dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cb5340bf9e12420f961f85565674a2d1
N#Cc1cccc(O)c1.O=[N+]([O-])c1ccc(F)c(Cl)c1>>N#Cc1cccc(Oc2ccc([N+](=O)[O-])cc2Cl)c1
O.ClC1=C(C=CC(=C1)[N+](=O)[O-])F.OC=1C=C(C#N)C=CC1.C([O-])([O-])=O.[K+].[K+]>>ClC1=C(OC=2C=C(C#N)C=CC2)C=CC(=C1)[N+](=O)[O-]
[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([OH:8])[cH:19]1.F[c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[cH:16][c:17]1[Cl:18]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[cH:16][c:17]2[Cl:18])[cH:19]1
N#Cc1cccc(O)c1.O=[N+]([O-])c1ccc(F)c(Cl)c1
N#Cc1cccc(Oc2ccc([N+](=O)[O-])cc2Cl)c1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
e4ea1e38252bc3b9c5ec04486386725e6570ab3860d45e337a1d131319bbf0fc
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccccc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Cl;D1;H0:5]):[c:6].[OH;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[Cl;D1;H0:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[O;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]):[c:2]:[c:3]
91.9
[{"value": 91.9, "product": "ClC1=C(OC=2C=C(C#N)C=CC2)C=CC(=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
4
HOUR
To a solution of 2-chloro-1-fluoro-4-nitrobenzene (3.7 g) and 3-hydroxybenzonitrile (2.5 g) in N,N-dimethylformamide (50 mL) was added potassium carbonate (4.4 g), and the mixture was stirred at 60° C. for 4 hrs. After the completion of the reaction, water (50 mL) was added, and the mixture was stirred for 10 min. The ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HF
CN(C=O)C
60
4
N#Cc1cccc(O)c1.O=[N+]([O-])c1ccc(F)c(Cl)c1>CN(C=O)C>N#Cc1cccc(Oc2ccc([N+](=O)[O-])cc2Cl)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0a1d4a4e58c14dbb8c71ddea5d96011e
N#Cc1cccc(Oc2ccc([N+](=O)[O-])cc2Cl)c1>>N#Cc1cccc(Oc2ccc(N)cc2Cl)c1
ClC1=C(OC=2C=C(C#N)C=CC2)C=CC(=C1)[N+](=O)[O-].[Cl-].[Ca+2].[Cl-]>>NC1=CC(=C(OC=2C=C(C#N)C=CC2)C=C1)Cl
O=[N+:13]([O-])[c:12]1[cH:11][cH:10][c:9]([O:8][c:7]2[cH:6][cH:5][cH:4][c:3]([C:2]#[N:1])[cH:17]2)[c:15]([Cl:16])[cH:14]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([NH2:13])[cH:14][c:15]2[Cl:16])[cH:17]1
N#Cc1cccc(Oc2ccc([N+](=O)[O-])cc2Cl)c1
N#Cc1cccc(Oc2ccc(N)cc2Cl)c1
null
null
C(C)O.O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Oc2ccccc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
70.2
[{"value": 70.2, "product": "NC1=CC(=C(OC=2C=C(C#N)C=CC2)C=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
10
MINUTE
To a solution of 3-(2-chloro-4-nitrophenoxy)benzonitrile (2.0 g) in ethanol/water (9:1, 40 mL) was added calcium chloride (90%, 449 mg), and the mixture was stirred at 100° C. for 10 min. Reduced iron (90%, 2.7 g) was added at room temperature, and the mixture was stirred at 100° C. for 5 hrs. After the completion of t...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccccc1
Other
C(C)O.O
100
0.166667
N#Cc1cccc(Oc2ccc([N+](=O)[O-])cc2Cl)c1>C(C)O.O>N#Cc1cccc(Oc2ccc(N)cc2Cl)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0af3ceb8b6bd4b00a89823f37bb0fddb
CCO.O=C(O)c1cc([N+](=O)[O-])ccc1F>>CCOC(=O)c1cc([N+](=O)[O-])ccc1F
S(=O)(Cl)Cl.FC1=C(C(=O)O)C=C(C=C1)[N+](=O)[O-].C(C)O>>FC1=C(C(=O)OCC)C=C(C=C1)[N+](=O)[O-]
[CH3:1][CH2:2][OH:3].O[C:4](=[O:5])[c:6]1[cH:7][c:8]([N+:9](=[O:10])[O-:11])[cH:12][cH:13][c:14]1[F:15]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([N+:9](=[O:10])[O-:11])[cH:12][cH:13][c:14]1[F:15]
CCO.O=C(O)c1cc([N+](=O)[O-])ccc1F
CCOC(=O)c1cc([N+](=O)[O-])ccc1F
null
null
null
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C;D1;H3:6]-[C:7]-[OH;D1;+0:8]>>[C;D1;H3:6]-[C:7]-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
80
CELSIUS
4
HOUR
Under ice-cooling, thionyl chloride (8.02 mL) was added dropwise to ethanol (200 mL), and 2-fluoro-5-nitrobenzoic acid (13.81 g) was added. This mixture was stirred at 80° C. for 4 hrs. and concentrated under reduced pressure. A saturated aqueous sodium hydrogen carbonate solution was added to the reaction mixture and ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
c1ccccc1
HO-
null
80
4
CCO.O=C(O)c1cc([N+](=O)[O-])ccc1F>>CCOC(=O)c1cc([N+](=O)[O-])ccc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e1755d888fa243c2bda0a67feb7d57c2
CCOC(=O)c1cc([N+](=O)[O-])ccc1F.Oc1ccccc1>>CCOC(=O)c1cc(N)ccc1Oc1ccccc1
FC1=C(C(=O)OCC)C=C(C=C1)[N+](=O)[O-].C1(=CC=CC=C1)O.C([O-])([O-])=O.[K+].[K+]>>NC=1C=CC(=C(C(=O)OCC)C1)OC1=CC=CC=C1
O=[N+:9]([O-])[c:8]1[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:12](F)[cH:11][cH:10]1.[OH:13][c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([NH2:9])[cH:10][cH:11][c:12]1[O:13][c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1
CCOC(=O)c1cc([N+](=O)[O-])ccc1F.Oc1ccccc1
CCOC(=O)c1cc(N)ccc1Oc1ccccc1
null
null
CN(C=O)C
Functional Group Interconversion
OtherReaction
fcde22d25a281822013269b17d8b3414bea830a4bf58d8806a9dfee8028580dd
62abf9f7921a98ccae96c82f80f078cf7b92f589fff664adf63edbf966dddb72
c1ccc(Oc2ccccc2)cc1
F-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[N+;H0;D3:5](=O)-[O-]):[c:6]:[c:7]:1-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11].[OH;D1;+0:12]-[c:13](:[c:14]):[c:15]>>[C:11]-[#8:10]-[C:8](=[O;D1;H0:9])-[c:7]1:[c:6]:[c:4](-[NH2;D1;+0:5]):[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[O;H0;D2;+0:12]-[c:13](:[c:14]):[c:15]
82.9
[{"value": 82.9, "product": "NC=1C=CC(=C(C(=O)OCC)C1)OC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
4
HOUR
A mixture of ethyl 2-fluoro-5-nitrobenzoate (1.07 g), phenol (565 mg), potassium carbonate (1.38 g) and N,N-dimethylformamide (20 mL) was stirred at 80° C. for 4 hrs. The reaction mixture was concentrated under reduced pressure. Water was added to the residue and the mixture was extracted with ethyl acetate. The extrac...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Nitro group.Aromatic alcohol
Ether.Primary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
Other
CN(C=O)C
80
4
CCOC(=O)c1cc([N+](=O)[O-])ccc1F.Oc1ccccc1>CN(C=O)C>CCOC(=O)c1cc(N)ccc1Oc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ef295f3049624ba9a6f932b5d9010853
CCOC(=O)c1ccc(CBr)cc1.CSc1ncnc2cn[nH]c12>>COC(=O)c1ccc(Cn2cc3ncnc(SC)c3n2)cc1.COC(=O)c1ccc(Cn2ncc3ncnc(SC)c32)cc1
BrCC1=CC=C(C(=O)OCC)C=C1.CSC=1C2=C(N=CN1)C=NN2.[H-].[Na+]>>CSC=1C2=C(N=CN1)C=NN2CC2=CC=C(C(=O)OC)C=C2.CSC=1C=2C(N=CN1)=CN(N2)CC2=CC=C(C(=O)OC)C=C2
Br[CH2:31][c:30]1[cH:29][cH:28][c:5]([C:3]([O:2][CH2:1][CH3:35])=[O:4])[cH:44][cH:43]1.[n:10]1[cH:11][c:12]2[n:13][cH:14][n:15][c:16]([S:17][CH3:18])[c:19]2[nH:32]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][n:10]2[cH:11][c:12]3[n:13][cH:14][n:15][c:16]([S:17][CH3:18])[c:19]3[n:20]2)[cH:21][cH:22]1.[CH3:...
CCOC(=O)c1ccc(CBr)cc1.CSc1ncnc2cn[nH]c12
COC(=O)c1ccc(Cn2cc3ncnc(SC)c3n2)cc1.COC(=O)c1ccc(Cn2ncc3ncnc(SC)c32)cc1
null
null
CN(C=O)C.C(C)(=O)OCC
Aromatic Heterocycle Formation
OtherReaction
69f8b9b6349b792a0dee6d904c29ee7cfdff387e4eb2eb980499c901083fef5f
08b2a64655eebd58f53d97b92771b7d831c3b6cc8b1b6b6d538729fc2ee365d7
c1ccc(Cn2cc3ncncc3n2)cc1.c1ccc(Cn2ncc3ncncc32)cc1
Br-[CH2;D2;+0:1]-[c:2]1:[c:3]:[cH;D2;+0:4]:[c;H0;D3;+0:5](-[C:6](=[O;D1;H0:7])-[#8:8]-[CH2;D2;+0:9]-[CH3;D1;+0:10]):[cH;D2;+0:11]:[c:12]:1.[#16:13]-[c:14]1:[#7;a:15]:[c:16]:[#7;a:17]:[c:18]2:[c:19]:[n;H0;D2;+0:20]:[nH;D2;+0:21]:[c;H0;D3;+0:22]:2:1>>[#16:13]-[c:14]1:[#7;a:15]:[c:16]:[#7;a:17]:[c:18]2:[c:19]:[n;H0;D3;+0:...
null
[]
null
null
10
MINUTE
To a solution of 7-(methylthio)-1H-pyrazolo[4,3-d]pyrimidine (400 mg) in N,N-dimethylformamide (8 mL) was added 60% sodium hydride (98 mg) under ice-cooling, and the mixture was stirred at room temperature for 10 min. Then, ethyl 4-(bromomethyl)benzoate (606 mg) was added under ice-cooling, and the mixture was stirred ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Ester.Ester.Monosulfide
c1ccccc1.c1ncc2n[nH]cc2n1
c1ccccc1.c1ncnc2c[nH]nc12.c1ccccc1.c1ncnc2cn[nH]c12
c1ccccc1.c1ncnc2c[nH]nc12.c1ccccc1.c1ncnc2cn[nH]c12
Br-
CN(C=O)C.C(C)(=O)OCC
null
0.166667
CCOC(=O)c1ccc(CBr)cc1.CSc1ncnc2cn[nH]c12>CN(C=O)C.C(C)(=O)OCC>COC(=O)c1ccc(Cn2cc3ncnc(SC)c3n2)cc1.COC(=O)c1ccc(Cn2ncc3ncnc(SC)c32)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-86ec5f319157400a82c7853df2ab732b
CSc1ncnc2cn[nH]c12.O=C(OCCI)c1ccccc1.O=C([O-])[O-]>>CSc1ncnc2cn(CCOC(=O)c3ccccc3)nc12.CSc1ncnc2cnn(CCOC(=O)c3ccccc3)c12
O.CSC=1C2=C(N=CN1)C=NN2.C(C1=CC=CC=C1)(=O)OCCI.C([O-])([O-])=O.[K+].[K+]>>C(C1=CC=CC=C1)(=O)OCCN1N=CC=2N=CN=C(C21)SC.C(C1=CC=CC=C1)(=O)OCCN1N=C2C(N=CN=C2SC)=C1
[CH3:1][S:2][c:3]1[n:4][cH:5][n:6][c:7]2[c:22]1[nH:9][n:31][cH:30]2.I[CH2:33][CH2:34][O:35][C:36](=[O:37])[c:38]1[cH:39][cH:8][cH:41][cH:42][cH:43]1.[O-][C:13]([O-:12])=[O:14]>>[CH3:1][S:2][c:3]1[n:4][cH:5][n:6][c:7]2[cH:8][n:9]([CH2:10][CH2:11][O:12][C:13](=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19][cH:20]3)[n:21][c:2...
CSc1ncnc2cn[nH]c12.O=C(OCCI)c1ccccc1.O=C([O-])[O-]
CSc1ncnc2cn(CCOC(=O)c3ccccc3)nc12.CSc1ncnc2cnn(CCOC(=O)c3ccccc3)c12
null
null
CN(C=O)C.C(C)(=O)OCC
Aromatic Heterocycle Formation
OtherReaction
2bb4372b727939bd66414920f948f4a18409fc06951c5403c00c20d9203b9606
9259a53dabfdb3b1d2386fadb2d5599dab233d24a6464e15b3982bff7ce113b5
O=C(OCCn1cc2ncncc2n1)c1ccccc1.O=C(OCCn1ncc2ncncc21)c1ccccc1
I-[CH2;D2;+0:1]-[C:2]-[#8:3]-[C:4](=[O;D1;H0:5])-[c:6]1:[c:7]:[c:8]:[cH;D2;+0:9]:[cH;D2;+0:10]:[cH;D2;+0:11]:1.[#16:12]-[c:13]1:[#7;a:14]:[c:15]:[#7;a:16]:[c;H0;D3;+0:17]2:[cH;D2;+0:18]:[n;H0;D2;+0:19]:[nH;D2;+0:20]:[c;H0;D3;+0:21]:1:2.[O-;H0;D1:22]-[C;H0;D3;+0:23](-[O-])=[O;D1;H0:24]>>[#16:12]-[c:13]1:[#7;a:14]:[c:15]...
null
[]
60
CELSIUS
1
HOUR
To a solution of 7-(methylthio)-1H-pyrazolo[4,3-d]pyrimidine (300 mg) and 2-iodoethyl benzoate (548 mg) in N,N-dimethylformamide (10 mL) was added potassium carbonate (374 mg), and the mixture was stirred at 60° C. for 1 hr. After the completion of the reaction, water was added to the reaction mixture. The mixture was ...
10.6084/m9.figshare.5104873.v1
null
Primary halide
Ester.Monosulfide
c1ncc2[nH]ncc2n1.c1ccccc1
c1ncnc2c[nH]nc12.c1ccccc1.c1ncnc2c[nH]nc12.c1ccccc1
c1ncnc2c[nH]nc12.c1ccccc1.c1ncnc2c[nH]nc12.c1ccccc1
I-
CN(C=O)C.C(C)(=O)OCC
60
1
CSc1ncnc2cn[nH]c12.O=C(OCCI)c1ccccc1.O=C([O-])[O-]>CN(C=O)C.C(C)(=O)OCC>CSc1ncnc2cn(CCOC(=O)c3ccccc3)nc12.CSc1ncnc2cnn(CCOC(=O)c3ccccc3)c12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-05c9281cf7174921872b575bc7b9f531
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>Cl.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1
ClC=1C2=C(N=CN1)C=CN2.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>Cl.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2
[Cl:1][c:15]1[n:16][cH:17][n:18][c:19]2[cH:20][cH:21][nH:22][c:23]12.[F:2][c:3]1[cH:4][cH:5][cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13]([NH2:14])[cH:24][c:25]2[Cl:26])[cH:27]1>>[ClH:1].[F:2][c:3]1[cH:4][cH:5][cH:6][c:7]([CH2:8][O:9][c:10]2[cH:11][cH:12][c:13]([NH:14][c:15]3[n:16][cH:17][n:18][c:19]4[cH:20][cH:2...
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
Cl.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1
null
null
CN1C(CCC1)=O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]2:[c:7]:[c:8]:[#7;a:9]:[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[ClH;D0;+0:1].[c:13]:[c:12](-[NH;D2;+0:11]-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]2:[c:7]:[c:8]:[#7;a:9]:[c:10]:2:1):[c:14]
79.7
[{"value": 79.7, "product": "Cl.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
null
null
4-Chloro-5H-pyrrolo[3,2-d]pyrimidine (770 mg) and 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (2.52 g) were dissolved in 1-methyl-2-pyrrolidone (10 mL), and the mixture was stirred with heating at 140° C. for 2.5 hrs. After cooling to room temperature, the mixture was diluted with ethyl acetate (300 mL), and stirred at roo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ccccc1.c1ncc2[nH]ccc2n1
null
CN1C(CCC1)=O.C(C)(=O)OCC
140
null
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>CN1C(CCC1)=O.C(C)(=O)OCC>Cl.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-db16c6dc72874539acf910e6e61b0c11
Clc1ncnc2cc[nH]c12.OCc1ccc(CCl)cc1>>OCc1ccc(Cn2ccc3ncnc(Cl)c32)cc1
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[K+].[K+].OCC1=CC=C(CCl)C=C1>>ClC=1C2=C(N=CN1)C=CN2CC2=CC=C(C=C2)CO
[nH:8]1[cH:9][cH:10][c:11]2[n:12][cH:13][n:14][c:15]([Cl:16])[c:17]12.Cl[CH2:7][c:6]1[cH:5][cH:4][c:3]([CH2:2][OH:1])[cH:19][cH:18]1>>[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][n:8]2[cH:9][cH:10][c:11]3[n:12][cH:13][n:14][c:15]([Cl:16])[c:17]23)[cH:18][cH:19]1
Clc1ncnc2cc[nH]c12.OCc1ccc(CCl)cc1
OCc1ccc(Cn2ccc3ncnc(Cl)c32)cc1
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Cn2ccc3ncncc32)cc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[Cl;D1;H0:5]-[c:6]1:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]2:[c:11]:[c:12]:[nH;D2;+0:13]:[c:14]:2:1>>[Cl;D1;H0:5]-[c:6]1:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]2:[c:11]:[c:12]:[n;H0;D3;+0:13](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]):[c:14]:2:1
70
[{"value": 70.0, "product": "ClC=1C2=C(N=CN1)C=CN2CC2=CC=C(C=C2)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
4-Chloro-5H-pyrrolo[3,2-d]pyrimidine (307 mg) was dissolved in N,N-dimethylformamide (2 mL), potassium carbonate (304 mg) was added, and the mixture was stirred at room temperature for 30 min. 4-Hydroxymethylbenzyl chloride (377 mg) was added, and the mixture was stirred at room temperature for 16 hrs. After diluting w...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ccccc1.c1ncnc2cc[nH]c12
HCl
O.CN(C=O)C
null
0.5
Clc1ncnc2cc[nH]c12.OCc1ccc(CCl)cc1>O.CN(C=O)C>OCc1ccc(Cn2ccc3ncnc(Cl)c32)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4f9d637c337140aeb493704722b3ec7d
Nc1ccc(OCc2cccc(F)c2)c(Cl)c1.OCc1ccc(Cn2ccc3ncnc(Cl)c32)cc1>>OCc1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
ClC=1C2=C(N=CN1)C=CN2CC2=CC=C(C=C2)CO.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C=C2)CO
[NH2:16][c:17]1[cH:18][cH:19][c:20]([O:21][CH2:22][c:23]2[cH:24][cH:25][cH:26][c:27]([F:28])[cH:29]2)[c:30]([Cl:31])[cH:32]1.Cl[c:15]1[n:14][cH:13][n:12][c:11]2[cH:10][cH:9][n:8]([CH2:7][c:6]3[cH:5][cH:4][c:3]([CH2:2][OH:1])[cH:35][cH:34]3)[c:33]21>>[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][n:8]2[cH:9][cH:10][c:11]3...
Nc1ccc(OCc2cccc(F)c2)c(Cl)c1.OCc1ccc(Cn2ccc3ncnc(Cl)c32)cc1
OCc1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
null
null
CN1C(CCC1)=O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccccc5)c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
93
[{"value": 93.0, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C=C2)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
null
null
{4-[(4-Chloro-5H-pyrrolo[3,2-d]pyrimidin-5-yl)methyl]phenyl}methanol (354 mg) and 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (488 mg) were dissolved in 1-methyl-2-pyrrolidone (2.58 mL), and the mixture was stirred with heating at 140° C. for 2 hrs. After cooling to room temperature, the reaction mixture was diluted with e...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
CN1C(CCC1)=O.C(C)(=O)OCC
140
null
Nc1ccc(OCc2cccc(F)c2)c(Cl)c1.OCc1ccc(Cn2ccc3ncnc(Cl)c32)cc1>CN1C(CCC1)=O.C(C)(=O)OCC>OCc1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f5c0dd2c63a3498bb2f7c23fcfcac790
COc1ccc(C(=O)Cl)cc1OC.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1>>COc1ccc(C(=O)n2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1OC
Cl.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[K+].[K+].COC=1C=C(C(=O)Cl)C=CC1OC>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2C(C2=CC(=C(C=C2)OC)OC)=O
Cl[C:7]([c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[c:36]([O:37][CH3:38])[cH:35]1)=[O:8].[nH:9]1[cH:10][cH:11][c:12]2[n:13][cH:14][n:15][c:16]([NH:17][c:18]3[cH:19][cH:20][c:21]([O:22][CH2:23][c:24]4[cH:25][cH:26][cH:27][c:28]([F:29])[cH:30]4)[c:31]([Cl:32])[cH:33]3)[c:34]12>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])...
COc1ccc(C(=O)Cl)cc1OC.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1
COc1ccc(C(=O)n2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1OC
null
null
CN(C=O)C
Acylation
N-alkylation of secondary amines with alkyl halides
9634436895a68d22c17052eb8c6668ee472dd157e0a2b08481637c8cdacda3d9
edbcca52d877d662e04f0d6de1a7107a8eca1d366ee6da0d92e37eb02a291876
O=C(c1ccccc1)n1ccc2ncnc(Nc3ccc(OCc4ccccc4)cc3)c21
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#7:6]-[c:7]1:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]2:[c:12]:[c:13]:[nH;D2;+0:14]:[c:15]:2:1>>[#7:6]-[c:7]1:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]2:[c:12]:[c:13]:[n;H0;D3;+0:14](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]):[c:15]:2:1
52.7
[{"value": 52.7, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2C(C2=CC(=C(C=C2)OC)OC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Under ice-cooling, to a suspension of N-{3-chloro-4-[(3-fluorobenzyl)oxy]phenyl}-5H-pyrrolo[3,2-d]pyrimidin-4-amine hydrochloride (150 mg) and potassium carbonate (102 mg) in N,N-dimethylformamide (1.5 mL) was added 3,4-dimethoxybenzoyl chloride (82 mg), and the mixture was stirred under ice-cooling, for 1 hr. The mixt...
10.6084/m9.figshare.5104873.v1
null
Acyl halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
CN(C=O)C
null
null
COc1ccc(C(=O)Cl)cc1OC.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1>CN(C=O)C>COc1ccc(C(=O)n2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2a0c8916f36844eab3c72dcde4c1fc95
COC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1>>O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)OC)C=C2.Cl>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)O)C=C2
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][c:7]([CH2:8][n:9]2[cH:10][cH:11][c:12]3[n:13][cH:14][n:15][c:16]([NH:17][c:18]4[cH:19][cH:20][c:21]([O:22][CH2:23][c:24]5[cH:25][cH:26][cH:27][c:28]([F:29])[cH:30]5)[c:31]([Cl:32])[cH:33]4)[c:34]23)[cH:35][cH:36]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][n:9]2[cH:10][cH:...
COC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
null
null
O1CCCC1.O.[OH-].[Na+].C(C)O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccccc5)c34)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
89.2
[{"value": 89.2, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)O)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
HOUR
Methyl 4-{[4-({3-chloro-4-[(3-fluorobenzyl)oxy]phenyl}amino)-5H-pyrrolo[3,2-d]pyrimidin-5-yl]methyl}benzoate (850 mg) was dissolved in a mixed solvent of ethanol (3.29 mL)/tetrahydrofuran (3.29 mL), 1N aqueous sodium hydroxide solution (3.29 mL) was added, and the mixture was stirred at room temperature for 20 hrs. 1N ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
Other
O1CCCC1.O.[OH-].[Na+].C(C)O
null
20
COC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1>O1CCCC1.O.[OH-].[Na+].C(C)O>O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cfe79ba3cb824953b3c05068c2172966
O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1.OC1CCNCC1>>O=C(c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1)N1CCC(O)CC1
ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)O)C=C2.OC1CCNCC1.O.ON1N=NC2=C1C=CC=C2.Cl.C(C)N=C=NCCCN(C)C>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)N1CCC(CC1)O)C=C2
O[C:2](=[O:1])[c:3]1[cH:4][cH:5][c:6]([CH2:7][n:8]2[cH:9][cH:10][c:11]3[n:12][cH:13][n:14][c:15]([NH:16][c:17]4[cH:18][cH:19][c:20]([O:21][CH2:22][c:23]5[cH:24][cH:25][cH:26][c:27]([F:28])[cH:29]5)[c:30]([Cl:31])[cH:32]4)[c:33]23)[cH:34][cH:35]1.[NH:36]1[CH2:37][CH2:38][CH:39]([OH:40])[CH2:41][CH2:42]1>>[O:1]=[C:2]([c:...
O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1.OC1CCNCC1
O=C(c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1)N1CCC(O)CC1
null
null
C(C)N(CC)CC.CN(C=O)C
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccc5)cc4)c32)cc1)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]>>[C:6]-[C:7]-[N;H0;D3;+0:8](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:9]-[C:10]
96.1
[{"value": 96.1, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)N1CCC(CC1)O)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a mixture of 4-{[4-({3-chloro-4-[(3-fluorobenzyl)oxy]phenyl}amino)-5H-pyrrolo[3,2-d]pyrimidin-5-yl]methyl}benzoic acid (150 mg), 4-hydroxypiperidine (33.2 mg) and 1-hydroxybenzotriazole monohydrate (60 mg) in N,N-dimethylformamide (3 mL) were added 1-ethyl-3-(3-dimethylaminopropyl)carbodiimide hydrochloride (86 mg) ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1.C1CC[NH]CC1
HO-
C(C)N(CC)CC.CN(C=O)C
null
8
O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1.OC1CCNCC1>C(C)N(CC)CC.CN(C=O)C>O=C(c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1)N1CCC(O)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d85f0c7f3e0e46c785ab92c76a8cebc7
Cc1ccc(Oc2ccc(N)cc2C)cn1.O=[N+]([O-])c1c(Cl)ncnc1Cl>>Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3[N+](=O)[O-])cc2C)cn1.Cl
ClC1=NC=NC(=C1[N+](=O)[O-])Cl.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C>>Cl.ClC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)[N+](=O)[O-]
[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH2:11])[cH:22][c:23]2[CH3:24])[cH:25][n:26]1.[c:12]1([Cl:27])[n:13][cH:14][n:15][c:16]([Cl:17])[c:18]1[N+:19](=[O:20])[O-:21]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n:13][cH:14][n:15][c:16]([Cl:17])[c:18]3[N+:19](=[O:20...
Cc1ccc(Oc2ccc(N)cc2C)cn1.O=[N+]([O-])c1c(Cl)ncnc1Cl
Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3[N+](=O)[O-])cc2C)cn1.Cl
null
null
CN1C(CCC1)=O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
c38b7155556ff28144ae37859ff6668b20d59da60c705d26b158542b6d8385da
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cncc(Oc2ccc(Nc3ccncn3)cc2)c1
[#7;+:1]-[c:2]1:[c:3](-[Cl;D1;H0:4]):[#7;a:5]:[c:6]:[#7;a:7]:[c;H0;D3;+0:8]:1-[Cl;H0;D1;+0:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[#7;+:1]-[c:2]1:[c:3](-[Cl;D1;H0:4]):[#7;a:5]:[c:6]:[#7;a:7]:[c;H0;D3;+0:8]:1-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13].[ClH;D0;+0:9]
72
[{"value": 72.0, "product": "Cl.ClC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-15
CELSIUS
1
HOUR
4,6-Dichloro-5-nitropyrimidine (9.7 g) was dissolved in 1-methyl-2-pyrrolidone (25.7 mL), a solution of 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (5.35 g) in 1-methyl-2-pyrrolidone (10 mL) was added dropwise under cooling at −15° C., and the mixture was stirred at −10° C. to 0° C. for 1 hr. The mixture was diluted ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cncnc1
c1cncnc1
c1ccncc1.c1ccccc1.c1cncnc1
null
CN1C(CCC1)=O.C(C)(=O)OCC
-15
1
Cc1ccc(Oc2ccc(N)cc2C)cn1.O=[N+]([O-])c1c(Cl)ncnc1Cl>CN1C(CCC1)=O.C(C)(=O)OCC>Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3[N+](=O)[O-])cc2C)cn1.Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8e7acefcc0d942839d9faaf8e8293dc5
Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3[N+](=O)[O-])cc2C)cn1>>Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3N)cc2C)cn1
[OH-].[Na+].O.O.[Sn](Cl)(Cl)(Cl)Cl.Cl.ClC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)[N+](=O)[O-].C(C)(=O)OCC>>ClC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N
O=[N+:19]([O-])[c:18]1[c:12]([NH:11][c:10]2[cH:9][cH:8][c:7]([O:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[n:24][cH:23]3)[c:21]([CH3:22])[cH:20]2)[n:13][cH:14][n:15][c:16]1[Cl:17]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n:13][cH:14][n:15][c:16]([Cl:17])[c:18]3[NH2:19])[cH:20][c:21]2[CH3:22]...
Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3[N+](=O)[O-])cc2C)cn1
Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3N)cc2C)cn1
null
null
Cl.C(C)OCC
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1cncc(Oc2ccc(Nc3ccncn3)cc2)c1
O=[N+;H0;D3:1](-[O-])-[c:2]1:[c:3](-[#7:4]):[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:1-[Cl;D1;H0:9]>>[#7:4]-[c:3]1:[#7;a:5]:[c:6]:[#7;a:7]:[c:8](-[Cl;D1;H0:9]):[c:2]:1-[NH2;D1;+0:1]
76.1
[{"value": 76.1, "product": "ClC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
6-Chloro-N-{3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}-5-nitropyrimidin-4-amine hydrochloride (2.04 g) was suspended in diethyl ether (9.45 mL) and a solution of tin(IV) chloride dihydrate (9.1 g) in conc. hydrochloric acid (20.17 mL) was added under ice-cooling. After stirring at room temperature for 3 hrs, the rea...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccncc1.c1ccccc1.c1cncnc1
Other
Cl.C(C)OCC
null
3
Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3[N+](=O)[O-])cc2C)cn1>Cl.C(C)OCC>Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3N)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4226dfb0ba9b476a983799e165bc9e57
Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3N)cc2C)cn1.[I-]>>Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1.I
C(O)([O-])=O.[Na+].ClC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N.[I-].[Na+].O>>I.IC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N
Cl[c:16]1[n:15][cH:14][n:13][c:12]([NH:11][c:10]2[cH:9][cH:8][c:7]([O:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[n:24][cH:23]3)[c:21]([CH3:22])[cH:20]2)[c:18]1[NH2:19].[I-:17]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n:13][cH:14][n:15][c:16]([I:17])[c:18]3[NH2:19])[cH:20][c:21]2[CH3:22])[cH:...
Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3N)cc2C)cn1.[I-]
Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1.I
null
null
I.C(C)(=O)OCC
Functional Group Interconversion
OtherReaction
0e5e018dae2d5b301dea7fbf3d4d324b1e81c774be63c615b15b41b2296e4e71
4131cd1655d0ec8ecf7e181a36ab37eb3293d734e38ece0acf0e59405d170401
c1cncc(Oc2ccc(Nc3ccncn3)cc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#7:6]):[c:7]:1-[N;D1;H2:8].[I-;H0;D0:9]>>[#7:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[I;H0;D1;+0:9]):[c:7]:1-[N;D1;H2:8]
95.3
[{"value": 95.3, "product": "I.IC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
6-Chloro-N4-{3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}pyrimidine-4,5-diamine (400 mg) was suspended in 55% hydriodic acid (6.16 mL), sodium iodide (878 mg) was added, and the mixture was stirred with heating at 70° C. for 10 min. After cooling to room temperature, water (40 mL)/ethyl acetate (30 mL) was added. Afte...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Aromatic halide
c1cncnc1
c1cncnc1
c1ccncc1.c1ccccc1.c1cncnc1
null
I.C(C)(=O)OCC
70
null
Cc1ccc(Oc2ccc(Nc3ncnc(Cl)c3N)cc2C)cn1.[I-]>I.C(C)(=O)OCC>Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1.I
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-31e1da1d74164f3a9392798a95736361
CC#N.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>>Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4cccc(N)c4)c3N)cc2C)cn1
I.IC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N.C(C)#N>>NC=1C=C(C=CC1)C#CC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N
[C:17]([CH3:21])#[N:24].I[c:16]1[n:15][cH:14][n:13][c:12]([NH:11][c:10]2[cH:9][cH:8][c:7]([O:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[n:32][cH:31]3)[c:29]([CH3:30])[cH:28]2)[c:26]1[NH2:27]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n:13][cH:14][n:15][c:16]([C:17]#[C:18][c:19]4[cH:20][cH:21][...
CC#N.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1
Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4cccc(N)c4)c3N)cc2C)cn1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I
C(C)N(CC)CC.C(#C)C=1C=C(N)C=CC1
Aromatic Heterocycle Formation
OtherReaction
9479db21649e30fa62ec6536b7f69bbd536b5b3c68b5c30e0fb864e7cf23f38c
ecdc94851be19e19a274edc6d2f8ac2fade83b0d0869127678215e856fcafd6f
C(#Cc1cc(Nc2ccc(Oc3cccnc3)cc2)ncn1)c1ccccc1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#7:6]):[c:7]:1-[N;D1;H2:8].[CH3;D1;+0:9]-[C;H0;D2;+0:10]#[N;H0;D1;+0:11]>>[#7:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[C;H0;D2;+0:10]#[C:12]-[c:13]2:[c:14]:[cH;D2;+0:9]:[c:15]:[c:16](-[NH2;D1;+0:11]):[c:17]:2):[c:7]:1-[N;D1;H2:8]
null
[]
null
null
1.5
HOUR
6-Iodo-N4-{3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}pyrimidine-4,5-diamine hydroiodide (200 mg) was dissolved in a mixed solvent of acetonitrile (7.6 mL)/triethylamine (5.72 mL), 3-ethynylaniline (0.0574 mL), trans-dichlorobis(triphenylphosphine)palladium(II) (15.4 mg) and copper(I) iodide (5.3 mg) were sequentiall...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Nitrile
Primary amine.Alkyne
c1cncnc1
c1cncnc1.c1ccccc1
c1ccncc1.c1ccccc1.c1cncnc1.c1ccccc1
I-
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)N(CC)CC.C(#C)C=1C=C(N)C=CC1
null
1.5
CC#N.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)N(CC)CC.C(#C)C=1C=C(N)C=CC1>Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4cccc(N)c4)c3N)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2ab1f8bae8a043e4b9fa9fee77ad79a2
C#Cc1ccc(N)cc1.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>>Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4ccc(N)cc4)c3N)cc2C)cn1
I.IC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N.C(#C)C1=CC=C(N)C=C1>>NC1=CC=C(C=C1)C#CC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N
[CH:17]#[C:18][c:19]1[cH:20][cH:21][c:22]([NH2:23])[cH:24][cH:25]1.I[c:16]1[n:15][cH:14][n:13][c:12]([NH:11][c:10]2[cH:9][cH:8][c:7]([O:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[n:32][cH:31]3)[c:29]([CH3:30])[cH:28]2)[c:26]1[NH2:27]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n:13][cH:14][n:15...
C#Cc1ccc(N)cc1.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1
Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4ccc(N)cc4)c3N)cc2C)cn1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I
C(C)#N.C(C)N(CC)CC
C-C Coupling
Sonogashira alkyne_aryl halide
6c841971a35ffd50215936cda19c192218792b140679c95a1b7a8fa56d8a741b
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
C(#Cc1cc(Nc2ccc(Oc3cccnc3)cc2)ncn1)c1ccccc1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#7:6]):[c:7]:1-[N;D1;H2:8].[CH;D1;+0:9]#[C:10]-[c:11]>>[#7:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[C;H0;D2;+0:9]#[C:10]-[c:11]):[c:7]:1-[N;D1;H2:8]
65.9
[{"value": 65.9, "product": "NC1=CC=C(C=C1)C#CC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
6-Iodo-N4-{3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}pyrimidine-4,5-diamine hydroiodide (270 mg) was dissolved in a mixed solvent of acetonitrile (10.3 mL)/triethylamine (7.72 mL), and 4-ethynylaniline (80.3 mg), trans-dichlorobis(triphenylphosphine)palladium(II) (20.8 mg) and copper(I) iodide (7.16 mg) were sequent...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1cncnc1
c1cncnc1
c1ccncc1.c1ccccc1.c1cncnc1.c1ccccc1
HI
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC
null
null
C#Cc1ccc(N)cc1.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC>Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4ccc(N)cc4)c3N)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2b9adc720be54eb48d919d4ef7b1d0db
COCC(=O)O.Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccc(N)cc5)[nH]c34)cc2C)cn1>>COCC(=O)Nc1ccc(-c2cc3ncnc(Nc4ccc(Oc5ccc(C)nc5)c(C)c4)c3[nH]2)cc1
Cl.C(C)N=C=NCCCN(C)C.NC1=CC=C(C=C1)C1=CC=2N=CN=C(C2N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C.COCC(=O)O.O.ON1N=NC2=C1C=CC=C2>>COCC(=O)NC1=CC=C(C=C1)C1=CC=2N=CN=C(C2N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C
O[C:4]([CH2:3][O:2][CH3:1])=[O:5].[NH2:6][c:7]1[cH:8][cH:9][c:10](-[c:11]2[cH:12][c:13]3[n:14][cH:15][n:16][c:17]([NH:18][c:19]4[cH:20][cH:21][c:22]([O:23][c:24]5[cH:25][cH:26][c:27]([CH3:28])[n:29][cH:30]5)[c:31]([CH3:32])[cH:33]4)[c:34]3[nH:35]2)[cH:36][cH:37]1>>[CH3:1][O:2][CH2:3][C:4](=[O:5])[NH:6][c:7]1[cH:8][cH:9...
COCC(=O)O.Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccc(N)cc5)[nH]c34)cc2C)cn1
COCC(=O)Nc1ccc(-c2cc3ncnc(Nc4ccc(Oc5ccc(C)nc5)c(C)c4)c3[nH]2)cc1
null
null
ClCCl.C(C)N(CC)CC.CN(C=O)C
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
c1ccc(-c2cc3ncnc(Nc4ccc(Oc5cccnc5)cc4)c3[nH]2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#8:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[#8:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]
null
[]
null
null
8
HOUR
To a mixture of 6-(4-aminophenyl)-N-{3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}-5H-pyrrolo[3,2-d]pyrimidin-4-amine (40 mg), methoxyacetic acid (0.0145 mL) and 1-hydroxybenzotriazole monohydrate (38 mg) in N,N-dimethylformamide (1.9 mL) were added 1-ethyl-3-(3-dimethylaminopropyl)carbodiimide hydrochloride (54 mg) an...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1.c1ccncc1
HO-
ClCCl.C(C)N(CC)CC.CN(C=O)C
null
8
COCC(=O)O.Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccc(N)cc5)[nH]c34)cc2C)cn1>ClCCl.C(C)N(CC)CC.CN(C=O)C>COCC(=O)Nc1ccc(-c2cc3ncnc(Nc4ccc(Oc5ccc(C)nc5)c(C)c4)c3[nH]2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7c26f329438144e5a573a4dafd81a192
CCOC(=O)c1[nH]c(-c2ccc(OC)cc2)cc1N.N=CN>>COc1ccc(-c2cc3ncnc(O)c3[nH]2)cc1
NC1=C(NC(=C1)C1=CC=C(C=C1)OC)C(=O)OCC.C(=N)N>>COC1=CC=C(C=C1)C1=CC=2N=CN=C(C2N1)O
CCO[C:13](=[O:14])[c:15]1[c:9]([NH2:10])[cH:8][c:7](-[c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:18][cH:17]2)[nH:16]1.N[CH:11]=[NH:12]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][c:9]3[n:10][cH:11][n:12][c:13]([OH:14])[c:15]3[nH:16]2)[cH:17][cH:18]1
CCOC(=O)c1[nH]c(-c2ccc(OC)cc2)cc1N.N=CN
COc1ccc(-c2cc3ncnc(O)c3[nH]2)cc1
null
null
O1CCCC1.C(C)O
Aromatic Heterocycle Formation
OtherReaction
18676698bc1e56bd5ff1be71d10b0382d6f0e2c88c191655a5947d8927e09a11
be53a05fe81ad29ab5edbac9868dcfdb06310f53b9ff1c00e98e247b0cca57da
c1ccc(-c2cc3ncncc3[nH]2)cc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3]1:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[NH2;D1;+0:8].N-[CH;D2;+0:9]=[NH;D1;+0:10]>>[OH;D1;+0:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:10]:[cH;D2;+0:9]:[n;H0;D2;+0:8]:[c:7]2:[c:6]:[c:5]:[#7;a:4]:[c:3]:2:1
11.5
[{"value": 11.5, "product": "COC1=CC=C(C=C1)C1=CC=2N=CN=C(C2N1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
16
HOUR
Ethyl 3-amino-5-(4-methoxyphenyl)-1H-pyrrole-2-carboxylate (7.2 g) was dissolved in tetrahydrofuran (16 mL)/ethanol (32 mL), formamidine (3.46 g) was added, and the mixture was stirred at 90° C. for 16 hrs. After cooling to room temperature, tetrahydrofuran was evaporated under reduced pressure. The residue was diluted...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine.Primary amine
Aromatic alcohol
c1cc[nH]c1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1
HO-
O1CCCC1.C(C)O
90
16
CCOC(=O)c1[nH]c(-c2ccc(OC)cc2)cc1N.N=CN>O1CCCC1.C(C)O>COc1ccc(-c2cc3ncnc(O)c3[nH]2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e43e5db6e580456d9a4f69a348f2ca38
COc1ccc(-c2cc3ncnc(O)c3[nH]2)cc1.O=P(Cl)(Cl)Cl>>COc1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1
COC1=CC=C(C=C1)C1=CC=2N=CN=C(C2N1)O.N.P(=O)(Cl)(Cl)Cl.ClCCCl>>ClC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C=C2)OC
O[c:13]1[n:12][cH:11][n:10][c:9]2[cH:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:18][cH:17]3)[nH:16][c:15]21.O=P(Cl)(Cl)[Cl:14]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][c:9]3[n:10][cH:11][n:12][c:13]([Cl:14])[c:15]3[nH:16]2)[cH:17][cH:18]1
COc1ccc(-c2cc3ncnc(O)c3[nH]2)cc1.O=P(Cl)(Cl)Cl
COc1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1
null
null
O1CCCC1.C(C)N(C1=CC=CC=C1)CC
Functional Group Interconversion
Alcohol to chloride_POCl3_ortho
2abe710ccd285a9ab92e9161186a087fb3ea26b59ffc48b8e24881a6657aca35
e71580a8ffadb7b2717ecd7d68c1d3c0ca161ba5e6a787a49dad5a1359adc993
c1ccc(-c2cc3ncncc3[nH]2)cc1
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]2:[c:7]:[c:8]:[#7;a:9]:[c:10]:2:1>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]2:[c:7]:[c:8]:[#7;a:9]:[c:10]:2:1
null
[]
110
CELSIUS
null
null
6-(4-Methoxyphenyl)-5H-pyrrolo[3,2-d]pyrimidin-4-ol (500 mg) was suspended in N,N-diethylaniline (1.11 mL)/1,2-dichloroethane (3.73 mL), phosphorus oxychloride (2.29 mL) was added, and the mixture was stirred with heating at 110° C. for 2 hrs. After cooling to room temperature, the reaction mixture was treated with ice...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol
Aromatic halide
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1
HCl
O1CCCC1.C(C)N(C1=CC=CC=C1)CC
110
null
COc1ccc(-c2cc3ncnc(O)c3[nH]2)cc1.O=P(Cl)(Cl)Cl>O1CCCC1.C(C)N(C1=CC=CC=C1)CC>COc1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ae0ffbc24bf94abf8f27c817017de8b9
C#Cc1cccc(CNC(=O)OC(C)(C)C)c1.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>>Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4cccc(CNC(=O)OC(C)(C)C)c4)c3N)cc2C)cn1
I.IC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N.C(#C)C=1C=C(CNC(OC(C)(C)C)=O)C=CC1>>NC=1C(=NC=NC1NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)C#CC=1C=C(CNC(OC(C)(C)C)=O)C=CC1
[CH:17]#[C:18][c:19]1[cH:20][cH:21][cH:22][c:23]([CH2:24][NH:25][C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32])[cH:33]1.I[c:16]1[n:15][cH:14][n:13][c:12]([NH:11][c:10]2[cH:9][cH:8][c:7]([O:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[n:40][cH:39]3)[c:37]([CH3:38])[cH:36]2)[c:34]1[NH2:35]>>[CH3:1][c:2]1[cH:3][cH:4][c:5](...
C#Cc1cccc(CNC(=O)OC(C)(C)C)c1.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1
Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4cccc(CNC(=O)OC(C)(C)C)c4)c3N)cc2C)cn1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I
C(C)#N.C(C)N(CC)CC
C-C Coupling
Sonogashira alkyne_aryl halide
6c841971a35ffd50215936cda19c192218792b140679c95a1b7a8fa56d8a741b
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
C(#Cc1cc(Nc2ccc(Oc3cccnc3)cc2)ncn1)c1ccccc1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#7:6]):[c:7]:1-[N;D1;H2:8].[CH;D1;+0:9]#[C:10]-[c:11]>>[#7:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[C;H0;D2;+0:9]#[C:10]-[c:11]):[c:7]:1-[N;D1;H2:8]
78.6
[{"value": 78.6, "product": "NC=1C(=NC=NC1NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)C#CC=1C=C(CNC(OC(C)(C)C)=O)C=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
6-Iodo-N4-{3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}pyrimidine-4,5-diamine hydroiodide (500 mg) was dissolved in a mixed solvent of acetonitrile (14.8 mL)/triethylamine (11.0 mL), and tert-butyl 3-ethynylbenzylcarbamate (247 mg), trans-dichlorobis(triphenylphosphine)palladium(II) (31.3 mg) and copper(I) iodide (10....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1cncnc1
c1cncnc1
c1ccncc1.c1ccccc1.c1cncnc1.c1ccccc1
HI
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC
null
null
C#Cc1cccc(CNC(=O)OC(C)(C)C)c1.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC>Cc1ccc(Oc2ccc(Nc3ncnc(C#Cc4cccc(CNC(=O)OC(C)(C)C)c4)c3N)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5c17533672144538af8d2d4610f9827a
Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5cccc(CNC(=O)OC(C)(C)C)c5)[nH]c34)cc2C)cn1>>Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5cccc(CN)c5)[nH]c34)cc2C)cn1
CC=1C=C(C=CC1OC=1C=NC(=CC1)C)NC=1C2=C(N=CN1)C=C(N2)C=2C=C(CNC(OC(C)(C)C)=O)C=CC2.Cl.[OH-].[Na+]>>NCC=1C=C(C=CC1)C1=CC=2N=CN=C(C2N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C
CC(C)(C)OC(=O)[NH:25][CH2:24][c:23]1[cH:22][cH:21][cH:20][c:19](-[c:18]2[cH:17][c:16]3[n:15][cH:14][n:13][c:12]([NH:11][c:10]4[cH:9][cH:8][c:7]([O:6][c:5]5[cH:4][cH:3][c:2]([CH3:1])[n:33][cH:32]5)[c:30]([CH3:31])[cH:29]4)[c:28]3[nH:27]2)[cH:26]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12...
Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5cccc(CNC(=O)OC(C)(C)C)c5)[nH]c34)cc2C)cn1
Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5cccc(CN)c5)[nH]c34)cc2C)cn1
null
null
O1CCCC1
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
c1ccc(-c2cc3ncnc(Nc4ccc(Oc5cccnc5)cc4)c3[nH]2)cc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]-[c:3]>>[NH2;D1;+0:1]-[C:2]-[c:3]
87.7
[{"value": 87.7, "product": "NCC=1C=C(C=CC1)C1=CC=2N=CN=C(C2N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
tert-Butyl 3-[4-({3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}amino)-5H-pyrrolo[3,2-d]pyrimidin-6-yl]benzylcarbamate (230 mg) was suspended in tetrahydrofuran (2.3 mL), 2N hydrochloric acid (2.3 mL) was added, and the mixture was stirred with heating at 60° C. for 3 hrs. After cooling to room temperature, 1N aqueous s...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccncc1.c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
HO-
O1CCCC1
60
null
Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5cccc(CNC(=O)OC(C)(C)C)c5)[nH]c34)cc2C)cn1>O1CCCC1>Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5cccc(CN)c5)[nH]c34)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ad29a69ef23740bf8672496c4623d8d1
C#CCNC(=O)OC(C)(C)C.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>>Cc1ccc(Oc2ccc(Nc3ncnc(C#CCNC(=O)OC(C)(C)C)c3N)cc2C)cn1
I.IC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N.C(C#C)NC(OC(C)(C)C)=O>>NC=1C(=NC=NC1NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)C#CCNC(OC(C)(C)C)=O
[CH:17]#[C:18][CH2:19][NH:20][C:21](=[O:22])[O:23][C:24]([CH3:25])([CH3:26])[CH3:27].I[c:16]1[n:15][cH:14][n:13][c:12]([NH:11][c:10]2[cH:9][cH:8][c:7]([O:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[n:34][cH:33]3)[c:31]([CH3:32])[cH:30]2)[c:28]1[NH2:29]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3...
C#CCNC(=O)OC(C)(C)C.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1
Cc1ccc(Oc2ccc(Nc3ncnc(C#CCNC(=O)OC(C)(C)C)c3N)cc2C)cn1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I
C(C)#N.C(C)N(CC)CC
C-C Coupling
Sonogashira alkyne_aryl halide
6c841971a35ffd50215936cda19c192218792b140679c95a1b7a8fa56d8a741b
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
c1cncc(Oc2ccc(Nc3ccncn3)cc2)c1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#7:6]):[c:7]:1-[N;D1;H2:8].[C:9]-[C:10]#[CH;D1;+0:11]>>[#7:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[C;H0;D2;+0:11]#[C:10]-[C:9]):[c:7]:1-[N;D1;H2:8]
73.8
[{"value": 73.8, "product": "NC=1C(=NC=NC1NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)C#CCNC(OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
6-Iodo-N4-{3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}pyrimidine-4,5-diamine hydroiodide (500 mg) was dissolved in a mixed solvent of acetonitrile (14.8 mL)/triethylamine (11.0 mL), and tert-butyl 2-propynylcarbamate (166 mg), trans-dichlorobis(triphenylphosphine)palladium(II) (31.3 mg) and copper(I) iodide (10.2 mg)...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1cncnc1
c1cncnc1
c1ccncc1.c1ccccc1.c1cncnc1
HI
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC
null
null
C#CCNC(=O)OC(C)(C)C.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC>Cc1ccc(Oc2ccc(Nc3ncnc(C#CCNC(=O)OC(C)(C)C)c3N)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8076fb2b785b432da01a6555b29f9f2b
C#C/C=C/CNC(=O)OC(C)(C)C.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>>Cc1ccc(Oc2ccc(Nc3ncnc(C#C/C=C/CNC(=O)OC(C)(C)C)c3N)cc2C)cn1
I.IC1=C(C(=NC=N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)N.C(\C=C\C#C)NC(OC(C)(C)C)=O>>NC=1C(=NC=NC1NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)C#C/C=C/CNC(OC(C)(C)C)=O
[CH:17]#[C:18]/[CH:19]=[CH:20]/[CH2:21][NH:22][C:23](=[O:24])[O:25][C:26]([CH3:27])([CH3:28])[CH3:29].I[c:16]1[n:15][cH:14][n:13][c:12]([NH:11][c:10]2[cH:9][cH:8][c:7]([O:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[n:36][cH:35]3)[c:33]([CH3:34])[cH:32]2)[c:30]1[NH2:31]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:1...
C#C/C=C/CNC(=O)OC(C)(C)C.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1
Cc1ccc(Oc2ccc(Nc3ncnc(C#C/C=C/CNC(=O)OC(C)(C)C)c3N)cc2C)cn1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I
C(C)#N.C(C)N(CC)CC
C-C Coupling
Sonogashira alkyne_aryl halide
6c841971a35ffd50215936cda19c192218792b140679c95a1b7a8fa56d8a741b
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
c1cncc(Oc2ccc(Nc3ccncn3)cc2)c1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#7:6]):[c:7]:1-[N;D1;H2:8].[C:9]/[C:10]=[C:11]/[C:12]#[CH;D1;+0:13]>>[#7:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[C;H0;D2;+0:13]#[C:12]/[C:11]=[C:10]/[C:9]):[c:7]:1-[N;D1;H2:8]
45.9
[{"value": 45.9, "product": "NC=1C(=NC=NC1NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C)C#C/C=C/CNC(OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
6-Iodo-N4-{3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}pyrimidine-4,5-diamine hydroiodide (500 mg) was dissolved in a mixed solvent of acetonitrile (14.8 mL)/triethylamine (11.0 mL), and tert-butyl (2E)-2-penten-4-yn-1-ylcarbamate (194 mg), trans-dichlorobis(triphenylphosphine)palladium(II) (31.3 mg) and copper(I) iod...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1cncnc1
c1cncnc1
c1ccncc1.c1ccccc1.c1cncnc1
HI
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC
null
null
C#C/C=C/CNC(=O)OC(C)(C)C.Cc1ccc(Oc2ccc(Nc3ncnc(I)c3N)cc2C)cn1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC>Cc1ccc(Oc2ccc(Nc3ncnc(C#C/C=C/CNC(=O)OC(C)(C)C)c3N)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ded10e89a71c4d389ae0f9a7b910f953
Nc1c(I)ncnc1I.Oc1ccccc1>>Nc1c(I)ncnc1Oc1ccccc1
IC1=NC=NC(=C1N)I.C1(=CC=CC=C1)O.C([O-])([O-])=O.[K+].[K+]>>IC1=NC=NC(=C1N)OC1=CC=CC=C1
I[c:8]1[c:2]([NH2:1])[c:3]([I:4])[n:5][cH:6][n:7]1.[OH:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1>>[NH2:1][c:2]1[c:3]([I:4])[n:5][cH:6][n:7][c:8]1[O:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1
Nc1c(I)ncnc1I.Oc1ccccc1
Nc1c(I)ncnc1Oc1ccccc1
null
null
CN1C(CCC1)=O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
38da1e480b17968341fc50d07104da93d31f20765e3b36e5a0790cb6b1d88a10
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccncn2)cc1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[I;D1;H0:6]):[c:7]:1-[N;D1;H2:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[I;D1;H0:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:9]-[c:10](:[c:11]):[c:12]):[c:7]:1-[N;D1;H2:8]
100.7
[{"value": 100.7, "product": "IC1=NC=NC(=C1N)OC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
16
HOUR
4,6-Diiodopyrimidin-5-amine (2.2 g) was dissolved in 1-methyl-2-pyrrolidone (11.5 mL), phenol (656 mg) and potassium carbonate (964 mg) were added, and the mixture was stirred at 100° C. for 16 hrs. After cooling to room temperature, the mixture was diluted with ethyl acetate (200 mL) and washed successively with water...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1cncnc1
c1cncnc1
c1cncnc1.c1ccccc1
HI
CN1C(CCC1)=O.C(C)(=O)OCC
100
16
Nc1c(I)ncnc1I.Oc1ccccc1>CN1C(CCC1)=O.C(C)(=O)OCC>Nc1c(I)ncnc1Oc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ccbcaae9a5f940c3a8350c0dd2d6f435
C#C/C=C/CO[Si](C)(C)C(C)(C)C.Nc1c(I)ncnc1Oc1ccccc1>>CC(C)(C)[Si](C)(C)OC/C=C/C#Cc1ncnc(Oc2ccccc2)c1N
IC1=NC=NC(=C1N)OC1=CC=CC=C1.C(C)(C)(C)[Si](OC\C=C\C#C)(C)C>>[Si](C)(C)(C(C)(C)C)OC/C=C/C#CC1=NC=NC(=C1N)OC1=CC=CC=C1
[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][CH2:9]/[CH:10]=[CH:11]/[C:12]#[CH:13].I[c:14]1[n:15][cH:16][n:17][c:18]([O:19][c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[c:26]1[NH2:27]>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][CH2:9]/[CH:10]=[CH:11]/[C:12]#[C:13][c:14]1[n:15][cH:16][n:17...
C#C/C=C/CO[Si](C)(C)C(C)(C)C.Nc1c(I)ncnc1Oc1ccccc1
CC(C)(C)[Si](C)(C)OC/C=C/C#Cc1ncnc(Oc2ccccc2)c1N
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I
C(C)#N.C(C)N(CC)CC
C-C Coupling
Sonogashira alkyne_aryl halide
6c841971a35ffd50215936cda19c192218792b140679c95a1b7a8fa56d8a741b
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
c1ccc(Oc2ccncn2)cc1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#8:6]):[c:7]:1-[N;D1;H2:8].[C:9]/[C:10]=[C:11]/[C:12]#[CH;D1;+0:13]>>[#8:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[C;H0;D2;+0:13]#[C:12]/[C:11]=[C:10]/[C:9]):[c:7]:1-[N;D1;H2:8]
87.8
[{"value": 87.8, "product": "[Si](C)(C)(C(C)(C)C)OC/C=C/C#CC1=NC=NC(=C1N)OC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
4-Iodo-6-phenoxypyrimidin-5-amine (1.0 g) was dissolved in a mixed solvent of acetonitrile (53 mL)/triethylamine (39 mL), and tert-butyl(dimethyl)[(2E)-2-penten-4-ynyloxy]silane (753 mg), trans-dichlorobis(triphenylphosphine)palladium(II) (112 mg) and copper(I) iodide (36.5 mg) were sequentially added. The title compou...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1cncnc1
c1cncnc1
c1cncnc1.c1ccccc1
HI
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC
null
null
C#C/C=C/CO[Si](C)(C)C(C)(C)C.Nc1c(I)ncnc1Oc1ccccc1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC>CC(C)(C)[Si](C)(C)OC/C=C/C#Cc1ncnc(Oc2ccccc2)c1N
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ad3b6a294f744dfd8cf1500c0e64560d
CC(C)(C)[Si](C)(C)OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1.CCI>>CCn1c(/C=C/CO[Si](C)(C)C(C)(C)C)cc2ncnc(Oc3ccccc3)c21
[Si](C)(C)(C(C)(C)C)OC/C=C/C1=CC=2N=CN=C(C2N1)OC1=CC=CC=C1.C([O-])([O-])=O.[Cs+].[Cs+].ICC>>[Si](C)(C)(C(C)(C)C)OC/C=C/C1=CC=2N=CN=C(C2N1CC)OC1=CC=CC=C1
[nH:3]1[c:4](/[CH:5]=[CH:6]/[CH2:7][O:8][Si:9]([CH3:10])([CH3:11])[C:12]([CH3:13])([CH3:14])[CH3:15])[cH:16][c:17]2[n:18][cH:19][n:20][c:21]([O:22][c:23]3[cH:24][cH:25][cH:26][cH:27][cH:28]3)[c:29]12.I[CH2:2][CH3:1]>>[CH3:1][CH2:2][n:3]1[c:4](/[CH:5]=[CH:6]/[CH2:7][O:8][Si:9]([CH3:10])([CH3:11])[C:12]([CH3:13])([CH3:14...
CC(C)(C)[Si](C)(C)OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1.CCI
CCn1c(/C=C/CO[Si](C)(C)C(C)(C)C)cc2ncnc(Oc3ccccc3)c21
null
null
CN(C=O)C.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
e9fbaa0885668a0db6604d7955d2895802f0f03f498828bb48474e6359c120b7
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Oc2ncnc3cc[nH]c23)cc1
I-[CH2;D2;+0:1]-[C;D1;H3:2].[#8:3]-[c:4]1:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]2:[c:9]:[c:10](/[C:11]=[C:12]/[C:13]):[nH;D2;+0:14]:[c:15]:2:1>>[#8:3]-[c:4]1:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]2:[c:9]:[c:10](/[C:11]=[C:12]/[C:13]):[n;H0;D3;+0:14](-[CH2;D2;+0:1]-[C;D1;H3:2]):[c:15]:2:1
null
[]
null
null
20
MINUTE
6-((1E)-3-{[tert-Butyl(dimethyl)silyl]oxy}-1-propenyl)-4-phenoxy-5H-pyrrolo[3,2-d]pyrimidine (100 mg) was dissolved in N,N-dimethylformamide (0.786 mL), cesium carbonate (102.6 mg) was added, and the mixture was stirred at room temperature for 20 min. Iodoethane (0.0231 mL) was added and the mixture was stirred at room...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1cc2ncncc2[nH]1
c1cc2ncncc2[nH]1.c1ccccc1
HI
CN(C=O)C.C(C)(=O)OCC
null
0.333333
CC(C)(C)[Si](C)(C)OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1.CCI>CN(C=O)C.C(C)(=O)OCC>CCn1c(/C=C/CO[Si](C)(C)C(C)(C)C)cc2ncnc(Oc3ccccc3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eb44393fedd44638a22d225f917392a8
CCn1c(/C=C/CO[Si](C)(C)C(C)(C)C)cc2ncnc(Oc3ccccc3)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1>>CCn1c(/C=C/CO)cc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
[Si](C)(C)(C(C)(C)C)OC/C=C/C1=CC=2N=CN=C(C2N1CC)OC1=CC=CC=C1.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C.Cl.N1=CC=CC=C1.C1(=CC=CC=C1)O>>C(C)N1C(=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C)/C=C/CO
CC(C)(C)[Si](C)(C)[O:8][CH2:7]/[CH:6]=[CH:5]/[c:4]1[n:3]([CH2:2][CH3:1])[c:31]2[c:10]([cH:9]1)[n:11][cH:12][n:13][c:14]2Oc1ccccc1.[NH2:15][c:16]1[cH:17][cH:18][c:19]([O:20][c:21]2[cH:22][cH:23][c:24]([CH3:25])[n:26][cH:27]2)[c:28]([CH3:29])[cH:30]1>>[CH3:1][CH2:2][n:3]1[c:4](/[CH:5]=[CH:6]/[CH2:7][OH:8])[cH:9][c:10]2[n...
CCn1c(/C=C/CO[Si](C)(C)C(C)(C)C)cc2ncnc(Oc3ccccc3)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1
CCn1c(/C=C/CO)cc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
null
null
ClCCl
Heteroatom Alkylation and Arylation
OtherReaction
a1eaf5ebc4b4900f6857056acac1768d131704c45cce2efb15e191262f5f7179
f5f4bef2dd57edef4ab5c305326a2437314e70311439cfd2555321357dbf7835
c1cncc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)c1
C-C(-C)(-C)-[Si](-C)(-C)-[O;H0;D2;+0:1]-[C:2]/[C:3]=[C:4]/[c:5]1:[c:6]:[c:7]2:[#7;a:8]:[c:9]:[#7;a:10]:[c;H0;D3;+0:11](-O-c3:c:c:c:c:c:3):[c:12]:2:[#7;a:13]:1-[C:14].[NH2;D1;+0:15]-[c:16](:[c:17]):[c:18]>>[C:14]-[#7;a:13]1:[c:12]2:[c:7](:[#7;a:8]:[c:9]:[#7;a:10]:[c;H0;D3;+0:11]:2-[NH;D2;+0:15]-[c:16](:[c:17]):[c:18]):[...
40.4
[{"value": 40.4, "product": "C(C)N1C(=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C)/C=C/CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
A mixture of 6-((1E)-3-{[tert-butyl(dimethyl)silyl]oxy}-1-propenyl)-5-ethyl-4-phenoxy-5H-pyrrolo[3,2-d]pyrimidine (78 mg), 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (61.2 mg), pyridine hydrochloride (26 mg) and phenol (122 mg) was stirred with heating at 120° C. for 16 hrs. After cooling to room temperature, the mi...
10.6084/m9.figshare.5104873.v1
null
Ether.Primary amine.TMS ether protective group
Primary alcohol.Secondary amine
c1cc2ncncc2[nH]1.c1ccccc1
c1cc2ncncc2[nH]1
c1cc2ncncc2[nH]1.c1ccccc1.c1ccncc1
HO-
ClCCl
120
null
CCn1c(/C=C/CO[Si](C)(C)C(C)(C)C)cc2ncnc(Oc3ccccc3)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1>ClCCl>CCn1c(/C=C/CO)cc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1faed6812f684d00b3aaf60cd35bf7e6
Nc1c(I)ncnc1Oc1ccccc1>>Nc1c(C#CCO)ncnc1Oc1ccccc1
IC1=NC=NC(=C1N)OC1=CC=CC=C1>>NC=1C(=NC=NC1OC1=CC=CC=C1)C#CCO
I[c:3]1[c:2]([NH2:1])[c:11]([O:7][c:13]2[cH:4][cH:17][cH:16][cH:15][cH:14]2)[n:10][cH:9][n:8]1>>[NH2:1][c:2]1[c:3]([C:4]#[C:5][CH2:6][OH:7])[n:8][cH:9][n:10][c:11]1[O:12][c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1
Nc1c(I)ncnc1Oc1ccccc1
Nc1c(C#CCO)ncnc1Oc1ccccc1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I
C(C)#N.C(C)N(CC)CC.C(C#C)O
Functional Group Interconversion
OtherReaction
57ebbe5fd5c1741fec67270624e2926453ae7b2f9493e06540b1b522a4865675
44d512cffe65b29b4402cc366a02515ed1e944ff9cea2dc70b9806744975fec2
c1ccc(Oc2ccncn2)cc1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c;H0;D3;+0:5](-[O;H0;D2;+0:6]-[c;H0;D3;+0:7]2:[c:8]:[c:9]:[c:10]:[cH;D2;+0:11]:[cH;D2;+0:12]:2):[c:13]:1-[N;D1;H2:14]>>[N;D1;H2:14]-[c:13]1:[c;H0;D3;+0:5](-[#8:15]-[c;H0;D3;+0:7]2:[c:8]:[c:9]:[c:10]:[cH;D2;+0:11]:[c:16]:2):[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[C;H0;D2;+0:1...
174.8
[{"value": 174.8, "product": "NC=1C(=NC=NC1OC1=CC=CC=C1)C#CCO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
4-Iodo-6-phenoxypyrimidin-5-amine (3.0 g) was dissolved in a mixed solvent of acetonitrile (159 mL)/triethylamine (117 mL), and 2-propyn-1-ol (0.669 mL), trans-dichlorobis(triphenylphosphine)palladium(II) (336 mg) and copper(I) iodide (109.5 mg) were sequentially added. The title compound (2.02 g) was obtained as cryst...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether
Ether.Primary alcohol.Alkyne
c1cncnc1.c1ccccc1
c1cncnc1.c1ccccc1
c1cncnc1.c1ccccc1
I-
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC.C(C#C)O
null
null
Nc1c(I)ncnc1Oc1ccccc1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC.C(C#C)O>Nc1c(C#CCO)ncnc1Oc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f1465727f5cd409da766af7fb0f88633
C#CC=CCO.Nc1c(I)ncnc1Oc1ccccc1>>Nc1c(C#C/C=C/CO)ncnc1Oc1ccccc1
IC1=NC=NC(=C1N)OC1=CC=CC=C1.C(C=CC#C)O>>NC=1C(=NC=NC1OC1=CC=CC=C1)C#C/C=C/CO
[CH:4]#[C:5][CH:6]=[CH:7][CH2:8][OH:9].I[c:3]1[c:2]([NH2:1])[c:13]([O:14][c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[n:12][cH:11][n:10]1>>[NH2:1][c:2]1[c:3]([C:4]#[C:5]/[CH:6]=[CH:7]/[CH2:8][OH:9])[n:10][cH:11][n:12][c:13]1[O:14][c:15]1[cH:16][cH:17][cH:18][cH:19][cH:20]1
C#CC=CCO.Nc1c(I)ncnc1Oc1ccccc1
Nc1c(C#C/C=C/CO)ncnc1Oc1ccccc1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I
C(C)#N.C(C)N(CC)CC
C-C Coupling
Sonogashira alkyne_aryl halide
6c841971a35ffd50215936cda19c192218792b140679c95a1b7a8fa56d8a741b
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
c1ccc(Oc2ccncn2)cc1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#8:6]):[c:7]:1-[N;D1;H2:8].[C:9]-[C:10]=[C:11]-[C:12]#[CH;D1;+0:13]>>[#8:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[C;H0;D2;+0:13]#[C:12]/[C:11]=[C:10]/[C:9]):[c:7]:1-[N;D1;H2:8]
59.9
[{"value": 59.9, "product": "NC=1C(=NC=NC1OC1=CC=CC=C1)C#C/C=C/CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
4-Iodo-6-phenoxypyrimidin-5-amine (3.5 g) was dissolved in a mixed solvent of acetonitrile (185 mL)/triethylamine (136 mL), and 2-penten-4-yn-1-ol (1.1 g), trans-dichlorobis(triphenylphosphine)palladium(II) (392 mg) and copper(I) iodide (127 mg) were sequentially added. The title compound (1.79 g) was obtained as a pow...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1cncnc1
c1cncnc1
c1cncnc1.c1ccccc1
HI
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC
null
null
C#CC=CCO.Nc1c(I)ncnc1Oc1ccccc1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.[Cu]I.C(C)#N.C(C)N(CC)CC>Nc1c(C#C/C=C/CO)ncnc1Oc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-026c3dfd89c6443588b4b5eb3201a1cf
O=C(Cl)c1ccccc1.OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1>>O=C(OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1)c1ccccc1
O(C1=CC=CC=C1)C=1C2=C(N=CN1)C=C(N2)/C=C/CO.C(C)N(CC)CC.C(C1=CC=CC=C1)(=O)Cl>>C(C1=CC=CC=C1)(=O)OC\C=C\C1=CC=2N=CN=C(C2N1)OC1=CC=CC=C1
Cl[C:2](=[O:1])[c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1.[OH:3][CH2:4]/[CH:5]=[CH:6]/[c:7]1[cH:8][c:9]2[n:10][cH:11][n:12][c:13]([O:14][c:15]3[cH:16][cH:17][cH:18][cH:19][cH:20]3)[c:21]2[nH:22]1>>[O:1]=[C:2]([O:3][CH2:4]/[CH:5]=[CH:6]/[c:7]1[cH:8][c:9]2[n:10][cH:11][n:12][c:13]([O:14][c:15]3[cH:16][cH:17][cH:18][cH:1...
O=C(Cl)c1ccccc1.OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1
O=C(OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1)c1ccccc1
null
null
O1CCCC1.C(C)(=O)OCC
Acylation
Schotten-Baumann to ester
6cefe709828c5bd4655f254e75d5dff9e8876e192e7dd47256c1bc0067bc5291
d8a7643b81ed07a6f633aa99465180dfa0565e61ae25aef36338ebb9837c9cef
O=C(OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#7;a:6]:[c:7]/[C:8]=[C:9]/[C:10]-[OH;D1;+0:11]>>[#7;a:6]:[c:7]/[C:8]=[C:9]/[C:10]-[O;H0;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
(2E)-3-(4-Phenoxy-5H-pyrrolo[3,2-d]pyrimidin-6-yl)-2-propen-1-ol (1.0 g) was suspended in tetrahydrofuran (20 mL), and triethylamine (0.651 mL) and benzoyl chloride (0.86 mL) were sequentially added under ice-cooling. The mixture was stirred under ice-cooling for 2 hrs, diluted with ethyl acetate (200 mL) and washed wi...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary alcohol
Ester
null
null
c1ncc2[nH]ccc2n1.c1ccccc1.c1ccccc1
HCl
O1CCCC1.C(C)(=O)OCC
null
null
O=C(Cl)c1ccccc1.OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1>O1CCCC1.C(C)(=O)OCC>O=C(OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c63d315ef4ab4bcd8927f3798919df88
CI.O=C(OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1)c1ccccc1>>Cn1c(/C=C/COC(=O)c2ccccc2)cc2ncnc(Oc3ccccc3)c21
O.C([O-])([O-])=O.[K+].[K+].IC.C(C1=CC=CC=C1)(=O)OC\C=C\C1=CC=2N=CN=C(C2N1)OC1=CC=CC=C1>>C(C1=CC=CC=C1)(=O)OC\C=C\C1=CC=2N=CN=C(C2N1C)OC1=CC=CC=C1
I[CH3:1].[nH:2]1[c:3](/[CH:4]=[CH:5]/[CH2:6][O:7][C:8](=[O:9])[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16][c:17]2[n:18][cH:19][n:20][c:21]([O:22][c:23]3[cH:24][cH:25][cH:26][cH:27][cH:28]3)[c:29]12>>[CH3:1][n:2]1[c:3](/[CH:4]=[CH:5]/[CH2:6][O:7][C:8](=[O:9])[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16][c:1...
CI.O=C(OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1)c1ccccc1
Cn1c(/C=C/COC(=O)c2ccccc2)cc2ncnc(Oc3ccccc3)c21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
984dc1e2f23276e16434cf60f0728fced0721ac085a767b5a5daa33828d25b2d
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
O=C(OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1)c1ccccc1
I-[CH3;D1;+0:1].[#8:2]-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]2:[c:8]:[c:9](/[C:10]=[C:11]/[C:12]):[nH;D2;+0:13]:[c:14]:2:1>>[#8:2]-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]2:[c:8]:[c:9](/[C:10]=[C:11]/[C:12]):[n;H0;D3;+0:13](-[CH3;D1;+0:1]):[c:14]:2:1
58
[{"value": 58.0, "product": "C(C1=CC=CC=C1)(=O)OC\\C=C\\C1=CC=2N=CN=C(C2N1C)OC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
(2E)-3-(4-Phenoxy-5H-pyrrolo[3,2-d]pyrimidin-6-yl)-2-propenyl benzoate (500 mg) was dissolved in N,N-dimethylformamide (4 mL), and potassium carbonate (279 mg) and iodomethane (0.1 mL) were sequentially added. After stirring at room temperature for 4 hrs, water (30 mL) was added to the reaction mixture and the mixture ...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ncc2[nH]ccc2n1
c1cc2ncncc2[nH]1
c1ccccc1.c1cc2ncncc2[nH]1.c1ccccc1
HI
CN(C=O)C
null
4
CI.O=C(OC/C=C/c1cc2ncnc(Oc3ccccc3)c2[nH]1)c1ccccc1>CN(C=O)C>Cn1c(/C=C/COC(=O)c2ccccc2)cc2ncnc(Oc3ccccc3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eeec170076bf4b1ca4a54008ee18cd62
Cn1c(/C=C/COC(=O)c2ccccc2)cc2ncnc(Oc3ccccc3)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>Cn1c(/C=C/CO)cc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
C(O)([O-])=O.[Na+].C(C1=CC=CC=C1)(=O)OC\C=C\C1=CC=2N=CN=C(C2N1C)OC1=CC=CC=C1.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F.Cl.N1=CC=CC=C1>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=C(N2C)/C=C/CO
O=C(c1ccccc1)[O:7][CH2:6]/[CH:5]=[CH:4]/[c:3]1[n:2]([CH3:1])[c:31]2[c:9]([cH:8]1)[n:10][cH:11][n:12][c:13]2Oc1ccccc1.[NH2:14][c:15]1[cH:16][cH:17][c:18]([O:19][CH2:20][c:21]2[cH:22][cH:23][cH:24][c:25]([F:26])[cH:27]2)[c:28]([Cl:29])[cH:30]1>>[CH3:1][n:2]1[c:3](/[CH:4]=[CH:5]/[CH2:6][OH:7])[cH:8][c:9]2[n:10][cH:11][n:1...
Cn1c(/C=C/COC(=O)c2ccccc2)cc2ncnc(Oc3ccccc3)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
Cn1c(/C=C/CO)cc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
OtherReaction
9f6cea6349504a91cdc9768f306167e35ded894249acbabf53cef7dbb2dc035d
c0530de767090fee49882d17b28eb70d542ad27db18bea6a2b0fe04643a324d6
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
O=C(-[O;H0;D2;+0:1]-[C:2]/[C:3]=[C:4]/[c:5]1:[c:6]:[c:7]2:[#7;a:8]:[c:9]:[#7;a:10]:[c;H0;D3;+0:11](-O-c3:c:c:c:c:c:3):[c:12]:2:[#7;a:13]:1-[C;D1;H3:14])-c1:c:c:c:c:c:1.[NH2;D1;+0:15]-[c:16](:[c:17]):[c:18]>>[C;D1;H3:14]-[#7;a:13]1:[c:12]2:[c:7](:[#7;a:8]:[c:9]:[#7;a:10]:[c;H0;D3;+0:11]:2-[NH;D2;+0:15]-[c:16](:[c:17]):[...
39.5
[{"value": 39.5, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=C(N2C)/C=C/CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
null
null
A mixture of (2E)-3-(5-methyl-4-phenoxy-5H-pyrrolo[3,2-d]pyrimidin-6-yl)-2-propenyl benzoate (100 mg), 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (130 mg), pyridine hydrochloride (36 mg) and 1-methyl-2-pyrrolidone (0.518 mL) was stirred with heating at 140° C. for 4 hrs. After cooling to room temperature, aqueous sodium h...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether.Primary amine
Primary alcohol.Secondary amine
c1ccccc1.c1cc2ncncc2[nH]1.c1ccccc1
c1cc2ncncc2[nH]1
c1cc2ncncc2[nH]1.c1ccccc1.c1ccccc1
HO-
CN1C(CCC1)=O
140
null
Cn1c(/C=C/COC(=O)c2ccccc2)cc2ncnc(Oc3ccccc3)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>CN1C(CCC1)=O>Cn1c(/C=C/CO)cc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-381c2a8b9ebc472ebe4185d0e3002404
COc1ccc(S(=O)(=O)Cl)cc1OC.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1>>COc1ccc(S(=O)(=O)n2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1OC
Cl.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[K+].[K+].COC=1C=C(C=CC1OC)S(=O)(=O)Cl>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2S(=O)(=O)C2=CC(=C(C=C2)OC)OC
Cl[S:7]([c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[c:37]([O:38][CH3:39])[cH:36]1)(=[O:8])=[O:9].[nH:10]1[cH:11][cH:12][c:13]2[n:14][cH:15][n:16][c:17]([NH:18][c:19]3[cH:20][cH:21][c:22]([O:23][CH2:24][c:25]4[cH:26][cH:27][cH:28][c:29]([F:30])[cH:31]4)[c:32]([Cl:33])[cH:34]3)[c:35]12>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([S:7...
COc1ccc(S(=O)(=O)Cl)cc1OC.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1
COc1ccc(S(=O)(=O)n2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1OC
null
null
CN(C=O)C.C(C)(=O)OCC
Acylation
OtherReaction
f39da367e5fdb20ca9cc942039331e6a114631a43c775eca773ad2c497773002
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1ccccc1)n1ccc2ncnc(Nc3ccc(OCc4ccccc4)cc3)c21
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[#7:7]-[c:8]1:[#7;a:9]:[c:10]:[#7;a:11]:[c:12]2:[c:13]:[c:14]:[nH;D2;+0:15]:[c:16]:2:1>>[#7:7]-[c:8]1:[#7;a:9]:[c:10]:[#7;a:11]:[c:12]2:[c:13]:[c:14]:[n;H0;D3;+0:15](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]):[c:16]:2:1
45.1
[{"value": 45.1, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2S(=O)(=O)C2=CC(=C(C=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
N-{3-Chloro-4-[(3-fluorobenzyl)oxy]phenyl}-5H-pyrrolo[3,2-d]pyrimidin-4-amine hydrochloride (150 mg) was dissolved in N,N-dimethylformamide (1.5 mL), and potassium carbonate (102 mg) and (3,4-dimethoxyphenyl)sulfonyl chloride (96.9 mg) were sequentially added under ice-cooling. The mixture was stirred under ice-cooling...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
CN(C=O)C.C(C)(=O)OCC
null
1
COc1ccc(S(=O)(=O)Cl)cc1OC.Fc1cccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2Cl)c1>CN(C=O)C.C(C)(=O)OCC>COc1ccc(S(=O)(=O)n2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-45c2cfdc65294e048ee9111b2f7ed667
CCOC(=O)c1ccc(CCl)o1.Clc1ncnc2cc[nH]c12>>CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[K+].[K+].ClCC1=CC=C(O1)C(=O)OCC>>ClC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC
Cl[CH2:10][c:9]1[cH:8][cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[o:21]1.[nH:11]1[cH:12][cH:13][c:14]2[n:15][cH:16][n:17][c:18]([Cl:19])[c:20]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([CH2:10][n:11]2[cH:12][cH:13][c:14]3[n:15][cH:16][n:17][c:18]([Cl:19])[c:20]23)[o:21]1
CCOC(=O)c1ccc(CCl)o1.Clc1ncnc2cc[nH]c12
CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1coc(Cn2ccc3ncncc32)c1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[#8;a:4]:[c:5]-[C:6](-[#8:7])=[O;D1;H0:8].[Cl;D1;H0:9]-[c:10]1:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]2:[c:15]:[c:16]:[nH;D2;+0:17]:[c:18]:2:1>>[#8:7]-[C:6](=[O;D1;H0:8])-[c:5]:[#8;a:4]:[c:2](-[CH2;D2;+0:1]-[n;H0;D3;+0:17]1:[c:16]:[c:15]:[c:14]2:[#7;a:13]:[c:12]:[#7;a:11]:[c:10](-[Cl;D1;H0:9]):...
82.9
[{"value": 82.9, "product": "ClC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (500 mg) in N,N-dimethylformamide (6.5 mL) was added potassium carbonate (541 mg) under ice-cooling, and the mixture was stirred for 15 min. while warming to room temperature. Ethyl 5-(chloromethyl)-2-furoate (737 mg) was added to the reaction mixture, and the mix...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ccoc1.c1ncnc2cc[nH]c12
HCl
O.CN(C=O)C
null
0.25
CCOC(=O)c1ccc(CCl)o1.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-96d72946e7734e8bb4ca9c2e9dc1bbd9
CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1
ClC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC
Cl[c:18]1[n:17][cH:16][n:15][c:14]2[cH:13][cH:12][n:11]([CH2:10][c:9]3[cH:8][cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[o:37]3)[c:36]21.[NH2:19][c:20]1[cH:21][cH:22][c:23]([O:24][CH2:25][c:26]2[cH:27][cH:28][cH:29][c:30]([F:31])[cH:32]2)[c:33]([Cl:34])[cH:35]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9](...
CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccco5)c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
90.1
[{"value": 90.1, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
2
HOUR
To a solution of ethyl 5-[(4-chloro-5H-pyrrolo[3,2-d]pyrimidin-5-yl)methyl]-2-furoate (200 mg) in 1-methyl-2-pyrrolidone (1.3 mL) was added 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (247 mg), and the mixture was heated to 140° C. and stirred for 2 hrs. The reaction mixture was allowed to cool to room temperature, diluted...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ccoc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
140
2
CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2af15c3b75014d909849c558f42f50fa
CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1>>O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1
Cl.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC.O1CCCC1.[OH-].[Na+]>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)O
CC[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][c:7]([CH2:8][n:9]2[cH:10][cH:11][c:12]3[n:13][cH:14][n:15][c:16]([NH:17][c:18]4[cH:19][cH:20][c:21]([O:22][CH2:23][c:24]5[cH:25][cH:26][cH:27][c:28]([F:29])[cH:30]5)[c:31]([Cl:32])[cH:33]4)[c:34]23)[o:35]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][n:9]2[cH:10][cH:11][c:1...
CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1
O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1
null
null
O.C(C)O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccco5)c34)cc2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
67.2
[{"value": 67.2, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
To a solution of ethyl 5-{[4-({3-chloro-4-[(3-fluorobenzyl)oxy]phenyl}amino)-5H-pyrrolo[3,2-d]pyrimidin-5-yl]methyl}-2-furoate (280 mg) in a mixed solvent of tetrahydrofuran (1.34 mL) and ethanol (1.34 mL) was added 1N aqueous sodium hydroxide solution (1.34 mL) and the mixture was stirred at room temperature for 14 hr...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccoc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
Other
O.C(C)O
null
14
CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1>O.C(C)O>O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-285c49e9ed884122946d87b7b96a5cf7
C[C@@H]1CNC[C@H](C)N1.O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1>>C[C@@H]1CN(C(=O)c2ccc(Cn3ccc4ncnc(Nc5ccc(OCc6cccc(F)c6)c(Cl)c5)c43)cc2)C[C@H](C)N1
Cl.CN(CCCN=C=NCC)C.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)O)C=C2.C[C@@H]1N[C@@H](CNC1)C.N1(N=NC2=C1C=CC=C2)O>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C=C2)C(=O)N2C[C@H](N[C@H](C2)C)C
[CH3:1][C@@H:2]1[CH2:3][NH:4][CH2:40][C@H:41]([CH3:42])[NH:43]1.O[C:5](=[O:6])[c:7]1[cH:8][cH:9][c:10]([CH2:11][n:12]2[cH:13][cH:14][c:15]3[n:16][cH:17][n:18][c:19]([NH:20][c:21]4[cH:22][cH:23][c:24]([O:25][CH2:26][c:27]5[cH:28][cH:29][cH:30][c:31]([F:32])[cH:33]5)[c:34]([Cl:35])[cH:36]4)[c:37]23)[cH:38][cH:39]1>>[CH3:...
C[C@@H]1CNC[C@H](C)N1.O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
C[C@@H]1CN(C(=O)c2ccc(Cn3ccc4ncnc(Nc5ccc(OCc6cccc(F)c6)c(Cl)c5)c43)cc2)C[C@H](C)N1
null
null
O.C(C)N(CC)CC.CN(C=O)C
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
203ddbdbf21b4a3928a7e2e8444b5d8cfa36fbee68b5748d7a1dfab63f3fb59d
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccc5)cc4)c32)cc1)N1CCNCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#7:6]1-[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]-1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[N;H0;D3;+0:9]1-[C:8]-[C:7]-[#7:6]-[C:11]-[C:10]-1)-[c:3](:[c:4]):[c:5]
59.5
[{"value": 59.5, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C=C2)C(=O)N2C[C@H](N[C@H](C2)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
To a solution of 4-{[4-({3-chloro-4-[(3-fluorobenzyl)oxy]phenyl}amino)-5H-pyrrolo[3,2-d]pyrimidin-5-yl]methyl}benzoic acid (120 mg) in N,N-dimethylformamide (2.4 mL) were added cis-2,6-dimethylpiperazine (95 mg) and 1H-1,2,3-benzotriazol-1-ol (65 mg), and the mixture was stirred at room temperature for 15 min. N-[3-(Di...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CNCCN1
C1CNCC[NH]1
C1CNCC[NH]1.c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HO-
O.C(C)N(CC)CC.CN(C=O)C
null
0.25
C[C@@H]1CNC[C@H](C)N1.O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1>O.C(C)N(CC)CC.CN(C=O)C>C[C@@H]1CN(C(=O)c2ccc(Cn3ccc4ncnc(Nc5ccc(OCc6cccc(F)c6)c(Cl)c5)c43)cc2)C[C@H](C)N1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b64d3bebe9a04930bb2f6c508bd9e7b0
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccn2)c(Cl)c1>>Clc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccn1
ClC=1C2=C(N=CN1)C=CN2.ClC=1C=C(N)C=CC1OCC1=NC=CC=C1>>ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2
Cl[c:6]1[n:7][cH:8][n:9][c:10]2[cH:11][cH:12][nH:13][c:14]12.[Cl:1][c:2]1[cH:3][c:4]([NH2:5])[cH:15][cH:16][c:17]1[O:18][CH2:19][c:20]1[cH:21][cH:22][cH:23][cH:24][n:25]1>>[Cl:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[n:7][cH:8][n:9][c:10]3[cH:11][cH:12][nH:13][c:14]23)[cH:15][cH:16][c:17]1[O:18][CH2:19][c:20]1[cH:21][cH:22][cH...
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccn2)c(Cl)c1
Clc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccn1
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)nc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
77.6
[{"value": 77.6, "product": "ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
2
HOUR
To a solution of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (63 mg) in 1-methyl-2-pyrrolidone (0.8 mL), was added 3-chloro-4-(pyridin-2-ylmethoxy)aniline (149 mg), and the mixture was heated to 140° C. and stirred for 2 hrs. The reaction mixture was allowed to cool to room temperature, diluted with 5% aqueous sodium hydrogen...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccncc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
140
2
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccn2)c(Cl)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>Clc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-731fce796aab4a369b82472af434926b
CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1.Nc1ccc(OCc2ccccn2)c(Cl)c1>>CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1
ClC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC.ClC=1C=C(N)C=CC1OCC1=NC=CC=C1>>ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC
Cl[c:18]1[n:17][cH:16][n:15][c:14]2[cH:13][cH:12][n:11]([CH2:10][c:9]3[cH:8][cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[o:36]3)[c:35]21.[NH2:19][c:20]1[cH:21][cH:22][c:23]([O:24][CH2:25][c:26]2[cH:27][cH:28][cH:29][cH:30][n:31]2)[c:32]([Cl:33])[cH:34]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([CH2:10]...
CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1.Nc1ccc(OCc2ccccn2)c(Cl)c1
CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccco5)c34)cc2)nc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
89
[{"value": 89.0, "product": "ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
1.5
HOUR
To a solution of ethyl 5-[(4-chloro-5H-pyrrolo[3,2-d]pyrimidin-5-yl)methyl]-2-furoate (300 mg) in 1-methyl-2-pyrrolidone (2.0 mL) was added 3-chloro-4-(pyridin-2-ylmethoxy)aniline (360 mg), and the mixture was heated to 140° C. and stirred for 1.5 hrs. The reaction mixture was allowed to cool to room temperature, dilut...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ccoc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccncc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
140
1.5
CCOC(=O)c1ccc(Cn2ccc3ncnc(Cl)c32)o1.Nc1ccc(OCc2ccccn2)c(Cl)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-65b6906c23394a31be9fb8b1fbdbef01
CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1>>O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1
Cl.ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)OCC.O1CCCC1.[OH-].[Na+]>>ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)O
CC[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][c:7]([CH2:8][n:9]2[cH:10][cH:11][c:12]3[n:13][cH:14][n:15][c:16]([NH:17][c:18]4[cH:19][cH:20][c:21]([O:22][CH2:23][c:24]5[cH:25][cH:26][cH:27][cH:28][n:29]5)[c:30]([Cl:31])[cH:32]4)[c:33]23)[o:34]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][n:9]2[cH:10][cH:11][c:12]3[n:13...
CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1
O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1
null
null
O.C(C)O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccco5)c34)cc2)nc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#8;a:5]>>[#8;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
74.6
[{"value": 74.6, "product": "ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(O2)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
To a solution of ethyl 5-[(4-{[3-chloro-4-(pyridin-2-ylmethoxy)phenyl]amino}-5H-pyrrolo[3,2-d]pyrimidin-5-yl)methyl]-2-furoate (440 mg) in a mixed solvent of tetrahydrofuran (2.0 mL) and ethanol (2.0 mL) was added 1N aqueous sodium hydroxide solution (2.0 mL), and the mixture was stirred at room temperature for 5 hrs. ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccoc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccncc1
Other
O.C(C)O
null
5
CCOC(=O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1>O.C(C)O>O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5ccccn5)c(Cl)c4)c32)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0593a72cc06840998137ea7460b90b2c
CCOC(=O)c1cc(N)ccc1Oc1cc(Cl)cc(Cl)c1.Clc1ncnc2cc[nH]c12>>CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1
ClC=1C2=C(N=CN1)C=CN2.NC=1C=CC(=C(C(=O)OCC)C1)OC1=CC(=CC(=C1)Cl)Cl>>ClC=1C=C(OC2=C(C(=O)OCC)C=C(C=C2)NC=2C3=C(N=CN2)C=CN3)C=C(C1)Cl
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([NH2:9])[cH:19][cH:20][c:21]1[O:22][c:23]1[cH:24][c:25]([Cl:26])[cH:27][c:28]([Cl:29])[cH:30]1.Cl[c:10]1[n:11][cH:12][n:13][c:14]2[cH:15][cH:16][nH:17][c:18]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([NH:9][c:10]2[n:11][cH:12][n:13][c:14]3[cH:15][cH:16][nH:17...
CCOC(=O)c1cc(N)ccc1Oc1cc(Cl)cc(Cl)c1.Clc1ncnc2cc[nH]c12
CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
84.6
[{"value": 84.6, "product": "ClC=1C=C(OC2=C(C(=O)OCC)C=C(C=C2)NC=2C3=C(N=CN2)C=CN3)C=C(C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
2.5
HOUR
To a solution of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (61 mg) in 1-methyl-2-pyrrolidone (0.8 mL), was added ethyl 5-amino-2-(3,5-dichlorophenoxy)benzoate (186 mg), and the mixture was heated to 140° C. and stirred for 2.5 hrs. The reaction mixture was allowed to cool to room temperature, diluted with 5% aqueous sodium ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
140
2.5
CCOC(=O)c1cc(N)ccc1Oc1cc(Cl)cc(Cl)c1.Clc1ncnc2cc[nH]c12>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-faa4cab3877747e885404fcff18c5d88
CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1>>O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1
Cl.ClC=1C=C(OC2=C(C(=O)OCC)C=C(C=C2)NC=2C3=C(N=CN2)C=CN3)C=C(C1)Cl.O1CCCC1.[OH-].[Na+]>>ClC=1C=C(OC2=C(C(=O)O)C=C(C=C2)NC=2C3=C(N=CN2)C=CN3)C=C(C1)Cl
CC[O:3][C:2](=[O:1])[c:4]1[cH:5][c:6]([NH:7][c:8]2[n:9][cH:10][n:11][c:12]3[cH:13][cH:14][nH:15][c:16]23)[cH:17][cH:18][c:19]1[O:20][c:21]1[cH:22][c:23]([Cl:24])[cH:25][c:26]([Cl:27])[cH:28]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][c:6]([NH:7][c:8]2[n:9][cH:10][n:11][c:12]3[cH:13][cH:14][nH:15][c:16]23)[cH:17][cH:18][c:19]1[O...
CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1
O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1
null
null
O.C(C)O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
81.1
[{"value": 81.1, "product": "ClC=1C=C(OC2=C(C(=O)O)C=C(C=C2)NC=2C3=C(N=CN2)C=CN3)C=C(C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
To a solution of ethyl 2-(3,5-dichlorophenoxy)-5-(5H-pyrrolo[3,2-d]pyrimidin-4-ylamino)benzoate (100 mg) in a mixed solvent of tetrahydrofuran (0.68 mL) and ethanol (0.68 mL) was added 1N aqueous sodium hydroxide solution (0.68 mL), and the mixture was stirred at room temperature for 16 hrs. 1N Hydrochloric acid (0.68 ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
Other
O.C(C)O
null
16
CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1>O.C(C)O>O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1cc(Cl)cc(Cl)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5d84124ecc41478eb68773bd82261c72
CCI.Clc1ncnc2cc[nH]c12>>CCn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[K+].[K+].ICC>>ClC=1C2=C(N=CN1)C=CN2CC
I[CH2:2][CH3:1].[nH:3]1[cH:4][cH:5][c:6]2[n:7][cH:8][n:9][c:10]([Cl:11])[c:12]12>>[CH3:1][CH2:2][n:3]1[cH:4][cH:5][c:6]2[n:7][cH:8][n:9][c:10]([Cl:11])[c:12]12
CCI.Clc1ncnc2cc[nH]c12
CCn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
I-[CH2;D2;+0:1]-[C;D1;H3:2].[Cl;D1;H0:3]-[c:4]1:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]2:[c:9]:[c:10]:[nH;D2;+0:11]:[c:12]:1:2>>[C;D1;H3:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:11]1:[c:10]:[c:9]:[c:8]2:[#7;a:7]:[c:6]:[#7;a:5]:[c:4](-[Cl;D1;H0:3]):[c:12]:2:1
79.1
[{"value": 79.1, "product": "ClC=1C2=C(N=CN1)C=CN2CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (200 mg) in N,N-dimethylformamide (1.3 mL) was added potassium carbonate (269 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. Iodoethane (305 mg) was added to the reaction mixture, and the mixture was stirred at roo...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HI
O.CN(C=O)C
null
null
CCI.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c3865050c042497a812c2daf532247a2
CCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>CCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ClC=1C2=C(N=CN1)C=CN2CC.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC
Cl[c:10]1[n:9][cH:8][n:7][c:6]2[cH:5][cH:4][n:3]([CH2:2][CH3:1])[c:28]21.[NH2:11][c:12]1[cH:13][cH:14][c:15]([O:16][CH2:17][c:18]2[cH:19][cH:20][cH:21][c:22]([F:23])[cH:24]2)[c:25]([Cl:26])[cH:27]1>>[CH3:1][CH2:2][n:3]1[cH:4][cH:5][c:6]2[n:7][cH:8][n:9][c:10]([NH:11][c:12]3[cH:13][cH:14][c:15]([O:16][CH2:17][c:18]4[cH:...
CCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
CCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
52.8
[{"value": 52.8, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 4-chloro-5-ethyl-5H-pyrrolo[3,2-d]pyrimidine (85 mg) in 1-methyl-2-pyrrolidone (0.94 mL) was added 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (177 mg). The title compound (98 mg) was obtained as a pale-purple powder crystals by the reaction in the same manner as in Example 29. Conditions: See reaction.not...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
CN1C(CCC1)=O
null
null
CCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>CN1C(CCC1)=O>CCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e6c84b33f0e041e3a58eb0e0d7f38cd5
CCn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1>>CCn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
ClC=1C2=C(N=CN1)C=CN2CC.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C>>C(C)N1C=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C
Cl[c:10]1[n:9][cH:8][n:7][c:6]2[cH:5][cH:4][n:3]([CH2:2][CH3:1])[c:27]21.[NH2:11][c:12]1[cH:13][cH:14][c:15]([O:16][c:17]2[cH:18][cH:19][c:20]([CH3:21])[n:22][cH:23]2)[c:24]([CH3:25])[cH:26]1>>[CH3:1][CH2:2][n:3]1[cH:4][cH:5][c:6]2[n:7][cH:8][n:9][c:10]([NH:11][c:12]3[cH:13][cH:14][c:15]([O:16][c:17]4[cH:18][cH:19][c:2...
CCn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1
CCn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cncc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
39.8
[{"value": 39.8, "product": "C(C)N1C=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 4-chloro-5-ethyl-5H-pyrrolo[3,2-d]pyrimidine (85 mg) in 1-methyl-2-pyrrolidone (0.94 mL) was added 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (150 mg). The title compound (67 mg) was obtained as white powder crystals by the reaction in the same manner as in Example 29. Conditions: See reaction.notes...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccncc1
HCl
CN1C(CCC1)=O
null
null
CCn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1>CN1C(CCC1)=O>CCn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1f0c06619788479f8a64d0a7472d9305
Clc1ncnc2cc[nH]c12.Nc1cccc(NC(=O)NCc2ccccc2)c1>>O=C(NCc1ccccc1)Nc1cccc(Nc2ncnc3cc[nH]c23)c1
ClC=1C2=C(N=CN1)C=CN2.NC=1C=C(C=CC1)NC(=O)NCC1=CC=CC=C1>>C(C1=CC=CC=C1)NC(=O)NC1=CC(=CC=C1)NC=1C2=C(N=CN1)C=CN2
Cl[c:18]1[n:19][cH:20][n:21][c:22]2[cH:23][cH:24][nH:25][c:26]12.[O:1]=[C:2]([NH:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[NH:11][c:12]1[cH:13][cH:14][cH:15][c:16]([NH2:17])[cH:27]1>>[O:1]=[C:2]([NH:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[NH:11][c:12]1[cH:13][cH:14][cH:15][c:16]([NH:17][c:18]2[n:19][cH:...
Clc1ncnc2cc[nH]c12.Nc1cccc(NC(=O)NCc2ccccc2)c1
O=C(NCc1ccccc1)Nc1cccc(Nc2ncnc3cc[nH]c23)c1
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
O=C(NCc1ccccc1)Nc1cccc(Nc2ncnc3cc[nH]c23)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
41.6
[{"value": 41.6, "product": "C(C1=CC=CC=C1)NC(=O)NC1=CC(=CC=C1)NC=1C2=C(N=CN1)C=CN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
1.5
HOUR
To a solution of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (100 mg) in 1-methyl-2-pyrrolidone (1.3 mL), was added N-(3-aminophenyl)-N′-benzylurea (220 mg), and the mixture was heated to 140° C. and stirred for 1.5 hrs. The reaction mixture was allowed to cool to room temperature, diluted with 5% aqueous sodium hydrogen carb...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ccccc1.c1ncc2[nH]ccc2n1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
140
1.5
Clc1ncnc2cc[nH]c12.Nc1cccc(NC(=O)NCc2ccccc2)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>O=C(NCc1ccccc1)Nc1cccc(Nc2ncnc3cc[nH]c23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7959b1b4975645ba81c5467d367bf55b
NCCO.O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1>>O=C(NCCO)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)O)C=C2.Cl.CN(CCCN=C=NCC)C.ON1C(CCC1=O)=O.NCCO.C(O)([O-])=O.[Na+]>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)NCCO)C=C2
[NH2:3][CH2:4][CH2:5][OH:6].O[C:2](=[O:1])[c:7]1[cH:8][cH:9][c:10]([CH2:11][n:12]2[cH:13][cH:14][c:15]3[n:16][cH:17][n:18][c:19]([NH:20][c:21]4[cH:22][cH:23][c:24]([O:25][CH2:26][c:27]5[cH:28][cH:29][cH:30][c:31]([F:32])[cH:33]5)[c:34]([Cl:35])[cH:36]4)[c:37]23)[cH:38][cH:39]1>>[O:1]=[C:2]([NH:3][CH2:4][CH2:5][OH:6])[c...
NCCO.O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
O=C(NCCO)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
null
null
O.CN(C=O)C
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccccc5)c34)cc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
76.8
[{"value": 76.8, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC2=CC=C(C(=O)NCCO)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a solution of 4-{[4-({3-chloro-4-[(3-fluorobenzyl)oxy]phenyl}amino)-5H-pyrrolo[3,2-d]pyrimidin-5-yl]methyl}benzoic acid (126 mg) in N,N-dimethylformamide (1.2 mL) were added N-[3-(dimethylamino)propyl]-N′-ethylcarbodiimide hydrochloride (72 mg) and 1-hydroxypyrrolidine-2,5-dione (43 mg), and the mixture was stirred ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HO-
O.CN(C=O)C
null
3
NCCO.O=C(O)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1>O.CN(C=O)C>O=C(NCCO)c1ccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eadd9b22a18e4769b5ecf878d7f7f15e
CCOCCBr.Clc1ncnc2cc[nH]c12>>CCOCCn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCCOCC>>ClC=1C2=C(N=CN1)C=CN2CCOCC
Br[CH2:5][CH2:4][O:3][CH2:2][CH3:1].[nH:6]1[cH:7][cH:8][c:9]2[n:10][cH:11][n:12][c:13]([Cl:14])[c:15]12>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][n:6]1[cH:7][cH:8][c:9]2[n:10][cH:11][n:12][c:13]([Cl:14])[c:15]12
CCOCCBr.Clc1ncnc2cc[nH]c12
CCOCCn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
Br-[CH2;D2;+0:1]-[C:2]-[#8:3].[Cl;D1;H0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:1:2>>[#8:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:12]1:[c:11]:[c:10]:[c:9]2:[#7;a:8]:[c:7]:[#7;a:6]:[c:5](-[Cl;D1;H0:4]):[c:13]:2:1
94.9
[{"value": 94.9, "product": "ClC=1C2=C(N=CN1)C=CN2CCOCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (500 mg) in N,N-dimethylformamide (4.5 mL) was added cesium carbonate (1324 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. 1-Bromo-2-ethoxyethane (1016 mg) was added to the reaction mixture, and the mixture was sti...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
CCOCCBr.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CCOCCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5c61120ddc004022a087a9c366708edb
CCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>CCOCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ClC=1C2=C(N=CN1)C=CN2CCOCC.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CCOCC
Cl[c:13]1[n:12][cH:11][n:10][c:9]2[cH:8][cH:7][n:6]([CH2:5][CH2:4][O:3][CH2:2][CH3:1])[c:31]21.[NH2:14][c:15]1[cH:16][cH:17][c:18]([O:19][CH2:20][c:21]2[cH:22][cH:23][cH:24][c:25]([F:26])[cH:27]2)[c:28]([Cl:29])[cH:30]1>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][n:6]1[cH:7][cH:8][c:9]2[n:10][cH:11][n:12][c:13]([NH:14][c:15]3[c...
CCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
CCOCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
51.2
[{"value": 51.2, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CCOCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
7
HOUR
To a solution of 4-chloro-5-(2-ethoxyethyl)-5H-pyrrolo[3,2-d]pyrimidine (90 mg) in 1-methyl-2-pyrrolidone (0.7 mL), 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (151 mg) was added, and the mixture was heated to 140° C. and stirred for 7 hrs. The reaction mixture was allowed to cool to room temperature. The reaction mixture ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
140
7
CCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>CCOCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f589859e47ab4ee292a820807646d4f8
CI.Clc1ncnc2cc[nH]c12>>Cn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[K+].[K+].IC>>ClC=1C2=C(N=CN1)C=CN2C
I[CH3:1].[nH:2]1[cH:3][cH:4][c:5]2[n:6][cH:7][n:8][c:9]([Cl:10])[c:11]12>>[CH3:1][n:2]1[cH:3][cH:4][c:5]2[n:6][cH:7][n:8][c:9]([Cl:10])[c:11]12
CI.Clc1ncnc2cc[nH]c12
Cn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
5bf74b4cd1577c88a528f020d69fbb295924bf4265fb986aea2d18f2c235ec34
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
c1ncc2[nH]ccc2n1
I-[CH3;D1;+0:1].[Cl;D1;H0:2]-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]2:[c:8]:[c:9]:[nH;D2;+0:10]:[c:11]:2:1>>[CH3;D1;+0:1]-[n;H0;D3;+0:10]1:[c:9]:[c:8]:[c:7]2:[#7;a:6]:[c:5]:[#7;a:4]:[c:3](-[Cl;D1;H0:2]):[c:11]:2:1
93.1
[{"value": 93.1, "product": "ClC=1C2=C(N=CN1)C=CN2C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (320 mg) in N,N-dimethylformamide (2.0 mL), was added potassium carbonate (452 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. Iodomethane (444 mg) was added to the reaction mixture, and the mixture was stirred at r...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HI
O.CN(C=O)C
null
null
CI.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>Cn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-dac486025bf4490ea2c870eb0aa30ccd
Cn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>Cn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ClC=1C2=C(N=CN1)C=CN2C.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2C
Cl[c:9]1[n:8][cH:7][n:6][c:5]2[cH:4][cH:3][n:2]([CH3:1])[c:27]21.[NH2:10][c:11]1[cH:12][cH:13][c:14]([O:15][CH2:16][c:17]2[cH:18][cH:19][cH:20][c:21]([F:22])[cH:23]2)[c:24]([Cl:25])[cH:26]1>>[CH3:1][n:2]1[cH:3][cH:4][c:5]2[n:6][cH:7][n:8][c:9]([NH:10][c:11]3[cH:12][cH:13][c:14]([O:15][CH2:16][c:17]4[cH:18][cH:19][cH:20...
Cn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
Cn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C;D1;H3:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C;D1;H3:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
53
[{"value": 53.0, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
1.5
HOUR
To a solution of 4-chloro-5-methyl-5H-pyrrolo[3,2-d]pyrimidine (100 mg) in 1-methyl-2-pyrrolidone (1.0 mL) was added 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (225 mg), and the mixture was heated to 140° C. and stirred for 1.5 hrs. The reaction mixture was allowed to cool to room temperature, diluted with 5% aqueous sodi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
140
1.5
Cn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>Cn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5ee2addd3ec74a60b158f1e5ea3cd0a9
Cc1ccc(Oc2ccc(N)cc2C)cn1.Cn1ccc2ncnc(Cl)c21>>Cc1ccc(Oc2ccc(Nc3ncnc4ccn(C)c34)cc2C)cn1
ClC=1C2=C(N=CN1)C=CN2C.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C>>CN1C=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C
[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH2:11])[cH:22][c:23]2[CH3:24])[cH:25][n:26]1.Cl[c:12]1[n:13][cH:14][n:15][c:16]2[cH:17][cH:18][n:19]([CH3:20])[c:21]12>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n:13][cH:14][n:15][c:16]4[cH:17][cH:18][n:19]([CH3:20])[c:21]...
Cc1ccc(Oc2ccc(N)cc2C)cn1.Cn1ccc2ncnc(Cl)c21
Cc1ccc(Oc2ccc(Nc3ncnc4ccn(C)c34)cc2C)cn1
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cncc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C;D1;H3:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C;D1;H3:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
51.4
[{"value": 51.4, "product": "CN1C=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 4-chloro-5-methyl-5H-pyrrolo[3,2-d]pyrimidine (100 mg) in 1-methyl-2-pyrrolidone (1.0 mL) was added 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (192 mg). The title compound (106 mg) was obtained as white powder crystals by the reaction in the same manner as in Example 39 (ii). Conditions: See reactio...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ccncc1.c1ccccc1.c1ncnc2cc[nH]c12
HCl
CN1C(CCC1)=O
null
null
Cc1ccc(Oc2ccc(N)cc2C)cn1.Cn1ccc2ncnc(Cl)c21>CN1C(CCC1)=O>Cc1ccc(Oc2ccc(Nc3ncnc4ccn(C)c34)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c1b3355afb9a4ae08a2a4286f9f66d3b
CC(C)(C)[Si](C)(C)OCCI.Clc1ncnc2cc[nH]c12>>CC(C)(C)[Si](C)(C)OCCn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].C(C)(C)(C)[Si](C)(C)OCCI>>[Si](C)(C)(C(C)(C)C)OCCN1C=CC=2N=CN=C(C21)Cl
I[CH2:10][CH2:9][O:8][Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7].[nH:11]1[cH:12][cH:13][c:14]2[n:15][cH:16][n:17][c:18]([Cl:19])[c:20]12>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][CH2:9][CH2:10][n:11]1[cH:12][cH:13][c:14]2[n:15][cH:16][n:17][c:18]([Cl:19])[c:20]12
CC(C)(C)[Si](C)(C)OCCI.Clc1ncnc2cc[nH]c12
CC(C)(C)[Si](C)(C)OCCn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
I-[CH2;D2;+0:1]-[C:2]-[#8:3].[Cl;D1;H0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:2:1>>[#8:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:12]1:[c:11]:[c:10]:[c:9]2:[#7;a:8]:[c:7]:[#7;a:6]:[c:5](-[Cl;D1;H0:4]):[c:13]:2:1
94.8
[{"value": 94.8, "product": "[Si](C)(C)(C(C)(C)C)OCCN1C=CC=2N=CN=C(C21)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (307 mg) in N,N-dimethylformamide (2.0 mL) was added cesium carbonate (977 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added tert-butyl(2-iodoethoxy)dimethylsilane (839 mg), and the m...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HI
O.CN(C=O)C
null
null
CC(C)(C)[Si](C)(C)OCCI.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CC(C)(C)[Si](C)(C)OCCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8ab98b28434e43a4b3f45e237b938e87
CC(C)(C)[Si](C)(C)OCCn1ccc2ncnc(Cl)c21>>OCCn1ccc2ncnc(Cl)c21
[Si](C)(C)(C(C)(C)C)OCCN1C=CC=2N=CN=C(C21)Cl.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC>>ClC=1C2=C(N=CN1)C=CN2CCO
CC(C)(C)[Si](C)(C)[O:1][CH2:2][CH2:3][n:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][n:10][c:11]([Cl:12])[c:13]12>>[OH:1][CH2:2][CH2:3][n:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][n:10][c:11]([Cl:12])[c:13]12
CC(C)(C)[Si](C)(C)OCCn1ccc2ncnc(Cl)c21
OCCn1ccc2ncnc(Cl)c21
null
null
O1CCCC1.O
Deprotection
Alcohol deprotection from silyl ethers
6ff8c9c41093ab5237b871dd4689ba6431022d615e227d3774901a983c846e4b
84d9f5b4e7757c58e584c26c7d52c9a3f594fbcb0c0d22f34765a93a932fcd5b
c1ncc2[nH]ccc2n1
C-C(-C)(-C)-[Si](-C)(-C)-[O;H0;D2;+0:1]-[C:2]-[C:3]>>[C:3]-[C:2]-[OH;D1;+0:1]
110.2
[{"value": 110.2, "product": "ClC=1C2=C(N=CN1)C=CN2CCO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
To a solution of 5-(2-{[tert-butyl(dimethyl)silyl]oxy}ethyl)-4-chloro-5H-pyrrolo[3,2-d]pyrimidine (560 mg) in tetrahydrofuran (1.7 mL), was added tetrabutylammonium fluoride (1M tetrahydrofuran solution) (2.69 mL) under ice-cooling, and the mixture was stirred for 4 hrs. The reaction mixture was diluted with water (20 ...
10.6084/m9.figshare.5104873.v1
null
TMS ether protective group
Primary alcohol
null
null
c1ncnc2cc[nH]c12
Other
O1CCCC1.O
null
4
CC(C)(C)[Si](C)(C)OCCn1ccc2ncnc(Cl)c21>O1CCCC1.O>OCCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-71e2d5916b8f49d3be0669749205c538
Nc1ccc(OCc2cccc(F)c2)c(Cl)c1.OCCn1ccc2ncnc(Cl)c21>>OCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
C(C)(=O)OCC.ClC=1C2=C(N=CN1)C=CN2CCO.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CCO
[NH2:12][c:13]1[cH:14][cH:15][c:16]([O:17][CH2:18][c:19]2[cH:20][cH:21][cH:22][c:23]([F:24])[cH:25]2)[c:26]([Cl:27])[cH:28]1.Cl[c:11]1[n:10][cH:9][n:8][c:7]2[cH:6][cH:5][n:4]([CH2:3][CH2:2][OH:1])[c:29]21>>[OH:1][CH2:2][CH2:3][n:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][n:10][c:11]([NH:12][c:13]3[cH:14][cH:15][c:16]([O:17][CH2:...
Nc1ccc(OCc2cccc(F)c2)c(Cl)c1.OCCn1ccc2ncnc(Cl)c21
OCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
75.9
[{"value": 75.9, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CCO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
2
HOUR
To a solution of 2-(4-chloro-5H-pyrrolo[3,2-d]pyrimidin-5-yl)ethanol (130 mg) in 1-methyl-2-pyrrolidone (1.3 mL) was added 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (193 mg), and the reaction mixture was stirred at 120° C. for 2 hrs. The reaction mixture was allowed to cool to room temperature and ethyl acetate (20 mL) w...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
CN1C(CCC1)=O
120
2
Nc1ccc(OCc2cccc(F)c2)c(Cl)c1.OCCn1ccc2ncnc(Cl)c21>CN1C(CCC1)=O>OCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8912d900096a459d8f3ace15cc22d79a
CCCBr.Clc1ncnc2cc[nH]c12>>CCCn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCCC>>ClC=1C2=C(N=CN1)C=CN2CCC
Br[CH2:3][CH2:2][CH3:1].[nH:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][n:10][c:11]([Cl:12])[c:13]12>>[CH3:1][CH2:2][CH2:3][n:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][n:10][c:11]([Cl:12])[c:13]12
CCCBr.Clc1ncnc2cc[nH]c12
CCCn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
Br-[CH2;D2;+0:1]-[C:2]-[C;D1;H3:3].[Cl;D1;H0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:1:2>>[C;D1;H3:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:12]1:[c:11]:[c:10]:[c:9]2:[#7;a:8]:[c:7]:[#7;a:6]:[c:5](-[Cl;D1;H0:4]):[c:13]:2:1
84.2
[{"value": 84.2, "product": "ClC=1C2=C(N=CN1)C=CN2CCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (150 mg) in N,N-dimethylformamide (1.6 mL) was added cesium carbonate (798 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added 1-bromopropane (301 mg), and the mixture was stirred at ro...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
CCCBr.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CCCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ac3c1030d70b4c1380b61eccb5781071
CCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>CCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ClC=1C2=C(N=CN1)C=CN2CCC.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CCC
Cl[c:11]1[n:10][cH:9][n:8][c:7]2[cH:6][cH:5][n:4]([CH2:3][CH2:2][CH3:1])[c:29]21.[NH2:12][c:13]1[cH:14][cH:15][c:16]([O:17][CH2:18][c:19]2[cH:20][cH:21][cH:22][c:23]([F:24])[cH:25]2)[c:26]([Cl:27])[cH:28]1>>[CH3:1][CH2:2][CH2:3][n:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][n:10][c:11]([NH:12][c:13]3[cH:14][cH:15][c:16]([O:17][CH...
CCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
CCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
57.1
[{"value": 57.1, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
2
HOUR
To a solution of 4-chloro-5-propyl-5H-pyrrolo[3,2-d]pyrimidine (80 mg) in 1-methyl-2-pyrrolidone (0.8 mL) was added 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (193 mg), and the reaction mixture was stirred at 120° C. for 2 hrs. The reaction mixture was allowed to cool to room temperature, diluted with 5% aqueous sodium hy...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
120
2
CCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>CCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a35c64370fce46cc9a8074af65db6f3d
CC(C)CBr.Clc1ncnc2cc[nH]c12>>CC(C)Cn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCC(C)C>>ClC=1C2=C(N=CN1)C=CN2CC(C)C
Br[CH2:4][CH:2]([CH3:1])[CH3:3].[nH:5]1[cH:6][cH:7][c:8]2[n:9][cH:10][n:11][c:12]([Cl:13])[c:14]12>>[CH3:1][CH:2]([CH3:3])[CH2:4][n:5]1[cH:6][cH:7][c:8]2[n:9][cH:10][n:11][c:12]([Cl:13])[c:14]12
CC(C)CBr.Clc1ncnc2cc[nH]c12
CC(C)Cn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
Br-[CH2;D2;+0:1]-[C:2](-[C;D1;H3:3])-[C;D1;H3:4].[Cl;D1;H0:5]-[c:6]1:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]2:[c:11]:[c:12]:[nH;D2;+0:13]:[c:14]:1:2>>[C;D1;H3:3]-[C:2](-[C;D1;H3:4])-[CH2;D2;+0:1]-[n;H0;D3;+0:13]1:[c:12]:[c:11]:[c:10]2:[#7;a:9]:[c:8]:[#7;a:7]:[c:6](-[Cl;D1;H0:5]):[c:14]:2:1
102.5
[{"value": 102.5, "product": "ClC=1C2=C(N=CN1)C=CN2CC(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (150 mg) in N,N-dimethylformamide (1.6 mL) was added cesium carbonate (478 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added 1-bromo-2-methylpropane (336 mg), and the mixture was stir...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
CC(C)CBr.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CC(C)Cn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1af6b08c45f54bfca40b81075bc3390d
BrCC1CCCO1.Clc1ncnc2cc[nH]c12>>Clc1ncnc2ccn(CC3CCCO3)c12
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCC1OCCC1>>ClC=1C2=C(N=CN1)C=CN2CC2OCCC2
Br[CH2:10][CH:11]1[CH2:12][CH2:13][CH2:14][O:15]1.[Cl:1][c:2]1[n:3][cH:4][n:5][c:6]2[cH:7][cH:8][nH:9][c:16]12>>[Cl:1][c:2]1[n:3][cH:4][n:5][c:6]2[cH:7][cH:8][n:9]([CH2:10][CH:11]3[CH2:12][CH2:13][CH2:14][O:15]3)[c:16]12
BrCC1CCCO1.Clc1ncnc2cc[nH]c12
Clc1ncnc2ccn(CC3CCCO3)c12
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2c(ccn2CC2CCCO2)n1
Br-[CH2;D2;+0:1]-[C:2](-[C:3])-[#8:4]-[C:5].[Cl;D1;H0:6]-[c:7]1:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]2:[c:12]:[c:13]:[nH;D2;+0:14]:[c:15]:1:2>>[C:3]-[C:2](-[CH2;D2;+0:1]-[n;H0;D3;+0:14]1:[c:13]:[c:12]:[c:11]2:[#7;a:10]:[c:9]:[#7;a:8]:[c:7](-[Cl;D1;H0:6]):[c:15]:2:1)-[#8:4]-[C:5]
86.1
[{"value": 86.1, "product": "ClC=1C2=C(N=CN1)C=CN2CC2OCCC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (150 mg) in N,N-dimethylformamide (1.0 mL) was added cesium carbonate (478 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added 2-(bromomethyl)tetrahydrofuran (242 mg), and the mixture w...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.C1CCOC1
HBr
O.CN(C=O)C
null
null
BrCC1CCCO1.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>Clc1ncnc2ccn(CC3CCCO3)c12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4ee4b6defa4449d0873f4d7e722d8845
COC(=O)c1cccc(CBr)c1.Clc1ncnc2cc[nH]c12>>COC(=O)c1cccc(Cn2ccc3ncnc(Cl)c32)c1
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCC=1C=C(C(=O)OC)C=CC1>>ClC=1C2=C(N=CN1)C=CN2CC=2C=C(C(=O)OC)C=CC2
Br[CH2:10][c:9]1[cH:8][cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:21]1.[nH:11]1[cH:12][cH:13][c:14]2[n:15][cH:16][n:17][c:18]([Cl:19])[c:20]12>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([CH2:10][n:11]2[cH:12][cH:13][c:14]3[n:15][cH:16][n:17][c:18]([Cl:19])[c:20]23)[cH:21]1
COC(=O)c1cccc(CBr)c1.Clc1ncnc2cc[nH]c12
COC(=O)c1cccc(Cn2ccc3ncnc(Cl)c32)c1
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Cn2ccc3ncncc32)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[Cl;D1;H0:5]-[c:6]1:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]2:[c:11]:[c:12]:[nH;D2;+0:13]:[c:14]:2:1>>[Cl;D1;H0:5]-[c:6]1:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]2:[c:11]:[c:12]:[n;H0;D3;+0:13](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]):[c:14]:2:1
54.1
[{"value": 54.1, "product": "ClC=1C2=C(N=CN1)C=CN2CC=2C=C(C(=O)OC)C=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (300 mg) in N,N-dimethylformamide (2.0 mL) was added cesium carbonate (955 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added methyl 3-(bromomethyl)benzoate (671 mg), and the mixture w...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ccccc1.c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
COC(=O)c1cccc(CBr)c1.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>COC(=O)c1cccc(Cn2ccc3ncnc(Cl)c32)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a846403657914eb1b1e28cee4ab548cb
COC(=O)c1cccc(Cn2ccc3ncnc(Cl)c32)c1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>COC(=O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1
ClC=1C2=C(N=CN1)C=CN2CC=2C=C(C(=O)OC)C=CC2.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC=2C=C(C(=O)OC)C=CC2
Cl[c:18]1[n:17][cH:16][n:15][c:14]2[cH:13][cH:12][n:11]([CH2:10][c:9]3[cH:8][cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:37]3)[c:36]21.[NH2:19][c:20]1[cH:21][cH:22][c:23]([O:24][CH2:25][c:26]2[cH:27][cH:28][cH:29][c:30]([F:31])[cH:32]2)[c:33]([Cl:34])[cH:35]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([...
COC(=O)c1cccc(Cn2ccc3ncnc(Cl)c32)c1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
COC(=O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccccc5)c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
89.6
[{"value": 89.6, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC=2C=C(C(=O)OC)C=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
1.5
HOUR
To a solution of methyl 3-[(4-chloro-5H-pyrrolo[3,2-d]pyrimidin-5-yl)methyl]benzoate (670 mg) in 1-methyl-2-pyrrolidone (3.0 mL) was added 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (549 mg), and the reaction mixture was stirred at 120° C. for 1.5 hrs. The reaction mixture was allowed to cool to room temperature, diluted ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
120
1.5
COC(=O)c1cccc(Cn2ccc3ncnc(Cl)c32)c1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>COC(=O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b2285d8165eb40c08165abfd88ccf1b0
COC(=O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1>>O=C(O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1
Cl.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC=2C=C(C(=O)OC)C=CC2.O1CCCC1.[OH-].[Na+]>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC=2C=C(C(=O)O)C=CC2
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][n:10]2[cH:11][cH:12][c:13]3[n:14][cH:15][n:16][c:17]([NH:18][c:19]4[cH:20][cH:21][c:22]([O:23][CH2:24][c:25]5[cH:26][cH:27][cH:28][c:29]([F:30])[cH:31]5)[c:32]([Cl:33])[cH:34]4)[c:35]23)[cH:36]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][n:10]2[cH:...
COC(=O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1
O=C(O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1
null
null
O.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(COc2ccc(Nc3ncnc4ccn(Cc5ccccc5)c34)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
78.4
[{"value": 78.4, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CC=2C=C(C(=O)O)C=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
To a solution of methyl 3-{[4-({3-chloro-4-[(3-fluorobenzyl)oxy]phenyl}amino)-5H-pyrrolo[3,2-d]pyrimidin-5-yl]methyl}benzoate (800 mg) in a mixed solvent of tetrahydrofuran (4.0 mL) and methanol (4.0 mL) was added 1N aqueous sodium hydroxide solution (4.0 mL), and the mixture was stirred at room temperature for 12 hrs....
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
Other
O.CO
null
12
COC(=O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1>O.CO>O=C(O)c1cccc(Cn2ccc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c32)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-af73e68d64c447fda2f1e598bbd4b33d
CCOCCn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1>>CCOCCn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
ClC=1C2=C(N=CN1)C=CN2CCOCC.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C>>C(C)OCCN1C=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C
Cl[c:13]1[n:12][cH:11][n:10][c:9]2[cH:8][cH:7][n:6]([CH2:5][CH2:4][O:3][CH2:2][CH3:1])[c:30]21.[NH2:14][c:15]1[cH:16][cH:17][c:18]([O:19][c:20]2[cH:21][cH:22][c:23]([CH3:24])[n:25][cH:26]2)[c:27]([CH3:28])[cH:29]1>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][n:6]1[cH:7][cH:8][c:9]2[n:10][cH:11][n:12][c:13]([NH:14][c:15]3[cH:16][...
CCOCCn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1
CCOCCn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cncc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
66.8
[{"value": 66.8, "product": "C(C)OCCN1C=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
2
HOUR
To a solution of 4-chloro-5-(2-ethoxyethyl)-5H-pyrrolo[3,2-d]pyrimidine (160 mg) in 1-methyl-2-pyrrolidone (1.4 mL) was added 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (228 mg), and the reaction mixture was stirred at 120° C. for 2 hrs. The reaction mixture was allowed to cool to room temperature, diluted with 5% a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccncc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
120
2
CCOCCn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>CCOCCn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2c549748491a4043be9951f2fb8a73be
CCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2ccccn2)c(Cl)c1>>CCOCCn1ccc2ncnc(Nc3ccc(OCc4ccccn4)c(Cl)c3)c21
ClC=1C2=C(N=CN1)C=CN2CCOCC.ClC=1C=C(N)C=CC1OCC1=NC=CC=C1>>ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2CCOCC
Cl[c:13]1[n:12][cH:11][n:10][c:9]2[cH:8][cH:7][n:6]([CH2:5][CH2:4][O:3][CH2:2][CH3:1])[c:30]21.[NH2:14][c:15]1[cH:16][cH:17][c:18]([O:19][CH2:20][c:21]2[cH:22][cH:23][cH:24][cH:25][n:26]2)[c:27]([Cl:28])[cH:29]1>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][n:6]1[cH:7][cH:8][c:9]2[n:10][cH:11][n:12][c:13]([NH:14][c:15]3[cH:16][cH...
CCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2ccccn2)c(Cl)c1
CCOCCn1ccc2ncnc(Nc3ccc(OCc4ccccn4)c(Cl)c3)c21
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)nc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
53.2
[{"value": 53.2, "product": "ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=CN2CCOCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 4-chloro-5-(2-ethoxyethyl)-5H-pyrrolo[3,2-d]pyrimidine (160 mg) in 1-methyl-2-pyrrolidone (1.4 mL) was added 3-chloro-4-(pyridin-2-ylmethoxy)aniline (250 mg). The title compound (160 mg) was obtained as pale-yellow needle crystals by the reaction in the same manner as in Example 42 (ii). Conditions: Se...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccncc1
HCl
CN1C(CCC1)=O
null
null
CCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2ccccn2)c(Cl)c1>CN1C(CCC1)=O>CCOCCn1ccc2ncnc(Nc3ccc(OCc4ccccn4)c(Cl)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ae288ca3a3cf4c82b267bc4f518883c6
Clc1ncnc2cc[nH]c12.FCCBr>>FCCn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCCF>>ClC=1C2=C(N=CN1)C=CN2CCF
[nH:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][n:10][c:11]([Cl:12])[c:13]12.Br[CH2:3][CH2:2][F:1]>>[F:1][CH2:2][CH2:3][n:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][n:10][c:11]([Cl:12])[c:13]12
Clc1ncnc2cc[nH]c12.FCCBr
FCCn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
Br-[CH2;D2;+0:1]-[C:2]-[F;D1;H0:3].[Cl;D1;H0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:1:2>>[Cl;D1;H0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[n;H0;D3;+0:12](-[CH2;D2;+0:1]-[C:2]-[F;D1;H0:3]):[c:13]:1:2
84.6
[{"value": 84.6, "product": "ClC=1C2=C(N=CN1)C=CN2CCF", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (100 mg) in N,N-dimethylformamide (0.6 mL) was added cesium carbonate (281 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added 1-bromo-2-fluoroethane (124 mg), and the mixture was stirr...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
Clc1ncnc2cc[nH]c12.FCCBr>O.CN(C=O)C>FCCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fb3778ac0e464ea3a0e98d0b215f25a3
CCOC(=O)CBr.Clc1ncnc2cc[nH]c12>>CCOC(=O)Cn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCC(=O)OCC>>ClC=1C2=C(N=CN1)C=CN2CC(=O)OCC
Br[CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].[nH:7]1[cH:8][cH:9][c:10]2[n:11][cH:12][n:13][c:14]([Cl:15])[c:16]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][n:7]1[cH:8][cH:9][c:10]2[n:11][cH:12][n:13][c:14]([Cl:15])[c:16]12
CCOC(=O)CBr.Clc1ncnc2cc[nH]c12
CCOC(=O)Cn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
6c94e785ea287624ec6e807461cf2b4f21051c0d5237d4978c0a9b50260bba0a
6007d70cc3173f3039a472489995dad2781e8d749be1f1aa209b0bf2f190a4b4
c1ncc2[nH]ccc2n1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5].[Cl;D1;H0:6]-[c:7]1:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]2:[c:12]:[c:13]:[nH;D2;+0:14]:[c:15]:2:1>>[C:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[CH2;D2;+0:1]-[n;H0;D3;+0:14]1:[c:13]:[c:12]:[c:11]2:[#7;a:10]:[c:9]:[#7;a:8]:[c:7](-[Cl;D1;H0:6]):[c:15]:2:1
67.3
[{"value": 67.3, "product": "ClC=1C2=C(N=CN1)C=CN2CC(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (200 mg) in N,N-dimethylformamide (1.3 mL) was added cesium carbonate (615 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added ethyl bromoacetate (326 mg), and the mixture was stirred a...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Ester
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
CCOC(=O)CBr.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CCOC(=O)Cn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-385d48fc52af48e984fd4154ad554256
CCOC(=O)Cn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1>>CCOC(=O)Cn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
ClC=1C2=C(N=CN1)C=CN2CC(=O)OCC.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C>>C(C)OC(CN1C=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C)=O
Cl[c:14]1[n:13][cH:12][n:11][c:10]2[cH:9][cH:8][n:7]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:31]21.[NH2:15][c:16]1[cH:17][cH:18][c:19]([O:20][c:21]2[cH:22][cH:23][c:24]([CH3:25])[n:26][cH:27]2)[c:28]([CH3:29])[cH:30]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][n:7]1[cH:8][cH:9][c:10]2[n:11][cH:12][n:13][c:14]([NH:15][...
CCOC(=O)Cn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1
CCOC(=O)Cn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
null
null
C(O)([O-])=O.[Na+].C(C)(C)O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cncc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]-[C:10](-[#8:11])=[O;D1;H0:12]):[c:13]:2:1.[NH2;D1;+0:14]-[c:15](:[c:16]):[c:17]>>[#8:11]-[C:10](=[O;D1;H0:12])-[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:14]-[c:15](:[c:16]):[c:17]):[c:13]:1:2
86.1
[{"value": 86.1, "product": "C(C)OC(CN1C=CC=2N=CN=C(C21)NC2=CC(=C(C=C2)OC=2C=NC(=CC2)C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
110
CELSIUS
2
HOUR
To a solution of ethyl (4-chloro-5H-pyrrolo[3,2-d]pyrimidin-5-yl)acetate (140 mg) in isopropyl alcohol (0.6 mL) was added 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (188 mg), and the mixture was stirred in an oil bath at a temperature of 110° C. for 2 hrs. The reaction mixture was allowed to cool to room temperature...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccncc1
HCl
C(O)([O-])=O.[Na+].C(C)(C)O
110
2
CCOC(=O)Cn1ccc2ncnc(Cl)c21.Cc1ccc(Oc2ccc(N)cc2C)cn1>C(O)([O-])=O.[Na+].C(C)(C)O>CCOC(=O)Cn1ccc2ncnc(Nc3ccc(Oc4ccc(C)nc4)c(C)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ca7b932d10934bc78f79606ec5e7128b
CC(C)(C)[Si](C)(C)OCCCBr.Clc1ncnc2cc[nH]c12>>CC(C)(C)[Si](C)(C)OCCCn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCCCO[Si](C)(C)C(C)(C)C>>[Si](C)(C)(C(C)(C)C)OCCCN1C=CC=2N=CN=C(C21)Cl
Br[CH2:11][CH2:10][CH2:9][O:8][Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7].[nH:12]1[cH:13][cH:14][c:15]2[n:16][cH:17][n:18][c:19]([Cl:20])[c:21]12>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][CH2:9][CH2:10][CH2:11][n:12]1[cH:13][cH:14][c:15]2[n:16][cH:17][n:18][c:19]([Cl:20])[c:21]12
CC(C)(C)[Si](C)(C)OCCCBr.Clc1ncnc2cc[nH]c12
CC(C)(C)[Si](C)(C)OCCCn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[Cl;D1;H0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:2:1>>[C:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:12]1:[c:11]:[c:10]:[c:9]2:[#7;a:8]:[c:7]:[#7;a:6]:[c:5](-[Cl;D1;H0:4]):[c:13]:2:1
74.2
[{"value": 74.2, "product": "[Si](C)(C)(C(C)(C)C)OCCCN1C=CC=2N=CN=C(C21)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (400 mg) in N,N-dimethylformamide (2.6 mL) was added cesium carbonate (957 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added (3-bromopropoxy)(tert-butyl)dimethylsilane (979 mg), and t...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
CC(C)(C)[Si](C)(C)OCCCBr.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CC(C)(C)[Si](C)(C)OCCCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4ccb671408254f98a5fda480c7060e25
Clc1ncnc2cc[nH]c12.FC(F)(F)CCCBr>>FC(F)(F)CCCn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCCCC(F)(F)F>>ClC=1C2=C(N=CN1)C=CN2CCCC(F)(F)F
[nH:8]1[cH:9][cH:10][c:11]2[n:12][cH:13][n:14][c:15]([Cl:16])[c:17]12.Br[CH2:7][CH2:6][CH2:5][C:2]([F:1])([F:3])[F:4]>>[F:1][C:2]([F:3])([F:4])[CH2:5][CH2:6][CH2:7][n:8]1[cH:9][cH:10][c:11]2[n:12][cH:13][n:14][c:15]([Cl:16])[c:17]12
Clc1ncnc2cc[nH]c12.FC(F)(F)CCCBr
FC(F)(F)CCCn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[Cl;D1;H0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:2:1>>[C:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:12]1:[c:11]:[c:10]:[c:9]2:[#7;a:8]:[c:7]:[#7;a:6]:[c:5](-[Cl;D1;H0:4]):[c:13]:2:1
102.5
[{"value": 102.5, "product": "ClC=1C2=C(N=CN1)C=CN2CCCC(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (250 mg) in N,N-dimethylformamide (1.6 mL) was added cesium carbonate (675 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added 4-bromo-1,1,1-trifluorobutane (466 mg), and the mixture wa...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
Clc1ncnc2cc[nH]c12.FC(F)(F)CCCBr>O.CN(C=O)C>FC(F)(F)CCCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-067ac7b4543344aaa869db9cdbbb9194
CCOCCOCCBr.Clc1ncnc2cc[nH]c12>>CCOCCOCCn1ccc2ncnc(Cl)c21
ClC=1C2=C(N=CN1)C=CN2.C([O-])([O-])=O.[Cs+].[Cs+].BrCCOCCOCC>>ClC=1C2=C(N=CN1)C=CN2CCOCCOCC
Br[CH2:8][CH2:7][O:6][CH2:5][CH2:4][O:3][CH2:2][CH3:1].[nH:9]1[cH:10][cH:11][c:12]2[n:13][cH:14][n:15][c:16]([Cl:17])[c:18]12>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][O:6][CH2:7][CH2:8][n:9]1[cH:10][cH:11][c:12]2[n:13][cH:14][n:15][c:16]([Cl:17])[c:18]12
CCOCCOCCBr.Clc1ncnc2cc[nH]c12
CCOCCOCCn1ccc2ncnc(Cl)c21
null
null
O.CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
ecfdd3ebe7f504d096c44af08936ff56b52d45d78f82ef9c3a3c3047f20010b5
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ncc2[nH]ccc2n1
Br-[CH2;D2;+0:1]-[C:2]-[#8:3].[Cl;D1;H0:4]-[c:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:2:1>>[#8:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:12]1:[c:11]:[c:10]:[c:9]2:[#7;a:8]:[c:7]:[#7;a:6]:[c:5](-[Cl;D1;H0:4]):[c:13]:2:1
83.5
[{"value": 83.5, "product": "ClC=1C2=C(N=CN1)C=CN2CCOCCOCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (300 mg) in N,N-dimethylformamide (2.0 mL) was added cesium carbonate (728 mg) under ice-cooling, and the mixture was stirred while warming to room temperature for 15 min. To the reaction mixture was added 1-bromo-2-(2-ethoxyethoxy)ethane (496 mg), and the mixture...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2[nH]ccc2n1
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
HBr
O.CN(C=O)C
null
null
CCOCCOCCBr.Clc1ncnc2cc[nH]c12>O.CN(C=O)C>CCOCCOCCn1ccc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2efab3c64a44496bb732c531c5e493df
CCOCCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>CCOCCOCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ClC=1C2=C(N=CN1)C=CN2CCOCCOCC.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CCOCCOCC
Cl[c:16]1[n:15][cH:14][n:13][c:12]2[cH:11][cH:10][n:9]([CH2:8][CH2:7][O:6][CH2:5][CH2:4][O:3][CH2:2][CH3:1])[c:34]21.[NH2:17][c:18]1[cH:19][cH:20][c:21]([O:22][CH2:23][c:24]2[cH:25][cH:26][cH:27][c:28]([F:29])[cH:30]2)[c:31]([Cl:32])[cH:33]1>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][O:6][CH2:7][CH2:8][n:9]1[cH:10][cH:11][c:12...
CCOCCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
CCOCCOCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
null
null
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
b3e82b6ead9cdf4e2f8cbbcf91109747f4dd1119eb8fb5a3a7a9710387d7d6e5
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
54.1
[{"value": 54.1, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=CN2CCOCCOCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
1
HOUR
To a solution of 4-chloro-5-[2-(2-ethoxyethoxy)ethyl]-5H-pyrrolo[3,2-d]pyrimidine (150 mg) in 1-methyl-2-pyrrolidone (1.1 mL) was added 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (189 mg), and the reaction mixture was stirred at 120° C. for 1 hr. The reaction mixture was allowed to cool to room temperature, diluted with 5...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12
c1ncnc2cc[nH]c12.c1ccccc1.c1ccccc1
HCl
C(O)([O-])=O.[Na+].CN1C(CCC1)=O
120
1
CCOCCOCCn1ccc2ncnc(Cl)c21.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>C(O)([O-])=O.[Na+].CN1C(CCC1)=O>CCOCCOCCn1ccc2ncnc(Nc3ccc(OCc4cccc(F)c4)c(Cl)c3)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3b99d03249c546ccbf009a09b48b2bab
Cc1ccc(Oc2ccc(Nc3ncnc4ccn(CCO)c34)cc2C)cn1>>Cc1ccc(Oc2ccc(N3CCn4ccc5ncnc3c54)cc2C)cn1
CC=1C=C(C=CC1OC=1C=NC(=CC1)C)NC=1C2=C(N=CN1)C=CN2CCO.C(CCC)P(CCCC)CCCC.N(=N\C(=O)N1CCCCC1)/C(=O)N1CCCCC1>>CC=1C=C(C=CC1OC=1C=NC(=CC1)C)N1CCN2C3=C(N=CN=C13)C=C2
O[CH2:12][CH2:13][n:14]1[cH:15][cH:16][c:17]2[n:18][cH:19][n:20][c:21]([NH:11][c:10]3[cH:9][cH:8][c:7]([O:6][c:5]4[cH:4][cH:3][c:2]([CH3:1])[n:27][cH:26]4)[c:24]([CH3:25])[cH:23]3)[c:22]12>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([N:11]3[CH2:12][CH2:13][n:14]4[cH:15][cH:16][c:17]5[n:18][cH:19][n:20...
Cc1ccc(Oc2ccc(Nc3ncnc4ccn(CCO)c34)cc2C)cn1
Cc1ccc(Oc2ccc(N3CCn4ccc5ncnc3c54)cc2C)cn1
null
null
O.C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
83972de9d5aeac1a8f9201b9dcbe455b9704eb65f35518baa50eeca5c47387c2
87693a475e46c41583976158ec46dcaf8be8cc05c5635654a6a68033770f8d5c
c1cncc(Oc2ccc(N3CCn4ccc5ncnc3c54)cc2)c1
O-[CH2;D2;+0:1]-[C:2]-[#7;a:3](:[c:4]):[c:5]1:[c:6]:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:1-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]>>[c:4]:[#7;a:3]1:[c:5]2:[c:6]:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:2-[N;H0;D3;+0:11](-[c:12](:[c:13]):[c:14])-[CH2;D2;+0:1]-[C:2]-1
75.6
[{"value": 75.6, "product": "CC=1C=C(C=CC1OC=1C=NC(=CC1)C)N1CCN2C3=C(N=CN=C13)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a suspension of 2-[4-({3-methyl-4-[(6-methylpyridin-3-yl)oxy]phenyl}amino)-5H-pyrrolo[3,2-d]pyrimidin-5-yl]ethanol (50 mg) and tributylphosphine (54 mg) in toluene (2.5 mL) was added 1,1′-[(E)-diazene-1,2-diyldicarbonyl]dipiperidine (67 mg), and the mixture was stirred at room temperature for 3 hrs. The reaction mix...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Secondary amine
Tertiary amine
null
c1nc2c3c(ccn3CC[NH]2)n1
c1ccncc1.c1ccccc1.c1nc2c3c(ccn3CC[NH]2)n1
HO-
O.C1(=CC=CC=C1)C
null
3
Cc1ccc(Oc2ccc(Nc3ncnc4ccn(CCO)c34)cc2C)cn1>O.C1(=CC=CC=C1)C>Cc1ccc(Oc2ccc(N3CCn4ccc5ncnc3c54)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-39357e8768c7471a8bd07f459e37468c
CCOC(=O)c1cccc(N)c1.Clc1ncnc2cc[nH]c12>>CCOC(=O)c1cccc(Nc2ncnc3cc[nH]c23)c1
ClC=1C2=C(N=CN1)C=CN2.NC=1C=C(C(=O)OCC)C=CC1.CN1C(CCC1)=O.C(O)([O-])=O.[Na+]>>N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)OCC)C=CC2
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([NH2:11])[cH:21]1.Cl[c:12]1[n:13][cH:14][n:15][c:16]2[cH:17][cH:18][nH:19][c:20]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([NH:11][c:12]2[n:13][cH:14][n:15][c:16]3[cH:17][cH:18][nH:19][c:20]23)[cH:21]1
CCOC(=O)c1cccc(N)c1.Clc1ncnc2cc[nH]c12
CCOC(=O)c1cccc(Nc2ncnc3cc[nH]c23)c1
null
null
O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2ncnc3cc[nH]c23)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
55.8
[{"value": 55.8, "product": "N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)OCC)C=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
1.5
HOUR
A mixture of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (2.78 g), ethyl 3-aminobenzoate (4.49 g) and 1-methyl-2-pyrrolidone (20 mL) was stirred at 120° C. for 1.5 hrs. To the reaction mixture were added ethyl acetate, water and saturated aqueous sodium hydrogen carbonate solution. The insoluble material was filtered off, and...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1
HCl
O.C(C)(=O)OCC
120
1.5
CCOC(=O)c1cccc(N)c1.Clc1ncnc2cc[nH]c12>O.C(C)(=O)OCC>CCOC(=O)c1cccc(Nc2ncnc3cc[nH]c23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-240d07a3cd4f4b5f82d57410f500c678
CCOC(=O)c1cccc(Nc2ncnc3cc[nH]c23)c1>>O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1
N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)OCC)C=CC2.[OH-].[Na+].Cl>>N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)O)C=CC2
CC[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][cH:7][c:8]([NH:9][c:10]2[n:11][cH:12][n:13][c:14]3[cH:15][cH:16][nH:17][c:18]23)[cH:19]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][cH:7][c:8]([NH:9][c:10]2[n:11][cH:12][n:13][c:14]3[cH:15][cH:16][nH:17][c:18]23)[cH:19]1
CCOC(=O)c1cccc(Nc2ncnc3cc[nH]c23)c1
O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1
null
null
CO
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(Nc2ncnc3cc[nH]c23)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
102.7
[{"value": 102.7, "product": "N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)O)C=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A mixture of ethyl 3-(5H-pyrrolo[3,2-d]pyrimidin-4-ylamino)benzoate (3.34 g), 1N aqueous sodium hydroxide solution (25 mL) and methanol (50 mL) was stirred overnight at room temperature. To the reaction mixture was added 1N hydrochloric acid (25 mL), and methanol was evaporated under reduced pressure. The precipitated ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ncc2[nH]ccc2n1
Other
CO
null
8
CCOC(=O)c1cccc(Nc2ncnc3cc[nH]c23)c1>CO>O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cfff2fd8eaad455883e09882bfbe82d6
C1CCNCC1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1>>O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCCCC1
ON1N=NC2=C1C=CC=C2.N1CCCCC1.Cl.CN(CCCN=C=NCC)C.N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)O)C=CC2.N1CCCCC1.Cl.CN(CCCN=C=NCC)C>>N1(CCCCC1)C(=O)C=1C=C(C=CC1)NC=1C2=C(N=CN1)C=CN2
[NH:19]1[CH2:20][CH2:21][CH2:22][CH2:23][CH2:24]1.O[C:2](=[O:1])[c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][n:12][c:13]3[cH:14][cH:15][nH:16][c:17]23)[cH:18]1>>[O:1]=[C:2]([c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][n:12][c:13]3[cH:14][cH:15][nH:16][c:17]23)[cH:18]1)[N:19]1[CH2:20][CH2:21][CH2:2...
C1CCNCC1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1
O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCCCC1
null
null
[Cl-].[Na+].O.CN(C=O)C
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]>>[C:6]-[C:7]-[N;H0;D3;+0:8](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:9]-[C:10]
null
[]
null
null
2
HOUR
A mixture of 3-(5H-pyrrolo[3,2-d]pyrimidin-4-ylamino)benzoic acid (153 mg), piperidine (0.078 mL), 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (173 mg) and N,N-dimethylformamide (10 mL) was stirred at room temperature for 2 hrs. Piperidine (0.078 mL) and 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
c1ccccc1.c1ncc2[nH]ccc2n1.C1CC[NH]CC1
HO-
[Cl-].[Na+].O.CN(C=O)C
null
2
C1CCNCC1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1>[Cl-].[Na+].O.CN(C=O)C>O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCCCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-670f85c4b0dd4990b1819bec16530819
C1CSCCN1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1>>O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCSCC1
ON1N=NC2=C1C=CC=C2.N1CCSCC1.Cl.CN(CCCN=C=NCC)C.N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)O)C=CC2.N1CCSCC1.Cl.CN(CCCN=C=NCC)C>>N1(CCSCC1)C(=O)C=1C=C(C=CC1)NC=1C2=C(N=CN1)C=CN2
[NH:19]1[CH2:20][CH2:21][S:22][CH2:23][CH2:24]1.O[C:2](=[O:1])[c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][n:12][c:13]3[cH:14][cH:15][nH:16][c:17]23)[cH:18]1>>[O:1]=[C:2]([c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][n:12][c:13]3[cH:14][cH:15][nH:16][c:17]23)[cH:18]1)[N:19]1[CH2:20][CH2:21][S:22][C...
C1CSCCN1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1
O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCSCC1
null
null
[Cl-].[Na+].O.CN(C=O)C
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
592ef6f3ea027639e6c15db529b85acc14b91923fdff2065727707555f3732c7
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCSCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#16:6]1-[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]-1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[N;H0;D3;+0:9]1-[C:8]-[C:7]-[#16:6]-[C:11]-[C:10]-1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
2
HOUR
A mixture of 3-(5H-pyrrolo[3,2-d]pyrimidin-4-ylamino)benzoic acid (153 mg), thiomorpholine (0.091 mL), 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (173 mg) and N,N-dimethylformamide (10 mL) was stirred at room temperature for 2 hrs. Thiomorpholine (0.030 mL) and 1-[3-(dimethylamino)propyl]-3-ethylcarb...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CSCCN1
C1CSCC[NH]1
c1ccccc1.c1ncc2[nH]ccc2n1.C1CSCC[NH]1
HO-
[Cl-].[Na+].O.CN(C=O)C
null
2
C1CSCCN1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1>[Cl-].[Na+].O.CN(C=O)C>O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCSCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c80f3cb108714be381d6dca24574dc2e
O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1.c1ccc(CC2CCNCC2)cc1>>O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCC(Cc2ccccc2)CC1
N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)O)C=CC2.C(C1=CC=CC=C1)C1CCNCC1.Cl.CN(CCCN=C=NCC)C.ON1N=NC2=C1C=CC=C2>>C(C1=CC=CC=C1)C1CCN(CC1)C(=O)C=1C=C(C=CC1)NC=1C2=C(N=CN1)C=CN2
O[C:2](=[O:1])[c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][n:12][c:13]3[cH:14][cH:15][nH:16][c:17]23)[cH:18]1.[NH:19]1[CH2:20][CH2:21][CH:22]([CH2:23][c:24]2[cH:25][cH:26][cH:27][cH:28][cH:29]2)[CH2:30][CH2:31]1>>[O:1]=[C:2]([c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][n:12][c:13]3[cH:14][cH:15][n...
O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1.c1ccc(CC2CCNCC2)cc1
O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCC(Cc2ccccc2)CC1
null
null
CN(C=O)C
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
fbfce93ec1ece674255bb96c5cec09ad611382b41cf117dfe580015e21744a71
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCC(Cc2ccccc2)CC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]>>[C:6]-[C:7]-[N;H0;D3;+0:8](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:9]-[C:10]
81.2
[{"value": 81.2, "product": "C(C1=CC=CC=C1)C1CCN(CC1)C(=O)C=1C=C(C=CC1)NC=1C2=C(N=CN1)C=CN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A mixture of 3-(5H-pyrrolo[3,2-d]pyrimidin-4-ylamino)benzoic acid (153 mg), 4-benzylpiperidine (158 mg), 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (173 mg), 1-hydroxybenzotriazole (138 mg) and N,N-dimethylformamide (10 mL) was stirred at room temperature for 3 hrs. The reaction mixture was concentra...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNCC1
C1CC[NH]CC1
c1ccccc1.c1ncc2[nH]ccc2n1.C1CC[NH]CC1.c1ccccc1
HO-
CN(C=O)C
null
3
O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1.c1ccc(CC2CCNCC2)cc1>CN(C=O)C>O=C(c1cccc(Nc2ncnc3cc[nH]c23)c1)N1CCC(Cc2ccccc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-daf51b578f654598b965018c5face7ff
NCc1ccccc1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1>>O=C(NCc1ccccc1)c1cccc(Nc2ncnc3cc[nH]c23)c1
N1=CN=C(C2=C1C=CN2)NC=2C=C(C(=O)O)C=CC2.C(C1=CC=CC=C1)N.Cl.CN(CCCN=C=NCC)C.ON1N=NC2=C1C=CC=C2>>C(C1=CC=CC=C1)NC(C1=CC(=CC=C1)NC=1C2=C(N=CN1)C=CN2)=O
[NH2:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1.O[C:2](=[O:1])[c:11]1[cH:12][cH:13][cH:14][c:15]([NH:16][c:17]2[n:18][cH:19][n:20][c:21]3[cH:22][cH:23][nH:24][c:25]23)[cH:26]1>>[O:1]=[C:2]([NH:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][cH:14][c:15]([NH:16][c:17]2[n:18][cH:19][n:20][c:21]...
NCc1ccccc1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1
O=C(NCc1ccccc1)c1cccc(Nc2ncnc3cc[nH]c23)c1
null
null
CN(C=O)C
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCc1ccccc1)c1cccc(Nc2ncnc3cc[nH]c23)c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[C:7]-[c:8]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[C:7]-[c:8])-[c:3](:[c:4]):[c:5]
61.9
[{"value": 61.9, "product": "C(C1=CC=CC=C1)NC(C1=CC(=CC=C1)NC=1C2=C(N=CN1)C=CN2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
DAY
A mixture of 3-(5H-pyrrolo[3,2-d]pyrimidin-4-ylamino)benzoic acid (153 mg), benzylamine (96 mg), 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (173 mg), 1-hydroxybenzotriazole (138 mg) and N,N-dimethylformamide (10 mL) was stirred at room temperature for 3 days. The reaction mixture was concentrated und...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ncc2[nH]ccc2n1
HO-
CN(C=O)C
null
72
NCc1ccccc1.O=C(O)c1cccc(Nc2ncnc3cc[nH]c23)c1>CN(C=O)C>O=C(NCc1ccccc1)c1cccc(Nc2ncnc3cc[nH]c23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fad64d0f1a4e45a4b69194a647c21ad6
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccc2)c(CO)c1>>OCc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
ClC=1C2=C(N=CN1)C=CN2.NC=1C=CC(=C(C1)CO)OCC1=CC=CC=C1>>C(C1=CC=CC=C1)OC1=C(C=C(C=C1)NC=1C2=C(N=CN1)C=CN2)CO
Cl[c:7]1[n:8][cH:9][n:10][c:11]2[cH:12][cH:13][nH:14][c:15]12.[OH:1][CH2:2][c:3]1[cH:4][c:5]([NH2:6])[cH:16][cH:17][c:18]1[O:19][CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1>>[OH:1][CH2:2][c:3]1[cH:4][c:5]([NH:6][c:7]2[n:8][cH:9][n:10][c:11]3[cH:12][cH:13][nH:14][c:15]23)[cH:16][cH:17][c:18]1[O:19][CH2:20][c:21]1...
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccc2)c(CO)c1
OCc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
40.3
[{"value": 40.3, "product": "C(C1=CC=CC=C1)OC1=C(C=C(C=C1)NC=1C2=C(N=CN1)C=CN2)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
4
HOUR
A mixture of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (307 mg), [5-amino-2-(benzyloxy)phenyl]methanol (459 mg) and N,N-dimethylformamide (10 mL) was stirred at 80° C. for 4 hrs. The reaction mixture was concentrated under reduced pressure, aqueous sodium hydrogen carbonate solution was added and the mixture was extracted w...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
HCl
CN(C=O)C
80
4
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccc2)c(CO)c1>CN(C=O)C>OCc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bc3f968d5e284d2d81428d6a5969d4f0
COc1cc(N)ccc1OCc1ccccc1.Clc1ncnc2cc[nH]c12>>COc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
ClC=1C2=C(N=CN1)C=CN2.C(C1=CC=CC=C1)OC1=C(C=C(N)C=C1)OC.CN1C(CCC1)=O>>C(C1=CC=CC=C1)OC1=C(C=C(C=C1)NC=1C2=C(N=CN1)C=CN2)OC
[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[cH:16][cH:17][c:18]1[O:19][CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1.Cl[c:7]1[n:8][cH:9][n:10][c:11]2[cH:12][cH:13][nH:14][c:15]12>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH:6][c:7]2[n:8][cH:9][n:10][c:11]3[cH:12][cH:13][nH:14][c:15]23)[cH:16][cH:17][c:18]1[O:19][CH2:20][c:21]1[c...
COc1cc(N)ccc1OCc1ccccc1.Clc1ncnc2cc[nH]c12
COc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
null
null
CO
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
59.7
[{"value": 59.7, "product": "C(C1=CC=CC=C1)OC1=C(C=C(C=C1)NC=1C2=C(N=CN1)C=CN2)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
4
HOUR
A mixture of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (200 mg), 4-(benzyloxy)-3-methoxyaniline (298 mg) and 1-methyl-2-pyrrolidone (5 mL) was stirred at 80° C. for 4 hrs. Methanol and activated carbon were added to the reaction mixture and the mixture was stirred. The activated carbon was filtered off, aqueous sodium hydro...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
HCl
CO
80
4
COc1cc(N)ccc1OCc1ccccc1.Clc1ncnc2cc[nH]c12>CO>COc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-69cd76e25f794ae5ae52dfdfac3d9ec8
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccc2)c(Cl)c1>>Clc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
ClC=1C2=C(N=CN1)C=CN2.C(C1=CC=CC=C1)OC1=C(C=C(N)C=C1)Cl.CN1C(CCC1)=O>>C(C1=CC=CC=C1)OC1=C(C=C(C=C1)NC=1C2=C(N=CN1)C=CN2)Cl
Cl[c:6]1[n:7][cH:8][n:9][c:10]2[cH:11][cH:12][nH:13][c:14]12.[Cl:1][c:2]1[cH:3][c:4]([NH2:5])[cH:15][cH:16][c:17]1[O:18][CH2:19][c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1>>[Cl:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[n:7][cH:8][n:9][c:10]3[cH:11][cH:12][nH:13][c:14]23)[cH:15][cH:16][c:17]1[O:18][CH2:19][c:20]1[cH:21][cH:22][c...
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccc2)c(Cl)c1
Clc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
null
null
CO
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
49.5
[{"value": 49.5, "product": "C(C1=CC=CC=C1)OC1=C(C=C(C=C1)NC=1C2=C(N=CN1)C=CN2)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
4
HOUR
A mixture of 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (200 mg), 4-(benzyloxy)-3-chloroaniline (365 mg) and 1-methyl-2-pyrrolidone (3 mL) was stirred at 80° C. for 4 hrs. Methanol and activated carbon were added to the reaction mixture and the mixture was stirred. The activated carbon was filtered off, aqueous sodium hydrog...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
HCl
CO
80
4
Clc1ncnc2cc[nH]c12.Nc1ccc(OCc2ccccc2)c(Cl)c1>CO>Clc1cc(Nc2ncnc3cc[nH]c23)ccc1OCc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fdd7838e037f4837b5b2452a5e403701
CCO.CCc1nc(Cl)c2[nH]ccc2n1.Nc1ccc(Oc2ccccc2)c(C(=O)[O-])c1>>CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
C(C)C=1N=C(C2=C(N1)C=CN2)Cl.NC=1C=CC(=C(C(=O)[O-])C1)OC1=CC=CC=C1.CN1C(CCC1)=O.C(C)O>>O(C1=CC=CC=C1)C1=C(C(=O)OCC)C=C(C=C1)NC=1C2=C(N=CN1)C=CN2
O[CH2:2][CH3:1].CC[c:12]1[n:11][c:10](Cl)[c:18]2[c:14]([n:13]1)[cH:15][cH:16][nH:17]2.[O-:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([NH2:9])[cH:19][cH:20][c:21]1[O:22][c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([NH:9][c:10]2[n:11][cH:12][n:13][c:14]3[cH:15][cH:16][nH:17][c:18]2...
CCO.CCc1nc(Cl)c2[nH]ccc2n1.Nc1ccc(Oc2ccccc2)c(C(=O)[O-])c1
CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
b5bc02a189a8a2933e820f699bd5b360f72326a156ac3a6d1bded089e3b5c856
e2f3e76b9378ab2fa98631319547fb730cc7f03b13d2ec9dd6ca62bd7cba28be
c1ccc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
C-C-[c;H0;D3;+0:1]1:[#7;a:2]:[c;H0;D3;+0:3](-Cl):[c:4]2:[#7;a:5]:[c:6]:[c:7]:[c:8]:2:[#7;a:9]:1.O-[CH2;D2;+0:10]-[C;D1;H3:11].[NH2;D1;+0:12]-[c:13](:[c:14]):[c:15]:[c:16]-[C:17](-[O-;H0;D1:18])=[O;D1;H0:19]>>[C;D1;H3:11]-[CH2;D2;+0:10]-[O;H0;D2;+0:18]-[C:17](=[O;D1;H0:19])-[c:16]:[c:15]:[c:13](-[NH;D2;+0:12]-[c;H0;D3;+...
null
[]
80
CELSIUS
2
HOUR
A mixture of ethyl 4-chloro-5H-pyrrolo[3,2-d]pyrimidine (461 mg), 5-amino-2-phenoxybenzoate (926 mg) and 1-methyl-2-pyrrolidone (5 mL) was stirred at 80° C. for 2 hrs. Ethanol, water and activated carbon were added to the reaction mixture and the mixture was stirred. The activated carbon was filtered off, and the solve...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary alcohol.Primary amine
Ester.Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
HCl
O
80
2
CCO.CCc1nc(Cl)c2[nH]ccc2n1.Nc1ccc(Oc2ccccc2)c(C(=O)[O-])c1>O>CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f8b70c4375f04973a2417d592922d457
CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1>>O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
O(C1=CC=CC=C1)C1=C(C(=O)OCC)C=C(C=C1)NC=1C2=C(N=CN1)C=CN2.[OH-].[Na+].Cl>>O(C1=CC=CC=C1)C1=C(C(=O)O)C=C(C=C1)NC=1C2=C(N=CN1)C=CN2
CC[O:3][C:2](=[O:1])[c:4]1[cH:5][c:6]([NH:7][c:8]2[n:9][cH:10][n:11][c:12]3[cH:13][cH:14][nH:15][c:16]23)[cH:17][cH:18][c:19]1[O:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][c:6]([NH:7][c:8]2[n:9][cH:10][n:11][c:12]3[cH:13][cH:14][nH:15][c:16]23)[cH:17][cH:18][c:19]1[O:20][c:21]1[cH:2...
CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
null
null
CO
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
92.3
[{"value": 92.3, "product": "O(C1=CC=CC=C1)C1=C(C(=O)O)C=C(C=C1)NC=1C2=C(N=CN1)C=CN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
1.5
HOUR
A mixture of ethyl 2-phenoxy-5-(5H-pyrrolo[3,2-d]pyrimidin-4-ylamino)benzoate (899 mg), 1N aqueous sodium hydroxide solution (5 mL) and methanol (15 mL) was stirred at 60° C. for 1.5 hrs. To the reaction mixture was added 1N hydrochloric acid (5 mL), and methanol was evaporated under reduced pressure. The precipitated ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
Other
CO
60
1.5
CCOC(=O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1>CO>O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6e377384a0c74bea8556a6adfb81f9a4
O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1>>OCc1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
CO.[BH4-].[Na+].O(C1=CC=CC=C1)C1=C(C(=O)O)C=C(C=C1)NC=1C2=C(N=CN1)C=CN2.C(=O)(N1C=NC=C1)N1C=NC=C1>>O(C1=CC=CC=C1)C1=C(C=C(C=C1)NC=1C2=C(N=CN1)C=CN2)CO
O[C:2](=[O:1])[c:3]1[cH:4][c:5]([NH:6][c:7]2[n:8][cH:9][n:10][c:11]3[cH:12][cH:13][nH:14][c:15]23)[cH:16][cH:17][c:18]1[O:19][c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1>>[OH:1][CH2:2][c:3]1[cH:4][c:5]([NH:6][c:7]2[n:8][cH:9][n:10][c:11]3[cH:12][cH:13][nH:14][c:15]23)[cH:16][cH:17][c:18]1[O:19][c:20]1[cH:21][cH:22][cH:2...
O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
OCc1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
null
null
O.CN(C=O)C
Reduction
Reduction of carboxylic acid to primary alcohol
0db83a5ebe1e318b78b55461cf7eb8f7c004eef0f9e3b6666d3df4c96b5f665e
93b4621647b04d2ad2f2825215b1567f171ba61fe10d136b5db6ea0470aa4932
c1ccc(Oc2ccc(Nc3ncnc4cc[nH]c34)cc2)cc1
O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
26.5
[{"value": 26.5, "product": "O(C1=CC=CC=C1)C1=C(C=C(C=C1)NC=1C2=C(N=CN1)C=CN2)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 2-phenoxy-5-(5H-pyrrolo[3,2-d]pyrimidin-4-ylamino)benzoic acid (173 mg) in N,N-dimethylformamide (5 mL) was added 1,1′-carbonyldiimidazole (97 mg) and the mixture was stirred at room temperature for 1 hr. Sodium borohydride (38 mg) was added to the reaction mixture at room temperature, and methanol (1 ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary alcohol
null
null
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
Other
O.CN(C=O)C
null
1
O=C(O)c1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1>O.CN(C=O)C>OCc1cc(Nc2ncnc3cc[nH]c23)ccc1Oc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b8cb0c29e4c24630a8584314d898a303
Cc1ccc(S(=O)(=O)Cl)cc1.N#CCC(=O)c1ccco1>>Cc1ccc(S(=O)(=O)OC(=CC#N)c2ccco2)cc1
O1C(=CC=C1)C(CC#N)=O.C1(=CC=C(C=C1)S(=O)(=O)Cl)C.C(C)N(CC)CC>>CC1=CC=C(C=C1)S(=O)(=O)OC(=CC#N)C=1OC=CC1
Cl[S:6]([c:5]1[cH:4][cH:3][c:2]([CH3:1])[cH:20][cH:19]1)(=[O:7])=[O:8].[O:9]=[C:10]([CH2:11][C:12]#[N:13])[c:14]1[cH:15][cH:16][cH:17][o:18]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[O:9][C:10](=[CH:11][C:12]#[N:13])[c:14]2[cH:15][cH:16][cH:17][o:18]2)[cH:19][cH:20]1
Cc1ccc(S(=O)(=O)Cl)cc1.N#CCC(=O)c1ccco1
Cc1ccc(S(=O)(=O)OC(=CC#N)c2ccco2)cc1
null
null
ClCCl
Acylation
OtherReaction
9f8c97f001bd09a5896e1620aa92ed222c76fd261d4582b923c7f486d025fb40
ad2bf1a301061ff4de8cacf445aa6c9f6615e0daaa746ef88ba96d39fc5112df
[CH]=C(OS(=O)(=O)c1ccccc1)c1ccco1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[N;D1;H0:7]#[C:8]-[CH2;D2;+0:9]-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[c:12](:[c:13]):[#8;a:14]:[c:15]>>[N;D1;H0:7]#[C:8]-[CH;D2;+0:9]=[C;H0;D3;+0:10](-[O;H0;D2;+0:11]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[c:12](:[c:13]):[#8;a:14]:...
92.5
[{"value": 92.5, "product": "CC1=CC=C(C=C1)S(=O)(=O)OC(=CC#N)C=1OC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a mixture of 3-(2-furyl)-3-oxopropanenitrile (5.29 g), p-toluenesulfonyl chloride (9.00 g) and dichloromethane (60 mL) was added dropwise triethylamine (5.99 g) under ice-cooling. After stirring under ice-cooling for 1.5 hrs, the mixture was diluted with dichloromethane (100 mL). The mixture washed with water (150 m...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Ketone.Sulfonyl halide
Tosylate
null
null
c1ccccc1.c1ccoc1
HCl
ClCCl
null
null
Cc1ccc(S(=O)(=O)Cl)cc1.N#CCC(=O)c1ccco1>ClCCl>Cc1ccc(S(=O)(=O)OC(=CC#N)c2ccco2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-62e715fe296147099d7127fe67836a60
CCOC(=O)C(N)C(=O)OCC.Cc1ccc(S(=O)(=O)OC(=CC#N)c2ccco2)cc1>>CCOC(=O)c1[nH]c(-c2ccco2)cc1N
CC1=CC=C(C=C1)S(=O)(=O)OC(=CC#N)C=1OC=CC1.Cl.NC(C(=O)OCC)C(=O)OCC.[O-]CC.[Na+].Cl>>NC1=C(NC(=C1)C=1OC=CC1)C(=O)OCC
CCOC(=O)[CH:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[NH2:7].Cc1ccc(S(=O)(=O)O[C:8]([c:9]2[cH:10][cH:11][cH:12][o:13]2)=[CH:14][C:15]#[N:16])cc1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[nH:7][c:8](-[c:9]2[cH:10][cH:11][cH:12][o:13]2)[cH:14][c:15]1[NH2:16]
CCOC(=O)C(N)C(=O)OCC.Cc1ccc(S(=O)(=O)OC(=CC#N)c2ccco2)cc1
CCOC(=O)c1[nH]c(-c2ccco2)cc1N
null
null
O1CCCC1.C(C)O
Functional Group Interconversion
OtherReaction
d25017a4cc1663869a2ad8f70e12ba7e816f6e3bcd1c9ef62cf784d611fc306c
2761e1a6469897982b9f37673b7247d314aab4379d45b535816ae836a29bb8eb
c1c[nH]c(-c2ccco2)c1
C-C-O-C(=O)-[CH;D3;+0:1](-[NH2;D1;+0:2])-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6].C-c1:c:c:c(-S(=O)(=O)-O-[C;H0;D3;+0:7](=[CH;D2;+0:8]-[C;H0;D2;+0:9]#[N;H0;D1;+0:10])-[c;H0;D3;+0:11]2:[#8;a:12]:[c:13]:[c:14]:[c:15]:2):c:c:1>>[C:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[c;H0;D3;+0:1]1:[nH;D2;+0:2]:[c;H0;D3;+0:7](-[c;H0;D3;+0:11]2:[#8;a:12...
33.3
[{"value": 33.3, "product": "NC1=C(NC(=C1)C=1OC=CC1)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
To a solution of 2-cyano-1-(2-furyl)vinyl 4-methylbenzenesulfonate (10.48 g) and diethyl aminomalonate hydrochloride (7.67 g) in a mixed solvent of ethanol (120 mL)-tetrahydrofuran (64 mL) was added dropwise a solution (36.9 mL) of 20% sodium ethoxide in ethanol under ice-cooling. After stirring at room temperature for...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Ester.Ester.Nitrile.Primary amine
Ester.Primary amine
c1ccccc1
c1cc[nH]c1
c1cc[nH]c1.c1ccoc1
TsOH.HO-
O1CCCC1.C(C)O
null
12
CCOC(=O)C(N)C(=O)OCC.Cc1ccc(S(=O)(=O)OC(=CC#N)c2ccco2)cc1>O1CCCC1.C(C)O>CCOC(=O)c1[nH]c(-c2ccco2)cc1N
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-95a54f43fb5e4d08b1d87ebe133e79b5
CCOC(=O)c1[nH]c(-c2ccco2)cc1N.N=CN>>O=c1[nH]cnc2cc(-c3ccco3)[nH]c12
NC1=C(NC(=C1)C=1OC=CC1)C(=O)OCC.C(C)(=O)O.C(=N)N>>O1C(=CC=C1)C1=CC=2N=CNC(C2N1)=O
CCO[C:2](=[O:1])[c:15]1[c:6]([NH2:5])[cH:7][c:8](-[c:9]2[cH:10][cH:11][cH:12][o:13]2)[nH:14]1.N[CH:4]=[NH:3]>>[O:1]=[c:2]1[nH:3][cH:4][n:5][c:6]2[cH:7][c:8](-[c:9]3[cH:10][cH:11][cH:12][o:13]3)[nH:14][c:15]12
CCOC(=O)c1[nH]c(-c2ccco2)cc1N.N=CN
O=c1[nH]cnc2cc(-c3ccco3)[nH]c12
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
cf2d93c547f6b79e1ff78c4c95ac2a9882be6c07ff6c3d38d4ab70f7d93654ab
36efa24579e0043fdba8918e78f1d75cb4504837c08d344d01203f5fa64bfaef
O=c1[nH]cnc2cc(-c3ccco3)[nH]c12
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[NH2;D1;+0:8].N-[CH;D2;+0:9]=[NH;D1;+0:10]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[nH;D2;+0:10]:[cH;D2;+0:9]:[n;H0;D2;+0:8]:[c:7]2:[c:6]:[c:5]:[#7;a:4]:[c:3]:2:1
95.9
[{"value": 95.9, "product": "O1C(=CC=C1)C1=CC=2N=CNC(C2N1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of ethyl 3-amino-5-(2-furyl)-1H-pyrrole-2-carboxylate (2.58 g) in ethanol (35 mL) was added formamidine acetate (1.83 g), and the mixture was heated under reflux for 18 hrs. After cooling to room temperature, the precipitated solid was collected by filtration, washed with ethanol, and dried under reduced ...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine.Primary amine
null
c1cc[nH]c1
c1cc2ncncc2[nH]1
c1cc2ncncc2[nH]1.c1ccoc1
HO-
C(C)O
null
null
CCOC(=O)c1[nH]c(-c2ccco2)cc1N.N=CN>C(C)O>O=c1[nH]cnc2cc(-c3ccco3)[nH]c12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-60364eed59cf42df9902b300bf8ffe2b
O=P(Cl)(Cl)Cl.O=c1[nH]cnc2cc(-c3ccco3)[nH]c12>>Clc1ncnc2cc(-c3ccco3)[nH]c12
O1C(=CC=C1)C1=CC=2N=CNC(C2N1)=O.P(=O)(Cl)(Cl)Cl>>ClC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2
O=P(Cl)(Cl)[Cl:1].O=[c:2]1[nH:3][cH:4][n:5][c:6]2[cH:7][c:8](-[c:9]3[cH:10][cH:11][cH:12][o:13]3)[nH:14][c:15]12>>[Cl:1][c:2]1[n:3][cH:4][n:5][c:6]2[cH:7][c:8](-[c:9]3[cH:10][cH:11][cH:12][o:13]3)[nH:14][c:15]12
O=P(Cl)(Cl)Cl.O=c1[nH]cnc2cc(-c3ccco3)[nH]c12
Clc1ncnc2cc(-c3ccco3)[nH]c12
null
null
O1CCOCC1
Functional Group Interconversion
OtherReaction
990997bc80649f34ced0b0b8c9ec1b3d7f7bb4583bf26285f81a6c467d40b7b8
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1coc(-c2cc3ncncc3[nH]2)c1
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4]:[#7;a:5]:[c:6]2:[c:7]:[c:8]:[#7;a:9]:[c:10]:2:1>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4]:[#7;a:5]:[c:6]2:[c:7]:[c:8]:[#7;a:9]:[c:10]:2:1
91.2
[{"value": 91.2, "product": "ClC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
20
MINUTE
A mixture of 6-(2-furyl)-4,5-dihydro-3H-pyrrolo[3,2-d]pyrimidin-4-one (2.20 g) and phosphoryl chloride (10.7 g) was stirred at 100° C. for 20 min, dioxane (30 mL) was added, and the mixture was stirred at 100° C. for 3 hrs. After concentration under reduced pressure, saturated aqueous sodium hydrogen carbonate was adde...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1cc2ncncc2[nH]1
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1.c1ccoc1
HCl
O1CCOCC1
100
0.333333
O=P(Cl)(Cl)Cl.O=c1[nH]cnc2cc(-c3ccco3)[nH]c12>O1CCOCC1>Clc1ncnc2cc(-c3ccco3)[nH]c12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-12d14ab5c17b4725aa3770f42c1b9592
Cc1ccc(Oc2ccc(N)cc2C)cn1.Clc1ncnc2cc(-c3ccco3)[nH]c12>>Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2C)cn1
C(O)([O-])=O.[Na+].ClC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C.CN1C(CCC1)=O>>O1C(=CC=C1)C1=CC=2N=CN=C(C2N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C
[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH2:11])[cH:26][c:27]2[CH3:28])[cH:29][n:30]1.Cl[c:12]1[n:13][cH:14][n:15][c:16]2[cH:17][c:18](-[c:19]3[cH:20][cH:21][cH:22][o:23]3)[nH:24][c:25]12>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n:13][cH:14][n:15][c:16]4[cH:17][...
Cc1ccc(Oc2ccc(N)cc2C)cn1.Clc1ncnc2cc(-c3ccco3)[nH]c12
Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2C)cn1
null
null
O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cncc(Oc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
57.3
[{"value": 57.3, "product": "O1C(=CC=C1)C1=CC=2N=CN=C(C2N1)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
2
HOUR
A mixture of 4-chloro-6-(2-furyl)-5H-pyrrolo[3,2-d]pyrimidine (110 mg), 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (161 mg) and 1-methyl-2-pyrrolidinone (2.5 mL) was stirred at 140° C. for 2 hrs, poured into water (10 mL) and adjusted to pH 8 with saturated aqueous sodium hydrogen carbonate. The mixture was extracte...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccncc1.c1ccccc1.c1ncc2[nH]ccc2n1.c1ccoc1
HCl
O
140
2
Cc1ccc(Oc2ccc(N)cc2C)cn1.Clc1ncnc2cc(-c3ccco3)[nH]c12>O>Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7cc40eed89874974a268b62f889db214
Clc1ncnc2cc(-c3ccco3)[nH]c12.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>Fc1cccc(COc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2Cl)c1
C(O)([O-])=O.[Na+].ClC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F.CN1C(CCC1)=O>>ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2
Cl[c:14]1[n:15][cH:16][n:17][c:18]2[cH:19][c:20](-[c:21]3[cH:22][cH:23][cH:24][o:25]3)[nH:26][c:27]12.[F:1][c:2]1[cH:3][cH:4][cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][cH:11][c:12]([NH2:13])[cH:28][c:29]2[Cl:30])[cH:31]1>>[F:1][c:2]1[cH:3][cH:4][cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][cH:11][c:12]([NH:13][c:14]3[n:15][cH:16][n...
Clc1ncnc2cc(-c3ccco3)[nH]c12.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
Fc1cccc(COc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2Cl)c1
null
null
O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
56
[{"value": 56.0, "product": "ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
2
HOUR
A mixture of 4-chloro-6-(2-furyl)-5H-pyrrolo[3,2-d]pyrimidine (110 mg), 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (189 mg) and 1-methyl-2-pyrrolidinone (2.5 mL) was stirred at 140° C. for 2 hrs, poured into water (10 mL) and adjusted to pH 8 with saturated aqueous sodium hydrogen carbonate. The mixture was extracted with...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ccccc1.c1ncc2[nH]ccc2n1.c1ccoc1
HCl
O
140
2
Clc1ncnc2cc(-c3ccco3)[nH]c12.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>O>Fc1cccc(COc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2Cl)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-10af4feedcf24e3ba6816513f7f67db0
Clc1ncnc2cc(-c3ccco3)[nH]c12.Nc1ccc(OCc2ccccn2)c(Cl)c1>>Clc1cc(Nc2ncnc3cc(-c4ccco4)[nH]c23)ccc1OCc1ccccn1
C(O)([O-])=O.[Na+].ClC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2.ClC=1C=C(N)C=CC1OCC1=NC=CC=C1.CN1C(CCC1)=O>>ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2
Cl[c:6]1[n:7][cH:8][n:9][c:10]2[cH:11][c:12](-[c:13]3[cH:14][cH:15][cH:16][o:17]3)[nH:18][c:19]12.[Cl:1][c:2]1[cH:3][c:4]([NH2:5])[cH:20][cH:21][c:22]1[O:23][CH2:24][c:25]1[cH:26][cH:27][cH:28][cH:29][n:30]1>>[Cl:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[n:7][cH:8][n:9][c:10]3[cH:11][c:12](-[c:13]4[cH:14][cH:15][cH:16][o:17]4)[...
Clc1ncnc2cc(-c3ccco3)[nH]c12.Nc1ccc(OCc2ccccn2)c(Cl)c1
Clc1cc(Nc2ncnc3cc(-c4ccco4)[nH]c23)ccc1OCc1ccccn1
null
null
O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
4e9376aae532abc2c3c92cfa1996ed64a03a89441cc1d43f64dc118dec94ec57
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2)nc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
46.6
[{"value": 46.6, "product": "ClC=1C=C(C=CC1OCC1=NC=CC=C1)NC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
2
HOUR
A mixture of 4-chloro-6-(2-furyl)-5H-pyrrolo[3,2-d]pyrimidine (80 mg), 3-chloro-4-(pyridin-2-ylmethoxy)aniline (94 mg) and 1-methyl-2-pyrrolidinone (2.5 mL) was stirred at 140° C. for 2 hrs, poured into water (10 mL) and adjusted to pH 8 with saturated aqueous sodium hydrogen carbonate. The mixture was extracted with e...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccoc1.c1ccncc1
HCl
O
140
2
Clc1ncnc2cc(-c3ccco3)[nH]c12.Nc1ccc(OCc2ccccn2)c(Cl)c1>O>Clc1cc(Nc2ncnc3cc(-c4ccco4)[nH]c23)ccc1OCc1ccccn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8f590447ac0b433096884f53a5ace055
COC(=O)c1ccc(C(=O)CC#N)cc1.Cc1ccc(S(=O)(=O)Cl)cc1>>COC(=O)c1ccc(C(=CC#N)OS(=O)(=O)c2ccc(C)cc2)cc1
C(#N)CC(=O)C1=CC=C(C(=O)OC)C=C1.C1(=CC=C(C=C1)S(=O)(=O)Cl)C.C(C)N(CC)CC>>C(#N)C=C(OS(=O)(=O)C1=CC=C(C=C1)C)C1=CC=C(C(=O)OC)C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9]([CH2:10][C:11]#[N:12])=[O:13])[cH:24][cH:25]1.Cl[S:14](=[O:15])(=[O:16])[c:17]1[cH:18][cH:19][c:20]([CH3:21])[cH:22][cH:23]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9](=[CH:10][C:11]#[N:12])[O:13][S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][c:20]([CH3...
COC(=O)c1ccc(C(=O)CC#N)cc1.Cc1ccc(S(=O)(=O)Cl)cc1
COC(=O)c1ccc(C(=CC#N)OS(=O)(=O)c2ccc(C)cc2)cc1
null
null
ClCCl
Acylation
OtherReaction
9f8c97f001bd09a5896e1620aa92ed222c76fd261d4582b923c7f486d025fb40
ad2bf1a301061ff4de8cacf445aa6c9f6615e0daaa746ef88ba96d39fc5112df
[CH]=C(OS(=O)(=O)c1ccccc1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[N;D1;H0:7]#[C:8]-[CH2;D2;+0:9]-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[c:12](:[c:13]):[c:14]>>[N;D1;H0:7]#[C:8]-[CH;D2;+0:9]=[C;H0;D3;+0:10](-[O;H0;D2;+0:11]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[c:12](:[c:13]):[c:14]
97.2
[{"value": 97.2, "product": "C(#N)C=C(OS(=O)(=O)C1=CC=C(C=C1)C)C1=CC=C(C(=O)OC)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a mixture of methyl 4-(cyanoacetyl)benzoate (10.29 g), p-toluenesulfonyl chloride (11.58 g) and dichloromethane (110 mL) was added dropwise triethylamine (7.68 g) under ice-cooling. After stirring under ice-cooling for 2.5 hrs, the mixture was diluted with dichloromethane (100 mL), washed with water (150 mL), dried ...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Ketone.Sulfonyl halide
Tosylate
null
null
c1ccccc1.c1ccccc1
HCl
ClCCl
null
null
COC(=O)c1ccc(C(=O)CC#N)cc1.Cc1ccc(S(=O)(=O)Cl)cc1>ClCCl>COC(=O)c1ccc(C(=CC#N)OS(=O)(=O)c2ccc(C)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8ba17fa0a560407bb18f0473c2156def
CCOC(=O)C(N)C(=O)OCC.COC(=O)c1ccc(C(=CC#N)OS(=O)(=O)c2ccc(C)cc2)cc1>>CCOC(=O)c1ccc(-c2cc(N)c(C(=O)OCC)[nH]2)cc1
[O-]CC.[Na+].Cl.C(#N)C=C(OS(=O)(=O)C1=CC=C(C=C1)C)C1=CC=C(C(=O)OC)C=C1.Cl.NC(C(=O)OCC)C(=O)OCC>>NC1=C(NC(=C1)C1=CC=C(C=C1)C(=O)OCC)C(=O)OCC
O=C(O[CH2:2][CH3:1])[CH:14]([C:15](=[O:16])[O:17][CH2:18][CH3:19])[NH2:20].Cc1ccc(S(=O)(=O)O[C:10]([c:9]2[cH:8][cH:7][c:6]([C:4]([O:3]C)=[O:5])[cH:22][cH:21]2)=[CH:11][C:12]#[N:13])cc1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9](-[c:10]2[cH:11][c:12]([NH2:13])[c:14]([C:15](=[O:16])[O:17][CH2:18][CH3:19])[n...
CCOC(=O)C(N)C(=O)OCC.COC(=O)c1ccc(C(=CC#N)OS(=O)(=O)c2ccc(C)cc2)cc1
CCOC(=O)c1ccc(-c2cc(N)c(C(=O)OCC)[nH]2)cc1
null
null
O1CCCC1.C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
5a0500a596c38ffea4f79f3f3c03d502284d793b3d53693f26c30f1e46f66a23
43c496d8acff34bbf2f9380b19cdbc08333f79dbba42ae17715b324ab48e7f11
c1ccc(-c2ccc[nH]2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[c:6]:[c;H0;D3;+0:7](-[C;H0;D3;+0:8](-O-S(=O)(=O)-c2:c:c:c(-C):c:c:2)=[CH;D2;+0:9]-[C;H0;D2;+0:10]#[N;H0;D1;+0:11]):[c:12]:[c:13]:1.O=C(-O-[CH2;D2;+0:14]-[C;D1;H3:15])-[CH;D3;+0:16](-[NH2;D1;+0:17])-[C:18](=[O;D1;H0:19])-[#8:20]-[C:21]>>[C:21]-[#8:20]-[C:18](=[O;D1;H0:1...
null
[]
null
null
null
null
To a suspension of methyl 4-(2-cyano-1-{[(4-methylphenyl)sulfonyl]oxy}vinyl)benzoate (17.5 g) and diethyl aminomalonate hydrochloride (10.36 g) in a mixed solvent of ethanol (165 mL)-tetrahydrofuran (80 mL) was added dropwise a solution (50 mL) of 20% sodium ethoxide in ethanol under ice-cooling. After stirring under i...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Ester.Ester.Ester.Nitrile.Primary amine
Ester.Ester.Primary amine
c1ccccc1
c1cc[nH]c1
c1ccccc1.c1cc[nH]c1
TsOH.HO-
O1CCCC1.C(C)O
null
null
CCOC(=O)C(N)C(=O)OCC.COC(=O)c1ccc(C(=CC#N)OS(=O)(=O)c2ccc(C)cc2)cc1>O1CCCC1.C(C)O>CCOC(=O)c1ccc(-c2cc(N)c(C(=O)OCC)[nH]2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-23398c4f680f4fd6a53b3b6ec365b20c
CCOC(=O)c1ccc(-c2cc(N)c(C(=O)OCC)[nH]2)cc1.N=CN>>CCOC(=O)c1ccc(-c2cc3nc[nH]c(=O)c3[nH]2)cc1
NC1=C(NC(=C1)C1=CC=C(C=C1)C(=O)OCC)C(=O)OCC.C(C)(=O)O.C(=N)N>>O=C1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)OCC)C=C2
CCO[C:16](=[O:17])[c:18]1[c:12]([NH2:13])[cH:11][c:10](-[c:9]2[cH:8][cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:21][cH:20]2)[nH:19]1.N[CH:14]=[NH:15]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9](-[c:10]2[cH:11][c:12]3[n:13][cH:14][nH:15][c:16](=[O:17])[c:18]3[nH:19]2)[cH:20][cH:21]1
CCOC(=O)c1ccc(-c2cc(N)c(C(=O)OCC)[nH]2)cc1.N=CN
CCOC(=O)c1ccc(-c2cc3nc[nH]c(=O)c3[nH]2)cc1
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
cf2d93c547f6b79e1ff78c4c95ac2a9882be6c07ff6c3d38d4ab70f7d93654ab
36efa24579e0043fdba8918e78f1d75cb4504837c08d344d01203f5fa64bfaef
O=c1[nH]cnc2cc(-c3ccccc3)[nH]c12
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[c:6]:[c:7]:1-[NH2;D1;+0:8].N-[CH;D2;+0:9]=[NH;D1;+0:10]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[nH;D2;+0:10]:[cH;D2;+0:9]:[n;H0;D2;+0:8]:[c:7]2:[c:6]:[c:5]:[#7;a:4]:[c:3]:2:1
94.3
[{"value": 94.3, "product": "O=C1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)OCC)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of ethyl 3-amino-5-[4-(ethoxycarbonyl)phenyl]-1H-pyrrole-2-carboxylate (3.36 g), formamidine acetate (1.74 g) and ethanol (60 mL) was heated under reflux for 15 hrs. After cooling to room temperature, the precipitated solid was collected by filtration, washed with ethanol, and dried under reduced pressure at ...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine.Primary amine
null
c1cc[nH]c1
c1cc2ncncc2[nH]1
c1ccccc1.c1cc2ncncc2[nH]1
HO-
C(C)O
null
null
CCOC(=O)c1ccc(-c2cc(N)c(C(=O)OCC)[nH]2)cc1.N=CN>C(C)O>CCOC(=O)c1ccc(-c2cc3nc[nH]c(=O)c3[nH]2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f73f8bea7c904e2399764dcdefce25f6
CCOC(=O)c1ccc(-c2cc3nc[nH]c(=O)c3[nH]2)cc1.O=P(Cl)(Cl)Cl>>CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Cl
O=C1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)OCC)C=C2.P(=O)(Cl)(Cl)Cl>>Cl.ClC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)OCC)C=C2
O=[c:16]1[nH:15][cH:14][n:13][c:12]2[cH:11][c:10](-[c:9]3[cH:8][cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:21][cH:20]3)[nH:19][c:18]21.O=P(Cl)([Cl:17])[Cl:22]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9](-[c:10]2[cH:11][c:12]3[n:13][cH:14][n:15][c:16]([Cl:17])[c:18]3[nH:19]2)[cH:20][cH:21]1.[ClH:22]
CCOC(=O)c1ccc(-c2cc3nc[nH]c(=O)c3[nH]2)cc1.O=P(Cl)(Cl)Cl
CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Cl
null
null
O1CCOCC1
Functional Group Interconversion
OtherReaction
990997bc80649f34ced0b0b8c9ec1b3d7f7bb4583bf26285f81a6c467d40b7b8
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc(-c2cc3ncncc3[nH]2)cc1
Cl-P(=O)(-[Cl;H0;D1;+0:1])-[Cl;H0;D1;+0:2].O=[c;H0;D3;+0:3]1:[nH;D2;+0:4]:[c:5]:[#7;a:6]:[c:7]2:[c:8]:[c:9]:[#7;a:10]:[c:11]:2:1>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:3]1:[n;H0;D2;+0:4]:[c:5]:[#7;a:6]:[c:7]2:[c:8]:[c:9]:[#7;a:10]:[c:11]:2:1.[ClH;D0;+0:2]
94.2
[{"value": 94.2, "product": "Cl.ClC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)OCC)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
110
CELSIUS
1
HOUR
A mixture of ethyl 4-(4-oxo-4,5-dihydro-3H-pyrrolo[3,2-d]pyrimidin-6-yl)benzoate (2.97 g) and phosphoryl chloride (16.45 g) was stirred at 110° C. for 1 hr, dioxane (10 mL) was added and the mixture was heated under reflux for 4 hrs. After concentration under reduced pressure, ethanol (30 mL) was added to the residue a...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1cc2ncncc2[nH]1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1
Other
O1CCOCC1
110
1
CCOC(=O)c1ccc(-c2cc3nc[nH]c(=O)c3[nH]2)cc1.O=P(Cl)(Cl)Cl>O1CCOCC1>CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e690e0d37b5647b480ee3cba21bcd7dd
CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Cc1ccc(Oc2ccc(N)cc2C)cn1>>Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccc(C(=O)O)cc5)[nH]c34)cc2C)cn1
Cl.ClC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)OCC)C=C2.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C.C(C)(C)N(CC)C(C)C.CN1C(CCC1)=O>>Cl.CC=1C=C(C=CC1OC=1C=NC(=CC1)C)NC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)O)C=C2
CC[O:25][C:23]([c:22]1[cH:21][cH:20][c:19](-[c:18]2[cH:17][c:16]3[n:15][cH:14][n:13][c:12](Cl)[c:29]3[nH:28]2)[cH:27][cH:26]1)=[O:24].[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH2:11])[cH:30][c:31]2[CH3:32])[cH:33][n:34]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n...
CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Cc1ccc(Oc2ccc(N)cc2C)cn1
Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccc(C(=O)O)cc5)[nH]c34)cc2C)cn1
null
null
O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
521ad2e982ed77e44719df3f58454a49cf9127923079f040329e1018635dd0ce
de5a4a1c21f0a9f757d533080e1d67a6200de123fe2d9421ccc3db04c6765633
c1ccc(-c2cc3ncnc(Nc4ccc(Oc5cccnc5)cc4)c3[nH]2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4].Cl-[c;H0;D3;+0:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[#7;a:12]:[c:13]:2:1.[NH2;D1;+0:14]-[c:15](:[c:16]):[c:17]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4].[c:16]:[c:15](-[NH;D2;+0:14]-[c;H0;D3;+0:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[#7;a:12]:[c:13]:2:1):...
57.7
[{"value": 57.7, "product": "Cl.CC=1C=C(C=CC1OC=1C=NC(=CC1)C)NC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)O)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
3
HOUR
A mixture of ethyl 4-(4-chloro-5H-pyrrolo[3,2-d]pyrimidin-6-yl)benzoate hydrochloride (1.297 g), 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (1.00 g), diisopropylethylamine (0.834 g) and 1-methyl-2-pyrrolidinone (12.5 mL) was stirred at 140° C. for 3 hrs, poured into water (100 mL)-ethyl acetate (150 mL) and the prec...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Primary amine
Carboxylic acid.Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccncc1.c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1
HCl
O.C(C)(=O)OCC
140
3
CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Cc1ccc(Oc2ccc(N)cc2C)cn1>O.C(C)(=O)OCC>Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccc(C(=O)O)cc5)[nH]c34)cc2C)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-71723cd5d3864132b3a9cd98e9d39005
CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>>O=C(O)c1ccc(-c2cc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c3[nH]2)cc1
C(O)([O-])=O.[Na+].Cl.ClC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)OCC)C=C2.ClC=1C=C(N)C=CC1OCC1=CC(=CC=C1)F.CN1C(CCC1)=O>>Cl.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)O)C=C2
CC[O:4][C:3](=[O:2])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][c:11]3[n:12][cH:13][n:14][c:15](Cl)[c:33]3[nH:34]2)[cH:35][cH:36]1.[NH2:16][c:17]1[cH:18][cH:19][c:20]([O:21][CH2:22][c:23]2[cH:24][cH:25][cH:26][c:27]([F:28])[cH:29]2)[c:30]([Cl:31])[cH:32]1>>[O:2]=[C:3]([OH:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][c:11]3[n:1...
CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1
O=C(O)c1ccc(-c2cc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c3[nH]2)cc1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
521ad2e982ed77e44719df3f58454a49cf9127923079f040329e1018635dd0ce
de5a4a1c21f0a9f757d533080e1d67a6200de123fe2d9421ccc3db04c6765633
c1ccc(COc2ccc(Nc3ncnc4cc(-c5ccccc5)[nH]c34)cc2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4].Cl-[c;H0;D3;+0:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[#7;a:12]:[c:13]:2:1.[NH2;D1;+0:14]-[c:15](:[c:16]):[c:17]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4].[c:16]:[c:15](-[NH;D2;+0:14]-[c;H0;D3;+0:5]1:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]2:[c:10]:[c:11]:[#7;a:12]:[c:13]:2:1):...
62
[{"value": 62.0, "product": "Cl.ClC=1C=C(C=CC1OCC1=CC(=CC=C1)F)NC=1C2=C(N=CN1)C=C(N2)C2=CC=C(C(=O)O)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
5
HOUR
A mixture of ethyl 4-(4-chloro-5H-pyrrolo[3,2-d]pyrimidin-6-yl)benzoate hydrochloride (517 mg), 3-chloro-4-[(3-fluorobenzyl)oxy]aniline (462 mg) and 1-methyl-2-pyrrolidinone (8 mL) was stirred at 140° C. for 5 hrs, poured into water (40 mL), and adjusted to pH 8 with saturated aqueous sodium hydrogen carbonate. The pre...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Primary amine
Carboxylic acid.Secondary amine
c1ncc2[nH]ccc2n1
c1ncc2[nH]ccc2n1
c1ccccc1.c1ncc2[nH]ccc2n1.c1ccccc1.c1ccccc1
HCl
O
140
5
CCOC(=O)c1ccc(-c2cc3ncnc(Cl)c3[nH]2)cc1.Nc1ccc(OCc2cccc(F)c2)c(Cl)c1>O>O=C(O)c1ccc(-c2cc3ncnc(Nc4ccc(OCc5cccc(F)c5)c(Cl)c4)c3[nH]2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4b3bfb9f6ba64d338b3412fe35f0ed62
CI.Clc1ncnc2cc(-c3ccco3)[nH]c12>>Cn1c(-c2ccco2)cc2ncnc(Cl)c21
O.ClC=1C2=C(N=CN1)C=C(N2)C=2OC=CC2.C([O-])([O-])=O.[K+].[K+].CI>>ClC=1C2=C(N=CN1)C=C(N2C)C=2OC=CC2
I[CH3:1].[nH:2]1[c:3](-[c:4]2[cH:5][cH:6][cH:7][o:8]2)[cH:9][c:10]2[n:11][cH:12][n:13][c:14]([Cl:15])[c:16]12>>[CH3:1][n:2]1[c:3](-[c:4]2[cH:5][cH:6][cH:7][o:8]2)[cH:9][c:10]2[n:11][cH:12][n:13][c:14]([Cl:15])[c:16]12
CI.Clc1ncnc2cc(-c3ccco3)[nH]c12
Cn1c(-c2ccco2)cc2ncnc(Cl)c21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
984dc1e2f23276e16434cf60f0728fced0721ac085a767b5a5daa33828d25b2d
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
c1coc(-c2cc3ncncc3[nH]2)c1
I-[CH3;D1;+0:1].[#8;a:2]:[c:3]-[c:4]1:[c:5]:[c:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10](-[Cl;D1;H0:11]):[c:12]:2:[nH;D2;+0:13]:1>>[#8;a:2]:[c:3]-[c:4]1:[c:5]:[c:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10](-[Cl;D1;H0:11]):[c:12]:2:[n;H0;D3;+0:13]:1-[CH3;D1;+0:1]
40.2
[{"value": 40.2, "product": "ClC=1C2=C(N=CN1)C=C(N2C)C=2OC=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 4-chloro-6-(2-furyl)-5H-pyrrolo[3,2-d]pyrimidine (220 mg) in N,N-dimethylformamide (2.5 mL) were added potassium carbonate (139 mg) and methyl iodide (0.25 mL) and the mixture was stirred at room temperature for 8 hrs. The mixture was poured into water (30 mL) and extracted with ethyl acetate (30 mL×3)...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ncc2[nH]ccc2n1
c1cc2ncncc2[nH]1
c1ccoc1.c1cc2ncncc2[nH]1
HI
CN(C=O)C
null
8
CI.Clc1ncnc2cc(-c3ccco3)[nH]c12>CN(C=O)C>Cn1c(-c2ccco2)cc2ncnc(Cl)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c52e7509444a496d9253b6abe0ab4828
Cc1ccc(Oc2ccc(N)cc2C)cn1.Cn1c(-c2ccco2)cc2ncnc(Cl)c21>>Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccco5)n(C)c34)cc2C)cn1
C(O)([O-])=O.[Na+].ClC=1C2=C(N=CN1)C=C(N2C)C=2OC=CC2.CC=1C=C(N)C=CC1OC=1C=NC(=CC1)C.CN1C(CCC1)=O>>O1C(=CC=C1)C1=CC=2N=CN=C(C2N1C)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C
[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH2:11])[cH:27][c:28]2[CH3:29])[cH:30][n:31]1.Cl[c:12]1[n:13][cH:14][n:15][c:16]2[cH:17][c:18](-[c:19]3[cH:20][cH:21][cH:22][o:23]3)[n:24]([CH3:25])[c:26]12>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[cH:8][cH:9][c:10]([NH:11][c:12]3[n:13][cH:14][n:15][c:16]...
Cc1ccc(Oc2ccc(N)cc2C)cn1.Cn1c(-c2ccco2)cc2ncnc(Cl)c21
Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccco5)n(C)c34)cc2C)cn1
null
null
O
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
a761a23478bcca0adfe0c4dd4341ad165c5bf801aa5c397f8a3fb7ad8077557d
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cncc(Oc2ccc(Nc3ncnc4cc(-c5ccco5)[nH]c34)cc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5]2:[c:6]:[c:7]:[#7;a:8](-[C;D1;H3:9]):[c:10]:2:1.[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C;D1;H3:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5]2:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]):[c:10]:1:2
64.8
[{"value": 64.8, "product": "O1C(=CC=C1)C1=CC=2N=CN=C(C2N1C)NC1=CC(=C(C=C1)OC=1C=NC(=CC1)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
3.5
HOUR
A mixture of 4-chloro-6-(2-furyl)-5-methyl-5H-pyrrolo[3,2-d]pyrimidine (92 mg), 3-methyl-4-[(6-methylpyridin-3-yl)oxy]aniline (102 mg) and 1-methyl-2-pyrrolidinone (2.5 mL) was stirred at 140° C. for 3.5 hrs, poured into water (10 mL) and adjusted to pH 8 with saturated aqueous sodium hydrogen carbonate. The mixture wa...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cc2ncncc2[nH]1
c1cc2ncncc2[nH]1
c1ccncc1.c1ccccc1.c1cc2ncncc2[nH]1.c1ccoc1
HCl
O
140
3.5
Cc1ccc(Oc2ccc(N)cc2C)cn1.Cn1c(-c2ccco2)cc2ncnc(Cl)c21>O>Cc1ccc(Oc2ccc(Nc3ncnc4cc(-c5ccco5)n(C)c34)cc2C)cn1