO)cc2n1C(=O)OC(C)(C)C>>COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C
C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)CO)C1=C(N=NC(=C1)C1=CC=NC=C1)OC>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)C=O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC
[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1-[c:15]1[cH:16][c:17]2[cH:18][cH:19][c:20]([CH2:21][OH:22])[cH:23][c:24]2[n:25]1[C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32]>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][c:14]1-[c:1...
COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CO)cc2n1C(=O)OC(C)(C)C
COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C
null
[O-2].[Mn+4].[O-2].[O-2].[Mn+4].[O-2]
ClCCl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
[#7;a:1]:[c:2]:[c:3]:[c:4](-[CH2;D2;+0:5]-[OH;D1;+0:6]):[c:7]>>[#7;a:1]:[c:2]:[c:3]:[c:4](-[CH;D2;+0:5]=[O;H0;D1;+0:6]):[c:7]
82
[{"value": 82.0, "product": "C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)C=O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.9, "product": "C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)C=O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2 g 6-Hydroxymethyl-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-indole-1-carboxylic acid tert-butyl ester is dissolved in 46 mL dichloromethane. After addition of 1.61 g activated manganese (IV) oxide the reaction mixture is heated to reflux for 1 hour. Then every two hours additional manganese (IV) oxide is added unti...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccnnc1.c1ccncc1.c1ccc2cc[nH]c2c1
null
[O-2].[Mn+4].[O-2].[O-2].[Mn+4].[O-2].ClCCl
null
null
COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CO)cc2n1C(=O)OC(C)(C)C>[O-2].[Mn+4].[O-2].[O-2].[Mn+4].[O-2].ClCCl>COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-16e15281ca544ab5b7ef7ac523cb9677
C1CCNCC1.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C>>COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CN3CCCCC3)cc2n1C(=O)OC(C)(C)C
C(=O)(O)[O-].[Na+].C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)C=O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.N1CCCCC1.C(=O)=O.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+]>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)CN1CCCCC1)C1=C(N=NC(=C1)C1=CC=NC=C1)OC
[NH:22]1[CH2:23][CH2:24][CH2:25][CH2:26][CH2:27]1.O=[CH:21][c:20]1[cH:19][cH:18][c:17]2[cH:16][c:15](-[c:14]3[c:3]([O:2][CH3:1])[n:4][n:5][c:6](-[c:7]4[cH:8][cH:9][n:10][cH:11][cH:12]4)[cH:13]3)[n:30]([C:31](=[O:32])[O:33][C:34]([CH3:35])([CH3:36])[CH3:37])[c:29]2[cH:28]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8...
C1CCNCC1.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C
COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CN3CCCCC3)cc2n1C(=O)OC(C)(C)C
null
null
ClCCl.ClC(C)Cl.C(C)(=O)O
Heteroatom Alkylation and Arylation
reductive amination
d0e659bc8d1e29e09a61320b4c537e66ad57335a51368c8bd48de9bdffa59372
2d03f38884b1fbb0c0d6e6f2de31afb25102fec87f347c3a123e064c1bfef0ad
c1cc(-c2cc(-c3cc4ccc(CN5CCCCC5)cc4[nH]3)cnn2)ccn1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6].[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[CH2;D2;+0:1]-[N;H0;D3;+0:9](-[C:8]-[C:7])-[C:10]-[C:11]):[c:3]
83
[{"value": 83.0, "product": "C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)CN1CCCCC1)C1=C(N=NC(=C1)C1=CC=NC=C1)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
79 mg 6-formyl-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-indole-1-carboxylic acid tert-butyl ester is dissolved in 14 mL dichloroethane. 182 mL piperidine and then 0.7 mL acetic acid are added. 334 mg sodium triacetoxyborohydride is added in several portions over 6 hours. Sat. aq. NaHCO3-solution is added and the rea...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
c1ccnnc1.c1ccncc1.c1ccc2cc[nH]c2c1.C1CC[NH]CC1
Other
ClCCl.ClC(C)Cl.C(C)(=O)O
null
null
C1CCNCC1.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C>ClCCl.ClC(C)Cl.C(C)(=O)O>COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CN3CCCCC3)cc2n1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b6617c3e1efe40648bbe980703bbf55d
CCOC(=O)c1cc(-c2ccncc2)n[nH]c1=O.NN>>NNC(=O)c1cc(-c2ccncc2)n[nH]c1=O
C(C)OC(=O)C=1C(NN=C(C1)C1=CC=NC=C1)=O.O.NN>>O=C1NN=C(C=C1C(=O)NN)C1=CC=NC=C1
CCO[C:3](=[O:4])[c:5]1[cH:6][c:7](-[c:8]2[cH:9][cH:10][n:11][cH:12][cH:13]2)[n:14][nH:15][c:16]1=[O:17].[NH2:1][NH2:2]>>[NH2:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7](-[c:8]2[cH:9][cH:10][n:11][cH:12][cH:13]2)[n:14][nH:15][c:16]1=[O:17]
CCOC(=O)c1cc(-c2ccncc2)n[nH]c1=O.NN
NNC(=O)c1cc(-c2ccncc2)n[nH]c1=O
null
null
C(C)O
Acylation
Aminolysis of esters
2e40a14c7d71c6b9001f460fbb953805c923b2db988c8c04f234b9bb5f04424f
3b636feb164ef0f3c8a4f1764f18a25b9eee32ed1463e3bb4b6f1becb871ca74
O=c1ccc(-c2ccncc2)n[nH]1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1=[O;D1;H0:9].[N;D1;H2:10]-[NH2;D1;+0:11]>>[N;D1;H2:10]-[NH;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1=[O;D1;H0:9]
null
[]
null
null
null
null
10 g of 3-oxo-6-pyridin-4-yl-2,3-dihydro-pyridazine-4 -carboxylic acid ethyl ester are dissolved in 150 ml of ethanol, 4.2 ml of hydrazine hydrate is added and the mixture is refluxed for 5 hours. After cooling to room temperature, the solid is collected by filtration and dried in vacuo at 40° C. Conditions: See reacti...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Ester
Acylhydrazine
null
null
c1cnncc1.c1ccncc1
HO-
C(C)O
null
null
CCOC(=O)c1cc(-c2ccncc2)n[nH]c1=O.NN>C(C)O>NNC(=O)c1cc(-c2ccncc2)n[nH]c1=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9975cf0fb56142daa5f77fd28abbd97c
CC(N)=S.NNC(=O)c1cc(-c2ccncc2)n[nH]c1=O>>Cc1nnc(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]1
O=C1NN=C(C=C1C(=O)NN)C1=CC=NC=C1.C(C)(=S)N.C(C)N(CC)CC.N1=CC=CC=C1>>CC=1NC(=NN1)C=1C(NN=C(C1)C1=CC=NC=C1)=O
S=[C:2]([CH3:1])[NH2:19].O=[C:5]([NH:4][NH2:3])[c:6]1[cH:7][c:8](-[c:9]2[cH:10][cH:11][n:12][cH:13][cH:14]2)[n:15][nH:16][c:17]1=[O:18]>>[CH3:1][c:2]1[n:3][n:4][c:5](-[c:6]2[cH:7][c:8](-[c:9]3[cH:10][cH:11][n:12][cH:13][cH:14]3)[n:15][nH:16][c:17]2=[O:18])[nH:19]1
CC(N)=S.NNC(=O)c1cc(-c2ccncc2)n[nH]c1=O
Cc1nnc(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]1
null
null
C(CCC)O
Aromatic Heterocycle Formation
OtherReaction
22397ef88a4b6ba0343586e53e3e20e2055f46904a3043f30a9bf08906917011
1e7b5d45c28f5d1767d2abb0c78792aee2714d99002ea329b67f9a89a7e53301
O=c1[nH]nc(-c2ccncc2)cc1-c1nnc[nH]1
O=[C;H0;D3;+0:1](-[NH;D2;+0:2]-[NH2;D1;+0:3])-[c;H0;D3;+0:4]1:[c:5]:[c:6](-[c:7]):[#7;a:8]:[#7;a:9]:[c:10]:1=[O;D1;H0:11].S=[C;H0;D3;+0:12](-[C;D1;H3:13])-[NH2;D1;+0:14]>>[C;D1;H3:13]-[c;H0;D3;+0:12]1:[n;H0;D2;+0:3]:[n;H0;D2;+0:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:4]2:[c:5]:[c:6](-[c:7]):[#7;a:8]:[#7;a:9]:[c:10]:2=[O;D1;H0:1...
null
[]
null
null
null
null
A mixture of 100 mg of 3-oxo-6-pyridin-4-yl-2,3-dihydro-pyridazine-4-carboxylic acid hydrazide, 130 mg thioacetamide, 87 mg triethylamine, 1 ml of pyridine and 5 ml of butanol is refluxed for 15 hours. After cooling and stirring at room temperature, a solid precipitated is collected by filtration, washed with cold isop...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Thioamide
null
null
c1nc[nH]n1
c1nc[nH]n1.c1cnncc1.c1ccncc1
Other
C(CCC)O
null
null
CC(N)=S.NNC(=O)c1cc(-c2ccncc2)n[nH]c1=O>C(CCC)O>Cc1nnc(-c2cc(-c3ccncc3)n[nH]c2=O)[nH]1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7bf3e54ab9a1423e8dedda95b8b729dc
COC[P+](c1ccccc1)(c1ccccc1)c1ccccc1.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C>>COC=Cc1ccc2cc(-c3cc(-c4ccncc4)nnc3OC)n(C(=O)OC(C)(C)C)c2c1
C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)C=O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.[Cl-].COC[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C(CCC)[Li]>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)C=COC)C1=C(N=NC(=C1)C1=CC=NC=C1)OC
c1ccc([P+](c2ccccc2)(c2ccccc2)[CH2:3][O:2][CH3:1])cc1.O=[CH:4][c:5]1[cH:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][c:13](-[c:14]4[cH:15][cH:16][n:17][cH:18][cH:19]4)[n:20][n:21][c:22]3[O:23][CH3:24])[n:25]([C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32])[c:33]2[cH:34]1>>[CH3:1][O:2][CH:3]=[CH:4][c:5]1[cH:6][cH:...
COC[P+](c1ccccc1)(c1ccccc1)c1ccccc1.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C
COC=Cc1ccc2cc(-c3cc(-c4ccncc4)nnc3OC)n(C(=O)OC(C)(C)C)c2c1
null
null
C1CCOC1
C-C Coupling
Wittig with Phosphonium
1b762435fe6b580b808a6e9f0dae00ddd254c0b88d607d21a223e11776d2e3a4
bf4569804906d66c98adaac7df334e96eee508d45c26c621eb5069c3e4f1df77
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6].[C;D1;H3:7]-[#8:8]-[CH2;D2;+0:9]-[P+](-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[CH;D2;+0:1]=[CH;D2;+0:9]-[#8:8]-[C;D1;H3:7]):[c:3]
null
[]
-78
CELSIUS
30
MINUTE
1.23 g methoxymethyltriphenylphoshonium chloride is suspended in 10 mL THF and cooled to −78° C. 2.20 mL butyllithium (1.6 M in hexanes) is added dropwise and the resulting mixture is stirred for 30 min at −78° C. and then warmed in an ice bath to 0° C. After addition of a solution of 734 mg 6-formyl-2-(3-methoxy-6-pyr...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Ether
Ether
c1ccccc1.c1ccccc1.c1ccccc1
null
c1ccc2cc[nH]c2c1.c1ccnnc1.c1ccncc1
HO-
C1CCOC1
-78
0.5
COC[P+](c1ccccc1)(c1ccccc1)c1ccccc1.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(C=O)cc2n1C(=O)OC(C)(C)C>C1CCOC1>COC=Cc1ccc2cc(-c3cc(-c4ccncc4)nnc3OC)n(C(=O)OC(C)(C)C)c2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-88b4576dce994509ad8426d3567f2f13
COC=Cc1ccc2cc(-c3cc(-c4ccncc4)nnc3OC)n(C(=O)OC(C)(C)C)c2c1>>COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CC=O)cc2n1C(=O)OC(C)(C)C
C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)C=COC)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.[I-].[K+].Cl[Si](C)(C)C>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)CC=O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC
C[O:23][CH:22]=[CH:21][c:20]1[cH:19][cH:18][c:17]2[cH:16][c:15](-[c:14]3[c:3]([O:2][CH3:1])[n:4][n:5][c:6](-[c:7]4[cH:8][cH:9][n:10][cH:11][cH:12]4)[cH:13]3)[n:26]([C:27](=[O:28])[O:29][C:30]([CH3:31])([CH3:32])[CH3:33])[c:25]2[cH:24]1>>[CH3:1][O:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][n:10][cH:11][cH:12]2)[cH:13][...
COC=Cc1ccc2cc(-c3cc(-c4ccncc4)nnc3OC)n(C(=O)OC(C)(C)C)c2c1
COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CC=O)cc2n1C(=O)OC(C)(C)C
null
null
C(C)#N
Miscellaneous
OtherReaction
c341fdc42e48cf7e12789f1fb10a9c65f84ba2f1b42598f190b56c95d40c7caa
f3a920ec0ed1e7a5c2088300ae22a9e2e42203bc8efef555e3e9c02778626f07
c1ccc2[nH]c(-c3cnnc(-c4ccncc4)c3)cc2c1
C-[O;H0;D2;+0:1]-[CH;D2;+0:2]=[CH;D2;+0:3]-[c:4](:[c:5]):[c:6]:[c:7]:[#7;a:8]>>[#7;a:8]:[c:7]:[c:6]:[c:4](-[CH2;D2;+0:3]-[CH;D2;+0:2]=[O;H0;D1;+0:1]):[c:5]
114.6
[{"value": 114.6, "product": "C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)CC=O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
180 mg 6-(2-methoxyvinyl)-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-indole-1-carboxylic acid tert-butyl ester are dissolved in 10 mL acetonitrile. Then 196 mg potassium iodide and 125 μL chlorotrimethylsilane are added. The reaction mixture is stirred for 2 hours at rt. The solvent is removed in vacuo and the obtaine...
10.6084/m9.figshare.5104873.v1
null
Ether
Aldehyde
null
null
c1ccnnc1.c1ccncc1.c1ccc2cc[nH]c2c1
Other
C(C)#N
null
2
COC=Cc1ccc2cc(-c3cc(-c4ccncc4)nnc3OC)n(C(=O)OC(C)(C)C)c2c1>C(C)#N>COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CC=O)cc2n1C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ae220e267c754d6f871b184be7eb4cda
C1COCCN1.CC(C)(C)OC(=O)n1c(-c2cc(-c3ccncc3)n[nH]c2=O)cc2ccc(CC=O)cc21.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CC=O)cc2n1C(=O)OC(C)(C)C>>CC(C)(C)OC(=O)n1c(-c2cc(-c3ccncc3)n[nH]c2=O)cc2ccc(CCC3CCCCN3)cc21
C(=O)(O)[O-].[Na+].C(=O)=O.N1CCOCC1.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+].C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)CC=O)C1=C(N=NC(=C1)C1=CC=NC=C1)OC.C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)CC=O)C=1C(NN=C(C1)C1=CC=NC=C1)=O>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)CCC1NCCCC1)C=1C(NN=C(C1)C1=CC=NC=C1)=O
O1[CH2:31][CH2:30][NH:35][CH2:34][CH2:33]1.O=[CH:29][CH2:28][c:27]1[cH:26][cH:25][c:24]2[cH:23][c:9](-[c:10]3[cH:11][c:12](-[c:13]4[cH:14][cH:15][n:16][cH:17][cH:18]4)[n:19][nH:20][c:21]3=[O:22])[n:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[c:37]2[cH:36]1.COc1nnc(-c2ccn[cH:32]c2)cc1-c1cc2ccc(CC=O)cc2n1C(=O)OC...
C1COCCN1.CC(C)(C)OC(=O)n1c(-c2cc(-c3ccncc3)n[nH]c2=O)cc2ccc(CC=O)cc21.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CC=O)cc2n1C(=O)OC(C)(C)C
CC(C)(C)OC(=O)n1c(-c2cc(-c3ccncc3)n[nH]c2=O)cc2ccc(CCC3CCCCN3)cc21
null
null
ClCCl.ClC(C)Cl.C(C)(=O)O
C-C Coupling
OtherReaction
a135ff1e65bd5b14a2374c578f9ed1943f615e583da5eed342dd0f111218ee05
5b03a5b9e4b0906e57b3451f053f1aa86667b6e59f1733c15a6fe7ccbeb48e6f
O=c1[nH]nc(-c2ccncc2)cc1-c1cc2ccc(CCC3CCCCN3)cc2[nH]1
C-O-c1:n:n:c(-c2:c:[cH;D2;+0:1]:n:c:c:2):c:c:1-c1:c:c2:c:c:c(-C-C=O):c:c:2:n:1-C(=O)-O-C(-C)(-C)-C.O1-[CH2;D2;+0:2]-[CH2;D2;+0:3]-[#7:4]-[C:5]-[CH2;D2;+0:6]-1.O=[CH;D2;+0:7]-[C:8]-[c:9]>>[c:9]-[C:8]-[CH2;D2;+0:7]-[CH;D3;+0:3]1-[#7:4]-[C:5]-[CH2;D2;+0:6]-[CH2;D2;+0:1]-[CH2;D2;+0:2]-1
null
[]
null
null
null
null
54 mg of a mixture of 6-(2-oxoethyl)-2-(3-methoxy-6-pyridin-4-yl-pyridazin-4-yl)-indole-1-carboxylic acid tert-butyl ester and 6-(2-oxoethyl)-2-(3-Oxo-6-pyridin-4-yl-2,3-dihydro-pyridazin-4-yl)indole-1-carboxylic acid tert-butyl ester are dissolved in 9 mL dichloroethane. 160 μL morpholine and then 0.46 mL acetic acid ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Aldehyde.Ether.Ether.Ether.Boc
null
C1COCCN1.c1ccnnc1.c1ccncc1.c1ccc2[nH]ccc2c1
C1CCNCC1
c1cnncc1.c1ccncc1.c1ccc2cc[nH]c2c1.C1CCNCC1
HO-
ClCCl.ClC(C)Cl.C(C)(=O)O
null
null
C1COCCN1.CC(C)(C)OC(=O)n1c(-c2cc(-c3ccncc3)n[nH]c2=O)cc2ccc(CC=O)cc21.COc1nnc(-c2ccncc2)cc1-c1cc2ccc(CC=O)cc2n1C(=O)OC(C)(C)C>ClCCl.ClC(C)Cl.C(C)(=O)O>CC(C)(C)OC(=O)n1c(-c2cc(-c3ccncc3)n[nH]c2=O)cc2ccc(CCC3CCCCN3)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-dbbb1c6c81804f80891a6abbf08e6b2f
CC(=O)c1cccc(OB(O)O)c1.CCc1cccc(C(=O)O)c1Br>>CCOC(=O)c1ccccc1-c1cccc(C(C)=O)c1
C(C)C=1C(=C(C(=O)O)C=CC1)Br.C(C)(=O)C=1C=C(C=CC1)OB(O)O.C(OC)COC.C([O-])(O)=O.[Na+].C([O-])([O-])=O.[Na+].[Na+]>>C(C)OC(=O)C=1C(=CC=CC1)C1=CC(=CC=C1)C(C)=O
OB(O)O[c:12]1[cH:13][cH:14][cH:15][c:16]([C:17]([CH3:18])=[O:19])[cH:20]1.Br[c:11]1[c:6]([C:4]([OH:3])=[O:5])[cH:7][cH:8][cH:9][c:10]1[CH2:2][CH3:1]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][cH:10][c:11]1-[c:12]1[cH:13][cH:14][cH:15][c:16]([C:17]([CH3:18])=[O:19])[cH:20]1
CC(=O)c1cccc(OB(O)O)c1.CCc1cccc(C(=O)O)c1Br
CCOC(=O)c1ccccc1-c1cccc(C(C)=O)c1
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
1c8c48036a0f06e6ffc9673466d4bff5319e6174ce2f1a0d2bea2aab2e9cd80f
169f4e097ffba4530d9f6d9673651b55f261578d3ebd32e9612e5b32deecfd8e
c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2](-[C:3](=[O;D1;H0:4])-[OH;D1;+0:5]):[c:6]:[c:7]:[c:8]:[c;H0;D3;+0:9]:1-[CH2;D2;+0:10]-[C;D1;H3:11].O-B(-O)-O-[c;H0;D3;+0:12](:[c:13]:[c:14]):[c:15]:[c:16]-[C:17](-[C;D1;H3:18])=[O;D1;H0:19]>>[C;D1;H3:18]-[C:17](=[O;D1;H0:19])-[c:16]:[c:15]:[c;H0;D3;+0:12](-[c;H0;D3;+0:1]1:[cH;D2;+0:9]:[c:8]:[c:7...
95
[{"value": 95.0, "product": "C(C)OC(=O)C=1C(=CC=CC1)C1=CC(=CC=C1)C(C)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of ethyl 2-bromobenzoic acid (10.0 g) and 3-acetylphenylboric acid (7.87 g) in dimethoxyethane (200 ml) was added 2 N sodium carbonate solution (50 ml), and the mixture was deaerated and argon-substituted. To this mixture was added tetrakis(triphenylphosphine) palladium (0) (5.04 g), and the mixture was...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carboxylic acid
Ester
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HBr.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(C)(=O)OCC
null
null
CC(=O)c1cccc(OB(O)O)c1.CCc1cccc(C(=O)O)c1Br>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(C)(=O)OCC>CCOC(=O)c1ccccc1-c1cccc(C(C)=O)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-246bbab43f254048a1c6b8ae5710095b
CC(C)(C)OC(=O)NCCN.CC(NC1CCN(Cc2ccccc2)CC1)c1cccc(-c2ccccc2C(=O)NCCNC(=O)OC(C)(C)C)c1.CCN=C=NCCCN(C)C.CN(C)C=O.On1nnc2ccccc21>>CC(c1cccc(-c2ccccc2C(=O)NCCNC(=O)OC(C)(C)C)c1)N(C(=O)Cc1ccc2ccccc2c1)C1CCN(Cc2ccccc2)CC1
CCN=C=NCCCN(C)C.C(C1=CC=CC=C1)N1CCC(CC1)NC(C)C=1C=C(C=CC1)C=1C(=CC=CC1)C(=O)NCCNC(=O)OC(C)(C)C.C(C)(C)(C)OC(NCCN)=O.C=1C=CC2=C(C1)N=NN2O.CN(C)C=O>>C(C1=CC=CC=C1)N1CCC(CC1)N(C(CC1=CC2=CC=CC=C2C=C1)=O)C(C)C=1C=C(C=CC1)C=1C(=CC=CC1)C(=O)NCCNC(=O)OC(C)(C)C
C[C:32](OC(=O)NCCN)([CH3:33])[CH3:41].[CH3:1][CH:2]([c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[C:14](=[O:15])[NH:16][CH2:17][CH2:18][NH:19][C:20](=[O:21])[O:22][C:23]([CH3:24])([CH3:25])[CH3:26])[cH:27]1)[NH:28][CH:42]1[CH2:43][CH2:44][N:45]([CH2:46][c:47]2[cH:48][cH:49][cH:50][cH:51][cH:52...
CC(C)(C)OC(=O)NCCN.CC(NC1CCN(Cc2ccccc2)CC1)c1cccc(-c2ccccc2C(=O)NCCNC(=O)OC(C)(C)C)c1.CCN=C=NCCCN(C)C.CN(C)C=O.On1nnc2ccccc21
CC(c1cccc(-c2ccccc2C(=O)NCCNC(=O)OC(C)(C)C)c1)N(C(=O)Cc1ccc2ccccc2c1)C1CCN(Cc2ccccc2)CC1
null
null
C([O-])(O)=O.[Na+].C(C)N(CC)CC
Acylation
OtherReaction
4fdacd17504eb9e80ea86f61c59068935c60b7876057a860926c772402aa7434
858d275fb1dd4d064077f2884ff6972234e8a0ea65372d1e70759265e87e0c43
O=C(Cc1ccc2ccccc2c1)N(Cc1cccc(-c2ccccc2)c1)C1CCN(Cc2ccccc2)CC1
C-N(-C)-C-C-C-N=[C;H0;D2;+0:1]=N-C-[CH3;D1;+0:2].C-N(-C)-[CH;D2;+0:3]=[O;D1;H0:4].C-[C;H0;D4;+0:5](-[CH3;D1;+0:6])(-[CH3;D1;+0:7])-O-C(=O)-N-C-C-N.O-n1:n:n:[c;H0;D3;+0:8]2:[c:9]:[c:10]:[c:11]:[c:12]:[c;H0;D3;+0:13]:2:1.[C:14]-[C:15](-[NH;D2;+0:16]-[C:17](-[C;D1;H3:18])-[c:19])-[C:20]>>[C:14]-[C:15](-[N;H0;D3;+0:16](-[C...
null
[]
null
null
18
HOUR
To a solution of the compound obtained in Reference Example 3 (1.20 g) in DMF (40 ml) were added N-(2-aminoethyl)carbamic acid tert-butyl ester (310 mg), HOBt (262 mg) and triethylamine (196 mg). WSC (372 mg) was further added to this mixture under ice-cooling, and the mixture was stirred for 18 hours at room temperatu...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Tertiary amide.Primary amine.Secondary amine.Tertiary amine.Boc
Tertiary amide
c1ccc2[nH]nnc2c1
c1ccc2ccccc2c1
c1ccccc1.c1ccccc1.c1ccc2ccccc2c1.C1CC[NH]CC1.c1ccccc1
HO-
C([O-])(O)=O.[Na+].C(C)N(CC)CC
null
18
CC(C)(C)OC(=O)NCCN.CC(NC1CCN(Cc2ccccc2)CC1)c1cccc(-c2ccccc2C(=O)NCCNC(=O)OC(C)(C)C)c1.CCN=C=NCCCN(C)C.CN(C)C=O.On1nnc2ccccc21>C([O-])(O)=O.[Na+].C(C)N(CC)CC>CC(c1cccc(-c2ccccc2C(=O)NCCNC(=O)OC(C)(C)C)c1)N(C(=O)Cc1ccc2ccccc2c1)C1CCN(Cc2ccccc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d8d8511fd6714c77bb469f6797f331c4
NCc1ccccc1Br>>CC(C)(C)OC(=O)NCc1ccccc1Br
Cl.BrC1=C(CN)C=CC=C1.C([O-])(O)=O.[Na+]>>C(C)(C)(C)OC(NCC1=C(C=CC=C1)Br)=O
[cH:1]1[cH:12][cH:11][c:10]([CH2:9][NH2:8])[c:15]([Br:16])[cH:14]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][c:15]1[Br:16]
NCc1ccccc1Br
CC(C)(C)OC(=O)NCc1ccccc1Br
null
null
O.C(C)(=O)OCC
Functional Group Addition
OtherReaction
7ebc72dfbd368f2957e1d9209ce0e4f43e00e1e6eb015c59f70700923a5b5214
787734300905392fc3f0ea9fb3cf35858edc27da77afa0faeeb2270fd92e7178
c1ccccc1
[Br;D1;H0:1]-[c:2]1:[cH;D2;+0:3]:[cH;D2;+0:4]:[cH;D2;+0:5]:[c:6]:[c:7]:1-[C:8]-[NH2;D1;+0:9]>>[Br;D1;H0:1]-[c:2]1:[cH;D2;+0:3]:[c:10]:[cH;D2;+0:5]:[c:6]:[c:7]:1-[C:8]-[NH;D2;+0:9]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[CH3;D1;+0:4]
95
[{"value": 95.0, "product": "C(C)(C)(C)OC(NCC1=C(C=CC=C1)Br)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
To a solution of 2-bromobenzylamine hydrochloride (5.00 g) and di-tert-butoxycarbonyl (5.39 g) in ethyl acetate (30 ml) was added saturated sodium bicarbonate solution (30 ml), and stirred at room temperature for 16 hours. The obtained reaction mixture was diluted with water, and extracted with ethyl acetate. The organ...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Carbamic ester.Ether.Boc
c1ccccc1
c1ccccc1
c1ccccc1
Other
O.C(C)(=O)OCC
null
16
NCc1ccccc1Br>O.C(C)(=O)OCC>CC(C)(C)OC(=O)NCc1ccccc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-48f5b29454ff4ffa8f8e635f369abe30
CC(C)(C)OC(=O)NCCC(=O)O.Nc1ccccc1Br>>CC(C)(C)OC(=O)NCCCC(=O)Nc1ccccc1Br
C(C)(C)(C)OC(=O)NCCC(=O)O.N1=CC=CC=C1.C(C(=O)Cl)(=O)Cl.BrC1=C(N)C=CC=C1>>BrC1=C(C=CC=C1)NC(=O)CCCNC(=O)OC(C)(C)C
O[C:11]([CH2:10][CH2:9][NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])=[O:13].[NH2:14][c:15]1[cH:16][cH:17][cH:18][cH:19][c:20]1[Br:21]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][CH2:9][CH2:10][CH2:11][C:12](=[O:13])[NH:14][c:15]1[cH:16][cH:17][cH:18][cH:19][c:20]1[Br:21]
CC(C)(C)OC(=O)NCCC(=O)O.Nc1ccccc1Br
CC(C)(C)OC(=O)NCCCC(=O)Nc1ccccc1Br
null
CN(C)C=O.CN(C1=CC=NC=C1)C
C(C)#N.C([O-])(O)=O.[Na+].C(C)N(CC)CC.C1CCOC1
Acylation
OtherReaction
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
c1ccccc1
O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3]-[C:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C:4]-[C:3]-[CH2;D2;+0:1]-[C:9](=[O;H0;D1;+0:2])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]
18
[{"value": 18.0, "product": "BrC1=C(C=CC=C1)NC(=O)CCCNC(=O)OC(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 3-(tert-butoxycarbonylamino)propionic acid (4.3 g) and pyridine (3.6 ml) in THF (40 ml) were added oxalyl chloride (3.0 ml) and DMF(3 drops) under ice-cooling, and the mixture was stirred at room temperature for 1 hour. To the obtained reaction solution were added o-bromoaniline (2.6 g), triethylamine ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1
null
CN(C)C=O.CN(C1=CC=NC=C1)C.C(C)#N.C([O-])(O)=O.[Na+].C(C)N(CC)CC.C1CCOC1
null
1
CC(C)(C)OC(=O)NCCC(=O)O.Nc1ccccc1Br>CN(C)C=O.CN(C1=CC=NC=C1)C.C(C)#N.C([O-])(O)=O.[Na+].C(C)N(CC)CC.C1CCOC1>CC(C)(C)OC(=O)NCCCC(=O)Nc1ccccc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e29922bd31954e4c9a42c73495a770ab
CC(c1cccc(-c2ccccc2CN)c1)N(C(=O)Cc1ccc(Cl)cc1)C1CCN(Cc2ccccc2)CC1.Cl.NC(=O)CCl>>CC(c1cccc(-c2ccccc2CNCC(N)=O)c1)N(C(=O)Cc1ccc(Cl)cc1)C1CCN(Cc2ccccc2)CC1.Cl
Cl.Cl.Cl.NCC1=C(C=CC=C1)C1=CC(=CC=C1)C(C)N(C(CC1=CC=C(C=C1)Cl)=O)C1CCN(CC1)CC1=CC=CC=C1.ClCC(=O)N.C([O-])([O-])=O.[K+].[K+]>>Cl.Cl.C(C1=CC=CC=C1)N1CCC(CC1)N(C(CC1=CC=C(C=C1)Cl)=O)C(C)C=1C=C(C=CC1)C1=C(C=CC=C1)CNCC(=O)N
[CH3:1][CH:2]([c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[CH2:14][NH2:15])[cH:20]1)[N:21]([C:22](=[O:23])[CH2:24][c:25]1[cH:26][cH:27][c:28]([Cl:29])[cH:30][cH:31]1)[CH:32]1[CH2:33][CH2:34][N:35]([CH2:36][c:37]2[cH:38][cH:39][cH:40][cH:41][cH:42]2)[CH2:43][CH2:44]1.[ClH:46].Cl[CH2:16][C:17](...
CC(c1cccc(-c2ccccc2CN)c1)N(C(=O)Cc1ccc(Cl)cc1)C1CCN(Cc2ccccc2)CC1.Cl.NC(=O)CCl
CC(c1cccc(-c2ccccc2CNCC(N)=O)c1)N(C(=O)Cc1ccc(Cl)cc1)C1CCN(Cc2ccccc2)CC1.Cl
null
null
C([O-])(O)=O.[Na+].CCOCC.C(C)#N.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
fc19a1445ff204e66e51735d0191465bda3c6691fd233624a54742c9d4828411
0b1d32f56ad00f1e5bdae9390f9227bbea012fa2f8203aac34726b8a6761cc7c
O=C(Cc1ccccc1)N(Cc1cccc(-c2ccccc2)c1)C1CCN(Cc2ccccc2)CC1
Cl-[CH2;D2;+0:1]-[C:2](-[N;D1;H2:3])=[O;D1;H0:4].[NH2;D1;+0:5]-[C:6]-[c:7]>>[N;D1;H2:3]-[C:2](=[O;D1;H0:4])-[CH2;D2;+0:1]-[NH;D2;+0:5]-[C:6]-[c:7]
77
[{"value": 77.0, "product": "Cl.Cl.C(C1=CC=CC=C1)N1CCC(CC1)N(C(CC1=CC=C(C=C1)Cl)=O)C(C)C=1C=C(C=CC1)C1=C(C=CC=C1)CNCC(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
72
HOUR
To a solution of the compound obtained in Example 43 (100 mg) in acetonitrile (10 ml) was added 2-chloroacetic acid amide (22 mg) and potassium carbonate (66 mg), and the mixture was stirred at room temperature for 72 hours, and at 60° C. for 6 hours. The reaction mixture was diluted with saturated sodium bicarbonate (...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccccc1.c1ccccc1.C1CC[NH]CC1.c1ccccc1
HCl
C([O-])(O)=O.[Na+].CCOCC.C(C)#N.C(C)(=O)OCC
null
72
CC(c1cccc(-c2ccccc2CN)c1)N(C(=O)Cc1ccc(Cl)cc1)C1CCN(Cc2ccccc2)CC1.Cl.NC(=O)CCl>C([O-])(O)=O.[Na+].CCOCC.C(C)#N.C(C)(=O)OCC>CC(c1cccc(-c2ccccc2CNCC(N)=O)c1)N(C(=O)Cc1ccc(Cl)cc1)C1CCN(Cc2ccccc2)CC1.Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ad4a09b75ec84bed8558cde3ba78f108
ClCl.O=S([O-])c1ccccc1>>O=S(=O)(Cl)c1ccccc1
ClCl.C1(=CC=CC=C1)S(=O)[O-].[Na+].C1(=CC=CC=C1)S(=O)[O-].C1(=CC=CC=C1)C>>C1(=CC=CC=C1)S(=O)(=O)Cl
Cl[Cl:4].[O-:1][S:2](=[O:3])[c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1>>[O:1]=[S:2](=[O:3])([Cl:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1
ClCl.O=S([O-])c1ccccc1
O=S(=O)(Cl)c1ccccc1
null
null
O
Functional Group Interconversion
OtherReaction
03debb230351596239cbc9a8ae249800b74565d1aa45c11b464d4b120a8250ec
3855ae08274369907addf9929af01c270ce61e1e09fc64d8a51fac7fbb45a76b
c1ccccc1
Cl-[Cl;H0;D1;+0:1].[O-;H0;D1:2]-[S;H0;D3;+0:3](=[O;D1;H0:4])-[c:5](:[c:6]):[c:7]>>[Cl;H0;D1;+0:1]-[S;H0;D4;+0:3](=[O;D1;H0:4])(=[O;H0;D1;+0:2])-[c:5](:[c:6]):[c:7]
133.1
[{"value": 93.9, "product": "C1(=CC=CC=C1)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 133.1, "product": "C1(=CC=CC=C1)S(=O)(=O)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A reactor was charged with 29.3 g of sodium benzenesulfinate (0.14 mole) obtained by the fourth step, and the benzenesulfinate was dissolved in 65 mL of water. Then, 105 mL of toluene was charged, and 10.3 g (0.1456 mole, 1.04 times moles) of chlorine was, little by little, blown into the reactor at a temperature of 18...
10.6084/m9.figshare.5104873.v1
null
null
Sulfonyl halide
null
null
c1ccccc1
Other
O
null
null
ClCl.O=S([O-])c1ccccc1>O>O=S(=O)(Cl)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-18aca290182c4aa0a2257fc9e441bb3d
BrBr.O=S([O-])c1ccccc1>>O=S(=O)(Br)c1ccccc1
C1(=CC=CC=C1)S(=O)[O-].[Na+].BrBr>>C1(=CC=CC=C1)S(=O)(=O)Br
Br[Br:4].[O-:1][S:2](=[O:3])[c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1>>[O:1]=[S:2](=[O:3])([Br:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1
BrBr.O=S([O-])c1ccccc1
O=S(=O)(Br)c1ccccc1
null
null
null
Functional Group Interconversion
OtherReaction
03debb230351596239cbc9a8ae249800b74565d1aa45c11b464d4b120a8250ec
3855ae08274369907addf9929af01c270ce61e1e09fc64d8a51fac7fbb45a76b
c1ccccc1
Br-[Br;H0;D1;+0:1].[O-;H0;D1:2]-[S;H0;D3;+0:3](=[O;D1;H0:4])-[c:5](:[c:6]):[c:7]>>[Br;H0;D1;+0:1]-[S;H0;D4;+0:3](=[O;D1;H0:4])(=[O;H0;D1;+0:2])-[c:5](:[c:6]):[c:7]
null
[]
null
null
null
null
Benzenesulfonyl bromide was synthesized with 1316.0 g of the mother liquid containing sodium benzenesulfinate by procedures similar to those of the fourth step and the fifth step of Example 1 except that bromine was used instead of chlorine in the fifth step. Thus, 36.0 g of benzenesulfonyl bromide was yielded. Gas chr...
10.6084/m9.figshare.5104873.v1
null
null
Sulfonyl halide
null
null
c1ccccc1
Br-
null
null
null
BrBr.O=S([O-])c1ccccc1>>O=S(=O)(Br)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8c8d4afcbe4e4f69bad780bdcf58c27e
O=P12OP3(=O)OP(=O)(O1)OP(=O)(O2)O3>>O=P(O)(O)O
O=P12OP3(=O)OP(=O)(O1)OP(=O)(O2)O3.N1=C(N)N=C(N)N=C1N>>P(=O)(O)(O)O.N1=C(N)N=C(N)N=C1N
O=P12OP3(=O)OP(=O)(O1)[O:14][P:11](=[O:10])([O:12]2)[O:13]3>>[O:10]=[P:11]([OH:12])([OH:13])[OH:14]
O=P12OP3(=O)OP(=O)(O1)OP(=O)(O2)O3
O=P(O)(O)O
null
null
null
Reduction
OtherReaction
be33e0461de99a67340dcc65697c47721b35c23585c71f3b6499cfaa484c58ac
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
null
O=P12-O-P3(=O)-O-P(=O)(-O-1)-[O;H0;D2;+0:1]-[#15:2](=[O;D1;H0:3])(-[O;H0;D2;+0:4]-2)-[O;H0;D2;+0:5]-3>>[O;D1;H0:3]=[#15:2](-[OH;D1;+0:4])(-[OH;D1;+0:5])-[OH;D1;+0:1]
null
[]
null
null
null
null
Under atmosphere, charged in a twin-screw extruder were 70.97 g (0.5 moles) of diphosphorus pentoxide and 126.06 g (1.0 moles) of melamine (commercial name: Chang Chun Melamine), and a bar like product was formed at the extrusion temperature of 340° C. After being cooled, the bar like product is pulverized, thereby a p...
10.6084/m9.figshare.5104873.v1
null
null
null
O1P2OP3OP1OP(O2)O3
null
null
Other
null
null
null
O=P12OP3(=O)OP(=O)(O1)OP(=O)(O2)O3>>O=P(O)(O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-03b8a4bd98cb48cebc60c1aa63086a6b
O=C(O)CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl.OCCO>>O=C(CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl)OCCO
C(C)N(CC)CC.ClC(=O)OCC.Cl[C@@H]1C[C@H]([C@@H]([C@H]1C\C=C/CCCC(=O)O)COC1=CC(=CC(=C1)Cl)Cl)O.C(C)N(CC)CC.C(CO)O>>OCCOC(CCC\C=C/C[C@@H]1[C@H]([C@@H](C[C@H]1Cl)O)COC1=CC(=CC(=C1)Cl)Cl)=O
[O:1]=[C:2]([CH2:3][CH2:4][CH2:5]/[CH:6]=[CH:7]\[CH2:8][C@@H:9]1[C@@H:10]([CH2:11][O:12][c:13]2[cH:14][c:15]([Cl:16])[cH:17][c:18]([Cl:19])[cH:20]2)[C@H:21]([OH:22])[CH2:23][C@H:24]1[Cl:25])[OH:26].O[CH2:27][CH2:28][OH:29]>>[O:1]=[C:2]([CH2:3][CH2:4][CH2:5]/[CH:6]=[CH:7]\[CH2:8][C@@H:9]1[C@@H:10]([CH2:11][O:12][c:13]2[...
O=C(O)CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl.OCCO
O=C(CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl)OCCO
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
Esterification of Carboxylic Acids
3f9a9ace480b666da05fcfe5450d12b5c1ea5b0d435c195e1dd4bd20281604bb
dcbf04ec563ed0e9dfc79070490a028958024079a671c385858bb18cc8ec995a
c1ccc(OCC2CCCC2)cc1
O-[CH2;D2;+0:1]-[C:2]-[O;D1;H1:3].[C:4]-[C:5](=[O;D1;H0:6])-[OH;D1;+0:7]>>[C:4]-[C:5](=[O;D1;H0:6])-[O;H0;D2;+0:7]-[CH2;D2;+0:1]-[C:2]-[O;D1;H1:3]
22
[{"value": 22.0, "product": "OCCOC(CCC\\C=C/C[C@@H]1[C@H]([C@@H](C[C@H]1Cl)O)COC1=CC(=CC(=C1)Cl)Cl)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2.5
HOUR
Triethylamine (15 μL, 0.11 mmol) and ethyl chloroformate (15 μL, 0.16 mmol) were added sequentially to a solution of (Z)-7-[(1R,2S,3R,5R)-5-chloro-2-(3,5-dichloro-phenoxymethyl)-3-hydroxy-cyclopentyl]-hept-5-enoic acid (U.S. Provisional Patent Application No. 60/644,069, filed on Jan. 14, 2005, incorporated by referenc...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
C1CCCC1.c1ccccc1
HO-
C(Cl)Cl
null
2.5
O=C(O)CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl.OCCO>C(Cl)Cl>O=C(CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl)OCCO
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9cab839b31194353a02ded500c33c0b4
O=C(O)CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl.OCCN1CCOCC1>>O=C(CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl)OCCN1CCOCC1
C(C)N(CC)CC.ClC(=O)OCC.Cl[C@@H]1C[C@H]([C@@H]([C@H]1C\C=C/CCCC(=O)O)COC1=CC(=CC(=C1)Cl)Cl)O.C(C)N(CC)CC.OCCN1CCOCC1>>N1(CCOCC1)CCOC(CCC\C=C/C[C@@H]1[C@H]([C@@H](C[C@H]1Cl)O)COC1=CC(=CC(=C1)Cl)Cl)=O
O[C:2](=[O:1])[CH2:3][CH2:4][CH2:5]/[CH:6]=[CH:7]\[CH2:8][C@@H:9]1[C@@H:10]([CH2:11][O:12][c:13]2[cH:14][c:15]([Cl:16])[cH:17][c:18]([Cl:19])[cH:20]2)[C@H:21]([OH:22])[CH2:23][C@H:24]1[Cl:25].[OH:26][CH2:27][CH2:28][N:29]1[CH2:30][CH2:31][O:32][CH2:33][CH2:34]1>>[O:1]=[C:2]([CH2:3][CH2:4][CH2:5]/[CH:6]=[CH:7]\[CH2:8][C...
O=C(O)CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl.OCCN1CCOCC1
O=C(CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl)OCCN1CCOCC1
null
null
C(Cl)Cl
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
O=C(CCC/C=C\C[C@H]1CCC[C@@H]1COc1ccccc1)OCCN1CCOCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[C:5]-[C:6]-[OH;D1;+0:7]>>[C:5]-[C:6]-[O;H0;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]
20.3
[{"value": 20.0, "product": "N1(CCOCC1)CCOC(CCC\\C=C/C[C@@H]1[C@H]([C@@H](C[C@H]1Cl)O)COC1=CC(=CC(=C1)Cl)Cl)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 20.3, "product": "N1(CCOCC1)CCOC(CCC\\C=C/C[C@@H]1[C@H]([C@@H](C[C@H]1Cl)O)COC1=CC(=CC(=C1)Cl)Cl)=O", "details": "CALCULATEDPERCENTYIELD", "is_desir...
null
null
2.5
HOUR
Triethylamine (6.5 μL, 0.047 mmol) and ethyl chloroformate (7 μL, 0.073 mmol) were added sequentially to a solution of (Z)-7-[(1R,2S,3R,5R)-5-chloro-2-(3,5-dichloro-phenoxymethyl)-3-hydroxy-cyclopentyl]-hept-5-enoic acid (see U.S. 60/644,069, 20 mg, 0.047 mmol) in CH2Cl2 (0.47 mL) at room temperature. After 2.5 h, trie...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
c1ccccc1.C1CCCC1.C1COCC[NH]1
HO-
C(Cl)Cl
null
2.5
O=C(O)CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl.OCCN1CCOCC1>C(Cl)Cl>O=C(CCC/C=C\C[C@@H]1[C@@H](COc2cc(Cl)cc(Cl)c2)[C@H](O)C[C@H]1Cl)OCCN1CCOCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-416ea1cf0f1a47d29ae88e86e018323e
COC(=O)c1ccc(CN2CCN(C)CC2)cc1.Cc1ccc(N)cc1[N+](=O)[O-]>>Cc1ccc(NC(=O)c2ccc(CN3CCN(C)CC3)cc2)cc1[N+](=O)[O-]
CC=1C=CC(=CC1NC=2N=CC=C(N2)C=3C=CC=NC3)NC(=O)C=4C=CC(=CC4)CN5CCN(CC5)C.COC(C1=CC=C(C=C1)CN1CCN(CC1)C)=O.[N+](=O)([O-])C=1C=C(N)C=CC1C>>CC1=C(C=C(C=C1)NC(C1=CC=C(C=C1)CN1CCN(CC1)C)=O)[N+](=O)[O-]
CO[C:7](=[O:8])[c:9]1[cH:10][cH:11][c:12]([CH2:13][N:14]2[CH2:15][CH2:16][N:17]([CH3:18])[CH2:19][CH2:20]2)[cH:21][cH:22]1.[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH2:6])[cH:23][c:24]1[N+:25](=[O:26])[O-:27]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH:6][C:7](=[O:8])[c:9]2[cH:10][cH:11][c:12]([CH2:13][N:14]3[CH2:15][CH2:16][N:17]([CH3...
COC(=O)c1ccc(CN2CCN(C)CC2)cc1.Cc1ccc(N)cc1[N+](=O)[O-]
Cc1ccc(NC(=O)c2ccc(CN3CCN(C)CC3)cc2)cc1[N+](=O)[O-]
null
null
null
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
O=C(Nc1ccccc1)c1ccc(CN2CCNCC2)cc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9])-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
U.S. Pat. No. 5,521,184 and application WO 03/066613 describe several synthetic routes for preparing Imatinib. One synthetic process, described in Scheme 1, comprises reacting 4-(4-methyl-piperazin-1-ylmethyl)-benzoic acid methyl ester with 3-nitro-4-methyl-aniline to obtain N-(4-methyl-3-nitrophenyl)-4-(4-methyl-piper...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.C1C[NH]CC[NH]1
HO-
null
null
null
COC(=O)c1ccc(CN2CCN(C)CC2)cc1.Cc1ccc(N)cc1[N+](=O)[O-]>>Cc1ccc(NC(=O)c2ccc(CN3CCN(C)CC3)cc2)cc1[N+](=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e436ac9eddd74505a2e8805f5065c111
COC(=O)c1ccc(CN2CCN(C)CC2)cc1.Cc1ccc(N)cc1Br>>Cc1ccc(NC(=O)c2ccc(CN3CCN(C)CC3)cc2)cc1Br
BrC=1C=C(N)C=CC1C.COC(C1=CC=C(C=C1)CN1CCN(CC1)C)=O>>BrC=1C=C(C=CC1C)NC(C1=CC=C(C=C1)CN1CCN(CC1)C)=O
CO[C:7](=[O:8])[c:9]1[cH:10][cH:11][c:12]([CH2:13][N:14]2[CH2:15][CH2:16][N:17]([CH3:18])[CH2:19][CH2:20]2)[cH:21][cH:22]1.[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH2:6])[cH:23][c:24]1[Br:25]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH:6][C:7](=[O:8])[c:9]2[cH:10][cH:11][c:12]([CH2:13][N:14]3[CH2:15][CH2:16][N:17]([CH3:18])[CH2:19][CH...
COC(=O)c1ccc(CN2CCN(C)CC2)cc1.Cc1ccc(N)cc1Br
Cc1ccc(NC(=O)c2ccc(CN3CCN(C)CC3)cc2)cc1Br
null
null
null
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
O=C(Nc1ccccc1)c1ccc(CN2CCNCC2)cc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9])-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Yet another process, described in Scheme 3, comprises reacting 3-bromo-4-methyl-aniline with 4-(4-methyl-piperazin-1-ylmethyl)-benzoic acid methyl ester to obtain N-(3-bromo-4-methyl-phenyl)-4-(4-methyl-piperazin-1-ylmethyl)-benzamide. The latter is reacted with 4-(3-pyridyl)-2-pyrimidine amine (which is obtained by re...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.C1C[NH]CC[NH]1
HO-
null
null
null
COC(=O)c1ccc(CN2CCN(C)CC2)cc1.Cc1ccc(N)cc1Br>>Cc1ccc(NC(=O)c2ccc(CN3CCN(C)CC3)cc2)cc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8725b9be91ba463d97f26d5b8682a8f5
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1>>Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
ClC1=NC=CC(=N1)C=1C=NC=CC1.NC1=C(C=CC(=C1)[N+](=O)[O-])C>>CC1=C(C=C(C=C1)[N+](=O)[O-])NC1=NC=CC(=N1)C=1C=NC=CC1
[CH3:1][c:2]1[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][c:10]1[NH2:11].Cl[c:12]1[n:13][cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][cH:20][n:21][cH:22]2)[n:23]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][c:10]1[NH:11][c:12]1[n:13][cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][cH:20][n:21][cH:22]2)[n:23]1
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1
Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
null
null
null
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
c38b7155556ff28144ae37859ff6668b20d59da60c705d26b158542b6d8385da
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2nccc(-c3cccnc3)n2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]):[#7;a:4]:[c:5]
null
[]
null
null
null
null
Thus, Imatinib is obtained by a synthetic route comprising reacting 2-chloro-4-(3-pyridyl)-pyrimidine with 2-amino-4-nitro-toluene to obtain N-(2-methyl-5-nitrophenyl)-4-(3-pyridyl)-2-pyrimidine-amine, which is subsequently reduced and reacted with 4-(4-methyl-piperazine-1-ylmethyl)-benzoyl chloride to yield the final ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.c1ccncc1
HCl
null
null
null
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1>>Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b227e15041494e41aa620cd9dbef7f8b
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1>>Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
ClC1=NC=CC(=N1)C=1C=NC=CC1.NC1=C(C=CC(=C1)[N+](=O)[O-])C>>CC1=C(C=C(C=C1)[N+](=O)[O-])NC1=NC=CC(=N1)C=1C=NC=CC1
[CH3:1][c:2]1[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][c:10]1[NH2:11].Cl[c:12]1[n:13][cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][cH:20][n:21][cH:22]2)[n:23]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][c:10]1[NH:11][c:12]1[n:13][cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][cH:20][n:21][cH:22]2)[n:23]1
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1
Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
null
null
null
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
c38b7155556ff28144ae37859ff6668b20d59da60c705d26b158542b6d8385da
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2nccc(-c3cccnc3)n2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]):[#7;a:4]:[c:5]
null
[]
null
null
null
null
Thus, Imatinib or an addition salt thereof is obtained by a synthetic route comprising reacting 2-chloro-4-(3-pyridyl)-pyrimidine with 2-amino-4-nitro-toluene to obtain N-(2-methyl-5-nitrophenyl)-4-(3-pyridyl)-2-pyrimidine-amine, which is subsequently reduced and reacted with 4-(4-methyl-piperazine-1-ylmethyl)-benzoyl ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.c1ccncc1
HCl
null
null
null
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1>>Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-87bb5e01cf2e42c38248e11b31a483e7
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1>>Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
ClC1=NC=CC(=N1)C=1C=NC=CC1.NC1=C(C=CC(=C1)[N+](=O)[O-])C.[OH-].[Na+]>>CC1=C(C=C(C=C1)[N+](=O)[O-])NC1=NC=CC(=N1)C=1C=NC=CC1
[CH3:1][c:2]1[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][c:10]1[NH2:11].Cl[c:12]1[n:13][cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][cH:20][n:21][cH:22]2)[n:23]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][c:10]1[NH:11][c:12]1[n:13][cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][cH:20][n:21][cH:22]2)[n:23]1
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1
Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
null
Cl
C(CCC)O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
c38b7155556ff28144ae37859ff6668b20d59da60c705d26b158542b6d8385da
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2nccc(-c3cccnc3)n2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]):[#7;a:4]:[c:5]
null
[]
null
null
null
null
A 250 ml reactor, equipped with a mechanical stirrer and a reflux condenser, was charged with 2-chloro-4-(3-pyridyl)-pyrimidine (0.5 g, 2.6 mmol), 2-amino-4-nitrotoluene (0.5 g, 3.2 mmol), n-butanol (15 ml) and concentrated HCl (5 drops) and the mixture was refluxed for 38 hours. Then, the mixture was cooled, and 6 N N...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.c1ccncc1
HCl
Cl.C(CCC)O
null
null
Cc1ccc([N+](=O)[O-])cc1N.Clc1nccc(-c2cccnc2)n1>Cl.C(CCC)O>Cc1ccc([N+](=O)[O-])cc1Nc1nccc(-c2cccnc2)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ff18a2aec00d4640b92b602960780621
OC(CN1CCCC1)c1ccccc1>>O[C@@H](CN1CCCC1)c1ccccc1
C(C1=CC=CC=C1)(=O)OC([C@H](O)[C@@H](O)C(=O)OC(C1=CC=CC=C1)=O)=O.C1(=CC=CC=C1)C(CN1CCCC1)O>>C1(=CC=CC=C1)[C@H](CN1CCCC1)O
[OH:1][CH:2]([CH2:3][N:4]1[CH2:5][CH2:6][CH2:7][CH2:8]1)[c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1>>[OH:1][C@@H:2]([CH2:3][N:4]1[CH2:5][CH2:6][CH2:7][CH2:8]1)[c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1
OC(CN1CCCC1)c1ccccc1
O[C@@H](CN1CCCC1)c1ccccc1
null
null
CO.[OH-].[Na+]
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
c1ccc(CCN2CCCC2)cc1
null
null
[]
null
null
2
DAY
Solutions of 35.8 g of di-O-benzoyl-L-tartaric acid in 150 ml methanol and 19.1 g of 1-phenyl-2-(1-pyrrolidinyl)-ethanol in 100 ml of methanol were mixed and the mixture left standing in a refrigerator for 2 days. The crystalline product was filtered off, washed with a small amount of cold methanol and diethyl ether an...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
C1CC[NH]C1.c1ccccc1
null
CO.[OH-].[Na+]
null
48
OC(CN1CCCC1)c1ccccc1>CO.[OH-].[Na+]>O[C@@H](CN1CCCC1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-86cc9ea167154d3690d3c13678780072
O=C(Cl)C(Cl)c1ccccc1Cl.O[C@@H](CN1CCCC1)c1ccccc1>>O=C(O[C@@H](CN1CCCC1)c1ccccc1)C(Cl)c1ccccc1Cl
C1(=CC=CC=C1)[C@H](CN1CCCC1)O.ClC1=C(C=CC=C1)C(C(=O)Cl)Cl>>N1(CCCC1)C[C@@H](C1=CC=CC=C1)OC(C(Cl)C1=C(C=CC=C1)Cl)=O
Cl[C:2](=[O:1])[CH:17]([Cl:18])[c:19]1[cH:20][cH:21][cH:22][cH:23][c:24]1[Cl:25].[OH:3][C@@H:4]([CH2:5][N:6]1[CH2:7][CH2:8][CH2:9][CH2:10]1)[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[O:1]=[C:2]([O:3][C@@H:4]([CH2:5][N:6]1[CH2:7][CH2:8][CH2:9][CH2:10]1)[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)[CH:17]([Cl:18])[c:19...
O=C(Cl)C(Cl)c1ccccc1Cl.O[C@@H](CN1CCCC1)c1ccccc1
O=C(O[C@@H](CN1CCCC1)c1ccccc1)C(Cl)c1ccccc1Cl
null
CN(C)C1=CC=NC=C1
O1CCCC1
Acylation
Schotten-Baumann to ester
27b76e29491fa7db5375755e15223de884a194f57a493147db0b5495ea981908
d47ab90ace9b5dcd818151c10aae400dcf599f5a3476072b8dfedc474e97c335
O=C(Cc1ccccc1)O[C@@H](CN1CCCC1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[Cl;D1;H0:4])-[c:5].[C:6]-[C:7](-[OH;D1;+0:8])-[c:9]>>[C:6]-[C:7](-[c:9])-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[Cl;D1;H0:4])-[c:5]
null
[]
null
null
null
null
A solution of 5.7 g of (R)-1-phenyl-2-(1-pyrrolidinyl)-ethanol in 25 ml of tetrahydrofurane was added to a solution of 6.5 g of 2,α-dichlorophenyl acetyl chloride in 25 ml of tetrahydrofurane containing 0.9 g of 4-dimethylamine pyridine. According to a similar procedure as in example 3, a mixture of diastereomeric este...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary alcohol
Ester
null
null
C1CC[NH]C1.c1ccccc1.c1ccccc1
HCl
CN(C)C1=CC=NC=C1.O1CCCC1
null
null
O=C(Cl)C(Cl)c1ccccc1Cl.O[C@@H](CN1CCCC1)c1ccccc1>CN(C)C1=CC=NC=C1.O1CCCC1>O=C(O[C@@H](CN1CCCC1)c1ccccc1)C(Cl)c1ccccc1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-735eeb16aa944771b06909321c4eb700
CN(C)CC(O)c1ccccc1>>CN(C)C[C@H](O)c1ccccc1
CN(CC(O)C1=CC=CC=C1)C.C1(=CC=CC=C1)[C@H](CN1CCCC1)O.NO>>CN(C[C@H](O)C1=CC=CC=C1)C
[CH3:1][N:2]([CH3:3])[CH2:4][CH:5]([OH:6])[c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1>>[CH3:1][N:2]([CH3:3])[CH2:4][C@H:5]([OH:6])[c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1
CN(C)CC(O)c1ccccc1
CN(C)C[C@H](O)c1ccccc1
null
null
CO
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
c1ccccc1
null
null
[]
null
null
null
null
Racemic 2-dimethylamino-1-phenyl ethanol was cleaved in accordance with the 2-pyrrolidinyl-1-phenyl ethanol (see example 6) using 16.5 g of crude amino alcohol as described in example 8. The yield of oily (R)-2-dimethyl-amino-1-phenyl ethanol with a [αD20] value of −45.5° (methanol) was 8.9 g. Conditions: See reaction....
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1
null
CO
null
null
CN(C)CC(O)c1ccccc1>CO>CN(C)C[C@H](O)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ebf0d7669a01422dbfdb9f26b0eb75bf
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC>>COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC.[OH-]
COC=1C=CN=C(C1OC)C[S+](C=2[N-]C=3C=CC(=CC3N2)OC(F)F)[O-].[Na+]>>COC=1C=CN=C(C1OC)C[S+](C=2NC=3C=CC(=CC3N2)OC(F)F)[O-].[OH-].[Na+]
[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([CH2:8][S+:9]([O-:10])[c:11]2[n:12][c:13]3[cH:14][c:15]([O:16][CH:17]([F:18])[F:19])[cH:20][cH:21][c:22]3[n-:23]2)[c:24]1[O:25][CH3:26]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([CH2:8][S+:9]([O-:10])[c:11]2[n:12][c:13]3[cH:14][c:15]([O:16][CH:17]([F:18])[F:19])[cH:20][cH:21][c:...
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC.[OH-]
null
null
CC(=O)C
Functional Group Interconversion
OtherReaction
0d6fc6eb01acfd45833b397c8f5a76a7184fae8843ce3428d595feb9c6adf18e
f1bbf9aa3c82f5e49be9f6d53533b6bb152f359232b6d32090c168949766aa71
c1ccc(C[SH+]c2nc3ccccc3[nH]2)nc1
[#16;+:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[n-;H0;D2:8]:1>>[#16;+:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[nH;D2;+0:8]:1
null
[]
null
null
null
null
Pantoprazole sodium Form II can be prepared by forming a solution of pantoprazole and excess sodium hydroxide in acetone and crystallizing Form II from the solution. Preferably, pantoprazole is added as the free base, though the sodium salt may be used. Excess sodium hydroxide is conveniently added as a concentrated aq...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2[n-]cnc2c1
c1ccc2[nH]cnc2c1
c1ccncc1.c1ccc2[nH]cnc2c1
null
CC(=O)C
null
null
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC>CC(=O)C>COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC.[OH-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-acbab0da268a4f189510e34f7728fec5
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC>>COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
[OH-].[Na+].[OH-].[Na+].COC=1C=CN=C(C1OC)C[S+](C=2NC=3C=CC(=CC3N2)OC(F)F)[O-].COC=1C=CN=C(C1OC)C[S+](C=2NC=3C=CC(=CC3N2)OC(F)F)[O-]>>COC=1C=CN=C(C1OC)C[S+](C=2[N-]C=3C=CC(=CC3N2)OC(F)F)[O-].[Na+]
[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([CH2:8][S+:9]([O-:10])[c:11]2[n:12][c:13]3[cH:14][c:15]([O:16][CH:17]([F:18])[F:19])[cH:20][cH:21][c:22]3[nH:23]2)[c:24]1[O:25][CH3:26]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([CH2:8][S+:9]([O-:10])[c:11]2[n:12][c:13]3[cH:14][c:15]([O:16][CH:17]([F:18])[F:19])[cH:20][cH:21][c:...
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
null
null
CC(=O)C
Reduction
OtherReaction
73e3c5abcbae739c230bd8787a8ba86237c4832ac4b8d9821b3e0022b929d7b0
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
c1ccc(C[SH+]c2nc3ccccc3[n-]2)nc1
[#16;+:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[nH;D2;+0:8]:1>>[#16;+:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[n-;H0;D2:8]:1
65
[{"value": 65.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
2
CELSIUS
2
HOUR
A 100 ml round bottomed flask equipped with a magnetic stir bar was charged with acetone (50 ml). Pantoprazole (10 g, 25.7 mmol) was then added to the flask. After the pantoprazole had completely dissolved, the solution was cooled to about 2° C. Forty seven percent sodium hydroxide (aq.) equivalent to 2.4 grams of soli...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2[nH]cnc2c1
c1ccc2[n-]cnc2c1
c1ccncc1.c1ccc2[n-]cnc2c1
null
CC(=O)C
2
2
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC>CC(=O)C>COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-accc83431eda449d8f9bf1d3f65d93f7
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC>>COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
COC=1C=CN=C(C1OC)C[S+](C=2NC=3C=CC(=CC3N2)OC(F)F)[O-].[OH-].[Na+]>>COC=1C=CN=C(C1OC)C[S+](C=2[N-]C=3C=CC(=CC3N2)OC(F)F)[O-].[Na+]
[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([CH2:8][S+:9]([O-:10])[c:11]2[n:12][c:13]3[cH:14][c:15]([O:16][CH:17]([F:18])[F:19])[cH:20][cH:21][c:22]3[nH:23]2)[c:24]1[O:25][CH3:26]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([CH2:8][S+:9]([O-:10])[c:11]2[n:12][c:13]3[cH:14][c:15]([O:16][CH:17]([F:18])[F:19])[cH:20][cH:21][c:...
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
null
null
C1(=CC=CC=C1)C
Reduction
OtherReaction
73e3c5abcbae739c230bd8787a8ba86237c4832ac4b8d9821b3e0022b929d7b0
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
c1ccc(C[SH+]c2nc3ccccc3[n-]2)nc1
[#16;+:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[nH;D2;+0:8]:1>>[#16;+:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[n-;H0;D2:8]:1
null
[]
null
null
null
null
A 100 ml flask was charged with toluene (50.0 ml). Pantoprazole (5.0 g, 12.8 mmol) and 47% aqueous NaOH (1.2 g) were added to the stirred solvent at room temperature. The mixture was stirred until dissolution and then overnight until precipitation. The solid was filtered giving pantoprazole sodium. The sample was dried...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2[nH]cnc2c1
c1ccc2[n-]cnc2c1
c1ccncc1.c1ccc2[n-]cnc2c1
null
C1(=CC=CC=C1)C
null
null
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC>C1(=CC=CC=C1)C>COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ee860321d9234dfc9df03d96e37fd037
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC>>COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
COC=1C=CN=C(C1OC)C[S+](C=2NC=3C=CC(=CC3N2)OC(F)F)[O-].[OH-].[Na+]>>COC=1C=CN=C(C1OC)C[S+](C=2[N-]C=3C=CC(=CC3N2)OC(F)F)[O-].[Na+]
[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([CH2:8][S+:9]([O-:10])[c:11]2[n:12][c:13]3[cH:14][c:15]([O:16][CH:17]([F:18])[F:19])[cH:20][cH:21][c:22]3[nH:23]2)[c:24]1[O:25][CH3:26]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([CH2:8][S+:9]([O-:10])[c:11]2[n:12][c:13]3[cH:14][c:15]([O:16][CH:17]([F:18])[F:19])[cH:20][cH:21][c:...
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
null
null
C(CCC)O
Reduction
OtherReaction
73e3c5abcbae739c230bd8787a8ba86237c4832ac4b8d9821b3e0022b929d7b0
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
c1ccc(C[SH+]c2nc3ccccc3[n-]2)nc1
[#16;+:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[nH;D2;+0:8]:1>>[#16;+:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[n-;H0;D2:8]:1
null
[]
null
null
8
HOUR
Pantoprazole (5.0 g, 12.8 mmol) and 98.5% NaOH (0.52 g, 12.8 mmol) were dissolved in 1-butanol (10.0 ml) at room temperature and the solution was stirred overnight at room temperature. The solution was cooled in a refrigerator and then stirred at room temperature until crystallization occurred. The crystals were filter...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2[nH]cnc2c1
c1ccc2[n-]cnc2c1
c1ccncc1.c1ccc2[n-]cnc2c1
null
C(CCC)O
null
8
COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[nH]2)c1OC>C(CCC)O>COc1ccnc(C[S+]([O-])c2nc3cc(OC(F)F)ccc3[n-]2)c1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0a84cd2ef25e4324b93bae980fdd2e4a
COc1ccc(C#N)cc1.[Cl][Mg][c]1ccccc1>>COc1ccc(-c2ccccc2)cc1
COC1=CC=C(C#N)C=C1.CCCCCCCCCCCCC.C1(=CC=CC=C1)[Mg]Cl.[Cl-].C1(=CC=CC=C1)[Zn+]>>C1(=CC=CC=C1)C1=CC=C(C=C1)OC
N#C[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:14][cH:13]1.[Cl][Mg][c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][cH:14]1
COc1ccc(C#N)cc1.[Cl][Mg][c]1ccccc1
COc1ccc(-c2ccccc2)cc1
null
[Cl-].[Zn+2].[Cl-]
C1CCOC1
C-C Coupling
OtherReaction
56fd8131e2b4058a94fc10996ce554527798dacc8dc497c879f344f9b79d88bf
b7d29fa9e0a7d9ae2f2a2797da751d9d03a466b58f528baa09db504746325a44
c1ccc(-c2ccccc2)cc1
N#C-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[Cl]-[Mg]-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
45
[{"value": 45.0, "product": "C1(=CC=CC=C1)C1=CC=C(C=C1)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A solution of zinc chloride (0.48 g; 3.5 mmol) in THF (5 mL) was treated at 0° C. with phenylmagnesium chloride (2.1 mL of a 1.40 M solution in THF; 3.0 mmol) and then stirred at room temperature for 30 min. The mixture of phenylzinc chloride thus obtained was then treated with a solution of 4-methoxybenzonitrile (0.27...
10.6084/m9.figshare.5104873.v1
null
Magnesium halide.Nitrile
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
Mg
[Cl-].[Zn+2].[Cl-].C1CCOC1
null
0.5
COc1ccc(C#N)cc1.[Cl][Mg][c]1ccccc1>[Cl-].[Zn+2].[Cl-].C1CCOC1>COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e718b5c472454dc0b21020ceafb9ad37
COc1ccc(C(=N)c2ccccc2)cc1>>COc1ccc(-c2ccccc2)cc1
CP(C)C.COC1=CC=C(C(C2=CC=CC=C2)=N)C=C1>>C1(=CC=CC=C1)C1=CC=C(C=C1)OC
N=C([c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:14][cH:13]1)[c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][cH:14]1
COc1ccc(C(=N)c2ccccc2)cc1
COc1ccc(-c2ccccc2)cc1
null
C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2].[Ni]
null
Miscellaneous
OtherReaction
999b65ddf01d6c95f0b4375b9a2a5471c9ffe6453f7cf55d73aa81009d3ea1a1
f84f44e4c005115224407dbb994558777a16078301b35734330b6ae282e29f41
c1ccc(-c2ccccc2)cc1
N=C(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
1,600
[{"value": 88.0, "product": "C1(=CC=CC=C1)C1=CC=C(C=C1)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 1600.0, "product": "C1(=CC=CC=C1)C1=CC=C(C=C1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
The procedure was identical to Example 1, with the exception that the nickel catalyst used was derived in situ from a combination of anhydrous nickel acetylacetonate (0.026 g; 5 mol %) and trimethylphosphine (0.20 mL of 1 M solution in toluene; 10 mol %). GC analysis of the organic phase of the hydrolyzed reaction samp...
10.6084/m9.figshare.5104873.v1
null
Unsubstituted imine
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
Other
C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2].[Ni]
null
2
COc1ccc(C(=N)c2ccccc2)cc1>C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2].[Ni]>COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f1e894c4dd8b47c4ba10a08c0c0a36ee
COc1ccc(C#N)cc1.[Li][c]1ccccc1>>COc1ccc(-c2ccccc2)cc1
[Br-].[Mg+2].[Br-].C1(=CC=CC=C1)[Li].COC1=CC=C(C(C2=CC=CC=C2)=N)C=C1.COC1=CC=C(C#N)C=C1.CCCCCCCCCCCCC.CC(C)([O-])C.[Li+]>>C1(=CC=CC=C1)C1=CC=C(C=C1)OC
N#C[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:14][cH:13]1.[Li][c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][cH:14]1
COc1ccc(C#N)cc1.[Li][c]1ccccc1
COc1ccc(-c2ccccc2)cc1
null
null
C1CCOC1
C-C Coupling
OtherReaction
a2248e0771f91e7acef322ad94f7832605ad21867c930450f56e5d8ce491f5d1
4318d1235968fbd93d528a51f6640671795eb99dc2e7ea1a67f893a1c90dbeea
c1ccc(-c2ccccc2)cc1
N#C-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[Li]-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
927.8
[{"value": 84.0, "product": "C1(=CC=CC=C1)C1=CC=C(C=C1)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 927.8, "product": "C1(=CC=CC=C1)C1=CC=C(C=C1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
1
HOUR
A slurry of magnesium bromide (0.74 g; 4.0 mmol) in THF (3 mL) was treated at room temperature with phenyllithium (2.4 mL of 1.7 M solution; 4.0 mmol). The solution was heated at 60° C. for 30 min, and was then treated at 60° with lithium t-butoxide (4.4 mL of 1.0 M solution in THF; 4.4 mmol) and heating was continued ...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Aryl lithium
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
Li
C1CCOC1
60
1
COc1ccc(C#N)cc1.[Li][c]1ccccc1>C1CCOC1>COc1ccc(-c2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fa11e0ea87004180a859d61e27aca6b0
N#Cc1ccncc1.[Cl][Mg][c]1ccccc1>>c1ccc(-c2ccncc2)cc1
C1(=CC=CC=C1)[Mg]Cl.C1(=CC=CC=C1)S[Li].C(CC(O)(C(=O)[O-])CC(=O)[O-])(=O)[O-].[Na+].[Na+].[Na+].C1(=CC=CC=C1)[Mg]Cl.[S-]C1=CC=CC=C1.[Li+].C(#N)C1=CC=NC=C1>>C1(=CC=CC=C1)C1=CC=NC=C1
N#C[c:5]1[cH:6][cH:7][n:8][cH:9][cH:10]1.[Cl][Mg][c:4]1[cH:3][cH:2][cH:1][cH:12][cH:11]1>>[cH:1]1[cH:2][cH:3][c:4](-[c:5]2[cH:6][cH:7][n:8][cH:9][cH:10]2)[cH:11][cH:12]1
N#Cc1ccncc1.[Cl][Mg][c]1ccccc1
c1ccc(-c2ccncc2)cc1
null
CP(C)C.C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2]
C1CCOC1
C-C Coupling
OtherReaction
c8abdf91a8398fd6e178d6f3f9e9bc7bc7bbe51804c0a725a9a427d4c11ded30
b7d29fa9e0a7d9ae2f2a2797da751d9d03a466b58f528baa09db504746325a44
c1ccc(-c2ccncc2)cc1
N#C-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5]:[c:6]:1.[Cl]-[Mg]-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]>>[c:9]:[c:8]:[c;H0;D3;+0:7](-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5]:[c:6]:1):[c:10]:[c:11]
94.5
[{"value": 91.0, "product": "C1(=CC=CC=C1)C1=CC=NC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.5, "product": "C1(=CC=CC=C1)C1=CC=NC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
10
MINUTE
In a 1 L 3-neck flask, equipped with a mechanical stirrer, were mixed phenyl magnesium chloride (96.1 mL; 192 mmol; 2.00 M in THF) and lithium thiophenoxide (211 mL; 211 mmol; 1.00 M THF) under a blanket of nitrogen. This mixture was heated to 60° C. for 1 h, and then cooled to 0-5° C. with an ice bath. In a separate 1...
10.6084/m9.figshare.5104873.v1
null
Magnesium halide.Nitrile
null
c1ccncc1.c1ccccc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
Mg
CP(C)C.C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2].C1CCOC1
60
0.166667
N#Cc1ccncc1.[Cl][Mg][c]1ccccc1>CP(C)C.C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Ni+2].C1CCOC1>c1ccc(-c2ccncc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5ce591e79cf64ac3bfff0cc32f5b5f8a
CN(C)c1ccc(CN)cc1.NCCCC(=O)OCc1ccccc1.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl>>CN(C)c1ccc(CNC(=O)NCCCC(=O)OCc2ccccc2)cc1
Cl.Cl.CN(C1=CC=C(CN)C=C1)C.C1(=CC=C(C=C1)S(=O)(=O)O)C.C(C1=CC=CC=C1)OC(CCCN)=O.ClC(Cl)(OC(OC(Cl)(Cl)Cl)=O)Cl.C(C)N(CC)CC.C(C)N(CC)CC>>C(C1=CC=CC=C1)OC(CCCNC(=O)NCC1=CC=C(C=C1)N(C)C)=O
[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][NH2:9])[cH:26][cH:27]1.[NH2:12][CH2:13][CH2:14][CH2:15][C:16](=[O:17])[O:18][CH2:19][c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1.ClC(Cl)(Cl)O[C:10](OC(Cl)(Cl)Cl)=[O:11]>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][NH:9][C:10](=[O:11])[NH:12][CH2:13][CH2:14][C...
CN(C)c1ccc(CN)cc1.NCCCC(=O)OCc1ccccc1.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl
CN(C)c1ccc(CNC(=O)NCCCC(=O)OCc2ccccc2)cc1
null
null
ClCCl.[Cl-].[Na+].O
Acylation
OtherReaction
28ee7ff95d738e45269fa5b469f275a1296c4b167a5d0563a291181ae7540ff4
9b884e2244637471aa1727f9c16919cb29ddb345e1156c83044a8879831c507f
O=C(NCCCC(=O)OCc1ccccc1)NCc1ccccc1
Cl-C(-Cl)(-Cl)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-O-C(-Cl)(-Cl)-Cl.[C:3]-[C:4]-[NH2;D1;+0:5].[NH2;D1;+0:6]-[C:7]-[c:8]>>[C:3]-[C:4]-[NH;D2;+0:5]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:6]-[C:7]-[c:8]
278.4
[{"value": 93.0, "product": "C(C1=CC=CC=C1)OC(CCCNC(=O)NCC1=CC=C(C=C1)N(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 278.4, "product": "C(C1=CC=CC=C1)OC(CCCNC(=O)NCC1=CC=C(C=C1)N(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a vigorous stirred suspension of 4-amino-butyric acid benzyl ester toluene-4-sulfonic acid (0.730 g, 2.00 mmol) and triphosgene (0.200 g, 0.667 mmol) in dichloromethane (40 mL) at −78° C. under nitrogen atmosphere, was added triethylamine (1.0 mL, 7.188 mmol, in 10 mL dichloromethane) dropwise via an additional f un...
10.6084/m9.figshare.5104873.v1
null
Trichloro group.Trichloro group.Carbonic Ester.Primary amine.Primary amine
Urea
null
null
c1ccccc1.c1ccccc1
HCl
ClCCl.[Cl-].[Na+].O
null
1
CN(C)c1ccc(CN)cc1.NCCCC(=O)OCc1ccccc1.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl>ClCCl.[Cl-].[Na+].O>CN(C)c1ccc(CNC(=O)NCCCC(=O)OCc2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-00df31b315224b0db81c5d1232c5d610
CN(C)c1ccc(CNC(=O)NCCCC(=O)NOCc2ccccc2)cc1>>CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1
C(C1=CC=CC=C1)ONC(CCCNC(=O)NCC1=CC=C(C=C1)N(C)C)=O>>CN(C1=CC=C(CNC(NCCCC(=O)NO)=O)C=C1)C
c1ccc(C[O:19][NH:18][C:16]([CH2:15][CH2:14][CH2:13][NH:12][C:10]([NH:9][CH2:8][c:7]2[cH:6][cH:5][c:4]([N:2]([CH3:1])[CH3:3])[cH:21][cH:20]2)=[O:11])=[O:17])cc1>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][NH:9][C:10](=[O:11])[NH:12][CH2:13][CH2:14][CH2:15][C:16](=[O:17])[NH:18][OH:19])[cH:20][cH:21]1
CN(C)c1ccc(CNC(=O)NCCCC(=O)NOCc2ccccc2)cc1
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1
null
[Pd]
CO
Deprotection
OtherReaction
94fa5e5ed4a5b32c4aba0dd3c8151bfdd08491d1bc6453e9fd01d7dc3e51cd0f
30a26bc929988d0041b9998cdccd1d65eb125114a78065ed35d40f50c965c0a7
c1ccccc1
[C:1]-[C:2](=[O;D1;H0:3])-[#7:4]-[O;H0;D2;+0:5]-C-c1:c:c:c:c:c:1>>[C:1]-[C:2](=[O;D1;H0:3])-[#7:4]-[OH;D1;+0:5]
92
[{"value": 92.0, "product": "CN(C1=CC=C(CNC(NCCCC(=O)NO)=O)C=C1)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
To a solution of the N-benzyloxy-4-[3-(4-dimethylamino-benzyl)-ureido]-butyramide (287 mg, 0.747 mmol) in methanol (15 mL) was added 10% palladium on carbon (30 mg) and the resulting reaction was allowed to stir under a hydrogen atmosphere for 18 hr, after which time the reaction mixture was filtered and concentrated i...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccccc1
null
c1ccccc1
Other
[Pd].CO
null
18
CN(C)c1ccc(CNC(=O)NCCCC(=O)NOCc2ccccc2)cc1>[Pd].CO>CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-18bf322cf855490798bee4e2e84b2ef0
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCCCCCCC(=O)OCc1ccccc1>>CN(C)c1ccc(CNC(=O)NCCCCCCC(=O)O)cc1
CN(C1=CC=C(CNC(NCCCC(=O)NO)=O)C=C1)C.C1(=CC=C(C=C1)S(=O)(=O)O)C.C(C1=CC=CC=C1)OC(CCCCCCN)=O>>CN(C1=CC=C(CNC(NCCCCCCC(=O)O)=O)C=C1)C
O=C(CCC[NH:12][C:10]([NH:9][CH2:8][c:7]1[cH:6][cH:5][c:4]([N:2]([CH3:1])[CH3:3])[cH:23][cH:22]1)=[O:11])NO.N[CH2:13][CH2:14][CH2:15][CH2:16][CH2:17][CH2:18][C:19](=[O:20])[O:21]Cc1ccccc1>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][NH:9][C:10](=[O:11])[NH:12][CH2:13][CH2:14][CH2:15][CH2:16][CH2:17][CH2:18][C:1...
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCCCCCCC(=O)OCc1ccccc1
CN(C)c1ccc(CNC(=O)NCCCCCCC(=O)O)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
84557db8ac0eb45fb3642de4953af83589cffc7690b4bd1e8855bf3ebb1bc4a3
e842414270b5e623bfbd8162311e9e13a2410702e3adaac65a4ee3622d82a9fc
c1ccccc1
N-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5](=[O;D1;H0:6])-[O;H0;D2;+0:7]-C-c1:c:c:c:c:c:1.O-N-C(=O)-C-C-C-[NH;D2;+0:8]-[C:9](=[O;D1;H0:10])-[#7:11]-[C:12]>>[C:4]-[C:5](=[O;D1;H0:6])-[OH;D1;+0:7].[C:3]-[C:2]-[CH2;D2;+0:1]-[NH;D2;+0:8]-[C:9](=[O;D1;H0:10])-[#7:11]-[C:12]
null
[]
null
null
null
null
Compound 5 was prepared using the methodology described for the preparation of compound 2, by substituting 4-amino-butyric acid benzyl ester toluene-4-sulfonic acid with 7-amino-heptanoic acid benzyl ester toluene-4-sulfonic acid. 1H NMR (300 MHz, DMSO-d6) δ (ppm) 10.33 (br, s, 1H), 8.66 (br s, 1H), 7.05 (d, J=8.7 Hz, ...
10.6084/m9.figshare.5104873.v1
null
Ester.Urea.Secondary amide.Primary amine
Carboxylic acid.Urea
c1ccccc1
null
c1ccccc1
HO-
null
null
null
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCCCCCCC(=O)OCc1ccccc1>>CN(C)c1ccc(CNC(=O)NCCCCCCC(=O)O)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2e7e9aaa12b44c748f460225f6b25d9c
CN(C)c1ccc(CN)cc1.Cc1ccc(S(=O)(=O)O)cc1.NCCCCCC(=O)OCc1ccccc1.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl>>O=C(NCCCCCC(=O)OCc1ccccc1)NC12CC3CC(CC(C3)C1)C2
Cl.Cl.CN(C1=CC=C(CN)C=C1)C.C1(=CC=C(C=C1)S(=O)(=O)O)C.C(C1=CC=CC=C1)OC(CCCCCN)=O.ClC(Cl)(OC(OC(Cl)(Cl)Cl)=O)Cl.C(C)N(CC)CC>>C(C1=CC=CC=C1)OC(CCCCCNC(=O)NC12CC3CC(CC(C1)C3)C2)=O
CN(C)[c:25]1c[cH:21][c:22]([CH2:20][NH2:19])[cH:27][cH:26]1.O=S(=O)(O)c1cc[c:24]([CH3:23])cc1.[NH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][C:9](=[O:10])[O:11][CH2:12][c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1.ClC(Cl)(Cl)O[C:2](OC(Cl)(Cl)Cl)=[O:1]>>[O:1]=[C:2]([NH:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][C:9](=[O:10])[O:11]...
CN(C)c1ccc(CN)cc1.Cc1ccc(S(=O)(=O)O)cc1.NCCCCCC(=O)OCc1ccccc1.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl
O=C(NCCCCCC(=O)OCc1ccccc1)NC12CC3CC(CC(C3)C1)C2
null
null
ClCCl
Acylation
OtherReaction
21ef8ba1fe1143ef552b8fde2d69ec6fde51120a86f799e368372b2b445551ea
b425761bd607612009c9c987139794a4be2c93d0d1248f685686bbb00d19b9c1
O=C(NCCCCCC(=O)OCc1ccccc1)NC12CC3CC(CC(C3)C1)C2
C-N(-C)-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[cH;D2;+0:3]:[c;H0;D3;+0:4](-[CH2;D2;+0:5]-[NH2;D1;+0:6]):[cH;D2;+0:7]:c:1.Cl-C(-Cl)(-Cl)-O-[C;H0;D3;+0:8](=[O;D1;H0:9])-O-C(-Cl)(-Cl)-Cl.O-S(=O)(=O)-c1:c:c:[c;H0;D3;+0:10](-[CH3;D1;+0:11]):c:c:1.[C:12]-[C:13]-[NH2;D1;+0:14]>>[C:12]-[C:13]-[NH;D2;+0:14]-[C;H0;D3;+0:8](=[O;D1;H0:9])-...
180.9
[{"value": 61.0, "product": "C(C1=CC=CC=C1)OC(CCCCCNC(=O)NC12CC3CC(CC(C1)C3)C2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 180.9, "product": "C(C1=CC=CC=C1)OC(CCCCCNC(=O)NC12CC3CC(CC(C1)C3)C2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a vigorously stirred suspension of 6-amino-hexanoic acid benzyl ester toluene-4-sulfonic acid (0.786 g, 2.00 mmol) and triphosgene (0.200 g, 0.667 mmol) in dichloromethane (30 mL) at −78° C. under inert atmosphere, was added triethylamine (1.0 mL, 7.188 mmol, in 10 mL dichloromethane) dropwise via additional funnel ...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Trichloro group.Trichloro group.Carbonic Ester.Primary amine.Primary amine.Tertiary amine
Urea
c1ccccc1.c1ccccc1
C1C2CC3CC1CC(C2)C3
c1ccccc1.C1C2CC3CC1CC(C2)C3
TsOH.HCl
ClCCl
null
1
CN(C)c1ccc(CN)cc1.Cc1ccc(S(=O)(=O)O)cc1.NCCCCCC(=O)OCc1ccccc1.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl>ClCCl>O=C(NCCCCCC(=O)OCc1ccccc1)NC12CC3CC(CC(C3)C1)C2
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e2450ec8f4ba404aa6c8454cf88d2725
COC(=O)CS.OC(c1ccccc1)(c1ccccc1)c1ccccc1>>COC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
SCC(=O)OC.C1(=CC=CC=C1)C(O)(C1=CC=CC=C1)C1=CC=CC=C1.FC(C(=O)O)(F)F>>COC(CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)=O
[CH3:1][O:2][C:3](=[O:4])[CH2:5][SH:6].O[C:7]([c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)([c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1)[c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][S:6][C:7]([c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)([c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1)[c:20]1[cH:2...
COC(=O)CS.OC(c1ccccc1)(c1ccccc1)c1ccccc1
COC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
null
null
C(Cl)(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
550a7964778c9f12760ef1f41256181c2082f29a84fb8f4bf2c9443b33dd6567
42963aad950e323e8799a3db4f42f888ff868551c22c911dbccb9f890bdeb2f6
c1ccc(C(c2ccccc2)c2ccccc2)cc1
O-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10].[C;D1;H3:11]-[#8:12]-[C:13](=[O;D1;H0:14])-[C:15]-[SH;D1;+0:16]>>[C;D1;H3:11]-[#8:12]-[C:13](=[O;D1;H0:14])-[C:15]-[S;H0;D2;+0:16]-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10]
91.3
[{"value": 91.0, "product": "COC(CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.3, "product": "COC(CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a mixture of methyl mercaptoacetate (5.30 g, 50 mmol) and triphenylmethanol (13.0 g, 50 mmol) in chloroform (20 mL) was added trifloroacetic acid (5 mL) in 5 min. After stirring at room temperature for 1 h, the volatiles were removed in vacuo. The crude product was purified by recrystallization (dichloromethane/Hexa...
10.6084/m9.figshare.5104873.v1
null
Tertiary alcohol.Aliphatic thiol
Monosulfide
null
null
c1ccccc1.c1ccccc1.c1ccccc1
HO-
C(Cl)(Cl)Cl
null
1
COC(=O)CS.OC(c1ccccc1)(c1ccccc1)c1ccccc1>C(Cl)(Cl)Cl>COC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-444cc2f5c962494f9efaf402bc1d7aa1
COC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1.NCCCCCN>>NCCCCCC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
NCCCCCN.COC(CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)=O.CO>>NCCCCCC(CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)=O
CO[C:7](=[O:8])[CH2:9][S:10][C:11]([c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)([c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1)[c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1.N[CH2:6][CH2:5][CH2:4][CH2:3][CH2:2][NH2:1]>>[NH2:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][C:7](=[O:8])[CH2:9][S:10][C:11]([c:12]1[cH:13][cH:14][cH:15][cH:...
COC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1.NCCCCCN
NCCCCCC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
null
null
ClCCl.CO.CCN(CC)CC
C-C Coupling
OtherReaction
1a69e220b52fe9824bfcad182fc3bd64f3f705c2ea3f3199bde2a17596886895
bed782162e5697dea9604bde8f3ba126d86aa25d57c682ebb8a09e1e7c81db45
c1ccc(C(c2ccccc2)c2ccccc2)cc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#16:4].N-[CH2;D2;+0:5]-[C:6]-[C:7]>>[#16:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH2;D2;+0:5]-[C:6]-[C:7]
56
[{"value": 54.0, "product": "NCCCCCC(CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 56.0, "product": "NCCCCCC(CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
1,5-Diaminopentane (0.75 g, 7.21 mmol) was stirred while tritylsulfanyl-acetic acid methyl ester (2.53 g, 7.27 mmol) was added slowly. The mixture was heated at 100° C. for 2 h while methyl alcohol escaped. The product was isolated by column chromatography (dichloromethane/MeOH/Et3N=10/1/0.1) to provide 7-Amino-1-trity...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Ketone
null
null
c1ccccc1.c1ccccc1.c1ccccc1
HO-
ClCCl.CO.CCN(CC)CC
null
null
COC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1.NCCCCCN>ClCCl.CO.CCN(CC)CC>NCCCCCC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3f7f3537cb99427f80f6b33da6f8e173
NCCCCCC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1.O=C=Nc1ccccc1>>O=C(CCCCCNC(=O)Nc1ccccc1)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
NCCCCCC(CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)=O.C1(=CC=CC=C1)N=C=O>>O=C(CCCCCNC(=O)NC1=CC=CC=C1)CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1
[O:1]=[C:2]([CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][NH2:8])[CH2:18][S:19][C:20]([c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1)([c:27]1[cH:28][cH:29][cH:30][cH:31][cH:32]1)[c:33]1[cH:34][cH:35][cH:36][cH:37][cH:38]1.[C:9](=[O:10])=[N:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[O:1]=[C:2]([CH2:3][CH2:4][CH2:5][CH2:6][CH2:...
NCCCCCC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1.O=C=Nc1ccccc1
O=C(CCCCCNC(=O)Nc1ccccc1)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
null
null
ClCCl
Acylation
Urea synthesis via isocyanate and primary amine
d39cd7dc52a79bb265ff8ef61ef7bf9dc7f7b5fb0150fcb4881bdfb18ab9c380
a5dc801930c765d2a435a0a2973e50163c305ba8e7641d6adbcc1550b7b96de7
O=C(CCCCCNC(=O)Nc1ccccc1)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D2;+0:5]=[N;H0;D2;+0:6]-[c:7](:[c:8]):[c:9]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:5](=[O;D1;H0:4])-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]
95.7
[{"value": 93.0, "product": "O=C(CCCCCNC(=O)NC1=CC=CC=C1)CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.7, "product": "O=C(CCCCCNC(=O)NC1=CC=CC=C1)CSC(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 7-amino-1-tritylsulfanyl-heptan-2-one (0.36 g, 0.86 mmol) in dichloromethane (10 mL) was added phenylisocyanate (0.10 mL, 0.92 mmol). The mixture was stirred at room temperature for 2 h. Solvent was then removed in vacuo and the crude product was purified by column chromatography (dichloromethane/MeOH=...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Primary amine
Urea
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1
null
ClCCl
null
2
NCCCCCC(=O)CSC(c1ccccc1)(c1ccccc1)c1ccccc1.O=C=Nc1ccccc1>ClCCl>O=C(CCCCCNC(=O)Nc1ccccc1)CSC(c1ccccc1)(c1ccccc1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a6670014d6824106b82c37823a9dd189
O=C(CS)NCCCCCNC(=O)Nc1ccccc1.O=C=NCc1ccccc1>>O=C(CS)NCCCCCNC(=O)NCc1ccccc1
SCC(=O)NCCCCCNC(=O)NC1=CC=CC=C1.C(C1=CC=CC=C1)N=C=O>>C(C1=CC=CC=C1)NC(NCCCCCNC(CS)=O)=O
c1ccc(N[C:12]([NH:11][CH2:10][CH2:9][CH2:8][CH2:7][CH2:6][NH:5][C:2](=[O:1])[CH2:3][SH:4])=[O:13])cc1.O=C=[N:14][CH2:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1>>[O:1]=[C:2]([CH2:3][SH:4])[NH:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][NH:11][C:12](=[O:13])[NH:14][CH2:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1
O=C(CS)NCCCCCNC(=O)Nc1ccccc1.O=C=NCc1ccccc1
O=C(CS)NCCCCCNC(=O)NCc1ccccc1
null
null
null
Acylation
OtherReaction
997a890dafa955c3130c49973d0afeebf85b599849c6eb3f0b38291cb66b3987
22ae2e47c0f9d9608f1cd96e274d7483289cea4f5380556a255e5dcab79311e7
c1ccccc1
O=C=[N;H0;D2;+0:1]-[C:2]-[c:3].[C:4]-[#7:5]-[C;H0;D3;+0:6](=[O;D1;H0:7])-N-c1:c:c:c:c:c:1>>[C:4]-[#7:5]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[NH;D2;+0:1]-[C:2]-[c:3]
null
[]
null
null
null
null
Compound 11 was prepared using the methodology described for the preparation of Compound 9, by substituting phenylisocyanate with benzylisocyanate. 1H NMR (300 MHz, DMSO-d6) δ (ppm) 7.98 (br s, 1H), 7.35-7.18 (m, 5H), 6.27 (br s, 1H), 5.91 (br s, 1H), 4.19 (s, 2H), 3.07 (d, J=8.1 Hz, 2H), 3.02 (m, 4H), 2.71 (t, J=8.1 H...
10.6084/m9.figshare.5104873.v1
null
Urea.Isocyanate
Urea
c1ccccc1
null
c1ccccc1
HO-
null
null
null
O=C(CS)NCCCCCNC(=O)Nc1ccccc1.O=C=NCc1ccccc1>>O=C(CS)NCCCCCNC(=O)NCc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-29509cc1ce7e4b3f968edc2171438e52
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCC(O)c1ccccc1>>O=C(CCCNC(=O)NCC(O)c1ccccc1)NO
CN(C1=CC=C(CNC(NCCCC(=O)NO)=O)C=C1)C.NCC(O)C1=CC=CC=C1>>ONC(CCCNC(=O)NCC(C1=CC=CC=C1)O)=O
CN(C)c1ccc(CN[C:7]([NH:6][CH2:5][CH2:4][CH2:3][C:2](=[O:1])[NH:19][OH:20])=[O:8])cc1.[NH2:9][CH2:10][CH:11]([OH:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[O:1]=[C:2]([CH2:3][CH2:4][CH2:5][NH:6][C:7](=[O:8])[NH:9][CH2:10][CH:11]([OH:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[NH:19][OH:20]
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCC(O)c1ccccc1
O=C(CCCNC(=O)NCC(O)c1ccccc1)NO
null
null
null
Acylation
OtherReaction
582f6ef5382ebd5e48252e738466d893c5ee2b077cb67f852c2b3d7225820053
0d4269d1abb31eda25c7cd91c24eadac3777eb70ce7cce8a6d7982c94492f078
c1ccccc1
C-N(-C)-c1:c:c:c(-C-N-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3]-[C:4]):c:c:1.[C:5]-[C:6]-[NH2;D1;+0:7]>>[C:5]-[C:6]-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3]-[C:4]
null
[]
null
null
null
null
Compound 15 was prepared using the methodology described for the preparation of compound 2, by substituting 4-dimethylaminobenzylamine dihydrochloride with 2-amino-1-phenyl-ethanol. 1H NMR (CD3OD) δ 7.42-7.24 (m, 5H), 4.73 (dd, J=7.8, 4.2 Hz, 1H), 3.43 (dd, J=13.8, 4.2 Hz, 1H), 3.26 (dd, J=13.8, 7.8 Hz, 1H), 3.14 (t, J...
10.6084/m9.figshare.5104873.v1
null
Urea.Primary amine.Tertiary amine
Urea
c1ccccc1
null
c1ccccc1
Other
null
null
null
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCC(O)c1ccccc1>>O=C(CCCNC(=O)NCC(O)c1ccccc1)NO
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b9591aaa88b34c50ad6e35f510dc7980
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCCc1ccccc1>>O=C(CCCNC(=O)NCCc1ccccc1)NO
CN(C1=CC=C(CNC(NCCCC(=O)NO)=O)C=C1)C.C(CC1=CC=CC=C1)N>>ONC(CCCNC(=O)NCCC1=CC=CC=C1)=O
CN(C)c1ccc(CN[C:7]([NH:6][CH2:5][CH2:4][CH2:3][C:2](=[O:1])[NH:18][OH:19])=[O:8])cc1.[NH2:9][CH2:10][CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[O:1]=[C:2]([CH2:3][CH2:4][CH2:5][NH:6][C:7](=[O:8])[NH:9][CH2:10][CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)[NH:18][OH:19]
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCCc1ccccc1
O=C(CCCNC(=O)NCCc1ccccc1)NO
null
null
null
Acylation
OtherReaction
582f6ef5382ebd5e48252e738466d893c5ee2b077cb67f852c2b3d7225820053
0d4269d1abb31eda25c7cd91c24eadac3777eb70ce7cce8a6d7982c94492f078
c1ccccc1
C-N(-C)-c1:c:c:c(-C-N-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3]-[C:4]):c:c:1.[C:5]-[C:6]-[NH2;D1;+0:7]>>[C:5]-[C:6]-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3]-[C:4]
null
[]
null
null
null
null
Compound 1 was prepared using the methodology described for the preparation of compound 2, by substituting 4-dimethylaminobenzylamine dihydrochloride with phenethylamine. 1H NMR (CD3OD) δ 7.30-7.15 (m, 5H), 3.34 (t, J=6.9 Hz, 2H), 3.11 (t, J=7.2 Hz, 2H), 2.76 (t, J=7.2 Hz, 2H), 2.09 (t, J=7.5Hz, 2H), 1.73 (m, 2H). 13C ...
10.6084/m9.figshare.5104873.v1
null
Urea.Primary amine.Tertiary amine
Urea
c1ccccc1
null
c1ccccc1
Other
null
null
null
CN(C)c1ccc(CNC(=O)NCCCC(=O)NO)cc1.NCCc1ccccc1>>O=C(CCCNC(=O)NCCc1ccccc1)NO
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-410a56935e554501b6be0dc88cc96e44
COC(=O)CCCCCCC(=O)NC12CC3CC(CC(C3)C1)C2.NO>>O=C(CCCCCCC(=O)NC12CC3CC(CC(C3)C1)C2)NO
[Na].Cl.NO.[Na].COC(CCCCCCC(NC12CC3CC(CC(C1)C3)C2)=O)=O.C(C)(=O)O>>ONC(CCCCCCC(=O)NC12CC3CC(CC(C1)C3)C2)=O
CO[C:2](=[O:1])[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][C:9](=[O:10])[NH:11][C:12]12[CH2:13][CH:14]3[CH2:15][CH:16]([CH2:17][CH:18]([CH2:19]3)[CH2:20]1)[CH2:21]2.[NH2:22][OH:23]>>[O:1]=[C:2]([CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][C:9](=[O:10])[NH:11][C:12]12[CH2:13][CH:14]3[CH2:15][CH:16]([CH2:17][CH:18]([CH2:19]...
COC(=O)CCCCCCC(=O)NC12CC3CC(CC(C3)C1)C2.NO
O=C(CCCCCCC(=O)NC12CC3CC(CC(C3)C1)C2)NO
null
C=1C=CC2=C(C1)C(=O)OC2(C=3C=CC(=CC3)O)C=4C=CC(=CC4)O
O.CO
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
C1C2CC3CC1CC(C2)C3
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[NH2;D1;+0:5]-[O;D1;H1:6]>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:5]-[O;D1;H1:6]
68
[{"value": 68.0, "product": "ONC(CCCCCCC(=O)NC12CC3CC(CC(C1)C3)C2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.0, "product": "ONC(CCCCCCC(=O)NC12CC3CC(CC(C1)C3)C2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
To a first solution of hydroxylamine hydrochloride (66 mg, 0.950 mmol) and phenolphthalein (0.5 mg) in methanol (3 mL), was added dropwise a second solution of sodium metal (33 mg, 1.435 mmol) in methanol (3 mL) via additional funnel until a pink endpoint was reached and precipitate appeared. To the reaction mixture wa...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
C1C2CC3CC1CC(C2)C3
HO-
C=1C=CC2=C(C1)C(=O)OC2(C=3C=CC(=CC3)O)C=4C=CC(=CC4)O.O.CO
null
24
COC(=O)CCCCCCC(=O)NC12CC3CC(CC(C3)C1)C2.NO>C=1C=CC2=C(C1)C(=O)OC2(C=3C=CC(=CC3)O)C=4C=CC(=CC4)O.O.CO>O=C(CCCCCCC(=O)NC12CC3CC(CC(C3)C1)C2)NO