dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9c1ae5b007ce40f89648f68658dddefe
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cccc3ncccc23)c1>>Cl.O=C(Cl)c1ccn(-c2cccc3ncccc23)c1
C(C(=O)Cl)(=O)Cl.C(=O)(O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1>>Cl.ClC(=O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1
O=C(C(=O)[Cl:4])[Cl:1].O[C:3](=[O:2])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][cH:11][cH:12][c:13]3[n:14][cH:15][cH:16][cH:17][c:18]23)[cH:19]1>>[ClH:1].[O:2]=[C:3]([Cl:4])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][cH:11][cH:12][c:13]3[n:14][cH:15][cH:16][cH:17][c:18]23)[cH:19]1
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cccc3ncccc23)c1
Cl.O=C(Cl)c1ccn(-c2cccc3ncccc23)c1
null
null
ClCCl
Functional Group Interconversion
Alcohol to chloride_Other
013cec2edeb273a7a148f349d36a52d99ff4e7bcf8eed78085df830088e387ac
aedb1f68dc5b7eb0583043e1125b741382b17974140a2f46554f0110e2ddc884
c1cc(-n2cccc2)c2cccnc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.O=C(-[Cl;H0;D1;+0:9])-C(=O)-[Cl;H0;D1;+0:10]>>[Cl;H0;D1;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.[ClH;D0;+0:9]
106.6
[{"value": 106.6, "product": "Cl.ClC(=O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
22
CELSIUS
15
HOUR
0.5 mL (5.73 mmol) of oxalyl chloride is added to a solution, cooled to a temperature in the region of 5° C., of 0.42 g (1.76 mmol) of 3-carboxy-1-(quinol-5-yl)-1H-pyrrole in 10 mL of dichloromethane under an argon atmosphere. After stirring at a temperature in the region of 22° C. for 15 hours, concentrating the react...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
Other
ClCCl
22
15
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cccc3ncccc23)c1>ClCCl>Cl.O=C(Cl)c1ccn(-c2cccc3ncccc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-07442da8730b42eca62689c2a93e2166
COC(=O)c1ccn(-c2cccc3ncccc23)c1>>O=C(O)c1ccn(-c2cccc3ncccc23)c1
O.[OH-].[Li+].O.COC(=O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1>>C(=O)(O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][n:7](-[c:8]2[cH:9][cH:10][cH:11][c:12]3[n:13][cH:14][cH:15][cH:16][c:17]23)[cH:18]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][n:7](-[c:8]2[cH:9][cH:10][cH:11][c:12]3[n:13][cH:14][cH:15][cH:16][c:17]23)[cH:18]1
COC(=O)c1ccn(-c2cccc3ncccc23)c1
O=C(O)c1ccn(-c2cccc3ncccc23)c1
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1cc(-n2cccc2)c2cccnc2c1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
89
[{"value": 89.0, "product": "C(=O)(O)C1=CN(C=C1)C1=C2C=CC=NC2=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
HOUR
0.36 g (8.58 mmol) of lithium hydroxide monohydrate and 20 mL of water are added to a solution at a temperature in the region of 22° C. of 0.5 g (1.98 mmol) of 3-methoxycarbonyl-1-(quinol-5-yl)-1H-pyrrole in 20 mL of tetrahydrofuran. After stirring at the reflux point of the solvent for 15 hours, the reaction mixture i...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
Other
O1CCCC1
null
15
COC(=O)c1ccn(-c2cccc3ncccc23)c1>O1CCCC1>O=C(O)c1ccn(-c2cccc3ncccc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-53e910dc6ecf4007b8f1e9f0503f1f12
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cccc3cccnc23)c1>>O=C(Cl)c1ccn(-c2cccc3cccnc23)c1
C(C(=O)Cl)(=O)Cl.C(C(=O)Cl)(=O)Cl.Cl.C(=O)(O)C1=CN(C=C1)C=1C=CC=C2C=CC=NC12>>Cl.ClC(=O)C1=CN(C=C1)C=1C=CC=C2C=CC=NC12
O=C(Cl)C(=O)[Cl:4].O[C:3](=[O:2])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][n:17][c:18]23)[cH:19]1>>[O:2]=[C:3]([Cl:4])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][n:17][c:18]23)[cH:19]1
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cccc3cccnc23)c1
O=C(Cl)c1ccn(-c2cccc3cccnc23)c1
null
null
ClCCl
Functional Group Interconversion
Alcohol to chloride_Other
013cec2edeb273a7a148f349d36a52d99ff4e7bcf8eed78085df830088e387ac
aedb1f68dc5b7eb0583043e1125b741382b17974140a2f46554f0110e2ddc884
c1cnc2c(-n3cccc3)cccc2c1
Cl-C(=O)-C(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[#7;a:6](-[c:7]:[c:8]:[#7;a:9]):[c:10]:[c:11]:1>>[#7;a:9]:[c:8]:[c:7]-[#7;a:6]1:[c:5]:[c:4](-[C;H0;D3;+0:2](-[Cl;H0;D1;+0:1])=[O;D1;H0:3]):[c:11]:[c:10]:1
86.9
[{"value": 86.9, "product": "Cl.ClC(=O)C1=CN(C=C1)C=1C=CC=C2C=CC=NC12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
22
CELSIUS
15
HOUR
0.45 mL (5.16 mmol) of oxalyl chloride is added to a solution, cooled to a temperature in the region of 5° C., of 0.45 g (1.64 mmol) of 3-carboxy-1-(quinol-8-yl)-1H-pyrrole hydrochloride in 20 mL of dichloromethane under an argon atmosphere. After stirring at a temperature in the region of 22° C. for 15 hours, the reac...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
ClCCl
22
15
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cccc3cccnc23)c1>ClCCl>O=C(Cl)c1ccn(-c2cccc3cccnc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5dc2a4c4c44e428ca878141a5f4b4e65
Brc1cccc2cccnc12.COC(=O)c1cc[nH]c1>>COC(=O)c1ccn(-c2cccc3cccnc23)c1
CCCCCCCCCCCC.BrC=1C=CC=C2C=CC=NC12.[C@@H]1([C@@H](CCCC1)N)N.COC(=O)C1=CNC=C1.P(=O)([O-])([O-])[O-].[K+].[K+].[K+]>>COC(=O)C1=CN(C=C1)C=1C=CC=C2C=CC=NC12
Br[c:9]1[cH:10][cH:11][cH:12][c:13]2[cH:14][cH:15][cH:16][n:17][c:18]12.[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][nH:8][cH:19]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][n:17][c:18]23)[cH:19]1
Brc1cccc2cccnc12.COC(=O)c1cc[nH]c1
COC(=O)c1ccn(-c2cccc3cccnc23)c1
null
[Cu](I)I
O1CCOCC1
Heteroatom Alkylation and Arylation
OtherReaction
0f41158080bd72518d9a6b2389c4c528ac037a6b5eac12dbe2506d72e4b3d2c9
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1cnc2c(-n3cccc3)cccc2c1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7].[#8:8]-[C:9](=[O;D1;H0:10])-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14]:[c:15]:1>>[#8:8]-[C:9](=[O;D1;H0:10])-[c:11]1:[c:12]:[n;H0;D3;+0:13](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]):[c:14]:[c:15]:1
124.1
[{"value": 124.1, "product": "COC(=O)C1=CN(C=C1)C=1C=CC=C2C=CC=NC12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
15
HOUR
20 mL of 1,4-dioxane, 0.32 mL of n-dodecane, 1.5 g (7.21 mmol) of 8-bromoquinoline and 0.77 mL (6.41 mmol) of trans-1,2-cyclohexanediamine are added at a temperature in the region of 22° C. under an argon atmosphere to 0.8 g (6.39 mmol) of 3-methoxycarbonyl-1H-pyrrole, 3 g (14.13 mmol) of potassium orthophosphate and 0...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccc2ncccc2c1.c1cc[nH]c1
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
HBr
[Cu](I)I.O1CCOCC1
100
15
Brc1cccc2cccnc12.COC(=O)c1cc[nH]c1>[Cu](I)I.O1CCOCC1>COC(=O)c1ccn(-c2cccc3cccnc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-711fc6486af344878cb5aa33070595c0
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cncc3ccccc23)c1>>Cl.O=C(Cl)c1ccn(-c2cncc3ccccc23)c1
C(C(=O)Cl)(=O)Cl.C(=O)(O)C1=CN(C=C1)C1=CN=CC2=CC=CC=C12>>Cl.ClC(=O)C1=CN(C=C1)C1=CN=CC2=CC=CC=C12
O=C(C(=O)[Cl:4])[Cl:1].O[C:3](=[O:2])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][n:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19]1>>[ClH:1].[O:2]=[C:3]([Cl:4])[c:5]1[cH:6][cH:7][n:8](-[c:9]2[cH:10][n:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19]1
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cncc3ccccc23)c1
Cl.O=C(Cl)c1ccn(-c2cncc3ccccc23)c1
null
null
ClCCl
Functional Group Interconversion
Alcohol to chloride_Other
013cec2edeb273a7a148f349d36a52d99ff4e7bcf8eed78085df830088e387ac
aedb1f68dc5b7eb0583043e1125b741382b17974140a2f46554f0110e2ddc884
c1ccc2c(-n3cccc3)cncc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]:[c:7]:[#7;a:8]):[c:9]:[c:10]:1.O=C(-[Cl;H0;D1;+0:11])-C(=O)-[Cl;H0;D1;+0:12]>>[#7;a:8]:[c:7]:[c:6]-[#7;a:5]1:[c:4]:[c:3](-[C;H0;D3;+0:1](-[Cl;H0;D1;+0:12])=[O;D1;H0:2]):[c:10]:[c:9]:1.[ClH;D0;+0:11]
null
[]
22
CELSIUS
15
HOUR
0.82 mL (9.4 mmol) of oxalyl chloride is added to a solution, cooled to a temperature in the region of 5° C., of 0.75 g (3.15 mmol) of 3-carboxy-1-(isoquinol-4-yl)-1H-pyrrole in 25 mL of dichloromethane under an argon atmosphere. After stirring at a temperature in the region of 22° C. for 15 hours, the reaction mixture...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2cnccc2c1
Other
ClCCl
22
15
O=C(Cl)C(=O)Cl.O=C(O)c1ccn(-c2cncc3ccccc23)c1>ClCCl>Cl.O=C(Cl)c1ccn(-c2cncc3ccccc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a71ed9b08627498493d90473bab0af9f
COC(=O)c1ccn(-c2cncc3ccccc23)c1>>O=C(O)c1ccn(-c2cncc3ccccc23)c1
[K+].[Br-].O.[OH-].[Li+].O.COC(=O)C1=CN(C=C1)C1=CN=CC2=CC=CC=C12>>C(=O)(O)C1=CN(C=C1)C1=CN=CC2=CC=CC=C12
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][n:7](-[c:8]2[cH:9][n:10][cH:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[cH:18]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][n:7](-[c:8]2[cH:9][n:10][cH:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[cH:18]1
COC(=O)c1ccn(-c2cncc3ccccc23)c1
O=C(O)c1ccn(-c2cncc3ccccc23)c1
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(-n3cccc3)cncc2c1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
15
HOUR
0.63 g (15.02 mmol) of lithium hydroxide monohydrate and 20 mL of water are added to a solution, at a temperature in the region of 22° C., of 0.95 g (376 mmol) of 3-methoxycarbonyl-1-(isoquinol-4-yl)-1H-pyrrole in 20 mL of tetrahydrofuran. After stirring at the reflux point of the solvent for 15 hours, the reaction mix...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cc[nH]c1.c1ccc2cnccc2c1
Other
O1CCCC1
null
15
COC(=O)c1ccn(-c2cncc3ccccc23)c1>O1CCCC1>O=C(O)c1ccn(-c2cncc3ccccc23)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1b5c08f7787d4c9ba741d3bb98e20248
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)Cl.N=C(N)N>>Cc1cn(-c2ccnc3ccccc23)cc1C(=O)NC(=N)N
ClC(=O)C1=CN(C=C1C)C1=CC=NC2=CC=CC=C12.C[O-].[Na+].CO.Cl.NC(=N)N>>N(C(=N)N)C(=O)C1=CN(C=C1C)C1=CC=NC2=CC=CC=C12
Cl[C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[cH:6][cH:7][n:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18].[NH2:19][C:20](=[NH:21])[NH2:22]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[cH:6][cH:7][n:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[NH:19][C:20](=[NH:21])[NH2:22]
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)Cl.N=C(N)N
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)NC(=N)N
null
null
COCCOC.C(Cl)(Cl)Cl
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccc2c(-n3cccc3)ccnc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH2;D1;+0:12]>>[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1
55
[{"value": 55.0, "product": "N(C(=N)N)C(=O)C1=CN(C=C1C)C1=CC=NC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
1
HOUR
1.4 g (25.5 mmol) of sodium methoxide is added at a temperature in the region of 20° C. under an argon atmosphere to 25 mL of methanol. After complete dissolution, 2.5 g (26.2 mmol) of guanidine hydrochloride are added. After stirring at a temperature in the region of 20° C. for 1 hour, the reaction mixture is concentr...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
COCCOC.C(Cl)(Cl)Cl
20
1
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)Cl.N=C(N)N>COCCOC.C(Cl)(Cl)Cl>Cc1cn(-c2ccnc3ccccc23)cc1C(=O)NC(=N)N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e3853d69d4f54b368c8fa00945753e65
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)O.O=S(Cl)Cl>>Cc1cn(-c2ccnc3ccccc23)cc1C(=O)Cl
S(=O)(Cl)Cl.C(=O)(O)C1=CN(C=C1C)C1=CC=NC2=CC=CC=C12>>ClC(=O)C1=CN(C=C1C)C1=CC=NC2=CC=CC=C12
O[C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[cH:6][cH:7][n:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18].O=S(Cl)[Cl:19]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[cH:6][cH:7][n:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[Cl:19]
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)O.O=S(Cl)Cl
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)Cl
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1ccc2c(-n3cccc3)ccnc2c1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[#7;a:6](-[c:7]):[c:8]:[c:9]:1>>[Cl;H0;D1;+0:1]-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[#7;a:6](-[c:7]):[c:8]:[c:9]:1
100
[{"value": 100.0, "product": "ClC(=O)C1=CN(C=C1C)C1=CC=NC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
10 mL (137 mmol) of sulphinyl chloride are added at a temperature in the region of 20° C. under an argon atmosphere to 1 g (3.97 mmol) of 3-carboxy-4-methyl-1-(quinol-4-yl)-1H-pyrrole dissolved in 20 mL of chloroform. After stirring at the reflux point of the solvent for 1 hour, the reaction mixture is concentrated to ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
C(Cl)(Cl)Cl
null
1
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)O.O=S(Cl)Cl>C(Cl)(Cl)Cl>Cc1cn(-c2ccnc3ccccc23)cc1C(=O)Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f2bee4fff69a42e4b9e7a6127aaa4781
COC(=O)c1cn(-c2ccnc3ccccc23)cc1C>>Cc1cn(-c2ccnc3ccccc23)cc1C(=O)O
O.[OH-].[Li+].COC(=O)C1=CN(C=C1C)C1=CC=NC2=CC=CC=C12>>C(=O)(O)C1=CN(C=C1C)C1=CC=NC2=CC=CC=C12
C[O:19][C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[cH:6][cH:7][n:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[cH:6][cH:7][n:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[OH:19]
COC(=O)c1cn(-c2ccnc3ccccc23)cc1C
Cc1cn(-c2ccnc3ccccc23)cc1C(=O)O
null
null
O1CCCC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(-n3cccc3)ccnc2c1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
null
null
0.63 g (15 mmol) of lithium hydroxide monohydrate is added at a temperature in the region of 20° C. to 1.21 g (4.54 mmol) of 3-methoxycarbonyl-4-methyl-1-(quinol-4-yl)-1H-pyrrole dissolved in 50 mL of tetrahydrofuran and 50 mL of water. After stirring at reflux for 22 hours, the reaction mixture is concentrated to dryn...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
Other
O1CCCC1.O
null
null
COC(=O)c1cn(-c2ccnc3ccccc23)cc1C>O1CCCC1.O>Cc1cn(-c2ccnc3ccccc23)cc1C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ec81f6d9662f4a75babd0b2c6e4714da
Cc1cn(-c2nccc3ccccc23)cc1C(=O)Cl.N=C(N)N>>Cc1cn(-c2nccc3ccccc23)cc1C(=O)NC(=N)N
ClC(=O)C1=CN(C=C1C)C1=NC=CC2=CC=CC=C12.Cl.NC(=N)N.C[O-].[Na+]>>Cl.N(C(=N)N)C(=O)C1=CN(C=C1C)C1=NC=CC2=CC=CC=C12
Cl[C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[n:6][cH:7][cH:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18].[NH2:19][C:20](=[NH:21])[NH2:22]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[n:6][cH:7][cH:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[NH:19][C:20](=[NH:21])[NH2:22]
Cc1cn(-c2nccc3ccccc23)cc1C(=O)Cl.N=C(N)N
Cc1cn(-c2nccc3ccccc23)cc1C(=O)NC(=N)N
null
null
COCCOC.C(Cl)(Cl)Cl.CO
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccc2c(-n3cccc3)nccc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]:[#7;a:7]):[c:8]:[c:9]:1.[N;D1;H1:10]=[C:11](-[N;D1;H2:12])-[NH2;D1;+0:13]>>[#7;a:7]:[c:6]-[#7;a:5]1:[c:4]:[c:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:13]-[C:11](=[N;D1;H1:10])-[N;D1;H2:12]):[c:9]:[c:8]:1
43.1
[{"value": 43.1, "product": "Cl.N(C(=N)N)C(=O)C1=CN(C=C1C)C1=NC=CC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
1
HOUR
1.37 g (25.37 mmol) of sodium methoxide are added at a temperature in the region of 20° C. under an argon atmosphere to 25 mL of methanol. After complete dissolution, 2.5 g (26.2 mmol) of guanidine hydrochloride are added. After stirring at a temperature in the region of 20° C. for 1 hour, the reaction mixture is conce...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1cc[nH]c1.c1ccc2cnccc2c1
HCl
COCCOC.C(Cl)(Cl)Cl.CO
20
1
Cc1cn(-c2nccc3ccccc23)cc1C(=O)Cl.N=C(N)N>COCCOC.C(Cl)(Cl)Cl.CO>Cc1cn(-c2nccc3ccccc23)cc1C(=O)NC(=N)N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5a042881dff64ef283d4dabdea62cd6d
Cc1cn(-c2nccc3ccccc23)cc1C(=O)O.O=S(Cl)Cl>>Cc1cn(-c2nccc3ccccc23)cc1C(=O)Cl
S(=O)(Cl)Cl.C(=O)(O)C1=CN(C=C1C)C1=NC=CC2=CC=CC=C12>>ClC(=O)C1=CN(C=C1C)C1=NC=CC2=CC=CC=C12
O[C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[n:6][cH:7][cH:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18].O=S(Cl)[Cl:19]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[n:6][cH:7][cH:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[Cl:19]
Cc1cn(-c2nccc3ccccc23)cc1C(=O)O.O=S(Cl)Cl
Cc1cn(-c2nccc3ccccc23)cc1C(=O)Cl
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1ccc2c(-n3cccc3)nccc2c1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[#7;a:6](-[c:7]:[#7;a:8]):[c:9]:[c:10]:1>>[#7;a:8]:[c:7]-[#7;a:6]1:[c:5]:[c:4](-[C;H0;D3;+0:2](-[Cl;H0;D1;+0:1])=[O;D1;H0:3]):[c:10]:[c:9]:1
100
[{"value": 100.0, "product": "ClC(=O)C1=CN(C=C1C)C1=NC=CC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
10 mL (137 mmol) of sulphinyl chloride are added at a temperature in the region of 20° C. under an argon atmosphere to 1.1 g (4.36 mmol) of 3-carboxy-1-(isoquinol-1-yl)-4-methyl-1H-pyrrole dissolved in 20 mL of chloroform. After stirring at the reflux point of the solvent for 2 hours, the reaction mixture is concentrat...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2cnccc2c1
HCl
C(Cl)(Cl)Cl
null
2
Cc1cn(-c2nccc3ccccc23)cc1C(=O)O.O=S(Cl)Cl>C(Cl)(Cl)Cl>Cc1cn(-c2nccc3ccccc23)cc1C(=O)Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4171eb3662dd4db3925a61d44be6d640
COC(=O)c1cn(-c2nccc3ccccc23)cc1C>>Cc1cn(-c2nccc3ccccc23)cc1C(=O)O
O.[OH-].[Li+].C1(=NC=CC2=CC=CC=C12)N1C=C(C(=C1)C)C(=O)OC>>C(=O)(O)C1=CN(C=C1C)C1=NC=CC2=CC=CC=C12
C[O:19][C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[n:6][cH:7][cH:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[n:6][cH:7][cH:8][c:9]3[cH:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[OH:19]
COC(=O)c1cn(-c2nccc3ccccc23)cc1C
Cc1cn(-c2nccc3ccccc23)cc1C(=O)O
null
null
O1CCCC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(-n3cccc3)nccc2c1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
null
null
0.63 g (15 mmol) of lithium hydroxide monohydrate is added at a temperature in the region of 20° C. to 1.35 g (5 mmol) of 1-(isoquinol-1-yl)-3-methoxycarbonyl-4-methyl-1H-pyrrole dissolved in 50 mL of tetrahydrofuran and 50 mL of water. After stirring at reflux for 25 hours, the reaction mixture is concentrated to dryn...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cc[nH]c1.c1ccc2cnccc2c1
Other
O1CCCC1.O
null
null
COC(=O)c1cn(-c2nccc3ccccc23)cc1C>O1CCCC1.O>Cc1cn(-c2nccc3ccccc23)cc1C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0a24db0bb7c94ee295f37e6984effbc5
COC(=O)c1c[nH]cc1C.Clc1nccc2ccccc12>>COC(=O)c1cn(-c2nccc3ccccc23)cc1C
ClC1=NC=CC2=CC=CC=C12.[H-].[Na+].COC(=O)C1=CNC=C1C.O>>C1(=NC=CC2=CC=CC=C12)N1C=C(C(=C1)C)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][cH:18][c:19]1[CH3:20].Cl[c:8]1[n:9][cH:10][cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]12>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][n:7](-[c:8]2[n:9][cH:10][cH:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[cH:18][c:19]1[CH3:20]
COC(=O)c1c[nH]cc1C.Clc1nccc2ccccc12
COC(=O)c1cn(-c2nccc3ccccc23)cc1C
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
64941681a78379ce7a568f1d8a1309e87b488f1d656284455a26054be1853b83
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3cccc3)nccc2c1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](:[c:5]):[c:6].[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[c:12]:[nH;D2;+0:13]:[c:14]:1>>[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[c:12]:[n;H0;D3;+0:13](-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](:[c:5]):[c:6]):[c:14]:1
null
[]
40
CELSIUS
0.3
HOUR
0.208 g (6.5 mmol) of sodium hydride, at 75% by weight in liquid petroleum jelly, is added at a temperature in the region of 20° C. under an argon atmosphere to a solution of 0.903 g (6.5 mmol) of 3-methoxycarbonyl-4-methyl-1H-pyrrole in 20 mL of dimethylformamide. After stirring at a temperature in the region of 40° C...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2cnccc2c1
c1cc[nH]c1.c1ccc2cnccc2c1
c1cc[nH]c1.c1ccc2cnccc2c1
HCl
CN(C=O)C
40
0.3
COC(=O)c1c[nH]cc1C.Clc1nccc2ccccc12>CN(C=O)C>COC(=O)c1cn(-c2nccc3ccccc23)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d0bdaf28d9484854bfe56b4706d69540
Cc1c(C(=O)Cl)cn(-c2ccnc3ccccc23)c1C.Cl.N=C(N)N>>Cc1c(C(=O)NC(=N)N)cn(-c2ccnc3ccccc23)c1C.Cl
Cl.Cl.NC(=N)N.ClC(=O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12.C[O-].[Na+]>>Cl.Cl.N(C(=N)N)C(=O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12
Cl[C:4]([c:3]1[c:2]([CH3:1])[c:22]([CH3:23])[n:11](-[c:12]2[cH:13][cH:14][n:15][c:16]3[cH:17][cH:18][cH:19][cH:20][c:21]23)[cH:10]1)=[O:5].[ClH:25].[NH2:6][C:7](=[NH:8])[NH2:9]>>[CH3:1][c:2]1[c:3]([C:4](=[O:5])[NH:6][C:7](=[NH:8])[NH2:9])[cH:10][n:11](-[c:12]2[cH:13][cH:14][n:15][c:16]3[cH:17][cH:18][cH:19][cH:20][c:21...
Cc1c(C(=O)Cl)cn(-c2ccnc3ccccc23)c1C.Cl.N=C(N)N
Cc1c(C(=O)NC(=N)N)cn(-c2ccnc3ccccc23)c1C.Cl
null
null
O1CCOCC1.C(Cl)(Cl)Cl.CO.COCCOC.C(C)O
Acylation
OtherReaction
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccc2c(-n3cccc3)ccnc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH2;D1;+0:12]>>[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1
61.6
[{"value": 61.6, "product": "Cl.Cl.N(C(=N)N)C(=O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
0.5
HOUR
1.78 g (33 mmol) of sodium methoxide are added at a temperature in the region of 20° C. under an argon atmosphere to 20 mL of methanol. After complete dissolution, 3.34 g (35 mmol) of guanidine hydrochloride are added. After stirring at a temperature in the region of 20° C. for 0.5 hour, the reaction mixture is concent...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
O1CCOCC1.C(Cl)(Cl)Cl.CO.COCCOC.C(C)O
20
0.5
Cc1c(C(=O)Cl)cn(-c2ccnc3ccccc23)c1C.Cl.N=C(N)N>O1CCOCC1.C(Cl)(Cl)Cl.CO.COCCOC.C(C)O>Cc1c(C(=O)NC(=N)N)cn(-c2ccnc3ccccc23)c1C.Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7e005a6ec3d348a894d4a05f8676e56e
Cc1c(C(=O)O)cn(-c2ccnc3ccccc23)c1C.O=S(Cl)Cl>>Cc1c(C(=O)Cl)cn(-c2ccnc3ccccc23)c1C
S(=O)(Cl)Cl.C(=O)(O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12>>ClC(=O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12
O[C:4]([c:3]1[c:2]([CH3:1])[c:19]([CH3:20])[n:8](-[c:9]2[cH:10][cH:11][n:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:7]1)=[O:5].O=S(Cl)[Cl:6]>>[CH3:1][c:2]1[c:3]([C:4](=[O:5])[Cl:6])[cH:7][n:8](-[c:9]2[cH:10][cH:11][n:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[c:19]1[CH3:20]
Cc1c(C(=O)O)cn(-c2ccnc3ccccc23)c1C.O=S(Cl)Cl
Cc1c(C(=O)Cl)cn(-c2ccnc3ccccc23)c1C
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1ccc2c(-n3cccc3)ccnc2c1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[c:6]:[#7;a:7](-[c:8]):[c:9]:1>>[Cl;H0;D1;+0:1]-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[c:6]:[#7;a:7](-[c:8]):[c:9]:1
100
[{"value": 100.0, "product": "ClC(=O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
10 mL (137 mmol) of sulphinyl chloride are added at a temperature in the region of 20° C. under an argon atmosphere to 1.1 g (4.1 mmol) of 3-carboxy-4,5-dimethyl-1-(quinol-4-yl)-1H-pyrrole dissolved in 20 mL of chloroform. After stirring at the reflux point of the solvent for 1.5 hours, the reaction mixture is concentr...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
C(Cl)(Cl)Cl
null
1.5
Cc1c(C(=O)O)cn(-c2ccnc3ccccc23)c1C.O=S(Cl)Cl>C(Cl)(Cl)Cl>Cc1c(C(=O)Cl)cn(-c2ccnc3ccccc23)c1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2a5c448614724de781c0c90100dd80fc
CCOC(=O)c1cn(-c2ccnc3ccccc23)c(C)c1C>>Cc1c(C(=O)O)cn(-c2ccnc3ccccc23)c1C
O.[OH-].[Li+].C(C)OC(=O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12>>C(=O)(O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12
CC[O:6][C:4]([c:3]1[c:2]([CH3:1])[c:19]([CH3:20])[n:8](-[c:9]2[cH:10][cH:11][n:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:7]1)=[O:5]>>[CH3:1][c:2]1[c:3]([C:4](=[O:5])[OH:6])[cH:7][n:8](-[c:9]2[cH:10][cH:11][n:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[c:19]1[CH3:20]
CCOC(=O)c1cn(-c2ccnc3ccccc23)c(C)c1C
Cc1c(C(=O)O)cn(-c2ccnc3ccccc23)c1C
null
null
Cl.O.O1CCCC1
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(-n3cccc3)ccnc2c1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
null
null
1.89 g (45 mmol) of lithium hydroxide monohydrate are added at a temperature in the region of 20° C. to 1.3 g (4.42 mmol) of 3-ethoxycarbonyl-4,5-dimethyl-1-(quinol-4-yl)-1H-pyrrole dissolved in 50 mL of tetrahydrofuran and 50 mL of water. After stirring at reflux for 42 hours, the reaction mixture is concentrated virt...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
Other
Cl.O.O1CCCC1
null
null
CCOC(=O)c1cn(-c2ccnc3ccccc23)c(C)c1C>Cl.O.O1CCCC1>Cc1c(C(=O)O)cn(-c2ccnc3ccccc23)c1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e151ce452e1241aabb17de853cb0412b
CCOC(=O)c1c[nH]c(C)c1C.Clc1ccnc2ccccc12>>CCOC(=O)c1cn(-c2ccnc3ccccc23)c(C)c1C
ClC1=CC=NC2=CC=CC=C12.[H-].[Na+].C(C)OC(=O)C1=CNC(=C1C)C.O>>C(C)OC(=O)C1=CN(C(=C1C)C)C1=CC=NC2=CC=CC=C12
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][nH:8][c:19]([CH3:20])[c:21]1[CH3:22].Cl[c:9]1[cH:10][cH:11][n:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][n:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[c:19]([CH3:20])[c:21]1[CH3:22]
CCOC(=O)c1c[nH]c(C)c1C.Clc1ccnc2ccccc12
CCOC(=O)c1cn(-c2ccnc3ccccc23)c(C)c1C
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
0f41158080bd72518d9a6b2389c4c528ac037a6b5eac12dbe2506d72e4b3d2c9
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3cccc3)ccnc2c1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14](-[C;D1;H3:15]):[nH;D2;+0:16]:[c:17]:1>>[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14](-[C;D1;H3:15]):[n;H0;D3;+0:16](-[c;H0;D3;+0:1]2:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:2:[c:8]):[c:17]:1
null
[]
40
CELSIUS
0.3
HOUR
0.285 g (8.9 mmol) of sodium hydride, at 75% by weight in liquid petroleum jelly, is added at a temperature in the region of 20° C. under an argon atmosphere to a solution of 1.35 g (8.1 mmol) of 3-ethoxycarbonyl-4,5-dimethyl-1H-pyrrole in 8 mL of dimethylformamide. After stirring at a temperature in the region of 40° ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
CN(C=O)C
40
0.3
CCOC(=O)c1c[nH]c(C)c1C.Clc1ccnc2ccccc12>CN(C=O)C>CCOC(=O)c1cn(-c2ccnc3ccccc23)c(C)c1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-488f452e1c6146b4a870ed73f4b787fe
N=C(N)N.O=C(Cl)c1cn(-c2ccnc3ccccc23)cc1C1CC1>>N=C(N)NC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
ClC(=O)C1=CN(C=C1C1CC1)C1=CC=NC2=CC=CC=C12.Cl.NC(=N)N.C[O-].[Na+]>>C1(CC1)C=1C(=CN(C1)C1=CC=NC2=CC=CC=C12)C(=O)NC(=N)N
[NH:1]=[C:2]([NH2:3])[NH2:4].Cl[C:5](=[O:6])[c:7]1[cH:8][n:9](-[c:10]2[cH:11][cH:12][n:13][c:14]3[cH:15][cH:16][cH:17][cH:18][c:19]23)[cH:20][c:21]1[CH:22]1[CH2:23][CH2:24]1>>[NH:1]=[C:2]([NH2:3])[NH:4][C:5](=[O:6])[c:7]1[cH:8][n:9](-[c:10]2[cH:11][cH:12][n:13][c:14]3[cH:15][cH:16][cH:17][cH:18][c:19]23)[cH:20][c:21]1[...
N=C(N)N.O=C(Cl)c1cn(-c2ccnc3ccccc23)cc1C1CC1
N=C(N)NC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
null
null
COCCOC.C(Cl)(Cl)Cl.CO
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccc2c(-n3ccc(C4CC4)c3)ccnc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[c:7]):[c:8]:1.[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH2;D1;+0:12]>>[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[c:7]):[c:8]:1
63.8
[{"value": 63.8, "product": "C1(CC1)C=1C(=CN(C1)C1=CC=NC2=CC=CC=C12)C(=O)NC(=N)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
0.5
HOUR
1.19 g (22 mmol) of sodium methoxide are added to 25 mL of methanol at a temperature in the region of 20° C. under an argon atmosphere. After total dissolution, 2.2 g (23 mmol) of guanidine hydrochloride are added. After stirring at a temperature in the region of 20° C. for 0.5 hour, the reaction mixture is concentrate...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1.C1CC1
HCl
COCCOC.C(Cl)(Cl)Cl.CO
20
0.5
N=C(N)N.O=C(Cl)c1cn(-c2ccnc3ccccc23)cc1C1CC1>COCCOC.C(Cl)(Cl)Cl.CO>N=C(N)NC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-705b602f839943f78bb12ba9d6253c13
O=C(O)c1cn(-c2ccnc3ccccc23)cc1C1CC1.O=S(Cl)Cl>>O=C(Cl)c1cn(-c2ccnc3ccccc23)cc1C1CC1
S(=O)(Cl)Cl.C(=O)(O)C1=CN(C=C1C1CC1)C1=CC=NC2=CC=CC=C12>>ClC(=O)C1=CN(C=C1C1CC1)C1=CC=NC2=CC=CC=C12
O[C:2](=[O:1])[c:4]1[cH:5][n:6](-[c:7]2[cH:8][cH:9][n:10][c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]23)[cH:17][c:18]1[CH:19]1[CH2:20][CH2:21]1.O=S(Cl)[Cl:3]>>[O:1]=[C:2]([Cl:3])[c:4]1[cH:5][n:6](-[c:7]2[cH:8][cH:9][n:10][c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]23)[cH:17][c:18]1[CH:19]1[CH2:20][CH2:21]1
O=C(O)c1cn(-c2ccnc3ccccc23)cc1C1CC1.O=S(Cl)Cl
O=C(Cl)c1cn(-c2ccnc3ccccc23)cc1C1CC1
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1ccc2c(-n3ccc(C4CC4)c3)ccnc2c1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[c:6]:[#7;a:7](-[c:8]):[c:9]:1>>[Cl;H0;D1;+0:1]-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5]:[c:6]:[#7;a:7](-[c:8]):[c:9]:1
100
[{"value": 100.0, "product": "ClC(=O)C1=CN(C=C1C1CC1)C1=CC=NC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
10 mL (137 mmol) of sulphinyl chloride are added to 1.05 g (3.78 mmol) of 3-carboxy-4-cyclopropyl-1-(quinolin-4-yl)-1H-pyrrole dissolved in 20 mL of chloroform at a temperature in the region of 20° C. under an argon atmosphere. After stirring for one hour at the reflux temperature of the solvent, the reaction mixture i...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1.C1CC1
HCl
C(Cl)(Cl)Cl
null
1
O=C(O)c1cn(-c2ccnc3ccccc23)cc1C1CC1.O=S(Cl)Cl>C(Cl)(Cl)Cl>O=C(Cl)c1cn(-c2ccnc3ccccc23)cc1C1CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-85bef526f5de461aa02d64133e4662c8
COC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1>>O=C(O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
O.[OH-].[Li+].C1(CC1)C=1C(=CN(C1)C1=CC=NC2=CC=CC=C12)C(=O)OC>>C(=O)(O)C1=CN(C=C1C1CC1)C1=CC=NC2=CC=CC=C12
C[O:3][C:2](=[O:1])[c:4]1[cH:5][n:6](-[c:7]2[cH:8][cH:9][n:10][c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]23)[cH:17][c:18]1[CH:19]1[CH2:20][CH2:21]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][n:6](-[c:7]2[cH:8][cH:9][n:10][c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]23)[cH:17][c:18]1[CH:19]1[CH2:20][CH2:21]1
COC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
O=C(O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
null
null
O1CCCC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(-n3ccc(C4CC4)c3)ccnc2c1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
26
HOUR
0.63 g (15 mmol) of lithium hydroxide monohydrate is added, at a temperature in the region of 20° C., to 1.3 g (4.4 mmol) of 4-cyclopropyl-3-methoxycarbonyl-1-(quinolin-4-yl)-1H-pyrrole dissolved in 50 mL of tetrahydrofuran and 50 mL of water. After stirring for 26 hours at the reflux temperature of the solvent, the re...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cc[nH]c1.c1ccc2ncccc2c1.C1CC1
Other
O1CCCC1.O
null
26
COC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1>O1CCCC1.O>O=C(O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0ef7b04f28b2421da6aa4ad91d5e166b
COC(=O)c1c[nH]cc1C1CC1.Clc1ccnc2ccccc12>>COC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
ClC1=CC=NC2=CC=CC=C12.[H-].[Na+].C1(CC1)C=1C(=CNC1)C(=O)OC>>C1(CC1)C=1C(=CN(C1)C1=CC=NC2=CC=CC=C12)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][cH:18][c:19]1[CH:20]1[CH2:21][CH2:22]1.Cl[c:8]1[cH:9][cH:10][n:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]12>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][n:7](-[c:8]2[cH:9][cH:10][n:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[cH:18][c:19]1[CH:20]1[CH2:21][CH2:22]1
COC(=O)c1c[nH]cc1C1CC1.Clc1ccnc2ccccc12
COC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
null
null
[Cl-].[Na+].O.CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
0f41158080bd72518d9a6b2389c4c528ac037a6b5eac12dbe2506d72e4b3d2c9
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3ccc(C4CC4)c3)ccnc2c1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14]:[nH;D2;+0:15]:[c:16]:1>>[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14]:[n;H0;D3;+0:15](-[c;H0;D3;+0:1]2:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:2:[c:8]):[c:16]:1
null
[]
40
CELSIUS
0.3
HOUR
0.208 g (6.5 mmol) of sodium hydride at 75% by weight in liquid petroleum jelly is added to a solution of 1.07 g (6.5 mmol) of 4-cyclopropyl-3-methoxycarbonyl-1H-pyrrole in 20 mL of dimethylformamide at a temperature in the region of 20° C. under an argon atmosphere. After the reaction mixture has been stirred at a tem...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1.C1CC1
HCl
[Cl-].[Na+].O.CN(C=O)C
40
0.3
COC(=O)c1c[nH]cc1C1CC1.Clc1ccnc2ccccc12>[Cl-].[Na+].O.CN(C=O)C>COC(=O)c1cn(-c2ccnc3ccccc23)cc1C1CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-af3ceb1fa390416d870629c341924f90
COC(=O)C=CC1CC1.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1>>COC(=O)c1c[nH]cc1C1CC1
C1(=CC=C(C=C1)S(=O)(=O)C[N+]#[C-])C.C1(CC1)C=CC(=O)OC.[H-].[Na+]>>C1(CC1)C=1C(=CNC1)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[CH:5]=[CH:9][CH:10]1[CH2:11][CH2:12]1.Cc1ccc(S(=O)(=O)[CH2:8][N+:7]#[C-:6])cc1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][cH:8][c:9]1[CH:10]1[CH2:11][CH2:12]1
COC(=O)C=CC1CC1.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1
COC(=O)c1c[nH]cc1C1CC1
null
null
CS(=O)C.[Cl-].[Na+].O.C(C)OCC
Functional Group Interconversion
OtherReaction
222aa38425ebd527cae949f4f6a41b16a79f5bedc3b38d407b2efba1132a0002
2b254751295ab0c58d4be59c7dc1148a5e0af4419b8080ba37410673480117ee
c1cc(C2CC2)c[nH]1
C-c1:c:c:c(-S(=O)(=O)-[CH2;D2;+0:1]-[N+;H0;D2:2]#[C-;H0;D1:3]):c:c:1.[C;D1;H3:4]-[#8:5]-[C:6](=[O;D1;H0:7])-[CH;D2;+0:8]=[CH;D2;+0:9]-[C:10]1-[C:11]-[C:12]-1>>[C;D1;H3:4]-[#8:5]-[C:6](=[O;D1;H0:7])-[c;H0;D3;+0:8]1:[cH;D2;+0:3]:[nH;D2;+0:2]:[cH;D2;+0:1]:[c;H0;D3;+0:9]:1-[C:10]1-[C:11]-[C:12]-1
86.1
[{"value": 86.1, "product": "C1(CC1)C=1C(=CNC1)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2.75
HOUR
A solution of 8.77 g of p-toluenesulphonylmethyl isocyanide and 5.67 g of methyl 3-cyclopropylacrylate in 72 mL of dimethyl sulphoxide and 145 mL of diethyl ether is added dropwise over 1.5 hours and under an argon atmosphere to a suspension of 1.73 g (54 mmol) of sodium hydride (at 75% by weight in liquid petroleum je...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Ester.Isocyanide
Ester
c1ccccc1
c1cc[nH]c1
c1cc[nH]c1.C1CC1
TsOH.HO-
CS(=O)C.[Cl-].[Na+].O.C(C)OCC
null
2.75
COC(=O)C=CC1CC1.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1>CS(=O)C.[Cl-].[Na+].O.C(C)OCC>COC(=O)c1c[nH]cc1C1CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7dbe4b69649d42f4930f731530a40827
Cc1cn(-c2cccc3ncccc23)cc1C(=O)Cl.N=C(N)N>>Cc1cn(-c2cccc3ncccc23)cc1C(=O)NC(=N)N
Cl.NC(=N)N.C[O-].[Na+].Cl.ClC(=O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1>>Cl.N(C(=N)N)C(=O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1
Cl[C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]3[n:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18].[NH2:19][C:20](=[NH:21])[NH2:22]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]3[n:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[NH:19][C:20](=[NH:21])[NH2:22]
Cc1cn(-c2cccc3ncccc23)cc1C(=O)Cl.N=C(N)N
Cc1cn(-c2cccc3ncccc23)cc1C(=O)NC(=N)N
null
null
CO
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1cc(-n2cccc2)c2cccnc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH2;D1;+0:12]>>[N;D1;H1:9]=[C:10](-[N;D1;H2:11])-[NH;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1
40.8
[{"value": 40.8, "product": "Cl.N(C(=N)N)C(=O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
1.06 g (11.18 mmol) of guanidine hydrochloride is added to a solution of 0.604 g (11.18 mmol) of sodium methoxide in 50 mL of methanol at a temperature in the region of 20° C. under an argon atmosphere. After stirring for 2 hours at this temperature, the mixture is concentrated to dryness under reduced pressure (2.7 kP...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
CO
null
2
Cc1cn(-c2cccc3ncccc23)cc1C(=O)Cl.N=C(N)N>CO>Cc1cn(-c2cccc3ncccc23)cc1C(=O)NC(=N)N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b00e031520ad46b79cebee264b8977d5
Cc1cn(-c2cccc3ncccc23)cc1C(=O)O.O=S(Cl)Cl>>Cc1cn(-c2cccc3ncccc23)cc1C(=O)Cl.Cl
S(=O)(Cl)Cl.C(=O)(O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1>>Cl.ClC(=O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1
O[C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]3[n:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18].O=S([Cl:19])[Cl:20]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]3[n:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[Cl:19].[ClH:20]
Cc1cn(-c2cccc3ncccc23)cc1C(=O)O.O=S(Cl)Cl
Cc1cn(-c2cccc3ncccc23)cc1C(=O)Cl.Cl
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1cc(-n2cccc2)c2cccnc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.O=S(-[Cl;H0;D1;+0:9])-[Cl;H0;D1;+0:10]>>[Cl;H0;D1;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.[ClH;D0;+0:10]
100
[{"value": 100.0, "product": "Cl.ClC(=O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
8 mL (110 mmol) of sulphinyl chloride are added to 0.47 g (1.86 mmol) of 3-carboxy-4-methyl-1-(quinolin-5-yl)-1H-pyrrole dissolved in 25 mL of chloroform at a temperature in the region of 20° C. under an argon atmosphere. After stirring for 1.5 hours at the reflux temperature of the solvent, the reaction mixture is con...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
Other
C(Cl)(Cl)Cl
null
1.5
Cc1cn(-c2cccc3ncccc23)cc1C(=O)O.O=S(Cl)Cl>C(Cl)(Cl)Cl>Cc1cn(-c2cccc3ncccc23)cc1C(=O)Cl.Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a2213ef54f2049318553c7dac6821260
COC(=O)c1cn(-c2cccc3ncccc23)cc1C>>Cc1cn(-c2cccc3ncccc23)cc1C(=O)O
O.[OH-].[Li+].COC(=O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1.O>>C(=O)(O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1
C[O:19][C:17]([c:16]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]3[n:10][cH:11][cH:12][cH:13][c:14]23)[cH:15]1)=[O:18]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]3[n:10][cH:11][cH:12][cH:13][c:14]23)[cH:15][c:16]1[C:17](=[O:18])[OH:19]
COC(=O)c1cn(-c2cccc3ncccc23)cc1C
Cc1cn(-c2cccc3ncccc23)cc1C(=O)O
null
null
O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1cc(-n2cccc2)c2cccnc2c1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
65.2
[{"value": 65.2, "product": "C(=O)(O)C1=CN(C=C1C)C1=C2C=CC=NC2=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
HOUR
0.504 g (12.2 mmol) of lithium hydroxide monohydrate is added to 0.8 g (3.04 mmol) of 3-methoxycarbonyl-4-methyl-1-(quinolin-5-yl)-1H-pyrrole dissolved in 25 mL of tetrahydrofuran and 25 mL of water at a temperature in the region of 20° C. After stirring for 30 hours at the reflux temperature of the solvent, the reacti...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cc[nH]c1.c1ccc2ncccc2c1
Other
O1CCCC1
null
30
COC(=O)c1cn(-c2cccc3ncccc23)cc1C>O1CCCC1>Cc1cn(-c2cccc3ncccc23)cc1C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3b5bd54644864a379c57521b24b68dd2
CCOC(=O)c1c[nH]cc1C(F)(F)F.Clc1ccnc2ccccc12>>CCOC(=O)c1cn(-c2ccnc3ccccc23)cc1C(F)(F)F
O.C([O-])([O-])=O.[K+].[K+].C(C)OC(=O)C1=CNC=C1C(F)(F)F.ClC1=CC=NC2=CC=CC=C12>>C(C)OC(=O)C1=CN(C=C1C(F)(F)F)C1=CC=NC2=CC=CC=C12
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][nH:8][cH:19][c:20]1[C:21]([F:22])([F:23])[F:24].Cl[c:9]1[cH:10][cH:11][n:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[cH:10][cH:11][n:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19][c:20]1[C:21]([F:22])([F:2...
CCOC(=O)c1c[nH]cc1C(F)(F)F.Clc1ccnc2ccccc12
CCOC(=O)c1cn(-c2ccnc3ccccc23)cc1C(F)(F)F
null
null
CS(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
0f41158080bd72518d9a6b2389c4c528ac037a6b5eac12dbe2506d72e4b3d2c9
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3cccc3)ccnc2c1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14]:[nH;D2;+0:15]:[c:16]:1>>[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14]:[n;H0;D3;+0:15](-[c;H0;D3;+0:1]2:[c:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:2:[c:8]):[c:16]:1
88.5
[{"value": 88.5, "product": "C(C)OC(=O)C1=CN(C=C1C(F)(F)F)C1=CC=NC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
110
CELSIUS
18
HOUR
1.73 g (12.5 mmol) of potassium carbonate are added to 1.036 g (5 mmol) of 3-ethoxycarbonyl-4-trifluoromethyl-1H-pyrrole and 0.82 g (5 mmol) of 4-chloroquinoline dissolved in 10 mL of dimethyl sulphoxide at a temperature in the region of 20° C. under an argon atmosphere. After stirring for 18 hours at a temperature in ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
CS(=O)C
110
18
CCOC(=O)c1c[nH]cc1C(F)(F)F.Clc1ccnc2ccccc12>CS(=O)C>CCOC(=O)c1cn(-c2ccnc3ccccc23)cc1C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dd8cf941d89e4753913048bb8c4aed3f
O=C(Cl)C(=O)Cl.O=C(O)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F>>Cl.O=C(Cl)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F
C(C(=O)Cl)(=O)Cl.C(=O)(O)C1=CN(C=C1C(F)(F)F)C1=NC=CC2=CC=CC=C12>>Cl.ClC(=O)C1=CN(C=C1C(F)(F)F)C1=NC=CC2=CC=CC=C12
O=C(C(=O)[Cl:4])[Cl:1].O[C:3](=[O:2])[c:5]1[cH:6][n:7](-[c:8]2[n:9][cH:10][cH:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[cH:18][c:19]1[C:20]([F:21])([F:22])[F:23]>>[ClH:1].[O:2]=[C:3]([Cl:4])[c:5]1[cH:6][n:7](-[c:8]2[n:9][cH:10][cH:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[cH:18][c:19]1[C:20]([F:21])([F:22])...
O=C(Cl)C(=O)Cl.O=C(O)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F
Cl.O=C(Cl)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F
null
null
ClCCl
Functional Group Interconversion
Alcohol to chloride_Other
013cec2edeb273a7a148f349d36a52d99ff4e7bcf8eed78085df830088e387ac
aedb1f68dc5b7eb0583043e1125b741382b17974140a2f46554f0110e2ddc884
c1ccc2c(-n3cccc3)nccc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[c:7]:[#7;a:8]):[c:9]:1.O=C(-[Cl;H0;D1;+0:10])-C(=O)-[Cl;H0;D1;+0:11]>>[#7;a:8]:[c:7]-[#7;a:6]1:[c:5]:[c:4]:[c:3](-[C;H0;D3;+0:1](-[Cl;H0;D1;+0:11])=[O;D1;H0:2]):[c:9]:1.[ClH;D0;+0:10]
94.1
[{"value": 94.1, "product": "Cl.ClC(=O)C1=CN(C=C1C(F)(F)F)C1=NC=CC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
2
HOUR
0.62 mL (7.18 mmol) of oxalyl chloride is added to 1.1 g (3.59 mmol) of 3-carboxy-4-trifluoromethyl-1-(isoquinolin-1-yl)-1H-pyrrole dissolved in 30 mL of dichloromethane at a temperature in the region of 20° C. under an argon atmosphere. After stirring for 2 hours at a temperature in the region of 20° C., the reaction ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Carboxylic acid
Acyl halide
null
null
c1cc[nH]c1.c1ccc2cnccc2c1
Other
ClCCl
20
2
O=C(Cl)C(=O)Cl.O=C(O)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F>ClCCl>Cl.O=C(Cl)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f8b8ad23069441068da762ab746c7678
CCOC(=O)c1c[nH]cc1C(F)(F)F.Clc1nccc2ccccc12>>CCOC(=O)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F
C(C)OC(=O)C1=CNC=C1C(F)(F)F.ClC1=NC=CC2=CC=CC=C12.C([O-])([O-])=O.[K+].[K+]>>C(C)OC(=O)C1=CN(C=C1C(F)(F)F)C1=NC=CC2=CC=CC=C12
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][nH:8][cH:19][c:20]1[C:21]([F:22])([F:23])[F:24].Cl[c:9]1[n:10][cH:11][cH:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8](-[c:9]2[n:10][cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19][c:20]1[C:21]([F:22])([F:2...
CCOC(=O)c1c[nH]cc1C(F)(F)F.Clc1nccc2ccccc12
CCOC(=O)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F
null
null
O.CS(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
64941681a78379ce7a568f1d8a1309e87b488f1d656284455a26054be1853b83
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3cccc3)nccc2c1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](:[c:5]):[c:6].[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[c:12]:[nH;D2;+0:13]:[c:14]:1>>[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[c:12]:[n;H0;D3;+0:13](-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](:[c:5]):[c:6]):[c:14]:1
87.3
[{"value": 87.3, "product": "C(C)OC(=O)C1=CN(C=C1C(F)(F)F)C1=NC=CC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
110
CELSIUS
17
HOUR
1.04 g (5 mmol) of 3-ethoxycarbonyl-4-trifluoromethyl-1H-pyrrole and 0.818 g (5 mmol) of 1-chloroisoquinoline are added to 1.73 g (12.5 mmol) of potassium carbonate suspended in 10 mL of dimethyl sulphoxide at a temperature in the region of 20° C. under an argon atmosphere. After stirring for 17 hours at a temperature ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2cnccc2c1
c1cc[nH]c1.c1ccc2cnccc2c1
c1cc[nH]c1.c1ccc2cnccc2c1
HCl
O.CS(=O)C
110
17
CCOC(=O)c1c[nH]cc1C(F)(F)F.Clc1nccc2ccccc12>O.CS(=O)C>CCOC(=O)c1cn(-c2nccc3ccccc23)cc1C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-99a153b06e49458686dfd8a4c0ec318a
COC(=O)c1c[nH]cc1C.Cc1cc(Cl)c2ccccc2n1>>COC(=O)c1cn(-c2cc(C)nc3ccccc23)cc1C
COC(=O)C1=CNC=C1C.ClC1=CC(=NC2=CC=CC=C12)C.C(=O)([O-])[O-].[Cs+].[Cs+]>>COC(=O)C1=CN(C=C1C)C1=CC(=NC2=CC=CC=C12)C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][cH:19][c:20]1[CH3:21].Cl[c:8]1[cH:9][c:10]([CH3:11])[n:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]12>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][n:7](-[c:8]2[cH:9][c:10]([CH3:11])[n:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[cH:19][c:20]1[CH3:21]
COC(=O)c1c[nH]cc1C.Cc1cc(Cl)c2ccccc2n1
COC(=O)c1cn(-c2cc(C)nc3ccccc23)cc1C
null
null
O.CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
0f41158080bd72518d9a6b2389c4c528ac037a6b5eac12dbe2506d72e4b3d2c9
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(-n3cccc3)ccnc2c1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[C;D1;H3:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9].[#8:10]-[C:11](=[O;D1;H0:12])-[c:13]1:[c:14]:[c:15]:[nH;D2;+0:16]:[c:17]:1>>[#8:10]-[C:11](=[O;D1;H0:12])-[c:13]1:[c:14]:[c:15]:[n;H0;D3;+0:16](-[c;H0;D3;+0:1]2:[c:2]:[c:3](-[C;D1;H3:4]):[#7;a:5]:[c:6](:[c:7]):[c:8]:2:[c:9]):[c:17]:1
null
[]
80
CELSIUS
60
HOUR
1 mmol (139 mg) of 4-methylpyrrole-3-carboxylic acid methyl ester, 1.1 mmol (195 mg) 4-chloro-2-methyl-quinoline and 1.2 mmol (390 mg) of Cs2CO3 are suspended in 3 mL of dry DMF. The mixture is stirred for 60 h at 80° C. under Argon, allowed to cool to room temperature, and diluted with water (20 mL). Part of the produ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
c1cc[nH]c1.c1ccc2ncccc2c1
HCl
O.CN(C)C=O
80
60
COC(=O)c1c[nH]cc1C.Cc1cc(Cl)c2ccccc2n1>O.CN(C)C=O>COC(=O)c1cn(-c2cc(C)nc3ccccc23)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-12e788a19bb94873a9b8a0a69a0fa889
COC(=O)c1cn(-c2ncccn2)cc1C.N=C(N)N>>Cc1cn(-c2ncccn2)cc1C(=O)NC(=N)N
COC(=O)C1=CN(C=C1C)C1=NC=CC=N1.NC(=N)N>>CC=1C(=CN(C1)C1=NC=CC=N1)C(=O)NC(=N)N
CO[C:13]([c:12]1[c:2]([CH3:1])[cH:3][n:4](-[c:5]2[n:6][cH:7][cH:8][cH:9][n:10]2)[cH:11]1)=[O:14].[NH2:15][C:16](=[NH:17])[NH2:18]>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[n:6][cH:7][cH:8][cH:9][n:10]2)[cH:11][c:12]1[C:13](=[O:14])[NH:15][C:16](=[NH:17])[NH2:18]
COC(=O)c1cn(-c2ncccn2)cc1C.N=C(N)N
Cc1cn(-c2ncccn2)cc1C(=O)NC(=N)N
null
null
O.CN1CCCC1=O
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
c1cnc(-n2cccc2)nc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5](-[c:6](:[#7;a:7]):[#7;a:8]):[c:9]:[c:10]:1.[N;D1;H1:11]=[C:12](-[N;D1;H2:13])-[NH2;D1;+0:14]>>[#7;a:7]:[c:6](-[#7;a:5]1:[c:4]:[c:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:14]-[C:12](=[N;D1;H1:11])-[N;D1;H2:13]):[c:10]:[c:9]:1):[#7;a:8]
53.4
[{"value": 53.4, "product": "CC=1C(=CN(C1)C1=NC=CC=N1)C(=O)NC(=N)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
250 mg 4-methyl-1-pyrimidin-2-yl-1H-pyrrole-3-carboxylic acid methyl ester was dissolved in 0.3 mL of NMP. After addition of 1 g guanidine (preparation according to known literature) the mixture was heated under argon for 1 h to 90° C. Completion of the reaction was checked by LCMS. The mixture was cooled to room tempe...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1cc[nH]c1.c1cncnc1
HO-
O.CN1CCCC1=O
null
null
COC(=O)c1cn(-c2ncccn2)cc1C.N=C(N)N>O.CN1CCCC1=O>Cc1cn(-c2ncccn2)cc1C(=O)NC(=N)N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c864c3cb49284f4dab9026da6cb4cf4e
Brc1ncccn1.COC(=O)c1c[nH]cc1C>>COC(=O)c1cn(-c2ncccn2)cc1C
COC(=O)C1=CNC=C1C.CCCCCCCCCCCC.NC1C(CCCC1)N.BrC1=NC=CC=N1.P(=O)([O-])([O-])[O-].[K+].[K+].[K+]>>COC(=O)C1=CN(C=C1C)C1=NC=CC=N1
Br[c:8]1[n:9][cH:10][cH:11][cH:12][n:13]1.[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][cH:14][c:15]1[CH3:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][n:7](-[c:8]2[n:9][cH:10][cH:11][cH:12][n:13]2)[cH:14][c:15]1[CH3:16]
Brc1ncccn1.COC(=O)c1c[nH]cc1C
COC(=O)c1cn(-c2ncccn2)cc1C
null
[Cu]I
O1CCOCC1.O
Heteroatom Alkylation and Arylation
OtherReaction
63bbfd98eb32b12003fd6c3367ae4b2d5032a668e503cabfa13b588e0290a766
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1cnc(-n2cccc2)nc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[c:11]:[nH;D2;+0:12]:[c:13]:1>>[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[c:11]:[n;H0;D3;+0:12](-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5]):[c:13]:1
69.1
[{"value": 69.1, "product": "COC(=O)C1=CN(C=C1C)C1=NC=CC=N1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
333.9 mg (2.4 mmol) 4-methyl-1H-pyrrole-3-carboxylic acid methyl ester, 891.5 mg (4.2 mmol) tri-potassium phosphate, 4 mg (0.02 mmol) CuI, 22 mg (0.2 mmol) 1,2-diaminocyclohexane and 317.9 mg (2 mmol) of 2-bromopyrimidine was suspended in 3 mL of dioxane. After addition of 90 μl of dodecane the mixture was heated in a ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cncnc1.c1cc[nH]c1
c1cc[nH]c1.c1cncnc1
c1cc[nH]c1.c1cncnc1
HBr
[Cu]I.O1CCOCC1.O
100
null
Brc1ncccn1.COC(=O)c1c[nH]cc1C>[Cu]I.O1CCOCC1.O>COC(=O)c1cn(-c2ncccn2)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e3dfb049cb4746e288a1f0696039d8f4
NC(=O)[C@@H]1CCCN1S(=O)(=O)Cc1ccccc1>>N#C[C@@H]1CCCN1S(=O)(=O)Cc1ccccc1
N1=CC=CC=C1.C1(=CC=CC=C1)CS(=O)(=O)N1[C@@H](CCC1)C(=O)N.CN(C)C=O.C(C(=O)Cl)(=O)Cl>>C1(=CC=CC=C1)CS(=O)(=O)N1[C@@H](CCC1)C#N
O=[C:2]([NH2:1])[C@@H:3]1[CH2:4][CH2:5][CH2:6][N:7]1[S:8](=[O:9])(=[O:10])[CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[N:1]#[C:2][C@@H:3]1[CH2:4][CH2:5][CH2:6][N:7]1[S:8](=[O:9])(=[O:10])[CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1
NC(=O)[C@@H]1CCCN1S(=O)(=O)Cc1ccccc1
N#C[C@@H]1CCCN1S(=O)(=O)Cc1ccccc1
null
null
O.C(C)#N
Miscellaneous
OtherReaction
5094e9d814705bbdc421edbf7e9198e499e70e93916e2cec6eefbc82d1ba5440
32b9893bcb5223559a9d02852f8392cf6473aacfb044a52ba4e9cb9c29edb170
O=S(=O)(Cc1ccccc1)N1CCCC1
O=[C;H0;D3;+0:1](-[NH2;D1;+0:2])-[C:3](-[C:4])-[#7:5](-[#16:6])-[C:7]>>[#16:6]-[#7:5](-[C:7])-[C:3](-[C;H0;D2;+0:1]#[N;H0;D1;+0:2])-[C:4]
80
[{"value": 80.0, "product": "C1(=CC=CC=C1)CS(=O)(=O)N1[C@@H](CCC1)C#N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.9, "product": "C1(=CC=CC=C1)CS(=O)(=O)N1[C@@H](CCC1)C#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
To a solution of 0.67 ml DMF (8.7 mmol)in 10 ml acetonitrile at 0° C. was added 0.70 ml (8.0 mmol) oxalyl chloride. A white precipitate was formed immediately and was accompanied by gas evolution. When complete, a solution of 2.0 g (7.5 mmol) of (2S)-1-(phenylmethyl)sulfonyl-2-pyrrolidinecarboxamide in 5.0 ml acetonitr...
10.6084/m9.figshare.5104873.v1
null
Primary amide
Nitrile
null
null
C1CC[NH]C1.c1ccccc1
HO-
O.C(C)#N
null
0.083333
NC(=O)[C@@H]1CCCN1S(=O)(=O)Cc1ccccc1>O.C(C)#N>N#C[C@@H]1CCCN1S(=O)(=O)Cc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e9a6a7c80639419f9d88502602309155
CC(C)CBr.N#Cc1ccc(O)cc1>>CC(C)COc1ccc(C#N)cc1
C(C(C)C)Br.C(#N)C1=CC=C(C=C1)O.C(C)N(CC)CC>>C(C(C)C)OC1=CC=C(C#N)C=C1
Br[CH2:4][CH:2]([CH3:1])[CH3:3].[OH:5][c:6]1[cH:7][cH:8][c:9]([C:10]#[N:11])[cH:12][cH:13]1>>[CH3:1][CH:2]([CH3:3])[CH2:4][O:5][c:6]1[cH:7][cH:8][c:9]([C:10]#[N:11])[cH:12][cH:13]1
CC(C)CBr.N#Cc1ccc(O)cc1
CC(C)COc1ccc(C#N)cc1
null
null
O.CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](-[C;D1;H3:3])-[C;D1;H3:4].[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C;D1;H3:3]-[C:2](-[C;D1;H3:4])-[CH2;D2;+0:1]-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8]
85.6
[{"value": 85.0, "product": "C(C(C)C)OC1=CC=C(C#N)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.6, "product": "C(C(C)C)OC1=CC=C(C#N)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
6
HOUR
To a solution of 4-cyanophenol (1.2 g, 10 mmol) in dry DMF (20 mL) was added triethylamine (20 mmol) followed by i-butyl bromide (2.7 g, 20 mmol). The resulting reaction mixture was stirred at 100° C. for 6 h. After cooling to room temperature, the reaction mixture was diluted with water (100 mL) and extracted with eth...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HBr
O.CN(C)C=O
100
6
CC(C)CBr.N#Cc1ccc(O)cc1>O.CN(C)C=O>CC(C)COc1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-677e608584e14eae9651397497b27789
CCOC(=O)c1cc[nH]n1.OB(O)c1ccc(Oc2ccccc2)cc1.c1ccncc1>>CCOC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1.CCOC(=O)c1ccnn1-c1ccc(Oc2ccccc2)cc1
N1=CC=CC=C1.O(C1=CC=CC=C1)C1=CC=C(C=C1)B(O)O.N1N=C(C=C1)C(=O)OCC>>C(C)OC(=O)C1=CC=NN1C1=CC=C(C=C1)OC1=CC=CC=C1.C(C)OC(=O)C1=NN(C=C1)C1=CC=C(C=C1)OC1=CC=CC=C1
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][nH:9][n:23]1.B([c:10]1[cH:11][cH:12][c:13]([O:14][c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[cH:21][cH:22]1)([OH:26])[OH:28].[cH:24]1[n:32][cH:45][cH:46][cH:34][cH:35]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][n:9](-[c:10]2[cH:11][cH:12][c:13]([O:14][c:15]3...
CCOC(=O)c1cc[nH]n1.OB(O)c1ccc(Oc2ccccc2)cc1.c1ccncc1
CCOC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1.CCOC(=O)c1ccnn1-c1ccc(Oc2ccccc2)cc1
null
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-]
C1CCOC1
Aromatic Heterocycle Formation
OtherReaction
a85630168167151eeafbcbe0f4bebb6ba9bb7c40ddfe690cf48700330de56629
c9a91b65b405014440f8dd316252f5fba458efc41eb66897e3c7221a91f12ced
c1ccc(Oc2ccc(-n3cccn3)cc2)cc1.c1ccc(Oc2ccc(-n3cccn3)cc2)cc1
[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#7;a:5]:[nH;D2;+0:6]:[c:7]:[c:8]:1.[OH;D1;+0:9]-B(-[OH;D1;+0:10])-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15].[c:16]1:[cH;D2;+0:17]:[cH;D2;+0:18]:[cH;D2;+0:19]:[n;H0;D2;+0:20]:[cH;D2;+0:21]:1>>[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#7;a:5]:[n;H0;D3;+0:6](-[c;H0;D3;+0:11](:[c:12]:[c:13])...
10.3
[{"value": 4.6, "product": "C(C)OC(=O)C1=CC=NN1C1=CC=C(C=C1)OC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 10.3, "product": "C(C)OC(=O)C1=NN(C=C1)C1=CC=C(C=C1)OC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
200
CELSIUS
2
DAY
To a suspension of 4-phenoxyphenylboronic acid (1.70 g, 7.85 mmol), ethyl 3-pyrazolecarboxylate (0.55 g, 3.92 mmol), copper(II)acetate (1.1 g, 5.89 mmol) and 4 Å molecular sieves (powdered and heated at 200° C. for 2 h prior to use) in 30 mL of anhydrous THF was added 0.6 mL of pyridine. The reaction was stirred open t...
10.6084/m9.figshare.5104873.v1
null
Boronic acid
Ester.Ether
c1cn[nH]c1.c1ccccc1.c1ccncc1
c1cc[nH]n1.c1ccccc1.c1cc[nH]n1.c1ccccc1.c1ccccc1
c1cc[nH]n1.c1ccccc1.c1ccccc1.c1cc[nH]n1.c1ccccc1.c1ccccc1
B
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].C1CCOC1
200
48
CCOC(=O)c1cc[nH]n1.OB(O)c1ccc(Oc2ccccc2)cc1.c1ccncc1>C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].C1CCOC1>CCOC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1.CCOC(=O)c1ccnn1-c1ccc(Oc2ccccc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-47043342eedf41c39c183b9b9d91e68b
CCOC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1.N>>NC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1
C(C)OC(=O)C1=NN(C=C1)C1=CC=C(C=C1)OC1=CC=CC=C1.N>>O(C1=CC=CC=C1)C1=CC=C(C=C1)N1N=C(C=C1)C(=O)N
CCO[C:2](=[O:3])[c:4]1[cH:5][cH:6][n:7](-[c:8]2[cH:9][cH:10][c:11]([O:12][c:13]3[cH:14][cH:15][cH:16][cH:17][cH:18]3)[cH:19][cH:20]2)[n:21]1.[NH3:1]>>[NH2:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][n:7](-[c:8]2[cH:9][cH:10][c:11]([O:12][c:13]3[cH:14][cH:15][cH:16][cH:17][cH:18]3)[cH:19][cH:20]2)[n:21]1
CCOC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1.N
NC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1
null
null
CO
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
c1ccc(Oc2ccc(-n3cccn3)cc2)cc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1.[NH3;D0;+0:9]>>[NH2;D1;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[#7;a:5](-[c:6]):[c:7]:[c:8]:1
52
[{"value": 52.0, "product": "O(C1=CC=CC=C1)C1=CC=C(C=C1)N1N=C(C=C1)C(=O)N", "details": "PERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
A solution of 3-ethoxycarbonyl-1-(4-phenoxyphenyl)-1H-pyrazole (120 mg, 0.39 mmol) in 5 mL of a 2N solution of ammonia in MeOH was stirred at rt for 4 d. TLC showed incomplete reaction and the solution was transferred to a sealed tube and heated at 70° C. overnight. The reaction was concentrated and purified by prepara...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
c1cc[nH]n1.c1ccccc1.c1ccccc1
HO-
CO
70
null
CCOC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1.N>CO>NC(=O)c1ccn(-c2ccc(Oc3ccccc3)cc2)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-146028626a484ff4b6f99e630f21f98f
O=[N+]([O-])c1ccc(F)cc1.Oc1ccc(-n2cncn2)cc1>>O=[N+]([O-])c1ccc(Oc2ccc(-n3cncn3)cc2)cc1
FC1=CC=C(C=C1)[N+](=O)[O-].N1(N=CN=C1)C1=CC=C(C=C1)O.C([O-])([O-])=O.[K+].[K+]>>[N+](=O)([O-])C1=CC=C(OC2=CC=C(C=C2)N2N=CN=C2)C=C1
F[c:7]1[cH:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:21][cH:20]1.[OH:8][c:9]1[cH:10][cH:11][c:12](-[n:13]2[cH:14][n:15][cH:16][n:17]2)[cH:18][cH:19]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12](-[n:13]3[cH:14][n:15][cH:16][n:17]3)[cH:18][cH:19]2)[cH:20][cH:21]1
O=[N+]([O-])c1ccc(F)cc1.Oc1ccc(-n2cncn2)cc1
O=[N+]([O-])c1ccc(Oc2ccc(-n3cncn3)cc2)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
e4ea1e38252bc3b9c5ec04486386725e6570ab3860d45e337a1d131319bbf0fc
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccc(-n3cncn3)cc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:8]:[c:7](-[O;H0;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]
37
[{"value": 37.0, "product": "[N+](=O)([O-])C1=CC=C(OC2=CC=C(C=C2)N2N=CN=C2)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 37.0, "product": "[N+](=O)([O-])C1=CC=C(OC2=CC=C(C=C2)N2N=CN=C2)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 1-fluoro-4-nitrobenzene (0.17 mL, 1.6 mmol), 4-{[1,2,4]triazol-1-yl}phenol (0.26 g, 1.58 mmol), and potassium carbonate (1.69 g, 12.2 mmol) in DMF was refluxed overnight. The reaction was cooled to room temperature, then partitioned between water and ethyl acetate. The aqueous layer was extracted with ethy...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1nc[nH]n1
HF
CN(C)C=O
null
null
O=[N+]([O-])c1ccc(F)cc1.Oc1ccc(-n2cncn2)cc1>CN(C)C=O>O=[N+]([O-])c1ccc(Oc2ccc(-n3cncn3)cc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ea5003e1ea4245e69a25cbcadf491b4f
O=N[O-].O=[N+]([O-])Nc1ccccc1.Oc1ccccc1>>O=[N+]([O-])c1cccc(O)c1N=Nc1ccccc1O
C1(=CC=CC=C1)O.[OH-].[Na+].N(=O)[O-].[Na+].[N+](=O)([O-])NC1=CC=CC=C1.Cl.NC1=CC=CC=C1>>[N+](=O)([O-])C=1C(=C(C=CC1)O)N=NC1=C(C=CC=C1)O
O=[N:12][O-:9].[O:1]=[N+:2]([O-:3])[NH:11][c:10]1[cH:4][cH:5][cH:6][cH:7][cH:8]1.[cH:13]1[cH:14][cH:15][cH:16][cH:17][c:18]1[OH:19]>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][cH:7][c:8]([OH:9])[c:10]1[N:11]=[N:12][c:13]1[cH:14][cH:15][cH:16][cH:17][c:18]1[OH:19]
O=N[O-].O=[N+]([O-])Nc1ccccc1.Oc1ccccc1
O=[N+]([O-])c1cccc(O)c1N=Nc1ccccc1O
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
7750ee4645b53126d634e4bc5688e84fdac9a5a48b07f7139ec6a9f4af77ecc3
bf95fff5da4183d154466c3f1c3dd8ab7274e4ee078306c8c32913076deed1be
c1ccc(N=Nc2ccccc2)cc1
O=[N;H0;D2;+0:1]-[O-;H0;D1:2].[O;-;D1;H0:3]-[N+;H0;D3:4](=[O;D1;H0:5])-[NH;D2;+0:6]-[c:7]1:[cH;D2;+0:8]:[c:9]:[c:10]:[c:11]:[cH;D2;+0:12]:1.[O;D1;H1:13]-[c:14](:[c:15]):[cH;D2;+0:16]:[c:17]:[c:18]>>[O;-;D1;H0:3]-[N+;H0;D3:4](=[O;D1;H0:5])-[c;H0;D3;+0:8]1:[c:9]:[c:10]:[c:11]:[c;H0;D3;+0:12](-[OH;D1;+0:2]):[c:7]:1-[N;H0;...
51.5
[{"value": 51.5, "product": "[N+](=O)([O-])C=1C(=C(C=CC1)O)N=NC1=C(C=CC=C1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Nitro aniline (138.13 g) was mixed with 500 mL of concentrated HCl and stirred for several min. When all the aniline was dissolved, the solution was cooled down to room temperature and diluted with water (300 mL), and then a solution of NaNO2 (69 g) in 250 mL of water was dropwise added at 0° C. The solution became a c...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Nitroso
Diazene.Nitro group.Aromatic alcohol
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HO-
O
null
null
O=N[O-].O=[N+]([O-])Nc1ccccc1.Oc1ccccc1>O>O=[N+]([O-])c1cccc(O)c1N=Nc1ccccc1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-bfe19503fdc247b9865afff196382cda
COc1c(Cl)cc(C)c(C)c1[N+](=O)[O-]>>COc1c(Cl)cc(C)c(C)c1N
ClC1=C(C(=C(C(=C1)C)C)[N+](=O)[O-])OC>>ClC=1C(=C(C(=C(C1)C)C)N)OC
O=[N+:12]([O-])[c:11]1[c:3]([O:2][CH3:1])[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:9]1[CH3:10]>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:9]([CH3:10])[c:11]1[NH2:12]
COc1c(Cl)cc(C)c(C)c1[N+](=O)[O-]
COc1c(Cl)cc(C)c(C)c1N
null
null
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
15
HOUR
1-Chloro-2-methoxy-4,5-dimethyl-3-nitro-benzene (10.0 g, 46.4 mmol; Stachel et. al., J. Org. Chem. 1997, 46, 4756) is dissolved in MeOH (200 mL) in a 500 mL round bottom flask. The flask is purged with N2 and 10% Pd on Carbon (0.7 g) is added and the reaction is again purged with N2. The reaction is purged with H2 and ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
CO
null
15
COc1c(Cl)cc(C)c(C)c1[N+](=O)[O-]>CO>COc1c(Cl)cc(C)c(C)c1N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c9c0277dacc746b3a8d39d989cf54fd1
CC(=O)OC(C)=O.COc1c(Cl)cc(C)c(C)c1N>>COc1c(Cl)cc(C)c(C)c1NC(C)=O
CO.N1=CC=CC=C1.ClC=1C(=C(C(=C(C1)C)C)N)OC.C(C)(=O)OC(C)=O>>ClC=1C(=C(C(=C(C1)C)C)NC(C)=O)OC
CC(=O)O[C:13]([CH3:14])=[O:15].[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:9]([CH3:10])[c:11]1[NH2:12]>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:9]([CH3:10])[c:11]1[NH:12][C:13]([CH3:14])=[O:15]
CC(=O)OC(C)=O.COc1c(Cl)cc(C)c(C)c1N
COc1c(Cl)cc(C)c(C)c1NC(C)=O
null
CN(C)C=1C=CN=CC1
ClCCl.CCOC(=O)C
Acylation
Aminolysis of esters
87d35e51b477fc9a658a6f307eb56d84c8879182772c9dd3a42ec0d584fd2684
627cbc0550c9f51ad0105d9fcf46677e8c93bed87ee95bfe69292a82550c95b7
c1ccccc1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[NH2;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[NH;D2;+0:4]-[c:5](:[c:6]):[c:7]
null
[]
null
null
2
HOUR
3-Chloro-2-methoxy-5,6-dimethyl-phenylamine (4.9 g, 26 mmol) is dissolved in dichloromethane (20 mL) and pyridine (8 mL) and cooled to 0° C. Acetic anhydride (3.7 mL, 39 mmol) and DMAP (85 mg, 0.7 mmol) are added and the reaction is allowed to warm to room temperature. After stirring 2 h, the reaction is diluted with E...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary amine
Secondary amide
null
null
c1ccccc1
HO-
CN(C)C=1C=CN=CC1.ClCCl.CCOC(=O)C
null
2
CC(=O)OC(C)=O.COc1c(Cl)cc(C)c(C)c1N>CN(C)C=1C=CN=CC1.ClCCl.CCOC(=O)C>COc1c(Cl)cc(C)c(C)c1NC(C)=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cc3d07a142de43c993bd55af94fd01c6
COc1c(Cl)cc(C)c(C)c1NC(C)=O>>COc1c(Cl)cc(C)c2cn[nH]c12
Cl.ClC=1C(=C(C(=C(C1)C)C)NC(C)=O)OC.N(=O)[O-].[Na+]>>ClC1=CC(=C2C=NNC2=C1OC)C
CC(=O)[NH:12][c:13]1[c:3]([O:2][CH3:1])[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:9]1[CH3:10]>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:9]2[cH:10][n:11][nH:12][c:13]12
COc1c(Cl)cc(C)c(C)c1NC(C)=O
COc1c(Cl)cc(C)c2cn[nH]c12
null
null
O.CC(=O)O
Aromatic Heterocycle Formation
OtherReaction
7c3f37568a0442a88eb873bc34c78039cddfa7e4dc5a6457eea74221a4843bd4
4c49decc0d3b49884847872e93a9c81862e00fd5fd04c96a796b9efc98b43f78
c1ccc2[nH]ncc2c1
C-C(=O)-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4](-[CH3;D1;+0:5]):[c:6]>>[c:3]:[c:2]1:[nH;D2;+0:1]:[#7;a:7]:[cH;D2;+0:5]:[c:4]:1:[c:6]
null
[]
0
CELSIUS
45
MINUTE
N-(3-Chloro-2-methoxy-5,6-dimethyl-phenyl)-acetamide (3.36 g, 17.4 mmol) is dissolved in HOAc (75 mL) and conc. HCl (30 mL) in a 1 L round bottom flask. The reaction is cooled to 0° C. with an ice/salt bath. Although some starting material crystallizes, a solution of NaNO2 (5.9 g, 86 mmol) in water (25 mL) is added por...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
null
c1ccccc1
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1
HO-
O.CC(=O)O
0
0.75
COc1c(Cl)cc(C)c(C)c1NC(C)=O>O.CC(=O)O>COc1c(Cl)cc(C)c2cn[nH]c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c5e831d81db04554ad370dbf099ba58f
COc1c(Cl)cc(C)c2cn[nH]c12.O=S(=O)(Cl)c1ccccc1>>COc1c(Cl)cc(C)c2cnn(S(=O)(=O)c3ccccc3)c12
ClC1=CC(=C2C=NNC2=C1OC)C.[H-].[Na+].C1(=CC=CC=C1)S(=O)(=O)Cl>>C1(=CC=CC=C1)S(=O)(=O)N1N=CC2=C(C=C(C(=C12)OC)Cl)C
[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:9]2[cH:10][n:11][nH:12][c:22]12.Cl[S:13](=[O:14])(=[O:15])[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:9]2[cH:10][n:11][n:12]([S:13](=[O:14])(=[O:15])[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[c:22]12
COc1c(Cl)cc(C)c2cn[nH]c12.O=S(=O)(Cl)c1ccccc1
COc1c(Cl)cc(C)c2cnn(S(=O)(=O)c3ccccc3)c12
null
null
CCOC(=O)C.C1CCOC1
Acylation
OtherReaction
9ac2dd9da4cf023ae9acc8d8197a5ce03307f6588facb195f026e0f0c7cbe262
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1ccccc1)n1ncc2ccccc21
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[c:7]:[c:8]1:[c:9]:[c:10]:[#7;a:11]:[nH;D2;+0:12]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6])-[n;H0;D3;+0:12]1:[#7;a:11]:[c:10]:[c:9]:[c:8]:1:[c:7]
null
[]
0
CELSIUS
10
MINUTE
6-Chloro-7-methoxy-4-methyl-1H-indazole (1.55 g, 9.2 mmol) is dissolved in THF (50 mL) and cooled to 0° C. Sodium hydride (60% in mineral oil, 0.40 g, 10 mmol) is added and the reaction is stirred 10 min. Benzenesulfonyl chloride (1.2 mL, 9.7 mmol) is added and the reaction is stirred 20 min. The reaction is diluted wi...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1ccc2n[nH]cc2c1
c1cc2n[nH]cc2cc1
c1cc2n[nH]cc2cc1.c1ccccc1
HCl
CCOC(=O)C.C1CCOC1
0
0.166667
COc1c(Cl)cc(C)c2cn[nH]c12.O=S(=O)(Cl)c1ccccc1>CCOC(=O)C.C1CCOC1>COc1c(Cl)cc(C)c2cnn(S(=O)(=O)c3ccccc3)c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-efa69b70099d4206978f2bc3d9f4c70b
COc1c(Cl)cc(C)c2cnn(S(=O)(=O)c3ccccc3)c12.O=C1CCC(=O)N1Br>>COc1c(Cl)cc(CBr)c2cnn(S(=O)(=O)c3ccccc3)c12
C1(=CC=CC=C1)S(=O)(=O)N1N=CC2=C(C=C(C(=C12)OC)Cl)C.BrN1C(CCC1=O)=O.C(C1=CC=CC=C1)(=O)OOC(C1=CC=CC=C1)=O>>C1(=CC=CC=C1)S(=O)(=O)N1N=CC2=C(C=C(C(=C12)OC)Cl)CBr
[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH3:8])[c:10]2[cH:11][n:12][n:13]([S:14](=[O:15])(=[O:16])[c:17]3[cH:18][cH:19][cH:20][cH:21][cH:22]3)[c:23]12.O=C1CCC(=O)N1[Br:9]>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH2:8][Br:9])[c:10]2[cH:11][n:12][n:13]([S:14](=[O:15])(=[O:16])[c:17]3[cH:18][cH:19][cH:20][cH:21][...
COc1c(Cl)cc(C)c2cnn(S(=O)(=O)c3ccccc3)c12.O=C1CCC(=O)N1Br
COc1c(Cl)cc(CBr)c2cnn(S(=O)(=O)c3ccccc3)c12
null
null
C(Cl)(Cl)(Cl)Cl
Functional Group Interconversion
Wohl-Ziegler bromination benzyl primary
45c0aca0d63a96f0092e6dded9c888827eaf6379dac179e1cefc99293896300a
08f5e7e34d3f321cce3e85421b38226d6240cca0939494ae61032d4f8405cf22
O=S(=O)(c1ccccc1)n1ncc2ccccc21
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[CH3;D1;+0:2]-[c:3](:[c:4]):[c:5]1:[c:6]:[#7;a:7]:[#7;a:8]:[c:9]:1>>[Br;H0;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]1:[c:6]:[#7;a:7]:[#7;a:8]:[c:9]:1
null
[]
null
null
null
null
1-Benzenesulfonyl-6-chloro-7-methoxy-4-methyl-1H-indazole (2.45 g, 7.3 mmol), recrystallized N-bromosuccinimide (1.36 g, 7.6 mmol) and benzoyl peroxide (90 mg, 0.37 mmol) are dissolved in carbon tetrachloride (25 mL). The reaction is degassed and then placed in a 80° C. bath. The reaction is heated (about 2 h) until no...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Primary halide
C1CCNC1
null
c1cc2n[nH]cc2cc1.c1ccccc1
HO-
C(Cl)(Cl)(Cl)Cl
null
null
COc1c(Cl)cc(C)c2cnn(S(=O)(=O)c3ccccc3)c12.O=C1CCC(=O)N1Br>C(Cl)(Cl)(Cl)Cl>COc1c(Cl)cc(CBr)c2cnn(S(=O)(=O)c3ccccc3)c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2fcc050a462145c7bb42d8662cfb0bda
COc1c(Cl)cc(CBr)c2cnn(S(=O)(=O)c3ccccc3)c12.O=C(CN=C(c1ccccc1)c1ccccc1)NCCCCc1ccccc1>>COc1c(Cl)cc(CC(N=C(c2ccccc2)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12
C[Si](C)(C)[N-][Si](C)(C)C.[K+].C1(=CC=CC=C1)C(C1=CC=CC=C1)=NCC(=O)NCCCCC1=CC=CC=C1.C1(=CC=CC=C1)S(=O)(=O)N1N=CC2=C(C=C(C(=C12)OC)Cl)CBr.[NH4+].[Cl-]>>C1(=CC=CC=C1)S(=O)(=O)N1N=CC2=C(C=C(C(=C12)OC)Cl)CC(C(=O)NCCCCC1=CC=CC=C1)N=C(C1=CC=CC=C1)C1=CC=CC=C1
Br[CH2:8][c:7]1[cH:6][c:4]([Cl:5])[c:3]([O:2][CH3:1])[c:50]2[c:37]1[cH:38][n:39][n:40]2[S:41](=[O:42])(=[O:43])[c:44]1[cH:45][cH:46][cH:47][cH:48][cH:49]1.[CH2:9]([N:10]=[C:11]([c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1)[C:24](=[O:25])[NH:26][CH2:27][CH2:28][CH2:29][CH2:30][...
COc1c(Cl)cc(CBr)c2cnn(S(=O)(=O)c3ccccc3)c12.O=C(CN=C(c1ccccc1)c1ccccc1)NCCCCc1ccccc1
COc1c(Cl)cc(CC(N=C(c2ccccc2)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12
null
null
C1CCOC1
C-C Coupling
OtherReaction
3eaaf72d0aea14ab64cbf2eaa034379ac1e018e2ca0aa69ec5bc55c38e063b81
5ea282f99a76ae0e99b6e606662ec1abb910dbc800826700b7b11b1baf068309
O=C(NCCCCc1ccccc1)C(Cc1cccc2c1cnn2S(=O)(=O)c1ccccc1)N=C(c1ccccc1)c1ccccc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]1:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1.[C:9]-[#7:10]-[C:11](=[O;D1;H0:12])-[CH2;D2;+0:13]-[#7:14]=[C:15](-[c:16])-[c:17]>>[C:9]-[#7:10]-[C:11](=[O;D1;H0:12])-[CH;D3;+0:13](-[#7:14]=[C:15](-[c:16])-[c:17])-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]1:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1
null
[]
-78
CELSIUS
15
MINUTE
2-(Diphenylmethylenamino)-N-(4-phenyl-butyl)-acetamide (7) (0.57 g, 1.5 mmol) is dissolved in dry THF (5 mL) and cooled to −78° C. A solution of KHMDS (0.5 M in PhMe, 3.0 mL, 1.5 mmol) is added slowly to the imide. The solution is warmed to 0° C. and then cooled to −78° C. A solution of 1-benzenesulfonyl-4-bromomethyl-...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Substituted imine
Substituted imine
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1cc2n[nH]cc2cc1.c1ccccc1
HBr
C1CCOC1
-78
0.25
COc1c(Cl)cc(CBr)c2cnn(S(=O)(=O)c3ccccc3)c12.O=C(CN=C(c1ccccc1)c1ccccc1)NCCCCc1ccccc1>C1CCOC1>COc1c(Cl)cc(CC(N=C(c2ccccc2)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0db2ae4f7d5149f7b444cdd22e60ad48
COc1c(Cl)cc(CC(N=C(c2ccccc2)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12>>COc1c(Cl)cc(CC(N)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12
C1(=CC=CC=C1)S(=O)(=O)N1N=CC2=C(C=C(C(=C12)OC)Cl)CC(C(=O)NCCCCC1=CC=CC=C1)N=C(C1=CC=CC=C1)C1=CC=CC=C1.Cl>>Cl.NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=NN(C2=C(C(=C1)Cl)OC)S(=O)(=O)C1=CC=CC=C1
c1ccc(C(c2ccccc2)=[N:10][CH:9]([CH2:8][c:7]2[cH:6][c:4]([Cl:5])[c:3]([O:2][CH3:1])[c:37]3[c:24]2[cH:25][n:26][n:27]3[S:28](=[O:29])(=[O:30])[c:31]2[cH:32][cH:33][cH:34][cH:35][cH:36]2)[C:11](=[O:12])[NH:13][CH2:14][CH2:15][CH2:16][CH2:17][c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)cc1>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[c...
COc1c(Cl)cc(CC(N=C(c2ccccc2)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12
COc1c(Cl)cc(CC(N)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12
null
null
CCOCC
Miscellaneous
OtherReaction
fe28e0513c54643a2e998df32fe9ad14c978580c0e1fa51268908e5a62d5d818
69d38cb38c5a54a23121b1c97287244fbbd5b6f97c6a1faf8cb1a05e149dd1cc
O=C(CCc1cccc2c1cnn2S(=O)(=O)c1ccccc1)NCCCCc1ccccc1
[C:1]-[#7:2]-[C:3](=[O;D1;H0:4])-[C:5](-[C:6])-[N;H0;D2;+0:7]=C(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[C:1]-[#7:2]-[C:3](=[O;D1;H0:4])-[C:5](-[C:6])-[NH2;D1;+0:7]
null
[]
null
null
null
null
3-(1-Benzenesulfonyl-6-chloro-7-methoxy-1H-indazol-4-yl)-2-(diphenylmethylenamino)-N-(4-phenyl-butyl)-propionamide (0.46 g, 0.65 mmol) is dissolved in Et2O (15 mL) and rapidly stirred with 2N HCl for 14 hours. The ether layer was decanted and the remaining aqueous layer was washed with Et2O. The aqueous layer was then ...
10.6084/m9.figshare.5104873.v1
null
Substituted imine
Primary amine
c1ccccc1.c1ccccc1
null
c1ccccc1.c1cc2n[nH]cc2cc1.c1ccccc1
Other
CCOCC
null
null
COc1c(Cl)cc(CC(N=C(c2ccccc2)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12>CCOCC>COc1c(Cl)cc(CC(N)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0dd0762a70394299b19c9382db300680
COc1c(Cl)cc(CC(N)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12.O=S(=O)(Cl)c1ccccc1>>COc1c(Cl)ccc2c(CC(NS(=O)(=O)c3ccccc3)C(=O)NCCCCc3ccccc3)nn(S(=O)(=O)c3ccccc3)c12
Cl.NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=NN(C2=C(C(=C1)Cl)OC)S(=O)(=O)C1=CC=CC=C1.N1=CC=CC=C1.C1(=CC=CC=C1)S(=O)(=O)Cl>>C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=NN(C2=C(C(=CC=C12)Cl)OC)S(=O)(=O)C1=CC=CC=C1
[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([CH2:10][CH:11]([NH2:12])[C:22](=[O:23])[NH:24][CH2:25][CH2:26][CH2:27][CH2:28][c:29]2[cH:30][cH:31][cH:32][cH:33][cH:34]2)[c:8]2[cH:9][n:35][n:36]([S:37](=[O:38])(=[O:39])[c:40]3[cH:41][cH:42][cH:43][cH:44][cH:45]3)[c:46]12.Cl[S:13](=[O:14])(=[O:15])[c:16]1[cH:17][cH:18][cH:1...
COc1c(Cl)cc(CC(N)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12.O=S(=O)(Cl)c1ccccc1
COc1c(Cl)ccc2c(CC(NS(=O)(=O)c3ccccc3)C(=O)NCCCCc3ccccc3)nn(S(=O)(=O)c3ccccc3)c12
null
null
ClCCl.CCOC(=O)C
Acylation
OtherReaction
552b5ee834d5fd6842eb06ae8172e5b392b00560296acf79784aebb4778c0007
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C(NCCCCc1ccccc1)C(Cc1nn(S(=O)(=O)c2ccccc2)c2ccccc12)NS(=O)(=O)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[#16:7]-[#7;a:8]1:[#7;a:9]:[cH;D2;+0:10]:[c:11]2:[c:12]:1:[c:13]:[c:14]:[c:15]:[c;H0;D3;+0:16]:2-[CH2;D2;+0:17]-[C:18](-[NH2;D1;+0:19])-[C:20](=[O;D1;H0:21])-[#7:22]-[C:23]>>[#16:7]-[#7;a:8]1:[#7;a:9]:[c;H0;D3;+0:10](-[CH2;D2;+0:17]-[C:18](-[NH;D2;+0:19]...
null
[]
null
null
18
HOUR
2-Amino-3-(1-benzenesulfonyl-6-chloro-7-methoxy-1H-indazol-4-yl)-N-(4-phenyl-butyl)-propionamide hydrochloride (0.31 g, 0.54 mmol) is dissolved in a mixture of dichloromethane (4 mL) and pyridine (1.5 mL). Benzenesulfonyl chloride (0.12 mL, 0.9 mmol) is added portionwise and the reaction is allowed to stir for a total ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
c1cc2n[nH]cc2cc1
c1cc2n[nH]cc2cc1
c1ccccc1.c1ccccc1.c1cc2n[nH]cc2cc1.c1ccccc1
HCl
ClCCl.CCOC(=O)C
null
18
COc1c(Cl)cc(CC(N)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12.O=S(=O)(Cl)c1ccccc1>ClCCl.CCOC(=O)C>COc1c(Cl)ccc2c(CC(NS(=O)(=O)c3ccccc3)C(=O)NCCCCc3ccccc3)nn(S(=O)(=O)c3ccccc3)c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-945f0118a4544b1b9d86e075f4bc99d9
COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12>>COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=NN(C2=C(C(=C1)Cl)OC)S(=O)(=O)C1=CC=CC=C1.C(=O)([O-])[O-].[K+].[K+]>>C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=NNC2=C(C(=C1)Cl)OC
O=S(=O)(c1ccccc1)[n:36]1[n:35][cH:34][c:33]2[c:7]([CH2:8][CH:9]([NH:10][S:11](=[O:12])(=[O:13])[c:14]3[cH:15][cH:16][cH:17][cH:18][cH:19]3)[C:20](=[O:21])[NH:22][CH2:23][CH2:24][CH2:25][CH2:26][c:27]3[cH:28][cH:29][cH:30][cH:31][cH:32]3)[cH:6][c:4]([Cl:5])[c:3]([O:2][CH3:1])[c:37]21>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:...
COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12
COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
null
null
CO
Reduction
OtherReaction
5f3909121e327cf6bb6aee1b4f3390bb46be143d2b86e61210c3173691ea78ef
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
O=C(NCCCCc1ccccc1)C(Cc1cccc2[nH]ncc12)NS(=O)(=O)c1ccccc1
O=S(=O)(-[n;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5]:1:[c:6])-c1:c:c:c:c:c:1>>[c:6]:[c:5]1:[c:4]:[c:3]:[#7;a:2]:[nH;D2;+0:1]:1
null
[]
null
null
1
HOUR
2-Benzenesulfonylamino-3-(1-benzenesulfonyl-6-chloro-7-methoxy-1H-indazol-4-yl)-N-(4-phenyl-butyl)-propionamide (0.17 g, 0.25 mmol) is dissolved in MeOH (2 mL) and K2CO3 is added and the reaction is stirred for 1 h. The reaction is quenched by the addition of 2 N HCl (0.1 mL) and then concentrated. The residue is disso...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccccc1.c1cc2[nH]ncc2cc1
c1ccc2n[nH]cc2c1
c1ccccc1.c1ccccc1.c1ccc2n[nH]cc2c1
HO-
CO
null
1
COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cnn(S(=O)(=O)c3ccccc3)c12>CO>COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a1f2beba88ac49209805ebde323201bc
COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12>>O=C(NCCCCc1ccccc1)C(Cc1cc(Cl)c(O)c2[nH]ncc12)NS(=O)(=O)c1ccccc1
C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=NNC2=C(C(=C1)Cl)OC.Cl.[NH+]1=CC=CC=C1>>C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=NNC2=C(C(=C1)Cl)O
C[O:21][c:20]1[c:18]([Cl:19])[cH:17][c:16]([CH2:15][CH:14]([C:2](=[O:1])[NH:3][CH2:4][CH2:5][CH2:6][CH2:7][c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[NH:27][S:28](=[O:29])(=[O:30])[c:31]2[cH:32][cH:33][cH:34][cH:35][cH:36]2)[c:26]2[c:22]1[nH:23][n:24][cH:25]2>>[O:1]=[C:2]([NH:3][CH2:4][CH2:5][CH2:6][CH2:7][c:8]1[cH:9][c...
COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
O=C(NCCCCc1ccccc1)C(Cc1cc(Cl)c(O)c2[nH]ncc12)NS(=O)(=O)c1ccccc1
null
null
null
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=C(NCCCCc1ccccc1)C(Cc1cccc2[nH]ncc12)NS(=O)(=O)c1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]1:[#7;a:5]:[#7;a:6]:[c:7]:[c:8]:1>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]1:[#7;a:5]:[#7;a:6]:[c:7]:[c:8]:1
null
[]
null
null
null
null
2-Benzenesulfonylamino-3-(6-chloro-7-methoxy-1H-indazol-4-yl)-N-(4-phenyl-butyl)-propionamide (0.10 g, 0.19 mmol) and pyridinium hydrochloride (ca. 0.7 g) are combined in a 2 mL pressure vial. The reaction is heated to obtain a melt (ca. 170° C. bath). After 50 min. the reaction is cooled and partitioned between EtOAc ...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccccc1.c1ccc2[nH]ncc2c1.c1ccccc1
Other
null
null
null
COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12>>O=C(NCCCCc1ccccc1)C(Cc1cc(Cl)c(O)c2[nH]ncc12)NS(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dac15edfccee490a90f39607a30309f9
COC(=O)CBr.O=C(NCCCCc1ccccc1)C(Cc1cc(Cl)c(O)c2[nH]ncc12)NS(=O)(=O)c1ccccc1>>O=C(O)COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
C(=O)([O-])[O-].[K+].[K+].C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=NNC2=C(C(=C1)Cl)O.BrCC(=O)OC>>C1(=CC=CC=C1)S(=O)(=O)NC(CC1=C2C=NNC2=C(C(=C1)Cl)OCC(=O)O)C(NCCCCC1=CC=CC=C1)=O
C[O:3][C:2](=[O:1])[CH2:4]Br.[OH:5][c:6]1[c:7]([Cl:8])[cH:9][c:10]([CH2:11][CH:12]([NH:13][S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[C:23](=[O:24])[NH:25][CH2:26][CH2:27][CH2:28][CH2:29][c:30]2[cH:31][cH:32][cH:33][cH:34][cH:35]2)[c:36]2[cH:37][n:38][nH:39][c:40]12>>[O:1]=[C:2]([OH:3])[CH2:4][...
COC(=O)CBr.O=C(NCCCCc1ccccc1)C(Cc1cc(Cl)c(O)c2[nH]ncc12)NS(=O)(=O)c1ccccc1
O=C(O)COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
null
null
CN(C)C=O.CCOC(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
c47049bacd28cc701f2e77df376a2fcefecd5392e081f9a62473cff265d23a8c
017337a0828c32d10d28543003ae15a8b492b5e2f69019c65a4461eabc617d95
O=C(NCCCCc1ccccc1)C(Cc1cccc2[nH]ncc12)NS(=O)(=O)c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[O;H0;D2;+0:4]-C.[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]1:[#7;a:9]:[#7;a:10]:[c:11]:[c:12]:1>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:4])-[CH2;D2;+0:1]-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8]1:[#7;a:9]:[#7;a:10]:[c:11]:[c:12]:1
null
[]
null
null
36
HOUR
2-Benzenesulfonylamino-3-(6-chloro-7-hydroxy-1H-indazol-4-yl)-N-(4-phenyl-butyl)-propionamide (30 mg, 0.057 mmol) is dissolved in DMF (1 mL) and K2CO3 is added followed by a slight excess of methyl bromoacetate (11 mg, 0.072 mmol). The reaction is allowed to stir for 36 h. The reaction is worked-up by diluting with EtO...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Aromatic alcohol
Carboxylic acid.Ether
null
null
c1ccccc1.c1ccccc1.c1ccc2n[nH]cc2c1
HBr
CN(C)C=O.CCOC(=O)C
null
36
COC(=O)CBr.O=C(NCCCCc1ccccc1)C(Cc1cc(Cl)c(O)c2[nH]ncc12)NS(=O)(=O)c1ccccc1>CN(C)C=O.CCOC(=O)C>O=C(O)COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-07c91a5812cd47a1a871308ec1152428
O=C(O)COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12>>O=C(O)COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
C1(=CC=CC=C1)S(=O)(=O)NC(CC1=C2C=NNC2=C(C(=C1)Cl)OCC(=O)O)C(NCCCCC1=CC=CC=C1)=O>>C1(=CC=CC=C1)S(=O)(=O)NC(CC1=C2C=NNC2=C(C=C1)OCC(=O)O)C(NCCCCC1=CC=CC=C1)=O
Cl[c:7]1[c:6]([O:5][CH2:4][C:2](=[O:1])[OH:3])[c:39]2[c:35]([c:9]([CH2:10][CH:11]([NH:12][S:13](=[O:14])(=[O:15])[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[C:22](=[O:23])[NH:24][CH2:25][CH2:26][CH2:27][CH2:28][c:29]3[cH:30][cH:31][cH:32][cH:33][cH:34]3)[cH:8]1)[cH:36][n:37][nH:38]2>>[O:1]=[C:2]([OH:3])[CH2:4][O:5][c:...
O=C(O)COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
O=C(O)COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
null
[Pd]
CO
Functional Group Interconversion
Aromatic dehalogenation
5b5272366f02afef2e4988c85e194014363ac9ecbefdea542e560764e740c539
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
O=C(NCCCCc1ccccc1)C(Cc1cccc2[nH]ncc12)NS(=O)(=O)c1ccccc1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]2:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:2:[c:9]:1-[#8:10]>>[#8:10]-[c:9]1:[cH;D2;+0:1]:[c:2]:[c:3]:[c:4]2:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:2:1
null
[]
null
null
null
null
{4-[2-Benzenesulfonylamino-2-(4-phenyl-butylcarbamoyl)-ethyl]-6-chloro-1H-indazol-7-yloxy}-acetic acid (8.0 mg, 0.014 mmol) is dissolved in MeOH (1.5 mL) and 10% Pd/C (5 mg) is added. The reaction is purged with N2 and then with H2. The reaction is rapidly stirred and monitored by HPLC until complete (approximately 30 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1
c1ccccc1.c1ccccc1.c1ccc2n[nH]cc2c1
Other
[Pd].CO
null
null
O=C(O)COc1c(Cl)cc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12>[Pd].CO>O=C(O)COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cn[nH]c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dcdc731f2cc84ee29c862d4a72fe44ae
COC(=O)c1ccc(OC)c2c1ccn2S(=O)(=O)c1ccccc1>>COc1ccc(CO)c2ccn(S(=O)(=O)c3ccccc3)c12
[H-].C(C(C)C)[Al+]CC(C)C.COC(=O)C=1C=2C=CN(C2C(=CC1)OC)S(=O)(=O)C1=CC=CC=C1>>C1(=CC=CC=C1)S(=O)(=O)N1C=CC2=C(C=CC(=C12)OC)CO
CO[C:7]([c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[c:22]2[c:9]1[cH:10][cH:11][n:12]2[S:13](=[O:14])(=[O:15])[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1)=[O:8]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][OH:8])[c:9]2[cH:10][cH:11][n:12]([S:13](=[O:14])(=[O:15])[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[c:22]12
COC(=O)c1ccc(OC)c2c1ccn2S(=O)(=O)c1ccccc1
COc1ccc(CO)c2ccn(S(=O)(=O)c3ccccc3)c12
null
null
[C@@H]([C@H](C(=O)[O-])O)(C(=O)[O-])O.[Na+].[K+].C(Cl)Cl
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
O=S(=O)(c1ccccc1)n1ccc2ccccc21
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]:[c:6]:[#7;a:7]>>[#7;a:7]:[c:6]:[c:5]:[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:4]
null
[]
null
null
1
HOUR
Diisobutylaluminum hydride (1.5 M toluene, 1.4 mL, 2.1 mmol) is added dropwise to a −78° C. solution of 1-benzenesulfonyl-7-methoxy-1H-indole-4-carboxylic acid methyl ester (0.34 g, 0.98 mmol, Santangelo, et. al., Synth. Commun. 1993, 23, 2717–2725) in CH2Cl2 (7 mL). After stirring for 1 h, the solution is diluted with...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1cccc2[nH]ccc12.c1ccccc1
Other
[C@@H]([C@H](C(=O)[O-])O)(C(=O)[O-])O.[Na+].[K+].C(Cl)Cl
null
1
COC(=O)c1ccc(OC)c2c1ccn2S(=O)(=O)c1ccccc1>[C@@H]([C@H](C(=O)[O-])O)(C(=O)[O-])O.[Na+].[K+].C(Cl)Cl>COc1ccc(CO)c2ccn(S(=O)(=O)c3ccccc3)c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-abb7f6e090d74c539d90ada5554ca473
COc1ccc(CC(N)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12.O=S(=O)(Cl)c1ccccc1>>COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12
CCN(C(C)C)C(C)C.[Cl-].NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=CN(C2=C(C=C1)OC)S(=O)(=O)C1=CC=CC=C1.C1(=CC=CC=C1)S(=O)(=O)Cl>>C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=CN(C2=C(C=C1)OC)S(=O)(=O)C1=CC=CC=C1
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][CH:8]([NH2:9])[C:19](=[O:20])[NH:21][CH2:22][CH2:23][CH2:24][CH2:25][c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[c:32]2[cH:33][cH:34][n:35]([S:36](=[O:37])(=[O:38])[c:39]3[cH:40][cH:41][cH:42][cH:43][cH:44]3)[c:45]12.Cl[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][cH:16][cH:1...
COc1ccc(CC(N)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12.O=S(=O)(Cl)c1ccccc1
COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12
null
null
CCOCC.C(Cl)Cl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C(NCCCCc1ccccc1)C(Cc1cccc2c1ccn2S(=O)(=O)c1ccccc1)NS(=O)(=O)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[#7:8]-[C:9](=[O;D1;H0:10])-[C:11](-[C:12])-[NH2;D1;+0:13]>>[C:7]-[#7:8]-[C:9](=[O;D1;H0:10])-[C:11](-[C:12])-[NH;D2;+0:13]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
null
[]
0
CELSIUS
2
HOUR
Hunig's base (2.1 g, 16 mmol) is added to a suspension of 2-amino-3-(1-benzenesulfonyl-7-methoxy-1H-indol-4-yl)-N-(4-phenyl-butyl)-propionamide, hydrogen chloride salt (3.0 g, 5.6 mmol) in CH2Cl2. The resulting solution is cooled to 0° C. and benzenesulfonyl chloride (1.2 g, 6.9 mmol) is added. After being warmed to rt...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccccc1.c1cccc2[nH]ccc12.c1ccccc1
HCl
CCOCC.C(Cl)Cl
0
2
COc1ccc(CC(N)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12.O=S(=O)(Cl)c1ccccc1>CCOCC.C(Cl)Cl>COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6fff82d4d9424ce1bcf30b2a374197da
COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12>>COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cc[nH]c12
C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=CN(C2=C(C=C1)OC)S(=O)(=O)C1=CC=CC=C1.[OH-].[K+].[NH4+].[Cl-]>>C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=CNC2=C(C=C1)OC
O=S(=O)(c1ccccc1)[n:35]1[cH:34][cH:33][c:32]2[c:6]([CH2:7][CH:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]3[cH:14][cH:15][cH:16][cH:17][cH:18]3)[C:19](=[O:20])[NH:21][CH2:22][CH2:23][CH2:24][CH2:25][c:26]3[cH:27][cH:28][cH:29][cH:30][cH:31]3)[cH:5][cH:4][c:3]([O:2][CH3:1])[c:36]21>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7...
COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12
COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cc[nH]c12
null
null
CO
Reduction
OtherReaction
706bab53972d8bd3783a9b076a1c50a9aa5a0e0970c926686a27ee7263dbdbaf
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
O=C(NCCCCc1ccccc1)C(Cc1cccc2[nH]ccc12)NS(=O)(=O)c1ccccc1
O=S(=O)(-[n;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[c:5]:1:[c:6])-c1:c:c:c:c:c:1>>[c:6]:[c:5]1:[c:4]:[c:3]:[c:2]:[nH;D2;+0:1]:1
null
[]
null
null
null
null
A mixture of 2-benzenesulfonylamino-3-(1-benzenesulfonyl-7-methoxy-1H-indol-4-yl)-N-(4-phenyl-butyl)-propionamide (1.0 g, 1.6 mmol) and 2.5 M KOH (2.0 mL, 5.0 mmol) is refluxed in MeOH (9 mL) for 22 h. The resulting solution is poured into a saturated NH4Cl solution and extracted twice with EtOAc. The organics are drie...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccccc1.c1cccc2[nH]ccc12
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1
HO-
CO
null
null
COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2ccn(S(=O)(=O)c3ccccc3)c12>CO>COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cc[nH]c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1983935f784b4f378a92c5cece0120c6
CCS.CCS.COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cc[nH]c12.[NH4+]>>O=C(CNS(=O)(=O)c1ccccc1)NCCC(Cc1ccccc1)c1ccc(O)c2[nH]ccc12.O=C(NCCCCc1ccccc1)C(Cc1ccc(O)c2[nH]ccc12)NS(=O)(=O)c1ccccc1
[NH4+].[Cl-].[Al+3].[Cl-].[Cl-].[Cl-].CCS.[Cl-].[Al+3].[Cl-].[Cl-].C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=CNC2=C(C=C1)OC.CCS>>C1(=CC=CC=C1)S(=O)(=O)NCC(=O)NCCC(CC1=CC=CC=C1)C1=C2C=CNC2=C(C=C1)O.C1(=CC=CC=C1)S(=O)(=O)NC(C(=O)NCCCCC1=CC=CC=C1)CC1=C2C=CNC2=C(C=C1)O
S[CH2:69][CH3:2].[CH3:52][CH2:53][SH:61].[O:1]=[S:5]([NH:4][CH:3]([C:36](=[O:35])[NH:37][CH2:38][CH2:39][CH2:40][CH2:41][c:42]1[cH:43][cH:44][cH:67][cH:46][cH:47]1)[CH2:49][c:50]1[cH:51][cH:27][c:28]([O:29][CH3:30])[c:55]2[nH:56][cH:57][cH:58][c:59]12)(=[O:6])[c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1.[NH4+:14]>>[O:1]=[...
CCS.CCS.COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cc[nH]c12.[NH4+]
O=C(CNS(=O)(=O)c1ccccc1)NCCC(Cc1ccccc1)c1ccc(O)c2[nH]ccc12.O=C(NCCCCc1ccccc1)C(Cc1ccc(O)c2[nH]ccc12)NS(=O)(=O)c1ccccc1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
567b2db691f6ce3fb6b04d1424187c27634f6d754d36d9131d981ba9e97e8fd8
5226fb5d9ca42e1d50c8eb885034d36c77e02fc537477bcb9240e41162aeaea2
O=C(CNS(=O)(=O)c1ccccc1)NCCC(Cc1ccccc1)c1cccc2[nH]ccc12.O=C(NCCCCc1ccccc1)C(Cc1cccc2[nH]ccc12)NS(=O)(=O)c1ccccc1
S-[CH2;D2;+0:1]-[CH3;D1;+0:2].[CH3;D1;+0:3]-[CH2;D2;+0:4]-[SH;D1;+0:5].[C:6]-[#7:7]-[C;H0;D3;+0:8](=[O;D1;H0:9])-[CH;D3;+0:10](-[#7:11]-[S;H0;D4;+0:12](=[O;D1;H0:13])(=[O;H0;D1;+0:14])-[c:15](:[c:16]):[c:17])-[CH2;D2;+0:18]-[c:19]1:[cH;D2;+0:20]:[cH;D2;+0:21]:[c;H0;D3;+0:22](-[O;H0;D2;+0:23]-[CH3;D1;+0:24]):[c;H0;D3;+0...
null
[]
null
null
3.5
HOUR
Aluminum chloride (0.13 g, 0.99 mmol) is added to a 0° C. solution of 2-benzenesulfonylamino-3-(7-methoxy-1H-indol-4-yl)-N-(4-phenyl-butyl)-propionamide (0.12 g, 0.25 mmol) and EtSH (0.061 g, 0.99 mmol). The mixture is stirred 3.5 h while being allowed to warm to rt. Additional AlCl3 (0.13 g, 0.99 mmol) and EtSH (0.061...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Ether.Secondary amide.Aliphatic thiol.Aliphatic thiol
Sulfonamide.Sulfonamide.Secondary amide.Secondary amide.Aromatic alcohol.Aromatic alcohol
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
null
null
null
3.5
CCS.CCS.COc1ccc(CC(NS(=O)(=O)c2ccccc2)C(=O)NCCCCc2ccccc2)c2cc[nH]c12.[NH4+]>>O=C(CNS(=O)(=O)c1ccccc1)NCCC(Cc1ccccc1)c1ccc(O)c2[nH]ccc12.O=C(NCCCCc1ccccc1)C(Cc1ccc(O)c2[nH]ccc12)NS(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-403720b4bef8437f92fc3e9aee7e95fe
CC(C)(C)OC(=O)NCC(=O)O.NCCCCc1ccccc1>>CC(C)(C)OC(=O)NCC(=O)NCCCCc1ccccc1
C1(=CC=CC=C1)CCCCN.N(CC(=O)O)C(=O)OC(C)(C)C>>C(C)(C)(C)OC(NCC(NCCCCC1=CC=CC=C1)=O)=O
O[C:10]([CH2:9][NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])=[O:11].[NH2:12][CH2:13][CH2:14][CH2:15][CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][CH2:9][C:10](=[O:11])[NH:12][CH2:13][CH2:14][CH2:15][CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]...
CC(C)(C)OC(=O)NCC(=O)O.NCCCCc1ccccc1
CC(C)(C)OC(=O)NCC(=O)NCCCCc1ccccc1
null
null
O1CCOCC1.C(Cl)Cl.C(=O)([O-])[O-].[K+].[K+]
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4]-[C:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11].[C:12]-[C:13]-[NH2;D1;+0:14]>>[C:12]-[C:13]-[NH;D2;+0:14]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4]-[C:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11]
null
[]
null
null
16
HOUR
Phenylbutylamine (8.2 g, 52 mmol) is added to a mixture of BOC-Gly-PNB (14.82 g, 50 mmol) in dioxane (60 mL) and 1 M K2CO3 (60 mL). The mixture is stirred 16 h and then diluted with CH2Cl2 and washed with a saturated NaHCO3 solution until the organic phase is colorless. The organics are dried (MgSO4) and concentrated t...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1
HO-
O1CCOCC1.C(Cl)Cl.C(=O)([O-])[O-].[K+].[K+]
null
16
CC(C)(C)OC(=O)NCC(=O)O.NCCCCc1ccccc1>O1CCOCC1.C(Cl)Cl.C(=O)([O-])[O-].[K+].[K+]>CC(C)(C)OC(=O)NCC(=O)NCCCCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7c03b28059c94baea3e7e6a4addbc311
CC(C)(C)OC(=O)NCC(=O)NCCCCc1ccccc1.Cl>>NCC(=O)NCCCCc1ccccc1.[Cl-]
C(C)(C)(C)OC(NCC(NCCCCC1=CC=CC=C1)=O)=O.Cl>>[Cl-].NCC(=O)NCCCCC1=CC=CC=C1
CC(C)(C)OC(=O)[NH:1][CH2:2][C:3](=[O:4])[NH:5][CH2:6][CH2:7][CH2:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1.[ClH:16]>>[NH2:1][CH2:2][C:3](=[O:4])[NH:5][CH2:6][CH2:7][CH2:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1.[Cl-:16]
CC(C)(C)OC(=O)NCC(=O)NCCCCc1ccccc1.Cl
NCC(=O)NCCCCc1ccccc1.[Cl-]
null
null
O1CCOCC1
Miscellaneous
OtherReaction
4812e39fa209f57a5a2564677791e5e37790c829f5742d8c7df33806c5ba4ce0
d7ecc2e7a68b8c20d378ac6004c3fdfc3efd09bbbd9efd577186f69427135737
c1ccccc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]-[C:3](=[O;D1;H0:4])-[#7:5]-[C:6].[ClH;D0;+0:7]>>[C:6]-[#7:5]-[C:3](=[O;D1;H0:4])-[C:2]-[NH2;D1;+0:1].[Cl-;H0;D0:7]
null
[]
null
null
null
null
The crude [(4-phenyl-butylcarbamoyl)-methyl]-carbamic acid tert-butyl ester is stirred in a solution of dioxane (150 mL) and HCl (4 M dioxane, 42 mL, 168 mmol) for 17 h. The volatiles are removed in vacuo to provide 2-amino-N-(4-phenyl-butyl)-acetamide, hydrogen chloride salt which is used as is without further purific...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccccc1
HO-
O1CCOCC1
null
null
CC(C)(C)OC(=O)NCC(=O)NCCCCc1ccccc1.Cl>O1CCOCC1>NCC(=O)NCCCCc1ccccc1.[Cl-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0425835e9f904429b2a1ada31b068d43
N=C(c1ccccc1)c1ccccc1.NCC(=O)NCCCCc1ccccc1>>O=C(CN=C(c1ccccc1)c1ccccc1)NCCCCc1ccccc1
Cl.NCC(=O)NCCCCC1=CC=CC=C1.C(C1=CC=CC=C1)(C1=CC=CC=C1)=N>>C1(=CC=CC=C1)C(C1=CC=CC=C1)=NCC(=O)NCCCCC1=CC=CC=C1
N=[C:5]([c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1)[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1.[O:1]=[C:2]([CH2:3][NH2:4])[NH:18][CH2:19][CH2:20][CH2:21][CH2:22][c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1>>[O:1]=[C:2]([CH2:3][N:4]=[C:5]([c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1)[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)[N...
N=C(c1ccccc1)c1ccccc1.NCC(=O)NCCCCc1ccccc1
O=C(CN=C(c1ccccc1)c1ccccc1)NCCCCc1ccccc1
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
5c2ecd1abe923724cb27d21ac6e885dd316245a236b29970f80eae667c9e6294
d626c897c8bd63d92b2ec938ee0af3ccbc3842d02f981457c923654bacf119df
O=C(CN=C(c1ccccc1)c1ccccc1)NCCCCc1ccccc1
N=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7].[C:8]-[#7:9]-[C:10](=[O;D1;H0:11])-[C:12]-[NH2;D1;+0:13]>>[C:8]-[#7:9]-[C:10](=[O;D1;H0:11])-[C:12]-[N;H0;D2;+0:13]=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7]
null
[]
null
null
null
null
2-Amino-N-(4-phenyl-butyl)-acetamide-hydrogen chloride salt is stirred with benzophenone imine (12.6 mL, 75 mmol) in CH2Cl2 (200 mL) for 24 h. The organics are then washed with water, dried (MgSO4), and concentrated to provide 2-(diphenylmethylenamino)-N-(4-phenyl-butyl)-acetamide (7) as a white solid which is used wit...
10.6084/m9.figshare.5104873.v1
null
Unsubstituted imine.Primary amine
Substituted imine
null
null
c1ccccc1.c1ccccc1.c1ccccc1
Other
C(Cl)Cl
null
null
N=C(c1ccccc1)c1ccccc1.NCC(=O)NCCCCc1ccccc1>C(Cl)Cl>O=C(CN=C(c1ccccc1)c1ccccc1)NCCCCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cc46d3f3c2e348ed877fbffad0cbf5b4
Brc1ccccc1.O=C1CCC(=O)O1>>O=C(O)CCC(=O)c1ccc(Br)cc1
[Al+3].[Cl-].[Cl-].[Cl-].C1(CCC(=O)O1)=O.BrC1=CC=CC=C1.Cl>>BrC1=CC=C(C=C1)C(CCC(=O)O)=O
[cH:8]1[cH:9][cH:10][c:11]([Br:12])[cH:13][cH:14]1.[O:1]=[C:2]1[O:3][C:6](=[O:7])[CH2:5][CH2:4]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][C:6](=[O:7])[c:8]1[cH:9][cH:10][c:11]([Br:12])[cH:13][cH:14]1
Brc1ccccc1.O=C1CCC(=O)O1
O=C(O)CCC(=O)c1ccc(Br)cc1
null
null
C(Cl)Cl
C-C Coupling
OtherReaction
95de0079bfd4d0e2b70eac1863ad8bac063c1a1557f674f5eb3c0cde67534555
4836357c99dfeeac9d5083fedc379181a858ae45ac77bd85eb46e7e1a9df36f0
c1ccccc1
[O;D1;H0:1]=[C:2]1-[C:3]-[C:4]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[O;H0;D2;+0:7]-1.[c:8]:[c:9]:[cH;D2;+0:10]:[c:11]:[c:12]>>[O;D1;H0:1]=[C:2](-[OH;D1;+0:7])-[C:3]-[C:4]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:9]:[c:8]
76.4
[{"value": 76.4, "product": "BrC1=CC=C(C=C1)C(CCC(=O)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
AlCl3 (128.8 g, 0.97 mol) was added by portions within 20 min to a suspension of succinic anhydride (44.3 g, 0.44 mol) and bromobenzene (100 ml, 0.99 mol) in DCM (500 ml) while the reaction flask was cooled in a water bath. After 1 h 30 min at RT, the reaction mixture was refluxed for 2 h. After cooling, the reaction m...
10.6084/m9.figshare.5104873.v1
null
Anhydride
Carboxylic acid.Ketone
c1ccccc1.C1CCOC1
c1ccccc1
c1ccccc1
null
C(Cl)Cl
null
0.5
Brc1ccccc1.O=C1CCC(=O)O1>C(Cl)Cl>O=C(O)CCC(=O)c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-59f9547cfdad422da5017d291877cbf6
CO.O=C(O)CCC(=O)c1ccc(Br)cc1>>COC(=O)CCC(=O)c1ccc(Br)cc1
BrC1=CC=C(C=C1)C(CCC(=O)O)=O.OS(=O)(=O)O.CO>>COC(CCC(=O)C1=CC=C(C=C1)Br)=O
[CH3:1][OH:2].O[C:3](=[O:4])[CH2:5][CH2:6][C:7](=[O:8])[c:9]1[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][C:7](=[O:8])[c:9]1[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]1
CO.O=C(O)CCC(=O)c1ccc(Br)cc1
COC(=O)CCC(=O)c1ccc(Br)cc1
null
null
null
Protection
Esterification of Carboxylic Acids
9cecdbd189c6f9c3648521d17154d013842a5498de4e76e65efb1d842973340b
af0b8064f2e82ebe66c4c29d2391785ac1b993104265ccdc4d67ca79e36fa3c8
c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]-[C:5]=[O;D1;H0:6].[C;D1;H3:7]-[OH;D1;+0:8]>>[C;D1;H3:7]-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]-[C:5]=[O;D1;H0:6]
null
[]
null
null
null
null
4-(4-Bromophenyl)-4-oxobutyric acid (86.4 g, 0.336 mol) (Preparation 1) in MeOH (1.7 l) containing H2SO4 (86 ml) was refluxed for 21 h. After cooling, the light precipitate was filtered off and the reaction mixture concentrated to dryness. The obtained solid was placed in water and extracted twice with EtOAc. The organ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Methanol
Ester
null
null
c1ccccc1
HO-
null
null
null
CO.O=C(O)CCC(=O)c1ccc(Br)cc1>>COC(=O)CCC(=O)c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0c37282cc8b64bfaa39e6296202f8b8f
Brc1ccccc1.O=C(Cl)CCBr>>O=C(CCBr)c1ccc(Br)cc1
[Al+3].[Cl-].[Cl-].[Cl-].BrC1=CC=CC=C1.BrCCC(=O)Cl>>BrCCC(=O)C1=CC=C(C=C1)Br
[cH:6]1[cH:7][cH:8][c:9]([Br:10])[cH:11][cH:12]1.Cl[C:2](=[O:1])[CH2:3][CH2:4][Br:5]>>[O:1]=[C:2]([CH2:3][CH2:4][Br:5])[c:6]1[cH:7][cH:8][c:9]([Br:10])[cH:11][cH:12]1
Brc1ccccc1.O=C(Cl)CCBr
O=C(CCBr)c1ccc(Br)cc1
null
null
null
C-C Coupling
Friedel-Crafts acylation
55541449ad4f182ef3dc0497085b282b1dcb76e0fb5ed140dc4eab4973eacb28
fe2a4a0dfbb5b71b9a065e092364c64b22b4eb1ad4d6ba2a1e8edc9d31fce3e4
c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[c:5]:[c:6]:[cH;D2;+0:7]:[c:8]:[c:9]>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c;H0;D3;+0:7](:[c:6]:[c:5]):[c:8]:[c:9]
84.5
[{"value": 84.5, "product": "BrCCC(=O)C1=CC=C(C=C1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
30
MINUTE
AlCl3 (23.8 g, 178 mmol) was added by portions to bromobenzene (155 ml, 1.47 mol) at 0° C. 3-Bromopropionyl chloride (25 g, 146 mmol) was added dropwise to the red solution kept at 0° C. over 30 min. After 1 h at RT, the reaction mixture was heated to 50° C. for 1 h. After cooling, the mixture was poured over ice/water...
10.6084/m9.figshare.5104873.v1
null
Acyl halide
Ketone
c1ccccc1
c1ccccc1
c1ccccc1
HCl
null
50
0.5
Brc1ccccc1.O=C(Cl)CCBr>>O=C(CCBr)c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cf1a9a59f9ca487388bf4e396618b9aa
O=C(CCBr)c1ccc(Br)cc1>>OC(CCBr)c1ccc(Br)cc1
[BH4-].[Na+].BrCCC(=O)C1=CC=C(C=C1)Br.Cl>>BrCCC(O)C1=CC=C(C=C1)Br
[O:1]=[C:2]([CH2:3][CH2:4][Br:5])[c:6]1[cH:7][cH:8][c:9]([Br:10])[cH:11][cH:12]1>>[OH:1][CH:2]([CH2:3][CH2:4][Br:5])[c:6]1[cH:7][cH:8][c:9]([Br:10])[cH:11][cH:12]1
O=C(CCBr)c1ccc(Br)cc1
OC(CCBr)c1ccc(Br)cc1
null
null
CO
Reduction
Reduction of ketone to secondary alcohol
02790ac194d8bf7ccb13d6247c59412024d87f77d2c906ef7804f021f57d5070
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1ccccc1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[c:5](:[c:6]):[c:7]>>[C:1]-[C:2]-[CH;D3;+0:3](-[OH;D1;+0:4])-[c:5](:[c:6]):[c:7]
94.4
[{"value": 94.4, "product": "BrCCC(O)C1=CC=C(C=C1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
NaBH4 (1.5 g, 39.7 mmol) was added by portions to a solution of 3-bromo-1-(4-bromophenyl)propan-1-one (11.7 g, 40 mmol) (Preparation 5) in MeOH while keeping the temperature below 10° C. After 1 h at RT, 1N aqueous hydrochloric acid was added at 5° C. to pH=1 and the mixture was concentrated in vacuum. The residue was ...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
null
null
c1ccccc1
null
CO
null
1
O=C(CCBr)c1ccc(Br)cc1>CO>OC(CCBr)c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-31b9b3e14509464ea943b6c60dbf1524
CCOC(=O)CN.S=C=Nc1cc(Cl)cc(Cl)c1>>O=C1CNC(=S)N1c1cc(Cl)cc(Cl)c1
ClC=1C=C(C=C(C1)Cl)N=C=S.Cl.NCC(=O)OCC>>ClC=1C=C(C=C(C1)Cl)N1C(NCC1=O)=S
CCO[C:2](=[O:1])[CH2:3][NH2:4].[C:5](=[S:6])=[N:7][c:8]1[cH:9][c:10]([Cl:11])[cH:12][c:13]([Cl:14])[cH:15]1>>[O:1]=[C:2]1[CH2:3][NH:4][C:5](=[S:6])[N:7]1[c:8]1[cH:9][c:10]([Cl:11])[cH:12][c:13]([Cl:14])[cH:15]1
CCOC(=O)CN.S=C=Nc1cc(Cl)cc(Cl)c1
O=C1CNC(=S)N1c1cc(Cl)cc(Cl)c1
null
null
C(Cl)Cl
Acylation
OtherReaction
661d52a20ffc4dc07f0b42d6e71f02d6f2df62b907a8af0280f593fa5e8af5d9
1f7b20b438a0e6db92fae47a6dad1d97dbcb6314195567f1c56db0099cef8267
O=C1CNC(=S)N1c1ccccc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[NH2;D1;+0:4].[S;D1;H0:5]=[C;H0;D2;+0:6]=[N;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:3]-[NH;D2;+0:4]-[C;H0;D3;+0:6](=[S;D1;H0:5])-[N;H0;D3;+0:7]-1-[c:8](:[c:9]):[c:10]
82.8
[{"value": 82.8, "product": "ClC=1C=C(C=C(C1)Cl)N1C(NCC1=O)=S", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
60
HOUR
3,5-Dichlorophenylisothiocyanate (5 g, 24.5 mmol) was added by portion to a suspension of the HCl salt of ethyl glycinate (3.4 g, 24.5 mmol) in a mixture of TEA (7.5 ml, 53.9 mmol) and dry DCM (40 ml) while cooling the flask in a water bath. After 60 h at RT, the solution was concentrated to dryness and partitioned bet...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine.Isothiocyanate
Thiourea.Tertiary amide
null
C1CNC[NH]1
C1CNC[NH]1.c1ccccc1
HO-
C(Cl)Cl
null
60
CCOC(=O)CN.S=C=Nc1cc(Cl)cc(Cl)c1>C(Cl)Cl>O=C1CNC(=S)N1c1cc(Cl)cc(Cl)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a0f6abd673fe44b59f2198c705e4c686
BrCCCC(Br)c1ccc(Br)cc1.CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=S>>CC(C)(C)OC(=O)N1C(=S)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
BrC1=CC=C(C=C1)C(CCCBr)Br.C(C)(C)(C)OC(=O)N1C(N(C(C1)=O)C1=CC(=CC(=C1)Cl)Cl)=S>>C(C)(C)(C)OC(=O)N1C(N(C([C@@]12[C@@H](CCC2)C2=CC=C(C=C2)Br)=O)C2=CC(=CC(=C2)Cl)Cl)=S
Br[CH2:23][CH2:24][CH2:25][CH:26](Br)[c:27]1[cH:28][cH:29][c:30]([Br:31])[cH:32][cH:33]1.[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[C:9](=[S:10])[N:11]([c:12]2[cH:13][c:14]([Cl:15])[cH:16][c:17]([Cl:18])[cH:19]2)[C:20](=[O:21])[CH2:22]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[C:9](=[S:10])[N...
BrCCCC(Br)c1ccc(Br)cc1.CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=S
CC(C)(C)OC(=O)N1C(=S)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
null
null
null
C-C Coupling
OtherReaction
f7705fcc55562dd1d514d37592f3026f1b985aed97988cbab983ce3221a43656
d4cf29bb0f2586f258c9eb5d3edb710b86094a4be60be4638a5468606055dcb5
O=C1N(c2ccccc2)C(=S)N[C@@]12CCC[C@H]2c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3]-[CH;D3;+0:4](-Br)-[c:5](:[c:6]):[c:7].[C;D1;H3:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[#8:12]-[C:13](=[O;D1;H0:14])-[#7:15]1-[CH2;D2;+0:16]-[C:17](=[O;D1;H0:18])-[#7:19](-[c:20])-[C:21]-1=[S;D1;H0:22]>>[C;D1;H3:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[#8:12]-[C:13](=[O;D1;H0:14])-[#7:15]1-[C...
null
[]
null
null
null
null
Using the same procedure as in Example 1 starting from 1-bromo-4-(1,4-dibromobutyl)benzene (423 mg, 1.1 mmol) (Preparation 4) and 3-(3,5-dichlorophenyl)-4-oxo-2-thioxoimidazolidine-1-carboxylic acid tert-butyl ester (361 mg, 1 mmol) (Preparation 9), (5R*,6S*)-6-(4-bromophenyl)-3-(3,5-dichlorophenyl)-4-oxo-2-thioxo-1,3-...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Primary halide
null
C1C[NH]C[NH]1
C1CCC2(C1)C[NH]C[NH]2
c1ccccc1.C1CCC2(C1)C[NH]C[NH]2.c1ccccc1
HBr
null
null
null
BrCCCC(Br)c1ccc(Br)cc1.CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=S>>CC(C)(C)OC(=O)N1C(=S)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c24b3f2993e946fcbda0dfb1310bbbb5
CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O.N#Cc1ccc(C=O)cc1>>CC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)/C1=C\c1ccc(C#N)cc1
C(C)(C)(C)OC(=O)N1C(N(C(C1)=O)C1=CC(=CC(=C1)Cl)Cl)=O.C(#N)C1=CC=C(C=O)C=C1.CC(=O)[O-].[Na+]>>C(C)(=O)N\1C(N(C(/C1=C\C1=CC=C(C#N)C=C1)=O)C1=CC(=CC(=C1)Cl)Cl)=O
CC(C)(C)OC(=O)[N:4]1[C:5](=[O:6])[N:7]([c:8]2[cH:9][c:10]([Cl:11])[cH:12][c:13]([Cl:14])[cH:15]2)[C:16](=[O:17])[CH2:18]1.O=[CH:19][c:20]1[cH:21][cH:22][c:23]([C:24]#[N:25])[cH:26][cH:27]1>>[CH3:1][C:2](=[O:3])[N:4]1[C:5](=[O:6])[N:7]([c:8]2[cH:9][c:10]([Cl:11])[cH:12][c:13]([Cl:14])[cH:15]2)[C:16](=[O:17])/[C:18]1=[CH...
CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O.N#Cc1ccc(C=O)cc1
CC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)/C1=C\c1ccc(C#N)cc1
null
null
CC(=O)OC(=O)C
Acylation
OtherReaction
c63cff6908ead9259865a72c3c86780707b1a88e0885e2beb31b19780f7a532b
84427fcabd93888189c50bbfb7aecd65f7823243b9794dda39c8490a956075b6
O=C1N/C(=C/c2ccccc2)C(=O)N1c1ccccc1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[#7:5](-[c:6])-[C:7]-1=[O;D1;H0:8].O=[CH;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[C;D1;H3:13]-[C:14](=[O;D1;H0:15])-[N;H0;D3;+0:1]1-[C:7](=[O;D1;H0:8])-[#7:5](-[c:6])-[C:3](=[O;D1;H0:4])/[C;H0;D3;+0:2]-1=[CH;D2;+0:9]\[c:10](:[c:11]):[c:12]
109.9
[{"value": 109.9, "product": "C(C)(=O)N\\1C(N(C(/C1=C\\C1=CC=C(C#N)C=C1)=O)C1=CC(=CC(=C1)Cl)Cl)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 3-(3,5-dichlorophenyl)-2,4-dioxoimidazolidine-1-carboxylic acid tert-butyl ester (3.45 g, 10 mmol) (Preparation 11), 4-cyanobenzaldehyde (1.31 g, 10 mmol) and NaOAc (0.82 g, 10 mmol) was refluxed for 3 h in Ac2O (50 ml). The solid obtained after concentration was taken into a mixture of ice/water and DCM. ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Carbamic ester.Ether.Urea.Substituted dicarboximide.Boc
Enamine.Urea.Substituted dicarboximide
C1C[NH]C[NH]1
C1C[NH]C[NH]1
C1C[NH]C[NH]1.c1ccccc1.c1ccccc1
HO-
CC(=O)OC(=O)C
null
null
CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O.N#Cc1ccc(C=O)cc1>CC(=O)OC(=O)C>CC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)/C1=C\c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a3b0ca61e6a744f0b37d526d63b480b5
CCOC(=O)CNC.O=C=Nc1cc(Cl)nc(Cl)c1>>CN1CC(=O)N(c2cc(Cl)nc(Cl)c2)C1=O
Cl.C(C)OC(CNC)=O.ClC1=NC(=CC(=C1)N=C=O)Cl>>ClC1=NC(=CC(=C1)N1C(N(CC1=O)C)=O)Cl
CCO[C:4]([CH2:3][NH:2][CH3:1])=[O:5].[N:6]([c:7]1[cH:8][c:9]([Cl:10])[n:11][c:12]([Cl:13])[cH:14]1)=[C:15]=[O:16]>>[CH3:1][N:2]1[CH2:3][C:4](=[O:5])[N:6]([c:7]2[cH:8][c:9]([Cl:10])[n:11][c:12]([Cl:13])[cH:14]2)[C:15]1=[O:16]
CCOC(=O)CNC.O=C=Nc1cc(Cl)nc(Cl)c1
CN1CC(=O)N(c2cc(Cl)nc(Cl)c2)C1=O
null
null
C(Cl)Cl
Acylation
OtherReaction
b625fb00e8984b3ab5a50595e831b3cf1c0e3d33ffe13b923a6e37bd004b081a
14fc722b35388e650c3f1c11183dfc37a5a1b84b5dc579a69d8278216faa51d7
O=C1CNC(=O)N1c1ccncc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[NH;D2;+0:4]-[C;D1;H3:5].[O;D1;H0:6]=[C;H0;D2;+0:7]=[N;H0;D2;+0:8]-[c:9]1:[c:10]:[c:11]:[#7;a:12]:[c:13]:[c:14]:1>>[C;D1;H3:5]-[N;H0;D3;+0:4]1-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:8](-[c:9]2:[c:10]:[c:11]:[#7;a:12]:[c:13]:[c:14]:2)-[C;H0;D3;+0:7]-1=[O;D1;H0:6]
155.4
[{"value": 155.4, "product": "ClC1=NC(=CC(=C1)N1C(N(CC1=O)C)=O)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
5
CELSIUS
96
HOUR
TEA (7.2 ml, 51 mmol) was added to a suspension of the HCl salt of sarcosine ethyl ester (3.4 g, 24.5 mmol) in dry DCM (80 ml). The formed triethylamine hydrochloride was filtered off and rinsed with DCM (20 ml). The filtrate was transferred into a 3-necked round bottom flask and cooled to 5° C. A solution of 2,6-dichl...
10.6084/m9.figshare.5104873.v1
null
Ester.Isocyanate.Secondary amine
Urea.Substituted dicarboximide
null
C1C[NH]C[NH]1
C1C[NH]C[NH]1.c1ccncc1
HO-
C(Cl)Cl
5
96
CCOC(=O)CNC.O=C=Nc1cc(Cl)nc(Cl)c1>C(Cl)Cl>CN1CC(=O)N(c2cc(Cl)nc(Cl)c2)C1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c368e0a839684f7b84c75961fa20ac31
CCOC(=O)c1csc(C)n1.O=C1CCC(=O)N1Br>>CCOC(=O)c1csc(CBr)n1
C(Cl)Cl.C(C)OC(=O)C=1N=C(SC1)C.BrN1C(CCC1=O)=O.C(C1=CC=CC=C1)(=O)OOC(C1=CC=CC=C1)=O>>BrCC=1SC=C(N1)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][s:8][c:9]([CH3:10])[n:12]1.O=C1CCC(=O)N1[Br:11]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][s:8][c:9]([CH2:10][Br:11])[n:12]1
CCOC(=O)c1csc(C)n1.O=C1CCC(=O)N1Br
CCOC(=O)c1csc(CBr)n1
null
null
ClCCCl
Functional Group Interconversion
Wohl-Ziegler bromination benzyl primary
45c0aca0d63a96f0092e6dded9c888827eaf6379dac179e1cefc99293896300a
08f5e7e34d3f321cce3e85421b38226d6240cca0939494ae61032d4f8405cf22
c1cscn1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[#7;a:6]:[c:7](-[CH3;D1;+0:8]):[#16;a:9]:[c:10]:1>>[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[#7;a:6]:[c:7](-[CH2;D2;+0:8]-[Br;H0;D1;+0:1]):[#16;a:9]:[c:10]:1
8
[{"value": 8.0, "product": "BrCC=1SC=C(N1)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
A mixture of ethyl-2-methylthiazole 4-carboxylate (500 mg, 2.9 mmol), N-bromosuccinimide (877 mg, 4.9 mmol), and benzoyl peroxide (5–10 mg) in 1,2-DCE (3 mL) was heated at 70° C. for 85 h. After cooling to room temperature, DCM (10 ml) was added and washed with water (3 times). The organic layer was dried over Na2SO4 a...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Primary halide
C1CCNC1
null
c1cscn1
HO-
ClCCCl
70
null
CCOC(=O)c1csc(C)n1.O=C1CCC(=O)N1Br>ClCCCl>CCOC(=O)c1csc(CBr)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4d73a3046c0e481b980eb7c2a6a7655d
CC(C)(C)OC(=O)c1ccc(O)cc1.O=S(=O)(OS(=O)(=O)C(F)(F)F)C(F)(F)F>>CC(C)(C)OC(=O)c1ccc(OS(=O)(=O)C(F)(F)F)cc1
O.FC(S(=O)(=O)OS(=O)(=O)C(F)(F)F)(F)F.OC1=CC=C(C(=O)OC(C)(C)C)C=C1>>C(C)(C)(C)OC(C1=CC=C(C=C1)OS(=O)(=O)C(F)(F)F)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[c:8]1[cH:9][cH:10][c:11]([OH:12])[cH:20][cH:21]1.O=S(=O)(O[S:13](=[O:14])(=[O:15])[C:16]([F:17])([F:18])[F:19])C(F)(F)F>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[c:8]1[cH:9][cH:10][c:11]([O:12][S:13](=[O:14])(=[O:15])[C:16]([F:17])([F:18])[F:19])[cH:20][cH:21]1
CC(C)(C)OC(=O)c1ccc(O)cc1.O=S(=O)(OS(=O)(=O)C(F)(F)F)C(F)(F)F
CC(C)(C)OC(=O)c1ccc(OS(=O)(=O)C(F)(F)F)cc1
null
null
C(Cl)Cl
Functional Group Interconversion
Alcohol to triflate conversion
934d625c86d5da305dd43240eee33b5e46f4d298c87ccdc218e9e2eb60c650b5
13e8f5cec02bd6a2d12ae535029c405c270682596231c5c8422ac50b2cb1ec74
c1ccccc1
F-C(-F)(-F)-S(=O)(=O)-O-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7].[OH;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[F;D1;H0:5]-[C:4](-[F;D1;H0:6])(-[F;D1;H0:7])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[O;H0;D2;+0:8]-[c:9](:[c:10]):[c:11]
87.1
[{"value": 87.1, "product": "C(C)(C)(C)OC(C1=CC=C(C=C1)OS(=O)(=O)C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
Trifluoromethanesulfonic anhydride (1.04 ml, 6.2 mmol) was added to a cooled (5° C.) solution of tert-butyl 4-hydroxybenzoate (1 g, 5.1 mmol) in a mixture of DCM (25 ml) and TEA (1.1 ml, 7.8 mmol). After 4 h at 5° C., water was added. The organic layer was separated, dried over MgSO4 and concentrated in vacuo. The resi...
10.6084/m9.figshare.5104873.v1
null
Triflate.Triflate.Aromatic alcohol
Triflate
null
null
c1ccccc1
HF
C(Cl)Cl
null
4
CC(C)(C)OC(=O)c1ccc(O)cc1.O=S(=O)(OS(=O)(=O)C(F)(F)F)C(F)(F)F>C(Cl)Cl>CC(C)(C)OC(=O)c1ccc(OS(=O)(=O)C(F)(F)F)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-05bc6480a1534adfa637df5896728945
Cc1ccccc1-c1nnn[nH]1.ClC(c1ccccc1)(c1ccccc1)c1ccccc1>>Cc1ccccc1-c1nnnn1C(c1ccccc1)(c1ccccc1)c1ccccc1
C1(=CC=CC=C1)C(C1=CC=CC=C1)(C1=CC=CC=C1)Cl.CC1=C(C=CC=C1)C1=NN=NN1>>C1(=C(C=CC=C1)C1=NN=NN1C(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)C
[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[n:9][n:10][n:11][nH:12]1.Cl[C:13]([c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1)([c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1)[c:26]1[cH:27][cH:28][cH:29][cH:30][cH:31]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[n:9][n:10][n:11][n:12]1[C:13]([c:14]1[cH:15][cH:16...
Cc1ccccc1-c1nnn[nH]1.ClC(c1ccccc1)(c1ccccc1)c1ccccc1
Cc1ccccc1-c1nnnn1C(c1ccccc1)(c1ccccc1)c1ccccc1
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
c814b61f4411b43802c99c033287485a681b4494d43aabc070529707b2f4fba2
677f263b618a481bcdc02c85060e6c44b1f44f328207057cd4782b98754b7773
c1ccc(-c2nnnn2C(c2ccccc2)(c2ccccc2)c2ccccc2)cc1
Cl-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10].[c:11]-[c:12]1:[#7;a:13]:[#7;a:14]:[#7;a:15]:[nH;D2;+0:16]:1>>[c:3]:[c:2](-[C;H0;D4;+0:1](-[c:5](:[c:6]):[c:7])(-[c:8](:[c:9]):[c:10])-[n;H0;D3;+0:16]1:[#7;a:15]:[#7;a:14]:[#7;a:13]:[c:12]:1-[c:11]):[c:4]
31.6
[{"value": 31.6, "product": "C1(=C(C=CC=C1)C1=NN=NN1C(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of triphenylmethyl chloride (348 mg, 1.25 mmol, 2 ml DCM) was added dropwise to a mixture of 5-(2-methylphenyl)-1H-tetrazole (200.5 mg, 1.25 mmol) and TEA (174 μl, 1.25 mmol) in 8 ml DCM. The reaction mixture was strirred overnight at RT, then washed with water (10 ml). The organic layer was dried over sodiu...
10.6084/m9.figshare.5104873.v1
null
Tertiary halide
null
c1nnn[nH]1
c1nnn[nH]1
c1ccccc1.c1nnn[nH]1.c1ccccc1.c1ccccc1.c1ccccc1
HCl
C(Cl)Cl
null
8
Cc1ccccc1-c1nnn[nH]1.ClC(c1ccccc1)(c1ccccc1)c1ccccc1>C(Cl)Cl>Cc1ccccc1-c1nnnn1C(c1ccccc1)(c1ccccc1)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d213834817a045fc9c40e9442c732d6e
N#Cc1csc(C=O)c1.[N-]=[N+]=[N-]>>O=Cc1cc(-c2nnn[nH]2)cs1
O.[N-]=[N+]=[N-].[Na+].C(=O)C1=CC(=CS1)C#N.Cl>>N1N=NN=C1C=1C=C(SC1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5]([C:6]#[N:7])[cH:11][s:12]1.[N-:8]=[N+:9]=[N-:10]>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[n:7][n:8][n:9][nH:10]2)[cH:11][s:12]1
N#Cc1csc(C=O)c1.[N-]=[N+]=[N-]
O=Cc1cc(-c2nnn[nH]2)cs1
null
null
CN(C)C=O
Aromatic Heterocycle Formation
OtherReaction
237b84aaa459abf427f233dc6a07a1d9de824f980714e458423189bb68f60f12
d8c808528b7ee68720aaeebd35cb6a2a30e344748d0066102cdae99843b93cf0
c1cc(-c2nnn[nH]2)cs1
[N-;H0;D1:1]=[N+;H0;D2:2]=[N-;H0;D1:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[c;H0;D3;+0:6]1:[c:7]:[#16;a:8]:[c:9](-[C:10]=[O;D1;H0:11]):[c:12]:1>>[O;D1;H0:11]=[C:10]-[c:9]1:[#16;a:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:5]2:[n;H0;D2;+0:4]:[n;H0;D2;+0:3]:[n;H0;D2;+0:2]:[nH;D2;+0:1]:2):[c:12]:1
20
[{"value": 20.0, "product": "N1N=NN=C1C=1C=C(SC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Sodium azide (2.9 g, 44.6 mmol) and TEA hydrochloride (4.13 g, 30 mmol) were added to a solution of 5-formyl-thiophene-3-carbonitrile (2 g, 15 mmol, prepared according to Intern. application WO 02126718) in DMF (50 ml). The solution was refluxed for 12 h. After cooling to RT, water was added and the solution was carefu...
10.6084/m9.figshare.5104873.v1
null
Nitrile
null
null
c1nnn[nH]1
c1ccsc1.c1nnn[nH]1
null
CN(C)C=O
null
null
N#Cc1csc(C=O)c1.[N-]=[N+]=[N-]>CN(C)C=O>O=Cc1cc(-c2nnn[nH]2)cs1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-505d61d455ad42dea1fa0ca92d5dd593
BrCCCC(Br)c1ccc(Br)cc1.CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
O.[OH-].[K+].BrC1=CC=C(C=C1)C(CCCBr)Br.ClC=1C=C(C=C(C1)Cl)N1C(N(CC1=O)C)=O>>BrC1=CC=C(C=C1)[C@H]1[C@@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1
Br[CH2:17][CH2:18][CH2:19][CH:20](Br)[c:21]1[cH:22][cH:23][c:24]([Br:25])[cH:26][cH:27]1.[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[CH2:16]1>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[C@:16]12[CH2:...
BrCCCC(Br)c1ccc(Br)cc1.CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
null
null
CS(=O)C
C-C Coupling
OtherReaction
f7705fcc55562dd1d514d37592f3026f1b985aed97988cbab983ce3221a43656
d4cf29bb0f2586f258c9eb5d3edb710b86094a4be60be4638a5468606055dcb5
O=C1N[C@@]2(CCC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3]-[CH;D3;+0:4](-Br)-[c:5](:[c:6]):[c:7].[C;D1;H3:8]-[#7:9]1-[CH2;D2;+0:10]-[C:11](=[O;D1;H0:12])-[#7:13](-[c:14])-[C:15]-1=[O;D1;H0:16]>>[C;D1;H3:8]-[#7:9]1-[C:15](=[O;D1;H0:16])-[#7:13](-[c:14])-[C:11](=[O;D1;H0:12])-[C@;H0;D4;+0:10]-12-[CH2;D2;+0:1]-[C:2]-[C:3]-[C@H;D3;+0:4]-2-[c:5](:[c:6])...
110.8
[{"value": 110.8, "product": "BrC1=CC=C(C=C1)[C@H]1[C@@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
HOUR
KOH flakes (1.3 g, 23.2 mmol) were added at RT to a solution of 1-bromo-4(1,4-dibromobutyl)benzene (4.08 g, 10.6 mmol) (Preparation 4) and 3-(3,5-dichlorophenyl)-1-methylimidazolidine-2,4-dione (2.5 g, 9.6 mmol, prepared according to Fujinami et al. cited above) in dry DMSO (40 ml). After 30 h at RT, the reaction mixtu...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Primary halide
null
C1C[NH]C[NH]1
C1CCC2(C1)C[NH]C[NH]2
c1ccccc1.C1CCC2(C1)C[NH]C[NH]2.c1ccccc1
HBr
CS(=O)C
null
30
BrCCCC(Br)c1ccc(Br)cc1.CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O>CS(=O)C>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2ba53f5111614be491e14902f7e9b2ca
CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O.ClC(CCBr)c1ccc(Br)cc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CC[C@H]2c1ccc(Br)cc1
BrC1=CC=C(C=C1)C(CCBr)Cl.ClC=1C=C(C=C(C1)Cl)N1C(N(CC1=O)C)=O>>BrC1=CC=C(C=C1)[C@@H]1CC[C@@]12N(C(N(C2=O)C2=CC(=CC(=C2)Cl)Cl)=O)C
[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[CH2:16]1.Cl[CH:19]([CH2:18][CH2:17]Br)[c:20]1[cH:21][cH:22][c:23]([Br:24])[cH:25][cH:26]1>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[C@:16]12[CH2:17][CH2:...
CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O.ClC(CCBr)c1ccc(Br)cc1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CC[C@H]2c1ccc(Br)cc1
null
null
null
C-C Coupling
OtherReaction
633122e91d14da7e197b20d59ad495d86526fe11b8586f717e52f0c369568b4b
d4cf29bb0f2586f258c9eb5d3edb710b86094a4be60be4638a5468606055dcb5
O=C1N[C@@]2(CC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]-[CH;D3;+0:3](-Cl)-[c:4](:[c:5]):[c:6].[C;D1;H3:7]-[#7:8]1-[CH2;D2;+0:9]-[C:10](=[O;D1;H0:11])-[#7:12](-[c:13])-[C:14]-1=[O;D1;H0:15]>>[C;D1;H3:7]-[#7:8]1-[C:14](=[O;D1;H0:15])-[#7:12](-[c:13])-[C:10](=[O;D1;H0:11])-[C@;H0;D4;+0:9]-12-[CH2;D2;+0:1]-[C:2]-[C@H;D3;+0:3]-2-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
Using the same procedure as in Example 1 starting from 1-bromo-4-(3-bromo-1-chloropropyl)benzene (Preparation 7) and 3-(3,5-dichlorophenyl)-1-methylimidazolidine-2,4-dione, the above titled compound was obtained after reverse phase HPLC purification (gradient from CH3CN/H2O/TFA: 5/95/0.05 to CH3CN/H2O[[FA: 80/20/0.05)....
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Primary halide
null
C1C[NH]C[NH]1
C1CC2(C1)C[NH]C[NH]2
c1ccccc1.C1CC2(C1)C[NH]C[NH]2.c1ccccc1
HCl.Br-
null
null
null
CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O.ClC(CCBr)c1ccc(Br)cc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CC[C@H]2c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-37e8e7fbf64f43989d779c703b77e07e
BrCCCCC(Br)c1ccc(Br)cc1.CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCCC[C@H]2c1ccc(Br)cc1
BrC1=CC=C(C=C1)C(CCCCBr)Br.ClC=1C=C(C=C(C1)Cl)N1C(N(CC1=O)C)=O>>BrC1=CC=C(C=C1)[C@H]1[C@@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CCCC1
Br[CH2:17][CH2:18][CH2:19][CH2:20][CH:21](Br)[c:22]1[cH:23][cH:24][c:25]([Br:26])[cH:27][cH:28]1.[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[CH2:16]1>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[C@:16...
BrCCCCC(Br)c1ccc(Br)cc1.CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCCC[C@H]2c1ccc(Br)cc1
null
null
null
C-C Coupling
OtherReaction
b5252ea826d331e6580a114bacf223f7ee0db41abb8410b94bbb79f77b0982ca
d4cf29bb0f2586f258c9eb5d3edb710b86094a4be60be4638a5468606055dcb5
O=C1N[C@@]2(CCCC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4]-[CH;D3;+0:5](-Br)-[c:6](:[c:7]):[c:8].[C;D1;H3:9]-[#7:10]1-[CH2;D2;+0:11]-[C:12](=[O;D1;H0:13])-[#7:14](-[c:15])-[C:16]-1=[O;D1;H0:17]>>[C;D1;H3:9]-[#7:10]1-[C:16](=[O;D1;H0:17])-[#7:14](-[c:15])-[C:12](=[O;D1;H0:13])-[C@;H0;D4;+0:11]-12-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4]-[C@H;D3;+0:5]-2...
null
[]
null
null
null
null
Using the same procedure as in Example 1 starting from 1-bromo-4-(1,5-dibromopentyl)benzene (4.2 g, 10.9 mmol) (Preparation 14) and 3-(3,5-dichlorophenyl)-1-methylimidazolidine-2,4-dione (2.59 g, 10 mmol), the above titled compound was obtained as a white solid (3.1 g, mp=118° C.). 1H NMR (CDCl3): 7.41 (2H, d, J=8.4 Hz...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Primary halide
null
C1C[NH]C[NH]1
C1CCC2(CC1)C[NH]C[NH]2
c1ccccc1.C1CCC2(CC1)C[NH]C[NH]2.c1ccccc1
HBr
null
null
null
BrCCCCC(Br)c1ccc(Br)cc1.CN1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCCC[C@H]2c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-975e51b9a41b4311b50a080c893fcfdd
BrCCCC(Br)c1ccc(Br)cc1.CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O>>CC(C)(C)OC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
BrC1=CC=C(C=C1)C(CCCBr)Br.C(C)(C)(C)OC(=O)N1C(N(C(C1)=O)C1=CC(=CC(=C1)Cl)Cl)=O>>C(C)(C)(C)OC(=O)N1C(N(C([C@@]12[C@@H](CCC2)C2=CC=C(C=C2)Br)=O)C2=CC(=CC(=C2)Cl)Cl)=O
Br[CH2:23][CH2:24][CH2:25][CH:26](Br)[c:27]1[cH:28][cH:29][c:30]([Br:31])[cH:32][cH:33]1.[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[C:9](=[O:10])[N:11]([c:12]2[cH:13][c:14]([Cl:15])[cH:16][c:17]([Cl:18])[cH:19]2)[C:20](=[O:21])[CH2:22]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[C:9](=[O:10])[N...
BrCCCC(Br)c1ccc(Br)cc1.CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O
CC(C)(C)OC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
null
null
null
C-C Coupling
OtherReaction
fcf323dbc98913cd643daae03149d5439e966c3e4b72498f18033d4ddeab87ee
f9ab306b4747162d02bd4f01c34c8064410ebdd862f2319d026ca31209db9bc0
O=C1N[C@@]2(CCC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3]-[CH;D3;+0:4](-Br)-[c:5](:[c:6]):[c:7].[C;D1;H3:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[#8:12]-[C:13](=[O;D1;H0:14])-[#7:15]1-[CH2;D2;+0:16]-[C:17](=[O;D1;H0:18])-[#7:19](-[c:20])-[C:21]-1=[O;D1;H0:22]>>[C;D1;H3:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[#8:12]-[C:13](=[O;D1;H0:14])-[#7:15]1-[C...
null
[]
null
null
null
null
Using the same procedure as in Example 1 starting from 1-bromo-4-(1,4-dibromobutyl)benzene (153 mg, 0.4 mmol) (Preparation 4) and 3-(3,5-dichlorophenyl)-2,4-dioxoimidazolidine-1-carboxylic acid tert-butyl ester (113 mg, 0.33 mmol) (Preparation 11), the above-titled compound was obtained (33 mg) as a white solid. 1H NMR...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Primary halide.Substituted dicarboximide
Substituted dicarboximide
C1C[NH]C[NH]1
C1CCC2(C1)C[NH]C[NH]2
c1ccccc1.C1CCC2(C1)C[NH]C[NH]2.c1ccccc1
HBr
null
null
null
BrCCCC(Br)c1ccc(Br)cc1.CC(C)(C)OC(=O)N1CC(=O)N(c2cc(Cl)cc(Cl)c2)C1=O>>CC(C)(C)OC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-350aa061377f413b88ef248f811e4b96
CC(C)(C)OC(=O)N1C(=S)N(c2cc(Cl)cc(Cl)c2)C(=O)C12CCCC2c1ccc(Br)cc1>>O=C1N(c2cc(Cl)cc(Cl)c2)C(=S)NC12CCCC2c1ccc(Br)cc1
C(C)(C)(C)OC(=O)N1C(N(C(C12C(CCC2)C2=CC=C(C=C2)Br)=O)C2=CC(=CC(=C2)Cl)Cl)=S.C(=O)(C(F)(F)F)O.C(Cl)Cl.O>>BrC1=CC=C(C=C1)C1C2(C(N(C(N2)=S)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1
CC(C)(C)OC(=O)[N:14]1[C:12](=[S:13])[N:3]([c:4]2[cH:5][c:6]([Cl:7])[cH:8][c:9]([Cl:10])[cH:11]2)[C:2](=[O:1])[C:15]12[CH2:16][CH2:17][CH2:18][CH:19]2[c:20]1[cH:21][cH:22][c:23]([Br:24])[cH:25][cH:26]1>>[O:1]=[C:2]1[N:3]([c:4]2[cH:5][c:6]([Cl:7])[cH:8][c:9]([Cl:10])[cH:11]2)[C:12](=[S:13])[NH:14][C:15]12[CH2:16][CH2:17]...
CC(C)(C)OC(=O)N1C(=S)N(c2cc(Cl)cc(Cl)c2)C(=O)C12CCCC2c1ccc(Br)cc1
O=C1N(c2cc(Cl)cc(Cl)c2)C(=S)NC12CCCC2c1ccc(Br)cc1
null
null
null
Reduction
Boc amine deprotection
fe11bba53ba77b759f0c7fd3a8717a8b7b48968896e428499fd61e4892b39186
a5b4fdded3cbffe70a4e1e726f93dd5004a2fc9b906892482e0785d7f6416d9f
O=C1N(c2ccccc2)C(=S)NC12CCCC2c1ccccc1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2](=[S;D1;H0:3])-[#7:4](-[c:5])-[C:6](=[O;D1;H0:7])-[C:8]-1(-[C:9])-[C:10]>>[C:9]-[C:8]1(-[C:10])-[NH;D2;+0:1]-[C:2](=[S;D1;H0:3])-[#7:4](-[c:5])-[C:6]-1=[O;D1;H0:7]
60.4
[{"value": 60.4, "product": "BrC1=CC=C(C=C1)C1C2(C(N(C(N2)=S)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
6-(4-Bromophenyl)-3-(3,5-dichlorophenyl)-4-oxo-2-thioxo-1,3-diazaspiro[4.4]nonane-1-carboxylic acid tert-butyl ester (42 mg, 74 μmol) (Preparation 10) was added to a TFA/DCM/H2O (1/1/0.1) solution (1 ml) at RT. After 30 min the reaction mixture was concentrated to give a beige solid which was washed with pentane to yie...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Thiourea.Boc
Thiourea
C1CCC2(C1)C[NH]C[NH]2
C1CCC2(C1)C[NH]CN2
c1ccccc1.C1CCC2(C1)C[NH]CN2.c1ccccc1
HO-
null
null
null
CC(C)(C)OC(=O)N1C(=S)N(c2cc(Cl)cc(Cl)c2)C(=O)C12CCCC2c1ccc(Br)cc1>>O=C1N(c2cc(Cl)cc(Cl)c2)C(=S)NC12CCCC2c1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-de085f3f17b64cf198ba4cd20b06db1d
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)C12CCCC2c1ccc(Br)cc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(C#N)cc1
BrC1=CC=C(C=C1)C1C2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1.C(#N)[Cu].C(CN)N>>ClC=1C=C(C=C(C1)Cl)N1C(N([C@@]2(C1=O)[C@@H](CCC2)C2=CC=C(C#N)C=C2)C)=O
Br[c:24]1[cH:23][cH:22][c:21]([CH:20]2[C:16]3([N:2]([CH3:1])[C:3](=[O:4])[N:5]([c:6]4[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]4)[C:14]3=[O:15])[CH2:17][CH2:18][CH2:19]2)[cH:28][cH:27]1>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[C@:16]12[CH2:17][CH2:18...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)C12CCCC2c1ccc(Br)cc1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(C#N)cc1
null
null
CN1CCCC1=O
Miscellaneous
OtherReaction
3ae4da8b7f110de99cf8afc091b6f0c8540050148e425770f8030bce1480042c
73a96fe5e833259ca394a42f82d6cc2ee7231bcde92d95030d2893b90c3fef76
O=C1N[C@@]2(CCC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]>>[N;D1;H0:6]#[C:7]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
180
CELSIUS
null
null
A mixture of 6-(4-bromophenyl)-3-(3,5-dichlorophenyl)-1-methyl-1,3-diazaspiro[4.4]nonane-2,4-dione (1 g, 2.1 mmol) (Example 1) and CuCN (0.45 g, 5 mmol) in NMP was heated to 180° C. for 6 h. After cooling, the reaction mixture was poured on a mixture of ice and ethylene diamine and extracted twice with DCM. The brown r...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Nitrile
c1ccccc1
c1ccccc1
c1ccccc1.C1CCC2(C1)C[NH]C[NH]2.c1ccccc1
Br-
CN1CCCC1=O
180
null
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)C12CCCC2c1ccc(Br)cc1>CN1CCCC1=O>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c46e7e76268b42ab83507814dbe2a19a
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1.OB(O)c1ccccc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(-c2ccccc2)cc1
BrC1=CC=C(C=C1)[C@H]1[C@@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1.C1(=CC=CC=C1)B(O)O.C(=O)([O-])[O-].[K+].[K+]>>C1(=CC=C(C=C1)[C@H]1[C@@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1)C1=CC=CC=C1
Br[c:24]1[cH:23][cH:22][c:21]([C@H:20]2[C@:16]3([N:2]([CH3:1])[C:3](=[O:4])[N:5]([c:6]4[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]4)[C:14]3=[O:15])[CH2:17][CH2:18][CH2:19]2)[cH:32][cH:31]1.OB(O)[c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:1...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1.OB(O)c1ccccc1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(-c2ccccc2)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1N[C@@]2(CCC[C@H]2c2ccc(-c3ccccc3)cc2)C(=O)N1c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
25.3
[{"value": 25.3, "product": "C1(=CC=C(C=C1)[C@H]1[C@@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
A solution of (5R*,6S*)-6-(4-bromophenyl)-3-(3,5-dichlorophenyl)-1-methyl-1,3-diazaspiro[4.4]nonane-2,4-dione (80 mg, 0.17 mmol) (Example 1), phenylboronic acid (73 mg, 0.6 mmol), (Ph3P)4Pd (20 mg, 0.02 mmol) and K2CO3 (80 mg, 0.6 mmol) in a mixture of DME (1.5 ml) and water (50 μl) was heated at 80° C. for 12 h. The i...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.C1CCC2(C1)C[NH]C[NH]2.c1ccccc1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
80
null
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1.OB(O)c1ccccc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(-c2ccccc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-439a77c73ae7453d917a074aa8cfea94
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1.OB(O)c1ccc(F)cc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(-c2ccc(F)cc2)cc1
BrC1=CC=C(C=C1)[C@H]1[C@@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CCC1.FC1=CC=C(C=C1)B(O)O>>ClC=1C=C(C=C(C1)Cl)N1C(N([C@@]2(C1=O)[C@@H](CCC2)C2=CC=C(C=C2)C2=CC=C(C=C2)F)C)=O
Br[c:24]1[cH:23][cH:22][c:21]([C@H:20]2[C@:16]3([N:2]([CH3:1])[C:3](=[O:4])[N:5]([c:6]4[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]4)[C:14]3=[O:15])[CH2:17][CH2:18][CH2:19]2)[cH:33][cH:32]1.OB(O)[c:25]1[cH:26][cH:27][c:28]([F:29])[cH:30][cH:31]1>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1.OB(O)c1ccc(F)cc1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(-c2ccc(F)cc2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1N[C@@]2(CCC[C@H]2c2ccc(-c3ccccc3)cc2)C(=O)N1c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
14.6
[{"value": 14.6, "product": "ClC=1C=C(C=C(C1)Cl)N1C(N([C@@]2(C1=O)[C@@H](CCC2)C2=CC=C(C=C2)C2=CC=C(C=C2)F)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using the procedure described in Example 8 (5R*,6S*)-6-(4-bromophenyl)-3-(3,5-dichlorophenyl)-1-methyl-1,3-diazaspiro[4.4]nonane-2,4-dione (80 mg, 0.17 mmol) (Example 1) was reacted with 4-fluorophenylboronic acid (71.4 mg, 0.51 mmol) to yield the above-titled compound (12 mg) as a white solid. 1H NMR (CDCl3) δ 7.45–7....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.C1CCC2(C1)C[NH]C[NH]2.c1ccccc1.c1ccccc1
HBr.B
null
null
null
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(Br)cc1.OB(O)c1ccc(F)cc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CCC[C@H]2c1ccc(-c2ccc(F)cc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-08d22c3fc77948e883a615f5285a17f6
CC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(C#N)cc1>>N#Cc1ccc([C@@H]2CN(Cc3ccccc3)C[C@@]23NC(=O)N(c2cc(Cl)cc(Cl)c2)C3=O)cc1
C(C)(=O)N1C(N(C([C@]12CN(C[C@H]2C2=CC=C(C#N)C=C2)CC2=CC=CC=C2)=O)C2=CC(=CC(=C2)Cl)Cl)=O.N1CCCC1>>C(C1=CC=CC=C1)N1C[C@]2(C(N(C(N2)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C#N)C=C1
CC(=O)[N:19]1[C@:18]2([C@H:7]([c:6]3[cH:5][cH:4][c:3]([C:2]#[N:1])[cH:34][cH:33]3)[CH2:8][N:9]([CH2:10][c:11]3[cH:12][cH:13][cH:14][cH:15][cH:16]3)[CH2:17]2)[C:31](=[O:32])[N:22]([c:23]2[cH:24][c:25]([Cl:26])[cH:27][c:28]([Cl:29])[cH:30]2)[C:20]1=[O:21]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([C@@H:7]2[CH2:8][N:9]([CH2:10]...
CC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(C#N)cc1
N#Cc1ccc([C@@H]2CN(Cc3ccccc3)C[C@@]23NC(=O)N(c2cc(Cl)cc(Cl)c2)C3=O)cc1
null
null
C1CCOC1
Reduction
Hydrogenolysis of tertiary amines
cca8e3a2dc6c2eee6e2fdc484fec1d1448c5181def3e7a4e759da140ec931cff
b3d6f616fb24bef205baf1bc6e3966e3715bac59493272a22ddc34f831a5b118
O=C1N[C@@]2(CN(Cc3ccccc3)C[C@H]2c2ccccc2)C(=O)N1c1ccccc1
C-C(=O)-[N;H0;D3;+0:1]1-[C:2](=[O;D1;H0:3])-[#7:4](-[c:5])-[C:6](=[O;D1;H0:7])-[C:8]-1(-[C:9])-[C:10]-[#7:11]>>[#7:11]-[C:10]-[C:8]1(-[C:9])-[NH;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#7:4](-[c:5])-[C:6]-1=[O;D1;H0:7]
113.3
[{"value": 113.3, "product": "C(C1=CC=CC=C1)N1C[C@]2(C(N(C(N2)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C#N)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of Example 11 (8.9 g, 16.7 mmol), TEA (3.8 ml) and pyrrolidine (2.2 ml) in THF (270 ml) was refluxed for 2 h 30 min. The mixture was concentrated in vacuo and taken into DCM, then washed with water. The organic layer was dried over MgSO4 and concentrated. The resulting solid was chromatographed over silica ge...
10.6084/m9.figshare.5104873.v1
null
Urea.Substituted dicarboximide
Urea
C1C[C@]2(C[NH]1)C[NH]C[NH]2
C1C[C@]2(C[NH]1)C[NH]CN2
c1ccccc1.c1ccccc1.C1C[C@]2(C[NH]1)C[NH]CN2.c1ccccc1
HO-
C1CCOC1
null
null
CC(=O)N1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(C#N)cc1>C1CCOC1>N#Cc1ccc([C@@H]2CN(Cc3ccccc3)C[C@@]23NC(=O)N(c2cc(Cl)cc(Cl)c2)C3=O)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7cb9e9d519f0413c8a1628a32eb49f53
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(C#N)cc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1
ClC(=O)OC(C)Cl.C(C1=CC=CC=C1)N1C[C@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C#N)C=C1>>ClC=1C=C(C=C(C1)Cl)N1C(N([C@]2(C1=O)CNC[C@H]2C2=CC=C(C#N)C=C2)C)=O
c1ccc(C[N:18]2[CH2:17][C@@:16]3([N:2]([CH3:1])[C:3](=[O:4])[N:5]([c:6]4[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]4)[C:14]3=[O:15])[C@H:20]([c:21]3[cH:22][cH:23][c:24]([C:25]#[N:26])[cH:27][cH:28]3)[CH2:19]2)cc1>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15]...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(C#N)cc1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1
null
null
C(Cl)Cl
Deprotection
Hydrogenolysis of tertiary amines
86a93e9e2e1e54d1e9087e31670820a5e059aff13afceb12a5a20228453b2f67
1c99dd446c0bf4ae872cd8df8de34955be195747c234e9f3c49f46d1de614f66
O=C1N[C@@]2(CNC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
[#7:1]-[C:2]1(-[C:3]-[N;H0;D3;+0:4](-C-c2:c:c:c:c:c:2)-[C:5]-[C:6]-1)-[C:7](=[O;D1;H0:8])-[#7:9]>>[#7:1]-[C:2]1(-[C:3]-[NH;D2;+0:4]-[C:5]-[C:6]-1)-[C:7](=[O;D1;H0:8])-[#7:9]
116.8
[{"value": 116.8, "product": "ClC=1C=C(C=C(C1)Cl)N1C(N([C@]2(C1=O)CNC[C@H]2C2=CC=C(C#N)C=C2)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
1-Chloroethyl chloroformate (4.4 ml, 40.3 mmol) was added to a cooled (5° C.) solution of Example 14 (5.1 g, 10.1 mmol) in DCM (250 ml). After 1 h at 5° C., the reaction mixture was stirred at RT for 20 h. The solution was concentrated to dryness and then refluxed in MeOH (350 ml) for 3 h. After concentration in vacuo,...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
Secondary amine
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2
C1C[C@]2(CN1)C[NH]C[NH]2
c1ccccc1.C1C[C@]2(CN1)C[NH]C[NH]2.c1ccccc1
Other
C(Cl)Cl
null
1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(C#N)cc1>C(Cl)Cl>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fa608298f4e84e2c916e95bf0375dc9c
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=C(O)c1cccc(S(=O)(=O)Cl)c1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(S(=O)(=O)c1cccc(C(=O)O)c1)C[C@H]2c1ccc(C#N)cc1
ClC=1C=C(C=C(C1)Cl)N1C(N([C@]2(C1=O)CNC[C@H]2C2=CC=C(C#N)C=C2)C)=O.ClS(=O)(=O)C=1C=C(C(=O)O)C=CC1.C([O-])(O)=O.[Na+]>>C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)S(=O)(=O)C=2C=C(C(=O)O)C=CC2
[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[C@:16]12[CH2:17][NH:18][CH2:31][C@H:32]2[c:33]1[cH:34][cH:35][c:36]([C:37]#[N:38])[cH:39][cH:40]1.Cl[S:19](=[O:20])(=[O:21])[c:22]1[cH:23][cH:24][cH:25][c:26]([C:27](=[O:28])[OH:29])[cH:30]1>>[CH3:1][N:2]1[C:3](=[O:4...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=C(O)c1cccc(S(=O)(=O)Cl)c1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(S(=O)(=O)c1cccc(C(=O)O)c1)C[C@H]2c1ccc(C#N)cc1
null
null
O.CC(=O)C
Acylation
Sulfonamide synthesis (Schotten-Baumann) secondary amine
1b2818293e715791db7c91df8d8a7422ce1fb5a109d0403b369edb71cf4e3394
b7aca5a5d690b0846685a854bc946849e1041bfc3965161290b5ffb2821af09e
O=C1N[C@@]2(CN(S(=O)(=O)c3ccccc3)C[C@H]2c2ccccc2)C(=O)N1c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[#7:7]-[C:8]1(-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]-1)-[C:13](=[O;D1;H0:14])-[#7:15]>>[#7:7]-[C:8]1(-[C:9]-[N;H0;D3;+0:10](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[C:11]-[C:12]-1)-[C:13](=[O;D1;H0:14])-[#7:15]
77
[{"value": 77.0, "product": "C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)S(=O)(=O)C=2C=C(C(=O)O)C=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a mixture of 4-[(5S,9R)-3-(3,5-Dichlorophenyl)-1-methyl-2,4-dioxo-1,3,7-triazaspiro[4.4]non-9-yl]-benzonitrile (Example 15a) (0.11 g, 0.26 mmol) and (3-(Chlorosulfonyl)benzoic acid (0.058 g, 0.26 mmol) in acetone and water (1:1 mL) was added sodium bicarbonate at room temperature. The reaction mixture was stirred at...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
C1C[C@]2(CN1)C[NH]C[NH]2
C1C[C@]2(C[NH]1)C[NH]C[NH]2
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccccc1.c1ccccc1
HCl
O.CC(=O)C
null
null
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=C(O)c1cccc(S(=O)(=O)Cl)c1>O.CC(=O)C>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(S(=O)(=O)c1cccc(C(=O)O)c1)C[C@H]2c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-35aad3b2b74b4113a221a93457d4b0e4
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=Cc1cc(C(=O)O)cs1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1
C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+].ClC=1C=C(C=C(C1)Cl)N1C(N([C@]2(C1=O)CNC[C@H]2C2=CC=C(C#N)C=C2)C)=O.C(=O)C1=CC(=CS1)C(=O)O.S(=O)(=O)([O-])[O-].[Na+].[Na+]>>C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC2=CC(=CS2)C(=O)O
[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]2)[C:14](=[O:15])[C@:16]12[CH2:17][NH:18][CH2:28][C@H:29]2[c:30]1[cH:31][cH:32][c:33]([C:34]#[N:35])[cH:36][cH:37]1.O=[CH:19][c:20]1[cH:21][c:22]([C:23](=[O:24])[OH:25])[cH:26][s:27]1>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=Cc1cc(C(=O)O)cs1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1
null
null
ClCCCl
Heteroatom Alkylation and Arylation
reductive amination
44097ca774a12d2e9795061525b666c24d17f0e2808f6b11d701443fa2eeefe0
2d03f38884b1fbb0c0d6e6f2de31afb25102fec87f347c3a123e064c1bfef0ad
O=C1N[C@@]2(CN(Cc3cccs3)C[C@H]2c2ccccc2)C(=O)N1c1ccccc1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[#16;a:4]:[c:5].[#7:6]-[C:7]1(-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]-1)-[C:12](=[O;D1;H0:13])-[#7:14]>>[#7:6]-[C:7]1(-[C:8]-[N;H0;D3;+0:9](-[CH2;D2;+0:1]-[c:2](:[c:3]):[#16;a:4]:[c:5])-[C:10]-[C:11]-1)-[C:12](=[O;D1;H0:13])-[#7:14]
75
[{"value": 75.0, "product": "C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC2=CC(=CS2)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
6
HOUR
To a solution of 4-[(5S,9R)-3-(3,5-Dichlorophenyl)-1-methyl-2,4-dioxo-1,3,7-triazaspiro[4.4]non-9-yl]-benzonitrile (0.1 g, 0.24 mmol) (Example 15a) in 1,2-DCE (4 mL) were sequentially added 5-Formyl-3-thiophenecarboxylic acid (0.045 g, 0.29 mmol) and sodium sulfate (150 mgs) under a nitrogen atmosphere at room temperat...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary amine
Tertiary amine
C1C[C@]2(CN1)C[NH]C[NH]2
C1C[C@]2(C[NH]1)C[NH]C[NH]2
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccsc1.c1ccccc1
Other
ClCCCl
null
6
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=Cc1cc(C(=O)O)cs1>ClCCCl>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-484a0e8cb7574f20af85d49d661496c8
CCN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=C(O)c1cccc(S(=O)(=O)Cl)c1>>CCN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(S(=O)(=O)c1cccc(C(=O)O)c1)C[C@H]2c1ccc(C#N)cc1
ClC=1C=C(C=C(C1)Cl)N1C(N([C@]2(C1=O)CNC[C@H]2C2=CC=C(C#N)C=C2)CC)=O.ClS(=O)(=O)C=1C=C(C(=O)O)C=CC1.CCN(C(C)C)C(C)C>>C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2CC)=O)C2=CC(=CC(=C2)Cl)Cl)=O)S(=O)(=O)C=2C=C(C(=O)O)C=CC2
[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[N:6]([c:7]2[cH:8][c:9]([Cl:10])[cH:11][c:12]([Cl:13])[cH:14]2)[C:15](=[O:16])[C@:17]12[CH2:18][NH:19][CH2:32][C@H:33]2[c:34]1[cH:35][cH:36][c:37]([C:38]#[N:39])[cH:40][cH:41]1.Cl[S:20](=[O:21])(=[O:22])[c:23]1[cH:24][cH:25][cH:26][c:27]([C:28](=[O:29])[OH:30])[cH:31]1>>[CH3:1][CH2:2][N...
CCN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=C(O)c1cccc(S(=O)(=O)Cl)c1
CCN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(S(=O)(=O)c1cccc(C(=O)O)c1)C[C@H]2c1ccc(C#N)cc1
null
null
C1CCOC1
Acylation
Sulfonamide synthesis (Schotten-Baumann) secondary amine
1b2818293e715791db7c91df8d8a7422ce1fb5a109d0403b369edb71cf4e3394
b7aca5a5d690b0846685a854bc946849e1041bfc3965161290b5ffb2821af09e
O=C1N[C@@]2(CN(S(=O)(=O)c3ccccc3)C[C@H]2c2ccccc2)C(=O)N1c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[#7:7]-[C:8]1(-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]-1)-[C:13](=[O;D1;H0:14])-[#7:15]>>[#7:7]-[C:8]1(-[C:9]-[N;H0;D3;+0:10](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[C:11]-[C:12]-1)-[C:13](=[O;D1;H0:14])-[#7:15]
44.6
[{"value": 44.6, "product": "C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2CC)=O)C2=CC(=CC(=C2)Cl)Cl)=O)S(=O)(=O)C=2C=C(C(=O)O)C=CC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
To a mixture of Example 50 (100 mg, 0.23 mmol) and 3-(chlorosulfonyl) benzoic acid (57 mg, 0.26 mmol) in THF (5 ml) was added DIEA (45 μl, 0.26 mmol) at room temperature. The reaction mixture was stirred at room temperature for 24 hours then concentrated under vacuum. The residue was partitioned between EtOAc and water...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
C1C[C@]2(CN1)C[NH]C[NH]2
C1C[C@]2(C[NH]1)C[NH]C[NH]2
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccccc1.c1ccccc1
HCl
C1CCOC1
null
24
CCN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1.O=C(O)c1cccc(S(=O)(=O)Cl)c1>C1CCOC1>CCN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(S(=O)(=O)c1cccc(C(=O)O)c1)C[C@H]2c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b83e80f1a9644bf9b7f8fbb2a3be31c8
CCOC(=O)CBr.CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1>>CCOC(=O)CN1C[C@@H](c2ccc(C#N)cc2)[C@]2(C1)C(=O)N(c1cc(Cl)cc(Cl)c1)C(=O)N2C
ClC=1C=C(C=C(C1)Cl)N1C(N([C@]2(C1=O)CNC[C@H]2C2=CC=C(C#N)C=C2)C)=O.CCOC(=O)CBr.C(=O)([O-])[O-].[K+].[K+]>>C(C)OC(CN1C[C@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C=C1)C#N)=O
Br[CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].[NH:7]1[CH2:8][C@@H:9]([c:10]2[cH:11][cH:12][c:13]([C:14]#[N:15])[cH:16][cH:17]2)[C@:18]2([CH2:19]1)[C:20](=[O:21])[N:22]([c:23]1[cH:24][c:25]([Cl:26])[cH:27][c:28]([Cl:29])[cH:30]1)[C:31](=[O:32])[N:33]2[CH3:34]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][N:7]1[CH2:8][C@@H:9]([c:...
CCOC(=O)CBr.CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1
CCOC(=O)CN1C[C@@H](c2ccc(C#N)cc2)[C@]2(C1)C(=O)N(c1cc(Cl)cc(Cl)c1)C(=O)N2C
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
7756ee7a94ed7c5f836f75b7b27466db82f96ec3c12774686e48b30bc41fb738
e09591825c4808efe257024fb4bbe3690a7cda9ee664fef9727988761bae5b4a
O=C1N[C@@]2(CNC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5].[#7:6]-[C:7](=[O;D1;H0:8])-[C:9]1(-[#7:10])-[C:11]-[NH;D2;+0:12]-[C:13]-[C:14]-1>>[#7:6]-[C:7](=[O;D1;H0:8])-[C:9]1(-[#7:10])-[C:11]-[N;H0;D3;+0:12](-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5])-[C:13]-[C:14]-1
39.2
[{"value": 39.2, "product": "C(C)OC(CN1C[C@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C=C1)C#N)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of Example 15 (100 mg, 0.24 mmol), ethyl bromo acetate (29 μl, 0.26 mmol) and K2CO3 (36.6 mg, 0.26 mmol) in toluene (2 ml) was heated to 100° C. for 5 h. After cooling to room temperature, the precipitate (unreacted starting material) was removed by filtration. The filtrate was concentrated and purified by ch...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Secondary amine
Ester.Tertiary amine
C1C[C@]2(CN1)C[NH]C[NH]2
C1C[C@]2(C[NH]1)C[NH]C[NH]2
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccccc1
HBr
C1(=CC=CC=C1)C
null
null
CCOC(=O)CBr.CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1>C1(=CC=CC=C1)C>CCOC(=O)CN1C[C@@H](c2ccc(C#N)cc2)[C@]2(C1)C(=O)N(c1cc(Cl)cc(Cl)c1)C(=O)N2C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2179b14edb1d4017bd86105da61999c7
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)OC(C)(C)C)C[C@H]2c1ccc(C#N)cc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)O)C[C@H]2c1ccc(C#N)cc1
FC(C(=O)O)(F)F.C(C)(C)(C)OC(CN1C[C@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C=C1)C#N)=O>>C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC(=O)O
CC(C)(C)[O:22][C:20]([CH2:19][N:18]1[CH2:17][C@@:16]2([N:2]([CH3:1])[C:3](=[O:4])[N:5]([c:6]3[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]3)[C:14]2=[O:15])[C@H:24]([c:25]2[cH:26][cH:27][c:28]([C:29]#[N:30])[cH:31][cH:32]2)[CH2:23]1)=[O:21]>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:1...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)OC(C)(C)C)C[C@H]2c1ccc(C#N)cc1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)O)C[C@H]2c1ccc(C#N)cc1
null
null
C(Cl)Cl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C1N[C@@]2(CNC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
Trifluoroacetic acid (4.8 ml, 59 mmol) was added to a solution of Example 63 (1.56 g, 2.95 mmol) in DCM (40 ml). The solution was refluxed for 3 h. It was then concentrated in vacuo and partitioned between EtOAc/aqueous NH4OH. The aqueous layer was acidified to pH=2 with SO2. The white precipitate was separated by filt...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccccc1
Other
C(Cl)Cl
null
null
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)OC(C)(C)C)C[C@H]2c1ccc(C#N)cc1>C(Cl)Cl>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)O)C[C@H]2c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-824e14e2ee4142ac9fd082ec66eda74c
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(Br)cc1.[CH3][Sn]([CH3])([CH3])[c]1cncnc1>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(-c2cncnc2)cc1
C(C1=CC=CC=C1)N1C[C@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C=C1)Br.C[Sn](C=1C=NC=NC1)(C)C>>C(C1=CC=CC=C1)N1C[C@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C=C1)C=1C=NC=NC1
Br[c:31]1[cH:30][cH:29][c:28]([C@H:27]2[C@:16]3([N:2]([CH3:1])[C:3](=[O:4])[N:5]([c:6]4[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]4)[C:14]3=[O:15])[CH2:17][N:18]([CH2:19][c:20]3[cH:21][cH:22][cH:23][cH:24][cH:25]3)[CH2:26]2)[cH:39][cH:38]1.[CH3][Sn]([CH3])([CH3])[c:32]1[cH:33][n:34][cH:35][n:36][cH:37]1>>[CH3:1][N...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(Br)cc1.[CH3][Sn]([CH3])([CH3])[c]1cncnc1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(-c2cncnc2)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C1(=CC=CC=C1)C
C-C Coupling
Stille reaction_aryl
39e618932e02f216bb32f365d3d5cace861d61f943e27ad5f6a4e36b8af3ac81
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
O=C1N[C@@]2(CN(Cc3ccccc3)C[C@H]2c2ccc(-c3cncnc3)cc2)C(=O)N1c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[CH3]-[Sn](-[CH3])(-[CH3])-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]:1>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]:1):[c:4]:[c:5]
null
[]
null
null
null
null
A mixture of Example 65 (2 g, 3.58 mmol), 5-trimethylstannyl-pyrimidine (1.3 g, 5.35 mmol, prepared according to patent WO 95/06636) and tetrakis(triphenylphosphine)palladium(0) (620 mg, 0.54 mmol) in toluene (50 ml) was refluxed for 10 h under a nitrogen atmosphere. After cooling to room temperature, the insoluble mat...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1ccccc1.c1cncnc1
c1ccccc1.c1cncnc1
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccccc1.c1ccccc1.c1cncnc1
HBr.Sn
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C
null
null
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1ccccc1)C[C@H]2c1ccc(Br)cc1.[CH3][Sn]([CH3])([CH3])[c]1cncnc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(...
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-56993d3e904b46e997c5ab995801993b
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)O)C[C@H]2c1ccc(C#N)cc1.N>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(N)=O)C[C@H]2c1ccc(C#N)cc1
C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC(=O)O.CN1CCOCC1.N.ClC(=O)OCC(C)C>>C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC(=O)N
O[C:20]([CH2:19][N:18]1[CH2:17][C@@:16]2([N:2]([CH3:1])[C:3](=[O:4])[N:5]([c:6]3[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]3)[C:14]2=[O:15])[C@H:24]([c:25]2[cH:26][cH:27][c:28]([C:29]#[N:30])[cH:31][cH:32]2)[CH2:23]1)=[O:22].[NH3:21]>>[CH3:1][N:2]1[C:3](=[O:4])[N:5]([c:6]2[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)O)C[C@H]2c1ccc(C#N)cc1.N
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(N)=O)C[C@H]2c1ccc(C#N)cc1
null
null
O.C(Cl)Cl
Acylation
Carboxylic acid to amide conversion
1283aef55d7ee699f097a8e5267689198c76ba671644401547f902657820236d
cb0a71c3fb37a76e96fbd81aae6f95a28398a03d1ad2c8e877085e735efb98f1
O=C1N[C@@]2(CNC[C@H]2c2ccccc2)C(=O)N1c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4].[NH3;D0;+0:5]>>[#7:4]-[C:3]-[C;H0;D3;+0:1](-[NH2;D1;+0:5])=[O;D1;H0:2]
55.3
[{"value": 55.3, "product": "C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Isobutyl chloroformate (27 μl, 0.21 mmol) was added to a cooled (5° C.) suspension of Example 64 (90 mg, 0.19 mmol) and N-methyl morpholine (23 μl, 0.2 mmol) in DCM (4 ml). After 1 h, ammonia (420 μl, 0.5 M in dioxane, 0.21 mmol) was added. After 1 h at 5° C. and 3 h at RT, water (2 ml) was added. The organic layer was...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary amide
null
null
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccccc1
HO-
O.C(Cl)Cl
null
1
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(=O)O)C[C@H]2c1ccc(C#N)cc1.N>O.C(Cl)Cl>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(CC(N)=O)C[C@H]2c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0c8cc087949049a8ae08d344d04c36da
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1.CS(N)(=O)=O>>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)NS(C)(=O)=O)cs1)C[C@H]2c1ccc(C#N)cc1
CCN=C=NCCCN(C)C.C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC2=CC(=CS2)C(=O)O.CS(=O)(=O)N.C(C)N(CC)CC>>C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC2=CC(=CS2)C(=O)NS(=O)(=O)C
O[C:23]([c:22]1[cH:21][c:20]([CH2:19][N:18]2[CH2:17][C@@:16]3([N:2]([CH3:1])[C:3](=[O:4])[N:5]([c:6]4[cH:7][c:8]([Cl:9])[cH:10][c:11]([Cl:12])[cH:13]4)[C:14]3=[O:15])[C@H:33]([c:34]3[cH:35][cH:36][c:37]([C:38]#[N:39])[cH:40][cH:41]3)[CH2:32]2)[s:31][cH:30]1)=[O:24].[NH2:25][S:26]([CH3:27])(=[O:28])=[O:29]>>[CH3:1][N:2]...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1.CS(N)(=O)=O
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)NS(C)(=O)=O)cs1)C[C@H]2c1ccc(C#N)cc1
null
CN(C)C=1C=CN=CC1
O.C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C1N[C@@]2(CN(Cc3cccs3)C[C@H]2c2ccccc2)C(=O)N1c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#16;a:6]:[c:7]:1.[C;D1;H3:8]-[#16:9](-[NH2;D1;+0:10])(=[O;D1;H0:11])=[O;D1;H0:12]>>[C;D1;H3:8]-[#16:9](=[O;D1;H0:11])(=[O;D1;H0:12])-[NH;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#16;a:6]:[c:7]:1
34.2
[{"value": 34.2, "product": "C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC2=CC(=CS2)C(=O)NS(=O)(=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
48
HOUR
EDCI (84 mg, 0.44 mmol) was added to a solution of Example 37 (100 mg, 0.18 mmol), methanesulfonamide (38 mg, 0.38 mmol), triethylamine (62 μl, 0.43 mmol) and a trace of DMAP in DCM (5 ml) at room temperature. After 48 h, water was added and the mixture was acidified by bubbling SO2. The organic layer was separated and...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccsc1.c1ccccc1
HO-
CN(C)C=1C=CN=CC1.O.C(Cl)Cl
null
48
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1.CS(N)(=O)=O>CN(C)C=1C=CN=CC1.O.C(Cl)Cl>CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)NS(C)(=O)=O)cs1)C[C@H]2c1ccc(C#N)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-851aa17fb191445b8977f327b3ffde44
CCOC(=O)CN=C=O.CN(C)C=O.CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1>>NC(CO)(CO)CO.[N-]=C=O
ClC=1C=C(C=C(C1)Cl)N1C(N([C@]2(C1=O)CNC[C@H]2C2=CC=C(C#N)C=C2)C)=O.N(=C=O)CC(=O)OCC.C1CCOC1.CN(C)C=O>>C(C(CO)(CO)N)O.[N-]=C=O
C[CH2:7]O[C:3]([CH2:2][N:1]=[C:10]=[O:11])=[O:4].CN(C)[CH:5]=[O:6].CN1C(=[O:8])[N:9](c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1>>[NH2:1][C:2]([CH2:3][OH:4])([CH2:5][OH:6])[CH2:7][OH:8].[N-:9]=[C:10]=[O:11]
CCOC(=O)CN=C=O.CN(C)C=O.CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1
NC(CO)(CO)CO.[N-]=C=O
null
null
null
C-C Coupling
OtherReaction
9db8d154f4f370a50652ea2322d698a91c7d9bf817cf458377313357946f97bf
64caabfaa7c7fda5b99edeec4590e69b73ca1c2191ff1cff7f9d26fe5e85b1b5
null
C-N(-C)-[CH;D2;+0:1]=[O;H0;D1;+0:2].C-N1-C(=[O;H0;D1;+0:3])-[N;H0;D3;+0:4](-c2:c:c(-Cl):c:c(-Cl):c:2)-C(=O)-[C@]-12-C-N-C-[C@@H]-2-c1:c:c:c(-C#N):c:c:1.C-[CH2;D2;+0:5]-O-[C;H0;D3;+0:6](=[O;H0;D1;+0:7])-[CH2;D2;+0:8]-[N;H0;D2;+0:9]=[C;H0;D2;+0:10]=[O;D1;H0:11]>>[N-;H0;D1:4]=[C;H0;D2;+0:10]=[O;D1;H0:11].[NH2;D1;+0:9]-[C;...
null
[]
null
null
8
HOUR
To a solution of Example 15 (24.9 mg, 0.06 mmol) in 1 ml THF/DMF (9/1), was added ethyl isocyanatoacetate (11.6 mg, 0.089 mmol), and the reaction mixture was stirred overnight at RT. The titled compound was obtained (33.3 mg) after treatment with PS-Trisamine (Argonaut, 73 mg, 0.267 mmol) and PS-Isocyanate (Argonaut, 8...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Ester.Urea.Substituted dicarboximide.Nitrile.Isocyanate.Tertiary amide.Secondary amine
Primary alcohol.Primary alcohol.Primary alcohol.Primary amine
c1ccccc1.C1C[C@]2(CN1)C[NH]CN2.c1ccccc1
null
null
HCl
null
null
8
CCOC(=O)CN=C=O.CN(C)C=O.CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CNC[C@H]2c1ccc(C#N)cc1>>NC(CO)(CO)CO.[N-]=C=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-00de50691c634edaa9e1945831f94a76
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1.C[Si](C)(C)C=[N+]=[N-]>>COC(=O)c1csc(CN2C[C@@H](c3ccc(C#N)cc3)[C@]3(C2)C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)N3C)c1
OP(=O)(O)O.OP(=O)(O)O.C(#N)C1=CC=C(C=C1)[C@@H]1CN(C[C@]12C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)CC2=CC(=CS2)C(=O)O.C[Si](C)(C)C=[N+]=[N-]>>COC(=O)C1=CSC(=C1)CN1C[C@]2(C(N(C(N2C)=O)C2=CC(=CC(=C2)Cl)Cl)=O)[C@@H](C1)C1=CC=C(C=C1)C#N
[OH:2][C:3](=[O:4])[c:5]1[cH:6][s:7][c:8]([CH2:9][N:10]2[CH2:11][C@@H:12]([c:13]3[cH:14][cH:15][c:16]([C:17]#[N:18])[cH:19][cH:20]3)[C@:21]3([CH2:22]2)[C:23](=[O:24])[N:25]([c:26]2[cH:27][c:28]([Cl:29])[cH:30][c:31]([Cl:32])[cH:33]2)[C:34](=[O:35])[N:36]3[CH3:37])[cH:38]1.C[Si](C)(C)[CH:1]=[N+]=[N-]>>[CH3:1][O:2][C:3](...
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1.C[Si](C)(C)C=[N+]=[N-]
COC(=O)c1csc(CN2C[C@@H](c3ccc(C#N)cc3)[C@]3(C2)C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)N3C)c1
null
null
O.C(Cl)Cl.CO.CO
Heteroatom Alkylation and Arylation
O-alkylation of carboxylic acids with diazo compounds
39589be0e9a30df66714fe618d22a8ac0fb24901dbf2ead1ab33e31556c7ac64
8b539baf7aeb5ab868833e33306bad77200a853d562904197e13de2e27e229d7
O=C1N[C@@]2(CN(Cc3cccs3)C[C@H]2c2ccccc2)C(=O)N1c1ccccc1
C-[Si](-C)(-C)-[CH;D2;+0:1]=[N+]=[N-].[#16;a:2]:[c:3]:[c:4]-[C:5](=[O;D1;H0:6])-[OH;D1;+0:7]>>[#16;a:2]:[c:3]:[c:4]-[C:5](=[O;D1;H0:6])-[O;H0;D2;+0:7]-[CH3;D1;+0:1]
null
[]
null
null
null
null
To a solution of 5-[(5S*,9R*)-9-(4-Cyanophenyl)-3-(3,5-dichlorophenyl)-1-methyl-2,4-dioxo-1,3,7-triazaspiro[4.4]non-7-ylmethyl]-thiophene-3-carboxylic acid (example 37) (0.150 g, 0.27 mmol) in DCM/MeOH (5:1 mL) was added trimethylsilyldiazomethane (2.0 M solution in hexane, 0.33 mL, 0.67 mmol) over a period of three mi...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Diazo.Silyl protective group
Ester
null
null
c1ccsc1.c1ccccc1.C1C[C@]2(C[NH]1)C[NH]C[NH]2.c1ccccc1
Other
O.C(Cl)Cl.CO.CO
null
null
CN1C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)[C@]12CN(Cc1cc(C(=O)O)cs1)C[C@H]2c1ccc(C#N)cc1.C[Si](C)(C)C=[N+]=[N-]>O.C(Cl)Cl.CO.CO>COC(=O)c1csc(CN2C[C@@H](c3ccc(C#N)cc3)[C@]3(C2)C(=O)N(c2cc(Cl)cc(Cl)c2)C(=O)N3C)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d229ca0f699b42b4bc1c37a6d473d1ea
Brc1ccc2[nH]ccc2c1.OB(O)c1ccc(Cl)cc1>>Clc1ccc(-c2ccc3[nH]ccc3c2)cc1
C(=O)([O-])[O-].[K+].[K+].BrC=1C=C2C=CNC2=CC1.ClC1=CC=C(C=C1)B(O)O>>ClC1=CC=C(C=C1)C=1C=C2C=CNC2=CC1
Br[c:6]1[cH:7][cH:8][c:9]2[nH:10][cH:11][cH:12][c:13]2[cH:14]1.OB(O)[c:5]1[cH:4][cH:3][c:2]([Cl:1])[cH:16][cH:15]1>>[Cl:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]3[nH:10][cH:11][cH:12][c:13]3[cH:14]2)[cH:15][cH:16]1
Brc1ccc2[nH]ccc2c1.OB(O)c1ccc(Cl)cc1
Clc1ccc(-c2ccc3[nH]ccc3c2)cc1
null
null
O
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3[nH]ccc3c2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
40.7
[{"value": 40.7, "product": "ClC1=CC=C(C=C1)C=1C=C2C=CNC2=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A stirred slurry of 6.35 g (60 mmol) K2CO3, 2.94 g (15 mmol) 5-bromoindole, 2.50 g (16 mmol) 4-chlorophenylboronic acid, and 0.48 g (0.42 mmol) tetrakistriphenylphosphine palladium was heated to reflux for 2½ hours. The reaction mixture was allowed to cool and was then poured into 200 ml water and extracted with EtOAc....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1
HBr.B
O
null
null
Brc1ccc2[nH]ccc2c1.OB(O)c1ccc(Cl)cc1>O>Clc1ccc(-c2ccc3[nH]ccc3c2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-adb93e0d0c2c49a4a0813f54e45fa3b2
O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO>>O=C1O[C@H]([C@@H](O)CO)C(O)=C1O
C([C@@H]1[C@H]([C@@H]([C@H]([C@H](O1)O[C@]2([C@H]([C@@H]([C@H](O2)CO)O)O)CO)O)O)O)O.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO>>O=C1C(O)=C(O)[C@H](O1)[C@@H](O)CO
[O:1]=[CH:2][C@@H:11]([C@H:9]([C@H:4]([OH:3])[C@H:5]([OH:6])[CH2:7][OH:8])[OH:10])[OH:12]>>[O:1]=[C:2]1[O:3][C@H:4]([C@@H:5]([OH:6])[CH2:7][OH:8])[C:9]([OH:10])=[C:11]1[OH:12]
O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO
O=C1O[C@H]([C@@H](O)CO)C(O)=C1O
null
null
null
Oxidation
OtherReaction
67e880f982e1ec20ff3e01ab27faa94976fdbdbfa80b39d1e5a327af5f5676c8
bd2ab3fbcaddb67c8972abe9138d0a67a3d3cea6378334aebb0d07cc0e195b46
O=C1C=CCO1
[C:1]-[C:2](-[OH;D1;+0:3])-[C@H;D3;+0:4](-[O;D1;H1:5])-[C@@H;D3;+0:6](-[O;D1;H1:7])-[CH;D2;+0:8]=[O;D1;H0:9]>>[C:1]-[C:2]1-[O;H0;D2;+0:3]-[C;H0;D3;+0:8](=[O;D1;H0:9])-[C;H0;D3;+0:6](-[O;D1;H1:7])=[C;H0;D3;+0:4]-1-[O;D1;H1:5]
null
[]
null
null
17.5
MINUTE
Isolation and Culture of Growth Plate Chondrocytes: Six- to eight-week old broiler chickens were obtained commercially, sacrificed by cervical displacement, and the tibiae harvested. Epiphyseal growth plate chondrocytes were obtained from the tibiae as described (Ali et al., 1970, Proc. Natl. Acad. Sci. USA 67: 1513–15...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary alcohol.Secondary alcohol.Secondary alcohol
Ester.Enol.Enol
null
C1=CCOC1
C1=CCOC1
null
null
null
0.291667
O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO>>O=C1O[C@H]([C@@H](O)CO)C(O)=C1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e19f693ac17d4f31bc9336f96c96004c
CC(C)(C)N.COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)Cl>>COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C
Cl.C(C)(C)(C)N.ClS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)[N+](=O)[O-]>>C(C)(C)(C)NS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)[N+](=O)[O-]
[NH2:17][C:18]([CH3:19])([CH3:20])[CH3:21].Cl[S:14]([c:13]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:6]([N+:7](=[O:8])[O-:9])[cH:10][cH:11][cH:12]1)(=[O:15])=[O:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([N+:7](=[O:8])[O-:9])[cH:10][cH:11][cH:12][c:13]1[S:14](=[O:15])(=[O:16])[NH:17][C:18]([CH3:19])([CH3:20])[CH3:21]
CC(C)(C)N.COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)Cl
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C
null
null
ClCCl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]-[C:7](-[#8:8])=[O;D1;H0:9].[C;D1;H3:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[NH2;D1;+0:14]>>[#8:8]-[C:7](=[O;D1;H0:9])-[c:6]:[c:4](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[NH;D2;+0:14]-[C:11](-[C;D1;H3:10])(-[C;D1;H3:12])-[C;D1;H3:13]):[c:5]
null
[]
null
null
2
HOUR
At 0° C., 1.4 ml (13.3 mmol) of tert-butylamine are added dropwise to a solution of 1.00 g (3.58 mmol) of methyl 2-(chlorosulfonyl)-6-nitrobenzoate in 8 ml of dichloromethane, and the reaction mixture is then allowed to warm to room temperature. After 2 h, the reaction mixture is poured into ice-water, adjusted to pH 3...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1
HCl
ClCCl
null
2
CC(C)(C)N.COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)Cl>ClCCl>COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ea74c890f4544289b988a34632edf185
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C>>COC(=O)c1c([N+](=O)[O-])cccc1S(N)(=O)=O
C(C)(C)(C)NS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)[N+](=O)[O-]>>NS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)[N+](=O)[O-]
CC(C)(C)[NH:15][S:14]([c:13]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:6]([N+:7](=[O:8])[O-:9])[cH:10][cH:11][cH:12]1)(=[O:16])=[O:17]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([N+:7](=[O:8])[O-:9])[cH:10][cH:11][cH:12][c:13]1[S:14]([NH2:15])(=[O:16])=[O:17]
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C
COC(=O)c1c([N+](=O)[O-])cccc1S(N)(=O)=O
null
null
FC(C(=O)O)(F)F
Deprotection
Tert-butyl deprotection of amine
f7e1da1b4c254f1e6d5afbf8cb56733a4fabd145b80e971e3b7e31007de9e7d6
278d0fb11b582c058ac903379d7fbe11ab8c395937a204965031cf0c344845a9
c1ccccc1
C-C(-C)(-C)-[NH;D2;+0:1]-[#16:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5]>>[NH2;D1;+0:1]-[#16:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5]
null
[]
null
null
null
null
300 mg (0.948 mmol) of methyl 2-[(tert-butylamino)sulfonyl]-6-nitrobenzoate in 8 ml of trifluoroacetic acid are stirred at room temperature for 4 h. The mixture is subsequently concentrated to dryness under reduced pressure and the residue is digested with diethyl ether. After filtration with suction and drying, 230 mg...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide
Sulfonamide
null
null
c1ccccc1
Other
FC(C(=O)O)(F)F
null
null
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C>FC(C(=O)O)(F)F>COC(=O)c1c([N+](=O)[O-])cccc1S(N)(=O)=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3a5a0447e048426b955fee6516a6daf5
CC(C)=O.COC(=O)c1c(N)cccc1S(=O)(=O)NC(C)(C)C>>COC(=O)c1c(NC(C)C)cccc1S(=O)(=O)NC(C)(C)C
[BH4-].[Na+].CC(=O)C.N.NC1=C(C(=O)OC)C(=CC=C1)S(=O)(=O)NC(C)(C)C>>C(C)(C)(C)NS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)NC(C)C
O=[C:8]([CH3:9])[CH3:10].[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH2:7])[cH:11][cH:12][cH:13][c:14]1[S:15](=[O:16])(=[O:17])[NH:18][C:19]([CH3:20])([CH3:21])[CH3:22]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH:7][CH:8]([CH3:9])[CH3:10])[cH:11][cH:12][cH:13][c:14]1[S:15](=[O:16])(=[O:17])[NH:18][C:19]([CH3:20])([CH3:21])[CH...
CC(C)=O.COC(=O)c1c(N)cccc1S(=O)(=O)NC(C)(C)C
COC(=O)c1c(NC(C)C)cccc1S(=O)(=O)NC(C)(C)C
null
null
C(C)(=O)O
Heteroatom Alkylation and Arylation
Reductive amination with ketone
4940e8ed9a0db9bde699fdcdc3aff2cff0409c19478aa0ed1acfd98213338adf
07faf85ffe990e88a1de7fd04a339bf226f78d8bfae9712ea59eebd76bb54b9f
c1ccccc1
O=[C;H0;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3].[#8:4]-[C:5](=[O;D1;H0:6])-[c:7]:[c:8](-[NH2;D1;+0:9]):[c:10]>>[#8:4]-[C:5](=[O;D1;H0:6])-[c:7]:[c:8](-[NH;D2;+0:9]-[CH;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3]):[c:10]
null
[]
null
null
1
HOUR
At a temperature of 5-10° C., 925 mg (24.4 mmol) of sodium borohydride are stirred into 14 ml of acetic acid. After 1 h, this mixture is admixed first with 1.42 g (24.4 mmol) of acetone and then with 700 mg (2.44 mmol) of methyl 2-amino-6-[(tert-butylamino)sulfonyl]benzoate and stirred at 5-10° C. for 2.5 h. For work-u...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Secondary amine
null
null
c1ccccc1
Other
C(C)(=O)O
null
1
CC(C)=O.COC(=O)c1c(N)cccc1S(=O)(=O)NC(C)(C)C>C(C)(=O)O>COC(=O)c1c(NC(C)C)cccc1S(=O)(=O)NC(C)(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e109df869bcb46d5a4484519939d7541
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C>>COC(=O)c1c(N)cccc1S(=O)(=O)NC(C)(C)C
C(C)(C)(C)NS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)[N+](=O)[O-]>>NC1=C(C(=O)OC)C(=CC=C1)S(=O)(=O)NC(C)(C)C
O=[N+:7]([O-])[c:6]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:11]([S:12](=[O:13])(=[O:14])[NH:15][C:16]([CH3:17])([CH3:18])[CH3:19])[cH:10][cH:9][cH:8]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH2:7])[cH:8][cH:9][cH:10][c:11]1[S:12](=[O:13])(=[O:14])[NH:15][C:16]([CH3:17])([CH3:18])[CH3:19]
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C
COC(=O)c1c(N)cccc1S(=O)(=O)NC(C)(C)C
null
[Pd]
null
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]-[C:5](-[#8:6])=[O;D1;H0:7]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
86
[{"value": 86.0, "product": "NC1=C(C(=O)OC)C(=CC=C1)S(=O)(=O)NC(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.0, "product": "NC1=C(C(=O)OC)C(=CC=C1)S(=O)(=O)NC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 8.00 g (25.3 mmol) of methyl 2-[(tert-butylamino)sulfonyl]-6-nitrobenzoate is admixed with 3.2 g of palladium on activated carbon (5%) and hydrogenated at room temperature and under atmospheric pressure for 6 h. The reaction mixture is then filtered, the filtrate is concentrated to dryness and the residue...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
[Pd]
null
null
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(C)(C)C>[Pd]>COC(=O)c1c(N)cccc1S(=O)(=O)NC(C)(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-da6af9e359ff40a1bbd60764a87e247b
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)Cl.COc1nc(N)nc(OC)n1.N#C[O-]>>COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1
ClS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)[N+](=O)[O-].NC1=NC(=NC(=N1)OC)OC.[O-]C#N.[Na+].N1=CC=CC=C1>>COC1=NC(=NC(=N1)OC)NC(=O)NS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)[N+](=O)[O-]
Cl[S:14]([c:13]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:6]([N+:7](=[O:8])[O-:9])[cH:10][cH:11][cH:12]1)(=[O:15])=[O:16].[NH2:20][c:21]1[n:22][c:23]([O:24][CH3:25])[n:26][c:27]([O:28][CH3:29])[n:30]1.[N:17]#[C:18][O-:19]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([N+:7](=[O:8])[O-:9])[cH:10][cH:11][cH:12][c:13]1[S:14](=[O:15])(=[...
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)Cl.COc1nc(N)nc(OC)n1.N#C[O-]
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1
null
null
ClCCl.C(C)#N
Acylation
OtherReaction
19bf7d753876392b4c2ac67bd5974bb402735841e5fbc22644f0435dcb2c464c
3c780a65212b9deef596951b8d8a6ff51e2202acb785b2c2d65dd03dbc33bec4
O=C(Nc1ncncn1)NS(=O)(=O)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]-[C:7](-[#8:8])=[O;D1;H0:9].[N;H0;D1;+0:10]#[C;H0;D2;+0:11]-[O-;H0;D1:12].[NH2;D1;+0:13]-[c:14]1:[#7;a:15]:[c:16]:[#7;a:17]:[c:18]:[#7;a:19]:1>>[#8:8]-[C:7](=[O;D1;H0:9])-[c:6]:[c:4](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[NH;D2;+0:10]-[C;H0;D3;+0:11...
null
[]
null
null
7
HOUR
At 55-60° C. and under argon, a solution of 5.0 g (17.9 mmol) of methyl 2-chlorosulfonyl-6-nitrobenzoate in 55 ml of dry dichloromethane is added dropwise over 2 h to a suspension of 2.79 g (17.9 mmol) of 2-amino-4,6-dimethoxy-1,3,5-triazine, 1.28 g (19.7 mmol) of sodium cyanate, 1.45 ml (17.9 mmol) of pyridine and 500...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine.Sulfonyl halide
Sulfonamide.Urea
null
null
c1ccccc1.c1ncncn1
Other
ClCCl.C(C)#N
null
7
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)Cl.COc1nc(N)nc(OC)n1.N#C[O-]>ClCCl.C(C)#N>COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-27ef5de7ff154d3ebc40d5c7ed2e1902
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1>>COC(=O)c1c(N)cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1
COC1=NC(=NC(=N1)OC)NC(=O)NS(=O)(=O)C1=C(C(=O)OC)C(=CC=C1)[N+](=O)[O-]>>NC1=C(C(=O)OC)C(=CC=C1)S(=O)(=O)NC(=O)NC1=NC(=NC(=N1)OC)OC
O=[N+:7]([O-])[c:6]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:11]([S:12](=[O:13])(=[O:14])[NH:15][C:16](=[O:17])[NH:18][c:19]2[n:20][c:21]([O:22][CH3:23])[n:24][c:25]([O:26][CH3:27])[n:28]2)[cH:10][cH:9][cH:8]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH2:7])[cH:8][cH:9][cH:10][c:11]1[S:12](=[O:13])(=[O:14])[NH:15][C:16](=[O:17...
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1
COC(=O)c1c(N)cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1
null
[Pd].[O-][V](=O)=O.[Na+]
CO.CN(C=O)C
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
O=C(Nc1ncncn1)NS(=O)(=O)c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]-[C:5](-[#8:6])=[O;D1;H0:7]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
null
[]
null
null
10
MINUTE
50 mg (113 μmol) of methyl 2-[([(4,6-dimethoxy-1,3,5-triazin-2-yl)amino]-carbonylamino)sulfonyl]-6-nitrobenzoate are suspended in a mixture of 3 ml of methanol/dimethylformamide (5:1), admixed with 10 mg of palladium on activated carbon (5%) and 1 mg (8.20 μmol) of sodium (meta)vanadate and hydrogenated under atmospher...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ncncn1
Other
[Pd].[O-][V](=O)=O.[Na+].CO.CN(C=O)C
null
0.166667
COC(=O)c1c([N+](=O)[O-])cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1>[Pd].[O-][V](=O)=O.[Na+].CO.CN(C=O)C>COC(=O)c1c(N)cccc1S(=O)(=O)NC(=O)Nc1nc(OC)nc(OC)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9223dc2964844701a6f6ccfee85268c6
CCCCCCCCN.O=S(=O)(Cl)Cc1ccccc1>>NS(=O)(=O)Cc1ccccc1
C1(=CC=CC=C1)CS(=O)(=O)Cl.C(CCCCCCC)N>>C1(=CC=CC=C1)CS(=O)(=O)N
CCCCCCCC[NH2:1].Cl[S:2](=[O:3])(=[O:4])[CH2:5][c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1>>[NH2:1][S:2](=[O:3])(=[O:4])[CH2:5][c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1
CCCCCCCCN.O=S(=O)(Cl)Cc1ccccc1
NS(=O)(=O)Cc1ccccc1
null
null
C(Cl)Cl
Miscellaneous
OtherReaction
a86b0632821e188c0a5dc5a5a2aac298ab3eccaee8a52ba46078c3d5975a290d
50f8fbf3d327483c3eeff8f6cbd4065e4c7600bb501fbe08958a5c79a0926428
c1ccccc1
C-C-C-C-C-C-C-C-[NH2;D1;+0:1].Cl-[S;H0;D4;+0:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[C:5]-[c:6]>>[NH2;D1;+0:1]-[S;H0;D4;+0:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[C:5]-[c:6]
93
[{"value": 93.0, "product": "C1(=CC=CC=C1)CS(=O)(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 15.3, "product": "C1(=CC=CC=C1)CS(=O)(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
The synthesis of the sulfonamide containing carboxylic acid precursor corresponding to the autoinducer analog 10 was accomplished by the two step sequence described below. Accordingly, a solution of α-toluenesulfonyl chloride (10 mmol) in CH2Cl2 (5 mL) was added dropwise to a stirred solution of octylamine (20 mmol) in...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1
HCl
C(Cl)Cl
null
0.5
CCCCCCCCN.O=S(=O)(Cl)Cc1ccccc1>C(Cl)Cl>NS(=O)(=O)Cc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-61d100dc066b46178c90cd89026a6194
CCOC(=O)CC1c2ccccc2C(=O)N1C.NC(N)=[NH2+]>>CN1C(=O)c2ccccc2C1CC(=O)NC(=N)N
Cl.[Cl-].NC(=[NH2+])N.CC(C)([O-])C.[K+].CN1C(C2=CC=CC=C2C1=O)CC(=O)OCC>>CN1C(C2=CC=CC=C2C1=O)CC(=O)NC(=N)N
CCO[C:13]([CH2:12][CH:11]1[N:2]([CH3:1])[C:3](=[O:4])[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]21)=[O:14].[NH2:15][C:16]([NH2:17])=[NH2+:18]>>[CH3:1][N:2]1[C:3](=[O:4])[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[CH:11]1[CH2:12][C:13](=[O:14])[NH:15][C:16](=[NH:17])[NH2:18]
CCOC(=O)CC1c2ccccc2C(=O)N1C.NC(N)=[NH2+]
CN1C(=O)c2ccccc2C1CC(=O)NC(=N)N
null
null
O.CN(C=O)C
Acylation
OtherReaction
2a0d0bb811d7d0d78ab0e0e0dd422aa0d95347cc6185304b02293baab0b54666
bd0631f52f11765fc496c7945dc73cbc70f74ea4cf87d492a8fafb124a54fd13
O=C1NCc2ccccc21
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]-[#7:5].[NH2+;D1:6]=[C;H0;D3;+0:7](-[NH2;D1;+0:8])-[NH2;D1;+0:9]>>[#7:5]-[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:8]-[C;H0;D3;+0:7](-[NH2;D1;+0:6])=[NH;D1;+0:9]
16.6
[{"value": 16.6, "product": "CN1C(C2=CC=CC=C2C1=O)CC(=O)NC(=N)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
1
HOUR
4.3 g of guanidinium chloride are added to a suspension of 5.2 g of potassium tertbutoxide in 100 cm3 of dimethylformamide. The reaction mixture is stirred under an inert atmosphere at a temperature in the region of 20° C. for 1 hour, followed by addition of a solution of 2 g of ethyl (2-methyl-3-oxo-2,3-dihydro-1H-iso...
10.6084/m9.figshare.5104873.v1
null
Amidinium.Amidinium.Ester
Secondary amide.Primary amine
null
null
c1ccc2c(c1)C[NH]C2
HO-
O.CN(C=O)C
20
1
CCOC(=O)CC1c2ccccc2C(=O)N1C.NC(N)=[NH2+]>O.CN(C=O)C>CN1C(=O)c2ccccc2C1CC(=O)NC(=N)N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6605c43fbed34c8ab0a97880ec653a0c
CCOC(=O)C=P(c1ccccc1)(c1ccccc1)c1ccccc1.CN1C(=O)c2ccccc2C1O>>CCOC(=O)CC1c2ccccc2C(=O)N1C
C(C)OC(=O)C=P(C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.OC1N(C(C2=CC=CC=C12)=O)C>>CN1C(C2=CC=CC=C2C1=O)CC(=O)OCC
c1ccc(P(c2ccccc2)(c2ccccc2)=[CH:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])cc1.O[CH:7]1[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[C:14](=[O:15])[N:16]1[CH3:17]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH:7]1[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[C:14](=[O:15])[N:16]1[CH3:17]
CCOC(=O)C=P(c1ccccc1)(c1ccccc1)c1ccccc1.CN1C(=O)c2ccccc2C1O
CCOC(=O)CC1c2ccccc2C(=O)N1C
null
null
C1(=CC=CC=C1)C
C-C Coupling
OtherReaction
14c878cf46bb0acf53cb2263c3ebbadf4b36f4102a6ffade3bdc981212d4612e
ec740fdba0adc3c659d56447beb3ee7a35d222db2ebbeacae7f761e1e85567b3
O=C1NCc2ccccc21
O-[CH;D3;+0:1]1-[#7:2](-[C;D1;H3:3])-[C:4](=[O;D1;H0:5])-[c:6]:[c:7]-1:[c:8].[C:9]-[#8:10]-[C:11](=[O;D1;H0:12])-[CH;D2;+0:13]=P(-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[C:9]-[#8:10]-[C:11](=[O;D1;H0:12])-[CH2;D2;+0:13]-[CH;D3;+0:1]1-[#7:2](-[C;D1;H3:3])-[C:4](=[O;D1;H0:5])-[c:6]:[c:7]-1:[c:8]
63.7
[{"value": 63.7, "product": "CN1C(C2=CC=CC=C2C1=O)CC(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
16
HOUR
11.5 g of ethoxycarbonylmethylenetriphenylphosphorane are added to a suspension of 4.5 g of 3-hydroxy-2-methyl-2,3-dihydroisoindol-1-one in 110 cm3 of toluene. The reaction mixture is refluxed with stirring for 16 hours and then cooled to a temperature in the region of 20° C. The mixture is then concentrated to dryness...
10.6084/m9.figshare.5104873.v1
null
Ester.Secondary alcohol
Ester
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2
HO-
C1(=CC=CC=C1)C
20
16
CCOC(=O)C=P(c1ccccc1)(c1ccccc1)c1ccccc1.CN1C(=O)c2ccccc2C1O>C1(=CC=CC=C1)C>CCOC(=O)CC1c2ccccc2C(=O)N1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-726e35a76abe402388792535b5c24847
CN1C(=O)c2ccccc2C1=O>>CN1C(=O)c2ccccc2C1O
[BH4-].[K+].CN1C(C=2C(C1=O)=CC=CC2)=O.O>>OC1N(C(C2=CC=CC=C12)=O)C
[CH3:1][N:2]1[C:3](=[O:4])[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[C:11]1=[O:12]>>[CH3:1][N:2]1[C:3](=[O:4])[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[CH:11]1[OH:12]
CN1C(=O)c2ccccc2C1=O
CN1C(=O)c2ccccc2C1O
null
null
CO
Reduction
OtherReaction
e8ffc87e9d14ec555652bcd3de186a7602297c1d65bf6096cdb1ce7e169ed644
6c2222fa5333790df8c936ae3761255cb080c6e237292637f62137781815b926
O=C1NCc2ccccc21
[C;D1;H3:1]-[#7:2]1-[C:3](=[O;D1;H0:4])-[c:5]:[c:6](:[c:7])-[C;H0;D3;+0:8]-1=[O;H0;D1;+0:9]>>[C;D1;H3:1]-[#7:2]1-[C:3](=[O;D1;H0:4])-[c:5]:[c:6](:[c:7])-[CH;D3;+0:8]-1-[OH;D1;+0:9]
44.4
[{"value": 44.4, "product": "OC1N(C(C2=CC=CC=C12)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
20
HOUR
3.4 g of potassium borohydride are added slowly to a suspension of 10 g of N-methylphthalimide in 220 cm3 of methanol under an inert atmosphere. The reaction mixture is stirred at a temperature in the region of 20° C. for 20 hours, followed by dropwise addition of 200 cm3 of distilled water. The solvent is then partial...
10.6084/m9.figshare.5104873.v1
null
Substituted dicarboximide
Secondary alcohol
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2
null
CO
20
20
CN1C(=O)c2ccccc2C1=O>CO>CN1C(=O)c2ccccc2C1O