dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-28c886cb9ce14ef9a1ee1b4b0580332d
CC(=O)c1ccc(Br)cc1.SCCCS>>CC(c1ccc(Br)cc1)C1SCCCS1
BrC1=CC=C(C=C1)C(C)=O.C(CCS)S.B(F)(F)F.CCOCC>>BrC1=CC=C(C=C1)C(C)C1SCCCS1
O=[C:2]([CH3:1])[c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][cH:9]1.[SH:11][CH2:12][CH2:13][CH2:14][SH:15]>>[CH3:1][CH:2]([c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][cH:9]1)[CH:10]1[S:11][CH2:12][CH2:13][CH2:14][S:15]1
CC(=O)c1ccc(Br)cc1.SCCCS
CC(c1ccc(Br)cc1)C1SCCCS1
null
null
ClCCl.ClC(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
4758dc84fa113e6f0c3b6850de21934960e643c3350412341d86e1faa5438e76
cca0c476bcede45e7917ec20f9c51c08f1c759c1b0a2d2c92077062e73c24406
c1ccc(CC2SCCCS2)cc1
O=[C;H0;D3;+0:1](-[C;D1;H3:2])-[c:3](:[c:4]):[c:5].[SH;D1;+0:6]-[C:7]-[C:8]-[C:9]-[SH;D1;+0:10]>>[C;D1;H3:2]-[CH;D3;+0:1](-[C:11]1-[S;H0;D2;+0:6]-[C:7]-[C:8]-[C:9]-[S;H0;D2;+0:10]-1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
48
HOUR
To the compound p-bromoacetophenone (36.85 g, 0.185 mol) in trichloromethane (300 ml) was added 1,3-propanedithiol (25 g, 0.23 mol) and boron trifluoride etherate (3 ml). The resulting mixture was stirred at room temperature for 48 hours. The mixture was diluted with dichloromethane (500 ml), washed twice with 10% sodi...
10.6084/m9.figshare.5104873.v1
null
Ketone.Aliphatic thiol.Aliphatic thiol
Monosulfide.Monosulfide
null
C1CSCSC1
c1ccccc1.C1CSCSC1
null
ClCCl.ClC(Cl)Cl
null
48
CC(=O)c1ccc(Br)cc1.SCCCS>ClCCl.ClC(Cl)Cl>CC(c1ccc(Br)cc1)C1SCCCS1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e1d06b03b61c4832b159fc423e9257f9
BrCCCCBr.CC(c1ccc(Br)cc1)C1SCCCS1>>CC(c1ccc(CCCCBr)cc1)C1SCCCS1
C(C)(=O)OCC.BrCCCCBr.BrC1=CC=C(C=C1)C(C)C1SCCCS1.C(C)(CC)[Li]>>BrCCCCC1=CC=C(C=C1)C(C)C1SCCCS1
Br[CH2:7][CH2:8][CH2:9][CH2:10][Br:11].Br[c:6]1[cH:5][cH:4][c:3]([CH:2]([CH3:1])[CH:14]2[S:15][CH2:16][CH2:17][CH2:18][S:19]2)[cH:13][cH:12]1>>[CH3:1][CH:2]([c:3]1[cH:4][cH:5][c:6]([CH2:7][CH2:8][CH2:9][CH2:10][Br:11])[cH:12][cH:13]1)[CH:14]1[S:15][CH2:16][CH2:17][CH2:18][S:19]1
BrCCCCBr.CC(c1ccc(Br)cc1)C1SCCCS1
CC(c1ccc(CCCCBr)cc1)C1SCCCS1
null
null
O1CCCC1
C-C Coupling
Negishi
530a9bd1eaaebd54d09786b6168a1d1d89df12b3fda60e0c00afadb98df85946
84e12b0159f1d183204538a38a0b22f090552039c6c4b4ca4a95700e436c4e5e
c1ccc(CC2SCCCS2)cc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].Br-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:7]:[c:8]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:7]:[c:8]
null
[]
null
null
1.5
HOUR
A solution of 4-bromo-1-(1,3-dithian-2-yl)ethylbenzene (27.2 g, 94 moles) in tetrahydrofuran (200 ml) was charged with sec-butyllithium (99 ml, 1.3M in cyclohexane, 0.13 mole) dropwise at −78° C. under nitrogen. The mixture was stirred at ambient temperature for 1.5 hours, and then quenched with 1,4-dibromobutane (4.2 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary halide
null
c1ccccc1
c1ccccc1
c1ccccc1.C1CSCSC1
Br-
O1CCCC1
null
1.5
BrCCCCBr.CC(c1ccc(Br)cc1)C1SCCCS1>O1CCCC1>CC(c1ccc(CCCCBr)cc1)C1SCCCS1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4913b0e304f84c2a81beefe32b706a4c
NO.O=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1>>ON=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1
FC1=C(C=CC(=C1)F)C(=O)C1CN(CC1)CC1=CC=CC=C1.NO.Cl.C(C)(=O)[O-].[NH4+]>>FC1=C(C=CC(=C1)F)C(=NO)C1CN(CC1)CC1=CC=CC=C1
[OH:1][NH2:2].O=[C:3]([c:4]1[cH:5][cH:6][c:7]([F:8])[cH:9][c:10]1[F:11])[CH:12]1[CH2:13][CH2:14][N:15]([CH2:16][c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[CH2:23]1>>[OH:1][N:2]=[C:3]([c:4]1[cH:5][cH:6][c:7]([F:8])[cH:9][c:10]1[F:11])[CH:12]1[CH2:13][CH2:14][N:15]([CH2:16][c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[CH...
NO.O=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1
ON=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1
null
null
O.C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
b5fd91d879f097d0ef2e8e2d3ef7d2ef0195968870a9602a47b8324c601790b9
1a0ef15294bdb221fb8888b5d4c7fcf00473b11e53da288791d32747daa48d23
N=C(c1ccccc1)C1CCN(Cc2ccccc2)C1
O=[C;H0;D3;+0:1](-[C:2](-[C:3])-[C:4]-[#7:5])-[c:6](:[c:7]):[c:8].[NH2;D1;+0:9]-[O;D1;H1:10]>>[#7:5]-[C:4]-[C:2](-[C;H0;D3;+0:1](=[N;H0;D2;+0:9]-[O;D1;H1:10])-[c:6](:[c:7]):[c:8])-[C:3]
52
[{"value": 52.0, "product": "FC1=C(C=CC(=C1)F)C(=NO)C1CN(CC1)CC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
To the compound (2,4-difluorophenyl)[1-(phenylmethyl)-3-pyrrolidinyl]methanone (22 g) in 95% ethanol (350 ml) and water (100 ml) was added NH2OH.HCl (10.1 g) and ammonium acetate (12.7 g, 2.1 eq). The resulting mixture was refluxed for 3.5 hours. The mixture was then allowed to stir at room temperature for 24 hours. Th...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Oxime
null
null
c1ccccc1.C1CC[NH]C1.c1ccccc1
HO-
O.C(C)O
null
24
NO.O=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1>O.C(C)O>ON=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1c2866d7ff1e496ea78a346f834c26e9
ON=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1>>Fc1ccc2c(C3CCN(Cc4ccccc4)C3)noc2c1
FC1=C(C=CC(=C1)F)C(=NO)C1CN(CC1)CC1=CC=CC=C1.[OH-].[K+].O.C(\C=C\C(=O)O)(=O)O>>C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CN(CC2)CC2=CC=CC=C2)C=C1
F[c:21]1[c:5]([C:6]([CH:7]2[CH2:8][CH2:9][N:10]([CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][cH:17]3)[CH2:18]2)=[N:19][OH:20])[cH:4][cH:3][c:2]([F:1])[cH:22]1>>[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][N:10]([CH2:11][c:12]4[cH:13][cH:14][cH:15][cH:16][cH:17]4)[CH2:18]3)[n:19][o:20][c:21]2[cH:22]1
ON=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1
Fc1ccc2c(C3CCN(Cc4ccccc4)C3)noc2c1
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
cfebb679a94a29342a57758c91b6c629149cdccb6d62df316a2e291ec25d681b
c3af886e80a4d8a4db0b9015a14ae7edf5d5d18deb2717f7ce3620ceac08ea61
c1ccc(CN2CCC(c3noc4ccccc34)C2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C;H0;D3;+0:5](=[N;H0;D2;+0:6]-[OH;D1;+0:7])-[C:8](-[C:9])-[C:10]-[#7:11]):[c:12]>>[#7:11]-[C:10]-[C:8](-[c;H0;D3;+0:5]1:[n;H0;D2;+0:6]:[o;H0;D2;+0:7]:[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:1:[c:12])-[C:9]
74.8
[{"value": 74.8, "product": "C(\\C=C\\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CN(CC2)CC2=CC=CC=C2)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of (2,4-difluorophenyl)[1-(phenylmethyl)-3-pyrrolidinyl]methanone oxime (10.8 g, 34.2 mmoles), potassium hydroxide (10 g), water (100 ml), and ethanol (100 ml) was heated at reflux for 2 hr. At the end of the reaction, the solution was cooled and ethanol was removed on a rotary evaporator. The aqueous mixture...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Oxime
null
c1ccccc1
c1ccc2oncc2c1
C1CC[NH]C1.c1ccccc1.c1ccc2oncc2c1
HF
C(C)O
null
null
ON=C(c1ccc(F)cc1F)C1CCN(Cc2ccccc2)C1>C(C)O>Fc1ccc2c(C3CCN(Cc4ccccc4)C3)noc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6b793585f62848809ec01c140b495935
COc1cc(C=O)ccc1O.ClCCCBr>>COc1cc(C=O)ccc1OCCCCl
O.O=CC1=CC(OC)=C(O)C=C1.C(=O)([O-])[O-].[K+].[K+].BrCCCCl>>ClCCCOC1=C(C=C(C=O)C=C1)OC
[CH3:1][O:2][c:3]1[cH:4][c:5]([CH:6]=[O:7])[cH:8][cH:9][c:10]1[OH:11].Br[CH2:12][CH2:13][CH2:14][Cl:15]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([CH:6]=[O:7])[cH:8][cH:9][c:10]1[O:11][CH2:12][CH2:13][CH2:14][Cl:15]
COc1cc(C=O)ccc1O.ClCCCBr
COc1cc(C=O)ccc1OCCCCl
null
null
CC(=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[OH;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]
37
[{"value": 37.0, "product": "ClCCCOC1=C(C=C(C=O)C=C1)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 5.9, "product": "ClCCCOC1=C(C=C(C=O)C=C1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of vanillin (30.4 g, 0.2 mol), K2CO3 (27.6 g) and acetone (150 ml) was stirred and refluxed for 0.5 hours. Heating was removed and 1-bromo-3-chloropropane (40.8 g, 0.26 mol) in acetone was added dropwise. The reaction was stirred and refluxed for 16 hours, and then it was poured into water. The aqueous mixtur...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HBr
CC(=O)C
null
null
COc1cc(C=O)ccc1O.ClCCCBr>CC(=O)C>COc1cc(C=O)ccc1OCCCCl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-080ed4d2582e48539c815fdf98dc7577
C=COC(=O)N1CCC(c2noc3cc(F)ccc23)C1>>Fc1ccc2c(C3CCNC3)noc2c1
C(=C)OC(=O)N1CC(CC1)C1=NOC2=C1C=CC(=C2)F.Cl>>Cl.FC1=CC2=C(C(=NO2)C2CNCC2)C=C1
C=COC(=O)[N:11]1[CH2:10][CH2:9][CH:8]([c:7]2[c:6]3[cH:5][cH:4][c:3]([F:2])[cH:16][c:15]3[o:14][n:13]2)[CH2:12]1>>[F:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([CH:8]3[CH2:9][CH2:10][NH:11][CH2:12]3)[n:13][o:14][c:15]2[cH:16]1
C=COC(=O)N1CCC(c2noc3cc(F)ccc23)C1
Fc1ccc2c(C3CCNC3)noc2c1
null
null
C(C)(C)O
Reduction
Hydrogenolysis of tertiary amines
b8f95e8847b8644bde7f55684fbdd5ce4dd641748931e44ce5a651614b5011ea
4693d071c7195c4d1d1e30a5794ffc365d4c1fab9edd2d709ddf2a18cef75754
c1ccc2c(C3CCNC3)noc2c1
C=C-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-1>>[C:2]1-[C:3]-[C:4]-[C:5]-[NH;D2;+0:1]-1
null
[]
0
CELSIUS
null
null
A mixture of 3-(6-fluoro-1,2-benzisoxazol-3-yl)-1-pyrrolidinylcarboxylic acid ethenyl ester (5.1 g, 18.4 mmol, hydrochloride acid (5 ml), and isopropyl alcohol (50 ml) was heated at reflux for 3.5 hr. At the end of the reaction, the solvent was reduced to about 30 ml on a rotary evaporator and the mixture was cooled to...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Vinyl
Secondary amine
C1CC[NH]C1
C1CCNC1
C1CCNC1.c1ccc2oncc2c1
HO-
C(C)(C)O
0
null
C=COC(=O)N1CCC(c2noc3cc(F)ccc23)C1>C(C)(C)O>Fc1ccc2c(C3CCNC3)noc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-27cda37f683d45c0a64365778b1ece4b
BrCCCCBr.Fc1ccc2c(C3CCNCC3)noc2c1>>Fc1ccc2c(C3CCN(CCCCBr)CC3)noc2c1
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.C(=O)([O-])[O-].[K+].[K+].BrCCCCBr>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCCBr)C=C1
Br[CH2:11][CH2:12][CH2:13][CH2:14][Br:15].[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][NH:10][CH2:16][CH2:17]3)[n:18][o:19][c:20]2[cH:21]1>>[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][N:10]([CH2:11][CH2:12][CH2:13][CH2:14][Br:15])[CH2:16][CH2:17]3)[n:18][o:19][c:20]2[cH:21]1
BrCCCCBr.Fc1ccc2c(C3CCNCC3)noc2c1
Fc1ccc2c(C3CCN(CCCCBr)CC3)noc2c1
null
null
C(C)#N
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc2c(C3CCNCC3)noc2c1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:6](-[C:5]-[C:4])-[C:7]-[C:8]
null
[]
null
null
8
HOUR
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (12 in, 55 mmol), K2CO3 (13 m) and 1,4-dibromobutane (20 m, 9.3 mmol, 1.7 eq) in acetonitrile (300 ml) was stirred at room temperature overnight. The inorganic material was filtered. The solution was concentrated to ˜80 ml, when crystals crashed out. The product...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2oncc2c1
HBr
C(C)#N
null
8
BrCCCCBr.Fc1ccc2c(C3CCNCC3)noc2c1>C(C)#N>Fc1ccc2c(C3CCN(CCCCBr)CC3)noc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-208e7a31260143b7baa9163c46186c76
CC(=O)OCCBr.Fc1ccc2c(C3CCNCC3)noc2c1>>CC(=O)OCCN1CCC(c2noc3cc(F)ccc23)CC1
C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.C(=O)([O-])[O-].[K+].[K+].C(C)(=O)OCCBr>>C(\C=C\C(=O)O)(=O)O.C(C)(=O)OCCN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F
Br[CH2:6][CH2:5][O:4][C:2]([CH3:1])=[O:3].[NH:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18][cH:19][c:20]23)[CH2:21][CH2:22]1>>[CH3:1][C:2](=[O:3])[O:4][CH2:5][CH2:6][N:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18][cH:19][c:20]23)[CH2:21][CH2:22]1
CC(=O)OCCBr.Fc1ccc2c(C3CCNCC3)noc2c1
CC(=O)OCCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
C(C)#N.C(C)O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc2c(C3CCNCC3)noc2c1
Br-[CH2;D2;+0:1]-[C:2]-[#8:3]-[C:4](-[C;D1;H3:5])=[O;D1;H0:6].[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]>>[C:7]-[C:8]-[N;H0;D3;+0:9](-[CH2;D2;+0:1]-[C:2]-[#8:3]-[C:4](-[C;D1;H3:5])=[O;D1;H0:6])-[C:10]-[C:11]
null
[]
null
null
null
null
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (3.0 gm, 13.6 mmol), K2CO3 (3.5 m, 25 mmol), 2-bromoethyl acetate (4 gm, 26.5 mmol) in acetonitrile (50 ml) was heated at reflux for 4 hr. After cooling to room temperature, the inorganic salts were filtered and washed with DCM (dichloromethane 50 ml). The organ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2oncc2c1
HBr
C(C)#N.C(C)O
null
null
CC(=O)OCCBr.Fc1ccc2c(C3CCNCC3)noc2c1>C(C)#N.C(C)O>CC(=O)OCCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7f0c453459844830a5dfe770f1ee7a44
ClCCN1CCOCC1.Fc1ccc2c(C3CCNCC3)noc2c1>>Fc1ccc2c(C3CCN(CCN4CCOCC4)CC3)noc2c1
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.Cl.ClCCN1CCOCC1.C(=O)([O-])[O-].[K+].[K+]>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2CCOCC2)C=C1
Cl[CH2:11][CH2:12][N:13]1[CH2:14][CH2:15][O:16][CH2:17][CH2:18]1.[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][NH:10][CH2:19][CH2:20]3)[n:21][o:22][c:23]2[cH:24]1>>[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][N:10]([CH2:11][CH2:12][N:13]4[CH2:14][CH2:15][O:16][CH2:17][CH2:18]4)[CH2:19][CH2:20]3)[...
ClCCN1CCOCC1.Fc1ccc2c(C3CCNCC3)noc2c1
Fc1ccc2c(C3CCN(CCN4CCOCC4)CC3)noc2c1
null
null
C(C)#N.C(Cl)Cl
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc2c(C3CCN(CCN4CCOCC4)CC3)noc2c1
Cl-[CH2;D2;+0:1]-[C:2]-[#7:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:6](-[C:5]-[C:4])-[C:7]-[C:8]
null
[]
null
null
null
null
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (3.0 gm, 13.6 mmol), 2-chloroethyl morpholine hydrochloride (4.46 gm, 29.7 mmol) and K2CO3 (7.3 gm, 2.2 eq) in acetonitrile (60 ml) was heated at reflux for 24 hr. The crude mixture was diluted with DCM and filtered. The solvent was concentrated to an oil (˜7.1 ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1COCC[NH]1.c1ccc2oncc2c1
HCl
C(C)#N.C(Cl)Cl
null
null
ClCCN1CCOCC1.Fc1ccc2c(C3CCNCC3)noc2c1>C(C)#N.C(Cl)Cl>Fc1ccc2c(C3CCN(CCN4CCOCC4)CC3)noc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a453c7ef0c45442b84a793728bfaaf18
Fc1ccc2c(C3CCNCC3)noc2c1.O=C1NC(=O)c2c(CCBr)cccc21>>O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.C(=O)([O-])[O-].[K+].[K+].BrCCC1=C2C(C(=O)NC2=O)=CC=C1.C(C)#N>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC=CC3)=O)C=C1
[NH:14]1[CH2:15][CH2:16][CH:17]([c:18]2[n:19][o:20][c:21]3[cH:22][c:23]([F:24])[cH:25][cH:26][c:27]23)[CH2:28][CH2:29]1.Br[CH2:12][CH2:13][c:4]1[c:3]2[c:8]([cH:7][cH:6][cH:5]1)[C:9](=[O:10])[NH:11][C:2]2=[O:1]>>[O:1]=[C:2]1[c:3]2[cH:4][cH:5][cH:6][cH:7][c:8]2[C:9](=[O:10])[N:11]1[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][...
Fc1ccc2c(C3CCNCC3)noc2c1.O=C1NC(=O)c2c(CCBr)cccc21
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
caede2b65a541826d0816af10d43f7c550425032c949a27fc1d2af4936a75676
4f85b4d0af17555b490073b5bd8727ffab737e6008592e3cbb27e5b30c359ff1
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
Br-[CH2;D2;+0:1]-[CH2;D2;+0:2]-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6]1:[c:7]-[C:8](=[O;D1;H0:9])-[NH;D2;+0:10]-[C:11]-1=[O;D1;H0:12].[C:13]-[C:14]-[NH;D2;+0:15]-[C:16]-[C:17]>>[C:13]-[C:14]-[N;H0;D3;+0:15](-[CH2;D2;+0:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:10]1-[C:11](=[O;D1;H0:12])-[c:6](:[c:7]-[C:8]-1=[O;D1;H0:9]):[cH;D2;+0:3]:[c:...
null
[]
null
null
null
null
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (5 15 gm 23 4 mmol) K2CO3 (4.2 gm, 30.4 mmol) and 2-bromoethyl phthalimide (7.13 gm, 28 mmol) in acetonitrile (250 ml) was heated at reflux for 3.5 hr. The solids and solvent were removed. The residue was purified by flash chromatography (SiO2, 110 m, eluted wit...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Unsubstituted dicarboximide.Secondary amine
Substituted dicarboximide.Tertiary amine
C1CCNCC1.c1ccc2c(c1)CNC2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HBr
null
null
null
Fc1ccc2c(C3CCNCC3)noc2c1.O=C1NC(=O)c2c(CCBr)cccc21>>O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5ab47f7791f64971b641945e6dcd0293
COCCBr.Fc1ccc2c(C3CCNCC3)noc2c1>>COCCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.C(=O)([O-])[O-].[K+].[K+].COCCBr.C(\C=C\C(=O)O)(=O)O>>C(\C=C\C(=O)O)(=O)O.COCCN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F
Br[CH2:4][CH2:3][O:2][CH3:1].[NH:5]1[CH2:6][CH2:7][CH:8]([c:9]2[n:10][o:11][c:12]3[cH:13][c:14]([F:15])[cH:16][cH:17][c:18]23)[CH2:19][CH2:20]1>>[CH3:1][O:2][CH2:3][CH2:4][N:5]1[CH2:6][CH2:7][CH:8]([c:9]2[n:10][o:11][c:12]3[cH:13][c:14]([F:15])[cH:16][cH:17][c:18]23)[CH2:19][CH2:20]1
COCCBr.Fc1ccc2c(C3CCNCC3)noc2c1
COCCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
C(C)#N.C(C)O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc2c(C3CCNCC3)noc2c1
Br-[CH2;D2;+0:1]-[C:2]-[#8:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[#8:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:6](-[C:5]-[C:4])-[C:7]-[C:8]
null
[]
null
null
null
null
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (3.75 gm, 17 mmol), K2CO3 (3 gm, 21.7 mmol), bromoethyl methyl ether (2.84 gm, 20.4 mmol) in acetonitrile (150 ml) was heated at reflux for 3.5 hr. The reaction was cooled. The inorganics were filtered and rinsed with DCM. The organic solution was concentrated d...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2oncc2c1
HBr
C(C)#N.C(C)O
null
null
COCCBr.Fc1ccc2c(C3CCNCC3)noc2c1>C(C)#N.C(C)O>COCCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6eac25b428c242fcae169939f1e30c6f
CC(=O)OCCCCBr.Fc1ccc2c(C3CCNCC3)noc2c1>>CC(=O)OCCCCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.C(=O)([O-])[O-].[K+].[K+].C(C)(=O)OCCCCBr.C(\C=C\C(=O)O)(=O)O>>C(\C=C\C(=O)O)(=O)O.C(C)(=O)OCCCCN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F
Br[CH2:8][CH2:7][CH2:6][CH2:5][O:4][C:2]([CH3:1])=[O:3].[NH:9]1[CH2:10][CH2:11][CH:12]([c:13]2[n:14][o:15][c:16]3[cH:17][c:18]([F:19])[cH:20][cH:21][c:22]23)[CH2:23][CH2:24]1>>[CH3:1][C:2](=[O:3])[O:4][CH2:5][CH2:6][CH2:7][CH2:8][N:9]1[CH2:10][CH2:11][CH:12]([c:13]2[n:14][o:15][c:16]3[cH:17][c:18]([F:19])[cH:20][cH:21]...
CC(=O)OCCCCBr.Fc1ccc2c(C3CCNCC3)noc2c1
CC(=O)OCCCCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
C(C)#N.C(C)O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc2c(C3CCNCC3)noc2c1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[C:4]-[C:5]-[N;H0;D3;+0:6](-[CH2;D2;+0:1]-[C:2]-[C:3])-[C:7]-[C:8]
null
[]
null
null
null
null
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (9.5 gm, 41 mmol), K2CO3 (7.2 m, 51 mmol), and 4-bromobutyl acetate (10 gm, 51 mmol) in acetonitrile (200 ml) was heated at reflux for 3½ hr. At the end of the reaction, the solution was cooled and filtered. The inorganic salt was washed with DCM (50 ml). The or...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2oncc2c1
HBr
C(C)#N.C(C)O
null
null
CC(=O)OCCCCBr.Fc1ccc2c(C3CCNCC3)noc2c1>C(C)#N.C(C)O>CC(=O)OCCCCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c0f8749e22164827b4b11ae7a7ae291f
CCN(CC)CC.O=C(O)/C=C/C(=O)O.OCCCCN1CCC(c2noc3cc(F)ccc23)CC1>>CCCCCCCCCC(=O)OCCCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCCO)C=C1.C(C)N(CC)CC.C(Cl)Cl.C(\C=C\C(=O)O)(=O)O>>C(\C=C\C(=O)O)(=O)O.C(CCCCCCCCC)(=O)OCCCCN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F
N([CH2:2][CH3:1])([CH2:6][CH3:3])[CH2:8][CH3:9].[C:10](=[O:11])([OH:35])/[CH:36]=[CH:37]/[C:38](=[O:39])[OH:40].[OH:12][CH2:13][CH2:14][CH2:15][CH2:16][N:17]1[CH2:18][CH2:19][CH:20]([c:21]2[n:22][o:23][c:24]3[cH:25][c:26]([F:27])[cH:28][cH:29][c:30]23)[CH2:31][CH2:32]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7]...
CCN(CC)CC.O=C(O)/C=C/C(=O)O.OCCCCN1CCC(c2noc3cc(F)ccc23)CC1
CCCCCCCCCC(=O)OCCCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
null
null
C(C)O
C-C Coupling
OtherReaction
751760910e5f360277c3f4d3befcb89bbe0e920df03a91877e36a8d024b51b87
c343030799bb933f3375c7d72f59363fd1b700abfc69826f97b066628943b37c
c1ccc2c(C3CCNCC3)noc2c1
[C;D1;H3:1]-[CH2;D2;+0:2]-N(-[CH2;D2;+0:3]-[CH3;D1;+0:4])-[CH2;D2;+0:5]-[CH3;D1;+0:6].[C:7]-[C:8]-[OH;D1;+0:9].[O;D1;H0:10]=[C;H0;D3;+0:11](-[OH;D1;+0:12])/[CH;D2;+0:13]=[C:14]/[C:15](=[O;D1;H0:16])-[O;D1;H1:17]>>[C:7]-[C:8]-[O;H0;D2;+0:9]-[C;H0;D3;+0:11](=[O;D1;H0:10])-[CH2;D2;+0:6]-[CH2;D2;+0:5]-[C:18]-[CH2;D2;+0:3]-...
null
[]
null
null
1
HOUR
To a solution of 4-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]butanol (2.0 gm, 6.84 mmol), triethylamine (1.0 gm, 10 mmol) in DCM (70 ml) decanoyl chloride (1.7 gm, 8.9 mmol) was added dropwise at room temperature. The mixture was stirred for 1 hr., then was concentrated to a crude solid. The solid was extracted...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol.Tertiary amine
Carboxylic acid.Ester
null
null
C1CC[NH]CC1.c1ccc2oncc2c1
null
C(C)O
null
1
CCN(CC)CC.O=C(O)/C=C/C(=O)O.OCCCCN1CCC(c2noc3cc(F)ccc23)CC1>C(C)O>CCCCCCCCCC(=O)OCCCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8a727adcde214391bd3c5969455176ae
CCCCCCCCCC(=O)Cl.OCCCN1CCC(c2noc3cc(F)ccc23)CC1>>CCCCCCCCCC(=O)OCCCN1CCC(c2noc3cc(F)ccc23)CC1
C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCO)C=C1.C(CCCCCCCCC)(=O)Cl>>C(\C=C\C(=O)O)(=O)O.C(CCCCCCCCC)(=O)OCCCN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F
Cl[C:10]([CH2:9][CH2:8][CH2:7][CH2:6][CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])=[O:11].[OH:12][CH2:13][CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH:19]([c:20]2[n:21][o:22][c:23]3[cH:24][c:25]([F:26])[cH:27][cH:28][c:29]23)[CH2:30][CH2:31]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][C:10](=[O:11])[O:12][CH2...
CCCCCCCCCC(=O)Cl.OCCCN1CCC(c2noc3cc(F)ccc23)CC1
CCCCCCCCCC(=O)OCCCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
C(Cl)Cl.C(C)O
Acylation
Schotten-Baumann to ester
6cefe709828c5bd4655f254e75d5dff9e8876e192e7dd47256c1bc0067bc5291
d8a7643b81ed07a6f633aa99465180dfa0565e61ae25aef36338ebb9837c9cef
c1ccc2c(C3CCNCC3)noc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[C:5]-[C:6]-[OH;D1;+0:7]>>[C:5]-[C:6]-[O;H0;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]
null
[]
null
null
20
MINUTE
To a solution 3-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]propanol (1.81 gm, 6.5 mmol) triethylamine (0.9 gm, 9.0 mmol) in DCM (45 ml) was added decanoyl chloride (1.5 gm, 7.8 mmol) dropwise at room temperature. The mixture was stirred for 20 minutes, then concentrated down to a crude solid. The solid was extra...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary alcohol
Ester
null
null
C1CC[NH]CC1.c1ccc2oncc2c1
HCl
C(Cl)Cl.C(C)O
null
0.333333
CCCCCCCCCC(=O)Cl.OCCCN1CCC(c2noc3cc(F)ccc23)CC1>C(Cl)Cl.C(C)O>CCCCCCCCCC(=O)OCCCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-44dfbbff125c48ba970c1659d05f896a
NN.O.O=C1NC(=O)c2c(CCN3CCC(c4noc5cc(F)ccc45)CC3)cccc21>>NCCN1CCC(c2noc3cc(F)ccc23)CC1.NCCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCC2=C3C(C(=O)NC3=O)=CC=C2)C=C1.O.NN.C(\C=C\C(=O)O)(=O)O.Cl>>C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1
[NH2:1][NH2:23].[OH2:29].O=[C:21]1[NH:20][C:36](=O)[c:30]2[c:27]1[c:26]([CH2:2][CH2:3][N:4]1[CH2:5][CH2:6][CH:7]([c:8]3[n:9][o:10][c:11]4[cH:12][c:13]([F:14])[cH:15][cH:16][c:17]34)[CH2:18][CH2:19]1)[cH:37][cH:32][cH:31]2>>[NH2:1][CH2:2][CH2:3][N:4]1[CH2:5][CH2:6][CH:7]([c:8]2[n:9][o:10][c:11]3[cH:12][c:13]([F:14])[cH:...
NN.O.O=C1NC(=O)c2c(CCN3CCC(c4noc5cc(F)ccc45)CC3)cccc21
NCCN1CCC(c2noc3cc(F)ccc23)CC1.NCCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
O.CO.C(C)O
Aromatic Heterocycle Formation
OtherReaction
06df55fe7c20d2715d727c9ec277605163a83d63b338374b860fa13df9ceedd9
5524a9ed289118e58677b024c9c4475283bf219d6776b1f22527577b82e343ea
c1ccc2c(C3CCNCC3)noc2c1.c1ccc2c(C3CCNCC3)noc2c1
O=[C;H0;D3;+0:1]1-[NH;D2;+0:2]-[C;H0;D3;+0:3](=O)-[c;H0;D3;+0:4]2:[c:5]:[cH;D2;+0:6]:[cH;D2;+0:7]:[c;H0;D3;+0:8](-[CH2;D2;+0:9]-[C:10]-[#7:11]):[c;H0;D3;+0:12]:2-1.[NH2;D1;+0:13]-[NH2;D1;+0:14].[OH2;D0;+0:15]>>[#7:11]-[C:10]-[CH2;D2;+0:9]-[NH2;D1;+0:13].[F;D1;H0:16]-[c;H0;D3;+0:6]1:[c:5]:[c;H0;D3;+0:4]2:[o;H0;D2;+0:15]...
null
[]
null
null
null
null
A mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethyl phthalimide (4.6 in, 11.7 mmol) and hydrazine monohydrate (1.17 gm, 23.4 mmol) in methanol (50 ml) was heated at reflux overnight. At the end of the reaction, methanol was removed to leave a crude solid. This was stirred with water (150 ml) and acid...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Unsubstituted dicarboximide
Aromatic halide.Primary amine.Primary amine.Tertiary amine
c1ccc2c(c1)CNC2
C1CC[NH]CC1.c1ccc2oncc2c1
C1CC[NH]CC1.c1ccc2oncc2c1.C1CC[NH]CC1.c1ccc2oncc2c1
null
O.CO.C(C)O
null
null
NN.O.O=C1NC(=O)c2c(CCN3CCC(c4noc5cc(F)ccc45)CC3)cccc21>O.CO.C(C)O>NCCN1CCC(c2noc3cc(F)ccc23)CC1.NCCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f34710d665c9438d879b93c90a0182d6
CC(=O)Cl.NCCN1CCC(c2noc3cc(F)ccc23)CC1>>NC(=O)CCCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.C(C)N(CC)CC.C(\C=C\C(=O)O)(=O)O.C(C)(=O)Cl>>C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCC(=O)N)C=C1
Cl[C:2](=[O:3])[CH3:4].[NH2:1][CH2:5][CH2:6][N:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18][cH:19][c:20]23)[CH2:21][CH2:22]1>>[NH2:1][C:2](=[O:3])[CH2:4][CH2:5][CH2:6][N:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18][cH:19][c:20]23)[CH2:21][CH2:22]1
CC(=O)Cl.NCCN1CCC(c2noc3cc(F)ccc23)CC1
NC(=O)CCCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
C(Cl)Cl.C(C)O
Acylation
OtherReaction
74356bef414ba31a0485b52d7495e90a08f4a5b89d028b8ec303ccdb6ed5504f
5d86061e72bfd6a9511ca0dd8b67e7f96dd93b070d7199a24f9e8328c94bd93b
c1ccc2c(C3CCNCC3)noc2c1
Cl-[C;H0;D3;+0:1](-[CH3;D1;+0:2])=[O;D1;H0:3].[#7:4]-[C:5]-[CH2;D2;+0:6]-[NH2;D1;+0:7]>>[#7:4]-[C:5]-[CH2;D2;+0:6]-[CH2;D2;+0:2]-[C;H0;D3;+0:1](-[NH2;D1;+0:7])=[O;D1;H0:3]
null
[]
null
null
4
HOUR
A mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.56 g, 9.7 mmol) and triethylamine (1.45 gm, 14.5 mmol) in DCM (50 ml) was treated with dropwise addition of acetyl chloride (1.0 gm, 12.7 mmol) at room temperature. The mixture was stirred for 4 hr at room temperature. The reaction mixture w...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Primary amide
null
null
C1CC[NH]CC1.c1ccc2oncc2c1
HCl
C(Cl)Cl.C(C)O
null
4
CC(=O)Cl.NCCN1CCC(c2noc3cc(F)ccc23)CC1>C(Cl)Cl.C(C)O>NC(=O)CCCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e7e61fdfcdac4dda8221a474935e3d54
COC(=O)Cl.NCCN1CCC(c2noc3cc(F)ccc23)CC1>>O=C(O)NCCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.C(C)N(CC)CC.C(\C=C\C(=O)O)(=O)O.ClC(=O)OC>>C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CCN(CC2)CCNC(O)=O)C=C1
C[O:11][C:10](Cl)=[O:9].[NH2:12][CH2:13][CH2:14][N:15]1[CH2:16][CH2:17][CH:18]([c:19]2[n:20][o:21][c:22]3[cH:23][c:24]([F:25])[cH:26][cH:27][c:28]23)[CH2:29][CH2:30]1>>[O:9]=[C:10]([OH:11])[NH:12][CH2:13][CH2:14][N:15]1[CH2:16][CH2:17][CH:18]([c:19]2[n:20][o:21][c:22]3[cH:23][c:24]([F:25])[cH:26][cH:27][c:28]23)[CH2:29...
COC(=O)Cl.NCCN1CCC(c2noc3cc(F)ccc23)CC1
O=C(O)NCCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
C(Cl)Cl.C(C)O
Acylation
OtherReaction
6c80fd18c280df460041be8a8c98767c9dba71f5f4f3f6ff808fe4bb8396e9cb
2b67592a38ea6fc1c1963f5b8261965724e5e16c9a8cee8da26ed8100d66dfbc
c1ccc2c(C3CCNCC3)noc2c1
C-[O;H0;D2;+0:1]-[C;H0;D3;+0:2](-Cl)=[O;D1;H0:3].[C:4]-[C:5]-[NH2;D1;+0:6]>>[C:4]-[C:5]-[NH;D2;+0:6]-[C;H0;D3;+0:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
1
HOUR
A mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.0 gm, 7.6 mmol) and triethylamine (1.0 gm, 10 mmol) in DCM (50 ml) was treated with methyl chloroformate (860 mg, 9.12 mmol) dropwise at room temperature. The mixture was stirred for 1 hr. The reaction mixture was diluted with DCM and washed...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine
Carbamic acid
null
null
C1CC[NH]CC1.c1ccc2oncc2c1
HCl
C(Cl)Cl.C(C)O
null
1
COC(=O)Cl.NCCN1CCC(c2noc3cc(F)ccc23)CC1>C(Cl)Cl.C(C)O>O=C(O)NCCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f4bc8b7e39bb44548882008d588dd63a
ClCCCN1CCCCC1.Fc1ccc2c(C3CCNCC3)noc2c1.O.O=C([O-])[O-]>>Fc1ccc2c(C3CCN(CCCN4CCCCC4)CC3)noc2c1.O=C(O)/C=C/C(=O)O.O=C(O)/C=C/C(=O)O
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.Cl.ClCCCN1CCCCC1.C(=O)([O-])[O-].[K+].[K+].O>>C(\C=C\C(=O)O)(=O)O.C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCN2CCCCC2)C=C1
Cl[CH2:11][CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18][CH2:19]1.[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][NH:10][CH2:20][CH2:21]3)[n:22][o:23][c:24]2[cH:25]1.[OH2:34].[O-:26][C:31](=[O:32])[O-:40]>>[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][N:10]([CH2:11][CH2:12][CH2:13][N:14]4[C...
ClCCCN1CCCCC1.Fc1ccc2c(C3CCNCC3)noc2c1.O.O=C([O-])[O-]
Fc1ccc2c(C3CCN(CCCN4CCCCC4)CC3)noc2c1.O=C(O)/C=C/C(=O)O.O=C(O)/C=C/C(=O)O
null
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC
C(C)#N
Acylation
OtherReaction
5abf4ce96638af1fef71fa30c86fff983bcc6ae0a81b871495c8ad14ff13da86
1e44655a39628ea3cd903509b7d5e10cb6ac6bc1b1eb03e5733de839f4a001b9
c1ccc2c(C3CCN(CCCN4CCCCC4)CC3)noc2c1
Cl-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8].[O-;H0;D1:9]-[C;H0;D3;+0:10](-[O-;H0;D1:11])=[O;D1;H0:12].[OH2;D0;+0:13]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:6](-[C:5]-[C:4])-[C:7]-[C:8].[O;D1;H0:12]=[C;H0;D3;+0:10](-[O;D1;H1:14])/[C:15]=[C:16]/[C:17](-[O;D1;H1:18])=[O;H0;D1;+0:9].[O;D1;H1:19]-[C:20...
null
[]
null
null
null
null
A mixture of 4-(6-fluoro-1,2-benzisoxazol-3-yl)piperidine (3.0 gm, 13.6 mmol), N-(3-chloropropyl)piperidine hydrochloride (4.05 gm, 20.4 mmol), K2CO3 (6 gm, 43.4 mmol), tetrabutyl-ammonium hydrogen sulfate (phase transfer catalyst, 2.3 gm) in acetonitrile (100 ml) and water (15 ml) was heated at reflux for 16 hr. The m...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Carboxylic acid.Carboxylic acid.Carboxylic acid.Carboxylic acid.Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]CC1.c1ccc2oncc2c1
null
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)#N
null
null
ClCCCN1CCCCC1.Fc1ccc2c(C3CCNCC3)noc2c1.O.O=C([O-])[O-]>S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)#N>Fc1ccc2c(C3CCN(CCCN4CCCCC4)CC3)noc2c1.O=C(O)/C=C/C(=O)O.O=C(O)/C=C/C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5b098cfa176148babb9f4997ef60a01a
CN(C)CCCCl.Fc1ccc2c(C3CCNCC3)noc2c1.O=C([O-])[O-]>>CN(C)CCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.Cl.CN(CCCCl)C.C(=O)([O-])[O-].[K+].[K+].C(\C=C\C(=O)O)(=O)O>>C(\C=C\C(=O)O)(=O)O.C(\C=C\C(=O)O)(=O)O.CN(CCCN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F)C
Cl[CH2:6][CH2:5][CH2:4][N:2]([CH3:1])[CH3:3].[NH:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18][cH:19][c:20]23)[CH2:21][CH2:22]1.[O-:23][C:24]([O-:25])=[O:29]>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][CH2:6][N:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18][cH...
CN(C)CCCCl.Fc1ccc2c(C3CCNCC3)noc2c1.O=C([O-])[O-]
CN(C)CCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
null
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC
C(C)#N.O.C(C)O
Acylation
OtherReaction
6e81dd2143b34ac8493b8c7a465af8abf3dc938c48f958db6f7d226ebb2c3120
5f494da60710a056b9f0e23ca9ed5ee350fb03b6598e6ff6e0034b17ff171889
c1ccc2c(C3CCNCC3)noc2c1
Cl-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8].[O-;H0;D1:9]-[C;H0;D3;+0:10](-[O-;H0;D1:11])=[O;H0;D1;+0:12]>>[C:4]-[C:5]-[N;H0;D3;+0:6](-[CH2;D2;+0:1]-[C:2]-[C:3])-[C:7]-[C:8].[O;D1;H1:13]-[C:14](=[O;H0;D1;+0:12])/[C:15]=[C:16]/[C;H0;D3;+0:10](=[O;H0;D1;+0:9])-[OH;D1;+0:11]
56.9
[{"value": 56.9, "product": "C(\\C=C\\C(=O)O)(=O)O.C(\\C=C\\C(=O)O)(=O)O.CN(CCCN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (3.05 gm, 13.8 mmol), 3-dimethylaminopropyl chloride hydrochloride (3.4 gm, 21 mmol), K2CO3 (6.2 gm 45 mmol), tetrabutylammonium hydrogen sulfate (phase transfer catalyst, 1.5 gm) in acetonitrile (100 ml) and water (50 ml) was heated at 60° C. overnight. The aqu...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Carboxylic acid.Carboxylic acid.Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2oncc2c1
null
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)#N.O.C(C)O
60
null
CN(C)CCCCl.Fc1ccc2c(C3CCNCC3)noc2c1.O=C([O-])[O-]>S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)#N.O.C(C)O>CN(C)CCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d802e192d083454a9e2106c1e317bb29
ClCCCOc1ccc2[nH]ccc2c1.Fc1ccc2c(C3CCNCC3)noc2c1>>Fc1ccc2c(C3CCN(CCCOc4ccc5[nH]ccc5c4)CC3)noc2c1
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.C(=O)([O-])[O-].[K+].[K+].ClCCCOC=1C=C2C=CNC2=CC1.CC#N>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCOC=2C=C3C=CNC3=CC2)C=C1
Cl[CH2:11][CH2:12][CH2:13][O:14][c:15]1[cH:16][cH:17][c:18]2[nH:19][cH:20][cH:21][c:22]2[cH:23]1.[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][NH:10][CH2:24][CH2:25]3)[n:26][o:27][c:28]2[cH:29]1>>[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][N:10]([CH2:11][CH2:12][CH2:13][O:14][c:15]4[cH:16][cH:17...
ClCCCOc1ccc2[nH]ccc2c1.Fc1ccc2c(C3CCNCC3)noc2c1
Fc1ccc2c(C3CCN(CCCOc4ccc5[nH]ccc5c4)CC3)noc2c1
null
null
O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc2c(C3CCN(CCCOc4ccc5[nH]ccc5c4)CC3)noc2c1
Cl-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:6](-[C:5]-[C:4])-[C:7]-[C:8]
123.4
[{"value": 123.4, "product": "FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCOC=2C=C3C=CNC3=CC2)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (2.6 g, 11.8 mmol), K2CO3 (1.6 g, 11.6 mmol), KI (200 mg), 5-(3-chloropropoxy)indole (2.2 g, 10.5 mmol) and CH3CN (100 ml) was stirred at reflux under N2 for 18 hours. The cooled reaction was poured into H2O and the aqueous mixture was extracted with EtOAc. The ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2[nH]ccc2c1.c1ccc2oncc2c1
HCl
O
null
null
ClCCCOc1ccc2[nH]ccc2c1.Fc1ccc2c(C3CCNCC3)noc2c1>O>Fc1ccc2c(C3CCN(CCCOc4ccc5[nH]ccc5c4)CC3)noc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-eebec035ef6e40b0b4a66840ba1b5bd7
ClCCCOc1cccc2[nH]ccc12.Fc1ccc2c(C3CCNCC3)noc2c1>>Fc1ccc2c(C3CCN(CCCOc4cccc5[nH]ccc45)CC3)noc2c1
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.C(=O)([O-])[O-].[K+].[K+].ClCCCOC1=C2C=CNC2=CC=C1.CC#N.C(=O)([O-])[O-].[K+].[K+]>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCOC2=C3C=CNC3=CC=C2)C=C1
Cl[CH2:11][CH2:12][CH2:13][O:14][c:15]1[cH:16][cH:17][cH:18][c:19]2[nH:20][cH:21][cH:22][c:23]12.[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][NH:10][CH2:24][CH2:25]3)[n:26][o:27][c:28]2[cH:29]1>>[F:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([CH:7]3[CH2:8][CH2:9][N:10]([CH2:11][CH2:12][CH2:13][O:14][c:15]4[cH:16][cH:17...
ClCCCOc1cccc2[nH]ccc12.Fc1ccc2c(C3CCNCC3)noc2c1
Fc1ccc2c(C3CCN(CCCOc4cccc5[nH]ccc45)CC3)noc2c1
null
null
O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1cc(OCCCN2CCC(c3noc4ccccc34)CC2)c2cc[nH]c2c1
Cl-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:6](-[C:5]-[C:4])-[C:7]-[C:8]
103.5
[{"value": 103.5, "product": "FC1=CC2=C(C(=NO2)C2CCN(CC2)CCCOC2=C3C=CNC3=CC=C2)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
68
HOUR
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisoxazole (3.5 g, 16 mmol), K2CO3 (2.2 g, 16 mmol), KI (200 mg), 4-(3-chloropropoxy)indole (3.0 g, 14 mmol) and CH3CN (100 ml) was stirred at reflux under N2 for 7 hours and then at ambient temperature for 68 hours. Reflux was resumed for an additional 6 hours whereupon a...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2[nH]ccc2c1.c1ccc2oncc2c1
HCl
O
null
68
ClCCCOc1cccc2[nH]ccc12.Fc1ccc2c(C3CCNCC3)noc2c1>O>Fc1ccc2c(C3CCN(CCCOc4cccc5[nH]ccc45)CC3)noc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-15941cc2a1ba4b54bcc2e6719487eb85
CC(=O)c1ccc(OCCCCl)c(O)c1.Fc1ccc2c(C3CCNCC3)nsc2c1>>CC(=O)c1ccc(OCCCN2CCC(c3nsc4cc(F)ccc34)CC2)c(O)c1
FC1=CC2=C(C(=NS2)C2CCNCC2)C=C1.ClCCCOC1=C(C=C(C=C1)C(C)=O)O.C(=O)(O)[O-].[Na+].CC#N>>FC1=CC2=C(C(=NS2)C2CCN(CC2)CCCOC2=C(C=C(C=C2)C(C)=O)O)C=C1
Cl[CH2:11][CH2:10][CH2:9][O:8][c:7]1[cH:6][cH:5][c:4]([C:2]([CH3:1])=[O:3])[cH:30][c:28]1[OH:29].[NH:12]1[CH2:13][CH2:14][CH:15]([c:16]2[n:17][s:18][c:19]3[cH:20][c:21]([F:22])[cH:23][cH:24][c:25]23)[CH2:26][CH2:27]1>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]([O:8][CH2:9][CH2:10][CH2:11][N:12]2[CH2:13][CH2:14][CH:15]...
CC(=O)c1ccc(OCCCCl)c(O)c1.Fc1ccc2c(C3CCNCC3)nsc2c1
CC(=O)c1ccc(OCCCN2CCC(c3nsc4cc(F)ccc34)CC2)c(O)c1
null
null
O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc(OCCCN2CCC(c3nsc4ccccc34)CC2)cc1
Cl-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[C:4]-[C:5]-[N;H0;D3;+0:6](-[CH2;D2;+0:1]-[C:2]-[C:3])-[C:7]-[C:8]
97
[{"value": 97.0, "product": "FC1=CC2=C(C(=NS2)C2CCN(CC2)CCCOC2=C(C=C(C=C2)C(C)=O)O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisothiazole (2.4 g, 10.1 mmol), 1-[4-(3-chloropropoxy)-3-hydroxyphenyl]ethanone (2.5 g, 11.1 mmol), NaHCO3 (0.94 g, 11.1 mmol), KI (100 mg) and CH3CN (100 ml) was stirred at reflux under N2 for 65 hours. The cooled reaction was poured into H2O and the aqueous mixture was ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
c1ccccc1.C1CC[NH]CC1.c1ccc2sncc2c1
HCl
O
null
null
CC(=O)c1ccc(OCCCCl)c(O)c1.Fc1ccc2c(C3CCNCC3)nsc2c1>O>CC(=O)c1ccc(OCCCN2CCC(c3nsc4cc(F)ccc34)CC2)c(O)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cfcfc056b45c4e1180bae03eef4d47d8
CS(=O)(=O)Cl.C[C@@H](CO)CN1CCC(c2noc3cc(F)ccc23)CC1>>C[C@@H](COS(C)(=O)=O)CN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)C[C@H](CO)C)C=C1.C(C)N(CC)CC.CS(=O)(=O)Cl>>CS(=O)(=O)OC[C@@H](CN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F)C
Cl[S:5]([CH3:6])(=[O:7])=[O:8].[CH3:1][C@@H:2]([CH2:3][OH:4])[CH2:9][N:10]1[CH2:11][CH2:12][CH:13]([c:14]2[n:15][o:16][c:17]3[cH:18][c:19]([F:20])[cH:21][cH:22][c:23]23)[CH2:24][CH2:25]1>>[CH3:1][C@@H:2]([CH2:3][O:4][S:5]([CH3:6])(=[O:7])=[O:8])[CH2:9][N:10]1[CH2:11][CH2:12][CH:13]([c:14]2[n:15][o:16][c:17]3[cH:18][c:1...
CS(=O)(=O)Cl.C[C@@H](CO)CN1CCC(c2noc3cc(F)ccc23)CC1
C[C@@H](COS(C)(=O)=O)CN1CCC(c2noc3cc(F)ccc23)CC1
null
null
C(Cl)Cl
Acylation
Formation of Sulfonic Esters
2fa969eb2c954bb96793348a1b2335ec63fbd290dadec6e3e02295e1768e64cf
cb77b899e4adf980b1def97230ef2861660fd7f9602260ec64747d9afd3a795a
c1ccc2c(C3CCNCC3)noc2c1
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].[C:5]-[C:6]-[OH;D1;+0:7]>>[C:5]-[C:6]-[O;H0;D2;+0:7]-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4]
null
[]
null
null
1
HOUR
To a mixture of (R)-(−)-3-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]-2-methyl-1-propanol (7.26 gm, 24.8 mmoles), triethylamine (3ml, 30 mmoles) in methylene chloride (DCM, 120 ml), methanesulfonyl chloride (3.13 gm, 27.3 moles) was added dropwise at 0° C. The mixture was stirred at room temperature for 1 hr., t...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Sulfonyl halide
Mesylate
null
null
C1CC[NH]CC1.c1ccc2oncc2c1
HCl
C(Cl)Cl
null
1
CS(=O)(=O)Cl.C[C@@H](CO)CN1CCC(c2noc3cc(F)ccc23)CC1>C(Cl)Cl>C[C@@H](COS(C)(=O)=O)CN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d78e644e407743eda8c6368ad1321293
CC(C)(CO)CBr.Fc1ccc2c(C3CCNCC3)noc2c1.O=C([O-])[O-]>>CC(C)(CO)CN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
FC1=CC2=C(C(=NO2)C2CCNCC2)C=C1.C(=O)([O-])[O-].[K+].[K+].BrCC(CO)(C)C>>C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CCN(CC2)CC(CO)(C)C)C=C1
Br[CH2:6][C:2]([CH3:1])([CH2:4][OH:5])[CH3:27].[NH:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18][cH:19][c:20]23)[CH2:21][CH2:22]1.[O-:23][C:28]([O-:25])=[O:29]>>[CH3:1][C:2]([CH3:3])([CH2:4][OH:5])[CH2:6][N:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18]...
CC(C)(CO)CBr.Fc1ccc2c(C3CCNCC3)noc2c1.O=C([O-])[O-]
CC(C)(CO)CN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
null
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC
O.C(C)#N
Acylation
OtherReaction
6e81dd2143b34ac8493b8c7a465af8abf3dc938c48f958db6f7d226ebb2c3120
5f494da60710a056b9f0e23ca9ed5ee350fb03b6598e6ff6e0034b17ff171889
c1ccc2c(C3CCNCC3)noc2c1
Br-[CH2;D2;+0:1]-[C;H0;D4;+0:2](-[C;D1;H3:3])(-[CH3;D1;+0:4])-[C:5]-[O;D1;H1:6].[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11].[O-;H0;D1:12]-[C;H0;D3;+0:13](-[O-;H0;D1:14])=[O;D1;H0:15]>>[C:7]-[C:8]-[N;H0;D3;+0:9](-[CH2;D2;+0:1]-[C;H0;D4;+0:2](-[C;D1;H3:3])(-[C;D1;H3:16])-[C:5]-[O;D1;H1:6])-[C:10]-[C:11].[O;D1;H0:15]=[C;H0;D3;...
null
[]
null
null
null
null
A mixture of 4-(6-fluoro-1,2-benzisoxazol-3-yl)piperidine (3.0 gm, 13.6 mmoles), K2CO3 (12.5 gm, 17.5 mmoles), 3-bromo-2,2-dimethyl-1-propanol (3 gm, 21 mmoles, 1.5 eq.), tetrabutylammonium hydrogen sulfate (1 gm, phase transfer catalyst) in water (5 ml) and acetonitrile (150 ml) was heated at reflux for 43 days. TLC s...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Carboxylic acid.Carboxylic acid.Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2oncc2c1
Br-
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.O.C(C)#N
null
null
CC(C)(CO)CBr.Fc1ccc2c(C3CCNCC3)noc2c1.O=C([O-])[O-]>S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.O.C(C)#N>CC(C)(CO)CN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-aec7caf706e040a6bfae5c1b2f424356
CS(=O)(=O)Cl.C[C@H](CO)CN1CCC(c2noc3cc(F)ccc23)CC1>>C[C@H](COS(C)(=O)=O)CN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)C[C@@H](CO)C)C=C1.C(C)N(CC)CC.CS(=O)(=O)Cl>>CS(=O)(=O)OC[C@H](CN1CCC(CC1)C1=NOC2=C1C=CC(=C2)F)C
Cl[S:5]([CH3:6])(=[O:7])=[O:8].[CH3:1][C@H:2]([CH2:3][OH:4])[CH2:9][N:10]1[CH2:11][CH2:12][CH:13]([c:14]2[n:15][o:16][c:17]3[cH:18][c:19]([F:20])[cH:21][cH:22][c:23]23)[CH2:24][CH2:25]1>>[CH3:1][C@H:2]([CH2:3][O:4][S:5]([CH3:6])(=[O:7])=[O:8])[CH2:9][N:10]1[CH2:11][CH2:12][CH:13]([c:14]2[n:15][o:16][c:17]3[cH:18][c:19]...
CS(=O)(=O)Cl.C[C@H](CO)CN1CCC(c2noc3cc(F)ccc23)CC1
C[C@H](COS(C)(=O)=O)CN1CCC(c2noc3cc(F)ccc23)CC1
null
null
ClCCl
Acylation
Formation of Sulfonic Esters
2fa969eb2c954bb96793348a1b2335ec63fbd290dadec6e3e02295e1768e64cf
cb77b899e4adf980b1def97230ef2861660fd7f9602260ec64747d9afd3a795a
c1ccc2c(C3CCNCC3)noc2c1
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].[C:5]-[C:6]-[OH;D1;+0:7]>>[C:5]-[C:6]-[O;H0;D2;+0:7]-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4]
null
[]
null
null
1
HOUR
To a mixture of (S)-(+)-3-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]-2-methyl-1-propanol (8.8 gm, 30 mmoles), triethylamine (3.2 gm, 32 mmoles) in dichloromethane (DCM, 150 ml), methanesulfonyl chloride (4 gm, 35 mmoles) was added dropwise at 0° C. over 10 minutes. The mixture was stirred at room temperature fo...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Sulfonyl halide
Mesylate
null
null
C1CC[NH]CC1.c1ccc2oncc2c1
HCl
ClCCl
null
1
CS(=O)(=O)Cl.C[C@H](CO)CN1CCC(c2noc3cc(F)ccc23)CC1>ClCCl>C[C@H](COS(C)(=O)=O)CN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7a5a5ee8a3f740d1ac15cb2fc748681b
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(Cl)c(Cl)cc21>>O=C1c2cc(Cl)c(Cl)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.ClC=1C=C2C(C(=O)OC2=O)=CC1Cl>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC(=C(C3)Cl)Cl)=O)C=C1
[NH2:13][CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH:19]([c:20]2[n:21][o:22][c:23]3[cH:24][c:25]([F:26])[cH:27][cH:28][c:29]23)[CH2:30][CH2:31]1.O1[C:2](=[O:1])[c:3]2[cH:4][c:5]([Cl:6])[c:7]([Cl:8])[cH:9][c:10]2[C:11]1=[O:12]>>[O:1]=[C:2]1[c:3]2[cH:4][c:5]([Cl:6])[c:7]([Cl:8])[cH:9][c:10]2[C:11](=[O:12])[N:13]1[CH2:14][C...
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(Cl)c(Cl)cc21
O=C1c2cc(Cl)c(Cl)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
C(Cl)Cl
Acylation
Phthalic anhydride to phthalimide
c3c986d6e09320348d40a4a59ca107882ce771f249842049dc55e55f334c675b
2bbbf7b24648445e31d33a2a26f8618c2067bd23957587cc459f3c45a03ed48a
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10]-1:[c:11]>>[C:1]-[C:2]-[N;H0;D3;+0:3]1-[C;H0;D3;+0:5](=[O;D1;H0:4])-[c:10](:[c:11]):[c:8](:[c:9])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
null
[]
null
null
2
HOUR
A mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.83 gm, 10.7 mmol) and 4,5-dichlorophthalic anhydride (2.56 gm, 11.93 mmol, 1.1 eq) in methylene chloride (100 ml, DCM) was stirred for 2 h, white solids precipitated and the TLC showed disappearance of the starting material. The solvent was ...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Primary amine
Substituted dicarboximide
c1ccc2c(c1)COC2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HO-
C(Cl)Cl
null
2
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(Cl)c(Cl)cc21>C(Cl)Cl>O=C1c2cc(Cl)c(Cl)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-53f8ae7ab9224b6e8cb83e5ed899aaa3
Fc1ccc2c(C3CCNCC3)nsc2c1.O=C1c2ccccc2C(=O)N1CCBr>>O=C1c2ccccc2C(=O)N1CCN1CCC(c2nsc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NS2)C2CCNCC2)C=C1.C([O-])([O-])=O.[K+].[K+].BrCCN1C(C=2C(C1=O)=CC=CC2)=O>>FC1=CC2=C(C(=NS2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC=CC3)=O)C=C1
[NH:14]1[CH2:15][CH2:16][CH:17]([c:18]2[n:19][s:20][c:21]3[cH:22][c:23]([F:24])[cH:25][cH:26][c:27]23)[CH2:28][CH2:29]1.Br[CH2:13][CH2:12][N:11]1[C:2](=[O:1])[c:3]2[cH:4][cH:5][cH:6][cH:7][c:8]2[C:9]1=[O:10]>>[O:1]=[C:2]1[c:3]2[cH:4][cH:5][cH:6][cH:7][c:8]2[C:9](=[O:10])[N:11]1[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH...
Fc1ccc2c(C3CCNCC3)nsc2c1.O=C1c2ccccc2C(=O)N1CCBr
O=C1c2ccccc2C(=O)N1CCN1CCC(c2nsc3cc(F)ccc23)CC1
null
null
C(C)#N
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0240b8450ff2c489d02f5f0d90bc953079d7a3ab239d35a03f26392fc248b4ef
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
O=C1c2ccccc2C(=O)N1CCN1CCC(c2nsc3ccccc23)CC1
Br-[CH2;D2;+0:1]-[C:2]-[#7:3](-[C:4]=[O;D1;H0:5])-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]>>[C:8]-[C:9]-[N;H0;D3;+0:10](-[CH2;D2;+0:1]-[C:2]-[#7:3](-[C:4]=[O;D1;H0:5])-[C:6]=[O;D1;H0:7])-[C:11]-[C:12]
null
[]
null
null
null
null
A stirred mixture of 6-fluoro-3-(4-piperidinyl)-1,2-benzisothiazole (4.72 g, 0.02 mole), potassium carbonate (4.14 g, 0.03 mole) and N-(2-bromoethyl)phthalimide (6.35 g, 0.0025 mole) in 200 ml of acetonitrile is heated at reflux for 4 hours. The solids are then removed by filtration and the filtrate is concentrated und...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2sncc2c1
HBr
C(C)#N
null
null
Fc1ccc2c(C3CCNCC3)nsc2c1.O=C1c2ccccc2C(=O)N1CCBr>C(C)#N>O=C1c2ccccc2C(=O)N1CCN1CCC(c2nsc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9aed2845cc6048e8a7650bf7674284d6
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2c(Cl)ccc(Cl)c21>>O=C1c2c(Cl)ccc(Cl)c2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.ClC1=C2C(C(=O)OC2=O)=C(C=C1)Cl>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=C(C=CC3Cl)Cl)=O)C=C1
[NH2:13][CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH:19]([c:20]2[n:21][o:22][c:23]3[cH:24][c:25]([F:26])[cH:27][cH:28][c:29]23)[CH2:30][CH2:31]1.O1[C:2](=[O:1])[c:3]2[c:4]([Cl:5])[cH:6][cH:7][c:8]([Cl:9])[c:10]2[C:11]1=[O:12]>>[O:1]=[C:2]1[c:3]2[c:4]([Cl:5])[cH:6][cH:7][c:8]([Cl:9])[c:10]2[C:11](=[O:12])[N:13]1[CH2:14][C...
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2c(Cl)ccc(Cl)c21
O=C1c2c(Cl)ccc(Cl)c2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
ClCCl
Acylation
Phthalic anhydride to phthalimide
c3c986d6e09320348d40a4a59ca107882ce771f249842049dc55e55f334c675b
2bbbf7b24648445e31d33a2a26f8618c2067bd23957587cc459f3c45a03ed48a
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10]-1:[c:11]>>[C:1]-[C:2]-[N;H0;D3;+0:3]1-[C;H0;D3;+0:5](=[O;D1;H0:4])-[c:10](:[c:11]):[c:8](:[c:9])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
null
[]
null
null
1
HOUR
A mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.44 gm, 9.24 mmoles) and 3,6-dichlorophthalic anhydride (2.01 gm; 9.27 mmoles) in dichloromethane (DCM, 50 ml) was stirred at room temperature for 1 hr. White precipitates formed and the TLC of the reaction mixture showed that there was no st...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Primary amine
Substituted dicarboximide
c1ccc2c(c1)COC2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HO-
ClCCl
null
1
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2c(Cl)ccc(Cl)c21>ClCCl>O=C1c2c(Cl)ccc(Cl)c2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3b0ed7012d3c4352aefc14fd34658495
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(Cl)ccc21>>O=C1c2ccc(Cl)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.ClC=1C=C2C(C(=O)OC2=O)=CC1>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC(=CC3)Cl)=O)C=C1
[NH2:12][CH2:13][CH2:14][N:15]1[CH2:16][CH2:17][CH:18]([c:19]2[n:20][o:21][c:22]3[cH:23][c:24]([F:25])[cH:26][cH:27][c:28]23)[CH2:29][CH2:30]1.O1[C:2](=[O:1])[c:3]2[cH:4][cH:5][c:6]([Cl:7])[cH:8][c:9]2[C:10]1=[O:11]>>[O:1]=[C:2]1[c:3]2[cH:4][cH:5][c:6]([Cl:7])[cH:8][c:9]2[C:10](=[O:11])[N:12]1[CH2:13][CH2:14][N:15]1[CH...
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(Cl)ccc21
O=C1c2ccc(Cl)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
ClCCl
Acylation
Phthalic anhydride to phthalimide
c3c986d6e09320348d40a4a59ca107882ce771f249842049dc55e55f334c675b
2bbbf7b24648445e31d33a2a26f8618c2067bd23957587cc459f3c45a03ed48a
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10]-1:[c:11]>>[C:1]-[C:2]-[N;H0;D3;+0:3]1-[C;H0;D3;+0:5](=[O;D1;H0:4])-[c:10](:[c:11]):[c:8](:[c:9])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
null
[]
null
null
3
HOUR
A stirred mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.63 g, 0.01 mole) and 4-chlorophthalic anhydride (1.82 g, 0.01 mole) in dichloromethane (100 ml) is stirred at room temperature for 3 hours. The solvent is removed under reduced pressure and the residual material is purified by flash ...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Primary amine
Substituted dicarboximide
c1ccc2c(c1)COC2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HO-
ClCCl
null
3
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(Cl)ccc21>ClCCl>O=C1c2ccc(Cl)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6e4a7b80558741188209f2cf0424ce21
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)c1cccc(F)c1C(=O)O>>O=C1c2cccc(F)c2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.FC1=C(C(C(=O)O)=CC=C1)C(=O)O.C1(CCCCC1)N=C=NC1CCCCC1>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=C(C=CC3)F)=O)C=C1
[NH2:12][CH2:13][CH2:14][N:15]1[CH2:16][CH2:17][CH:18]([c:19]2[n:20][o:21][c:22]3[cH:23][c:24]([F:25])[cH:26][cH:27][c:28]23)[CH2:29][CH2:30]1.O[C:2](=[O:1])[c:3]1[cH:4][cH:5][cH:6][c:7]([F:8])[c:9]1[C:10](O)=[O:11]>>[O:1]=[C:2]1[c:3]2[cH:4][cH:5][cH:6][c:7]([F:8])[c:9]2[C:10](=[O:11])[N:12]1[CH2:13][CH2:14][N:15]1[CH2...
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)c1cccc(F)c1C(=O)O
O=C1c2cccc(F)c2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
ClCCl
Acylation
OtherReaction
03989296fe7fd00d3061010c1aadbbfb4b9eaa9ca91856790fffb1e1bf4b4c50
b7eb222f11e89f2ccff57aab9a5106ae4173f0ba94ac518e1a9f3b22a378531d
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;H0;D3;+0:6](-O)=[O;D1;H0:7]):[c:8].[C:9]-[C:10]-[NH2;D1;+0:11]>>[C:9]-[C:10]-[N;H0;D3;+0:11]1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](:[c:8])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
null
[]
null
null
18
HOUR
A mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.37 gm, 8.98 mmoles), 3-fluorophthalic acid (1.82 in, 9.9 moles) and dicyclohexylcarbodiimide (DCC, 5.5 gm, 26.7 mmoles, 2.6 eq) in dichloromethane (DCM, 250 ml) was stirred at room temperature for 18 hrs. The solids were filtered off. The or...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid.Primary amine
Substituted dicarboximide
null
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HO-
ClCCl
null
18
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)c1cccc(F)c1C(=O)O>ClCCl>O=C1c2cccc(F)c2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7639107c90d449fe9f91df6fcf8fe0ee
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(F)ccc21>>O=C1c2ccc(F)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.FC=1C=C2C(C(=O)OC2=O)=CC1>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC(=CC3)F)=O)C=C1
[NH2:12][CH2:13][CH2:14][N:15]1[CH2:16][CH2:17][CH:18]([c:19]2[n:20][o:21][c:22]3[cH:23][c:24]([F:25])[cH:26][cH:27][c:28]23)[CH2:29][CH2:30]1.O1[C:2](=[O:1])[c:3]2[cH:4][cH:5][c:6]([F:7])[cH:8][c:9]2[C:10]1=[O:11]>>[O:1]=[C:2]1[c:3]2[cH:4][cH:5][c:6]([F:7])[cH:8][c:9]2[C:10](=[O:11])[N:12]1[CH2:13][CH2:14][N:15]1[CH2:...
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(F)ccc21
O=C1c2ccc(F)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
ClCCl
Acylation
Phthalic anhydride to phthalimide
c3c986d6e09320348d40a4a59ca107882ce771f249842049dc55e55f334c675b
2bbbf7b24648445e31d33a2a26f8618c2067bd23957587cc459f3c45a03ed48a
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10]-1:[c:11]>>[C:1]-[C:2]-[N;H0;D3;+0:3]1-[C;H0;D3;+0:5](=[O;D1;H0:4])-[c:10](:[c:11]):[c:8](:[c:9])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
null
[]
null
null
4
HOUR
A stirred mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.63 g, 0.01 mole) and 4-fluorophthalic anhydride (1.83 g, 0.011 mole) in dichloromethane (100 ml) is stirred at room temperature for 4 hours. The solvent is then removed under reduced pressure and the residual solids are purified by f...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Primary amine
Substituted dicarboximide
c1ccc2c(c1)COC2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HO-
ClCCl
null
4
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc(F)ccc21>ClCCl>O=C1c2ccc(F)cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6b40f52e296841cf8e544064850b09d8
Cc1ccc2c(c1)C(=O)OC2=O.NCCN1CCC(c2noc3cc(F)ccc23)CC1>>Cc1ccc2c(c1)C(=O)N(CCN1CCC(c3noc4cc(F)ccc34)CC1)C2=O
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.CC=1C=C2C(C(=O)OC2=O)=CC1.C1(CCCCC1)N=C=NC1CCCCC1>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC(=CC3)C)=O)C=C1
O1[C:8](=[O:9])[c:6]2[c:5]([cH:4][cH:3][c:2]([CH3:1])[cH:7]2)[C:29]1=[O:30].[NH2:10][CH2:11][CH2:12][N:13]1[CH2:14][CH2:15][CH:16]([c:17]2[n:18][o:19][c:20]3[cH:21][c:22]([F:23])[cH:24][cH:25][c:26]23)[CH2:27][CH2:28]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[C:8](=[O:9])[N:10]([CH2:11][CH2:12][N:13]1[CH2:14][CH2...
Cc1ccc2c(c1)C(=O)OC2=O.NCCN1CCC(c2noc3cc(F)ccc23)CC1
Cc1ccc2c(c1)C(=O)N(CCN1CCC(c3noc4cc(F)ccc34)CC1)C2=O
null
null
ClCCl
Acylation
Phthalic anhydride to phthalimide
c3c986d6e09320348d40a4a59ca107882ce771f249842049dc55e55f334c675b
2bbbf7b24648445e31d33a2a26f8618c2067bd23957587cc459f3c45a03ed48a
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10]-1:[c:11]>>[C:1]-[C:2]-[N;H0;D3;+0:3]1-[C;H0;D3;+0:5](=[O;D1;H0:4])-[c:10](:[c:11]):[c:8](:[c:9])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
17.7
[{"value": 17.7, "product": "FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC(=CC3)C)=O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.44 gm, 9.24 mmoles), 4-methylphthalic anhydride (1.76 gm, 10.8 moles) and dicyclohexylcarbodiimide (2.1 gm, 1.0 moles) in dichloromethane (DCM, 100 ml) was stirred at room temperature for 2 hr. The insolubles were filtered off. The DCM solut...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Primary amine
Substituted dicarboximide
c1ccc2c(c1)COC2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HO-
ClCCl
null
2
Cc1ccc2c(c1)C(=O)OC2=O.NCCN1CCC(c2noc3cc(F)ccc23)CC1>ClCCl>Cc1ccc2c(c1)C(=O)N(CCN1CCC(c3noc4cc(F)ccc34)CC1)C2=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2f53caabb6c3450d950e9dfb4b5e9cc7
COc1ccc2c(c1)C(=O)OC2=O.NCCN1CCC(c2noc3cc(F)ccc23)CC1>>COc1ccc2c(c1)C(=O)N(CCN1CCC(c3noc4cc(F)ccc34)CC1)C2=O
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.COC=1C=C2C(C(=O)OC2=O)=CC1>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC(=CC3)OC)=O)C=C1
O1[C:9](=[O:10])[c:7]2[c:6]([cH:5][cH:4][c:3]([O:2][CH3:1])[cH:8]2)[C:30]1=[O:31].[NH2:11][CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH:17]([c:18]2[n:19][o:20][c:21]3[cH:22][c:23]([F:24])[cH:25][cH:26][c:27]23)[CH2:28][CH2:29]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[C:9](=[O:10])[N:11]([CH2:12][CH2:13][N:14]1...
COc1ccc2c(c1)C(=O)OC2=O.NCCN1CCC(c2noc3cc(F)ccc23)CC1
COc1ccc2c(c1)C(=O)N(CCN1CCC(c3noc4cc(F)ccc34)CC1)C2=O
null
null
ClCCl
Acylation
Phthalic anhydride to phthalimide
c3c986d6e09320348d40a4a59ca107882ce771f249842049dc55e55f334c675b
2bbbf7b24648445e31d33a2a26f8618c2067bd23957587cc459f3c45a03ed48a
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10]-1:[c:11]>>[C:1]-[C:2]-[N;H0;D3;+0:3]1-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10](:[c:11])-[C;H0;D3;+0:5]-1=[O;D1;H0:4]
null
[]
null
null
3
HOUR
A stirred mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.63 g, 0.01 mole) and 4-methoxyphthalic anhydride (1.78 g, 0.01 mole) in dichloromethane (100 ml) is stirred at room temperature for 3 hours. The solvent is then removed under reduced pressure and the residual material is purified by ...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Primary amine
Substituted dicarboximide
c1ccc2c(c1)COC2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HO-
ClCCl
null
3
COc1ccc2c(c1)C(=O)OC2=O.NCCN1CCC(c2noc3cc(F)ccc23)CC1>ClCCl>COc1ccc2c(c1)C(=O)N(CCN1CCC(c3noc4cc(F)ccc34)CC1)C2=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0b42a3522df94a06bdc0e5cfb8737820
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc([N+](=O)[O-])ccc21>>O=C1c2ccc([N+](=O)[O-])cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN)C=C1.[N+](=O)([O-])C=1C=C2C(C(=O)OC2=O)=CC1>>FC1=CC2=C(C(=NO2)C2CCN(CC2)CCN2C(C=3C(C2=O)=CC(=CC3)[N+](=O)[O-])=O)C=C1
[NH2:14][CH2:15][CH2:16][N:17]1[CH2:18][CH2:19][CH:20]([c:21]2[n:22][o:23][c:24]3[cH:25][c:26]([F:27])[cH:28][cH:29][c:30]23)[CH2:31][CH2:32]1.O1[C:2](=[O:1])[c:3]2[cH:4][cH:5][c:6]([N+:7](=[O:8])[O-:9])[cH:10][c:11]2[C:12]1=[O:13]>>[O:1]=[C:2]1[c:3]2[cH:4][cH:5][c:6]([N+:7](=[O:8])[O-:9])[cH:10][c:11]2[C:12](=[O:13])[...
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc([N+](=O)[O-])ccc21
O=C1c2ccc([N+](=O)[O-])cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
null
null
ClCCl
Acylation
Phthalic anhydride to phthalimide
c3c986d6e09320348d40a4a59ca107882ce771f249842049dc55e55f334c675b
2bbbf7b24648445e31d33a2a26f8618c2067bd23957587cc459f3c45a03ed48a
O=C1c2ccccc2C(=O)N1CCN1CCC(c2noc3ccccc23)CC1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10]-1:[c:11]>>[C:1]-[C:2]-[N;H0;D3;+0:3]1-[C;H0;D3;+0:5](=[O;D1;H0:4])-[c:10](:[c:11]):[c:8](:[c:9])-[C;H0;D3;+0:6]-1=[O;D1;H0:7]
null
[]
null
null
3
HOUR
A stirred mixture of 2-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]ethylamine (2.63 g, 0.01 mole) and 4-nitrophthalic anhydride (1.93 g, 0.01 mole) in dichloromethane (200 ml) is stirred at room temperature for 3 hours. The solvent is then removed under reduced pressure and the residual material is purified by fl...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Primary amine
Substituted dicarboximide
c1ccc2c(c1)COC2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1.c1ccc2oncc2c1
HO-
ClCCl
null
3
NCCN1CCC(c2noc3cc(F)ccc23)CC1.O=C1OC(=O)c2cc([N+](=O)[O-])ccc21>ClCCl>O=C1c2ccc([N+](=O)[O-])cc2C(=O)N1CCN1CCC(c2noc3cc(F)ccc23)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-24d57af412c04f3eb1d3565ef87c50ca
CCOC(=O)CCN1CCC(c2noc3cc(F)ccc23)CC1.CCOC(C)=O>>CC(C)(O)CCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
[NH4+].[Cl-].CCOC(=O)C.FC1=CC2=C(C(=NO2)C2CCN(CC2)CCC(=O)OCC)C=C1.C[Mg]Br>>C(\C=C\C(=O)O)(=O)O.FC1=CC2=C(C(=NO2)C2CCN(CC2)CCC(C)(O)C)C=C1
C([CH3:3])[O:4][C:2]([CH2:5][CH2:6][N:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([F:17])[cH:18][cH:19][c:20]23)[CH2:21][CH2:22]1)=[O:23].[CH2:24]([O:25][C:28]([CH3:27])=[O:29])[CH3:26]>>[CH3:1][C:2]([CH3:3])([OH:4])[CH2:5][CH2:6][N:7]1[CH2:8][CH2:9][CH:10]([c:11]2[n:12][o:13][c:14]3[cH:15][c:16]([...
CCOC(=O)CCN1CCC(c2noc3cc(F)ccc23)CC1.CCOC(C)=O
CC(C)(O)CCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
null
null
O1CCCC1
Functional Group Addition
OtherReaction
07e99f91e500affa0451dbbfb1ccdfc6c2bf1d992b11b74db56debe2dbd4b3e4
15308189f1479c7a0725eea178834fcdf99915b1d89a0f1b88a28657dab684ab
c1ccc2c(C3CCNCC3)noc2c1
[CH3;D1;+0:1]-[CH2;D2;+0:2]-[O;H0;D2;+0:3]-[C;H0;D3;+0:4](-[CH3;D1;+0:5])=[O;D1;H0:6].[C:7]-[C:8]-[C;H0;D3;+0:9](=[O;H0;D1;+0:10])-[O;H0;D2;+0:11]-C-[CH3;D1;+0:12]>>[C:7]-[C:8]-[C;H0;D4;+0:9](-[C;D1;H3:13])(-[CH3;D1;+0:12])-[OH;D1;+0:11].[O;D1;H0:6]=[C;H0;D3;+0:4](-[O;D1;H1:14])/[CH;D2;+0:5]=[CH;D2;+0:1]/[C;H0;D3;+0:2]...
null
[]
null
null
16
HOUR
To a solution of ethyl 3-[4-(6-fluoro-1,2-benzisoxazol-3-yl)-1-piperidinyl]propionate (3.21 gm, 10 mmoles) in tetrahydrofuran (THF, 100 ml), methylmagnesium bromide (10 ml, 30 moles, 3M solution in ether) was added dropwise over 15 minutes at room temperature under N2. The resulting mixture was stirred for 16 hours. Th...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Carboxylic acid.Carboxylic acid.Tertiary alcohol
null
null
C1CC[NH]CC1.c1ccc2oncc2c1
Other
O1CCCC1
null
16
CCOC(=O)CCN1CCC(c2noc3cc(F)ccc23)CC1.CCOC(C)=O>O1CCCC1>CC(C)(O)CCN1CCC(c2noc3cc(F)ccc23)CC1.O=C(O)/C=C/C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-16738fd4d2a14dc786bb52e64ff9fd58
CCOCCl.Nc1cccc(O)c1>>CCOCOc1cccc(N)c1
C(C)OCCl.[H-].[Na+].NC=1C=C(C=CC1)O>>C(C)OCOC=1C=C(C=CC1)N
Cl[CH2:4][O:3][CH2:2][CH3:1].[OH:5][c:6]1[cH:7][cH:8][cH:9][c:10]([NH2:11])[cH:12]1>>[CH3:1][CH2:2][O:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]([NH2:11])[cH:12]1
CCOCCl.Nc1cccc(O)c1
CCOCOc1cccc(N)c1
null
null
C(C)#N
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
6e90ffbf0683e1a3ee55c5e3ea453aefc5ddd369c0150ed0150f9546d7e47f4f
efd670663709b79afcad1306da9f69b33a0147cfa3639ca4c0b54b35ef4b1852
c1ccccc1
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3].[OH;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C:3]-[#8:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]
null
[]
0
CELSIUS
3
HOUR
A dispersion of 12 g (274.9 mmol) of sodium hydride (55% in oil) was added portionwise at 0° C. to a solution of 20.0 g (183.3 mmol) of 3-aminophenol in 450 mL of dried acetonitrile. The mixture was then allowed to agitate at 0° C. for 3 hours. A solution of 25 g (210.8 mmol) of chloromethyl ethyl ether in 30 mL of ace...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ether.Aromatic alcohol
Ether.Ether
null
null
c1ccccc1
HCl
C(C)#N
0
3
CCOCCl.Nc1cccc(O)c1>C(C)#N>CCOCOc1cccc(N)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b608a34733c04a159168cf9668226fb4
O=[N+]([O-])[O-].[Al+3]>>O=[N+]([O-])[O-].[Al+3]
O.[N+](=O)([O-])[O-].[Al+3].[N+](=O)([O-])[O-].[N+](=O)([O-])[O-]>>[N+](=O)([O-])[O-].[Al+3].[N+](=O)([O-])[O-].[N+](=O)([O-])[O-]
[O:5]=[N+:6]([O-:7])[O-:8].[Al+3:13]>>[O:5]=[N+:6]([O-:7])[O-:8].[Al+3:13]
O=[N+]([O-])[O-].[Al+3]
O=[N+]([O-])[O-].[Al+3]
null
null
O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
null
[]
null
null
null
null
375.13 g (1 mol) of aluminum nitrate hydrate [Al(NO3)3.9H2O, manufactured by Wako Pure Chemical Industries Ltd., guaranteed reagent] was dissolved in 777.87 g of pure water, to obtain 1000 cm3 of an aluminum nitrate aqueous solution. To 100 cm3 of the aluminum nitrate aqueous solution was added 2.83 g of the above-ment...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
O
null
null
O=[N+]([O-])[O-].[Al+3]>O>O=[N+]([O-])[O-].[Al+3]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ab66ece575e14f4f88417ae953a68374
O=C(O)c1ccccc1O>>O=C(O)c1ccccc1O
C(O)CN.C(C=1C(O)=CC=CC1)(=O)O.C(O)CN.C(C=1C(O)=CC=CC1)(=O)O.C(O)CN.C(C=1C(O)=CC=CC1)(=O)O>>C(C=1C(O)=CC=CC1)(=O)O.C(O)CN
[O:5]=[C:6]([OH:7])[c:8]1[cH:9][cH:10][cH:11][cH:12][c:13]1[OH:14]>>[O:5]=[C:6]([OH:7])[c:8]1[cH:9][cH:10][cH:11][cH:12][c:13]1[OH:14]
O=C(O)c1ccccc1O
O=C(O)c1ccccc1O
null
null
C(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
c1ccccc1
null
null
[]
null
null
null
null
In a 100 ml glass, heat 50 g of ethyl alcohol (C16H34O) to 40° C. and maintain temperature. Slowly add, while stirring, 5 g of salicylic acid (C7H6O3) until dissolved. Add 2 g of monoethanolamine (C2H7NO) until completely mixed. Repeat above process of sequentially adding salicylic acid and monoethanolamine until a tot...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1
null
C(C)O
null
null
O=C(O)c1ccccc1O>C(C)O>O=C(O)c1ccccc1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e390010f5a66490cb26092ec478635e2
NCCO>>NCCO
C(C(O)C)(=O)O.C(O)CN>>C(C(O)C)(=O)O.C(O)CN
[NH2:7][CH2:8][CH2:9][OH:10]>>[NH2:7][CH2:8][CH2:9][OH:10]
NCCO
NCCO
null
null
O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
null
[]
null
null
null
null
In a 100 ml glass, heat 50 g of distilled water to 40° C. and maintain temperature. Add 18 g of lactic acid (C3H6O3). Test pH and slowly add monoethanolamine (C2H7NO) until a pH of 7.0 is achieved. Conditions: See reaction.notes.procedure_details. Workup: maintain temperature
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
O
null
null
NCCO>O>NCCO
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-091c27d4f7224d0588963ff866073830
CC(C)(C)[Si](C)(C)Cl.CC1=C[C@H]2O[C@@H]3C[C@H]4OC(=O)/C=C\C=C\[C@H]([C@@H](C)O)OCC[C@@H](C)[C@H](O)C(=O)OC[C@@]2(CC1)[C@]4(C)[C@]31CO1>>CC(=O)[O-].CCCCCC
N1C=NC=C1.C[C@@H]1CCO[C@H](/C=C/C=C\C(=O)O[C@@H]2C[C@@H]3[C@]4([C@]2([C@]5(CCC(=C[C@H]5O3)C)COC(=O)[C@H]1O)C)CO4)[C@@H](C)O.[Si](C)(C)(C(C)(C)C)Cl>>C(C)(=O)[O-].CCCCCC
CC(C)(C)[Si](C)(Cl)[CH3:10].C[C@@H]1CCO[C@@H]([C@@H](C)[OH:4])/C=C/C=C\C(=[O:3])O[C@@H]2C[C@H:5]3O[C@@H:8]4[CH:7]=[C:2]([CH3:1])CC[C@:9]4(COC(=O)[C@H]1O)[C@]2(C)[C@:6]31CO1>>[CH3:1][C:2](=[O:3])[O-:4].[CH3:5][CH2:6][CH2:7][CH2:8][CH2:9][CH3:10]
CC(C)(C)[Si](C)(C)Cl.CC1=C[C@H]2O[C@@H]3C[C@H]4OC(=O)/C=C\C=C\[C@H]([C@@H](C)O)OCC[C@@H](C)[C@H](O)C(=O)OC[C@@]2(CC1)[C@]4(C)[C@]31CO1
CC(=O)[O-].CCCCCC
null
null
CN(C=O)C
Acylation
OtherReaction
c8232f623ab73fbf3810b05a736c00e1f43fa1c847c2d009e4183f9615ca7dff
d06328b0c6e4b8bb67b99325c4e743e8e3912b9c8541c8956dcd0b540634f10c
null
null
49
[{"value": 49.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
-5
CELSIUS
null
null
Preparation of 13′-O-tert-butyldimethylsilyl-Roridin A. 100 mg (1.47 mmol) of imidazole was added to a solution of 232 mg (0.436 mmol) of Roridin A in 3 ml of dry dimethylformamide. The mixture was cooled to −5° C. and then 72 mg (0.478 mmol) of tert-butyldimethylsilyl chloride (Aldrich Chemical Co.) was added. The res...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Ether.Ether.Secondary alcohol.Secondary alcohol.Conjugated diene.Silyl protective group
null
C1=C[C@H]2O[C@@H]3C[C@H]4OC/C=C\C=C\COCCCCCOC[C@@]2(CC1)[C@@H]4[C@]31CO1
null
null
HCl
CN(C=O)C
-5
null
CC(C)(C)[Si](C)(C)Cl.CC1=C[C@H]2O[C@@H]3C[C@H]4OC(=O)/C=C\C=C\[C@H]([C@@H](C)O)OCC[C@@H](C)[C@H](O)C(=O)OC[C@@]2(CC1)[C@]4(C)[C@]31CO1>CN(C=O)C>CC(=O)[O-].CCCCCC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-09ab9db1af874cec8afef85218a51322
C[C@@H](NC(=O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21)C(=O)O.O=C1CCC(=O)N1O>>O=C(O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21
C(CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@H]12)(=O)N[C@H](C)C(=O)O.ON1C(CCC1=O)=O.N[C@H](C)C(=O)O.N[C@H](C)C(=O)O.Cl.CN(CCCN=C=NCC)C.ON1C(CCC1=O)=O.C1CN(CCN(CCN(CCN1CC(=O)O)CC(=O)O)CC(=O)O)CC(=O)O.NC1=CC=CC=C1>>C1CN(CCN(CCN(CCN1CC(=O)O)CC(=O)O)CC(=O)O)CC(=O)O.OC(=O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@H]12
C[C@@H](N[C:2](=[O:1])[CH2:4][CH2:5][CH2:6][CH2:7][C@@H:8]1[S:9][CH2:10][C@@H:11]2[NH:12][C:13](=[O:14])[NH:15][C@H:16]12)C(=O)O.O=C1CCC(=O)N1[OH:3]>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][CH2:6][CH2:7][C@@H:8]1[S:9][CH2:10][C@@H:11]2[NH:12][C:13](=[O:14])[NH:15][C@H:16]12
C[C@@H](NC(=O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21)C(=O)O.O=C1CCC(=O)N1O
O=C(O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21
null
null
null
Protection
OtherReaction
543cca1236900bb17bf1a8c15e07d003211565da567f1ebfb51f915575e6f61e
b784e02ce9726a9c587d2fe85af8e013bee9ce99cbd3e00a5a9731977fbc070a
O=C1N[C@H]2CSC[C@H]2N1
C-[C@@H](-N-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4])-C(-O)=O.O=C1-C-C-C(=O)-N-1-[OH;D1;+0:5]>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[OH;D1;+0:5]
null
[]
null
null
null
null
The D-alanine-linked conjugate was prepared by first coupling D-alanine (Sigma Chemical Co.) to biotin-NHS ester. The resultant biotinyl-D-alanine was then activated with 1-(3-dimethylaminopropyl)-3-ethyl-carbodiimide hydrochloride (EDCI) and N-hydroxysuccinimide (NHS). This NHS ester was reacted in situ with DOTA-anil...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amide.Tertiary amide.Tertiary amide
Carboxylic acid
C1CCNC1
null
C1N[C@H]2CSC[C@H]2N1
HO-
null
null
null
C[C@@H](NC(=O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21)C(=O)O.O=C1CCC(=O)N1O>>O=C(O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6f2c79ee34a843c588714067f901ff68
CNCC(=O)O.O=C(O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21>>CNCC(=O)C(CCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21)C(=O)O
C1CN(CCN(CCN(CCN1CC(=O)O)CC(=O)O)CC(=O)O)CC(=O)O.OC(=O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@H]12.CNCC(=O)O.C1CN(CCN(CCN(CCN1CC(=O)O)CC(=O)O)CC(=O)O)CC(=O)O.OC(=O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@H]12.CNCC(=O)O.N[C@H](C)C(=O)O>>CNCC(=O)C(C(O)=O)CCC[C@@H]1SC[C@@H]2NC(=O)N[C@H]12
O[C:4]([CH2:3][NH:2][CH3:1])=[O:5].[CH2:6]([CH2:7][CH2:8][CH2:9][C@@H:10]1[S:11][CH2:12][C@@H:13]2[NH:14][C:15](=[O:16])[NH:17][C@H:18]12)[C:19](=[O:20])[OH:21]>>[CH3:1][NH:2][CH2:3][C:4](=[O:5])[CH:6]([CH2:7][CH2:8][CH2:9][C@@H:10]1[S:11][CH2:12][C@@H:13]2[NH:14][C:15](=[O:16])[NH:17][C@H:18]12)[C:19](=[O:20])[OH:21]
CNCC(=O)O.O=C(O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21
CNCC(=O)C(CCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21)C(=O)O
null
null
C(C)N(CC)CC.CN(C)C=O
C-C Coupling
OtherReaction
c7f5ceb44a158fca900911601e13571b0c23016ff9943f5f31fa4dc39e0733d6
a49756d2995b35bf1c4b6840928f031562470ef5bd676447fb43ce2575147daa
O=C1N[C@H]2CSC[C@H]2N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[C:5]-[C:6]-[CH2;D2;+0:7]-[C:8](=[O;D1;H0:9])-[O;D1;H1:10]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH;D3;+0:7](-[C:6]-[C:5])-[C:8](=[O;D1;H0:9])-[O;D1;H1:10]
null
[]
null
null
null
null
The N-methyl glycine-linked DOTA-biotin conjugate was prepared by an analogous method to that used to prepare D-alanine-linked DOTA-biotin conjugates. N-methyl-glycine (trivial name sarcosine, available from Sigma Chemical Co.) was condensed with biotin-NHS ester in DMF and triethylamine to obtain N-methyl glycyl-bioti...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ketone
null
null
C1N[C@H]2CSC[C@H]2N1
HO-
C(C)N(CC)CC.CN(C)C=O
null
null
CNCC(=O)O.O=C(O)CCCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21>C(C)N(CC)CC.CN(C)C=O>CNCC(=O)C(CCC[C@@H]1SC[C@@H]2NC(=O)N[C@@H]21)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1ada602000694563b5e654f716cc2616
NCCN(CCN)CCN.O=Cc1ccc[nH]1>>NCCN=Cc1ccc[nH]1
N1C(=CC=C1)C=O.NCCN(CCN)CCN.O.[N+](=O)([O-])[O-].[Ga+3].[N+](=O)([O-])[O-].[N+](=O)([O-])[O-]>>N1C(=CC=C1)C=NCCN
NCC[N:4](CCN)[CH2:3][CH2:2][NH2:1].O=[CH:5][c:6]1[cH:7][cH:8][cH:9][nH:10]1>>[NH2:1][CH2:2][CH2:3][N:4]=[CH:5][c:6]1[cH:7][cH:8][cH:9][nH:10]1
NCCN(CCN)CCN.O=Cc1ccc[nH]1
NCCN=Cc1ccc[nH]1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
5bb9c36afdb852f191d9594668534907f259dfeb583790227b1a574002b4e65b
5c8cd5b23108f7c707e25ca3918d21afec7c9f4fa7304db3754585c916616b1b
c1cc[nH]c1
N-C-C-[N;H0;D3;+0:1](-C-C-N)-[C:2]-[C:3].O=[CH;D2;+0:4]-[c:5](:[c:6]):[#7;a:7]:[c:8]>>[C:3]-[C:2]-[N;H0;D2;+0:1]=[CH;D2;+0:4]-[c:5](:[c:6]):[#7;a:7]:[c:8]
null
[]
null
null
30
MINUTE
The ligand [(((pyrrole-2-yl)methylidene)amino)ethyl]amine was prepared by adding a methanolic solution of pyrrole-2-carboxaldehyde (1.430 g, 15 mmol, 100 mL) to a methanolic solution of tris(2-aminoethyl)amine (0.720 g, 5 mmol, 10 mL). The resulting yellow solution was stirred at room temperature for 30 min. A methanol...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine.Primary amine.Tertiary amine
Substituted imine
null
null
c1cc[nH]c1
HO-
null
null
0.5
NCCN(CCN)CCN.O=Cc1ccc[nH]1>>NCCN=Cc1ccc[nH]1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ece6613157344bb187f4933ca95baeda
C=CC(=O)OCCCC.C=Cc1ccccc1>>C.C=Cc1ccccc1C=C
C=CC1=CC=CC=C1.C(C=C)(=O)OCCCC>>C(=C)C1=C(C=CC=C1)C=C.C
O=C(C=[CH2:2])O[CH2:5]CC[CH3:1].[cH:3]1[cH:4][c:9]([CH:10]=[CH2:11])[cH:8][cH:7][cH:6]1>>[CH4:1].[CH2:2]=[CH:3][c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1[CH:10]=[CH2:11]
C=CC(=O)OCCCC.C=Cc1ccccc1
C.C=Cc1ccccc1C=C
null
null
null
C-C Coupling
OtherReaction
332e40b06097a8e57aa0a40e096053d40e54a716c6cf2fb9a4bd519069c2082d
2644636eb772ef30c3c03a169846da42c5eac653f3889977ab8870ecd4f5a157
c1ccccc1
O=C(-C=[CH2;D1;+0:1])-O-[CH2;D2;+0:2]-C-C-[CH3;D1;+0:3].[C;D1;H2:4]=[C:5]-[c:6]1:[c:7]:[c:8]:[cH;D2;+0:9]:[cH;D2;+0:10]:[cH;D2;+0:11]:1>>[C;D1;H2:4]=[C:5]-[c:6]1:[c:7]:[c:8]:[cH;D2;+0:9]:[cH;D2;+0:2]:[c;H0;D3;+0:11]:1-[CH;D2;+0:10]=[CH2;D1;+0:1].[CH4;D0;+0:3]
null
[]
null
null
null
null
A polymerizable monomer consisting of 80.5 parts of styrene and 19.5 parts of n-butyl acrylate (Tg of the copolymer obtained by copolymerizing these monomers=55° C.), 0.3 part of polymethacrylic acid ester macromonomer (manufactured by Toagosei Co., Ltd.; trade name: AA6; Tg=94° C.), 0.5 part of divinyl benzene, 1.2 pa...
10.6084/m9.figshare.5104873.v1
null
Ester.Vinyl
Vinyl
c1ccccc1
c1ccccc1
c1ccccc1
HO-
null
null
null
C=CC(=O)OCCCC.C=Cc1ccccc1>>C.C=Cc1ccccc1C=C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0465103634f94e318ae0c256b9e2a45a
C=Cc1ccccc1>>C=Cc1ccccc1
C=CC1=CC=CC=C1.COCCO.[Cl-].C(=C)C[N+](C)(C)CC1=CC=CC=C1>>C=CC1=CC=CC=C1.[Cl-].C(=C)C[N+](C)(C)CC1=CC=CC=C1
[CH2:14]=[CH:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1>>[CH2:14]=[CH:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1
C=Cc1ccccc1
C=Cc1ccccc1
null
null
CCCCCC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
c1ccccc1
null
null
[]
75
CELSIUS
2
HOUR
Styrene (102.96 g) (0.99 mol), 44.2 g (0.21 mol) of vinylbenzyltrimethylammonium chloride and 446 g of 2-methoxy-ethanol were put in a three necked flask and heated at constant temperature of 75° C. with stirring under nitrogen gas flow. Thereafter, 76 g (12 mmol) of 2,2-azobis(dimethyl-2-isobutyrate) was added to the ...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1
null
CCCCCC
75
2
C=Cc1ccccc1>CCCCCC>C=Cc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9e45e151aa224cd2bbf20a160c7e8c1d
CCCC[CH2][Mg][Br].O=C(Cl)c1ccc(F)cc1>>CCCCCC(=O)c1ccc(F)cc1
FC1=CC=C(C(=O)Cl)C=C1.C(CCCC)[Mg]Br.Cl>>FC1=CC=C(C=C1)C(CCCCC)=O
[Br][Mg][CH2:5][CH2:4][CH2:3][CH2:2][CH3:1].Cl[C:6](=[O:7])[c:8]1[cH:9][cH:10][c:11]([F:12])[cH:13][cH:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][C:6](=[O:7])[c:8]1[cH:9][cH:10][c:11]([F:12])[cH:13][cH:14]1
CCCC[CH2][Mg][Br].O=C(Cl)c1ccc(F)cc1
CCCCCC(=O)c1ccc(F)cc1
null
C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Fe+3]
O1CCCC1
C-C Coupling
OtherReaction
ca01e82953d4193c8592b623fe014a93dd536ac2b9b6be24fdd2696e9d29c72c
86a375217dac1e7e5af56ac35ada272b3baae86d3f59f8e623e6beaa450ef46e
c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[Br]-[Mg]-[CH2;D2;+0:6]-[C:7]-[C:8]>>[C:8]-[C:7]-[CH2;D2;+0:6]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
100 mL of tetrahydrofuran was placed into a four-neck round-bottom flask, then 7.92 g (0.05 mol) of 4-fluorobenzoyl chloride and 0.53 g (1.5 mmol) of tris(acetylacetone)iron (III) were added and stirred under a nitrogen atmosphere. To this solution pentylmagnesium bromide was added at a room temperature and stirred at ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Magnesium halide
Ketone
null
null
c1ccccc1
Br-.Mg
C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Fe+3].O1CCCC1
null
null
CCCC[CH2][Mg][Br].O=C(Cl)c1ccc(F)cc1>C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].C/C(=C/C(=O)C)/[O-].[Fe+3].O1CCCC1>CCCCCC(=O)c1ccc(F)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-da622c2e851144e18b5e32b81f602c38
NC(=O)c1ccc(Cl)cc1Cl.O=C(Cl)C(=O)Cl>>O=C=NC(=O)c1ccc(Cl)cc1Cl
ClC1=C(C(=O)N)C=CC(=C1)Cl.C(C(=O)Cl)(=O)Cl>>ClC1=C(C(=O)N=C=O)C=CC(=C1)Cl
[NH2:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][c:12]1[Cl:13].O=C(Cl)[C:2](Cl)=[O:1]>>[O:1]=[C:2]=[N:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][c:12]1[Cl:13]
NC(=O)c1ccc(Cl)cc1Cl.O=C(Cl)C(=O)Cl
O=C=NC(=O)c1ccc(Cl)cc1Cl
null
null
ClCCl
Miscellaneous
OtherReaction
cf02c1bb181b7aadb44446ed25edbc69c91d5a48ce29f9b928a8d564b5d912a5
90d98ee68a4149445e7f059170d2980413d9d8f59364f936e59a8702f0d050b3
c1ccccc1
Cl-C(=O)-[C;H0;D3;+0:1](-Cl)=[O;D1;H0:2].[NH2;D1;+0:3]-[C:4](=[O;D1;H0:5])-[c:6]>>[O;D1;H0:2]=[C;H0;D2;+0:1]=[N;H0;D2;+0:3]-[C:4](=[O;D1;H0:5])-[c:6]
null
[]
null
null
null
null
2,4-Dichlorobenzamide was dissolved in dichloromethane, after which 1.5 eq. of oxalyl chloride were added and the mixture was heated to reflux for 16 hours. The reaction mixture was then concentrated under high vacuum and reacted in step b without any further purification. Conditions: See reaction.notes.procedure_detai...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Primary amide
Isocyanate
null
null
c1ccccc1
HCl
ClCCl
null
null
NC(=O)c1ccc(Cl)cc1Cl.O=C(Cl)C(=O)Cl>ClCCl>O=C=NC(=O)c1ccc(Cl)cc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a4215c2a13f74ffca2c62378fa5f5a43
COc1ccc(C(=O)O)cc1N.O=C=NC(=O)c1ccc(Cl)cc1Cl>>COc1ccc(C(=O)O)cc1NC(=O)NC(=O)c1ccc(Cl)cc1Cl
NC=1C=C(C(=O)O)C=CC1OC.ClC1=C(C(=O)N=C=O)C=CC(=C1)Cl>>ClC1=C(C(=O)NC(NC=2C=C(C(=O)O)C=CC2OC)=O)C=CC(=C1)Cl
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[OH:9])[cH:10][c:11]1[NH2:12].[C:13](=[O:14])=[N:15][C:16](=[O:17])[c:18]1[cH:19][cH:20][c:21]([Cl:22])[cH:23][c:24]1[Cl:25]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[OH:9])[cH:10][c:11]1[NH:12][C:13](=[O:14])[NH:15][C:16](=[O:17])[c:18]1[cH:19][cH:20][c:21]([Cl...
COc1ccc(C(=O)O)cc1N.O=C=NC(=O)c1ccc(Cl)cc1Cl
COc1ccc(C(=O)O)cc1NC(=O)NC(=O)c1ccc(Cl)cc1Cl
null
null
C(C)#N
Acylation
Urea synthesis via isocyanate and primary amine
d39cd7dc52a79bb265ff8ef61ef7bf9dc7f7b5fb0150fcb4881bdfb18ab9c380
a5dc801930c765d2a435a0a2973e50163c305ba8e7641d6adbcc1550b7b96de7
O=C(NC(=O)c1ccccc1)Nc1ccccc1
[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H0:5]=[C;H0;D2;+0:6]=[N;H0;D2;+0:7]-[C:8](=[O;D1;H0:9])-[c:10]>>[O;D1;H0:5]=[C;H0;D3;+0:6](-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4])-[NH;D2;+0:7]-[C:8](=[O;D1;H0:9])-[c:10]
96
[{"value": 96.0, "product": "ClC1=C(C(=O)NC(NC=2C=C(C(=O)O)C=CC2OC)=O)C=CC(=C1)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.7, "product": "ClC1=C(C(=O)NC(NC=2C=C(C(=O)O)C=CC2OC)=O)C=CC(=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
20 g (120 mmol) of 3-amino-4-methoxybenzoic acid were made to react with 36 g (168 mmol) of 2,4-dichlorobenzoyl isocyanate from step a in 400 ml of acetonitrile and left to react therewith at reflux for 2 hours. After the mixture has cooled down to room temperature, the precipitate is filtered off with suction, washed ...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Primary amine
Urea
null
null
c1ccccc1.c1ccccc1
null
C(C)#N
null
null
COc1ccc(C(=O)O)cc1N.O=C=NC(=O)c1ccc(Cl)cc1Cl>C(C)#N>COc1ccc(C(=O)O)cc1NC(=O)NC(=O)c1ccc(Cl)cc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e8d135ce721f44c28b38da57cc1c2746
COc1ccc(S)cc1.O=[N+]([O-])c1ccc(Cl)cc1>>COc1ccc(Sc2ccc([N+](=O)[O-])cc2)cc1
COC1=CC=C(C=C1)S.[H-].[Na+].ClC1=CC=C(C=C1)[N+](=O)[O-]>>COC1=CC=C(C=C1)SC1=CC=C(C=C1)[N+](=O)[O-]
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([SH:7])[cH:17][cH:18]1.Cl[c:8]1[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][cH:16]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([S:7][c:8]2[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][cH:16]2)[cH:17][cH:18]1
COc1ccc(S)cc1.O=[N+]([O-])c1ccc(Cl)cc1
COc1ccc(Sc2ccc([N+](=O)[O-])cc2)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution thiol
58418ec60768d81d36d89dd63ae654278dbe4f345ecf281628c70cd9ed7fe768
97e4acce9b485bd597e518526ab4e9623782b1c9043b6e30dd257d386e3e5b01
c1ccc(Sc2ccccc2)cc1
Cl-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[SH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[S;H0;D2;+0:6]-[c:7](:[c:8]):[c:9]):[c:2]:[c:3]
96.8
[{"value": 96.0, "product": "COC1=CC=C(C=C1)SC1=CC=C(C=C1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.8, "product": "COC1=CC=C(C=C1)SC1=CC=C(C=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
To a suspension of NaH (4.2 g) in 100 mL of dry DMF under nitrogen was slowly added 14.02 g of 4-methoxythiophenol. The reaction mix was stirred until no further gas evolution occurred (circa 20 minutes). To this solution was added 15.76 g of 4-chloronitrobenzene dissolved in 100 ml of dry DMF, after which the mixture ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic thiol
Monosulfide
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HCl
CN(C)C=O
120
null
COc1ccc(S)cc1.O=[N+]([O-])c1ccc(Cl)cc1>CN(C)C=O>COc1ccc(Sc2ccc([N+](=O)[O-])cc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9dd4fd30ac414a2e8efe65060324f68e
COc1ccc(Sc2ccc([N+](=O)[O-])cc2)cc1>>COc1ccc(Sc2ccc(N)cc2)cc1
COC1=CC=C(C=C1)SC1=CC=C(C=C1)[N+](=O)[O-]>>COC1=CC=C(C=C1)SC1=CC=C(C=C1)N
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]([S:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:16][cH:15]2)[cH:14][cH:13]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([S:7][c:8]2[cH:9][cH:10][c:11]([NH2:12])[cH:13][cH:14]2)[cH:15][cH:16]1
COc1ccc(Sc2ccc([N+](=O)[O-])cc2)cc1
COc1ccc(Sc2ccc(N)cc2)cc1
null
null
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Sc2ccccc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
68.1
[{"value": 68.0, "product": "COC1=CC=C(C=C1)SC1=CC=C(C=C1)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.1, "product": "COC1=CC=C(C=C1)SC1=CC=C(C=C1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of 13.06 g of 4-(4-methoxy-phenylsulfanyl)-nitrobenzene from step 1 in 100 mL of ethanol was added 33.85 g of SnCl2−2H2O. The resulting mixture was stirred for 30 minutes at room temperature, then heated to reflux for 2 hours. The mixture was then cooled to room temperature, concentrated in vacuo, and tre...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccccc1
Other
C(C)O
null
0.5
COc1ccc(Sc2ccc([N+](=O)[O-])cc2)cc1>C(C)O>COc1ccc(Sc2ccc(N)cc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-819fdb30593b4783b14fd368375a0969
N#Cc1ccc(Sc2ccc(Cl)cc2)cc1>>NCc1ccc(Sc2ccc(Cl)cc2)cc1
ClC1=CC=C(C=C1)SC1=CC=C(C#N)C=C1.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>ClC1=CC=C(C=C1)SC1=CC=C(CN)C=C1
[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([S:7][c:8]2[cH:9][cH:10][c:11]([Cl:12])[cH:13][cH:14]2)[cH:15][cH:16]1>>[NH2:1][CH2:2][c:3]1[cH:4][cH:5][c:6]([S:7][c:8]2[cH:9][cH:10][c:11]([Cl:12])[cH:13][cH:14]2)[cH:15][cH:16]1
N#Cc1ccc(Sc2ccc(Cl)cc2)cc1
NCc1ccc(Sc2ccc(Cl)cc2)cc1
null
null
C1CCOC1
Reduction
Reduction of nitrile to amine
65bec2d9f430701d30dc9fcbe1c5418f3dfa174d67be035c50edfc71895dc9c7
e8d1bc928b94bd4f5bf4b23363ce8f88b1ce7d146ba93829e7b8ad8dbe0007a7
c1ccc(Sc2ccccc2)cc1
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[NH2;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
93.6
[{"value": 93.6, "product": "ClC1=CC=C(C=C1)SC1=CC=C(CN)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3.5
HOUR
To a solution of 4-(4-chloro-phenylsulfanyl)-benzonitrile (4.91 g) in 100 mL of dry THF under nitrogen stirring at room temperature was added 40 mL of lithium aluminum hydride solution (1.0 M in THF) via syringe. The reaction mix was allowed to stir for 3.5 hours at room temperature, and was then heated to reflux for 4...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amine
null
null
c1ccccc1.c1ccccc1
null
C1CCOC1
null
3.5
N#Cc1ccc(Sc2ccc(Cl)cc2)cc1>C1CCOC1>NCc1ccc(Sc2ccc(Cl)cc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-787609c5fc094e55af8b9d71496b9fb7
O=Cc1ccc(O)cc1.OCCC1CCN(c2ccc(Cl)nn2)CC1>>O=Cc1ccc(OCCC2CCCCN2c2ccc(Cl)nn2)cc1
OC1=CC=C(C=O)C=C1.ClC1=CC=C(N=N1)N1CCC(CC1)CCO.C(C)O>>ClC1=CC=C(N=N1)N1C(CCCC1)CCOC1=CC=C(C=O)C=C1
[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]([OH:7])[cH:23][cH:24]1.O[CH2:8][CH2:9][CH:10]1[CH2:11][CH2:12][N:15]([c:16]2[cH:17][cH:18][c:19]([Cl:20])[n:21][n:22]2)[CH2:14][CH2:13]1>>[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]([O:7][CH2:8][CH2:9][CH:10]2[CH2:11][CH2:12][CH2:13][CH2:14][N:15]2[c:16]2[cH:17][cH:18][c:19]([Cl:20])[n:21][n...
O=Cc1ccc(O)cc1.OCCC1CCN(c2ccc(Cl)nn2)CC1
O=Cc1ccc(OCCC2CCCCN2c2ccc(Cl)nn2)cc1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
0f06477de7cd0c35e538a8fa5bdf57f341aa4a1ddd11263adeb94973dcb5a072
65d9257b508e1839cdbbf508d968410ece9529492834fd6acdca7e25f839a3f0
c1ccc(OCCC2CCCCN2c2cccnn2)cc1
O-[CH2;D2;+0:1]-[C:2]-[CH;D3;+0:3]1-[C:4]-[CH2;D2;+0:5]-[N;H0;D3;+0:6](-[c:7](:[c:8]):[#7;a:9]:[#7;a:10]:[c:11])-[C:12]-[CH2;D2;+0:13]-1.[OH;D1;+0:14]-[c:15](:[c:16]):[c:17]>>[c:8]:[c:7](-[N;H0;D3;+0:6]1-[C:12]-[CH2;D2;+0:13]-[CH2;D2;+0:5]-[C:4]-[CH;D3;+0:3]-1-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:14]-[c:15](:[c:16]):[c:17])...
44
[{"value": 44.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
4- {2-[1-(6-Chloro-3-pyridazinyl)piperidinyl]ethoxy}benzaldehyde (Intermediate IIa) was prepared from 4-hydroxybenzaldehyde and 2-[1-(6-Chloro-3-pyridazinyl)-4-piperidinyl]ethanol using a Mitsunobu Reaction and following the general methods described in U.S. Pat. No. 4,992,433. The aldehyde (60 mg, 0.17 mmol) was disso...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol.Tertiary amine
Ether.Tertiary amine
C1CC[NH]CC1
C1CC[NH]CC1
c1ccccc1.C1CC[NH]CC1.c1ccnnc1
HO-
O
null
null
O=Cc1ccc(O)cc1.OCCC1CCN(c2ccc(Cl)nn2)CC1>O>O=Cc1ccc(OCCC2CCCCN2c2ccc(Cl)nn2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-631c2fe64f044b65aedaec9cf6bcb544
CCON.O=Cc1ccc(O)cc1>>CCON=Cc1ccc(O)cc1
OC1=CC=C(C=O)C=C1.C(C)ON.ClCCl>>C(C)ON=CC1=CC=C(C=C1)O
[CH3:1][CH2:2][O:3][NH2:4].O=[CH:5][c:6]1[cH:7][cH:8][c:9]([OH:10])[cH:11][cH:12]1>>[CH3:1][CH2:2][O:3][N:4]=[CH:5][c:6]1[cH:7][cH:8][c:9]([OH:10])[cH:11][cH:12]1
CCON.O=Cc1ccc(O)cc1
CCON=Cc1ccc(O)cc1
null
null
O1CCOCC1
Heteroatom Alkylation and Arylation
OtherReaction
54882f986dad145756472fc79464161665827db6af7b3780cb2b83c72b495424
3d6c7b6a0f29252ce5dcda36fa3ef05efc366c421f47850a88ae430c686fc79d
c1ccccc1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[#8:6]-[NH2;D1;+0:7]>>[C:5]-[#8:6]-[N;H0;D2;+0:7]=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]
92.5
[{"value": 92.5, "product": "C(C)ON=CC1=CC=C(C=C1)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.0, "product": "C(C)ON=CC1=CC=C(C=C1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-hydroxybenzaldehyde (100 mg, 0.88 mmol) and 50% O-ethylhydroxylamine aqueous solution (0.6 ml, 4.9 mmol) in dioxane (2 ml) was stirred under an atmosphere of argon at room temperature for 16 hours and then heated at 90-100° for 3 hours when thin layer chromatography (silica, dichloromethane) indicated t...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
null
null
null
c1ccccc1
HO-
O1CCOCC1
null
null
CCON.O=Cc1ccc(O)cc1>O1CCOCC1>CCON=Cc1ccc(O)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-81fb2facae8544069721ab1464838751
C#CCCCO.CCON=Cc1cc(C)c(O)c(C)c1>>C#CCCCOc1c(C)cc(C=NOCC)cc1C
C(CCC#C)O.C(C)ON=CC1=CC(=C(C(=C1)C)O)C>>C(C)ON=CC1=CC(=C(C(=C1)C)OCCCC#C)C
O[CH2:5][CH2:4][CH2:3][C:2]#[CH:1].[OH:6][c:7]1[c:8]([CH3:9])[cH:10][c:11]([CH:12]=[N:13][O:14][CH2:15][CH3:16])[cH:17][c:18]1[CH3:19]>>[CH:1]#[C:2][CH2:3][CH2:4][CH2:5][O:6][c:7]1[c:8]([CH3:9])[cH:10][c:11]([CH:12]=[N:13][O:14][CH2:15][CH3:16])[cH:17][c:18]1[CH3:19]
C#CCCCO.CCON=Cc1cc(C)c(O)c(C)c1
C#CCCCOc1c(C)cc(C=NOCC)cc1C
null
null
null
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
86bfb73617450d22f9456ed5ce4d96a73f1f8fc0c016bebae57fda68e2da86a2
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
c1ccccc1
O-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4]#[C;D1;H1:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[C;D1;H1:5]#[C:4]-[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:6]-[c:7](:[c:8]):[c:9]
null
[]
null
null
null
null
Condensation of 4-pentyn-1-ol and 4-hydroxy-3,5-dimethylbenzaldehyde O-ethyloxime using Mitsunobu Reaction conditions (see for example J. Med. Chem., 36, 3240, 1993 and references cited therein) gave 3,5-dimethyl4-(4-pentyn-1-yloxy)benzaldehyde O-ethyl oxime in good yield. Conditions: See reaction.notes.procedure_detai...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
null
null
c1ccccc1
HO-
null
null
null
C#CCCCO.CCON=Cc1cc(C)c(O)c(C)c1>>C#CCCCOc1c(C)cc(C=NOCC)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9a6681b884134483bf8b684de6addf88
C#CCCCOc1c(C)cc(C=NOCC)cc1C.ON=Cc1ccccc1>>CCON=Cc1cc(C)c(OCCCc2cc(-c3ccccc3)no2)c(C)c1
C(C)N(CC)CC.C(C)ON=CC1=CC(=C(C(=C1)C)OCCCC#C)C.C(C1=CC=CC=C1)=NO.ClN1C(CCC1=O)=O>>C(C)ON=CC1=CC(=C(C(=C1)C)OCCCC1=CC(=NO1)C1=CC=CC=C1)C
[CH3:1][CH2:2][O:3][N:4]=[CH:5][c:6]1[cH:7][c:8]([CH3:9])[c:10]([O:11][CH2:12][CH2:13][CH2:14][C:15]#[CH:16])[c:26]([CH3:27])[cH:28]1.[CH:17]([c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1)=[N:24][OH:25]>>[CH3:1][CH2:2][O:3][N:4]=[CH:5][c:6]1[cH:7][c:8]([CH3:9])[c:10]([O:11][CH2:12][CH2:13][CH2:14][c:15]2[cH:16][c:17](-[c...
C#CCCCOc1c(C)cc(C=NOCC)cc1C.ON=Cc1ccccc1
CCON=Cc1cc(C)c(OCCCc2cc(-c3ccccc3)no2)c(C)c1
null
N1=CC=CC=C1
CN(C)C=O
Aromatic Heterocycle Formation
OtherReaction
16b6cd102ecd71fbe2a5e7bfcc7c52ec8c6ac47b948d2e926aa77fed51055f5c
d59db5f5144aec61a5a64ca529856dc804630d654f00918274d989b69216eb79
c1ccc(OCCCc2cc(-c3ccccc3)no2)cc1
[C:1]-[C:2]-[C;H0;D2;+0:3]#[CH;D1;+0:4].[OH;D1;+0:5]-[N;H0;D2;+0:6]=[CH;D2;+0:7]-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[C:1]-[C:2]-[c;H0;D3;+0:3]1:[cH;D2;+0:4]:[c;H0;D3;+0:7](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[n;H0;D2;+0:6]:[o;H0;D2;+0:5]:1
32
[{"value": 32.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
90
MINUTE
A solution of benzaldehyde oxime (45 mg, 0.372 mmol) in DMF (0.5 ml) was added dropwise to a solution of N-chlorosuccinimide (50 mg, 0.374 mmol) and pyridine (1 drop) in DMF (0.5 ml), keeping the temperature between 25-30° C. The resulting solution was allowed to stir at room temperature for 90 minutes. To this was add...
10.6084/m9.figshare.5104873.v1
null
Alkyne.Oxime
null
null
c1cnoc1
c1ccccc1.c1cnoc1.c1ccccc1
null
N1=CC=CC=C1.CN(C)C=O
null
1.5
C#CCCCOc1c(C)cc(C=NOCC)cc1C.ON=Cc1ccccc1>N1=CC=CC=C1.CN(C)C=O>CCON=Cc1cc(C)c(OCCCc2cc(-c3ccccc3)no2)c(C)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-67d1d9cf48ee4a3e80ffd966c1a31e3d
CC(C)(C)[Si](C)(C)OCc1csc(Cl)n1>>CC(C)(C)[Si](C)(C)OCc1cscn1
ClC=1SC=C(N1)CO[Si](C)(C)C(C)(C)C.[H-].[Na+].CC1=CC=C(N=N1)N1CCC(CC1)CCO>>[Si](C)(C)(C(C)(C)C)OCC=1N=CSC1
Cl[c:13]1[s:12][cH:11][c:10]([CH2:9][O:8][Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7])[n:14]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][CH2:9][c:10]1[cH:11][s:12][cH:13][n:14]1
CC(C)(C)[Si](C)(C)OCc1csc(Cl)n1
CC(C)(C)[Si](C)(C)OCc1cscn1
null
null
CCOCC.C(OC)COC
Functional Group Interconversion
Aromatic dehalogenation
4f6106989807e1170e2da8f2e1925119dcd1a22ece2cb0c7a904100c5bae54f5
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1cscn1
Cl-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[#7;a:5]:1>>[#16;a:2]1:[c:3]:[c:4]:[#7;a:5]:[cH;D2;+0:1]:1
81.8
[{"value": 54.0, "product": "[Si](C)(C)(C(C)(C)C)OCC=1N=CSC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.8, "product": "[Si](C)(C)(C(C)(C)C)OCC=1N=CSC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A suspension of sodium hydride (60%, 135 mg, 3.4 mmol) and 1-(6-methyl-3-pyridazinyl)-4-(2-hydroxyethyl)-piperidine (250 mg, 1.1 mmol) in dimethoxyethane (DME; 4 ml) was stirred at room temperature for 2 hr. A solution of 2-chloro-4-t-butyldimethylsilyloxymethylthiazole (385 mg, 1.46 mmol) in DME (1 ml) was added and t...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cscn1
c1cscn1
c1cscn1
Other
CCOCC.C(OC)COC
null
2
CC(C)(C)[Si](C)(C)OCc1csc(Cl)n1>CCOCC.C(OC)COC>CC(C)(C)[Si](C)(C)OCc1cscn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7b93615a1aee4f05861c3a6bb484f95d
Clc1ccnnc1Cl.NCCCCCO>>OCCCCCNc1ccc(Cl)nn1
NCCCCCO.ClC1=C(N=NC=C1)Cl.C([O-])([O-])=O.[Na+].[Na+]>>ClC1=CC=C(N=N1)NCCCCCO
Cl[c:8]1[c:11]([Cl:12])[cH:10][cH:9][n:13][n:14]1.[OH:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][NH2:7]>>[OH:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][NH:7][c:8]1[cH:9][cH:10][c:11]([Cl:12])[n:13][n:14]1
Clc1ccnnc1Cl.NCCCCCO
OCCCCCNc1ccc(Cl)nn1
null
null
O1CCOCC1
Heteroatom Alkylation and Arylation
OtherReaction
5aea7debdfe3eec85b0d59584066bcd465b3d955619b62e42ce7f0f0ee817111
d6fde1e16668e06119c1512640e5d4978b03666a9981f61cec109523a7356b3c
c1ccnnc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[n;H0;D2;+0:3]:[cH;D2;+0:4]:[c:5]:[c;H0;D3;+0:6]:1-[Cl;D1;H0:7].[C:8]-[C:9]-[NH2;D1;+0:10]>>[C:8]-[C:9]-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[n;H0;D2;+0:3]:[c;H0;D3;+0:6](-[Cl;D1;H0:7]):[c:5]:[cH;D2;+0:4]:1
22
[{"value": 22.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 5-amino-1-pentanol (433 mg, 4.2 mmol), dichloropyridazine (1.25 g, 8.39 mmol) and sodium carbonate (890 mg, 8.39 mmol) was stirred in 1,4-dioxane (40 ml) and heated at 70-80° for 3 days under an atmosphere of argon. The solvent was removed under reduced pressure and the residue was partitioned between dich...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Primary amine
Aromatic halide.Secondary amine
c1ccnnc1
c1ccnnc1
c1ccnnc1
HCl
O1CCOCC1
null
null
Clc1ccnnc1Cl.NCCCCCO>O1CCOCC1>OCCCCCNc1ccc(Cl)nn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-13dd3bfb9a69454a9e9066abb2cd96db
CI.O=Cc1ccc(OCCCCCNc2ccc(Cl)nn2)cc1>>CN(CCCCCOc1ccc(C=O)cc1)c1ccc(Cl)nn1
O.[H-].[Na+].ClC1=CC=C(N=N1)NCCCCCOC1=CC=C(C=O)C=C1.CI>>ClC1=CC=C(N=N1)N(CCCCCOC1=CC=C(C=O)C=C1)C
I[CH3:1].[NH:2]([CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][O:8][c:9]1[cH:10][cH:11][c:12]([CH:13]=[O:14])[cH:15][cH:16]1)[c:17]1[cH:18][cH:19][c:20]([Cl:21])[n:22][n:23]1>>[CH3:1][N:2]([CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][O:8][c:9]1[cH:10][cH:11][c:12]([CH:13]=[O:14])[cH:15][cH:16]1)[c:17]1[cH:18][cH:19][c:20]([Cl:21])[n:22][n...
CI.O=Cc1ccc(OCCCCCNc2ccc(Cl)nn2)cc1
CN(CCCCCOc1ccc(C=O)cc1)c1ccc(Cl)nn1
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
e1587a52a1bca6a80c6048d43276d8bccf8d3e94e692e6b210e5fd3b22494187
7cc25fba33369069673bac5bd8fc404dc064da8d6c8cf4a77f21f4df0a617fe3
c1ccc(OCCCCCNc2cccnn2)cc1
I-[CH3;D1;+0:1].[C:2]-[C:3]-[NH;D2;+0:4]-[c:5](:[c:6]):[#7;a:7]:[#7;a:8]:[c:9]>>[C:2]-[C:3]-[N;H0;D3;+0:4](-[CH3;D1;+0:1])-[c:5](:[c:6]):[#7;a:7]:[#7;a:8]:[c:9]
30
[{"value": 30.0, "product": "ClC1=CC=C(N=N1)N(CCCCCOC1=CC=C(C=O)C=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 30.0, "product": "ClC1=CC=C(N=N1)N(CCCCCOC1=CC=C(C=O)C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
Sodium hydride (10 mg, 0.24 mmol) was added to a solution of 4-{N-(6-Chloro-3-pyridazinyl)-5-aminopentan-1-oxy}benzaldehyde (51 mg, 0.16 mmol) in THF (3.5 ml) and the mixture was stirred at room temperature for 30 minutes. Methyl iodide (50 μl, 0.8 mmol) was added to the reaction mixture and the suspension was stirred ...
10.6084/m9.figshare.5104873.v1
null
Secondary amine
Tertiary amine
null
null
c1ccccc1.c1ccnnc1
HI
C1CCOC1
null
0.5
CI.O=Cc1ccc(OCCCCCNc2ccc(Cl)nn2)cc1>C1CCOC1>CN(CCCCCOc1ccc(C=O)cc1)c1ccc(Cl)nn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6c0677b2b364456290183131bbb7d1a5
CCON.CN(CCCCCOc1ccc(C=O)cc1)c1ccc(Cl)nn1>>CCON=Cc1ccc(OCCCCCN(C)c2ccc(Cl)nn2)cc1
ClC1=CC=C(N=N1)N(CCCCCOC1=CC=C(C=O)C=C1)C.C(C)ON>>C(C)ON=CC1=CC=C(C=C1)OCCCCCN(C)C=1N=NC(=CC1)Cl
[CH3:1][CH2:2][O:3][NH2:4].O=[CH:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][N:16]([CH3:17])[c:18]2[cH:19][cH:20][c:21]([Cl:22])[n:23][n:24]2)[cH:25][cH:26]1>>[CH3:1][CH2:2][O:3][N:4]=[CH:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][N:16]([CH3:17])[c:18]2[cH:19][...
CCON.CN(CCCCCOc1ccc(C=O)cc1)c1ccc(Cl)nn1
CCON=Cc1ccc(OCCCCCN(C)c2ccc(Cl)nn2)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
54882f986dad145756472fc79464161665827db6af7b3780cb2b83c72b495424
3d6c7b6a0f29252ce5dcda36fa3ef05efc366c421f47850a88ae430c686fc79d
c1ccc(OCCCCCNc2cccnn2)cc1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[#8:6]-[NH2;D1;+0:7]>>[C:5]-[#8:6]-[N;H0;D2;+0:7]=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
Reaction of 4-{N-(6-Chloro-3-pyridazinyl)-N-methyl-5-aminopentan-1-oxy}benzaldehyde with ethoxyamine following similar conditions to those in Example 1 gave 4-{N-(6-Chloro-3-pyridazinyl)-N-methyl-5-aminopentan-1-oxy}benzaldehyde O-ethyloxime (Compound 161) as a colourless oil. The nmr and mass spectral data are given b...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
null
null
null
c1ccccc1.c1ccnnc1
HO-
null
null
null
CCON.CN(CCCCCOc1ccc(C=O)cc1)c1ccc(Cl)nn1>>CCON=Cc1ccc(OCCCCCN(C)c2ccc(Cl)nn2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c15051d52f544451954de1882d51f1db
Cc1nnc(Br)s1.OCCC1CCNCC1>>Cc1nnc(N2CCC(CCO)CC2)s1
BrC=1SC(=NN1)C.N1CCC(CC1)CCO.C([O-])([O-])=O.[K+].[K+]>>CC1=NN=C(S1)N1CCC(CC1)CCO
Br[c:5]1[n:4][n:3][c:2]([CH3:1])[s:15]1.[NH:6]1[CH2:7][CH2:8][CH:9]([CH2:10][CH2:11][OH:12])[CH2:13][CH2:14]1>>[CH3:1][c:2]1[n:3][n:4][c:5]([N:6]2[CH2:7][CH2:8][CH:9]([CH2:10][CH2:11][OH:12])[CH2:13][CH2:14]2)[s:15]1
Cc1nnc(Br)s1.OCCC1CCNCC1
Cc1nnc(N2CCC(CCO)CC2)s1
null
null
null
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution amine
d5ef7977e5c684ef51d2ba431a770308c0f27af177e447e091c94f6e40be2275
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1nnc(N2CCCCC2)s1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3](-[C;D1;H3:4]):[#7;a:5]:[#7;a:6]:1.[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]>>[C:7]-[C:8]-[N;H0;D3;+0:9](-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3](-[C;D1;H3:4]):[#7;a:5]:[#7;a:6]:1)-[C:10]-[C:11]
32.2
[{"value": 2.5, "product": null, "details": "PERCENTYIELD", "is_desired": false}, {"value": 32.0, "product": "CC1=NN=C(S1)N1CCC(CC1)CCO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 32.2, "product": "CC1=NN=C(S1)N1CCC(CC1)CCO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
A suspension containing 2-bromo-5-methyl-1,3,4-thiadiazole (Modarai, B., et al. J. Heterocyclic Chem. (1974) 11, 343-5) (100 mg, 0.56 mmol), 4-piperidine ethanol (87 mg, 0.67 mmol) and potassium carbonate (77 mg, 0.56 mmol) was heated overnight at 120° C. The reaction was cooled and the mixture partitioned between wate...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1nncs1.C1CCNCC1
c1nncs1.C1CC[NH]CC1
c1nncs1.C1CC[NH]CC1
HBr
null
120
null
Cc1nnc(Br)s1.OCCC1CCNCC1>>Cc1nnc(N2CCC(CCO)CC2)s1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3702316ac7f642d386c91c6e27215180
Fc1ccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)cc1Cl>>O=S1(=O)CCCOc2cc3ncnc(Nc4ccc(F)c(Cl)c4)c3cc2OCCC1
ClC=1C=C(C=CC1F)NC1=NC=NC2=CC=3OCCCSCCCOC3C=C12.OOS(=O)[O-].[K+].O>>ClC=1C=C(C=CC1F)NC1=NC=NC2=CC=3OCCCS(CCCOC3C=C12)(=O)=O
[S:2]1[CH2:4][CH2:5][CH2:6][O:7][c:8]2[cH:9][c:10]3[n:11][cH:12][n:13][c:14]([NH:15][c:16]4[cH:17][cH:18][c:19]([F:20])[c:21]([Cl:22])[cH:23]4)[c:24]3[cH:25][c:26]2[O:27][CH2:28][CH2:29][CH2:30]1>>[O:1]=[S:2]1(=[O:3])[CH2:4][CH2:5][CH2:6][O:7][c:8]2[cH:9][c:10]3[n:11][cH:12][n:13][c:14]([NH:15][c:16]4[cH:17][cH:18][c:1...
Fc1ccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)cc1Cl
O=S1(=O)CCCOc2cc3ncnc(Nc4ccc(F)c(Cl)c4)c3cc2OCCC1
null
null
CO
Oxidation
OtherReaction
5fe02016886a03efcab5c1a4819f1ae138af81a1684b126fdae0d8c1b4c10b19
5cedc1bf0f43f21d78a249521ecfcec19fc5ac4895c41eed0e84f0c2618149fa
O=S1(=O)CCCOc2cc3ncnc(Nc4ccccc4)c3cc2OCCC1
[C:1]-[C:2]-[S;H0;D2;+0:3]-[C:4]-[C:5]>>[C:1]-[C:2]-[S;H0;D4;+0:3](=[O;D1;H0:6])(=[O;D1;H0:7])-[C:4]-[C:5]
null
[]
null
null
4
HOUR
(3-Chloro-4-fluoro-phenyl)-(2,10-dioxa-6-thia-14,16-diaza-tricyclo[9.8.0.013,18]nonadeca-1-(11),12,14,16,18-pentaen-17-yl)-amine (16, 140 mg, 0.33 mmol) was suspended in MeOH, to which was added a cloudy aqueous solution of oxone (monopersulfate compound) (820 mg, 1.33 mmol) at room temperature. The suspension was stir...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfone
c1ncc2cc3c(cc2n1)OCCCSCCCO3
c1ncc2cc3c(cc2n1)OCCCSCCCO3
c1ncc2cc3c(cc2n1)OCCCSCCCO3.c1ccccc1
null
CO
null
4
Fc1ccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)cc1Cl>CO>O=S1(=O)CCCOc2cc3ncnc(Nc4ccc(F)c(Cl)c4)c3cc2OCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cfcc94e67317414aafec216e4f7d7e4c
Clc1cccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)c1>>O=S1(=O)CCCOc2cc3ncnc(Nc4cccc(Cl)c4)c3cc2OCCC1
ClC=1C=C(C=CC1)NC1=NC=NC2=CC=3OCCCSCCCOC3C=C12.OOS(=O)[O-].[K+].O>>ClC=1C=C(C=CC1)NC1=NC=NC2=CC=3OCCCS(CCCOC3C=C12)(=O)=O
[S:2]1[CH2:4][CH2:5][CH2:6][O:7][c:8]2[cH:9][c:10]3[n:11][cH:12][n:13][c:14]([NH:15][c:16]4[cH:17][cH:18][cH:19][c:20]([Cl:21])[cH:22]4)[c:23]3[cH:24][c:25]2[O:26][CH2:27][CH2:28][CH2:29]1>>[O:1]=[S:2]1(=[O:3])[CH2:4][CH2:5][CH2:6][O:7][c:8]2[cH:9][c:10]3[n:11][cH:12][n:13][c:14]([NH:15][c:16]4[cH:17][cH:18][cH:19][c:2...
Clc1cccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)c1
O=S1(=O)CCCOc2cc3ncnc(Nc4cccc(Cl)c4)c3cc2OCCC1
null
null
CO
Oxidation
OtherReaction
5fe02016886a03efcab5c1a4819f1ae138af81a1684b126fdae0d8c1b4c10b19
5cedc1bf0f43f21d78a249521ecfcec19fc5ac4895c41eed0e84f0c2618149fa
O=S1(=O)CCCOc2cc3ncnc(Nc4ccccc4)c3cc2OCCC1
[C:1]-[C:2]-[S;H0;D2;+0:3]-[C:4]-[C:5]>>[C:1]-[C:2]-[S;H0;D4;+0:3](=[O;D1;H0:6])(=[O;D1;H0:7])-[C:4]-[C:5]
null
[]
null
null
4
HOUR
(3-Chloro-phenyl)-(2,10-dioxa-6-thia-14,16-diaza-tricyclo[9.8.0.013,18]nonadeca-1(11),12,14,16,18-pentaen-17-yl)-amine (19, 100 mg, 0.23 mmol) was suspended in MeOH, to which was added a cloudy aqueous solution of oxone (monopersulfate compound) (551 mg, 0.897 mmol) at room temperature. The suspension was stirred and m...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfone
c1ncc2cc3c(cc2n1)OCCCSCCCO3
c1ncc2cc3c(cc2n1)OCCCSCCCO3
c1ncc2cc3c(cc2n1)OCCCSCCCO3.c1ccccc1
null
CO
null
4
Clc1cccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)c1>CO>O=S1(=O)CCCOc2cc3ncnc(Nc4cccc(Cl)c4)c3cc2OCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6e24601995134034850c72b8f5f7927b
Brc1cccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)c1>>O=S1(=O)CCCOc2cc3ncnc(Nc4cccc(Br)c4)c3cc2OCCC1
BrC=1C=C(C=CC1)NC1=NC=NC2=CC=3OCCCSCCCOC3C=C12.OOS(=O)[O-].[K+].O>>BrC=1C=C(C=CC1)NC1=NC=NC2=CC=3OCCCS(CCCOC3C=C12)(=O)=O
[S:2]1[CH2:4][CH2:5][CH2:6][O:7][c:8]2[cH:9][c:10]3[n:11][cH:12][n:13][c:14]([NH:15][c:16]4[cH:17][cH:18][cH:19][c:20]([Br:21])[cH:22]4)[c:23]3[cH:24][c:25]2[O:26][CH2:27][CH2:28][CH2:29]1>>[O:1]=[S:2]1(=[O:3])[CH2:4][CH2:5][CH2:6][O:7][c:8]2[cH:9][c:10]3[n:11][cH:12][n:13][c:14]([NH:15][c:16]4[cH:17][cH:18][cH:19][c:2...
Brc1cccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)c1
O=S1(=O)CCCOc2cc3ncnc(Nc4cccc(Br)c4)c3cc2OCCC1
null
null
CO
Oxidation
OtherReaction
5fe02016886a03efcab5c1a4819f1ae138af81a1684b126fdae0d8c1b4c10b19
5cedc1bf0f43f21d78a249521ecfcec19fc5ac4895c41eed0e84f0c2618149fa
O=S1(=O)CCCOc2cc3ncnc(Nc4ccccc4)c3cc2OCCC1
[C:1]-[C:2]-[S;H0;D2;+0:3]-[C:4]-[C:5]>>[C:1]-[C:2]-[S;H0;D4;+0:3](=[O;D1;H0:6])(=[O;D1;H0:7])-[C:4]-[C:5]
null
[]
null
null
4
HOUR
(3-Bromo-phenyl)-(2,10-dioxa-6-thia-14,16-diaza-tricyclo[9.8.0.013,18]nonadeca-1(11),12,14,16,18-pentaen-17-yl)-amine (21, 17.8 mg, 0.04 mmol) was suspended in MeOH, to which was added a cloudy aqueous solution of oxone (monopersulfate compound) (73 mg, 0.12 mmol) at room temperature. The suspension was stirred and mon...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfone
c1ncc2cc3c(cc2n1)OCCCSCCCO3
c1ncc2cc3c(cc2n1)OCCCSCCCO3
c1ncc2cc3c(cc2n1)OCCCSCCCO3.c1ccccc1
null
CO
null
4
Brc1cccc(Nc2ncnc3cc4c(cc23)OCCCSCCCO4)c1>CO>O=S1(=O)CCCOc2cc3ncnc(Nc4cccc(Br)c4)c3cc2OCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9e262bb65ec44147a7abef9bcbc36b34
Brc1cccc(Nc2ncnc3cc4c(cc23)OCCOCCOCCO4)c1>>C#Cc1cccc(Nc2ncnc3cc4c(cc23)OCCOCCOCCO4)c1
C[Si](C)(C)C#C.C([O-])([O-])=O.[K+].[K+].BrC=1C=C(C=CC1)NC=1C=2C=C3C(=CC2N=CN1)OCCOCCOCCO3.BrC=1C=C(C=CC1)NC=1C=2C=C3C(=CC2N=CN1)OCCOCCOCCO3>>C(#C)C=1C=C(C=CC1)NC=1C=2C=C3C(=CC2N=CN1)OCCOCCOCCO3
Br[c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][n:12][c:13]3[cH:14][c:15]4[c:16]([cH:17][c:18]23)[O:19][CH2:20][CH2:21][O:22][CH2:23][CH2:24][O:25][CH2:26][CH2:27][O:28]4)[cH:29]1>>[CH:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][n:12][c:13]3[cH:14][c:15]4[c:16]([cH:17][c:18]23)[O:19][CH2:2...
Brc1cccc(Nc2ncnc3cc4c(cc23)OCCOCCOCCO4)c1
C#Cc1cccc(Nc2ncnc3cc4c(cc23)OCCOCCOCCO4)c1
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Cu]I
CN(C)C=O
Functional Group Interconversion
OtherReaction
95b76df7bbd0ba7aef764b8988925515b3c4e00700642b1df2a075a9fb68bd8a
3328c8f87c438567981cd74666102f3c9878dcf86df57abda9cd69bae6cfdc49
c1ccc(Nc2ncnc3cc4c(cc23)OCCOCCOCCO4)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]>>[C;D1;H1:6]#[C:7]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
10.2
[{"value": 10.2, "product": "C(#C)C=1C=C(C=CC1)NC=1C=2C=C3C(=CC2N=CN1)OCCOCCOCCO3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
(3-Bromo-phenyl)-(7,8,10,11,13,14-hexahydro-6,9,12,15-tetraoxa-1,3-diaza-cyclododeca[b]naphthalen-4-yl)-amine (Compound 10) (10 mg, 0.5 mmol) was dissolved in DMF (10 mL). Tetrakis(triphenylphosphine) palladium (20 mg), trimethylsilylacetylene (70 microliter, 0.65 mmol), potassium carbonate (10 mg) and copper (I) iodid...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Alkyne
c1ccccc1
c1ccccc1
c1ccccc1.c1ncc2cc3c(cc2n1)OCCOCCOCCO3
Br-
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Cu]I.CN(C)C=O
null
null
Brc1cccc(Nc2ncnc3cc4c(cc23)OCCOCCOCCO4)c1>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Cu]I.CN(C)C=O>C#Cc1cccc(Nc2ncnc3cc4c(cc23)OCCOCCOCCO4)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9b3103b72e3147378a37f482c253d6ca
C1OCOCO1.NS(=O)(=O)c1ccc([N+](=O)[O-])cc1>>O=[N+]([O-])c1ccc(S(=O)(=O)N2COCOC2)cc1
[N+](=O)([O-])C1=CC=C(C=C1)S(=O)(=O)N.O1COCOC1.CS(=O)(=O)O>>N1(COCOC1)S(=O)(=O)C1=CC=C(C=C1)[N+](=O)[O-]
O1[CH2:12][O:13][CH2:14][O:15][CH2:16]1.[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([S:8](=[O:9])(=[O:10])[NH2:11])[cH:17][cH:18]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([S:8](=[O:9])(=[O:10])[N:11]2[CH2:12][O:13][CH2:14][O:15][CH2:16]2)[cH:17][cH:18]1
C1OCOCO1.NS(=O)(=O)c1ccc([N+](=O)[O-])cc1
O=[N+]([O-])c1ccc(S(=O)(=O)N2COCOC2)cc1
null
null
O.C(C)(=O)O
Functional Group Addition
OtherReaction
000d2d3beb174d5f5006b387f6cc20960337f20dff053547c22014ac58a1f299
2b261c617f25c005ceda417aaba7c54cae1bc4064f563010f9e8bc2ae4ff331a
O=S(=O)(c1ccccc1)N1COCOC1
O1-[CH2;D2;+0:1]-[#8:2]-[C:3]-[#8:4]-[CH2;D2;+0:5]-1.[NH2;D1;+0:6]-[#16:7](=[O;D1;H0:8])(=[O;D1;H0:9])-[c:10]>>[O;D1;H0:8]=[#16:7](=[O;D1;H0:9])(-[c:10])-[N;H0;D3;+0:6]1-[CH2;D2;+0:1]-[#8:2]-[C:3]-[#8:4]-[CH2;D2;+0:5]-1
35
[{"value": 35.0, "product": "N1(COCOC1)S(=O)(=O)C1=CC=C(C=C1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 34.8, "product": "N1(COCOC1)S(=O)(=O)C1=CC=C(C=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
5
MINUTE
4-Nitrobenzenesulphonamide (2.02 g, 10 mmol) was added to a solution of 1,3,5-trioxane (1.96 g, 20 mmol) in acetic acid (5 ml). The mixture was stirred for 5 minutes and methanesulphonic acid (10 ml) was added slowly. The mixture was then stirred at 35° C. for 20 minutes, cooled to 0° C., diluted with water and extract...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Ether.Ether.Ether
Ether.Ether.Tertiary amine
C1OCOCO1
C1[NH]COCO1
c1ccccc1.C1[NH]COCO1
HO-
O.C(C)(=O)O
0
0.083333
C1OCOCO1.NS(=O)(=O)c1ccc([N+](=O)[O-])cc1>O.C(C)(=O)O>O=[N+]([O-])c1ccc(S(=O)(=O)N2COCOC2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cbba29ad300148f0b5dbff015b5c2449
CCN(CC)CCOc1ccc([N+](=O)[O-])cc1>>CCN(CC)CCOc1ccc(N)cc1
C(C)N(CCOC1=CC=C(C=C1)[N+](=O)[O-])CC>>C(C)N(CCOC1=CC=C(N)C=C1)CC
O=[N+:13]([O-])[c:12]1[cH:11][cH:10][c:9]([O:8][CH2:7][CH2:6][N:3]([CH2:2][CH3:1])[CH2:4][CH3:5])[cH:15][cH:14]1>>[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[CH2:6][CH2:7][O:8][c:9]1[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]1
CCN(CC)CCOc1ccc([N+](=O)[O-])cc1
CCN(CC)CCOc1ccc(N)cc1
null
[Pd]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
46
[{"value": 46.0, "product": "C(C)N(CCOC1=CC=C(N)C=C1)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 45.7, "product": "C(C)N(CCOC1=CC=C(N)C=C1)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A mixture of 4-(2-diethylaminoethoxy)-1-nitrobenzene (Method 10) (1.0 g, 4.2 mmol) and 10% palladium on charcoal catalyst (200 mg) in ethanol (30 ml) was stirred under an atmosphere of hydrogen for 3 hours. The catalyst was removed by filtration through diatomaceous earth and the filter pad was washed with methanol. Th...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
[Pd].C(C)O
null
3
CCN(CC)CCOc1ccc([N+](=O)[O-])cc1>[Pd].C(C)O>CCN(CC)CCOc1ccc(N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-40c029c48eb649dba92432924394188f
CCN(CC)CCCl.O=[N+]([O-])c1ccc([O-])cc1>>CCN(CC)CCOc1ccc([N+](=O)[O-])cc1
O.[N+](=O)([O-])C1=CC=C([O-])C=C1.[Na+].Cl.C(C)N(CCCl)CC.C([O-])([O-])=O.[K+].[K+]>>C(C)N(CCOC1=CC=C(C=C1)[N+](=O)[O-])CC
Cl[CH2:7][CH2:6][N:3]([CH2:2][CH3:1])[CH2:4][CH3:5].[O-:8][c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[cH:16][cH:17]1>>[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[CH2:6][CH2:7][O:8][c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[cH:16][cH:17]1
CCN(CC)CCCl.O=[N+]([O-])c1ccc([O-])cc1
CCN(CC)CCOc1ccc([N+](=O)[O-])cc1
null
null
C=1(C(=CC=CC1)C)C
Heteroatom Alkylation and Arylation
OtherReaction
3dd6ea90858eede84ece2f60931b760bd509d5f421f2feb2b0fe7a2c006d84f0
62c7c72c35b09d63ca1131e6cd8c0b88a31e29901d660456b77319cfd78354c7
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2]-[#7:3].[O-;H0;D1:4]-[c:5](:[c:6]):[c:7]>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]
67.1
[{"value": 52.0, "product": "C(C)N(CCOC1=CC=C(C=C1)[N+](=O)[O-])CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 67.1, "product": "C(C)N(CCOC1=CC=C(C=C1)[N+](=O)[O-])CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
Water (8 ml) and xylene (35 ml) were added to a mixture of sodium 4-nitrophenoxide (10.5 g, 65 mmol), 2-(diethylamino)ethylchloride hydrochloride (8.6 g, 50 mmol) and potassium carbonate (10.4 g, 75 mmol) and the resulting mixture was heated at reflux for 2 hours. A Dean-Stark apparatus was then fitted and the water wa...
10.6084/m9.figshare.5104873.v1
null
Primary halide
Ether
null
null
c1ccccc1
Other
C=1(C(=CC=CC1)C)C
null
18
CCN(CC)CCCl.O=[N+]([O-])c1ccc([O-])cc1>C=1(C(=CC=CC1)C)C>CCN(CC)CCOc1ccc([N+](=O)[O-])cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1dcb26f6d6184ee3b17c092fca446c72
BrCC1CO1.O=[N+]([O-])c1ccc(O)cc1>>O=[N+]([O-])c1ccc(OCC2CO2)cc1
[N+](=O)([O-])C1=CC=C(C=C1)O.C([O-])([O-])=O.[K+].[K+].C(Br)C1CO1>>[N+](=O)([O-])C1=CC=C(OCC2CO2)C=C1
Br[CH2:9][CH:10]1[CH2:11][O:12]1.[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([OH:8])[cH:13][cH:14]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([O:8][CH2:9][CH:10]2[CH2:11][O:12]2)[cH:13][cH:14]1
BrCC1CO1.O=[N+]([O-])c1ccc(O)cc1
O=[N+]([O-])c1ccc(OCC2CO2)cc1
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccc(OCC2CO2)cc1
Br-[CH2;D2;+0:1]-[C:2]1-[#8:3]-[C:4]-1.[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[c:7]:[c:6](-[O;H0;D2;+0:5]-[CH2;D2;+0:1]-[C:2]1-[#8:3]-[C:4]-1):[c:8]
77.7
[{"value": 77.7, "product": "[N+](=O)([O-])C1=CC=C(OCC2CO2)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
1-(4-Nitrophenoxy)-2,3-epoxypropane was prepared by an analogous method to that described by Zhen-Zhong Lui et. al. in Synthetic Communications (1994), 24, 833–838. 4-Nitrophenol (4.0 g), anhydrous potassium carbonate (8.0 g) and tetrabutylammonium bromide (0.4 g) were mixed with epibromohydrin (10 ml). The reaction mi...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.C1CO1
HBr
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)OCC
100
null
BrCC1CO1.O=[N+]([O-])c1ccc(O)cc1>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)OCC>O=[N+]([O-])c1ccc(OCC2CO2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-12f713cbd2b6455fa7fff07a664a3769
CN.Nc1ccc(S(=O)(=O)F)cc1>>CNS(=O)(=O)c1ccc(N)cc1
CN.C(C)N(CC)CC.S(=O)(C1=CC=C(C=C1)N)(=O)F>>CNS(=O)(=O)C1=CC=C(N)C=C1
[CH3:1][NH2:2].F[S:3](=[O:4])(=[O:5])[c:6]1[cH:7][cH:8][c:9]([NH2:10])[cH:11][cH:12]1>>[CH3:1][NH:2][S:3](=[O:4])(=[O:5])[c:6]1[cH:7][cH:8][c:9]([NH2:10])[cH:11][cH:12]1
CN.Nc1ccc(S(=O)(=O)F)cc1
CNS(=O)(=O)c1ccc(N)cc1
null
null
C(C)O
Miscellaneous
Sulfonamide synthesis (Schotten-Baumann) primary amine
a86b0632821e188c0a5dc5a5a2aac298ab3eccaee8a52ba46078c3d5975a290d
50f8fbf3d327483c3eeff8f6cbd4065e4c7600bb501fbe08958a5c79a0926428
c1ccccc1
F-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C;D1;H3:7]-[NH2;D1;+0:8]>>[C;D1;H3:7]-[NH;D2;+0:8]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
78.1
[{"value": 76.0, "product": "CNS(=O)(=O)C1=CC=C(N)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.1, "product": "CNS(=O)(=O)C1=CC=C(N)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
18
HOUR
Methylamine (3 ml of a 33% solution in ethanol) and then triethylamine (0.159 ml, 1.1 mmol) was added to sulphanilyl fluoride (200 mg, 1.1 mmol), and the mixture heated at 80° C. for 6 hours then at ambient temperature for 18 hours. The volatiles were removed by evaporation and the residue azeotroped with toluene to gi...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1
HF
C(C)O
80
18
CN.Nc1ccc(S(=O)(=O)F)cc1>C(C)O>CNS(=O)(=O)c1ccc(N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1606dffd93e44b718532834e0f8c1c8d
COCCN.Nc1ccc(S(=O)(=O)F)cc1>>COCCNS(=O)(=O)c1ccc(N)cc1
COCCN.S(=O)(C1=CC=C(C=C1)N)(=O)F.C(C)N(CC)CC>>COCCNS(=O)(=O)C1=CC=C(N)C=C1
[CH3:1][O:2][CH2:3][CH2:4][NH2:5].F[S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]1>>[CH3:1][O:2][CH2:3][CH2:4][NH:5][S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]1
COCCN.Nc1ccc(S(=O)(=O)F)cc1
COCCNS(=O)(=O)c1ccc(N)cc1
null
null
C(CCC)O
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
c1ccccc1
F-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[C:7]-[C:8]-[NH;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
65.4
[{"value": 65.0, "product": "COCCNS(=O)(=O)C1=CC=C(N)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.4, "product": "COCCNS(=O)(=O)C1=CC=C(N)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 2-methoxyethylamine (859 mg, 11.4 mmol), sulphanilyl fluoride (1.0 g, 5.71 mmol), and triethylamine (1.72 g, 22.9 mmol) in n-butanol (15 ml) was heated at reflux for 18 hours. The mixture was allowed to cool and the volatiles were removed by evaporation. The residue was purified by chromatography eluting w...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1
HF
C(CCC)O
null
null
COCCN.Nc1ccc(S(=O)(=O)F)cc1>C(CCC)O>COCCNS(=O)(=O)c1ccc(N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ec2c00ed3ca848f29957ef69ffc7e561
NCCCn1ccnc1.O=C(Cl)c1ccc(Br)cc1>>O=C(NCCCn1ccnc1)c1ccc(Br)cc1
NCCCN1C=NC=C1.BrC1=CC=C(C(=O)Cl)C=C1>>BrC1=CC=C(C(=O)NCCCN2C=NC=C2)C=C1
[NH2:3][CH2:4][CH2:5][CH2:6][n:7]1[cH:8][cH:9][n:10][cH:11]1.Cl[C:2](=[O:1])[c:12]1[cH:13][cH:14][c:15]([Br:16])[cH:17][cH:18]1>>[O:1]=[C:2]([NH:3][CH2:4][CH2:5][CH2:6][n:7]1[cH:8][cH:9][n:10][cH:11]1)[c:12]1[cH:13][cH:14][c:15]([Br:16])[cH:17][cH:18]1
NCCCn1ccnc1.O=C(Cl)c1ccc(Br)cc1
O=C(NCCCn1ccnc1)c1ccc(Br)cc1
null
null
C(C)O
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(NCCCn1ccnc1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
18
HOUR
1-(3-Aminopropyl)imidazole (2.39 ml, 0.02 mol) was added to a solution of 4-bromobenzoyl chloride (4.0 g, 0.018 mol) in ethanol (250 ml). The mixture was stirred at ambient temperature for 18 hours. The volatiles were removed by evaporation and the residue was purified by chromatography eluting with hexane/dichlorometh...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1c[nH]cn1.c1ccccc1
HCl
C(C)O
null
18
NCCCn1ccnc1.O=C(Cl)c1ccc(Br)cc1>C(C)O>O=C(NCCCn1ccnc1)c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b4541496d65843e8ba39b6459bbb8b7e
COCCN.O=S(=O)(Cl)c1ccc(Cl)cc1Cl>>COCCNS(=O)(=O)c1ccc(Cl)cc1Cl
ClC1=C(C=CC(=C1)Cl)S(=O)(=O)Cl.COCCN>>ClC1=C(C=CC(=C1)Cl)S(NCCOC)(=O)=O
[CH3:1][O:2][CH2:3][CH2:4][NH2:5].Cl[S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][c:12]([Cl:13])[cH:14][c:15]1[Cl:16]>>[CH3:1][O:2][CH2:3][CH2:4][NH:5][S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][c:12]([Cl:13])[cH:14][c:15]1[Cl:16]
COCCN.O=S(=O)(Cl)c1ccc(Cl)cc1Cl
COCCNS(=O)(=O)c1ccc(Cl)cc1Cl
null
null
C(CCC)O
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[C:7]-[C:8]-[NH;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
2,4-Dichlorobenzenesulphonyl chloride (500 mg 2.1 mmol) and 2-methoxyethylamine (230 mg, 3.1 mmol) in n-butanol (10 ml) was heated at reflux for one hour. The volatiles were removed by evaporation and residue purified by chromatography eluting with hexane/ethyl acetate (50:50) to give the title compound. NMR: 3.04 (t, ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1
HCl
C(CCC)O
null
null
COCCN.O=S(=O)(Cl)c1ccc(Cl)cc1Cl>C(CCC)O>COCCNS(=O)(=O)c1ccc(Cl)cc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c1cc11ebbe0d4252bbb59040cd5dbc06
CCCN.O=S(=O)(Cl)c1ccc(Cl)cc1Cl>>CCCNS(=O)(=O)c1ccc(Cl)cc1Cl
ClC1=C(C=CC(=C1)Cl)S(=O)(=O)Cl.C(CC)N>>ClC1=C(C=CC(=C1)Cl)S(NCCC)(=O)=O
[CH3:1][CH2:2][CH2:3][NH2:4].Cl[S:5](=[O:6])(=[O:7])[c:8]1[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]1[Cl:15]>>[CH3:1][CH2:2][CH2:3][NH:4][S:5](=[O:6])(=[O:7])[c:8]1[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]1[Cl:15]
CCCN.O=S(=O)(Cl)c1ccc(Cl)cc1Cl
CCCNS(=O)(=O)c1ccc(Cl)cc1Cl
null
null
C(CCC)O
Miscellaneous
Sulfonamide synthesis (Schotten-Baumann) primary amine
a86b0632821e188c0a5dc5a5a2aac298ab3eccaee8a52ba46078c3d5975a290d
50f8fbf3d327483c3eeff8f6cbd4065e4c7600bb501fbe08958a5c79a0926428
c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[C:7]-[C:8]-[NH;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
2,4-Dichlorobenzenesulphonyl chloride (500 mg 2.1 mmol) and 1-propylamine (0.2 ml, 2.4 mmol) in n-butanol (10 ml) was heated at reflux for 48 hours. The volatiles were removed by evaporation and the residue triturated with diethylene ether and the product collected by filtration to give the title compound. NMR: 0.78 (t...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1
HCl
C(CCC)O
null
null
CCCN.O=S(=O)(Cl)c1ccc(Cl)cc1Cl>C(CCC)O>CCCNS(=O)(=O)c1ccc(Cl)cc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e5c80abd908e434e87362660a829fe62
N#CNC(=O)c1ccccc1.Nc1ccc(S(N)(=O)=O)cc1>>N=C(N)Nc1ccc(S(N)(=O)=O)cc1
S(=O)(C1=CC=C(C=C1)N)(=O)N.C(C1=CC=CC=C1)(=O)NC#N>>S(N)(=O)(=O)C1=CC=C(C=C1)NC(=N)N
O=C(c1ccccc1)[NH:3][C:2]#[N:1].[NH2:4][c:5]1[cH:6][cH:7][c:8]([S:9]([NH2:10])(=[O:11])=[O:12])[cH:13][cH:14]1>>[NH:1]=[C:2]([NH2:3])[NH:4][c:5]1[cH:6][cH:7][c:8]([S:9]([NH2:10])(=[O:11])=[O:12])[cH:13][cH:14]1
N#CNC(=O)c1ccccc1.Nc1ccc(S(N)(=O)=O)cc1
N=C(N)Nc1ccc(S(N)(=O)=O)cc1
null
null
Cl.C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
dd44df42b31bde19fead74620111799f04dd5596f1feefd0c1ccb164c4aa5403
7bb7c5606a457b76cd0344df0a1af007033251255efdb0ed5da2ca492488bc21
c1ccccc1
O=C(-[NH;D2;+0:1]-[C;H0;D2;+0:2]#[N;H0;D1;+0:3])-c1:c:c:c:c:c:1.[NH2;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[NH2;D1;+0:1]-[C;H0;D3;+0:2](=[NH;D1;+0:3])-[NH;D2;+0:4]-[c:5](:[c:6]):[c:7]
null
[]
null
null
null
null
A mixture of sulphanilamide (20 g, 0.166 mol), benzoyl cyanamide (34 g, 0.33 mol) in ethanol (60 ml) and concentrated hydrochloric acid (11 ml) was heated on a steam bath until the solvent had evaporated. Water was added and the mixture heated at reflux for 5 minutes. Sodium hydroxide (14.4 g) was added and the mixture...
10.6084/m9.figshare.5104873.v1
null
Cyanamide.Secondary amide.Primary amine
Primary amine.Secondary amine
c1ccccc1
null
c1ccccc1
HO-
Cl.C(C)O
null
null
N#CNC(=O)c1ccccc1.Nc1ccc(S(N)(=O)=O)cc1>Cl.C(C)O>N=C(N)Nc1ccc(S(N)(=O)=O)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-59d1004777cc4d44834ff3f01f0bfc24
N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCO2.OCCBr>>N#Cc1c(N)nc(SCCO)c(C#N)c1-c1ccc2c(c1)OCO2
O.NC1=NC(=C(C(=C1C#N)C1=CC2=C(OCO2)C=C1)C#N)S.BrCCO.C([O-])(O)=O.[Na+]>>NC1=NC(=C(C(=C1C#N)C1=CC2=C(OCO2)C=C1)C#N)SCCO
[N:1]#[C:2][c:3]1[c:4]([NH2:5])[n:6][c:7]([SH:8])[c:12]([C:13]#[N:14])[c:15]1-[c:16]1[cH:17][cH:18][c:19]2[c:20]([cH:21]1)[O:22][CH2:23][O:24]2.Br[CH2:9][CH2:10][OH:11]>>[N:1]#[C:2][c:3]1[c:4]([NH2:5])[n:6][c:7]([S:8][CH2:9][CH2:10][OH:11])[c:12]([C:13]#[N:14])[c:15]1-[c:16]1[cH:17][cH:18][c:19]2[c:20]([cH:21]1)[O:22][...
N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCO2.OCCBr
N#Cc1c(N)nc(SCCO)c(C#N)c1-c1ccc2c(c1)OCO2
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
thioether_nucl_sub
26df88c6a3f5f203c89584658be4e126cb42994c98a2e16bc812e1036cdae857
8b2f52296c3a93039174c980b6042ba15754e04d6892a1284c3a32985220b214
c1cc(-c2ccc3c(c2)OCO3)ccn1
Br-[CH2;D2;+0:1]-[C:2]-[O;D1;H1:3].[SH;D1;+0:4]-[c:5](:[c:6]):[#7;a:7]:[c:8]>>[O;D1;H1:3]-[C:2]-[CH2;D2;+0:1]-[S;H0;D2;+0:4]-[c:5](:[c:6]):[#7;a:7]:[c:8]
null
[]
null
null
null
null
75 mg (0.19 mmol) of 2-amino-4-(1,3-benzodioxol-5-yl)-6-sulfanyl-3,5-pyridinedicarbonitrile [prepared analogously to Dyachenko et al., Russian Journal of Chemistry 33 (7), 1014–1017 (1997); 34 (4), 557–563 (1998)] and 47 mg (0.38 mmol) of 2-bromoethanol and 63 mg (0.75 mmol) of sodium bicarbonate are stirred in 1 ml of...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic thiol
Monosulfide
null
null
c1ccncc1.c1ccc2c(c1)OCO2
HBr
CN(C)C=O
null
null
N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCO2.OCCBr>CN(C)C=O>N#Cc1c(N)nc(SCCO)c(C#N)c1-c1ccc2c(c1)OCO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-84b5791973bb4e4b97ae5ec3d0a3b7e3
BrCc1ccccc1.N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCCO2>>N#Cc1c(N)nc(SCc2ccccc2)c(C#N)c1-c1ccc2c(c1)OCCO2
O.NC1=NC(=C(C(=C1C#N)C1=CC2=C(OCCO2)C=C1)C#N)S.C(C1=CC=CC=C1)Br.C([O-])(O)=O.[Na+]>>NC1=NC(=C(C(=C1C#N)C1=CC2=C(OCCO2)C=C1)C#N)SCC1=CC=CC=C1
Br[CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1.[N:1]#[C:2][c:3]1[c:4]([NH2:5])[n:6][c:7]([SH:8])[c:16]([C:17]#[N:18])[c:19]1-[c:20]1[cH:21][cH:22][c:23]2[c:24]([cH:25]1)[O:26][CH2:27][CH2:28][O:29]2>>[N:1]#[C:2][c:3]1[c:4]([NH2:5])[n:6][c:7]([S:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]([C:17]#[N...
BrCc1ccccc1.N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCCO2
N#Cc1c(N)nc(SCc2ccccc2)c(C#N)c1-c1ccc2c(c1)OCCO2
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
S-alkylation of thiols
26df88c6a3f5f203c89584658be4e126cb42994c98a2e16bc812e1036cdae857
8b2f52296c3a93039174c980b6042ba15754e04d6892a1284c3a32985220b214
c1ccc(CSc2cc(-c3ccc4c(c3)OCCO4)ccn2)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[SH;D1;+0:5]-[c:6](:[c:7]):[#7;a:8]:[c:9]>>[c:3]:[c:2](-[CH2;D2;+0:1]-[S;H0;D2;+0:5]-[c:6](:[c:7]):[#7;a:8]:[c:9]):[c:4]
null
[]
null
null
null
null
100 mg (0.32 mol) of 2-amino-6-sulfanyl-4-(2,3-dihydro-1,4-benzodioxin-6-yl)-3,5-pyridinedicarbonitrile [prepared analogously to Dyachenko et al., Russian Journal of Chemistry 33 (7), 1014–1017 (1997); 34 (4), 557–563 (1998)], 110 mg (0.64 mmol) of benzyl bromide and 108 mg (1.29 mmol) of sodium bicarbonate are stirred...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic thiol
Monosulfide
null
null
c1ccncc1.c1ccccc1.c1ccc2c(c1)OCCO2
HBr
CN(C)C=O
null
null
BrCc1ccccc1.N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCCO2>CN(C)C=O>N#Cc1c(N)nc(SCc2ccccc2)c(C#N)c1-c1ccc2c(c1)OCCO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8a06105050574671a0aa48f482262b47
N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCC(CO)O2.OCCBr>>N#Cc1c(N)nc(SCCO)c(C#N)c1-c1ccc2c(c1)OCC(CO)O2
OCCBr.C([O-])(O)=O.[Na+].NC1=NC(=C(C(=C1C#N)C1=CC2=C(OC(CO2)CO)C=C1)C#N)S>>NC1=NC(=C(C(=C1C#N)C1=CC2=C(OC(CO2)CO)C=C1)C#N)SCCO
[N:1]#[C:2][c:3]1[c:4]([NH2:5])[n:6][c:7]([SH:8])[c:12]([C:13]#[N:14])[c:15]1-[c:16]1[cH:17][cH:18][c:19]2[c:20]([cH:21]1)[O:22][CH2:23][CH:24]([CH2:25][OH:26])[O:27]2.Br[CH2:9][CH2:10][OH:11]>>[N:1]#[C:2][c:3]1[c:4]([NH2:5])[n:6][c:7]([S:8][CH2:9][CH2:10][OH:11])[c:12]([C:13]#[N:14])[c:15]1-[c:16]1[cH:17][cH:18][c:19]...
N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCC(CO)O2.OCCBr
N#Cc1c(N)nc(SCCO)c(C#N)c1-c1ccc2c(c1)OCC(CO)O2
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
thioether_nucl_sub
26df88c6a3f5f203c89584658be4e126cb42994c98a2e16bc812e1036cdae857
8b2f52296c3a93039174c980b6042ba15754e04d6892a1284c3a32985220b214
c1cc(-c2ccc3c(c2)OCCO3)ccn1
Br-[CH2;D2;+0:1]-[C:2]-[O;D1;H1:3].[SH;D1;+0:4]-[c:5](:[c:6]):[#7;a:7]:[c:8]>>[O;D1;H1:3]-[C:2]-[CH2;D2;+0:1]-[S;H0;D2;+0:4]-[c:5](:[c:6]):[#7;a:7]:[c:8]
null
[]
null
null
null
null
30 mg (0.09 mmol) of 2-amino-6-sulfanyl-4-[2-(hydroxymethyl)-2,3-dihydro-1,4-benzodioxin-6-yl]-3,5-pyridinedicarbonitrile [prepared analogously to Dyachenko et al., Russian Journal of Chemistry 33 (7), 1014–1017 (1997); 34 (4), 557–563 (1998)], 22 mg (0.18 mmol) of 2-hydroxyethyl bromide and 29 mg (0.35 mmol) of sodium...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic thiol
Monosulfide
null
null
c1ccncc1.c1ccc2c(c1)OCCO2
HBr
CN(C)C=O
null
null
N#Cc1c(N)nc(S)c(C#N)c1-c1ccc2c(c1)OCC(CO)O2.OCCBr>CN(C)C=O>N#Cc1c(N)nc(SCCO)c(C#N)c1-c1ccc2c(c1)OCC(CO)O2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a178a1c686c944a49105cd7cae4ba40a
O=C(O)C(=O)c1cccs1.OC12CCN(CC1)CC2>>O=C(OC12CCN(CC1)CC2)C(=O)c1cccs1
OC12CCN(CC1)CC2.C(C)N(CC)CC.C(C(=O)Cl)(=O)Cl.O=C(C(=O)O)C=1SC=CC1>>N12CCC(CC1)(CC2)OC(C(C=2SC=CC2)=O)=O
O[C:2](=[O:1])[C:12](=[O:13])[c:14]1[cH:15][cH:16][cH:17][s:18]1.[OH:3][C:4]12[CH2:5][CH2:6][N:7]([CH2:8][CH2:9]1)[CH2:10][CH2:11]2>>[O:1]=[C:2]([O:3][C:4]12[CH2:5][CH2:6][N:7]([CH2:8][CH2:9]1)[CH2:10][CH2:11]2)[C:12](=[O:13])[c:14]1[cH:15][cH:16][cH:17][s:18]1
O=C(O)C(=O)c1cccs1.OC12CCN(CC1)CC2
O=C(OC12CCN(CC1)CC2)C(=O)c1cccs1
null
CN(C=O)C
C(Cl)(Cl)Cl
Protection
Esterification of Carboxylic Acids
e9801f206cb4bb9d460f7386b8384e5e0a802882643ef8bad8c1d049e28011dd
802e74463aa64b37e080342ce437e7d11cc2ce6490f10646d6092e974faa7430
O=C(OC12CCN(CC1)CC2)C(=O)c1cccs1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[O;D1;H0:4])-[c:5]:[#16;a:6].[C:7]-[C:8](-[OH;D1;+0:9])(-[C:10])-[C:11]>>[#16;a:6]:[c:5]-[C:3](=[O;D1;H0:4])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:9]-[C:8](-[C:7])(-[C:10])-[C:11]
null
[]
null
null
null
null
Oxalyl chloride (1.5 ml, 0.017 mol) was added to a solution of oxothien-2-yl-acetic acid (2.24 g, 0.014 mol) and dimethylformamide (one drop) in 30 ml of chloroform (etanol free) at 01 C. The mixture was stirred and allowed to warm at room temperature. After one hour the solvent was evaporated. The residue was dissolve...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ketone.Tertiary alcohol
Ketone.Ester
null
null
c1ccsc1.C1CN2CCC1CC2
HO-
CN(C=O)C.C(Cl)(Cl)Cl
null
null
O=C(O)C(=O)c1cccs1.OC12CCN(CC1)CC2>CN(C=O)C.C(Cl)(Cl)Cl>O=C(OC12CCN(CC1)CC2)C(=O)c1cccs1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b970c2902fc343c48c131f9e85dd4144
O=C(O[C@H]1CN2CCC1CC2)C(=O)c1ccco1.[Br][Mg][c]1ccccc1>>O=C(O[C@H]1CN2CCC1CC2)C(O)(c1ccccc1)c1ccco1
[Cl-].[NH4+].CCOCC.C1(=CC=CC=C1)[Mg]Br.N12C[C@@H](C(CC1)CC2)OC(C(C=2OC=CC2)=O)=O>>N12C[C@@H](C(CC1)CC2)OC(C(C2=CC=CC=C2)(O)C=2OC=CC2)=O
[O:1]=[C:2]([O:3][C@H:4]1[CH2:5][N:6]2[CH2:7][CH2:8][CH:9]1[CH2:10][CH2:11]2)[C:12](=[O:13])[c:20]1[cH:21][cH:22][cH:23][o:24]1.[Br][Mg][c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1>>[O:1]=[C:2]([O:3][C@H:4]1[CH2:5][N:6]2[CH2:7][CH2:8][CH:9]1[CH2:10][CH2:11]2)[C:12]([OH:13])([c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1)[c...
O=C(O[C@H]1CN2CCC1CC2)C(=O)c1ccco1.[Br][Mg][c]1ccccc1
O=C(O[C@H]1CN2CCC1CC2)C(O)(c1ccccc1)c1ccco1
null
null
N#N.C1CCOC1
C-C Coupling
Grignard from ketone to alcohol
db2ad3a505f3141c37847e0af43be1bd81d942fe0a7bc68b74ef6bb430d08ffd
652461eb0cd30990fcbed359f728e518ea93a58c037f4fc210fcb30d2dae5f8d
O=C(O[C@H]1CN2CCC1CC2)C(c1ccccc1)c1ccco1
[Br]-[Mg]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[c:12](:[c:13]):[#8;a:14]:[c:15]>>[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C;H0;D4;+0:10](-[OH;D1;+0:11])(-[c:12](:[c:13]):[#8;a:14]:[c:15])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
40
[{"value": 40.0, "product": "N12C[C@@H](C(CC1)CC2)OC(C(C2=CC=CC=C2)(O)C=2OC=CC2)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Phenylmagnesium bromide, 0.0057 mol (5.7 ml of a solution 1M in THF), was added to a solution of 1.3 g ( 0.0052 mol) of oxofuran-2-ylacetic acid 1-azabicyclo[2.2.2]oct-3(R)-yl ester (intermediate I-4e-) dissolved in 15 ml of THF, at −701 C in N2 atmosphere. The mixture was stirred at this temperature for 10 minuts, and...
10.6084/m9.figshare.5104873.v1
null
Magnesium halide.Ketone.Ester
Ester.Tertiary alcohol
c1ccccc1
c1ccccc1
c1ccoc1.c1ccccc1.C1CN2CCC1CC2
Br-.Mg
N#N.C1CCOC1
null
1
O=C(O[C@H]1CN2CCC1CC2)C(=O)c1ccco1.[Br][Mg][c]1ccccc1>N#N.C1CCOC1>O=C(O[C@H]1CN2CCC1CC2)C(O)(c1ccccc1)c1ccco1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-441c2bf571bf4dfa9e5795142f06b44e
O=C(O)C(=O)c1ccco1.O[C@H]1CN2CCC1CC2>>O=C(O[C@H]1CN2CCC1CC2)C(=O)c1ccco1
N12C[C@@H](C(CC1)CC2)O.C(C(=O)Cl)(=O)Cl.O=C(C(=O)O)C=1OC=CC1>>N12C[C@@H](C(CC1)CC2)OC(C(C=2OC=CC2)=O)=O
O[C:2](=[O:1])[C:12](=[O:13])[c:14]1[cH:15][cH:16][cH:17][o:18]1.[OH:3][C@H:4]1[CH2:5][N:6]2[CH2:7][CH2:8][CH:9]1[CH2:10][CH2:11]2>>[O:1]=[C:2]([O:3][C@H:4]1[CH2:5][N:6]2[CH2:7][CH2:8][CH:9]1[CH2:10][CH2:11]2)[C:12](=[O:13])[c:14]1[cH:15][cH:16][cH:17][o:18]1
O=C(O)C(=O)c1ccco1.O[C@H]1CN2CCC1CC2
O=C(O[C@H]1CN2CCC1CC2)C(=O)c1ccco1
null
CN(C=O)C
C(Cl)(Cl)Cl
Protection
Esterification of Carboxylic Acids
c939a2b456dc028ef9b8da8e67cc8c2d4600899fd167913dc054d843bed73832
54434098f814b226cfe1782a0bf08b634994a82fd90bdbb778fb3463efef0433
O=C(O[C@H]1CN2CCC1CC2)C(=O)c1ccco1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[O;D1;H0:4])-[c:5]:[#8;a:6].[#7:7]-[C:8]-[C:9](-[OH;D1;+0:10])-[C:11]>>[#7:7]-[C:8]-[C:9](-[O;H0;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[O;D1;H0:4])-[c:5]:[#8;a:6])-[C:11]
52.8
[{"value": 52.5, "product": "N12C[C@@H](C(CC1)CC2)OC(C(C=2OC=CC2)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.8, "product": "N12C[C@@H](C(CC1)CC2)OC(C(C=2OC=CC2)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
HOUR
Oxalyl chloride (9.75 ml, 0.112 mol) was added to a solution of oxofuran-2-ylacetic acid (10 g, 0.071 mol) and dimethylformamide (one drop) in 150 ml of chloroform (etanol free) at 01 C. The mixture was stirred and allowed to warm at room temperature. After five hours the solvent was evaporated. The residue was dissolv...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ketone.Secondary alcohol
Ketone.Ester
null
null
c1ccoc1.C1CN2CCC1CC2
HO-
CN(C=O)C.C(Cl)(Cl)Cl
null
15
O=C(O)C(=O)c1ccco1.O[C@H]1CN2CCC1CC2>CN(C=O)C.C(Cl)(Cl)Cl>O=C(O[C@H]1CN2CCC1CC2)C(=O)c1ccco1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b1dd4ccd1fb84ffc9c14b89c3030a0e6
O=C(O)C(=O)c1cccs1.O[C@H]1CN2CCC1CC2>>O=C(O[C@H]1CN2CCC1CC2)C(=O)c1cccs1
N12C[C@@H](C(CC1)CC2)O.C(C(=O)Cl)(=O)Cl.O=C(C(=O)O)C=1SC=CC1>>N12C[C@@H](C(CC1)CC2)OC(C(C=2SC=CC2)=O)=O
O[C:2](=[O:1])[C:12](=[O:13])[c:14]1[cH:15][cH:16][cH:17][s:18]1.[OH:3][C@H:4]1[CH2:5][N:6]2[CH2:7][CH2:8][CH:9]1[CH2:10][CH2:11]2>>[O:1]=[C:2]([O:3][C@H:4]1[CH2:5][N:6]2[CH2:7][CH2:8][CH:9]1[CH2:10][CH2:11]2)[C:12](=[O:13])[c:14]1[cH:15][cH:16][cH:17][s:18]1
O=C(O)C(=O)c1cccs1.O[C@H]1CN2CCC1CC2
O=C(O[C@H]1CN2CCC1CC2)C(=O)c1cccs1
null
CN(C=O)C
C(Cl)(Cl)Cl
Protection
Esterification of Carboxylic Acids
c939a2b456dc028ef9b8da8e67cc8c2d4600899fd167913dc054d843bed73832
54434098f814b226cfe1782a0bf08b634994a82fd90bdbb778fb3463efef0433
O=C(O[C@H]1CN2CCC1CC2)C(=O)c1cccs1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[O;D1;H0:4])-[c:5]:[#16;a:6].[#7:7]-[C:8]-[C:9](-[OH;D1;+0:10])-[C:11]>>[#16;a:6]:[c:5]-[C:3](=[O;D1;H0:4])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:10]-[C:9](-[C:11])-[C:8]-[#7:7]
92.6
[{"value": 92.6, "product": "N12C[C@@H](C(CC1)CC2)OC(C(C=2SC=CC2)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.5, "product": "N12C[C@@H](C(CC1)CC2)OC(C(C=2SC=CC2)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
Oxalyl chloride (1.34 ml, 0.0154 mol) was added to a solution of oxothien-2-yl-acetic acid (2 g, 0.0128 mol) and dimethylformamide (one drop) in 30 ml of chloroform (etanol free) at 01 C. The mixture was stirred and allowed to warm at room temperature. After one hour the solvent was evaporated. The residue was dissolve...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ketone.Secondary alcohol
Ketone.Ester
null
null
c1ccsc1.C1CN2CCC1CC2
HO-
CN(C=O)C.C(Cl)(Cl)Cl
null
1.5
O=C(O)C(=O)c1cccs1.O[C@H]1CN2CCC1CC2>CN(C=O)C.C(Cl)(Cl)Cl>O=C(O[C@H]1CN2CCC1CC2)C(=O)c1cccs1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dbaa94bd32244bae89e10ca244ba911a
COC(=O)[C@H](NC(=O)OC(C)(C)C)[C@H](C)OC>>CO[C@@H](C)[C@@H](NC(=O)OC(C)(C)C)C(=O)O
COC([C@H](NC(=O)OC(C)(C)C)[C@@H](OC)C)=O.[Li+].[OH-]>>C(=O)(OC(C)(C)C)N[C@H]([C@@H](OC)C)C(=O)O
C[O:16][C:14]([C@@H:5]([C@@H:3]([O:2][CH3:1])[CH3:4])[NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])=[O:15]>>[CH3:1][O:2][C@@H:3]([CH3:4])[C@@H:5]([NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])[C:14](=[O:15])[OH:16]
COC(=O)[C@H](NC(=O)OC(C)(C)C)[C@H](C)OC
CO[C@@H](C)[C@@H](NC(=O)OC(C)(C)C)C(=O)O
null
null
O1CCOCC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
null
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
90.1
[{"value": 90.0, "product": "C(=O)(OC(C)(C)C)N[C@H]([C@@H](OC)C)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.1, "product": "C(=O)(OC(C)(C)C)N[C@H]([C@@H](OC)C)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of N-Boc-O-methyl-D-threonine methyl ester (8.09 mmol) in 1,4-dioxane (10 mL) is added a solution of LiOH (24.3 mmol) in water (20 mL). After stirring for 2–3 h, the solvents are removed in vacuo and the residue partitioned between water and ether. The aqueous layer is acidified with solid citric acid to ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
null
Other
O1CCOCC1.O
null
null
COC(=O)[C@H](NC(=O)OC(C)(C)C)[C@H](C)OC>O1CCOCC1.O>CO[C@@H](C)[C@@H](NC(=O)OC(C)(C)C)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-813543242f5f4c4dab084d52cfa4402d
CN(C)C[C@@H](N)C(=O)N1CCC(C2CCN(C)CC2)CC1.O=C(O)c1cc2ccc(Cl)cc2s1>>CN(C)C[C@@H](NC(=O)c1cc2ccc(Cl)cc2s1)C(=O)N1CCC(C2CCN(C)CC2)CC1.Cl
CN(C[C@@H](N)C(=O)N1CCC(CC1)C1CCN(CC1)C)C.ClC=1C=CC2=C(SC(=C2)C(=O)O)C1>>Cl.ClC=1C=CC2=C(SC(=C2)C(=O)N[C@H](CN(C)C)C(=O)N2CCC(CC2)C2CCN(CC2)C)C1
[CH3:1][N:2]([CH3:3])[CH2:4][C@@H:5]([NH2:6])[C:19](=[O:20])[N:21]1[CH2:22][CH2:23][CH:24]([CH:25]2[CH2:26][CH2:27][N:28]([CH3:29])[CH2:30][CH2:31]2)[CH2:32][CH2:33]1.O[C:7](=[O:8])[c:9]1[cH:10][c:11]2[cH:12][cH:13][c:14]([Cl:15])[cH:16][c:17]2[s:18]1>>[CH3:1][N:2]([CH3:3])[CH2:4][C@@H:5]([NH:6][C:7](=[O:8])[c:9]1[cH:1...
CN(C)C[C@@H](N)C(=O)N1CCC(C2CCN(C)CC2)CC1.O=C(O)c1cc2ccc(Cl)cc2s1
CN(C)C[C@@H](NC(=O)c1cc2ccc(Cl)cc2s1)C(=O)N1CCC(C2CCN(C)CC2)CC1.Cl
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC(=O)N1CCC(C2CCNCC2)CC1)c1cc2ccccc2s1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#16;a:5]:[c:6].[C:7]-[#7:8](-[C:9](=[O;D1;H0:10])-[C:11](-[C:12])-[NH2;D1;+0:13])-[C:14]>>[C:7]-[#7:8](-[C:9](=[O;D1;H0:10])-[C:11](-[C:12])-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#16;a:5]:[c:6])-[C:14]
null
[]
null
null
null
null
Prepared from 1-[β-dimethylamino-D-alaninyl]-4-(1-methylpiperidin-4-yl)piperidine and 6-chlorobenzo[b]thiophene-2-carboxylic acid using methods substantially equivalent to General Coupling Method 1. The HCl salt is prepared following General Salt Formation Method 1. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2sccc2c1.C1CC[NH]CC1.C1CC[NH]CC1
null
null
null
null
CN(C)C[C@@H](N)C(=O)N1CCC(C2CCN(C)CC2)CC1.O=C(O)c1cc2ccc(Cl)cc2s1>>CN(C)C[C@@H](NC(=O)c1cc2ccc(Cl)cc2s1)C(=O)N1CCC(C2CCN(C)CC2)CC1.Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7b3ab442c5d74a1997cdacd358df9401
C[C@@H](O)[C@@H](N)C(=O)N1CCN(C2CCN(C)CC2)CC1.O=C(O)c1cc2cc(Cl)ccc2[nH]1>>C[C@@H](O)[C@@H](NC(=O)c1cc2cc(Cl)ccc2[nH]1)C(=O)N1CCN(C2CCN(C)CC2)CC1
Cl.N[C@H]([C@H](O)C)C(=O)N1CCN(CC1)C1CCN(CC1)C.ClC=1C=C2C=C(NC2=CC1)C(=O)O.Cl>>Cl.ClC=1C=C2C=C(NC2=CC1)C(=O)N[C@H]([C@H](O)C)C(=O)N1CCN(CC1)C1CCN(CC1)C
[CH3:1][C@@H:2]([OH:3])[C@@H:4]([NH2:5])[C:18](=[O:19])[N:20]1[CH2:21][CH2:22][N:23]([CH:24]2[CH2:25][CH2:26][N:27]([CH3:28])[CH2:29][CH2:30]2)[CH2:31][CH2:32]1.O[C:6](=[O:7])[c:8]1[cH:9][c:10]2[cH:11][c:12]([Cl:13])[cH:14][cH:15][c:16]2[nH:17]1>>[CH3:1][C@@H:2]([OH:3])[C@@H:4]([NH:5][C:6](=[O:7])[c:8]1[cH:9][c:10]2[cH...
C[C@@H](O)[C@@H](N)C(=O)N1CCN(C2CCN(C)CC2)CC1.O=C(O)c1cc2cc(Cl)ccc2[nH]1
C[C@@H](O)[C@@H](NC(=O)c1cc2cc(Cl)ccc2[nH]1)C(=O)N1CCN(C2CCN(C)CC2)CC1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC(=O)N1CCN(C2CCNCC2)CC1)c1cc2ccccc2[nH]1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#7;a:5]:[c:6].[C:7]-[#7:8](-[C:9](=[O;D1;H0:10])-[C:11](-[C:12])-[NH2;D1;+0:13])-[C:14]>>[C:7]-[#7:8](-[C:9](=[O;D1;H0:10])-[C:11](-[C:12])-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#7;a:5]:[c:6])-[C:14]
null
[]
null
null
null
null
Prepared from 1-(D-allo-threoninyl)-4-(1-methylpiperidin-4-yl)piperazine hydrochloride and 5-chloroindole-2-carboxylic acid using methods substantially equivalent to General Coupling Method 1. The HCl salt is prepared following Salt Formation Method 1. The final crude product is treated with aqueous 0.2 N HCl and purif...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2[nH]ccc2c1.C1C[NH]CC[NH]1.C1CC[NH]CC1
HO-
null
null
null
C[C@@H](O)[C@@H](N)C(=O)N1CCN(C2CCN(C)CC2)CC1.O=C(O)c1cc2cc(Cl)ccc2[nH]1>>C[C@@H](O)[C@@H](NC(=O)c1cc2cc(Cl)ccc2[nH]1)C(=O)N1CCN(C2CCN(C)CC2)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3b2e1627169841bba8a95cfd46efda70
CC(C)c1oc(-c2ccccc2Cl)nc1CI.[C-]#N>>CC(C)c1oc(-c2ccccc2Cl)nc1CC#N
[C-]#N.[Na+].ClC1=C(C=CC=C1)C=1OC(=C(N1)CI)C(C)C.O>>ClC1=C(C=CC=C1)C=1OC(=C(N1)CC#N)C(C)C
I[CH2:16][c:15]1[c:4]([CH:2]([CH3:1])[CH3:3])[o:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[Cl:13])[n:14]1.[C-:17]#[N:18]>>[CH3:1][CH:2]([CH3:3])[c:4]1[o:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[Cl:13])[n:14][c:15]1[CH2:16][C:17]#[N:18]
CC(C)c1oc(-c2ccccc2Cl)nc1CI.[C-]#N
CC(C)c1oc(-c2ccccc2Cl)nc1CC#N
null
null
CC(=O)C
C-C Coupling
OtherReaction
347b040e695b34bb71d78d55beea9c7162795a061d052426f1f803b52c4cbe4d
1dbefa1fc17e03074aa3f6619987f71dfa9a1cb0d61de142a880cd3f05e4f004
c1ccc(-c2ncco2)cc1
I-[CH2;D2;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[#8;a:5]:[c:6]:1-[C:7].[C-;H0;D1:8]#[N;D1;H0:9]>>[C:7]-[c:6]1:[#8;a:5]:[c:4]:[#7;a:3]:[c:2]:1-[CH2;D2;+0:1]-[C;H0;D2;+0:8]#[N;D1;H0:9]
82
[{"value": 82.0, "product": "ClC1=C(C=CC=C1)C=1OC(=C(N1)CC#N)C(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 8.7, "product": "ClC1=C(C=CC=C1)C=1OC(=C(N1)CC#N)C(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In acetone (2 mL) was dissolved 2-(2-chlorophenyl)-4-iodomethyl-5-isopropyloxazole (590 mg, 1.63 mmol). Sodium cyanide (88 mg, 1.63 mmol) was added, and the resulting mixture was heated under reflux for 22 hours. The reaction mixture was cooled to room temperature, poured into water, and extracted with ethyl acetate. T...
10.6084/m9.figshare.5104873.v1
null
Primary halide
Nitrile
null
null
c1cocn1.c1ccccc1
I-
CC(=O)C
null
null
CC(C)c1oc(-c2ccccc2Cl)nc1CI.[C-]#N>CC(=O)C>CC(C)c1oc(-c2ccccc2Cl)nc1CC#N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d60196164a8444fbb56e9ca8a2f88c55
CC(C)c1oc(-c2ccccc2Cl)nc1CCO.Cc1ccc(S(=O)(=O)Cl)cc1>>Cc1ccc(S(=O)(=O)OCCc2nc(-c3ccccc3Cl)oc2C(C)C)cc1
Cl.ClC1=C(C=CC=C1)C=1OC(=C(N1)CCO)C(C)C.O.C1(=CC=C(C=C1)S(=O)(=O)Cl)C>>ClC1=C(C=CC=C1)C=1OC(=C(N1)CCOS(=O)(=O)C1=CC=C(C=C1)C)C(C)C
[OH:9][CH2:10][CH2:11][c:12]1[n:13][c:14](-[c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[Cl:21])[o:22][c:23]1[CH:24]([CH3:25])[CH3:26].Cl[S:6]([c:5]1[cH:4][cH:3][c:2]([CH3:1])[cH:28][cH:27]1)(=[O:7])=[O:8]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[O:9][CH2:10][CH2:11][c:12]2[n:13][c:14](-[c:15]3[cH:16][cH:17][...
CC(C)c1oc(-c2ccccc2Cl)nc1CCO.Cc1ccc(S(=O)(=O)Cl)cc1
Cc1ccc(S(=O)(=O)OCCc2nc(-c3ccccc3Cl)oc2C(C)C)cc1
null
null
N1=CC=CC=C1.C(Cl)Cl
Acylation
Formation of Sulfonic Esters
d05d91207659f8fa672c205a316a670adfe2b92492fc9adad2ee3f241e574fb9
a7748b0f3b0eba3868d0cf03ae67721db046202accaaea9cadb4edbc96ec8768
O=S(=O)(OCCc1coc(-c2ccccc2)n1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[OH;D1;+0:9]>>[C:7]-[C:8]-[O;H0;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
49
[{"value": 49.0, "product": "ClC1=C(C=CC=C1)C=1OC(=C(N1)CCOS(=O)(=O)C1=CC=C(C=C1)C)C(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 49.0, "product": "ClC1=C(C=CC=C1)C=1OC(=C(N1)CCOS(=O)(=O)C1=CC=C(C=C1)C)C(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
In a mixture of methylene chloride (1 mL) and pyridine (2 mL) was dissolved 2-[2-(2-chlorophenyl)-5-isopropyloxazol-4-yl]ethanol (159 mg, 0.598 mmol). Under cooling with water, to the solution was added p-toluenesulfonyl chloride (125 mg, 0.658 mmol). The mixture was stirred for 5 hours. The reaction mixture was poured...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Primary alcohol.Sulfonyl halide
Tosylate
null
null
c1ccccc1.c1cocn1.c1ccccc1
HCl
N1=CC=CC=C1.C(Cl)Cl
null
5
CC(C)c1oc(-c2ccccc2Cl)nc1CCO.Cc1ccc(S(=O)(=O)Cl)cc1>N1=CC=CC=C1.C(Cl)Cl>Cc1ccc(S(=O)(=O)OCCc2nc(-c3ccccc3Cl)oc2C(C)C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-591dbc95e67f486b9e9789c5d5d37fd9
Cc1ccc(S(=O)(=O)OCCc2nc(-c3ccccc3Cl)oc2C(C)C)cc1.[I-]>>CC(C)c1oc(-c2ccccc2Cl)nc1CCI
[I-].[Na+].ClC1=C(C=CC=C1)C=1OC(=C(N1)CCOS(=O)(=O)C1=CC=C(C=C1)C)C(C)C.O>>ClC1=C(C=CC=C1)C=1OC(=C(N1)CCI)C(C)C
Cc1ccc(S(=O)(=O)O[CH2:17][CH2:16][c:15]2[c:4]([CH:2]([CH3:1])[CH3:3])[o:5][c:6](-[c:7]3[cH:8][cH:9][cH:10][cH:11][c:12]3[Cl:13])[n:14]2)cc1.[I-:18]>>[CH3:1][CH:2]([CH3:3])[c:4]1[o:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[Cl:13])[n:14][c:15]1[CH2:16][CH2:17][I:18]
Cc1ccc(S(=O)(=O)OCCc2nc(-c3ccccc3Cl)oc2C(C)C)cc1.[I-]
CC(C)c1oc(-c2ccccc2Cl)nc1CCI
null
null
CC(=O)C
Functional Group Interconversion
OtherReaction
252212a616714f8874db6269dd7f8dd14d7a8ff04f2ae913f3f8b39c1296a9e4
7d4806481a626b7c7f4e5b69bd83274a88a40e4c6a2960dcfa212a4447a3de57
c1ccc(-c2ncco2)cc1
C-c1:c:c:c(-S(=O)(=O)-O-[CH2;D2;+0:1]-[C:2]-[c:3](:[#7;a:4]):[c:5]:[#8;a:6]):c:c:1.[I-;H0;D0:7]>>[#7;a:4]:[c:3](-[C:2]-[CH2;D2;+0:1]-[I;H0;D1;+0:7]):[c:5]:[#8;a:6]
96
[{"value": 96.0, "product": "ClC1=C(C=CC=C1)C=1OC(=C(N1)CCI)C(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.4, "product": "ClC1=C(C=CC=C1)C=1OC(=C(N1)CCI)C(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In acetone (2 mL) was dissolved 2-(2-chlorophenyl)-5-isopropyl-4-[2-(p-toluenesulfonyloxy)ethyl]oxazole (123 mg, 0.293 mmol). To the solution was added sodium iodide (176 mg, 1.17 mmol). The mixture was heated overnight under reflux. The reaction mixture was allowed to reach room temperature, poured into water, and ext...
10.6084/m9.figshare.5104873.v1
null
Tosylate
Primary halide
c1ccccc1
null
c1cocn1.c1ccccc1
TsOH.HO-
CC(=O)C
null
null
Cc1ccc(S(=O)(=O)OCCc2nc(-c3ccccc3Cl)oc2C(C)C)cc1.[I-]>CC(=O)C>CC(C)c1oc(-c2ccccc2Cl)nc1CCI
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-94ad8cdeae8d45b6af653a0441258466
COC(=O)c1cc[nH]c1.Clc1ccc2ccccc2n1>>COC(=O)c1ccn(-c2ccc3ccccc3n2)c1
O.C([O-])([O-])=O.[K+].[K+].COC(=O)C1=CNC=C1.ClC1=NC2=CC=CC=C2C=C1>>COC(=O)C1=CN(C=C1)C1=NC2=CC=CC=C2C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][nH:8][cH:19]1.Cl[c:9]1[cH:10][cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[n:18]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][cH:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]3[n:18]2)[cH:19]1
COC(=O)c1cc[nH]c1.Clc1ccc2ccccc2n1
COC(=O)c1ccn(-c2ccc3ccccc3n2)c1
null
null
CS(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
0f41158080bd72518d9a6b2389c4c528ac037a6b5eac12dbe2506d72e4b3d2c9
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2nc(-n3cccc3)ccc2c1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[nH;D2;+0:11]:[c:12]:[c:13]:1>>[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[n;H0;D3;+0:11](-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]):[c:12]:[c:13]:1
65.8
[{"value": 65.8, "product": "COC(=O)C1=CN(C=C1)C1=NC2=CC=CC=C2C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
23
HOUR
1.73 g (12.5 mmol) of potassium carbonate are added at 20° C. under an argon atmosphere to 0.625 g (5 mmol) of 3-methoxycarbonyl-1H-pyrrole and 0.82 g (5 mmol) of 2-chloroquinoline dissolved in 10 mL of dimethyl sulphoxide. After stirring at 100° C. for 23 hours, the reaction mixture is poured into 30 mL of water and i...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
CS(=O)C
100
23
COC(=O)c1cc[nH]c1.Clc1ccc2ccccc2n1>CS(=O)C>COC(=O)c1ccn(-c2ccc3ccccc3n2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-93014e71c52f43e1976c370c2c3121ae
COC(=O)c1cc[nH]c1.Clc1ccnc2ccccc12>>COC(=O)c1ccn(-c2ccnc3ccccc23)c1
O.C([O-])([O-])=O.[K+].[K+].COC(=O)C1=CNC=C1.ClC1=CC=NC2=CC=CC=C12>>COC(=O)C1=CN(C=C1)C1=CC=NC2=CC=CC=C12
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][nH:8][cH:19]1.Cl[c:9]1[cH:10][cH:11][n:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]12>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][cH:11][n:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19]1
COC(=O)c1cc[nH]c1.Clc1ccnc2ccccc12
COC(=O)c1ccn(-c2ccnc3ccccc23)c1
null
null
CS(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
0f41158080bd72518d9a6b2389c4c528ac037a6b5eac12dbe2506d72e4b3d2c9
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3cccc3)ccnc2c1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[nH;D2;+0:14]:[c:15]:[c:16]:1>>[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[n;H0;D3;+0:14](-[c;H0;D3;+0:1]2:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:2:[c:8]):[c:15]:[c:16]:1
59.5
[{"value": 59.5, "product": "COC(=O)C1=CN(C=C1)C1=CC=NC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
23
HOUR
1.73 g (12.5 mmol) of potassium carbonate are added at 20° C. under an argon atmosphere to 0.625 g (5 mmol) of 3-methoxycarbonyl-1H-pyrrole and 0.82 g (5 mmol) of 4-chloroquinoline dissolved in 10 mL of dimethyl sulphoxide. After stirring at 100° C. for 23 hours, the reaction mixture is poured into 30 mL of water and t...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
CS(=O)C
100
23
COC(=O)c1cc[nH]c1.Clc1ccnc2ccccc12>CS(=O)C>COC(=O)c1ccn(-c2ccnc3ccccc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0fdfc446bfd34bf9ba01fbb53c5b1065
Cc1c(C(=O)O)ccn1-c1ccnc2ccccc12.O=C(Cl)C(=O)Cl>>Cc1c(C(=O)Cl)ccn1-c1ccnc2ccccc12.Cl
C(C(=O)Cl)(=O)Cl.C(=O)(O)C1=C(N(C=C1)C1=CC=NC2=CC=CC=C12)C>>Cl.ClC(=O)C1=C(N(C=C1)C1=CC=NC2=CC=CC=C12)C
O[C:4]([c:3]1[c:2]([CH3:1])[n:9](-[c:10]2[cH:11][cH:12][n:13][c:14]3[cH:15][cH:16][cH:17][cH:18][c:19]23)[cH:8][cH:7]1)=[O:5].O=C(C(=O)[Cl:20])[Cl:6]>>[CH3:1][c:2]1[c:3]([C:4](=[O:5])[Cl:6])[cH:7][cH:8][n:9]1-[c:10]1[cH:11][cH:12][n:13][c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]12.[ClH:20]
Cc1c(C(=O)O)ccn1-c1ccnc2ccccc12.O=C(Cl)C(=O)Cl
Cc1c(C(=O)Cl)ccn1-c1ccnc2ccccc12.Cl
null
null
ClCCl
Functional Group Interconversion
Alcohol to chloride_Other
013cec2edeb273a7a148f349d36a52d99ff4e7bcf8eed78085df830088e387ac
aedb1f68dc5b7eb0583043e1125b741382b17974140a2f46554f0110e2ddc884
c1ccc2c(-n3cccc3)ccnc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[c:7]):[c:8]:1-[C;D1;H3:9].O=C(-[Cl;H0;D1;+0:10])-C(=O)-[Cl;H0;D1;+0:11]>>[C;D1;H3:9]-[c:8]1:[#7;a:6](-[c:7]):[c:5]:[c:4]:[c:3]:1-[C;H0;D3;+0:1](-[Cl;H0;D1;+0:11])=[O;D1;H0:2].[ClH;D0;+0:10]
98.9
[{"value": 98.9, "product": "Cl.ClC(=O)C1=C(N(C=C1)C1=CC=NC2=CC=CC=C12)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
16
HOUR
11.8 mL (134.8 mmol) of oxalyl chloride are added at 20° C. under an argon atmosphere to 2.09 g (7.24 mmol) of 3-carboxy-2-methyl-1-(quinol-4-yl)-1H-pyrrole dissolved in 150 mL of dichloromethane. After stirring at 20° C. for 16 hours, the reaction mixture is concentrated to dryness under reduced pressure (2.7 kPa) to ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Carboxylic acid
Acyl halide
null
null
c1c[nH]cc1.c1ccc2ncccc2c1
Other
ClCCl
20
16
Cc1c(C(=O)O)ccn1-c1ccnc2ccccc12.O=C(Cl)C(=O)Cl>ClCCl>Cc1c(C(=O)Cl)ccn1-c1ccnc2ccccc12.Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-116bbc84874e4ba3b9e0c615b3d8c0b2
CCOC(=O)c1ccn(-c2ccnc3ccccc23)c1C>>Cc1c(C(=O)O)ccn1-c1ccnc2ccccc12
O.[OH-].[Li+].C(C)OC(=O)C1=C(N(C=C1)C1=CC=NC2=CC=CC=C12)C>>C(=O)(O)C1=C(N(C=C1)C1=CC=NC2=CC=CC=C12)C
CC[O:6][C:4]([c:3]1[c:2]([CH3:1])[n:9](-[c:10]2[cH:11][cH:12][n:13][c:14]3[cH:15][cH:16][cH:17][cH:18][c:19]23)[cH:8][cH:7]1)=[O:5]>>[CH3:1][c:2]1[c:3]([C:4](=[O:5])[OH:6])[cH:7][cH:8][n:9]1-[c:10]1[cH:11][cH:12][n:13][c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]12
CCOC(=O)c1ccn(-c2ccnc3ccccc23)c1C
Cc1c(C(=O)O)ccn1-c1ccnc2ccccc12
null
null
O1CCCC1.O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(-n3cccc3)ccnc2c1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
98.6
[{"value": 98.6, "product": "C(=O)(O)C1=C(N(C=C1)C1=CC=NC2=CC=CC=C12)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2.226 g (53 mmol) of lithium hydroxide monohydrate, in portions of 0.742 g every 24 hours, are added at 20° C. to 2.48 g (8.4 mmol) of 3-ethoxycarbonyl-2-methyl-1-(quinol-4-yl)-1H-pyrrole dissolved in 75 mL of tetrahydrofuran and 75 mL of water. After stirring at reflux for 72 hours, the reaction mixture is concentrate...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1c[nH]cc1.c1ccc2ncccc2c1
Other
O1CCCC1.O
null
null
CCOC(=O)c1ccn(-c2ccnc3ccccc23)c1C>O1CCCC1.O>Cc1c(C(=O)O)ccn1-c1ccnc2ccccc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d88754c9caf5409f8c983d0f3a3e0b16
CCOC(=O)c1cc[nH]c1C.Clc1ccnc2ccccc12>>CCOC(=O)c1ccn(-c2ccnc3ccccc23)c1C
ClC1=CC=NC2=CC=CC=C12.C(C)OC(=O)C1=C(NC=C1)C.[H-].[Na+]>>C(C)OC(=O)C1=C(N(C=C1)C1=CC=NC2=CC=CC=C12)C
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][nH:9][c:20]1[CH3:21].Cl[c:10]1[cH:11][cH:12][n:13][c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][n:9](-[c:10]2[cH:11][cH:12][n:13][c:14]3[cH:15][cH:16][cH:17][cH:18][c:19]23)[c:20]1[CH3:21]
CCOC(=O)c1cc[nH]c1C.Clc1ccnc2ccccc12
CCOC(=O)c1ccn(-c2ccnc3ccccc23)c1C
null
[Cu]
O.CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
84a7a9e9603cb882bfa9bb185a61e5a07491a2d9b4ffd8cd0caa72c85e51157b
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3cccc3)ccnc2c1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14]:[nH;D2;+0:15]:[c:16]:1-[C;D1;H3:17]>>[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14]:[n;H0;D3;+0:15](-[c;H0;D3;+0:1]2:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:2:[c:8]):[c:16]:1-[C;D1;H3:17]
103.6
[{"value": 103.6, "product": "C(C)OC(=O)C1=C(N(C=C1)C1=CC=NC2=CC=CC=C12)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
0.2
HOUR
2.75 g (17.9 mmol) of 3-ethoxycarbonyl-2-methyl-1H-pyrrole are added at 20° C. under an argon atmosphere to 0.756 g (18.9 mmol) of sodium hydride, at 60% by weight in liquid petroleum jelly, suspended in 12 mL of dimethylformamide. After stirring at 20° C. for 0.2 hour, 0.114 g (1.79 mmol) of copper powder and 2.35 mL ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2ncccc2c1
c1c[nH]cc1.c1ccc2ncccc2c1
c1c[nH]cc1.c1ccc2ncccc2c1
HCl
[Cu].O.CN(C=O)C
20
0.2
CCOC(=O)c1cc[nH]c1C.Clc1ccnc2ccccc12>[Cu].O.CN(C=O)C>CCOC(=O)c1ccn(-c2ccnc3ccccc23)c1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ac28c993563b4f95b88d0b1c4390b3b0
Cc1c(C(=O)Cl)ccn1-c1ccc2ccccc2n1.N=C(N)N>>Cc1c(C(=O)NC(=N)N)ccn1-c1ccc2ccccc2n1
Cl.ClC(=O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C.[Na].CO.Cl.NC(=N)N>>Cl.N(C(=N)N)C(=O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C
Cl[C:4]([c:3]1[c:2]([CH3:1])[n:12](-[c:13]2[cH:14][cH:15][c:16]3[cH:17][cH:18][cH:19][cH:20][c:21]3[n:22]2)[cH:11][cH:10]1)=[O:5].[NH2:6][C:7](=[NH:8])[NH2:9]>>[CH3:1][c:2]1[c:3]([C:4](=[O:5])[NH:6][C:7](=[NH:8])[NH2:9])[cH:10][cH:11][n:12]1-[c:13]1[cH:14][cH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[n:22]1
Cc1c(C(=O)Cl)ccn1-c1ccc2ccccc2n1.N=C(N)N
Cc1c(C(=O)NC(=N)N)ccn1-c1ccc2ccccc2n1
null
null
COCCOC
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccc2nc(-n3cccc3)ccc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[c:7]:[#7;a:8]):[c:9]:1-[C;D1;H3:10].[N;D1;H1:11]=[C:12](-[N;D1;H2:13])-[NH2;D1;+0:14]>>[#7;a:8]:[c:7]-[#7;a:6]1:[c:5]:[c:4]:[c:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:14]-[C:12](=[N;D1;H1:11])-[N;D1;H2:13]):[c:9]:1-[C;D1;H3:10]
38.2
[{"value": 38.2, "product": "Cl.N(C(=N)N)C(=O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
0.5
HOUR
0.795 g (33.1 mmol) of sodium is added at 20° C. under an argon atmosphere to 30 mL of methanol. After complete dissolution, 2.97 g (31.2 mmol) of guanidine hydrochloride are added. After stirring at 20° C. for 0.5 hour, the reaction mixture is filtered under an argon atmosphere. The filtrate is concentrated to dryness...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1c[nH]cc1.c1ccc2ncccc2c1
HCl
COCCOC
20
0.5
Cc1c(C(=O)Cl)ccn1-c1ccc2ccccc2n1.N=C(N)N>COCCOC>Cc1c(C(=O)NC(=N)N)ccn1-c1ccc2ccccc2n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-52db778ef2ac4a7ab922a2d06b8de288
Cc1c(C(=O)O)ccn1-c1ccc2ccccc2n1.O=C(Cl)C(=O)Cl>>Cc1c(C(=O)Cl)ccn1-c1ccc2ccccc2n1.Cl
C(C(=O)Cl)(=O)Cl.C(=O)(O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C>>Cl.ClC(=O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C
O[C:4]([c:3]1[c:2]([CH3:1])[n:9](-[c:10]2[cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]3[n:19]2)[cH:8][cH:7]1)=[O:5].O=C(C(=O)[Cl:20])[Cl:6]>>[CH3:1][c:2]1[c:3]([C:4](=[O:5])[Cl:6])[cH:7][cH:8][n:9]1-[c:10]1[cH:11][cH:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]2[n:19]1.[ClH:20]
Cc1c(C(=O)O)ccn1-c1ccc2ccccc2n1.O=C(Cl)C(=O)Cl
Cc1c(C(=O)Cl)ccn1-c1ccc2ccccc2n1.Cl
null
null
ClCCl
Functional Group Interconversion
Alcohol to chloride_Other
013cec2edeb273a7a148f349d36a52d99ff4e7bcf8eed78085df830088e387ac
aedb1f68dc5b7eb0583043e1125b741382b17974140a2f46554f0110e2ddc884
c1ccc2nc(-n3cccc3)ccc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[c:7]:[#7;a:8]):[c:9]:1-[C;D1;H3:10].O=C(-[Cl;H0;D1;+0:11])-C(=O)-[Cl;H0;D1;+0:12]>>[#7;a:8]:[c:7]-[#7;a:6]1:[c:5]:[c:4]:[c:3](-[C;H0;D3;+0:1](-[Cl;H0;D1;+0:12])=[O;D1;H0:2]):[c:9]:1-[C;D1;H3:10].[ClH;D0;+0:11]
104.2
[{"value": 104.2, "product": "Cl.ClC(=O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
16
HOUR
10 mL (114.2 mmol) of oxalyl chloride are added at 20° C. under an argon atmosphere to 1.8 g (6.25 mmol) of 3-carboxy-2-methyl-1-(quinol-2-yl)-1H-pyrrole dissolved in 120 mL of dichloromethane. After stirring at 20° C. for 16 hours, the reaction mixture is concentrated to dryness under reduced pressure (2.7 kPa) to giv...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Carboxylic acid
Acyl halide
null
null
c1c[nH]cc1.c1ccc2ncccc2c1
Other
ClCCl
20
16
Cc1c(C(=O)O)ccn1-c1ccc2ccccc2n1.O=C(Cl)C(=O)Cl>ClCCl>Cc1c(C(=O)Cl)ccn1-c1ccc2ccccc2n1.Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2554c89ae0a34a9ea0efbd031f33274b
CCOC(=O)c1ccn(-c2ccc3ccccc3n2)c1C>>Cc1c(C(=O)O)ccn1-c1ccc2ccccc2n1
O.[OH-].[Li+].C(C)OC(=O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C.Cl>>C(=O)(O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C
CC[O:6][C:4]([c:3]1[c:2]([CH3:1])[n:9](-[c:10]2[cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]3[n:19]2)[cH:8][cH:7]1)=[O:5]>>[CH3:1][c:2]1[c:3]([C:4](=[O:5])[OH:6])[cH:7][cH:8][n:9]1-[c:10]1[cH:11][cH:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]2[n:19]1
CCOC(=O)c1ccn(-c2ccc3ccccc3n2)c1C
Cc1c(C(=O)O)ccn1-c1ccc2ccccc2n1
null
null
O1CCCC1.O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2nc(-n3cccc3)ccc2c1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
111.1
[{"value": 111.1, "product": "C(=O)(O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
3.9 g (93 mmol) of lithium hydroxide monohydrate, portionwise every 24 hours, are added at 20° C. to 1.9 g (6.78 mmol) of 3-ethoxycarbonyl-2-methyl-1-(quinol-2-yl)-1H-pyrrole dissolved in 50 mL of tetrahydrofuran and 50 mL of water. After stirring at reflux for 72 hours, the reaction mixture is concentrated to dryness ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1c[nH]cc1.c1ccc2ncccc2c1
Other
O1CCCC1.O
null
null
CCOC(=O)c1ccn(-c2ccc3ccccc3n2)c1C>O1CCCC1.O>Cc1c(C(=O)O)ccn1-c1ccc2ccccc2n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1ab15b1ea8ea4ab3a4f658cb729946cf
CCOC(=O)c1cc[nH]c1C.Clc1ccc2ccccc2n1>>CCOC(=O)c1ccn(-c2ccc3ccccc3n2)c1C
ClC1=NC2=CC=CC=C2C=C1.C(C)OC(=O)C1=C(NC=C1)C.[H-].[Na+]>>C(C)OC(=O)C1=C(N(C=C1)C1=NC2=CC=CC=C2C=C1)C
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][nH:9][c:20]1[CH3:21].Cl[c:10]1[cH:11][cH:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]2[n:19]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][n:9](-[c:10]2[cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]3[n:19]2)[c:20]1[CH3:21]
CCOC(=O)c1cc[nH]c1C.Clc1ccc2ccccc2n1
CCOC(=O)c1ccn(-c2ccc3ccccc3n2)c1C
null
[Cu]
O.CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
84a7a9e9603cb882bfa9bb185a61e5a07491a2d9b4ffd8cd0caa72c85e51157b
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2nc(-n3cccc3)ccc2c1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:1-[C;D1;H3:14]>>[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[c:11]:[n;H0;D3;+0:12](-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]):[c:13]:1-[C;D1;H3:14]
null
[]
20
CELSIUS
0.2
HOUR
2.75 g (17.9 mmol) of 3-ethoxycarbonyl-2-methyl-1H-pyrrole are added at 20° C. under an argon atmosphere to 0.756 g (18.9 mmol) of sodium hydride, at 60% by weight in liquid petroleum jelly, suspended in 12 mL of dimethylformamide. After stirring at 20° C. for 0.2 hour, 0.114 g (1.79 mmol) of copper powder and 2.93 g (...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2ncccc2c1
c1c[nH]cc1.c1ccc2ncccc2c1
c1c[nH]cc1.c1ccc2ncccc2c1
HCl
[Cu].O.CN(C=O)C
20
0.2
CCOC(=O)c1cc[nH]c1C.Clc1ccc2ccccc2n1>[Cu].O.CN(C=O)C>CCOC(=O)c1ccn(-c2ccc3ccccc3n2)c1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-312958cfe16b4c57aa0d1e032b302eaf
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2nccc3ccccc23)c1>>Cl.O=C(Cl)c1ccn(-c2nccc3ccccc23)c1
C(C(=O)Cl)(=O)Cl.C(=O)(O)C1=CN(C=C1)C1=NC=CC2=CC=CC=C12>>Cl.ClC(=O)C1=CN(C=C1)C1=NC=CC2=CC=CC=C12
O=C(C(=O)[Cl:4])[Cl:1].O[C:3](=[O:2])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[n:10][cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19]1>>[ClH:1].[O:2]=[C:3]([Cl:4])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[n:10][cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19]1
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2nccc3ccccc23)c1
Cl.O=C(Cl)c1ccn(-c2nccc3ccccc23)c1
null
null
ClCCl
Functional Group Interconversion
Alcohol to chloride_Other
013cec2edeb273a7a148f349d36a52d99ff4e7bcf8eed78085df830088e387ac
aedb1f68dc5b7eb0583043e1125b741382b17974140a2f46554f0110e2ddc884
c1ccc2c(-n3cccc3)nccc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]:[#7;a:7]):[c:8]:[c:9]:1.O=C(-[Cl;H0;D1;+0:10])-C(=O)-[Cl;H0;D1;+0:11]>>[#7;a:7]:[c:6]-[#7;a:5]1:[c:4]:[c:3](-[C;H0;D3;+0:1](-[Cl;H0;D1;+0:11])=[O;D1;H0:2]):[c:9]:[c:8]:1.[ClH;D0;+0:10]
100.8
[{"value": 100.8, "product": "Cl.ClC(=O)C1=CN(C=C1)C1=NC=CC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
0.5
HOUR
0.4 mL (4.5 mmol) of oxalyl chloride is added at 20° C. under an argon atmosphere to 0.58 g (2.2 mmol) of 3-carboxy-1-(isoquinol-1-yl)-1H-pyrrole dissolved in 45 mL of dichloromethane. After stirring at 20° C. for 0.5 hour, the reaction mixture is concentrated to dryness under reduced pressure (2.7 kPa) to give 0.65 g ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2cnccc2c1
Other
ClCCl
20
0.5
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2nccc3ccccc23)c1>ClCCl>Cl.O=C(Cl)c1ccn(-c2nccc3ccccc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-96c3dc202bcb4abf93b24b0126811e26
COC(=O)c1ccn(-c2nccc3ccccc23)c1>>O=C(O)c1ccn(-c2nccc3ccccc23)c1
O.[OH-].[Li+].COC(=O)C1=CN(C=C1)C1=NC=CC2=CC=CC=C12>>C(=O)(O)C1=CN(C=C1)C1=NC=CC2=CC=CC=C12
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][n:7](-[c:8]2[n:9][cH:10][cH:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[cH:18]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][n:7](-[c:8]2[n:9][cH:10][cH:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[cH:18]1
COC(=O)c1ccn(-c2nccc3ccccc23)c1
O=C(O)c1ccn(-c2nccc3ccccc23)c1
null
null
O1CCCC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(-n3cccc3)nccc2c1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
107.7
[{"value": 107.7, "product": "C(=O)(O)C1=CN(C=C1)C1=NC=CC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
0.237 g (5.65 mmol) of lithium hydroxide monohydrate is added at 20° C. to 0.57 g (2.26 mmol) of 3-methoxycarbonyl-1-(isoquinol-1-yl)-1H-pyrrole dissolved in 15 mL of tetrahydrofuran and 15 mL of water. After stirring at reflux for 2 hours, the reaction mixture is concentrated to dryness under reduced pressure (2.7 kPa...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cc[nH]c1.c1ccc2cnccc2c1
Other
O1CCCC1.O
null
null
COC(=O)c1ccn(-c2nccc3ccccc23)c1>O1CCCC1.O>O=C(O)c1ccn(-c2nccc3ccccc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7eea0a2e7ebc4fc99f7138cf5f09a335
COC(=O)c1cc[nH]c1.Clc1nccc2ccccc12>>COC(=O)c1ccn(-c2nccc3ccccc23)c1
O.C([O-])([O-])=O.[K+].[K+].COC(=O)C1=CNC=C1.ClC1=NC=CC2=CC=CC=C12>>COC(=O)C1=CN(C=C1)C1=NC=CC2=CC=CC=C12
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][nH:8][cH:19]1.Cl[c:9]1[n:10][cH:11][cH:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]12>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[n:10][cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19]1
COC(=O)c1cc[nH]c1.Clc1nccc2ccccc12
COC(=O)c1ccn(-c2nccc3ccccc23)c1
null
null
CS(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
64941681a78379ce7a568f1d8a1309e87b488f1d656284455a26054be1853b83
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3cccc3)nccc2c1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](:[c:5]):[c:6].[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[nH;D2;+0:12]:[c:13]:[c:14]:1>>[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[n;H0;D3;+0:12](-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](:[c:5]):[c:6]):[c:13]:[c:14]:1
88.5
[{"value": 88.5, "product": "COC(=O)C1=CN(C=C1)C1=NC=CC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
22
HOUR
1.04 g (7.5 mmol) of potassium carbonate are added at 20° C. under an argon atmosphere to 0.376 g (3 mmol) of 3-methoxycarbonyl-1H-pyrrole and 0.49 g (3 mmol) of 1-chloroisoquinoline dissolved in 6 mL of dimethyl sulphoxide. After stirring at 100° C. for 22 hours, the reaction mixture is poured into 15 mL of water and ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2cnccc2c1
c1cc[nH]c1.c1ccc2cnccc2c1
c1cc[nH]c1.c1ccc2cnccc2c1
HCl
CS(=O)C
100
22
COC(=O)c1cc[nH]c1.Clc1nccc2ccccc12>CS(=O)C>COC(=O)c1ccn(-c2nccc3ccccc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3300df1e364043fc82c01144ac6b645b
N=C(N)N.O=C(Cl)c1ccn(-c2cccc3ncccc23)c1>>N=C(N)NC(=O)c1ccn(-c2cccc3ncccc23)c1
Cl.ClC(=O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1.Cl.NC(=N)N.C[O-].[Na+]>>N(C(=N)N)C(=O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1
[NH:1]=[C:2]([NH2:3])[NH2:4].Cl[C:5](=[O:6])[c:7]1[cH:8][cH:9][n:10](-[c:11]2[cH:12][cH:13][cH:14][c:15]3[n:16][cH:17][cH:18][cH:19][c:20]23)[cH:21]1>>[NH:1]=[C:2]([NH2:3])[NH:4][C:5](=[O:6])[c:7]1[cH:8][cH:9][n:10](-[c:11]2[cH:12][cH:13][cH:14][c:15]3[n:16][cH:17][cH:18][cH:19][c:20]23)[cH:21]1
N=C(N)N.O=C(Cl)c1ccn(-c2cccc3ncccc23)c1
N=C(N)NC(=O)c1ccn(-c2cccc3ncccc23)c1
null
null
O1CCCC1.ClCCl.CO
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1cc(-n2cccc2)c2cccnc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH2;D1;+0:12]>>[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1
31.4
[{"value": 31.4, "product": "N(C(=N)N)C(=O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
22
CELSIUS
2
HOUR
0.9 g (9.42 mmol) of guanidine hydrochloride is added to a solution of 0.51 g (9.44 mmol) of sodium methoxide in 15 mL of methanol at a temperature in the region of 22° C. under an argon atmosphere. After stirring at a temperature in the region of 22° C. for 2 hours, the solvent is evaporated off under reduced pressure...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
O1CCCC1.ClCCl.CO
22
2
N=C(N)N.O=C(Cl)c1ccn(-c2cccc3ncccc23)c1>O1CCCC1.ClCCl.CO>N=C(N)NC(=O)c1ccn(-c2cccc3ncccc23)c1